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At least 415 records · Page 23

Aircraft deployment, and airborne arctic stratospheric expedition

The Airborne Arctic Stratospheric Expedition had two primary objectives: to study the production and loss mechanisms of ozone in the north polar stratosphere and to study the effect on ozone distribution of the Arctic Polar Vortex and of the cold temperatures associated with the formation of Polar Stratospheric Clouds. Two specially instrumented NASA aircraft were flown over the Arctic region. Each aircraft flew to acquire data on the meteorological, chemical and cloud physical phenomena that occur in the polar stratosphere during winter. The chemical processes which occur in the polar stratosphere during winter were also observed and studied. The data acquired are being analyzed.

Condon, Estelle↗

Seasonal variation of atmospheric nitric acid over the South Pole in 1992

We conducted year-around measurements of mid infrared atmospheric emission over the South Pole in 1992. We were able to observe a large seasonal change of the total column of nitric acid (HNO3) vapor. During the summer the HNO3 column abundance was about 2 x 10(exp 16) molecules/sq cm. There was a small increase in the fall. A rapid decrease of 50% was observed in late June, soon after the stratospheric temperature reached the threshold for formation of type I polar stratospheric clouds (PSCs). By early July, the stratospheric temperature was cold enough to form type II PSCs, and the HNO3 column decreased to 7 x 10(exp 15) molecules/sq cm. Measured nitric acid values in the spring remained extremely low even after the stratosphere warmed well above PSC temperatures. This may indicate permanent removal of HNO3 by gravitational settling, or long-term sequestering in large particles. Normal summer values were not observed until the vortex dissipated and allowed the lateral transport of HNO3 to the south polar region.

Allen, Renate Van↗

A Search for Interstellar Oxiranecarbonitrile (C3H3NO)

We report a search in cold, quiescent and in 'hot core' type interstellar molecular clouds for the small cyclic molecule oxiranecarbonitrile (C3H3NO), which has been suggested as a precursor of important prebiotic molecules. We have determined upper limits to the column density and fractional abundance for the observed sources and find that, typically, the fractional abundance by number relative to molecular hydrogen Of C3H3NO is less than a few times 10(exp -10). This limit is one to two orders of magnitude less than the measured abundance of such similarly complex species as CH3CH2CN and HCOOCH3 in well-studied hot cores. A number of astrochemical discoveries were made, including the first detection of the species CH3CH2CN in the massive star-forming clouds G34.3+0.2 and W51M and the first astronomical detections of some eight rotational transitions of CH3CH2CN, CH3CCH, and HCOOCH3. In addition, we found 8 emission lines in the 89 GHz region and 18 in the 102 GHz region which we were unable to assign.

Dicken, J. E.↗

IOCCG Report Number 16, 2015 Ocean Colour Remote Sensing in Polar Seas : The Polar Environment: Sun, Clouds, and Ice - Chapter 2

The polar regions are places of extremes. There are months when the regions are enveloped in unending darkness, and months when they are in continuous daylight. During the daylight months the sun is low on the horizon and often obscured by clouds. In the dark winter months temperatures are brutally cold, and high winds and blowing snow are common. Even in summer, temperatures seldom rise above 0degC. The cold winter temperatures cause the ocean to freeze, forming sea ice. This sea ice cover acts as a barrier limiting the transfer of heat, moisture, and momentum between the atmosphere and the ocean. It also greatly complicates the optical signature of the surface. Taken together, these factors make the polar regions a highly challenging environment for optical remote sensing of the ocean.

ocean colour↗

Long Term Stability Monitoring of Aqua MODIS Thermal Emissive Bands through Radiative Transfer Modeling

