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DOE OSTI2023

Influence of mass ablation on ignition and burn propagation in layered fusion capsules

After decades of research, recent laser-driven inertial fusion experiments have demonstrated rapid progress toward achieving thermonuclear ignition using capsule designs with cryogenic fuel layers. The ignition physics for these layered capsules involves a complex interplay between the dynamically forming hot spot and the dense surrounding fuel. Using analytic theory and numerical simulations, we demonstrate that the mass ablation rate into the hot spot depends sensitively upon the temperature of the dense fuel, resulting in ablative inflows up to [Formula: see text] faster than previous estimates. This produces an enthalpy flux into the hot spot that plays a critical role in controlling the hot spot temperature, the ignition threshold, and the subsequent burn propagation. The net influence of mass ablation on the ignition threshold is regulated by a dimensionless parameter that depends upon the temperature of the dense fuel. As a consequence, the ignition threshold is sensitive to any mechanism that heats the dense fuel, such as neutrons or radiation emitted from the hot spot. These predictions are confirmed using radiation-hydrodynamic simulations for a series of capsules near ignition conditions. This analysis may have relevance for understanding the variable performance of recent experiments and for guiding new capsule designs toward higher fusion yields.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2026

Influence of the drive design on ablation front hydrodynamic instability growth in a capsule implosion at the National Ignition Facility

A critical aspect of inertial confinement fusion experiments lies in the control of ablation front instabilities during the implosion process. The growth of Rayleigh–Taylor and Richtmyer–Meshkov instabilities, seeded by target defects, can significantly degrade the performance of the implosion. Here, this study explores the influence of drive design on ablation front stability using the hydro-growth radiography platform at the National Ignition Facility. This platform allows the measurement of the ablation front hydrodynamic instability growth. Because these measurements are restricted to early convergence, their primary role is to constrain the initial instability growth and benchmark the simulations used to infer shell integrity and performance at peak velocity and ignition. Three ignition designs, Hybrid-E (HyE), SQ-n (“S” for scaling and “Q” for quality), and High temperature, High thickness (HiT) were analyzed. The results demonstrated a high dependence of the growth factor on the choice of design, capsule scale as well as the hohlraum conditions, mainly the radiative temperature and the gold M-band emission. HyE and SQ-n display a similar growth factor range, but their evolution is different due to the design differences in hohlraum conditions. HiT has the lowest growth factor of the studied designs, which is a result of a higher radiative temperature. These results highlight the importance of design choices in controlling instability dynamics. These insights inform future drive design strategies to enhance stability and efficiency in fusion ignition experiments.

Physics↗

DOE OSTI2018

From ICF to laboratory astrophysics: ablative and classical Rayleigh-Taylor Instability experiments in turbulent-like regimes

Rayleigh–Taylor instability (RTI) occurs whenever fluids of different densities are accelerated against the density gradient, as is the case for the target ablator in ICF implosions. The advent of megajoule class lasers, like the National Ignition Facility (NIF) or Laser Mégajoule, offers novel opportunities to study turbulent mixing flows in high energy density plasmas for fundamental hydrodynamics or laboratory astrophysics experiments. Here, we review different RTI experiments, performed either at the ablation front or at a classical embedded interface. A two-dimensional bubble-merger, bubble-competition regime was evidenced for the first time at the ablation front in indirect-drive on the NIF thanks to an unprecedented long x-ray drive. Similarly, a novel large-area, planar platform enables the capabilities to perform long duration direct drive hydrodynamics experiments on NIF. Starting from imprinted seeds, a three-dimensional bubble-merger regime was also observed in direct-drive, as larger bubbles overtook and merged with smaller bubbles. In the astrophysical context, RTI also plays a role in supernova (SN) explosions, either of Type Ia or II. We report on experiments performed on the LULI2000 facility studying RTI in scaled laboratory conditions relevant for the physics of young SN remnants. Finally, using a light CH foam as a deceleration medium, we measured, for the first time, the RTI mixing zone by PW transverse radiography.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2019

Heating and ablation of high- Z cryogenic pellets in high temperature plasmas

A kinetic model is developed here to determine the power deposition from energetic electrons into the neutral gas shield of an ablating high-Z pellet. For high-Z, the velocity distribution of the hot electrons is nearly isotropic, and we use this feature to develop solutions to the kinetic equation. In contrast to pre-existing models, we consider the effect of gyro-motion as well as elastic scattering of the hot electrons. Two limits are considered: when the gyro-frequency is much greater than the elastic collision frequency, the hot electrons diffuse longitudinally along the field lines as they slow down; but if the gyro-frequency is much less than the elastic collision frequency, the hot electrons diffuse radially. In both limits, it is possible to express the kinetic equation describing the hot electrons independently of the gas density profile, and therefore, the power deposition model is universal in this respect. The emphasis on elastic scattering yields an ablation rate which scales as Z -7/6 which is different than Z -2/3 shown in Sergeev et al (2006 Plasma Phys. Rep. 32 5). It is also demonstrated that the sheath potential required to maintain ambipolarity in the cloud scales as Z -1/3 . Fluid simulations yield ablation rates that scale with the four-thirds power of the pellet radius in agreement with [2].

