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At least 433 records · Page 24

Nuclear Structure Studies at the Limits of Stability

On the quest for a predictive model of atomic nuclei, the properties of rare isotopes have emerged as critical observables that benchmark extrapolations, identify missing physics ingredients in models, or that enable discovery science. Formerly NSCL and now FRIB facilitate world-leading experiments due to the availability of fast, stopped, and reaccelerated rare-isotope beams in conjunction with unique instruments. DOE-SC NP Award DE-SC0020451 supported from 2019 to 2023 MSU’s nuclear structure and reactions program that tackles compelling questions in the field with complementary techniques, probing single-particle and collective degrees of freedom in relevant regions of the nuclear chart and enabled developments that positioned the PIs and their research groups for first FRIB science.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

RAON experimental facilities for nuclear science

The Rare Isotope Science Project (RISP) was established in December 2011 and has put quite an effort to carry out the design and construction of the accelerator complex facility named “RAON”. RAON is a rare isotope (RI) beam facility that aims to provide various RI beams of proton-and neutron-rich nuclei as well as variety of stable ion beams of wide ranges of energies up to a few hundreds MeV/nucleon for the researches in basic science and application. Proposed research programs for nuclear physics and nuclear astrophysics at RAON include studies of the properties of exotic nuclei, the equation of state of nuclear matter, the origin of the universe, process of nucleosynthesis, super heavy elements, etc. Various high performance magnetic spectrometers for nuclear science have been designed, which are KOBRA (KOrea Broad acceptance Recoil spectrometer and Apparatus), LAMPS (Large Acceptance Multi-Purpose Spectrometer), and ZDS (Zero Degree Spectrometer). The status of those spectrometers for nuclear science will be presented with a brief report on the RAON.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Does sedimentary organic delta 13C record variations in quaternary ocean [CO2(aq)]?

Ocean surface water [CO2(aq)] variations based on glacial/interglacial changes in sediment delta 13Corg are shown to compare favorably with reconstructions based on ice core [CO2]. In particular, an approximate 80 microatmospheres increase in atmospheric pCO2 during the last glacial-interglacial transition is calculated to correspond to a 3-4 micromolar increase in ocean surface water [CO2(aq)] at atmospheric equilibrium. A widespread marine delta 13Corg decrease of 1-2% accompanied this event and was not preceded by an equivalent isotopic change in surface water total dissolved inorganic carbon. These observations support the hypothesis that [CO2(aq)] influences photosynthetic isotope fractionation between marine inorganic and organic carbon pools, and therefore that plankton/sediment delta 13Corg may serve as a proxy for surface water [CO2(aq)].

NASA Program Exobiology↗

Design Optimization of A generic Fissile Solution for Mo99 production using Electron Beam-based Neutron Generator using MCNP+CFD

Molybdenum-99 ( 99 Mo) is a medical isotope used in 80% of all medical imaging procedures today. However, 99 Mo is not directly administered to patients for imaging; its decay product, technetium-99m ( 99 mTc), is a metastable isotope with a half-life of ~6 hours. Such a short half-life does not allow for production, separation, and application to a patient before decaying further. Therefore, the solution is to produce the precursor to 99 mTc, 99 Mo. 99 Mo has a half-life of 66 hours, long enough to produce the material and send it to the desired location before it fully decays. Under National Nuclear Security Administration’s (NNSA) highly enriched uranium (HEU) minimization mission, the Material Management and Minimization (M3) office leads the Molybdenum-99 (Mo-99) program. A major goal of the Mo-99 program is to develop methods of producing 99 Mo using low enriched uranium (LEU) opposed to the traditionally used HEU domestically in the U.S. Internationally, LEU is the new standard for use in research reactors and isotope production facility. In this study, we introduce a generic fissile solution system for 99 Mo production facility meeting the design requirement of 1) LEU usage as fissile material and 2) subcritical fissile system coupled with a horizontal electron beam (E-beam) accelerator. The focus of this research is to optimize a fissile solution configuration for maximum 99 Mo production yield using MCNP model, and ultimately implement the optimized design with computational fluid dynamics (CFD) model to understand thermal hydraulic behavior and solution convection characteristic. The report consists of two parts: 1) isotope yield calculation and criticality analysis with a wide range of parametric test matrix, and 2) thermal hydraulic analysis for solution mixing and cooling assessment.

