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NASA NTRS2019

AERONET Remotely Sensed Measurements and Retrievals of Biomass Burning Aerosol Optical Properties During the 2015 Indonesian Burning Season

An extreme biomass-burning event occurred in Indonesia from September through October 2015 due to severe drought conditions, partially caused by a major El Nino event, thereby allowing for significant burning of peatland that had been previously drained. This event had the highest sustained aerosol optical depths (AOD) ever monitored by the global Aerosol Robotic Network (AERONET). The newly developed AERONET Version 3 algorithms retain high AOD at the longer wavelengths when associated with high Angstrom Exponents (AEs), which thereby allowed for measurements of AOD at 675 nanometers as high as approximately 7, the upper limit of Sun photometry. Measured AEs at the highest monitored AOD levels were subsequently utilized to estimate instantaneous values of AOD at 550 nanometers in the range of 11 to 13, well beyond the upper measurement limit. Additionally, retrievals of complex refractive indices, size distributions, and single scattering albedos (SSA) were obtained at much higher AOD levels than possible from almucantar scans due to the ability to perform retrievals at smaller solar zenith angles with new hybrid sky radiance scans. For retrievals made at the highest AOD levels the fine mode volume median radii were approximately 0.25 to 0.30 microns, which are very large particles for biomass burning. Very high SSA values (approximately 0.975 from 440 to 1020 nanometers) are consistent with the domination by smoldering combustion of peat burning. Estimates of the percentage peat contribution to total biomass burning aerosol based on retrieved SSA and laboratory measured peat SSA were approximately 80-85 percent, in excellent agreement with independent estimates.

Eck, T. F.↗
NASA NTRS2018

Characteristics of In Situ Fine Fraction Aerosol Spectra from 300-700 nm Observed Around the Korean Peninsula During KORUS-OC

In situ aerosol extinction and absorption spectra covering the 300-700 nm range at ≤ 1 nm spectral resolution were measured aboard the R/V Onnuri during the Korea U.S. – Ocean Color (KORUS-OC) cruise around the Korean Peninsula from May 21 through June 3, 2016. Total absorption spectra were obtained from aerosols collected on glass fiber filters and subsequently placed in the center of an integrating sphere (Labsphere DRA-CA-30) attached to a dual beam spectrophotometer (Cary 100 Bio UV-Visible Spectrophotometer, 0.2 nm spectral resolution). Absorption spectra from methanol and deionized water extracts of aerosols collected on Teflon filters were measured in a liquid waveguide capillary cell (World Precision Instruments LWCC- 3100, ~0.4 nm spectral resolution). Extinction spectra were measured with a custom built instrument (SpEx, ~0.8 nm spectral resolution). The measurements were obtained at a height of ~10 m above the sea surface with an inlet that limited the measured aerosols to diameters ≤ 1.3 µm. All four sets of spectra exhibit curvature in log-log space with 2nd order polynomials providing a better fit to the measured spectra than power law fits. The deionized water extracts were also analyzed with an ion chromatograph (Dionex ICS-3000 Ion Chromatography System) and with an aerosol mass spectrometer (Aerodyne Research, Inc. HR-ToF High Resolution Aerosol Mass Spectrometer) to examine chemical composition. These data indicate the optical spectra are sensitive to differing chemical properties of the measured ambient aerosols and suggest differing sources and/or atmospheric processes influence the observed optical signatures. The measured suite of spectra are combined to examine the spectral characteristics of single scattering albedo, as well as to examine the contribution of soluble absorbing chromophores to the total absorption spectra. Additional measurements made during the affiliated Korea U.S. - Air Quality (KORUS-AQ) campaign will be used to provide further insight on the observed spectral characteristics.

