Measurement of the neutron-induced capture-to-fission cross section ratio in U 233 at LANSCE
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Neutron stars serve as excellent next-generation thermal detectors of dark matter, heated by the scattering and annihilation of dark matter accelerated to relativistic speeds in their deep gravitational wells. However, the dynamics of neutron star cores are uncertain, making it difficult at present to unequivocally compute dark matter scattering in this region. On the other hand, the physics of an outer layer of the neutron star, the crust, is more robustly understood. We show that dark matter scattering solely with the low-density crust still kinetically heats neutron stars to infrared temperatures detectable by forthcoming telescopes. We find that for both spin-independent and spin-dependent scattering on nucleons, the crust-only cross section sensitivity is 10 -43 - 10 -41 cm 2 for dark matter masses of 100 MeV - 1 PeV, with the best sensitivity arising from dark matter scattering with a crust constituent called nuclear pasta (including gnocchi, spaghetti, and lasagna phases). For dark matter masses from 10 eV to 1 MeV, the sensitivity is 10 -39 - 10 -34 cm 2 , arising from exciting collective phonon modes in a neutron superfluid in the inner crust. Furthermore, for any s-wave or p-wave annihilating dark matter, we show that dark matter will efficiently annihilate by thermalizing just with the neutron star crust, regardless of whether the dark matter ever scatters with the neutron star core. This implies efficient annihilation in neutron stars for any electroweakly interacting dark matter with inelastic mass splittings of up to 200 MeV, including Higgsinos. We conclude that neutron star crusts play a key role in dark matter scattering and annihilation in neutron stars.
We investigate how our baryon-loss limits from anomalous binary-pulsar period lengthening can be interpreted microscopically to yield specific constraints on the particle physics of baryon number violation within a neutron star. We focus on the possibility of anomalous baryon disappearance via dark baryon processes and on scenarios in which the produced dark-sector particles do not survive to influence the response of the star to baryon-number-violating effects. We flesh out the conditions for which this may occur, as well as other key assumptions. We then turn to the analysis of particle processes in the dense nuclear medium found at the core of a neutron star, employing the techniques of relativistic mean-field theory. Using our study of in-medium effects and limits on macroscopic baryon number violation, we extract limits on in-vacuum baryon-number-violating processes, and we determine them for various equations of state. We conclude by noting the implications of our results for models of dark-sector-enabled baryogenesis. Published by the American Physical Society 2024
We perform high-statistics simulations to study the impacts of nuclear structure on the ratios of anisotropic flow observables in 208 Pb + 208 Pb and 129 Xe + 129 Xe collisions at the Large Hadron Collider. Even with 40% difference in atomic numbers between 208 Pb and 129 Xe nuclei, the ratios of anisotropic flow in the same centrality class between the two collision systems are strongly affected by the nuclear structure inputs in the initial state. The ratios of v 2 {4}/v 2 {2} in these collisions are sensitive to the nuclear skin thickness of the colliding nuclei, providing indirect constraints on the nuclei's neutron skin. In conclusion, our model predictions serve as a benchmark to compare with experimental measurements.