Moderate Resolution Imaging Spectroradiometer (MODIS) on Aqua has been in operation providing continuous global observations for science research and applications since 2002. The long-term stability of thermal emissive bands (TEBs) of Aqua MODIS was monitored through inter-comparisons with measurements by hyperspectral infrared sensors, such as AIRS on Aqua and IASI on MetOp satellite, or through long term vicarious monitoring over cold targets, such as Dome- C and deep convective clouds (DCC). In this paper, a radiative transfer modeling-based simulation model using Community Radiative Transfer Model (CRTM) is developed to perform the long-term monitoring of the stability of TEBs of Aqua MODIS. CRTM is a fast-radiative transfer model for calculations of radiances for satellite infrared radiometers and is able to output infrared radiance and brightness temperature at spectral bands of MODIS. Long term European Centre for Medium-Range Weather Forecasts (ECMWF) global atmospheric reanalysis data, such as temperature and humidity profiles, are used as inputs to the CRTM simulation. By confining the area of interest to be over low to middle latitude ocean, the long-term stabilities of selected Aqua MODIS TEBs are monitored through Observation–Background (O-B) brightness temperature (BT) bias between MODIS measurements and BT retrieval from CRTM simulation. The consistency and relative stability between Aqua MODIS and ECMWF reanalysis data for surface channels of MODIS are evaluated. In addition, the radiative transfer modeling with CRTM enables us to evaluate the impacts of long term variation of global CO2 distribution on the O-B BT biases for CO2 channels of Aqua MODIS through comparison of simulations with constant or long term variable CO2 as inputs. The O-B analysis with RTM show that Aqua MODIS surface channels are all radiometrically stable with yearly BT bias drift less than 0.004K/year for B20, B22, B23 and ~0.01K/year for B31 and B32. The CO2 absorption channels of Aqua MODIS, e.g. B33-B36, are stable with BT bias drift < 0.005K/year.

MODIS↗

Large Anomalies in Lower Stratospheric Water Vapor and Ice During the 2015–2016 El Niño

The strong and unusual El Niño of 2015-2016 produced a remarkable perturbation to the hydrologic budget of the tropical tropopause layer (14-19 km). This region regulates stratospheric water vapor, which has a direct radiative impact on surface temperatures. To first order, the coldest tropical tropopause temperature regulates the amount of water vapor entering the stratosphere by controlling the amount of dehydration in the rising air. Here we show that tropical convective cloud ice and associated cirrus evaporating at unusually high altitudes might also have a role in stratospheric hydration. The 2015-2016 El Niño produced decadal record water vapor amounts in the tropical Western Pacific, coincident with warm tropopause temperature anomalies. In the Central Pacific, convective cloud ice was observed 2 km above the anomalously cold tropopause. A trajectory-based dehydration model based on two reanalysis temperature and wind fields can account for only about 0.5-0.6 ppmv of the ~0.9 ppmv tropical lower stratospheric moistening observed during this event. This suggests that unresolved convective dynamics and/or associated sublimation of lofted ice particles also contributed to lower stratospheric moistening. These observations suggest that convective moistening could contribute to future climate change-induced stratospheric water vapor increases.

Atmospheric chemistry↗

Isotopic Signature of Organic Molecules from Beyond the Solar System: An Enriched Methane D/H Ratio in the Interstellar Object 3I/ATLAS

Interstellar objects are interlopers from other planetary systems, and their volatile compositions provide a glimpse into planet formation around their host star. We present near-infrared spectra of the coma of interstellar object 3I/ATLAS measured with the James Webb Space Telescope. Our results demonstrate an unexpectedly high D/H = (3.31 ± 0.34)% for methane and represent an exceedingly rare detection of deuterated organic molecules in an interstellar object. This D/H ratio is a factor of 14 ± 2 higher than that measured in comet 67P/Churyumov-Gerasimenko by the Rosetta spacecraft, the only other comet for which CH3D has been detected, yet the ratio of deuteration in methane compared with water is consistent for both comets within 1.2σ. The D/H ratio in methane is observationally unconstrained in extrasolar sources to date, but the enriched ratio in 3I/ATLAS is most similar to those measured in other organic molecules toward primitive environments. The high D/H ratios of water and methane in 3I/ATLAS are a natural consequence of formation in a high D/H elemental ratio environment as a result of locally cold conditions in the protoplanetary disk and prior interstellar cloud. Thus, 3I/ATLAS formed in an environment very different from that in which our Sun and planets originated.

