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At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Shear-Induced Gelation of Self-Yielding Active Networks

An enticing feature of active materials is the possibility of controlling macroscale rheological properties through the activity of the microscopic constituents. Using a unique combination of microscopy and rheology we study three dimensional microtubule-based active materials whose autonomous flows are powered by a continually rearranging connected network. We quantify the relationship between the microscopic dynamics and the bulk mechanical properties of these nonequilibrium networks. Experiments reveal a surprising nonmonotonic viscosity that strongly depends on the relative magnitude of the rate of internally generated activity and the externally applied shear. Here, a simple two-state mechanical model that accounts for both the solidlike and yielded fluidlike elements of the network accurately describes the rheological measurements.

36 MATERIALS SCIENCE↗
DOE OSTI2025

CFD modeling and simulation for corrosive wear of refractory in molten slag

The development of high-wear resistant refractories having minimal production costs is facilitated by characterizing the wear mechanisms associated with their corrosive wear. Static cup testing is a commonly used method for comparing the corrosion resistance performance of two or more refractory materials. Although the static cup test conditions are not as severe as dynamic tests, this study shows that the thermal gradient present within the system during heating and cooling stages serves to generate movement of the slag leading to mechanical wear. The thermal gradient within the refractory, and between the slag and the refractory, occurs during the ramp stage of the test and lasts until the soaking stage is reached bringing the system to a thermal equilibrium. Using computational fluid dynamics (CFD) capabilities embedded within ANSYS software, this study modelled and quantified the convection currents within the slag and associated shear stresses generated on the refractory walls due to the thermal gradient. A traditional ladle furnace was employed as a case study to verify the results of the studied CFD model. The corrosion rate of the refractory lining was found to depend on the mass transfer coefficient of the refractory dissolution into the slag, and a velocity term which governs the extent of corrosion at any given location. This velocity term is a function of slag viscosity, as well as the concentration gradient and/or temperature gradient at the triple points. In this study, wall shear stress was used as a reliable proxy for identifying high-velocity regions prone to excessive corrosive wear. Elevated wall shear stress near the slag/air and slag/molten steel interfaces align with observed corrosion grooves, which reflects the intensified corrosive wear at these locations.

Ramteke, Rajat Rajat Durgesh Ramteke [University o↗
DOE OSTI2021

Viscosity Analysis of Battery Electrode Slurry

We report the effects of component ratios and mixing time on electrode slurry viscosity. Three component quantities were varied: active material (graphite), conductive material (carbon black), and polymer binder (carboxymethyl cellulose, CMC). The slurries demonstrated shear-thinning behavior, and suspension properties stabilized after a relatively short mixing duration. However, micrographs of the slurries suggested their internal structures did not stabilize after the same mixing time. Increasing the content of polymer binder CMC caused the greatest viscosity increase compared to that of carbon black and graphite.

25 ENERGY STORAGE↗
NASA NTRS2001

ZBLAN Viscosity Instrumentation

The past year's contribution from Dr. Kaukler's experimental effort consists of these 5 parts: a) Construction and proof-of-concept testing of a novel shearing plate viscometer designed to produce small shear rates and operate at elevated temperatures; b) Preparing nonlinear polymeric materials to serve as standards of nonlinear Theological behavior; c) Measurements and evaluation of above materials for nonlinear rheometric behavior at room temperature using commercial spinning cone and plate viscometers available in the lab; d) Preparing specimens from various forms of pitch for quantitative comparative testing in a Dynamic Mechanical Analyzer, Thermal Mechanical Analyzer; and Archeological Analyzer; e) Arranging to have sets of pitch specimens tested using the various instruments listed above, from different manufacturers, to form a baseline of the viscosity variation with temperature using the different test modes offered by these instruments by compiling the data collected from the various test results. Our focus in this project is the shear thinning behavior of ZBLAN glass over a wide range of temperature. Experimentally, there are no standard techniques to perform such measurements on glasses, particularly at elevated temperatures. Literature reviews to date have shown that shear thinning in certain glasses appears to occur, but no data is available for ZBLAN glass. The best techniques to find shear thinning behavior require the application of very low rates of shear. In addition, because the onset of the thinning behavior occurs at an unknown elevated temperature, the instruments used in this study must provide controlled low rates of shear and do so for temperatures approaching 600 C. In this regard, a novel shearing parallel plate viscometer was designed and a prototype built and tested.