This paper summarizes neutron dosimetry measurements made by the USF Physics Research Laboratory aboard US and Russian LEO spacecraft over the past 20 years using two types of passive detector. Thermal/resonance neutron detectors exploiting the 6Li(n,T) alpha reaction were used to measure neutrons of energies <1 MeV. Fission foil neutron detectors were used to measure neutrons of energies above 1 MeV. While originally analysed in terms of dose equivalent using the NCRP-38 definition of quality factor, for the purposes of this paper the measured neutron data have been reanalyzed and are presented in terms of ambient dose equivalent. Dose equivalent rate for neutrons <1 MeV ranged from 0.80 microSv/d on the low altitude, low inclination STS-41B mission to 22.0 microSv/d measured in the Shuttle's cargo bay on the highly inclined STS-51F Spacelab-2 mission. In one particular instance a detector embedded within a large hydrogenous mass on STS-61 (in the ECT experiment) measured 34.6 microSv/d. Dose equivalent rate measurements of neutrons >1 MeV ranged from 4.5 microSv/d on the low altitude STS-3 mission to 172 microSv/d on the ~6 year LDEF mission. Thermal neutrons (<0.3 eV) were observed to make a negligible contribution to neutron dose equivalent in all cases. The major fraction of neutron dose equivalent was found to be from neutrons >1 MeV and, on LDEF, neutrons >1 MeV are responsible for over 98% of the total neutron dose equivalent. Estimates of the neutron contribution to the total dose equivalent are somewhat lower than model estimates, ranging from 5.7% at a location under low shielding on LDEF to 18.4% on the highly inclined (82.3 degrees) Biocosmos-2044 mission. c2001 Elsevier Science Ltd. All rights reserved.
The paper aims to provide an update on the status of the Organization for Economic Cooperation and Development (OECD) / the Nuclear Energy Agency (NEA) Tennessee Valley Authority (TVA) Watts Bar 1 (WB1) Multi-Physics Multi-Cycle depletion benchmark and the results associated with Exercise 1. The benchmark relies on the set of benchmark progression problems developed by the Department of Energy (DOE) Consortium for the Advanced Simulation of Light Water Reactors (CASL) for the Virtual Environment for Reactor (VERA), which are based on real plant design and operational data. The OECD/NEA TVA WB1 benchmark is designed for validation of both traditional and novel high-fidelity multi-physics codes to analyze Pressurized Water Reactors (PWR) depletion cycles. The activities are conducted under the Expert Group on Reactor Systems Multi-Physics (EGMUP) at NEA/OECD. In this work, we analyze Exercise 1 of the benchmark: stand-alone Three-Dimensional (3D) neutronics at Start-up Zero Power Physics Test (ZPPT) at Hot Zero Power Conditions (HZP) and the resulting power maps. The code used to model the exercise is the continuous energy Monte Carlo code Serpent 2.1.31 along with the nuclear data library ENDF/B-VII.1. Serpent results are compared with the high-fidelity deterministic code MPACT, which is part of VERA. The paper presents three selected results from power calculations required output. The results compared are the normalized axially integrated radial core power maps, the normalized axial averaged core power shapes, and the normalized core hottest and coldest assemblies radial power maps. The Root Mean Square Deviation (RMSD) between Serpent and MPACT is 0.51 % for the axially integrated radial core power map, 1.41 % for the axial averaged core power shape, 2.42 % for the hottest assembly axial power shape, 0.88 % for the coldest assembly axial integrated hottest assembly radial pin power map, and 0.17 % for the axially integrated coldest assembly radial pin power map. (authors)
Core radial expansion in liquid-metal cooled fast reactor systems is a well-known phenomenon that produces strong reactivity feedback effects. It is crucial from a safety standpoint to design a reactor with the proper core restraint system to guide expansion of the fuel assemblies into a formation that produces negative reactivity feedback in accident conditions. However, the modeling of core radial expansion and its associated reactivity feedback is extremely challenging. Liquid metal-cooled fast reactor designers (both industry and commercial) have pointed to improved modeling of core radial expansion as a key modeling challenge for these types of reactors. The Department of Energy Nuclear Energy Advanced Modeling and Simulation (DOE-NEAMS) program has an important role to play in helping to develop a robust, predictive tool for this phenomenon. A literature review has been performed to identify current simulation capabilities applicable to the prediction of core radial expansion in liquid metal-cooled fast reactors and the resultant reactivity feedback effects. An overview as well as a detailed description of the multi-physics phenomena underlying core radial expansion is given in the first two chapters. The objective of this report is to identify existing software that has been or could be applied to the core radial expansion problem, and then to identify possible paths to develop a robust, coupled Multiphysics tool for advanced analysis, in which all three physics (radiation transport, structural mechanics, thermal fluids) are taken into account considering feedback effects from each physics to the other. Several computer codes and workflows have been developed in the United States and abroad to perform individual aspects of radial expansion calculations or to perform loosely coupled analysis. No code system currently exists which tightly and robustly couples the neutronics, thermal hydraulics, and thermal mechanical physics with enough detail to fully resolve the complex core radial expansion reactivity feedback effects. The future availability of such a code system is of vital importance to fully understanding the reactivity feedback effects that occur due to radial expansion, and consequently to optimizing the design of the core restraint system. A potential code development path forward using MOOSE-based tools is suggested in order to leverage the natural tight coupling and robustness of MOOSE-based applications. Additionally, potential gaps for modeling and common assumptions are listed which require further investigation to ensure accuracy for prediction of deformations.