60 APPLIED LIFE SCIENCES↗

Improved Nondestructive Isotopic Analysis with Practical Microcalorimeter Gamma Spectrometers

Advances in both instrumentation and data analysis software are now enabling the first ultra-high-resolution microcalorimeter gamma spectrometers designed for implementation in nuclear facilities and analytical laboratories. With approximately ten times better energy resolution than high-purity germanium detectors, these instruments can overcome important uncertainty limits. Microcalorimeter gamma spectroscopy is intended to provide nondestructive isotopic analysis capabilities with sufficient precision and accuracy to reduce the need for sampling, chemical separations, and mass spectrometry to meet safeguards and security goals. Key milestones were the development of the SOFIA instrument (Spectrometer Optimized for Facility Integrated Applications) and the SAPPY software (Spectral Analysis Program in PYthon). SOFIA is a compact instrument that combines advances in large multiplexed transition-edge sensor arrays with optimized cryogenic performance to overcome many practical limitations of previous systems. With a 256-pixel multiplexed detector array capable of 5,000 counts per second, measurement time can be comparable to high-purity germanium detectors. SAPPY was developed to determine isotopic ratios in data from SOFIA and other microcalorimeter instruments with an approach similar to the widely-used FRAM software. SAPPY provides a flexible framework with rigorous uncertainty analysis for both microcalorimeter and high purity germanium (HPGe) data, allowing direct comparison. Here, we present current results from the SOFIA instrument, preliminary isotopic analysis using SAPPY, and describe how the technology is being used to explore uncertainty limits of nondestructive isotopic characterization, inform safeguards models, and extract improved nuclear data including gamma-ray branching ratios.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

THE NASA NUCLEAR ELECTRIC POWER PROGRAM

The aim of the NASA nuclear electric power program is to provide long-lived reliable nuclear power sources in the range from tens of watts to tens of megawatts for advanced missions. The work is conducted in corporation with the U.S. Atomic Energy Commission which is developing isotope power sources and the reactor for the SNAP-8 project. Isotopes are considered for missions requiring up to several hundred watts of power. SNAP-8 will provide about 35 to 60 kilowatts for missions requiring tens of kilowatts and lifetimes of about one year. SNAP-8 has been redesigned to emphasize reliability and performance. This decision permits many components to operate at lower, more nearly state-of-the -art temperatures at the sacrifice of greater cooling requirements and increased weight. Beyond SNAP-8, an extensive applied research program has been conducted since 1959 to provide the technology required for the sound development of light weight nuclear electric systems in the megawatt range for lifetimes of up to several years. The work is accomplished in university, industrial and government laboratories.

SPACECRAFT POWER SUPPLY↗

Safeguards Technolgy Development Program FY2023 Mid-Year Report

We will develop specific aspects of ultra-high-resolution microcalorimetry that support IAEA NML needs in preparation for transfer of the technology. Two techniques will be considered: gamma spectroscopy for nondestructive isotopic analysis of milligram- to gram-scale uranium and plutonium samples, and decay energy spectroscopy (DES) for isotopic analysis of specially prepared nanogram- to microgram-scale samples of alpha decaying actinides.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Research on Spectroscopy, Opacity, and Atmospheres

To make my calculations more readily accessible I have set up a web site cfaku5.harvard.edu that can also be accessed by FTP. it has 5 9GB disks that hold all of my atomic and diatomic molecular data, my tables of distribution function opacities, my grids of model atmospheres, colors, fluxes, etc, my program that are ready for distribution, most of my recent papers. Atlases and computed spectra will be added as they are completed. New atomic and molecular calculations will be added as they are completed. I got my atomic programs that had been running on a Cray at the San Diego Supercomputer Center to run on my Vaxes and Alpha. I started with Ni and Co because there were new laboratory analyses that included isotopic and hyperfine splitting. Those calculations are described in the appended abstract for the 6th Atomic Spectroscopy and oscillator Strengths meeting in Victoria last summer. A surprising finding is that quadrupole transitions have been grossly in error because mixing with higher levels has not been included. I now have enough memory in my Alpha to treat 3000 x 3000 matrices. I now include all levels up through n=9 for Fe I and 11, the spectra for which the most information is available. I am finishing those calculations right now. After Fe I and Fe 11, all other spectra are "easy", and I will be in mass production. ATL;LS12, my opacity sampling program for computing models with arbitrary abundances, has been put on the web server. I wrote a new distribution function opacity program for workstations that replaces the one I used on the Cray at the San Diego Supercomputer Center. Each set of abundances would take 100 Cray hours costing $100,000. 1 ran 25 cases. Each of my opacity CDs contains three abundances. I have a new program -iinning on the Alpha that takes about a week. I am going to have to get a faster processor or I will have to dedicate a whole workstation just to opacities.