Kaukler, William↗
NASA NTRS1988

Extension of the Johnson-King turbulence model to the 3-D flows

A critical evaluation of the eddy viscosity model of Johnson and King extended to the three-dimensional case has been performed for three-dimensional boundary layer flows. The turbulence model is evaluated by a detailed comparison with available experimental data for incompressible flows over an infinite swept wing and near an idealized wing-body junction. The isotropic model of Johnson and King is found to work much better than the Cebeci-Smith model, especially in regions of strong cross flow. The significant decrease in the shear stress magnitude is almost reproduced. This means that this effect is as important as the nonisotropic eddy viscosity. The introduction of Rotta's modification to account for nonisotropic eddy viscosity in the Johnson-King formulation is found to have little effect on the predictions. The cross-flow properties are the most strongly affected.

Abid, Ridha↗
NASA NTRS1992

Enhanced damping of Alfven waves in the solar corona by a turbulent wave spectrum

The effect of a background spectrum of Alfven waves on the rate of dissipation of a test shear Alfven wave is numerically calculated. The results demonstrate that as the classical resistivity eta and classical viscosity mu become small, the damping rate of the Alfven wave remains large and depends only on the amplitude for the scalar potential of the wave spectrum and the wavenumber of the Alfven wave. The damping rate is virtually independent of eta and mu. The wave spectrum need not be turbulent or stochastic to affect the damping rate. The dissipation rate is nonlinear enhanced by nonstochastic spectra as well as by stochastic spectra if two conditions are met. First, the perpendicular magnetic field associated with Alfven wave spectrum must exceed a certain collision-frequency threshold and second, for nonstochastic spectra only, the magnetic field must exceed a threshold proportional to the parallel wavenumber of the shear Alfven wave. These conditions can be easily satisfied in the solar corona.

Kleva, Robert G.↗
DOE OSTI2020

A buoyancy–shear–drag-based turbulence model for Rayleigh–Taylor, reshocked Richtmyer–Meshkov, and Kelvin–Helmholtz mixing

A phenomenological turbulence model for Rayleigh–Taylor, reshocked Richtmyer–Meshkov, and Kelvin–Helmholtz instability-induced mixing is developed using a general buoyancy–shear–drag model. Analytic solutions to the simplified model equations corresponding to each instability are derived separately, which are then used to calibrate the model coefficients to predict specific values of the mixing layer growth parameters and exponents. The buoyancy-shear–drag equations for the bubble and spike mixing layer widths are then solved numerically, and a turbulent diffusivity (or viscosity) is constructed dimensionally as the product of the mixing layer width, h, and its time-derivative, dh/dt. Surrogate turbulent fields are then constructed by multiplying a presumed, approximate self-similar spatial profile by appropriate functions of h and dh/dt. Using several simplifying approximations, the turbulent diffusion equations satisfied by the mean mass fraction and mean shear velocity are solved analytically in a reference frame moving with the mean advection velocity, and it is shown that the mean fields evolve in space and time as expected. The explicit modeling and solution of turbulent transport equations (e.g., for the turbulent kinetic energy and its dissipation rate or a lengthscale) are not required. By using separate equations for the bubble and spike evolution, the model naturally captures the asymmetry induced by an increasing density contrast between the heavy and light fluids. The model also includes molecular dissipation and diffusion, and therefore, can describe transition to fully-developed turbulence if the initial turbulent diffusivity/viscosity is much smaller than the molecular diffusivity/viscosity. This model is applied to constant-acceleration Rayleigh–Taylor, impulsively reshocked Richtmyer–Meshkov, and variable-density Kelvin–Helmholtz mixing layers to demonstrate its utility. It is shown that the numerical solutions of the model calibrated using specific values of the instability growth parameters and exponents: (1) produces mixing layer widths in agreement with the expected self-similar growth power laws; (2) gives spatiotemporal profiles of turbulent fields that are expected and consistent with previous results; (3) predicts the expected power-law growths and decays of the spatially-integrated turbulent fields, and; (4) gives spatiotemporal profiles of the mean fields that are expected and consistent with previous results. This relatively simple model can be implemented numerically, and is expected to be useful for fundamental as well as astrophysical and inertial confinement fusion applications.