Jordan, Carolyn E↗
NASA NTRS2019

Developing an Aircraft-Based Angular Distribution Model of Solar Reflection from Wildfire Smoke to Aid Satellite-Based Radiative Flux Estimation

This study examines the angular distribution of scattered solar radiation associated with wildfire smoke aerosols observed over boreal forests in Canada during the ARCTAS (Arctic Research of the Composition of the Troposphere from Aircraft and Satellites) campaign. First, it estimates smoke radiative parameters (550 nm optical depth of 3.9 and single scattering albedo of 0.90) using quasi-simultaneous multiangular and multispectral airborne measurements by the Cloud Absorption Radiometer (CAR). Next, the paper estimates the broadband top-of-atmosphere radiances that a satellite instrument such as the Clouds and the Earth’s Radiant Energy System (CERES) could have observed, given the narrowband CAR measurements made from an aircraft circling about a kilometer above the smoke layer. This estimation includes both an atmospheric correction that accounts for the atmosphere above the aircraft and a narrowband-to-broadband conversion. The angular distribution of estimated radiances is found to be substantially different than the angular model used in the operational data processing of CERES observations over the same area. This is because the CERES model is a monthly average model that was constructed using observations taken under smoke-free conditions. Finally, a sensitivity analysis shows that the estimated angular distribution remains accurate for a fairly wide range of smoke and underlying surface parameters. Overall, results from this work suggest that airborne CAR measurements can bring some substantial improvements in the accuracy of satellite-based radiative flux estimates.

Varnai, Tamas↗
NASA NTRS2019

Retrieving Aerosol Characteristics From the PACE Mission, Part 2: Multi-Angle and Polarimetry

The Plankton, Aerosol, Clouds, ocean Ecosystem (PACE) mission presents new opportunities and new challenges in applying observations of two complementary multi-angle polarimeters for the space-based retrieval of global aerosol properties.Aerosol remote sensing from multi-angle radiometric-only observations enables aerosol characterization to a greater degree than single-view radiometers, as demonstrated by nearly two decades of heritage instruments. Adding polarimetry to the multi-angle observations allows for the retrieval of aerosol optical depth, Angstrom exponent,parameters of size distribution, measures of aerosol absorption, complex refractive index and degree of non-sphericity of the particles, as demonstrated by two independent retrieval algorithms applied to the heritage POLarization and Directionality of the Earth's Reflectance (POLDER) instrument. The reason why this detailed particle characterization is possible is because a multi-angle polarimeter measurement contains twice the number of Degrees of Freedom of Signal (DFS) compared to an observation from a single-view radiometer. The challenges of making use of this information content involve separating surface signal from atmospheric signal, especially when the surface is optically complex and especially in the ultraviolet portion of the spectrum where we show the necessity of polarization in making that separation. The path forward is likely to involve joint retrievalsthat will simultaneously retrieve aerosol and surface properties, although advances will berequired in radiative transfer modeling and in representing optically complex constituents in those models. Another challenge is in having the processing capability that can keep pace with the output of these instruments in an operational environment. Yet, preliminaryalgorithms applied to airborne multi-angle polarimeter observations offer encouraging results that demonstrate the advantages of these instruments to retrieve aerosol layer height, particle single scattering albedo, size distribution and spectral optical depth, and also show the necessity of polarization measurements, not just multi-angle radiometricmeasurements, to achieve these results.

Remer, Lorraine A.↗
NASA NTRS2020

Radiative Heating from Biomass Burning Aerosol and its Impact on Cloud Structure in the Southeast Atlantic

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Thermodynamic profiles will be analyzed through the unique combination of sounding data from radiosonde launches and microwave profiling radiometers, giving observations of additional quantities important for cloud development such as CAPE and CIN at a fine temporal resolution. The thermodynamic profiles will be presented in conjunction with detailed observations of the cloud structure over the site from a K-band cloud radar, micropulse lidar, and laser ceilometer. The observed thermodynamic and cloud profiles will be used as input forcing, alongside aerosols from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), for the Rapid Radiative Transfer Model (RRTM) to gain information regarding the radiative heating profiles. Idealized experiments using RRTM with and without aerosols will be used to quantify the impact of biomass burning carbonaceous aerosol plumes as they pass over the site. Due to documented discrepancies in the single scatter albedo (SSA) between models and observations, further sensitivity experiments will demonstrate the importance of the optical properties of biomass burning aerosol in accurately representing heating within the column. Finally, the heating rates will be put into context of the cloud structure over the site from the perspective of the mass flux closure from the University of Washington shallow convective scheme.