Kurucz, Robert L.↗

Carbon and nitrogen isotopic compositions of alkyl porphyrins from the Triassic Serpiano oil shale

The carbon and nitrogen isotopic compositions of seven of the most abundant alkylporphyrins from the Serpiano oil shale (marine, Triassic) were determined. For the C31 and C32 butanoporphyrins, values of delta 13CPDB and delta 15NAIR averaged -24.0% and -3.1%. In contrast, the C31 and C32 methylpropanoporphyrins, DPEP, and a C30 13-nor etioporphyrin had delta 13C and delta 15N values averaging -27.5 and -3.3%, respectively. Carbon and nitrogen isotopic values for kerogen averaged -30.8 and -0.9, whereas those for total extract averaged -31.6, and -4.0%. The butanoporphyrins apparently derive from a biological source different from that giving rise to the other porphyrins, their 13C enrichment not being related to carbon isotopic fractionation accompanying diagenetic reactions. The delta 15N values for all the porphyrins indicate that the depletion of 15N observed in the kerogen is of primary origin. Consistent with the very high abundance of hopanoids and methyl hopanoids in the aliphatic hydrocarbon fraction, it is suggested that cyanobacterial fixation of N2 may have been the main cause of 15N depletion.

NASA Discipline Exobiology↗

The ATLAS multi-user upgrade and potential applications

With the recent integration of the CARIBU-EBIS charge breeder into the ATLAS accelerator system to provide for more pure and efficient charge breeding of radioactive beams, a multi-user upgrade of the ATLAS facility is being proposed to serve multiple users simultaneously. ATLAS was the first superconducting ion linac in the world and is the US DOE low-energy Nuclear Physics National User Facility. The proposed upgrade will take advantage of the continuous-wave nature of ATLAS and the pulsed nature of the EBIS charge breeder in order to simultaneously accelerate two beams with very close mass-to-charge ratios; one stable from the existing ECR ion source and one radioactive from the newly commissioned EBIS charge breeder. In addition to enhancing the nuclear physics program, beam extraction at different points along the linac will open up the opportunity for other potential applications; for instance, material irradiation studies at ~ 1 MeV/u and isotope production at ~ 6 MeV/u or at the full ATLAS energy of ~ 15 MeV/u. Furthermore, the concept and proposed implementation of the ATLAS multi-user upgrade will be presented. Future plans to enhance the flexibility of this upgrade will also be presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Hawthorne Nevada Deep Direct-Use Feasibility Study - Temperature and Geochemistry Well Data

The objective of this project is to use a multi-disciplinary, three-tiered approach to assess the geothermal resource and determine the feasibility of implementing a large-scale, direct-use facility for the Hawthorne Army Depot (HAD) and the various town and county facilities in Hawthorne, Nevada. This assessment directly targets a geothermal resource recently characterized by the Navy Geothermal Program Office (GPO) as part of a focused exploration and development campaign. This data batch contains: Zip file containing well and water data from 2002, including reports, isotope analysis, shallow well data, and data by well; Zip folder containing 2009 GPO well data including well logs, geochemistry, and mud logs; Compiled data from 2010 in excel and word format; 2010 Final data from TG, well HAD-1; Zip file containing PDFs and Excel files for wells Haw1, HAD1, HWADD2-3, HWAD4-5; Zip folder containing Word docs and images pertaining to final well reports and discussion.

15 GEOTHERMAL ENERGY↗

Isotopic analysis of plutonium measured with very thick absorbers and high-granularity spectra

FRAM is LANL-designed software designed to extract plutonium and uranium isotopic information from gamma ray spectra. This is an important capability for NEST and STAB; however, FRAM performance has been poor when applied to field data collected in these programs. FRAM Version 5 (commercially available) was fine-tuned and validated for laboratory quality measurements but not for measurements of the high-mass and heavily shielded SNM items encountered in NEST. FRAM is untested for spectra collected with high-granularity lower resolution instruments such as the new 8-MeV Detective-X favored by STAB or the new custom electrocooled systems coming into use for NEST. FRAM Version 6.1 (unreleased) has improvements in physics capabilities, and parameter sets may be adapted that are more specific to NEST and STAB, which is what we have attempted for this assignment. Thick shielding attenuates gamma rays profoundly, especially those at low energy, making them too weak to be measured. The missing low-energy peaks force the analysis to employ only the highest-energy peaks. We adapted FRAM 6.1 for analysis of plutonium spectra obtained with very thick Pb filters (a surrogate for NEST-type configurations). New parameter sets employing only very high energy peaks were created for the analysis. High granularity and low resolution make deconvolution of the 600-keV region particularly challenging, and we have worked to optimally extract information from this region. The results shown in this paper give high confidence that we are on the right track. We used a combination of real and synthetically-modified data. Remaining work includes testing the new software and parameters against genuine data collected with Detective-X and new NEST systems, but such datasets at the moment are unavailable. It also remains to develop and test parameter sets specific to uranium and the new detectors.