Graphite has been of great interest since the dawn of the nuclear era. In this work, we will focus on the thermal neutron scattering of two types of nuclear graphite that have different microstructures, namely, the historic PGA which has a very anisotropic medium-grained needle coke, and the new G347A which is a near-isotropic fine-grained graphite. We report the results of room temperature inelastic neutron scattering measurements for the scattering function, double differential scattering cross-section, and phonon density of states. The obtained results are discussed in conjunction with results extracted from first-principles lattice dynamics simulations of crystalline graphite, using the incoherent approximation and by also including the coherent-one phonon contribution. Excellent agreements have been found between the measured and calculated scattering functions and phonon densities of states. The inclusion of the coherent-one phonon scattering shows a significant improvement of the calculated scattering functions, double differentials, and inelastic scattering cross-sections. We also highlight the physical concerns about the current thermal neutron scattering ENDF/B-VIII of nuclear graphite library and its corresponding phonon density of states. This work aims to provide a new presentation of neutron thermalization by graphite and offers a new set of high quality experimental and computational data for consideration.
Neutronics simulations of Molten Chloride Fast Reactors have quantifiable biases that arise from nuclear data, modeling choices, or numerical methods. The multiphysics nature of molten salt reactors makes it challenging to disentangle neutronics modeling biases from biases originating from other physical phenomena. In comparison to a mock-up reactor, criticality experiments can specifically assess the neutronics modeling bias while limiting multiphysics effects. The criticality experiment must be neutronically representative of the full-scale reactor to be valuable. Here, in this paper, we describe the design of a criticality experiment to validate only the neutronics of TerraPower’s Molten Chloride Reactor Experiment (MCRE) and its criticality safety upset scenarios. The proposed experiment uses different chlorine-containing materials to maximize its similarity to the MCRE. The design process uses a constrained Bayesian optimization algorithm to investigate different objective functions that use covariance information for 35 Cl nuclear data. The experiments could reduce the nuclear data–induced uncertainty in k eff of the MCRE from 2161 to 886 pcm. They would also increase the upper subcritical limit of the MCRE criticality safety upset scenario from 0.94101 to 0.94476 when using the WHISPER analysis framework.
Abstract Topological nodal semimetals are known to host a variety of fascinating electronic properties due to the topological protection of the band-touching nodes. Neutron scattering, despite its power in probing elementary excitations, has not been routinely applied to topological semimetals, mainly due to the lack of an explicit connection between the neutron response and the signature of topology. In this work, we theoretically investigate the role that neutron scattering can play to unveil the topological nodal features: a large magnetic neutron response with spectral non-analyticity can be generated solely from the nodal bands. A new formula for the dynamical structure factor for generic topological nodal metals is derived. For Weyl semimetals, we show that the locations of Weyl nodes, the Fermi velocities and the signature of chiral anomaly can all leave hallmark neutron spectral responses. Our work offers a neutron-based avenue toward probing bulk topological materials.