Interstellar Object 3I/ATLAS↗

Simulations of the Vertical Redistribution of HNO3 by NAT or NAD PSCs: The Sensitivity to the Number of Cloud Particles Formed and the Cloud Lifetime

Recent satellite and in situ measurements have indicated that limited denitrification can occur in the Arctic stratosphere. In situ measurements from the SOLVE campaign indicate polar stratospheric clouds (PSCs) composed of small numbers (about 3 x 10^ -4 cm^-3) of 10-20 micron particles (probably NAT or NAD). These observations raise the issue of whether low number density NAT PSCs can substantially denitrify the air with reasonable cloud lifetimes. In this study, we use a one dimensional cloud model to investigate the verticle redistribution of HNO3 by NAT/NAD PSCs. The cloud formation is driven by a temperature oscillation which drops the temperature below the NAT/NAD formation threshold (about 195 K) for a few days. We assume that a small fraction of the available aerosols act as NAT nuclei when the saturation ratio of HNO3 over NAT(NAD) exceeds 10(l.5). The result is a cloud between about 16 and 20 km in the model, with NAT/NAD particle effective radii as large as about 10 microns (in agreement with the SOLVE data). We find that for typical cloud lifetimes of 2-3 days or less, the net depletion of HNO3 is no more than 1-2 ppbv, regardless of the NAT or NAD particle number density. Repeated passes of the air column through the cold pool build up the denitrification to 3-4 ppbv, and the cloud altitude steadily decreases due to the downward transport of nitric acid. Increasing the cloud lifetime results in considerably more effective denitrification, even with very low cloud particle number densities. As expected, the degree of denitrification by NAT clouds is much larger than that by NAD Clouds. Significant denitrification by NAD Clouds is only possible if the cloud lifetime is several days or more. The clouds also cause a local maximum HNO3 mixing ratio at cloud base where the cloud particles sublimate.

Jensen, Eric J.↗

Using Satellite Observations to Infer the Relationship Between Cold Pools and Subsequent Convection Development

Cold pools are increasingly being recognized as important players in the evolution of both shallow and deep convection; hence, the incorporation of cold pool processes into a number of recently developed convective parameterizations. Unfortunately, observations serving to inform cold pool parameterization development are limited to select field programs and limited radar domains. However, a number of recent studies have noted that cold pools are often associated with arcs-lines of shallow clouds traversing 10 100 km in visible satellite imagery. Boundary layer thermodynamic perturbations are plausible at such scales, coincident with such mesoscale features. Atmospheric signatures of features at these spatial scales are potentially observable from satellites. In this presentation, we discuss recent work that uses multi-sensor, high-resolution satellite products for observing mesoscale wind vector fluctuations and boundary layer temperature depressions attributed to cold pools produced by antecedent convection. The relationship to subsequent convection as well as convective system longevity is discussed. As improvements in satellite technology occur and efforts to reduce noise in high-resolution orbital products progress, satellite pixel level (10 km) thermodynamic and dynamic (e.g. mesoscale convergence) parameters can increasingly serve as useful benchmarks for constraining convective parameterization development, including for regimes where organized convection contributes substantially to the cloud and rainfall climatology.

thermodynamics↗

MARCI-observed clouds in the Hellas Basin during northern hemisphere summer on Mars: Interpretation with the NASA/Ames Legacy Mars Global Climate Model

We present a study that is motivated by a population of water ice clouds in the Hellas Basin that has been observed by the MARs Color Imager (MARCI) instrument on the Mars Reconnaissance Orbiter (MRO) to persist throughout the majority of Northern Hemisphere (NH) summer. Although water ice clouds are present in Hellas at very low opacities throughout NH spring, they noticeably thicken after L(sub s) 60° and continue to do so until their peak optical thickness is attained at L(sub s) ~120°. They dissipate rapidly from L(sub s) 120° to 150°, and by L(sub s) 150°, the only clouds in Hellas are on the southern side of the basin and are indistinguishable from the polar hood clouds. We use the NASA/Ames Legacy Mars Global Climate Model (GCM), which is supported by the Agency’s Mars Climate Modeling Center, to investigate the dynamical and microphysical mechanisms that control the formation and evolution of Hellas water ice clouds. We show that water is transported from the North Polar Residual Cap (NPRC) southward across the equator and into the Hellas region. Water vapor is confined down low by cloud formation in the aphelion cloud belt, thus limiting the effectiveness of transport by the zonal mean overturning circulation (i.e., the Hadley cell). Thus, contrary to the commonly held conceptual understanding that the Hadley cell controls cross-equatorial water transport during this season, we show that the southward transport of water is done primarily in the vapor phase by stationary eddies at nearly all latitudes, including across the equator. Clouds form near the surface in the basin as moist air mixes with cold polar air on the western side of Hellas and are subsequently transported clockwise around the north side of the basin by the low-level cyclonic circulation. The simulated Hellas clouds have small particle sizes (~3–5 μm), are very low, and exist as long as the NPRC is exposed.