42 ENGINEERING↗
NASA NTRS1998

Sand Shear Band Thickness Measurements by Digital Imaging Techniques

Digital imaging analysis was used to study localized deformations in granular materials tested under plane strain condition. Two independent techniques were applied and compared. In the first, the digitized optical images of a grid printed on the latex membrane were used to measure the shear band orientation angle and thickness, and were found to be 54.5' and 3.01 mm respectively. The second technique involved introducing an ultra-low viscosity resin into the specimen in preparation for thin- sectioning and microscopic study of the internal fabric. A total of 24 microscopic images obtained from four thin sections were analyzed and void ratio variation was measured. The shear band thickness measurements from images located along the shear band axis (at two locations) were equal to 3.19 mm and 3.29 mm which are very close to the average value obtained from surface analysis. The study was then extended to investigate the effects of sand grain-size and properties, specimen density, and confining pressure on shear band thickness. It was found that the normalized shear band thickness decreases as grain-size and confining pressure increase and as density decreases. Finally, shear band thickness is highly influenced by the specimen dilatancy.

Alshibli, Khalid A.↗
NASA NTRS1976

Thermal and mechanical structure of the upper mantle: A comparison between continental and oceanic models

Temperature, velocity, and viscosity profiles for coupled thermal and mechanical models of the upper mantle beneath continental shields and old ocean basins show that under the continents, both tectonic plates and the asthenosphere, are thicker than they are beneath the oceans. The minimum value of viscosity in the continental asthenosphere is about an order of magnitude larger than in the shear zone beneath oceans. The shear stress or drag underneath continental plates is also approximately an order of magnitude larger than the drag on oceanic plates. Effects of shear heating may account for flattening of ocean floor topography and heat flux in old ocean basins.

Froidevaux, C.↗
NASA NTRS1991

Simulation of 3-D shear flows around a nozzle-afterbody at high speeds

3D, compressible, unsteady, Reynolds-averaged Navier-Stokes equations are presently solved by a finite-volume and alternating-direction-implicit method in order to simulate supersonic and hypersonic turbulent shear flows. The effect of turbulence is incorporated via a modified Baldwin-Lomax eddy viscosity model which reflects the influence of high-speed compressibility, multiple walls, near-wall vortices, and turbulent memory effects, as well as local equilibrium effects. Attention is given to the simulation of the flow around the nozzle-afterbody of a generic, scramjet-propelled hypersonic vehicle; computed pressure distributions are consonant with experimental surface and off-surface flow surveys.

Baysal, Oktay↗
DOE OSTI2020

Shear Thickening and Jamming of Dense Suspensions: The "Roll" of Friction.

Particle-based simulations of discontinuous shear thickening (DST) and shear jamming (SJ) suspensions are used to study the role of stress-activated constraints, with an emphasis on resistance to gearlike rolling. Rolling friction decreases the volume fraction required for DST and SJ, in quantitative agreement with real-life suspensions with adhesive surface chemistries and "rough" particle shapes. It sets a distinct structure of the frictional force network compared to only sliding friction, and from a dynamical perspective leads to an increase in the velocity correlation length, in part responsible for the increased viscosity. The physics of rolling friction is thus a key element in achieving a comprehensive understanding of strongly shear-thickening materials.

Singh, Abhinendra↗
DOE OSTI2021

Shear-free mixing to achieve accurate temporospatial nanoscale kinetics through scanning-SAXS: ion-induced phase transition of dispersed cellulose nanocrystals

