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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 451 records · Page 25
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

On the reachable cycles via the unified perspective of cryocoolers. Part B: Cryocoolers with isentropic expanders

Solvay, Stirling and Gifford-McMahon types of cryocoolers employ an isentropic expander which is their elementary mechanism for temperature reduction (following the unified model of cryocoolers as described in a previous paper, Part A). Solvay and Stirling cryocoolers are driven by a larger temperature reduction than that of the Gifford-McMahon cycle, for a similar compression ratio. These cryocoolers are compared from the view of the unified model, in terms of the lowest attainable temperature, compression ratio, the size of the interchanger and the applied heat load.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2014

Effect of dynamics on the elastic softening of vacancies in Si

Recently, elastic softening at temperatures below 20 K has been observed in nondoped floating zone silicon. From the experimental analysis, it has been suggested that this softening is caused by an intrinsic vacancy defect through the Jahn-Teller (JT) effect. We have theoretically studied the relations between softening and the vacancies. The ground state of the JT distortion is stiff. However, by considering atomistic dynamical and anharmonic effects, it is found that low-energy excitations exist in the E-mode distortion and that different polarizations of the E-distortion can be easily interchanged. The calculated energy barriers for the reorientation of JT distortions are consistent with other experiments and calculations. This low-lying mode can be the cause of softening in the elastic responses.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

On 3-gauge transformations, 3-curvatures, and Gray-categories

In the 3-gauge theory, a 3-connection is given by a 1-form A valued in the Lie algebra g, a 2-form B valued in the Lie algebra h, and a 3-form C valued in the Lie algebra l, where (g,h,l) constitutes a differential 2-crossed module. We give the 3-gauge transformations from one 3-connection to another, and show the transformation formulae of the 1-curvature 2-form, the 2-curvature 3-form, and the 3-curvature 4-form. The gauge configurations can be interpreted as smooth Gray-functors between two Gray 3-groupoids: the path 3-groupoid P{sub 3}(X) and the 3-gauge group G{sup L} associated to the 2-crossed module L, whose differential is (g,h,l). The derivatives of Gray-functors are 3-connections, and the derivatives of lax-natural transformations between two such Gray-functors are 3-gauge transformations. We give the 3-dimensional holonomy, the lattice version of the 3-curvature, whose derivative gives the 3-curvature 4-form. The covariance of 3-curvatures easily follows from this construction. This Gray-categorical construction explains why 3-gauge transformations and 3-curvatures have the given forms. The interchanging 3-arrows are responsible for the appearance of terms with the Peiffer commutator (, )

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

A portable high-resolution soft x-ray and extreme ultraviolet spectrometer designed for the Shanghai EBIT and the Shanghai low energy EBITs

A portable high resolution soft x-ray and extreme ultraviolet (EUV) spectrometer has been developed for spectroscopic research at the Shanghai Electron Beam Ion Trap (EBIT) laboratory. A unique way of aligning the grazing incidence spectrometer using the zero order of the grating is introduced. This method is realized by extending the range of the movement of the CCD detector to cover the zero order. The alignment can be done in a few minutes, thus leading to a portable spectrometer. The high vacuum needed to be compatible with the EBITs is reached by mounting most of the translation and rotation stages outside the chamber. Only one high vacuum compatible linear guide is mounted inside the chamber. This is to ensure the convenient interchange of the gratings needed to enable wavelength coverage of the whole range of 10 to 500 Å. Spectra recorded with one of our low energy EBITs shows that a resolving power of above 800 can be achieved. In the slitless configuration used in this work, we found the resolving power to be limited by the width of the EBIT plasma. When mounted on the Shanghai EBIT which is a high energy EBIT and has a narrower EBIT plasma width, the estimated resolving power will be around 1400 at 221.15 Å.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2014