M. A. Kahre↗

Automated Tracking of Shallow Maritime Clouds on Geostationary Imagery to Extract Lifecycle Characteristics

Shallow moist convection is ubiquitous throughout the tropics and represents a key player in boundary layer processes. Satellites have provided valuable insight on shallow clouds, such as size, structure, and geographical coverage, from static views of recurring cloud fields. But determining why certain cloud features appear and persist for different periods requires a time-evolving view of their behaviors. Geostationary satellites provide a unique opportunity to follow the time evolution of individual convective features, given their enhanced spatial and temporal sampling. A cloud-tracking tool was developed to identify properties of cloud lifecycle from the NASA Cloud, Aerosol, and Monsoon Processes Philippines Experiment (CAMP2EX) field campaign of 2019. The mission conducted intensive sampling of shallow cumulus in the West Pacific Ocean, in tandem with Rapid Scan imagery from the Advanced Himawari Imager (AHI) on the Japan Meteorological Agency’s (JMA) Himawari-8 satellite. Shallow cumulus were segmented according to thresholds in 0.5-km visible reflectance and with blurring techniques. Despite being limited to daytime hours, the segmentations yielded the best resolution available for capturing cloud initiation, growth, and decay. The tracking procedure is based on a computer vision package that includes Kalman filters for motion prediction, object overlap search, and the Hungarian (or Kuhn-Munkres) matching algorithm for track designation. AHI radiances available within the tracked cloud boundaries are assembled to form individual spectral histories. The resulting catalog provides thousands of cloud histories for domains measuring only a few degrees in latitude and longitude. We present an overview of the cloud-tracking tool and its results for cloud fields sampled throughout CAMP2EX by the airborne P-3. Cloud tracks were selected from about 10 flights to form ensembles, specific groups of tracks occurring in a region with airborne sampling. Cloud lifecycle properties, including duration and maximum area, are calculated for all ensemble members, and analyzed for cloud behavior and P-3 coincidences. By following this strategy, we quantitatively assess the degree of airborne sampling for specific cloud classes defined by the lifecycle calculations. We can summarize which cloud classes had more sampling, the stage of development during sampling, and general differences in character (e.g., isolated congestus vs. cold-pool producer).

Cloud Tracking↗

On the Global Character of Overlap Between Low and High Clouds

The global character of overlap between low and high clouds is examined using active satellite sensors. Low-cloud fraction has a strong land-ocean contrast with oceanic values double those over land. Major low-cloud regimes include not only the eastern ocean boundary stratocumulus and shallow cumulus but also those associated with cold air outbreaks downwind of wintertime continents and land stratus over particular geographic areas. Globally, about 30% of low clouds are overlapped by high clouds. The overlap rate exhibits strong spatial variability ranging from higher than 90% in the tropics to less than 5% in subsidence areas and is anticorrelated with subsidence rate and low-cloud fraction. The zonal mean of vertical separation between cloud layers is never smaller than 5 km and its zonal variation closely follows that of tropopause height, implying a tight connection with tropopause dynamics. Possible impacts of cloud overlap on low clouds are discussed.

cloud overlap↗

Condensed-Phase Nitric Acid in a Tropical Subvisible Cirrus Cloud

In situ observations in a tropical subvisible cirrus cloud during the Costa Rica Aura Validation Experiment on 2 February 2006 show the presence of condensed-phase nitric acid. The cloud was observed near the tropopause at altitudes of 16.3-17.7 km in an extremely cold (183-191 K) and dry 5 ppm H2O) air mass. Relative humidities with respect to ice ranged from 150-250% throughout most of the cloud. Optical particle measurements indicate the presence of ice crystals as large as 90 microns in diameter. Condensed RN031H20 molar ratios observed in the cloud particles were 1-2 orders of magnitude greater than ratios observed previously in cirrus clouds at similar RN03 partial pressures. Nitric acid trihydrate saturation ratios were 10 or greater during much of the cloud encounter, indicating that RN03 may be present in the cloud particles as a stable condensate and not simply physically adsorbed on or trapped in the particles.