07 ISOTOPE AND RADIATION SOURCES↗

Sources of carbon and sulfur nutrition for consumers in three meromictic lakes of New York State

The trophic importance of bacterioplankton as a source of carbon and sulfur nutrition for consumers in meromictic lakes was tested using stable carbon (delta 13C) and sulfur (delta 34S) isotopic measurements. Studies in three lakes near Syracuse, New York, showed that most consumers ultimately derive their C and S nutrition from a mixture of terrestrial detritus, phytoplankton, and littoral vegetation, rather than from bacterioplankton. Food webs in these meromictic lakes are thus similar to those in other lakes that lack dense populations of bacterioplankton.

NASA Discipline Exobiology↗

OECD NEA Benchmark Database of Spent Nuclear Fuel Isotopic Compositions for World Reactor Designs

Experimental data on the isotopic concentrations in irradiated nuclear fuel represent one of the primary methods for validating computational methods and nuclear data used for reactor and spent fuel depletion simulations that support nuclear fuel cycle safety and safeguards programs. Measurement data have previously not been available to users in a centralized or searchable format, and the majority of accessible information has been, for the most part, limited to light-water-reactor designs. This paper describes a recent initiative to compile spent fuel benchmark data for additional reactor designs used throughout the world that can be used to validate computer model simulations that support nuclear energy and nuclear safeguards missions. Experimental benchmark data have been expanded to include VVER-440, VVER-1000, RBMK, graphite moderated MAGNOX, gas cooled AGR, and several heavy-water moderated CANDU reactor designs. Additional experimental data for pressurized light water and boiling water reactor fuels has also been compiled for modern assembly designs and more extensive isotopic measurements. These data are being compiled and uploaded to a recently revised structured and searchable database, SFCOMPO, to provide the nuclear analysis community with a centrally-accessible resource of spent fuel compositions that can be used to benchmark computer codes, models, and nuclear data. The current version of SFCOMPO contains data for eight reactor designs, 20 fuel assembly designs, more than 550 spent fuel samples, and measured isotopic data for about 80 nuclides.

Gauld, Ian C↗

Precision Tests of the Electroweak Interaction using Trapped Atoms and Ions

The objective of the proposed research is to study fundamental aspects of the electroweak interaction via precision measurements in beta decay to test our current understanding of fundamental particles and forces as contained in the so-called "Standard Model" of particle physics. By comparing elegant experiments to rigorous theoretical predictions, we will either confirm the Standard Model to a higher degree and rule out models which seek to extend it, or find evidence of new physics and help guide theorists in developing the New Standard Model. The use of ion and neutral atom traps at radioactive ion beam facilities has opened up a new vista in precision low-energy nuclear physics experiments. Traps provide an ideal source of decaying atoms: they can be extremely cold (~1 mK); they are compact (~1 mm^3); and perhaps most importantly, the daughter particles escape with negligible distortions to their momenta in a scattering-free, open environment. The project is taking advantage of these technologies and applying them to precision beta-decay studies at radioactive beam facilities. The program consists of two complementary efforts: 1) Ion traps are an extremely versatile tool for purifying, cooling and bunching low-energy beams of short-lived nuclei. A large-bore (210~mm) superconducting 7-Tesla solenoid is at the heart of a Penning trap system for which there is a dedicated beamline at T-REX, the upgraded radioactive beam facility at the Cyclotron Institute, Texas A&M University. In addition to providing a general-purpose decay station, the flagship program for this system is measuring the ft-values and beta-neutrino correlation parameters from isospin T=2 superallowed beta-delayed proton decays, complimenting and expanding the already strong program in fundamental interactions at the Institute. 2) A magneto-optical trap is being used at the TRIUMF Neutral Atom Trap facility to observe the (un)polarized angular distribution parameters of isotopes of potassium. We are able to highly polarize laser-cooled atoms and observe their decay with unprecedented precision. The correlation of the daughter beta particle with the initial nuclear spin as well as other correlations are sensitive to physics beyond the Standard Model. Both of these cutting-edge and exciting research efforts will test our understanding of the fundamental symmetries underlying our current theory of electroweak interactions. Complementary to high-energy collider experiments, these low-energy nuclear physics "table-top" experiments will search for new particles and interactions which are not already described by the Standard Model of particle physics. The value of this research is recognized to be cross-disciplinary, exciting and potentially revolutionary in our understanding of nature's fundamental interactions. Accordingly, it has been endorsed by the recent (2007) Nuclear Science Advisory Committee's Long Range Plan as part of their recommendation for a "New Standard Model Initiative." In addition to the near-term benefits of scholarly publications and visibility through description of this work at international conferences, an important benefit of this research program is the training of new, young and enthusiastic nuclear physicists. Participants in this demanding and rewarding field develop a very strong background in physics with experience in a range of its subfields since we use atomic techniques and apply them to a nuclear physics experiment which in the end tests the theories of high-energy physics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Irradiation of Advanced Cladding Specimens in the High Flux Isotope Reactor: Capsule Designs and Test Matrix