Bi-fluid and neoclassical effect on a Double-Tearing mode in Tore Supra

Tearing modes associated to hollow current profiles are prone to grow in moderate performance plasmas and often constrain the realization of non-inductive discharges in the Tore Supra tokamak, where long pulse duration is performed using Lower Hybrid waves for providing most of the plasma current. The prediction of MHD boundaries in such scenarios is complicated by the importance of diamagnetic effects, combined with curvature stabilization, which determine the stability of these modes. We show that diamagnetic effects, as well as neoclassical forces, are playing a key role in the linear and nonlinear regimes of Double-Tearing Modes on q = 5/3 and q = 2 in these experimental conditions. Detailed comparison with experimental measurements, combined with a scaling in plasma resistivity, give constraints about the experimental equilibrium. Resistive-Interchange Modes destabilized by diamagnetic rotation could also play a role in degrading the energy confinement in the negative magnetic shear region.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Structure and tunneling dynamics in a model system of peptide co-solvents: Rotational spectroscopy of the 2,2,2-trifluoroethanol⋯water complex

The hydrogen-bonding topology and tunneling dynamics of the binary adduct, 2,2,2-trifluoroethanol (TFE)⋯water, were investigated using chirped pulse and cavity based Fourier transform microwave spectroscopy with the aid of high level ab initio calculations. Rotational spectra of the most stable binary TFE⋯water conformer and five of its deuterium isotopologues were assigned. A strong preference for the insertion binding topology where water is inserted into the existing intramolecular hydrogen-bonded ring of TFE was observed. Tunneling splittings were detected in all of the measured rotational transitions of TFE⋯water. Based on the relative intensity of the two tunneling components and additional isotopic data, the splitting can be unambiguously attributed to the tunneling motion of the water subunit, i.e., the interchange of the bonded and nonbonded hydrogen atoms of water. The absence of any other splitting in the rotational transitions of all isotopologues observed indicates that the tunneling between g+ and g− TFE is quenched in the TFE⋯H{sub 2}O complex.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Peeling-off of the external kink modes at tokamak plasma edge

It is pointed out that there is a current jump between the edge plasma inside the last closed flux surface and the scrape-off layer and that the current jump can lead the external kink modes to convert to the tearing modes, due to the current interchange effects [L. J. Zheng and M. Furukawa, Phys. Plasmas 17, 052508 (2010)]. The magnetic reconnection in the presence of tearing modes subsequently causes the tokamak edge plasma to be peeled off to link to the divertors. In particular, the peeling or peeling-ballooning modes can become the “peeling-off” modes in this sense. This phenomenon indicates that the tokamak edge confinement can be worse than the expectation based on the conventional kink mode picture.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Turbulence in the cylindrical slab

The cylindrical slab was the first and simplest model of intrinsically unstable microturbulence. The Helimak is an experimental realization of this model. Although finite, it is sufficiently large to escape boundary effects, with dimensionless parameters similar to those of a tokamak edge or scrape off layer. The essential drive is interchange-like, a pressure gradient with unfavorable magnetic curvature, leading to a non-linearly saturated state of large-amplitude turbulence, Δn{sub rms}/n ∼ 0.5. The nonlinear processes governing this saturation are unique, unlike any of those posited for the much weaker turbulence typical of confined plasma, e.g., in a tokamak. Neither linear stability theory, quasi-linear theory, zonal flows, nor flow shear stabilization is consistent with the observations. The mechanisms determining the non-linearly saturated state constitute an important challenge to our understanding of strongly nonlinear systems.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Spectrometer for X-ray emission experiments at FERMI free-electron-laser

A portable and compact photon spectrometer to be used for photon in-photon out experiments, in particular x-ray emission spectroscopy, is presented. The instrument operates in the 25–800 eV energy range to cover the full emissions of the FEL1 and FEL2 stages of FERMI. The optical design consists of two interchangeable spherical varied-lined-spaced gratings and a CCD detector. Different input sections can be accommodated, with/without an entrance slit and with/without an additional relay mirror, that allow to mount the spectrometer in different end-stations and at variable distances from the target area both at synchrotron and at free-electron-laser beamlines. The characterization on the Gas Phase beamline at ELETTRA Synchrotron (Italy) is presented.