Realizing the promise of fusion as a commercially attractive energy source requires the development of advanced structural materials capable of sustained operation in an incredibly hostile environment. The fusion environment presents many challenges associated with high cyclic thermal-mechanical loadings, welding and joining disparate materials, and achieving chemical compatibility with coolants and tritium breeders. Yet, the overarching concern is the degradation of physical and mechanical properties, resulting from a neutron energy spectrum peaked at 14 MeV. The high-energy fusion neutron irradiation produces both displacement damage and high levels of hydrogen and helium through transmutation reactions. Advanced materials development for use in such a hostile environment is predicated on understanding the underlying mechanisms responsible for physical and material property degradation. This project has closely combined computational, theoretical and experimental techniques within a multiscale materials science paradigm to determine the mechanisms controlling material degradation in the fusion environment.
Abstract Using the quantum information model of dynamical diffraction we consider a neutron cavity composed of two perfect crystal silicon blades capable of containing the neutron wavefunction. We show that the internal confinement of the neutrons through Bragg diffraction can be modelled by a quantum random walk. Furthermore, we introduce a toolbox for modelling crystal imperfections such as surface roughness and defects. Good agreement is found between the simulation and the experimental implementation, where leakage beams are present, modelling of which is impractical with the conventional theory of dynamical diffraction. Analysis of the standing neutron waves is presented in regards to the crystal geometry and parameters; and the conditions required for well-defined bounces are derived. The presented results enable new approaches to studying the setups utilizing neutron confinement, such as the experiments to measure neutron magnetic and electric dipole moments.
Kagome-lattice materials have attracted tremendous interest due to the broad prospect for seeking superconductivity, quantum spin liquid states, and topological electronic structures. Among them, the transition-metal kagome lattices are high-profile objects for the combination of topological properties, rich magnetism, and multiple-orbital physics. Here we report an inelastic neutron scattering study on the spin dynamics of a kagome-lattice antiferromagnetic metal Fe 0.89 Co 0.11 Sn. Although the magnetic excitations can be observed up to ~250 meV, well-defined spin waves are only identified below ~90 meV and can be modeled using Heisenberg exchange with ferromagnetic in-plane nearest-neighbor coupling J 1 , in-plane next-nearest-neighbor coupling J 2 , and antiferromagnetic (AFM) interlayer coupling J c under linear spin-wave theory. Above ~90 meV, the spin waves enter the itinerant Stoner continuum and become highly damped particle-hole excitations. At the K point of the Brillouin zone, we reveal a possible band crossing of the spin wave, which indicates a potential Dirac magnon. Finally, our results uncover the evolution of the spin excitations from the planar AFM state to the axial AFM state in Fe 0.89 Co 0.11 Sn, solve the magnetic Hamiltonian for both states, and confirm the significant influence of the itinerant magnetism on the spin excitations.
The NNSS has extensive historical experience with high-fidelity flash neutron imaging which may be applicable to the needs of NA-22. In recent neutron imaging tests, a dense plasma focus (DPF) discharges a capacitor bank across a hydrogen-filled diode to create a flash of fusion neutrons emitted from a point, which can be used for active interrogation. Object inspection may include both radiography transmission imaging as well as emission imaging of the subject via an aperture. A scintillator screen (coupled to a low-Z converter when necessary) converts deposited energy to visible light, which is relayed through optics to an ultra-sensitive visible imager contained in a light-tight box. Flash photon imaging, utilizing bremsstrahlung emission instead of fusion neutrons, is also available and is more mature.
The detection of fast neutrons is regarded technically challenging because the interaction probability of fast neutron with matter is extremely low. Based on our recent development of hexagonal boron nitride (BN) semiconductor thermal neutron detectors with a record high efficiency of 59%, we report here the feasibility studies of BN detectors for detecting fast neutrons. A BN detector with a detection area of 2.1 cm 2 was fabricated from a 90 $μ$m thick BN epilayer. In the presence of a bare Cf-252 source emitting fast neutrons ranging from 1 to 9 MeV, the detection efficiency was estimated to be about 0.1%. Furthermore, the measured mean free path of fast neutron in BN is about 7.6 cm. Together with the capability of BN for thermal neutron detection, the present results indicate that by incorporating BN with a large thickness, BN neutron detectors are expected to possess the unique capability of directly detecting thermal to fast neutrons as well as outstanding features resulting from the ultrawide bandgap of BN. The identification of a single material that is sensitive to both thermal and fast neutrons is valuable for the development of novel neutron detection technologies.