Collow, Allison↗
NASA NTRS2019

Observation of Absorbing Aerosols Above Clouds over the South-East Atlantic Ocean from the Geostationary Satellite SEVIRI – Part 1: Method Description and Sensitivity

High temporal resolution observations from satellites have a great potential for studying the impact of biomass burning aerosols and clouds over the South East Atlantic Ocean (SEAO). This paper presents a method developed to retrieve simultaneously aerosol and cloud properties in aerosol above cloud conditions from the geostationary instrument Meteosat Second Generation/Spinning Enhanced Visible and Infrared Imager (MSG/SEVIRI). The above-cloud Aerosol Optical Thickness (AOT), the Cloud Optical Thickness (COT) and the Cloud droplet Effective Radius (CER) are derived from the spectral contrast and the magnitude of the signal measured in three channels in the visible to shortwave infrared region. The impact of the absorption from atmospheric gases on the satellite signal is corrected by applying transmittances calculated using the water vapour profiles from a Met Office forecast model. The sensitivity analysis shows that a 10% error on the humidity profile leads to an 18.5% bias on the above-cloud AOT, which highlights the importance of an accurate atmospheric correction scheme. In situ measurements from the CLARIFY-2017 airborne field campaign are used to constrain the aerosol size distribution and refractive index that is assumed for the aforementioned retrieval algorithm. The sensitivities in the retrieved AOT, COT and CER to the aerosol model assumptions are assessed. Between 09:00-15:00 UTC, an uncertainty of 40% is estimated on the above-cloud AOT, which is dominated by the sensitivity of the retrieval to the single scattering albedo. The absorption AOT is less sensitive to the aerosol assumptions with an uncertainty generally lower than 17% between 09:00-15:00 UTC. Outside of that time range, as the scattering angle decreases, the sensitivity of the AOT and the absorption AOT to the aerosol model increases. The retrieved cloud properties are only weakly sensitive to the aerosol model assumptions throughout the day, with biases lower than 6% on the COT and 3% on the CER. The stability of the retrieval over time is analysed. For observations outside of the backscattering glory region, the time-series of the aerosol and cloud properties are physically consistent, which confirms the ability of the retrieval to monitor the temporal evolution of aerosol above cloud events over the SEAO.

Peers, Fanny↗
NASA NTRS2019

3+2+X: What Is the Most Useful Depolarization Input for Inverting Lidar Measurements of Non-Spherical Particles to Microphysical Properties?

The typical multiwavelength aerosol lidar data set for inversion of optical to microphysical parameters is composed of three backscatter coefficients (β ) at 355, 532, and 1064 nm and two extinction coefficients (α ) at 355 and 532 nm. This data combination is referred to as 3β +2α or 3+2 data set. This set of data is sufficient for retrieving some important microphysical particle parameters if the particles have spherical shape. Here, we investigate the effect of including the particle linear depolarization ratio (δ) as a third input parameter to the inversion of lidar data. The inversion algorithm is generally not used if measurements show values of δ that exceed 0.10 at 532 nm, i.e. in the presence of non-spherical particles such as desert dust, volcanic ash, and under special circumstances biomass-burning smoke.We use experimental data collected with instruments that are capable of measuring δ at all three lidar wavelengths with an inversion routine that uses the theory of light scattering by randomly oriented spheroids to replicate scattering properties of non-spherical particles. This is the first systematic test of the effect of using all theoretically possible combinations of δ taken at 355, 532, and 1064 nm as input in the lidar data inversion. We find that depolarization information at least at one wavelength already provides useful information in the in version of optical data that describe light-scattering by nonspherical particles. However, any choice of δ(λ) will give lower values of the single-scattering albedo than the traditional 3+2 data set. We find that input data sets that include 355 give a non-spherical fraction that closely resembles the dust ratio we obtain from using β(532) and δ(532) in a methodology applied in aerosol-type separation. The use of 355 in data sets of two or three reduces the fraction of non-spherical particles that is retrieved when using δ(532) and δ(1064). Use of the latter two without accounting for 355 generally leads to high fractions of non-spherical particles that we consider not trustworthy. The use of three δ(λ) instead of two δ(λ) including the constraint that one of these is measured at 355 nm does not provide any advantage over using 3+2+δ(355). Because of the technical challenges involved with accurately measuring δ(1064) we conclude that — depending on measurement capability — the future standard input for inversion using spheroid kernels might be 3+2+δ(355) or 3+2+δ(355)+δ(532).

