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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 451 records · Page 25
All sourcesNASA NTRSDOE OSTI
NASA NTRS1996

In-flight radiation measurements on STS-60

A joint investigation between the United States and Russia to study the radiation environment inside the Space Shuttle flight STS-60 was carried out as part of the Shuttle-Mir Science Program (Phase 1). This is the first direct comparison of a number of different dosimetric measurement techniques between the two countries. STS-60 was launched on 3 February 1994 in a nearly circular 57 degrees x 353 km orbit with five U.S. astronauts and one Russian cosmonaut for 8.3 days. A variety of instruments provided crew radiation exposure, absorbed doses at fixed locations, neutron fluence and dose equivalent, linear energy transfer (LET) spectra of trapped and galactic cosmic radiation, and energy spectra and angular distribution of trapped protons. In general, there is good agreement between the U.S. and Russian measurements. The AP8 Min trapped proton model predicts an average of 1.8 times the measured absorbed dose. The average quality factor determined from measured lineal energy, y, spectra using a tissue equivalent proportional counter (TEPC), is in good agreement with that derived from the high temperature peak in the 6LiF thermoluminescent detectors (TLDs). The radiation exposure in the mid-deck locker from neutrons below 1 MeV was 2.53 +/- 1.33 microSv/day. The absorbed dose rates measured using a tissue equivalent proportional counter, were 171.1 +/- 0.4 and 127.4 +/- 0.4 microGy/day for trapped particles and galactic cosmic rays, respectively. The combined dose rate of 298.5 +/- 0.82 microGy/day is about a factor of 1.4 higher than that measured using TLDs. The westward longitude drift of the South Atlantic Anomaly (SAA) is estimated to be 0.22 +/- 0.02 degrees/y. We evaluated the effects of spacecraft attitudes on TEPC dose rates due to the highly anisotropic low-earth orbit proton environment. Changes in spacecraft attitude resulted in dose-rate variations by factors of up to 2 at the location of the TEPC.

NASA Discipline Radiation Health↗
DOE OSTI2020

Phonons, Q-dependent Kondo spin fluctuations, and 4f phonon resonance in YbAl 3

4f intermediate valence (IV) compounds are canonical hosts of correlated electron physics and can contribute to our understanding of the larger class of correlated electron materials. In this work, we study the prototype IV compound YbAl 3 which exhibits a nonintegral valence with a moderately heavy fermion ground state and a large Kondo temperature (T K ~500–600K). To better characterize the correlated physics of YbAl 3 , we have measured the phonon and the magnetic excitation spectra on single crystals of this material by time-of-flight inelastic neutron scattering and inelastic x-ray scattering. We have also performed theoretical calculations of the phonon spectra. We present three findings of these measurements. First, we observe that the measured phonon spectra can be described adequately by a calculation based on standard DFT+U density functional theory. The calculated energies, however, are 10% too low compared to the measured energies. This discrepancy may reflect a hardening of the phonons due to dynamic 4f correlations. Second, the low-temperature spin fluctuations on the Kondo energy scale k B T K have a momentum (Q) dependence similar to that seen recently in the IV compound CePd 3 . For that system, the Q dependence has been attributed to particle-hole excitations in a coherent itinerant 4f correlated ground state. We suggest a similar origin for the momentum dependence seen in YbAl 3 . This Q dependence disappears as the temperature is raised towards room temperature and the 4f electron band states become increasingly incoherent. Such a coherent/incoherent crossover is expected to be generic for correlated electron systems. Third, a low-temperature magnetic peak observed in the neutron scattering near 30 meV shows dispersion identical to a particular optic-phonon branch. This 4f/phonon resonance disappears for T≥150K. The phonon spectrum appears to be unaffected by the resonance. We discuss several possibilities for the origin of this unusual excitation, which may be unique to YbAl 3 . We suggest that the excitation may arise from the large amplitude beating of the light Al atoms against the heavy Yb atoms, resulting in a dynamic 4f/3p hybridization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1995