This report details a fully coupled neutronics thermal hydraulics reference plant model for a thermal spectrum molten salt-fueled reactor. The Multiphysics model is developed on the Nuclear Regulatory Commission's Comprehensive Reactor Analysis Bundle available on the Idaho National Laboratory high-performance computer, which natively and seamlessly couples Griffin and Sam codes of the Multiphysics Object-Oriented Simulation Environment (MOOSE) based applications. Griffin provides the reactor physics capabilities, k-eigenvalue, delayed neutron precursor concentrations, and transient solutions for stationary and flowing fuels. Sam provides the solution of mass, momentum, and energy conservation equations of the whole system with a set of system components for one-dimensional single-phase flow. The neutronics feedback model relies primarily on fuel and moderator temperatures, fuel salt density, and delayed neutron precursors distributions. This report presents our results for the coupled steady state core and an unprotected loss of flow event. Although this model is prototypical regarding capabilities in the Comprehensive Reactor Analysis Bundle, its results are consistent with experimental data of the pump transient tests that were performed at zero power of the Molten Salt Reactor Experiment (MSRE).
Merging neutron stars produce “kilonovae”—electromagnetic transients powered by the decay of unstable nuclei synthesized via rapid neutron capture (the r-process) in material that is gravitationally unbound during inspiral and coalescence. Kilonova emission, if accurately interpreted, can be used to characterize the masses and compositions of merger-driven outflows, helping to resolve a long-standing debate about the origins of r-process material in the Universe. We explore how the uncertain properties of nuclei involved in the r-process complicate the inference of outflow properties from kilonova observations. Using r-process simulations, we show how nuclear physics uncertainties impact predictions of radioactive heating and element synthesis. For a set of models that span a large range in both predicted heating and final abundances, we carry out detailed numerical calculations of decay product thermalization and radiation transport in a kilonova ejecta with a fixed mass and density profile. The light curves associated with our models exhibit great diversity in their luminosities, with peak brightness varying by more than an order of magnitude. We also find variability in the shape of the kilonova light curves and their color, which in some cases runs counter to the expectation that increasing levels of lanthanide and/or actinide enrichment will be correlated with longer, dimmer, redder emission.
Missions like NASA's Imaging X-ray Polarimetry Explorer (IXPE) are poised to provide an unprecedented view of the Universe in polarized X-rays. Polarization probes physical anisotropies, a fact exploited by particle physicists to look for the anisotropic a E∙B operator in the axion-like-particle (ALP) Lagrangian. Such studies have typically focused on polarization in the radio and microwaves, through local or cosmic birefringence effects. To such polarization studies we add X-rays emanating from magnetars — a class of neutron stars with near-critical strength magnetic fields — that are important targets for IXPE. ALPs produced in the neutron star core convert to X-rays in the magnetosphere; such X-rays are polarized along the direction parallel to the dipolar magnetic field at the point of conversion. Here, we develop the full theoretical formalism for ALP-induced polarization in the presence of dipolar magnetic fields. For uncorrelated photon and ALP production mechanisms, we completely disentangle the ALP contributions to the Stokes parameters in terms of the ALP intensity, the ALP-to-photon conversion probability, and the ALP-induced birefringence. In the proper limit, our results demonstrate that the inclusion of ALPs suppresses the observed degree of circular polarization compared to its pure astrophysical value. Our results can also be used to impose limits on ALP couplings with IXPE polarization data from magnetars 4U 0142+61 and 1RXS J170849.0-400910, the subject of upcoming work.