Tesche, M.↗
NASA NTRS2018

A13H-2537: Above Cloud Aerosol Optical Properties in the South East Atlantic from airborne observations during ORACLES

Aerosol overlying marine stratocumulus clouds is a persistent feature in the southeast Atlantic during the biomass burning season, July through November. We sampled aerosol and cloud from an airborne research platform, the NASA P3, during the deployments of ObseRvations of CLouds above Aerosols and their intEractionS (ORACLES) encompassing the peak biomass burning season. We used the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) to quantify the aerosol’s optical properties, notably the aerosol optical depth (AOD) by directly measuring the amount of light attenuation. We present an overview of very recent AOD measurements and contrast those to previous deployments. We observed an average AOD at 500 nm of 0.33 (0.30) in September 2016 (August 2017), with similar spatial dependence as observed by the MODIS instrument on board the TERRA and AQUA satellites. We also show full spectral vertical dependence of AOD from flight profiles, which compares favorably to the integrated aerosol extinction profile obtained by the active remote sensing High Spectral Resolution Lidar-2 (HSRL-2). We also present a quantification of the gap extent separating cloud top and aerosol layer bottom. Using hyperspectral transmitted light measurements from 4STAR, in conjunction with hyperspectral hemispheric irradiance measurements from the Solar Spectral Flux Radiometers (SSFR), we retrieved aerosol intensive properties (asymmetry parameter, single scattering albedo), aerosol size distributions, cloud optical depth (COD), cloud particle effective radius, and cloud thermodynamic phase. Cloud properties, also presented here, are obtained from 4STAR measurements of scattered light below clouds.

Samuel E LeBlanc↗
NASA NTRS2018

A13H-2546: Intercomparison of biomass burning aerosol properties from in-situ and remote-sensing instruments in ORACLES-2016

The magnitude of the cumulative effects of aerosols, both directly and on cloud properties, remains the biggest source of uncertainty in our understanding of anthropogenic radiative forcing on the climate. The magnitude of aerosol effects in any given region will depend on not just the aerosol concentration, but also on the characteristics of the aerosol under consideration. The NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign was conducted in 2016-2018 over three deployments in the Southeast Atlantic Ocean (SEA), with the goal of making observations of seasonal biomass burning (BB) smoke plumes overlying persistent stratocumulus cloud decks. During the first ORACLES deployment (September 2016), two NASA aircraft (a P-3 and an ER-2) were flown with a suite of aerosol, cloud, radiation, and meteorological instruments for remote-sensing and in-situ observations. In ORACLES, data collected by eight different instrument teams are used to derive aerosol properties over this region by independent methods. Here we present a comparison of results from the different instrument retrievals with a focus on the measures of aerosol absorption. We focus on specific cases with near-coincident measurements from in-situ (PSAP or PTI for aerosol absorption combined with a nephelometer for aerosol scattering) and remote sensing (4STAR, AirMSPI, RSP, and SSFR) instruments from coordinated flights between the two aircraft. We use the single scattering albedo (SSA), a measure of the relative absorption versus total extinction by aerosols, as the main comparable property between the various remote sensing and in-situ methods. For the remote sensing instruments, we see general good agreement in the total aerosol loading (aerosol optical depth, AOD), though see some differences in the absorbing component (AAOD). We report values for the retrieved aerosol parameters measured in the ORACLES flights and comment upon the observed variability between different instruments. Finally, we discuss these ORACLES results in the context of previous measurements of BB aerosol over the SEA.

Kristina Pistone↗
NASA NTRS2019

TPSAS-NF1676L-34010-DND

We invert global black carbon (BC), organic carbon (OC) and desert dust (DD) aerosol emissions from POLDER/PARASOL spectral aerosol optical depth (AOD) and aerosol absorption optical depth (AAOD) using the GEOSChem inverse modelling framework. Our inverse modeling framework uses standard a priori emissions to provide a posteriori emissions that are constrained by POLDER/PARASOL AODs and AAODs. Our satellite-derived global aerosol emission database indicates an increase of BC and OC, while a decrease of DD with respect to the a priori emission inventories used in standard GEOS-Chem runs. The model simulations using a posteriori emissions (i.e. retrieved emissions) provide new estimate of global aerosol extinction and absorption constrained by observations. Additionally, the a posteriori model simulation of AOD, AAOD, single scattering albedo, Angstrom exponent, and absorption Angstrom exponent show better agreement with independent AERONET, MODIS, and OMI measurements than the a priori simulation. Thus, this study suggests that using satellite-constrained global aerosol emissions in aerosol transport models can improve the accuracy of simulated global aerosol properties and have potential to better understanding global aerosol effects on climate and human health.