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2017

Mechanism of single-pulse ablative generation of laser-induced periodic surface structures

One of the remarkable capabilities of ultrashort polarized laser pulses is the generation of laser-induced periodic surface structures (LIPSS). The origin of this phenomenon is largely attributed to the interference of the incident laser wave and surface electromagnetic wave that creates a periodic absorption pattern. Although, commonly, LIPSS are produced by repetitive irradiation of the same area by multiple laser pulses in the regime of surface melting and resolidification, recent reports demonstrate the formation of LIPSS in the single-pulse irradiation regime at laser fluences well above the ablation threshold. In this paper, we report results of a large-scale molecular dynamics simulation aimed at providing insights into the mechanisms of single-pulse ablative LIPSS formation. The simulation performed for a Cr target reveals an interplay of material removal and redistribution in the course of spatially modulated ablation, leading to the transient formation of an elongated liquid wall extending up to ~600 nm above the surface of the target at the locations of the minima of the laser energy deposition. The upper part of the liquid wall disintegrates into droplets while the base of the wall solidifies on the time scale of ~2 ns, producing a ~100-nm-tall frozen surface feature extending above the level of the initial surface of the target. The properties of the surface region of the target are modified by the presence of high densities of dislocations and vacancies generated due to the rapid and highly nonequilibrium nature of the melting and resolidification processes. The insights into the LIPSS formation mechanisms may help in designing approaches for increasing the processing speed and improving the quality of the laser-patterned periodic surface structures.

Materials Science↗

DOE OSTI2022

Magnetized ablative Rayleigh-Taylor instability in three dimensions

Three-dimensional extended-magnetohydrodynamics simulations of the magnetized ablative Rayleigh-Taylor instability are presented. Previous two-dimensional (2D) simulations claiming perturbation suppression by magnetic tension are shown to be misleading, as they do not include the most unstable dimension. For perturbation modes along the applied field direction, the magnetic field simultaneously reduces ablative stabilization and adds magnetic tension stabilization; the stabilizing term is found to dominate for applied fields > 5 T, with both effects increasing in importance at short wavelengths. Additionally, for modes perpendicular to the applied field, magnetic tension does not directly stabilize the perturbation but can result in moderately slower growth due to the perturbation appearing to be 2D (albeit in a different orientation to 2D inertial confinement fusion simulations). In cases where thermal ablative stabilization is dominant the applied field increases the peak bubble-spike height. Resistive diffusion is shown to be important for short wavelengths and long timescales, reducing the effectiveness of tension stabilization.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2018

Hydrodynamic instability seeding by oxygen nonuniformities in glow discharge polymer inertial fusion ablators

Here, the U.S. indirect drive inertial confinement fusion (ICF) program uses glow discharge polymer (GDP) as one of the ablator materials for the ICF experiments at the National Ignition Facility (NIF). The performance of those implosions may be adversely affected by photoactivated uptake of oxygen impurities in the surface of the GDP ablator. These impurities can induce significant perturbations in the shock waves generated in the ablator. These perturbed shocks generate mass modulations that are amplified by Rayleigh-Taylor (RT) instability and reduce the performance of the implosions. Here we report on experiments that provide a quantitative connection between photoactivated oxygen uptake in GDP samples and modulations in shock velocities in the samples. The observed shock nonuniformity confirms the hypothesis that irregular oxygenation is a competent seed for the RT and can have a significant effect on NIF GDP implosions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2013

Demonstration of the Improved Rocket Efficiency in Direct-Drive Implosions Using Different Ablator Materials

The success of direct-drive implosions depends critically on the ability to create high ablation pressures (~ 100 Mbar) and accelerating the imploding shell to ignition-relevant velocities (> 3:7 10^7 cm/s) using direct laser illumination. This Letter reports on an experimental study of the conversion of absorbed laser energy into kinetic energy of the shell (rocket efficiency) where different ablators were used to vary the ratio of the atomic number to the atomic mass. The implosion velocity of Be shells is increased by 20% compared to C and CH shells in direct-drive implosions when a constant initial target mass is maintained. These measurements are consistent with the predicted increase in the rocket efficiency of 28% for Be and 5% for C compared to a CH ablator.