The Advanced Fuels Campaign (AFC) has initiated the Advanced Reactor Cladding (ARC) irradiation campaign to generate irradiation performance data for candidate fuel cladding concepts. The campaign includes a diverse set of ferritic/martensitic steels, oxide dispersion strengthened (ODS) alloys, FeCrAlbased alloys, coated materials, and welded cladding specimens produced through multiple US Department of Energy (DOE) programs and international collaborations. Three complementary experimental thrusts comprise the campaign: tensile testing (ARC Tensile) to rapidly screen candidate alloys, fracture toughness testing (ARC Fracture) to evaluate irradiation effects on crack resistance, and tubular weld testing (ARC Weld) to quantify irradiation-induced changes in the mechanical performance of end cap welds. This report documents the irradiation campaign design, including the selected materials, specimen types, irradiation matrix, and capsule designs for irradiation within the High Flux Isotope Reactor (HFIR). A total of 14 irradiation capsules were developed to achieve target irradiation temperatures between 300°C and 600°C and doses up to 30 dpa. Thermal analyses were performed using finite element methods to establish capsule geometries capable of achieving the desired specimen temperatures while accommodating differences in specimen geometry and material properties. The resulting capsule designs provide the basis for irradiation of the AFC-ARC experimental matrix and subsequent post-irradiation examination to assess the effects of neutron irradiation on advanced cladding materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

History and Future of Isotope Production

Operations at the IPF were initiated in October 1976. LAMPF was delivering 800 MeV protons at a current of 300 µA. Initially, only pure-metal targets were selected for irradiation. These included Mo, Ni, Ta, Si, V, Al and Cu, which ranged in mass from a few to several hundred g. One program required a multi-Ci quantity of 88 Y that necessitated the irradiation and processing of more than 5 kg of Mo metal. As experience was gained, it was learned that oxide and salt targets could safely be irradiated, and eventually the sweeping and cold trapping of radioxenon gas from a molten CsCl during irradiation. Operations ended in 1992.

07 ISOTOPE AND RADIATION SOURCES↗

Preliminary assessment of rover power systems for the Mars Rover Sample Return Mission

Four isotope power system concepts were presented and compared on a common basis for application to on-board electrical prime power for an autonomous planetary rover vehicle. A representative design point corresponding to the Mars Rover Sample Return (MRSR) preliminary mission requirements (500 W) was selected for comparison purposes. All systems concepts utilize the General Purpose Heat Source (GPHS) isotope heat source developed by DOE. Two of the concepts employ thermoelectric (TE) conversion: one using the GPHS Radioisotope Thermoelectric Generator (RTG) used as a reference case, the other using an advanced RTG with improved thermoelectric materials. The other two concepts employed are dynamic isotope power systems (DIPS): one using a closed Brayton cycle (CBC) turboalternator, and the other using a free piston Stirling cycle engine/linear alternator (FPSE) with integrated heat source/heater head. Near term technology levels have been assumed for concept characterization using component technology figure-of-merit values taken from the published literature. For example, the CBC characterization draws from the historical test database accumulated from space Brayton cycle subsystems and components from the NASA B engine through the mini-Brayton rotating unit. TE system performance is estimated from Voyager/multihundred Watt (MHW)-RTG flight experience through Mod-RTG performance estimates considering recent advances in TE materials under the DOD/DOE/NASA SP-100 and NASA Committee on Scientific and Technological Information programs. The Stirling DIPS system is characterized from scaled-down Space Power Demonstrator Engine (SPDE) data using the GPHS directly incorporated into the heater head. The characterization/comparison results presented here differ from previous comparison of isotope power (made for Low Earth Orbit (LEO) applications) because of the elevated background temperature on the Martian surface compared to LEO, and the higher sensitivity of dynamic systems to elevated sink temperature. The mass advantage of dynamic systems is significantly reduced for this application due to Mars' elevated background temperature.

Bents, David J.↗