Cheng Chen↗
NASA NTRSDate not supplied

TPSAS-NF1676L-34796-DND

The recently completed 2015-2017 EVS-2 mission NAAMES (The North Atlantic Aerosols and Marine Ecosystems Study) provides a unique set of airborne remote sensing and ship-based in situ measurements in a remote and under-sampled region of the Earth?s ocean. The NASA SABOR (Ship-Aircraft Bio-Optical Research) campaign was conducted during the summer of 2014, also in the Atlantic Ocean, out of the Chesapeake Bay and in the eastern coastal region of the United States. For both campaigns, the NASA GISS Research Scanning Polarimeter, a multi-angle, multi-spectral polarimeter measured the upwelling polarized radiances from aircraft. And for both campaigns, ship-based in situ measurements of the ocean were collected jointly with the aircraft measurements. We present results from the new RSP-MAPP (1) that is based on optimal estimation and that can retrieve simultaneous aerosol microphysical properties (including effective radius, single-scattering albedo, and real refractive index) and ocean color products using accurate radiative transfer, Mie calculations, and the DP (Detritus Plankton) series of accurate, numerically efficient ocean bio-optical models. The RSP-MAPP algorithm was applied to data collected during SABOR and NAAMES to retrieve aerosol microphysics and ocean products for all Aerosols-Above-Ocean (AAO) scenes. The RSP-MAPP products are compared against i) collocated aerosol extinction and backscatter profiles collected by the NASA LaRC airborne High Spectral Resolution Lidar (HSRL-1), including lidar depth profiles of the ocean diffuse attenuation coefficient and the hemispherical backscatter coefficient, and ii) collocated ship-based in situ measurements of the ocean.

Snorre Stamnes↗
NASA NTRS2020

Aerosol Layer Height with Enhanced Spectral Coverage Achieved by Synergy between VIIRS and OMPS-NM Measurements

This letter presents a near production-ready algorithm to retrieve the height of biomass burning smoke and mineral dust aerosols as part of National Aeronautics and Space Administration (NASA)’s Deep Blue aerosol data product suite. It utilizes the enhanced spectral coverage achieved by using colocated data from the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM), both aboard the Suomi National Polar-orbiting Partnership (S-NPP) satellite. In particular, the 412-nm top-of-atmosphere (TOA) reflectance from VIIRS and the ultraviolet aerosol index from OMPS-NM are used to determine the height and single-scattering albedo of the absorbing aerosols simultaneously. Constraints on aerosol optical depth at 550 nm and surface reflectance for the 412-nm band are provided by the operational VIIRS Deep Blue aerosol product. Wildfire smoke layer heights obtained from the algorithm over North America, where smoke plumes often stretched thousands of kilometers, are shown to agree with those from Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements, with an uncertainty generally within 1–1.5 km. This new height data set will be included in the upcoming Version 2 VIIRS Deep Blue aerosol product.

aerosol↗
NASA NTRS2020

Influence of Cloud, Fog, and High Relative Humidity during Pollution Transport Events in South Korea: Aerosol Properties and PM2.5 Variability