Michel, D. T.↗

DOE OSTI2014

Measurements of an Ablator-Gas Atomic Mix in Indirectly Driven Implosions at the National Ignition Facility

We present the first results from an experimental campaign to measure the atomic ablator-gas mix in the deceleration phase of gas-filled capsule implosions on the National Ignition Facility. Plastic capsules containing CD layers were filled with tritium gas; as the reactants are initially separated, DT fusion yield provides a direct measure of the atomic mix of ablator into the hot spot gas. Capsules were imploded with x rays generated in hohlraums with peak radiation temperatures of ~294 eV. While the TT fusion reaction probes conditions in the central part (core) of the implosion hot spot, the DT reaction probes a mixed region on the outer part of the hot spot near the ablator–hot-spot interface. Experimental data were used to develop and validate the atomic-mix model used in two-dimensional simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

Ablating Ion Velocity Distributions in Short-Pulse-Heated Solids via X-Ray Doppler Shifts

Solids ablate under laser irradiation, but experiments have not previously characterized the initiation of this process at ultrarelativistic laser intensities. Here, we present first measurements of bulk ion velocity distributions as ablation begins, captured as a function of depth via Doppler-shifted x-ray line emission from two viewing angles. Bayesian analysis indicates that bulk ions are either nearly stationary or flowing outward at the plasma sound speed. The measurements quantitatively constrain the laser-plasma ablation mechanism, suggesting that a steplike electrostatic potential structure drives solid disassembly.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2026

Onset of Rayleigh-Bénard convection at fuel-ablator interfaces in inertial confinement fusion simulations

Here, we demonstrate the onset of Rayleigh-Bénard convection (RBC) near the fuel-ablator interface of inertial confinement fusion (ICF) implosion simulations for the scenario in which Rayleigh-Taylor or Richtmyer-Meshkov instabilities are suppressed. This convective heating within the cold fuel can degrade the adiabat and therefore performance of ICF implosions even without mixing of fuel and ablator. Our work suggests additional considerations to realize design adiabats in otherwise ideal ICF implosions: first, via control of the temperature differences between ablator and fuel and, second, control of the fuel acceleration which we show has a complex interplay with the RBC dynamics.

Physics - Plasma physics↗

DOE OSTI2015

TU-EF-210-03: Real-Time Ablation Monitoring and Lesion Quantification Using Harmonic Motion Imaging

The use of therapeutic ultrasound to provide targeted therapy is an active research area that has a broad application scope. The invited talks in this session will address currently implemented strategies and protocols for both hyperthermia and ablation applications using therapeutic ultrasound. The role of both ultrasound and MRI in the monitoring and assessment of these therapies will be explored in both pre-clinical and clinical applications. Katherine Ferrara: High Intensity Focused Ultrasound, Drug Delivery, and Immunotherapy Rajiv Chopra: Translating Localized Doxorubicin Delivery to Pediatric Oncology using MRI-guided HIFU Elisa Konofagou: Real-time Ablation Monitoring and Lesion Quantification using Harmonic Motion Imaging Keyvan Farahani: AAPM Task Groups in Interventional Ultrasound Imaging and Therapy Learning Objectives: Understand the role of ultrasound in localized drug delivery and the effects of immunotherapy when used in conjunction with ultrasound therapy. Understand potential targeted drug delivery clinical applications including pediatric oncology. Understand the technical requirements for performing targeted drug delivery. Understand how radiation-force approaches can be used to both monitor and assess high intensity focused ultrasound ablation therapy. Understand the role of AAPM task groups in ultrasound imaging and therapies. Chopra: Funding from Cancer Prevention and Research Initiative of Texas (CPRIT), Award R1308 Evelyn and M.R. Hudson Foundation; Research Support from Research Contract with Philips Healthcare; COI are Co-founder of FUS Instruments Inc Ferrara: Supported by NIH, UCDavis and California (CIRM and BHCE) Farahani: In-kind research support from Philips Healthcare.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2023

Mechanisms of ultrafast GHz burst fs laser ablation

Gigahertz (GHz) femtosecond (fs) lasers have opened possibilities for enhancing and controlling the laser machining quality to engineer the physicochemical properties of materials. However, fundamental understanding of laser-material interactions by GHz fs laser has remained unsolved due to the complexity of associated ablation dynamics. Here, we study the ablation dynamics of copper (Cu) by GHz fs bursts using in situ multimodal diagnostics, time-resolved scattering imaging, emission imaging, and emission spectroscopy. A combination of probing techniques reveals that GHz fs bursts rapidly remove molten Cu from the irradiated spot due to the recoil pressure exerted by following fs pulses. Material ejection essentially stops right after the burst irradiation due to the limited amount of remnant matter, combined with the suppressed heat conduction into the target material. Our work provides insights into the complex ablation mechanisms incurred by GHz fs bursts, which are critical in selecting optimal laser conditions in cross-cutting processing, micro/nano-fabrication, and spectroscopy applications.