Absorbed dose and LET spectra measurements on LDEF

Total absorbed doses measured with TLD's, linear energy transfer (LET) spectra measured with plastic track detectors, and low energy neutrons measured on LDEF have been compared with model calculations. The total absorbed doses measured in TLD's were higher than predicted in the calculations of Armstrong et al. and differ from the calculations of Atwell et al. LDEF LET spectra are dependent on detector orientation, shielding and experiment location. These factors need to be taken into account when modeling the LDEF LET spectra. LET spectra measured with plastic nuclear track detectors (PNTD's) also deviate significantly from calculations especially for high LET particles (LET(sub infinity) H2O greater than 100keV/micron). Modeling efforts to date do not include the contribution of proton induced secondaries. Analysis of polycarbonate PNTD's from the West-side of LDEF has revealed a very high fluence of tracks (greater than 1 x 10(exp 7) tracks/cm(exp 2) under 2 gm/cm(exp 2) shielding). Fluence drops off rapidly as shielding depth increases. Tracks only form in the region of the detector closest to the surface, not in the bulk of the detector. To date no adequate explanation for this observation has been found. We plan to measure range distribution of very high LET (LET (sub infinity) H2O greater than 500 keV/micron) secondary particles produced in silicon wafer by high energy primary cosmic ray particles. Refinements of experimental techniques and model calculations are being carried out in order to understand existing discrepancies between experimental measurements and calculations.

Benton, E. V.↗
NASA NTRS1984

Study of proton and neutron activation of metal samples in low Earth orbit

Progress in the following activities has been made: the analysis of the gamma ray spectra taken from samples flown in Spacelab 2; the search for and review of neutron and proton activation cross sections needed to analyze the results of the Long Duration Exposure Facility (LDEF) activation measurements; the consideration given to data analysis of the LDEF and Spacelab 2 samples; the plan to measure relevant cross sections with nuclear accelerator measurements; and the preparation of an extended gamma ray calibration sources continues through planning and direct measurement of gamma ray efficiency for a Ge(Li) as a function of position along the surface of the detector housing.

Laird, C. E.↗
NASA NTRS1986

IUE observations of V Sagittae

Observations of the nova-like variable V Sge are discussed, and the ground-based light curve is analyzed, compensating for the component interaction effect. Low-dispersion IUE spectra indicate that interstellar reddening is smaller than suggested from visible-band observations. The UV and visible continuum are modeled by a He-rich model and by a simple accretion disk, and the UV spectrum emission lines are used to determine ionization temperatures and a lower N(e) limit. The present data are consistent with the picture of the companion to the He star being embedded in an accretion disk, with the disk being large (of dimension comparable to that of the embedding Roche lobe as a result of vigorous mass transfer) at the time of the ground-based data, and with the disk having been diminished to a radius of the order of 200 times of the neutron star, at the time of the IUE spectra.

Koch, R. H.↗
DOE OSTI2025

Absolute Efficiency Characterization of Neutron Detectors within Radioisotope Identification Devices [Slides]

Some Radioisotope Identification Devices (RIIDs) have a low efficiency neutron detector that can provide a neutron singles counting rate along with the primary gamma spectra that can be used to identify a radioisotope. When we know absolute efficiency, other characteristics of a radioisotope can be estimated such as mass or source strength when accompanied by the identity of the isotope and other observable variables. This study focuses on characterizing and comparing the absolute neutron efficiencies of some commonly used RIIDs: the ORTEC Detective X, ORTEC RADEAGLET-R, and FLIR IDentifinder 2.

Nuclear Criticality Safety Program (NCSP)↗
DOE OSTI2020

Measurement of muon-induced high-energy neutrons from rock in an underground Gd-doped water detector

In this paper, we present a measurement of the rate of correlated neutron captures in the WATCHBOY detector, deployed at a depth of approximately 390 meters water equivalent (m.w.e.) in the Kimballton Underground Research Facility (KURF). WATCHBOY consists of a cylindrical 2 ton water target doped with 0.1% gadolinium, surrounded by a 40 ton undoped water hermetic shield. We present a comparison of our results with the expected rate of correlated neutron captures arising from high-energy neutrons incident on the outside of the WATCHBOY shield, predicted by a hybrid FLUKA/GEANT4-based simulation. The incident neutron energy distribution used in the simulation was measured by a fast neutron spectrometer, the 1.8-ton Multiplicity and Recoil Spectrometer (MARS) detector, at the same depth. We nd that the measured detection rate of two correlated neutrons is consistent with that predicted by simulation. The result lends additional confidence in the detection technique used by MARS, and therefore in the MARS spectra as measured at three different depths. Confirmation of the fast neutron flux and spectrum is important as it helps validate the scaling models used to predict the fast neutron fluxes at different overburdens.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