This investigation examines aerosol dynamics during major fine mode aerosol transboundary pollution events in South Korea primarily during the KORUS-AQ campaign from May 1 – June 10, 2016, particularly when cloud fraction was high and/or fog was present to quantify the change in aerosol characteristics due to near-cloud or fog interaction. We analyze the new AERONET Version 3 data that have significant changes to cloud screening algorithms, allowing many more fine-mode observations in the near vicinity of clouds or fog. Case studies for detailed investigation include May 25–26, 2016 when cloud fraction was high over much of the peninsula, associated with a weak frontal passage and advection of pollution from China. These cloud-influenced Chinese transport dates also had the highest aerosol optical depth (AOD), surface PM2.5 concentrations and fine mode particle sizes of the entire campaign. Another likewise cloud/high relative humidity (RH) case is June 9 and 10, 2016 when fog was present over the Yellow Sea that appears to have affected aerosol properties well downwind over the Korean peninsula. In comparison we also investigated aerosol properties on air stagnation days with very low cloud cover and relatively low RH (May 17 & 18, 2016), when local Korean emissions dominated. Aerosol volume size distributions show marked differences between the transport days (with high RH and cloud influences) and the local pollution stagnation days, with total column-integrated particle fine mode volume being an order of magnitude greater on the pollution transport dates. The PM2.5 over central Seoul were significantly greater than for coastal sites on the transboundary transport days yet not on stagnation days, suggesting addi-tional particle formation from gaseous urban emissions in cloud/fog droplets and/or in the high RH humidified aerosol environment. Many days had KORUS-AQ research aircraft flights that provided observations of aerosol absorption, particle chemistry and vertical profiles of extinction. AERONET retrievals and aircraft in situ mea-surements both showed high single scattering albedo (weak absorption) on the cloudy or cloud influenced days, plus aircraft profile in situ measurements showed large AOD enhancements (versus dried aerosol) at ambient relative humidity (RH) on the pollution transport days, consistent with the significantly larger fine mode particle radii and weak absorption.

Aerosol↗
NASA NTRS2020

Aerosol Layer Height With Enhanced Spectral Coverage Achieved by Synergy Between VIIRS and OMPS-NM Measurements

This study presents a near production-ready algorithm to retrieve the height of biomass burning smoke and mineral dust aerosols as part of NASA’s Deep Blue aerosol data product suite. It utilizes the enhanced spectral coverage achieved by using co-located data from the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM), both aboard the Suomi National Polar-orbiting Partnership (S-NPP) satellite. Specifically, the 412 nm top-of-atmosphere reflectance from VIIRS and the ultraviolet aerosol index from OMPS-NM are used to determine the height and single-scattering albedo of the absorbing aerosols simultaneously. Constraints on aerosol optical depth at 550 nm and surface reflectance for the 412 nm band are provided by the operational VIIRS Deep Blue aerosol product. Wildfire smoke layer heights obtained from the algorithm over North America, where smoke plumes often stretched thousands of kilometers, are shown to agree with those from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements, with an uncertainty generally within 1-1.5 km. This new height data set will be included in the upcoming Version 2 VIIRS Deep Blue aerosol product.

Aerosol↗
NASA NTRSDate not supplied

Uncertainty in Observational Estimates of the Aerosol Direct Radiative Effect and Forcing

Aerosols continue to be responsible for the largest uncertainty in determining the anthropogenic radiative forcing of the climate. To both reconcile the large range in satellite-based estimates of the aerosol direct radiative effect (DRE, the direct interaction with solar radiation by all aerosols) and to optimize the design of future observing systems, we build a framework for assessing uncertainty in aerosol DRE and the aerosol direct radiative forcing (DRF, the radiative effect of just anthropogenic aerosols, RF_ari). Shortwave aerosol radiative kernels (Jacobians) were derived using the MERRA-2 reanalysis data. These radiative kernels are used to compute a lower-bound on the systematic uncertainty in observational estimates of the aerosol DRE/DRF by making the optimistic assumption that global aerosol observations can be made with the accuracy found in the Aerosol Robotic Network (AERONET) sun photometer retrievals. The total uncertainty is shown to be dominated by contributions from the aerosol single scattering albedo uncertainty. These uncertainty estimates were compared to a literature survey of mostly satellite-based aerosol DRE/DRF values. Comparisons to previous studies reveal that most have significantly underestimated the aerosol DRE uncertainty. Past estimates of the aerosol DRF uncertainty are smaller (on average) than our optimistic observational estimates, including the aerosol DRF uncertainty given in the Intergovernmental Panel on Climate Change (IPCC) fifth assessment report (AR5).