47 OTHER INSTRUMENTATION↗

DOE OSTI2020

Ablating nanoscale pores in crystalline quartz using laser-induced micro-plasmas in tri-layer structures

We demonstrate a novel approach for achieving rapid, consistent, and controllable micro-pore fabrication in single-crystalline quartz. These micro-pores are essential for applications in biology, i.e., studying ion channels in general and mechano-sensitive channels (MSC) in particular. The fabrication process consists of direct material ablation using pulsed UV light from a 193 nm excimer laser. These pulses ablate single-crystalline quartz chips by burning a laser-induced plasma in a tri-layer structure. Controllable plasma confinement and thus pore size is achieved by sandwiching a thin layer of a selected organic solution between the quartz chip and different substrates. This solution causes the confined micro-plasma to generate special ablation conditions, to create uniformly sized and shaped nanopores.

36 MATERIALS SCIENCE↗

DOE OSTI2019

Preliminary Design Studies for a Hydro-Growth Radiography Platform to Study the Double Shell Ablator Joint

Double shell target assembly requires mating two hemispheres of aluminum to form the ablator, and the design of the mating joint governs the dimensions of the gap that remains following ablator assembly. Radiographic data from double shell implosions with two different joint designs demonstrate the importance of having a smaller outer gap to minimize perturbation growth, but higher quality data is desirable for validating simulations of such localized engineering features. A double shell hydrogrowth radiography platform is proposed to enable detailed measurements of the joint feature evolution for comparison to simulation predictions. The conservative design is based on a successfully fielded double shell keyhole target, but the tungsten inner shell is replaced with molybdenum to allow imaging with X-rays from a zirconium backlighter (16.3 keV). Eulerian radiation-hydrodynamics simulations with adaptive mesh refinement are used to predict joint feature evolution for several different joint designs. Synthetic radiographs produced from ablator-only calculations demonstrate that the evolution of different joint morphologies can be radiographed and distinguished. Feedthrough of the joint perturbation to a molybdenum inner shell is predicted to be measurable at a convergence ratio of 2.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Symmetry requirements for double shell capsules with aluminum ablators

Double shell targets present a promising avenue to obtain robust neutron yield on current laser facilities. The nature of the target, like current single shell designs, requires a symmetric implosion of an outer ablator to obtain a symmetric fuel volume that will lead to alpha heating and thermonuclear burn. Due to using aluminum as an ablator material and requiring different convergence than single shell symmetry studies at various energies are required. This paper moves forward from previous experiments conducted at 1MJ to show implosion symmetry at 1.25 and 1.5MJ. Symmetry in these experiments is sufficient to merit experiments using double shells to study the platform further. Additional studies are carried out on the outer shell symmetry impacts, showing that mitigating mode growth on the outer ablator is of great importance.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2023

Hypervelocity impact in stellar media: heat shielding, shock fronts and ablation clouds

The Frontier Plasma Science experiments proposed by our team will model the processes occurring during spacecraft atmospheric entries and meteorite planetary collisions by inserting material targets into the Scrape off Layer (SOL) and edge plasma of a tokamak. This project will investigate important plasma-material processes during high-enthalpy atmospheric entries, including heat flux generation and material ablation. Of particular interest is to explore heat and particle flux detachment in front of the sample using concepts and techniques developed in the latest studies of divertor detachment. Exploration missions to the Solar System’s gaseous giants and hyperbolic re-entries into the Earth’s atmosphere require spacecraft that can withstand high velocity (>10 km/s), high heat fluxes (>10 MW/m2), and corresponding enthalpies. Ablative materials have been used as thermal shields to protect the spacecraft from severe heating during entry. However, developing high enthalpy ablating materials is challenging due to the lack of adequate ground testing facilities. Our team stated that the performance of candidate shielding materials could be assessed in a laboratory environment with multiple in-situ diagnostics, which was enabled by the progress in the tokamak research. Modern machines feature relatively long discharges (~10 s) with well-controlled stable plasma conditions at the edge where the heat flux and the flow speed are similar to those experienced during atmospheric entries. The experiments were carried out at the DIII-D National Fusion Facility in San Diego, CA, operated by General Atomics (GA) for the DoE.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1960

Radiation and Ablation Cooling for Manned Reentry Vehicles

The necessity of reducing heat transfer to reentry vehicles has led I to the consideration of both radiative and ablation shields. The paper reviews briefly the heating problems for manned vehicles and the means whereby ablation and radiation afford thermal protection. The principal energy disposal and weight parameters are then presented and their relation to the vehicle and trajectory parameters is discussed. A comparative analysis of three types of ablation shield is made and broad conclusions are drawn as to the type of shield most appropriate to manned reentry vehicles.

Roberts, L.↗