AI-enabled Automation of Atomic Manipulation and Characterization in the STEM
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Roccapriore, Kevin↗
SEARCH · Engineering Papers
Results for “stemming”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Irradiation Effect on Noble Metal Particles in Water Using in situ Liquid Cell STEM Observation
During geologic disposal of spent nuclear fuel (SNF) in an engineered nuclear waste repository, once all other barriers have degraded, oxidizing may occur at the solid-water interface owing to a self-generated radiolytic field. The repository design includes large quantities of iron (Fe), that is anticipated to corrode under an anoxic environment, and generate hydrogen (H 2 ) gas. This H 2 gas is thought to be able to suppress the dissolution of SNF through a catalytic reaction with noble metal particles (NMP) that are pre-existing in the SNF. This interaction leads to the decomposition of the major oxidant, hydrogen peroxide (H 2 O 2 ). In conclusion, these processes are described in the Fuel Matrix Degradation (FMD) model that is being used to predict SNF degradation rates. The NMP, therefore, plays an important role within the FMD model.
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
Investigation of Cu Species in Dealuminated Beta Zeolite Studied by Operando Closed-Cell Gas Reaction STEM
Direct conversion of ethanol to C3+ olefins is an attractive pathway to produce sustainable aviation fuels [1]. We recently reported a copper-containing catalyst supported on dealuminated (DeAl) beta zeolite that is capable of catalyzing cascade ethanol to olefins reactions with high olefins selectivity (88% C3+ olefin selectivity at 100% ethanol conversion). However, one of the deactivation mechanisms of the catalyst is copper sintering [2]. It was found that copper agglomerates can be redispersed through a simple oxidative treatment. To better understand the kinetics and process conditions conducive to redispersion, we studied the atmosphere and temperature dependent Cu species in Cu/DeAl-Beta catalyst under conditions matching those of the working catalyst.
beta zeolite↗
Uncertainties on the EFT coupling limits for direct dark matter detection experiments stemming from uncertainties of target properties
Not Available
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Uncertainties in tellurium-based dark matter searches stemming from nuclear structure uncertainties
Using tellurium dioxide as a target, we calculate uncertainties on 90% upper confidence limits of Galilean effective field theory (Galilean EFT) couplings to a weakly interacting massive particle (WIMP) dark matter candidate due to uncertainties in nuclear shell models. We find that these uncertainties in naturally occurring tellurium isotopes are comparable across the different Galilean EFT couplings to uncertainties in xenon, with some reaching over 100%. We also consider the effect these nuclear uncertainties have on estimates of the annual modulation of dark matter from these searches, finding that the uncertainties in the modulation amplitude are proportional to the nonmodulating upper confidence limit uncertainties. We also show that the determination of the modulation phase is insensitive to changes in the nuclear model for a given isotope.
79 ASTRONOMY AND ASTROPHYSICS↗
Real-space visualization of atomic displacements in a long-wavelength charge density wave using cryogenic 4D-STEM
EuAl 4 , a known skyrmion magnet, represents a class of materials that show complex electronic behaviors involving long-wavelength charge density wave (CDW). Here we realize direct real-space imaging of the concomitant periodic lattice distortion (PLD) with picometer precision in EuAl 4 . Simultaneous imaging of microstructure, polarization, and interatomic distance is made possible using cryogenic four-dimensional scanning transmitting electron microscopy (cryo-4DSTEM). With this approach, we determined that the PLD in EuAl 4 incorporates two out-of-phase atomic displacement modes on the Eu and Al sublattices. The PLD introduces periodic local symmetry fluctuations from the average symmetry of the bulk EuAl 4 crystal. This critical local structural insight helps understanding of charge-spin-lattice couplings behind the intertwined quantum order in EuAl 4 . Furthermore, our results also demonstrate cryo-4DSTEM as an indispensable approach for probing CDW and related quantum materials at low temperatures.
Ni, Haoyang↗
Broad betacoronavirus neutralization by a stem helix–specific human antibody
Targeting a range of betacoranaviruses In the past 20 years, three highly pathogenic β-coronaviruses have crossed from animals to humans, including the most recent: severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2). A spike protein that decorates these viruses has an S1 domain that binds host cell receptors and an S2 domain that fuses the viral and cell membranes to allow cell entry. The S1 domain is the target of many neutralizing antibodies but is more genetically variable than S2, and antibodies can exert selective pressure, leading to resistant variants. Pinto et al . identified five monoclonal antibodies that interact with a helix in the S2 domain. The most broadly neutralizing antibody inhibited all β-coronavirus subgenera and reduced viral burden in hamsters infected with SARS-CoV-2. —VV
59 BASIC BIOLOGICAL SCIENCES↗
Reflections on Cyanobacterial Chromatic Acclimation: Exploring the Molecular Bases of Organismal Acclimation and Motivation for Rethinking the Promotion of Equity in STEM
Cyanobacteria are photosynthetic organisms that exhibit characteristic acclimation and developmental responses to dynamic changes in the external light environment. Photomorphogenesis is the tuning of cellular physiology, development, morphology, and metabolism in response to external light cues. The tuning of photosynthetic pigmentation, carbon fixation capacity, and cellular and filament morphologies to changes in the prevalent wavelengths and abundance of light have been investigated to understand the regulation and fitness implications of different aspects of cyanobacterial photomorphogenesis. Chromatic acclimation (CA) is the most common form of photomorphogenesis that has been explored in cyanobacteria. Multiple types of CA in cyanobacteria have been reported, and insights gained into the regulatory pathways and networks controlling some of these CA types. I examine the recent expansion of CA types that occur in nature and provide an overview of known regulatory factors involved in distinct aspects of cyanobacterial photomorphogenesis. Additionally, I explore lessons for cultivating success in scientific communities that can be drawn from a reflection on existing knowledge of and approaches to studying CA.