43 PARTICLE ACCELERATORS↗
DOE OSTI2014

On violation of local closure of transport relation in high-temperature magnetized plasmas

Rapid propagation of heat modulation and a hysteresis in the gradient-flux relation are found in a global nonlinear simulation of drift-interchange mode turbulence in toroidal helical plasmas. A global mode is excited nonlinearly and induces the turbulence flux in a limited radial region. The nonlinear couplings take a finite temporal duration for redistributing the energy. The mode also has a seesaw effect: increase of the amplitude of the global mode, at the other radii, works to absorb the energy form microscopic modes to suppress the turbulence. Successive excitations of microscopic modes cause the accelerated propagation of change of the heat flux like turbulence spreading after the onset of modulation. Owing to these processes, the hysteresis appears in the gradient-flux relation, which is compared with experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Post-deposition control of ferroelastic stripe domains and internal electric field by thermal treatment

The dependence of the formation of ferroelastic stripe domain patterns on the thermal history is investigated by detailed piezoresponse force microscopy and X-ray diffraction experiments after and during annealing of tensile strained tetragonal Pb(Ti,Zr)O{sub 3} epitaxial thin films on DyScO{sub 3} substrates. In particular, the ferroelastic pattern is reversibly interchanged between a cross-hatched and a stripe domain pattern if the films are cooled at different rates after annealing above the formation temperature of a-domains. Different types of 180° and non-180° patterns can be created, depending on the thermal treatment. The changes in the 180° domain structure and lattice parameters are attributed to a change of oxygen vacancy concentration, which results in a modification of the internal electric field and unit cell size, causing also a shift of T{sub C}. Thermal treatment is done on rhombohedral La:BiFeO{sub 3} thin films as well. It is observed that also in these films, appropriate heat treatment modifies the domain pattern and films with a stripe domain pattern can be created, confirming the general validity of the developed model.

36 MATERIALS SCIENCE↗
DOE OSTI2015

The effect of magnetic field on the intrinsic detection efficiency of superconducting single-photon detectors

We experimentally investigate the effect of a magnetic field on photon detection in superconducting single-photon detectors (SSPDs). At low fields, the effect of a magnetic field is through the direct modification of the quasiparticle density of states of the superconductor, and magnetic field and bias current are interchangeable, as is expected for homogeneous dirty-limit superconductors. At the field where a first vortex enters the detector, the effect of the magnetic field is reduced, up until the point where the critical current of the detector starts to be determined by flux flow. From this field on, increasing the magnetic field does not alter the detection of photons anymore, whereas it does still change the rate of dark counts. This result points at an intrinsic difference in dark and photon counts, and also shows that no enhancement of the intrinsic detection efficiency of a straight SSPD wire is achievable in a magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Generation of a magnetic island by edge turbulence in tokamak plasmas

We investigate, through extensive 3D magneto-hydro-dynamics numerical simulations, the nonlinear excitation of a large scale magnetic island and its dynamical properties due to the presence of small-scale turbulence. Turbulence is induced by a steep pressure gradient in the edge region [B. D. Scott, Plasma Phys. Controlled Fusion 49, S25 (2007)], close to the separatrix in tokamaks where there is an X-point magnetic configuration. We find that quasi-resonant localized interchange modes at the plasma edge can beat together and produce extended modes that transfer energy to the lowest order resonant surface in an inner stable zone and induce a seed magnetic island. The island width displays high frequency fluctuations that are associated with the fluctuating nature of the energy transfer process from the turbulence, while its mean size is controlled by the magnetic energy content of the turbulence.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Approaching the investigation of plasma turbulence through a rigorous verification and validation procedure: A practical example

In the present work, a Verification and Validation procedure is presented and applied showing, through a practical example, how it can contribute to advancing our physics understanding of plasma turbulence. Bridging the gap between plasma physics and other scientific domains, in particular, the computational fluid dynamics community, a rigorous methodology for the verification of a plasma simulation code is presented, based on the method of manufactured solutions. This methodology assesses that the model equations are correctly solved, within the order of accuracy of the numerical scheme. The technique to carry out a solution verification is described to provide a rigorous estimate of the uncertainty affecting the numerical results. A methodology for plasma turbulence code validation is also discussed, focusing on quantitative assessment of the agreement between experiments and simulations. The Verification and Validation methodology is then applied to the study of plasma turbulence in the basic plasma physics experiment TORPEX [Fasoli et al., Phys. Plasmas 13, 055902 (2006)], considering both two-dimensional and three-dimensional simulations carried out with the GBS code [Ricci et al., Plasma Phys. Controlled Fusion 54, 124047 (2012)]. The validation procedure allows progress in the understanding of the turbulent dynamics in TORPEX, by pinpointing the presence of a turbulent regime transition, due to the competition between the resistive and ideal interchange instabilities.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