Time-resolved in situ characterization of well-defined mixing processes using small-angle X-ray scattering (SAXS) is usually challenging, especially if the process involves changes of material viscoelasticity. In specific, it can be difficult to create a continuous mixing experiment without shearing the material of interest; a desirable situation since shear flow both affects nanoscale structures and flow stability as well as resulting in unreliable time-resolved data. Here, we demonstrate a flow-focusing mixing device for in situ nanostructural characterization using scanning-SAXS. Given the interfacial tension and viscosity ratio between core and sheath fluids, the core material confined by sheath flows is completely detached from the walls and forms a zero-shear plug flow at the channel center, allowing for a trivial conversion of spatial coordinates to mixing times. With this technique, the time-resolved gel formation of dispersed cellulose nanocrystals (CNCs) was studied by mixing with a sodium chloride solution. It is observed how locally ordered regions, so called tactoids, are disrupted when the added monovalent ions affect the electrostatic interactions, which in turn leads to a loss of CNC alignment through enhanced rotary diffusion. The demonstrated flow-focusing scanning-SAXS technique can be used to unveil important kinetics during structural formation of nanocellulosic materials. However, the same technique is also applicable in many soft matter systems to provide new insights into the nanoscale dynamics during mixing.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Theory and simulations of linear and nonlinear two-dimensional Rayleigh–Taylor dynamics with variable acceleration

Interfacial Rayleigh–Taylor mixing is crucial to describing important natural and engineering processes, such as exploding supernovae, laser micromachining, hot spots in inertial confinement fusion, and optical telecommunications. These require the characterization of the time dependence of the driving acceleration. We compare our theoretical formulation based on group theory foundations with interface-capturing numerical simulations for linear and nonlinear two-dimensional Rayleigh–Taylor instabilities in a finite-sized domain with time-varying acceleration over broad ranges of Atwood numbers and acceleration exponents. Detailed corroboration between theory and simulations is provided for this foundational case. Both demonstrate the strong interfacial nature of Rayleigh–Taylor instabilities, which suggests that practical flow fields can be reconstructed from the derived fluid potential using the proposed theory. A robust agreement is also obtained for the early and late-time evolution of the amplitudes of the bubble and spike, which demonstrate that the Rayleigh–Taylor flow can transition to the mixing regime even for a single-mode initial perturbation. Corroboration with experiments of high energy density plasmas motivated by studies of supernovae is also achieved. In addition, a long-standing puzzle in Rayleigh–Taylor dynamics on the interplay between the acceleration, the shear, and the interface morphology in the theory and simulations is resolved by accounting for finite viscosity of the fluids. The characterization of Rayleigh–Taylor instabilities as a highly interfacial phenomenon provides valuable insight into its multiscale nature, which enhances the design and understanding of numerous processes of practical interest.

42 ENGINEERING↗
DOE OSTI2020

A Pilot-Scale Evaluation of Natural Gas-Based Foam at Elevated Pressure and Temperature Conditions

Abstract Nitrogen (N2) and Carbon Dioxide (CO2) foams have been used as hydraulic fracturing fluids for several decades to reduce water usage and minimize damage in water-sensitive reservoirs. These foam treatments require gases to be liquefied and transported to site. An alternative approach would be to use natural gas (NG) that is readily available from nearby wells, pipelines, and processing facilities as the internal, gaseous phase to create a NG-based foam. Hydraulic fracturing with NG foam is a relatively inexpensive option, makes use of an abundant and often wasted resource, and may even provide production benefits in certain reservoirs. As part of an ongoing development project sponsored by the Department of Energy (DOE), the surface process to create NG foam is being developed and the properties of NG foam are being explored. This paper presents recent results from a rigorous pilot-scale demonstration of NG foam over a range of operating scenarios relevant to surface and bottomhole conditions with a variety of base-fluid mixtures. The Pilot-scale Foam Test Facility (PFTF) used in these investigations is first described. The PFTF is capable of generating foamed fluids at pressures up to 7,500 psig and at temperatures in excess of 300°F. Then, results from several investigations aimed at proving NG foam at conditions relevant to the field are presented. NG foam was characterized using rheology measurements and flow visualization techniques. Experiments were performed to investigate the texture and stability of NG foam generated by two different mixing methods: one using a custom designed tee to match mixing velocities in the field where the gas phase is jetted into the aqueous stream, and another to ensure comprehensive mixing for laboratory analysis. Parametric studies were conducted to explore the effects of flow rate, foam quality, and temperature on the stability of NG foam. Moreover, different fluid preparations were used to investigate the effect of base fluid and additive concentrations on the stability of NG foams. Additional laboratory studies that investigated foam stability with produced water and multicomponent NG mixtures are also reported. The NG foams explored in these investigations exhibited typical, shear-thinning behavior observed in rheological studies of N2- and CO2-based foams. The measured viscosity and observed stability indicate that NG foams are well suited for fracturing applications. Like other foams, NG foam exhibits sensitivity to operating temperature characterized by a decrease in apparent viscosity as temperature increases. Rapid foam breakdown was observed at significantly elevated temperatures exceeding 290°F. In addition to fluid characterization, these investigations also yielded several key lessons that should be applied to future field demonstrations of NG foam.