Tyler James Thorsen↗
NASA NTRSDate not supplied

Investigation of the Potential for Lidar & Polarimeter Combined Aerosol Retrievals Using Various Instrument Combinations

As a scientific community, we are motivated to achieve better observational capabilities for aerosols, to reduce uncertainties about aerosol’s role in climate. Encouraged by the National Academies Decadal Survey, many are looking to the synergy of lidar and polarimeter as a means of achieving improved measurements. Polarimetric observations of total-column radiances have excellent sensitivity to aerosol size distribution and absorption properties. Active lidar measurements have fewer wavelengths and view angles and therefore more limited sensitivity to aerosol microphysical properties such as complex refractive index. Yet the advantage of vertically resolved profiles is game-changing, especially given that models contain significant uncertainty about the vertical distribution of aerosol and that polarimeter and other passive retrievals must make assumptions about vertical distribution which can impact performance. To optimize the synergy, a joint polarimeter + lidar mission requires a joint retrieval. However, the exact instruments that will be launched on a future satellite are unknown, and the capabilities of polarimeters and lidars cover a large range. In this study, we perform information content analysis for a range of nominal instrument combinations. The methodology is ideal for assessing the impact of measurements and a priori information (assumptions and constraints) with respect to the desired retrieval products, and for comparing measurement systems. It has advantages that make it useful in advance of or in parallel with retrieval development, such as producing quantitatively useful comparisons even for retrieval scenarios that are significantly underdetermined and therefore impossible to retrieve without significant assumptions, and it is not impacted by retrieval-specific sources of error such as incomplete or incorrect convergence which can complicate the interpretation of a retrieval performance analysis. Here, we will derive the expected uncertainty in retrieved aerosol concentration, effective radius, fine mode fraction and single scattering albedo, for a combination of a polarimeter with various grades of lidar, from an elastic backscatter lidar, similar to the pathfinder CALIOP on the CALIPSO satellite, to a multi-wavelength high spectral resolution lidar.

Sharon P Burton↗
NASA NTRS2021

Hydrogen Abundance and Distribution on (101955) Bennu

Asteroids were likely a major source of volatiles and water to early Earth. Quantifying the hydration of asteroids is necessary to constrain models of the formation and evolution of the Solar System and the origin of Life on Earth. The OSIRIS-REx (Origins, Spectral Interpretation, Resource Identification, and Security–Regolith Explorer) mission showed that near-Earth asteroid (101955) Bennu contains widespread, abundant hydrated phyllosilicates, indicated by a ubiquitous absorption at ~ 2.7 μm. The objective of this work is to quantify the hydration—that is, the hydrogen content—of phyllosilicates on Bennu's surface and investigate how this hydration varies spatially. We analyse spectral parameters (normalized optical path length, NOPL; effective single-scattering albedo, ESPAT; and Gaussian modeling) computed from the hydrated phyllosilicate absorption band of spatially resolved visible–near-infrared spectra acquired by OVIRS (the OSIRIS-REx Visible and InfraRed Spectrometer). We also computed the same spectral parameters using laboratory-measured spectra of meteorites including CMs, CIs, and the ungrouped C2 Tagish Lake. We estimate the mean hydrogen content of water and hydroxyl groups in hydrated phyllosilicates on Bennu's surface to be 0.71 ± 0.16 wt%. This value is consistent with the hydration range of some aqueously altered meteorites (CMs, C2 Tagish Lake), but not the most aqueously altered group (CIs). The sample collection site of the OSIRIS-REx mission has slightly higher hydrogen content than average. Spatial variations in hydrogen content on Bennu's surface are linked to geomorphology, and may have been partially inherited from its parent body.

A. Praet↗
NASA NTRSDate not supplied

Update on EPIC MAIAC V2 Algorithm: Atmospheric Correction

Alexei Lyapustin presented a new v2 MAIAC atmospheric correction algorithm for EPIC. The v2 algorithm introduced new projection removing spatial distortions, a more accurate retrieval of spectral surface reflectance using ancillary MAIAC MODIS BRDF dataset, and a new technique for simultaneous retrieval of aerosol optical depth and spectral absorption. AERONET validation shows that v2 significantly improved AOD accuracy compared to v1, while the retrieved single scattering albedo in the Blue shows a very good accuracy comparable to that of AERONET for both biomass burning smoke and mineral dust aerosols.

Alexei Lyapustin↗