A reconfigurable gate architecture for Si/SiGe quantum dots

We demonstrate a reconfigurable quantum dot gate architecture that incorporates two interchangeable transport channels. One channel is used to form quantum dots, and the other is used for charge sensing. The quantum dot transport channel can support either a single or a double quantum dot. We demonstrate few-electron occupation in a single quantum dot and extract charging energies as large as 6.6 meV. Magnetospectroscopy is used to measure valley splittings in the range of 35–70 μeV. By energizing two additional gates, we form a few-electron double quantum dot and demonstrate tunable tunnel coupling at the (1,0) to (0,1) interdot charge transition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Note: A single-chamber tool for plasma activation and surface functionalization in microfabrication

We present a simple apparatus for improved surface modification of polydimethylsiloxane (PDMS) microfluidic devices. A single treatment chamber for plasma activation and chemical/physical vapor deposition steps minimizes the time-dependent degradation of surface activation that is inherent in multi-chamber techniques. Contamination and deposition irregularities are also minimized by conducting plasma activation and treatment phases in the same vacuum environment. An inductively coupled plasma driver allows for interchangeable treatment chambers. Atomic force microscopy confirms that silane deposition on PDMS gives much better surface quality than standard deposition methods, which yield a higher local roughness and pronounced irregularities in the surface.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2015

Intramolecular competition between n-pair and π-pair hydrogen bonding: Microwave spectrum and internal dynamics of the pyridine–acetylene hydrogen-bonded complex

a-type rotational spectra of the hydrogen-bonded complex formed from pyridine and acetylene are reported. Rotational and {sup 14}N hyperfine constants indicate that the complex is planar with an acetylenic hydrogen directed toward the nitrogen. However, unlike the complexes of pyridine with HCl and HBr, the acetylene moiety in HCCH—NC{sub 5}H{sub 5} does not lie along the symmetry axis of the nitrogen lone pair, but rather, forms an average angle of 46° with the C{sub 2} axis of the pyridine. The a-type spectra of HCCH—NC{sub 5}H{sub 5} and DCCD—NC{sub 5}H{sub 5} are doubled, suggesting the existence of a low lying pair of tunneling states. This doubling persists in the spectra of HCCD—NC{sub 5}H{sub 5}, DCCH—NC{sub 5}H{sub 5}, indicating that the underlying motion does not involve interchange of the two hydrogens of the acetylene. Single {sup 13}C substitution in either the ortho- or meta-position of the pyridine eliminates the doubling and gives rise to separate sets of spectra that are well predicted by a bent geometry with the {sup 13}C on either the same side (“inner”) or the opposite side (“outer”) as the acetylene. High level ab initio calculations are presented which indicate a binding energy of 1.2 kcal/mol and a potential energy barrier of 44 cm{sup −1} in the C{sub 2v} configuration. Taken together, these results reveal a complex with a bent hydrogen bond and large amplitude rocking of the acetylene moiety. It is likely that the bent equilibrium structure arises from a competition between a weak hydrogen bond to the nitrogen (an n-pair hydrogen bond) and a secondary interaction between the ortho-hydrogens of the pyridine and the π electron density of the acetylene.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Far-infrared VRT spectroscopy of the water dimer: Characterization of the 20 μm out-of-plane librational vibration

We report the first high-resolution spectra for the out-of-plane librational vibration in the water dimer. Three vibrational subbands comprising a total of 188 transitions have been measured by diode laser spectroscopy near 500 cm{sup −1} and assigned to (H{sub 2}O){sub 2} libration-rotation-tunneling eigenstates. The band origin for the K{sub a} = 1 subband is ~524 cm{sup −1}. Librational excitation increases the interchange and bifurcation hydrogen bond rearrangement tunneling splittings by factors of 3-5 and 4-40, respectively. Analysis of the rotational constants obtained from a nonlinear least squares fit indicates that additional external perturbations to the energy levels are likely.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