Beck, Griffin↗
NASA NTRS1982

Turbulence modeling for computational aerodynamics

The status of turbulence modeling for external aerodynamic flows is reviewed, and closure concepts for the compressible form of the Reynolds-averaged Navier-Stokes equations are briefly outlined to establish a framework for comparison. The importance of experimental requirements for developing and verifying turbulence models is emphasized. Attention is then given to three important flow categories: attached flows, separating and reattaching flows, and trailing-edge flows. Examples of comparisons between experiments and computations for twoand three-dimensional flows are presented to illustrate the status of modeling. It is shown that, for most two-dimensional attached flows, eddy viscosity concepts will probably be adequate. For attached three-dimensional flows, however, eddy-viscosity and Reynolds-stress models are both deficient, failing to predict the proper surface shear-stress in rapidly skewing boundary layers, regardless of whether they are pressure driven or strain driven.

Marvin, J. G.↗
NASA NTRS1984

Lubricant Rheology in Concentrated Contacts

A revue of experimental investigations of lubricant behaviour in highly stressed situations shows that a Newtonian model for lubricant rheology is insufficient for explanation of traction behaviour. The oil film build-up, on the other hand, is fairly well predicted using a Newtonian lubricant model except at high slide to roll ratios and at very high loads, where the non-Newtonian behaviour starts to be important already outside the Hertzian contact area. Two main types of experiments are reported: static and dynamic. In static experiments the pressure is typically applied to the lubricant more than a million times longer than in an EHD contact. Depending on the pressure-temperature history of the experiment the lubricant will become a crystallized or amorphous solid at high pressures. In dynamic experiments, where the pressure is applied as short time as in real EHD contacts, the oil is in an amorphous solid state. Depending on the viscosity, time-scale, elasticity of the oil and the bearing surfaces, the oil film pressure, shear strain rate and the type of lubricant, different properties of the oil are important for prediction of shear stresses in the oil. This can be seen from the different proposed models for the lubricant, where it is described as being for instance a Newtonian liquid, an elastic liquid, a plastic liquid and an elastic-plastic solid.

Bo O Jacobson↗
NASA NTRS1997

Turbulence Measurements in the Near Field of a Wingtip Vortex

The roll-up of a wingtip vortex, at Reynolds number based on chord of 4.6 million was studied with an emphasis on suction side and near wake measurements. The research was conducted in a 32 in. x 48 in. low-speed wind tunnel. The half-wing model had a semi-span of 36 in. a chord of 48 in. and a rounded tip. Seven-hole pressure probe measurements of the velocity field surrounding the wingtip showed that a large axial velocity of up to 1.77 U(sub infinity) developed in the vortex core. This level of axial velocity has not been previously measured. Triple-wire probes have been used to measure all components of the Reynolds stress tensor. It was determined from correlation measurements that meandering of the vortex was small and did not appreciably contribute to the turbulence measurements. The flow was found to be turbulent in the near-field (as high as 24 percent RMS w - velocity on the edge of the core) and the turbulence decayed quickly with streamwise distance because of the nearly solid body rotation of the vortex core mean flow. A streamwise variation of the location of peak levels of turbulence, relative to the core centerline, was also found. Close to the trailing edge of the wing, the peak shear stress levels were found at the edge of the vortex core, whereas in the most downstream wake planes they occurred at a radius roughly equal to one-third of the vortex core radius. The Reynolds shear stresses were not aligned with the mean strain rate, indicating that an isotropic-eddy-viscosity based prediction method cannot accurately model the turbulence in the cortex. In cylindrical coordinates, with the origin at the vortex centerline, the radial normal stress was found to be larger than the circumferential.

Chow, Jim↗