59 BASIC BIOLOGICAL SCIENCES↗
Deep tissue profiling of Populus stem at single nucleus level reveals uncharacterized cell types and cell-specific gene regulatory networks
Not provided.
Biotechnology & Applied Microbiology↗
SPRUCE: Shrub Leaf and Stem Functional Traits from 10-year Shrub Layer Biomass Harvests (August 2025)
This data set contains Leaf Mass Area (LMA), Specific Leaf Area (SLA), Leaf Area Index (LAI), and Huber value (Hv) measurements from the 10-year Shrub-layer Biomass harvests in the Spruce and Peatland Responses Under Environmental Change (SPRUCE) experiment in August 2025. The total ground-level cross-sectional sapwood area of Chamaedaphne calyculata (CHCA), Rhododendron groenlandicum (RHGR), and Vaccinium angustifolium (VAAN) were calculated for each of the three shrub-layer community survey plots located in each experimental enclosure. Representative current-year leaves were removed, scanned, dried, and weighed to derive SLA. Grab-samples for VAAN were used to calculate SLA when no biomass was harvested in the shrub-layer community plots. These SLA values were used to infer total one-sided leave surface area from the total species lead dry mass for calculation of LAI and Hv.
Birkebak, Joshua [ORNL] (ORCID:0009000955611494)↗
Grain boundary structure of two-dimensional tellurium revealed by 4D STEM
The recent realization of 2D tellurium (tellurene) has allowed scientists to demonstrate an air-stable monoelemental van der Waals material with remarkable potential for applications in electronics and optoelectronics. The chiral-chain structure of ultrathin Te allows controllable electronic and optical properties due to the non-monotonic carrier mobility and an increase in electronic band-gap as the thickness is reduced. Scalable and accurate production of 2D Te-based functional devices will require detailed knowledge of structural defects and strain field distributions that can be linked to transport properties.
36 MATERIALS SCIENCE↗
Longitudinal Gradients in Tree Stem Greenhouse Gas Concentrations Across Six Pacific Northwest
This report describes one study that was completed as part of the project titled “A critical gap in our ability to quantify and model earth system interactions - Development of a global, mechanistic understanding of methane emissions from trees.”
54 ENVIRONMENTAL SCIENCES↗
Towards durable resistance to Septoria stem canker and leaf spot: A molecular understanding of resistance (Final Technical Report)
To identify, validate, and functionally characterize alleles that confer resistance to Septoria canker and leaf spot in Populus. The proposed research will elucidate a major mechanism of resistance to Sphaerulina musiva, the major limiting factor to plantations in eastern North America. Genome-wide association mapping, CRISPR/Cas9, and protein-protein assays will be used, enabling marker-aided breeding, reducing costs, and accelerating development of resistant varieties.
59 BASIC BIOLOGICAL SCIENCES↗
Record of Treatment for Concrete Preservation Work at TA-6-0037 Concrete Bowl, TA-08 Gun Site, TA-16-0518 Stem Wall, and TA-18 Battleship Bunkers (Historic Buildings Report)
This completion report documents concrete preservation work that occurred in Fiscal Years 2019 and 2020. Work took place at four sites (Technical Areas [TAs] -06, -08, -16, and -18) that hold Manhattan Project–era significance. Seven buildings and structures were included in the project scope, with concentrated assessments and treatment plans accomplished before the start of preservation activities. The attended buildings and structures represent eligible or included Manhattan Project National Historical Park resources. The stabilization of original fabric and the retention of integrity and significance remained paramount throughout all phases of this project.
42 ENGINEERING↗
Measuring Electronic and Structural Transformations in Solar Thermochemical Water Splitting Materials with Aberration-Corrected STEM-EELS.
Abstract not provided.
Trindell, Jamie↗
Where can you go from here? Explore unusual STEM opportunities, Science has No Limits [Slides]
Abstract not provided.
29 ENERGY PLANNING, POLICY, AND ECONOMY↗
Optimizing Sub-Sampled STEM Imaging for Beam Sensitive Materials and Dynamic Processes
The goal of this research is to quantify how sub-sampling and inpainting (broadly classified as methods in Artificial Intelligence) can be used to obtain the highest resolution images under any experimental conditions, and to use this to reproducibly control dynamic in-situ processes in gases and liquids on the nanoscale. As atomic diffusion under non-extreme conditions is typically in the sub-ms time domain, the ability to use this sub-sampling approach to reduce the effect of the electron beam and to speed-up the imaging process represents the optimum combination of spatial and temporal resolution achievable in a conventional microscope. This LDRD funding demonstrated the feasibility of imaging dynamics in complex energy systems using this methodology by establishing the optimum experimental sampling conditions (optimizing the number of pixels, speed, contrast and resolution) for each experiment. For in-situ liquid cell experiments this analysis shows that simply by distributing the same dose and dose rate maximally in space and time, the kinetics for radiolysis products can be modified significantly. The final stage of this work, i.e. the experimental demonstration of its use for nucleation and growth, was severely curtailed by issues with COVID19. However, all the experiments are designed and currently underway, with the goal to complete the final demonstration and publication as soon as safety concerns for laboratory access are met.
36 MATERIALS SCIENCE↗