An all-digital associated particle imaging system for the 3D determination of isotopic distributions

Associated particle imaging (API) is a non-destructive nuclear technique for the 3D determination of isotopic distributions. By detecting the alpha particle associated with the emitted neutron in the deuterium–tritium fusion reaction with a position- and time-resolving detector, the direction of the 14.1 MeV neutron and its time of emission can be determined. Employing this method, isotope characteristic gamma rays emitted in inelastic neutron scattering events can be correlated with the neutron interaction location. Here, an API system consisting of a sealed-type neutron generator, gamma detectors, and a position-sensitive alpha detector was designed, constructed, and characterized. The system was tested with common soil elements and shown to be sensitive to 12 C, 16 O, 28 Si, 27 Al, and 56 Fe. New aspects of our approach are the use of a yttrium–aluminum–perovskite scintillator, using a sapphire window instead of a fiber-optic faceplate for light transport to the photomultiplier, and the all-digital data acquisition system. We present a description of the system with simulations and experimental results that show a position resolution on the alpha detector of 1 mm, a depth resolution using a LaBr 3 detector of 6.2 cm, and an angular resolution of 4.5°. Additionally, we present single-element gamma response measurements for the elements mentioned above together with a comparison to Monte Carlo simulations (MCNP6).

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Anharmonic phonons, thermal expansion, and nuclear quantum effects in Zn

The anharmonic behavior of phonons and thermal expansion of hexagonal zinc were studied from 15 to 690 K by inelastic neutron scattering (INS) and ab initio simulations. Phonon spectra were measured for Q-points covering the full Brillouin zone, giving the phonon density of states (DOS) and dispersions along high-symmetry directions. The dispersions were sharp at 15 K, but diffuse intensity was observed at energies above them. The dispersions broadened with temperature T and the diffuse intensity became stronger. This diffuse intensity appeared in all INS measurements and simulations, except for classical molecular dynamics at 15 K. The temperature-dependent effective potential (TDEP) method, which included the nuclear quantum effect from zero-point vibrational dynamics, was used to calculate the free energy and thermal expansion. For T < 100 K nuclear quantum effects were important for obtaining the correct negative thermal expansion, and path integral molecular dynamics (PIMD) was particularly effective for obtaining the negative thermal expansion in the basal plane. A Heisenberg-Langevin model for interacting phonons coupled to a thermal bath was able to reproduce the shape and intensity of the diffuse spectral features.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Reversible hydrogen storage in multilayer graphane: Lattice dynamics, compressibility, and heat capacity studies

Multilayer graphane (hydride of graphite) is a crystalline hydrocarbon of composition CH, which can be synthesized from graphite and molecular hydrogen at pressures above 2GPa [V.E. Antonov et al. Carbon 100 (2016) 465]. Using X-ray diffraction, this compound was tentatively identified as the “graphane II” phase of 3D-graphane predicted by ab initio calculations [X.-D. Wen et al. PNAS 108 (2011) 6833] and consisting of layers of 2D-graphane in the “chair” conformation. When heated in a vacuum, the compound does not form any intermediate hydrocarbons and reversibly decomposes back into graphite and hydrogen at 770–920 K. In the present work, almost single-phase samples of graphite hydride and deuteride were synthesized at 7.4 GPa and 870 K. Their investigation by inelastic neutron scattering supplemented by ab initio calculations gave spectra g(E) of the phonon density of states with a gap of about 15 meV at approx. 100 meV, which is a unique identifier for the chair form of graphane. The equation of state V(P) of the hydride was studied at room temperature and hydrogen pressures up to 53 GPa by synchrotron X-ray diffraction in a diamond anvil cell. Further, the graphane II phase did not react with the surrounding hydrogen and did not undergo any phase transformations upon the compression and after heating to 1500 K at 53GPa. The high thermal and pressure stability of this exotic phase makes it an important part of the C–H system. The obtained g(E) spectra of graphite hydride and deuteride were used to calculate temperature dependences of their heat capacity. Measurements of the heat capacity at temperatures 120–673 K confirmed the good accuracy of these calculations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2018

NICER Discovers mHz Oscillations in the "Clocked" Burster GS 1826-238

We report the discovery with the Neutron Star Interior Composition Explorer (NICER) of mHz X-ray brightness oscillations from the "clocked burster" GS 1826−238. NICER observed the source in the periods 2017 June 20–29, July 11–13, and September 9–15, for a total useful exposure of 34 ks. Two consecutive dwells obtained on 2017 September 9 revealed highly significant oscillations at a frequency of 8 mHz. The fractional, sinusoidal modulation amplitude increases from 0.7% at 1 keV to ≈2% at 6 keV. Similar oscillations were also detected at lower significance in three additional dwells. The oscillation frequency and amplitude are consistent with those of mHz QPOs reported in other accreting neutron star systems. A thermonuclear X-ray burst was also observed on 2017 June 22. The burst properties and X-ray colors are both consistent with GS 1826 being in a soft spectral state during these observations, findings that are confirmed by ongoing monitoring with MAXI and SWIFT-BAT. Assuming that the mHz oscillations are associated with blackbody emission from the neutron star surface, modeling of the phase-resolved spectra shows that the oscillation is consistent with being produced by modulation of the temperature component of this emission. In this interpretation, the blackbody normalization, proportional to the emitting surface area, is consistent with being constant through the oscillation cycle. We place the observations in the context of the current theory of marginally stable burning and briefly discuss the potential for constraining neutron star properties using mHz oscillations.

Strohmayer, T. E.↗
DOE OSTI2022

Preliminary Design of a New Pulsed-Neutron Die--Away Experiments with Absorbers (IER-552 CED-1)

This report presents the preliminary design (CED-1) of IER-552, pulsed-neutron die-away (PNDA) experiments with absorbers, to be conducted by Lawrence Livermore National Laboratory (LLNL). The goal of the PNDA experiments with absorbing materials is to produce high-quality, low-cost integral benchmarks that can be used to validate cross sections that are high priority nuclear data for the Department of Energy’s Nuclear Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them. The original PNDA experiments were set up at LLNL under IER-501. Extending the PNDA experiments to include absorbing materials leverages existing facilities and resources at LLNL to validate cross sections, with a basic experiment design that uses a neutron generator to impinge a short, mono-energetic neutron pulse on a poisoned, moderating target sample. The neutron pulse lasts 100 µs, after which the neutron population in the sample reaches thermal equilibrium and later spatial equilibrium. In this fully equilibrized state, the neutron population has a characteristic decay-time eigenvalue. The eigenvalue can be used as an integral parameter to validate nuclear data involved with neutron scattering and absorption. Two observables can be measured: the neutron population and the population of secondary γ-rays produced by inelastic and capture reactions. This report explores the feasibility of both approaches. For γ-ray measurements, this allows for direct measurement of reactions of interest for validation. During the neutron burst time, inelastic (prompt) γ-rays dominate, and these data can be isolated for validation of neutron inelastic scattering data. After the pulse ends, neutron capture (delayed) γ-rays dominate and are produced by many reaction channels as neutrons slow down to thermal energies. Two sets of γ-ray spectra (inelastic, capture) can be produced for validation. Additionally, the time-dependent decay of the capture γ-ray population when the neutron population is thermalized and in its fundamental mode can be used for validation. Two experiments can be imagined where pulsed neutrons are used to validate the nuclear data of absorbing materials. The first integrates well into the existing PNDA testbed at LLNL. The absorber material would be introduced into a moderating target and the same neutron generator, neutron detectors, electronics, and shielding box used for IER-501 would be employed. From the same experimental setup, many absorbing materials can be validated by simply changing the neutron poison in the moderator. The only significant modification would be the introduction of a γ-ray detector. Such an experiment would primarily serve to validate nuclear data in the thermal energy range. The second kind of experiment would validate the fast and epithermal energy range. It would involve pulsing neutron into a bare assembly of the absorber material and measuring the die-away of neutrons. The fast leakage of such an assembly requires nanosecond neutron-generator pulse widths and fast detectors/electronics that could measure ~200 ns die-away curves. This kind of experiment would ideally be performed at a cyclotron, like that available at Lawrence Berkeley National Laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Activation and surface reactions of CO and H 2 on ZnO powders and nanoplates under CO hydrogenation reaction conditions

Here, activation and surface reactions of CO and H 2 on ZnO powders and nanoplates under CO hydrogenation reaction conditions were (quasi) in situ studied using temperature programmed surface reaction spectra, diffuse reflectance Fourier transform infrared spectroscopy, inelastic neutron scattering spectroscopy and electron paramagnetic resonance. CO undergoes disproportion reaction to produce gaseous CO 2 and surface carbon adatoms, and adsorbs to form surface formate species. H 2 adsorption forms dominant irreversibly-adsorbed surface hydroxyl groups and interstitial H species and very minor surface Zn-H species. Surface formate species and hydroxyl groups react to produce CO 2 and H 2 , while surface carbon adatoms are hydrogenated by surface Zn-H species sequentially to produce CH(a), CH 2 (a), CH 3 (a) and eventually gaseous CH 4 . The ZnO nanoplates, exposing a higher fraction of Zn-ZnO(0001) and O-ZnO(000–1) polar facets, are more active than the ZnO powders to catalyze CO hydrogenation to CH 4 . These results provide fundamental understanding of the reaction mechanisms and structural effects of CO hydrogenation reaction catalyzed by ZnO-based catalysts.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1991

Cyclotron lines in gamma-ray bursts and magnetic field decay

The presence of cyclotron lines in a significant fraction of gamma-ray burst spectra suggests a source association with strongly magnetized neutron stars. The burster distance scale is not known, but it is constrained by their angular- and brightness distribution. Using pulsar data, the corresponding age distribution of Galactic neutron stars are calculated and an exponential field decay model is applied to test whether the observed incidence rate of cyclotron lines is consistent with decay time scales derived for radio pulsars. It is found that the statistical properties of gamma-ray bursts are inconsistent with the idea of events originating at arbitrary times on neutron stars whose fields decay on time scales shorter than about 10 yrs. Possible interpretations of this inconsistency with radio pulsar field decay models are discussed.

Hartmann, Dieter H.↗
NASA NTRS1994

A new transient pulsar in the Small Magellanic Cloud with an unusual x-ray spectrum

This article reports the discovery of a luminous (3.5 x 10(exp 37) ergs/sec over the 0.2 to 2 keV band) transient X-ray pulsar in the Small Magellanic Cloud (SMC) with an extremely soft component to its X-ray spectrum. This is the first time that a spectrum of this type has been seen in this class of X-ray source. The pulse period is 2.7632 s, and the pulse modulation appears to vary with energy from nearly unpulsed in the low-energy band of the ROSAT Position Sensitive Proportional Counter (PSPC) (0.07 to 0.4 keV) to about 50% in the high-energy band (1.0 to 2.4 keV). The object, RX J0059.2-7138, also shows flickering variability in its X-ray emission on timescales of 50 to 100s. The pulse-phase-averaged PSPC X-ray spectrum can be well described by a two-component source model seen through an absorbing column density of approximately 10(exp 21) atoms cm(exp -2). One spectral component is a power law with photon index 2.4. The other component is significantly softer and can be described by either a steeply falling power law or a blackbody with a temperature KT(sub BB) approximately 35 eV. Ths component is transient, but evidently upulsed, and, for the blackbody model fits, requires a large bolometric luminosity: near, or even several times greater than, the Eddington luminosity for a 1.4 solar mass object. When these characteristics of its soft emission are considered, RX J0059.2-7138 appears quite similar to other X-ray sources in the magellanic Clouds, such as CAL 83, CAL 87, and RX J0527.8-6954, which show only extreme ultrasoft (EUS) X-ray spectra. The discovery of RX J0059.2-7138, a probably high-mass X-ray binary, clearly indicates that EUS spectra may arise from accretion-powered neutron-star X-ray sources. This result lends support to the idea that some of the 'pure' EUS sources may be shrouded low-mass X-ray binaries rather than accreting white dwarfs.

Hughes, John P.↗
NASA NTRS1994

Observational features of cosmic gamma-ray bursts: Evidence for Galactic versus extragalactic origin

The recent observational data on gamma-ray bursts are reviewed. Burst time histories display features at the millisecond level which suggest a compact object origin. Lines in the energy spectra and spectral evolution point toward a Galactic neutron star origin, even though line features have not yet been confirmed in recent data. The Galactic distribution of burst sources, however, is both isotropic and sampled to its characteristic distance, making it unlikely that the sources are related to populations of Galactic neutrons stars we are familiar with. Counterpart searches, previously carried out years after the gamma-ray bursts, are now proceeding days after the events. Based on the current data, it is impossible to conclude whether bursters are Galactic, extragalactic, or both. Data being returned from current experiments, as well as data from new experiments to be launched in the next few years, may yet provide the answer.

Hurley, Kevin↗