Popp, P. J.↗

Dehydration of the Upper Troposphere and Lower Stratosphere by Subvisible Cirrus Clouds Near the Tropical Tropopause

The extreme dryness of the lower stratosphere is believed to be caused by freeze-drying of air as it enters the stratosphere through the cold tropical tropopause. Previous investigations have been focused on dehydration occurring at the tops of deep convective cloud systems, However, recent observations of a ubiquitous stratiform cirrus cloud layer near the tropical tropopause suggest the possibility of dehydration as air is slowly lifted by large-scale motions, In this study, we have evaluated this possibility using a detailed ice cloud model. Simulations of ice cloud formation in the temperature minima of gravity waves (wave periods of 1 - 2 hours) indicate that large numbers of ice crystals will likely form due to the low temperatures and rapid cooling. As a result, the crystals do not grow larger than about 10 microns, fallspeeds are no greater than a few cm/s, and little or no precipitation or dehydration occurs. However, ice cloud's formed by large-scale vertical motions (with lifetimes of a day or more) should have,fever crystals and more time for crystal sedimentation to occur, resulting in water vapor depletions as large as 1 ppmv near the tropopause. We suggest that gradual lifting near the tropical tropopause, accompanied by formation of thin cirrus, may account for the dehydration.

Jensen, Eric J.↗

A comprehensive model of ion diffusion and charge exchange in the cold Io torus

A comprehensive analytic model of radial diffusion in the cold Io torus is developed. The model involves a generalized molecular cloud theory of SO2 and its dissociation fragments SO, O2, S, and O, which are formed at a relatively large rate by solar UV photodissociation of SO2. The key component of the new theory is SO, which can react with S(+) through a near-resonant charge exchange process that is exothermic. This provides a mechanism for the rapid depletion of singly ionized sulfur in the cold torus and can account for the large decrease in the total flux tube content inward of Io's orbit. The model is used to demonstrate quantitatively the effects of radial diffusion in a charge exchange environment that acts as a combined source and sink for ions in various charge states. A detailed quantitative explanation for the O(2+) component of the cold torus is given, and insight is derived into the workings of the so-called plasma 'ribbon'.

Barbosa, D. D.↗

Convective Influence on the Humidity and Clouds in the Tropical Tropopause Layer During Boreal Summer

The impact of convection on the humidity and clouds in the tropical tropopause layer (TTL) during boreal summer 2007 is investigated in simulations of detailed cloud microphysical processes and their effects on the water vapor (H2O) profile along backward trajectories from the 379 K potential temperature (100‐hPa pressure) surface. Convective influence is determined by tracing the trajectories through time‐dependent fields of satellite‐based convective cloud top height. The simulated H2O mixing ratios at the 100‐hPa level and cloud occurrence fractions in the middle to upper (16–18 km) TTL exhibit a pronounced maximum over the Asian monsoon region as in observations; these local enhancements are virtually absent in the simulation without convection, indicating that convection is the dominant driver of the localized H2O and cloud maxima in the Asian summer monsoon region. Convection moistens the 100‐hPa level by 0.6 ppmv (~15%) averaged over the 10°S–50°N domain and increases tropical (10°S–30°N) mean cloud occurrence in the middle to upper TTL by ~170%. Nearly all of the convective enhancements in H2O and clouds are due to the effect of convective saturation; convectively detrained ice crystals have negligible impact. Parcels are most frequently hydrated by deep convection in the southern sector of the Asian monsoon anticyclone and subsequently dehydrated downstream of convection to the west, shifting the locations of final dehydration northwest of the cold temperature region in the northern Tropics. Infrequent, extreme deep convective systems (cloud tops exceeding 380 K) have a disproportionately large effect on TTL humidity and clouds.

Humidity↗

Precipitation -17 O-Excess Altered During Tropical Convection: Evidence From Monsoon Cold Surges in Singapore

Despite the recent recognition of -17 O-excess as a promising new tracer for hydrological processes, our knowledge of the control mechanisms underlying -17 O-excess in tropical regions remains limited. To understand how microphysical processes during tropical convection affect precipitation isotope ratios, particularly -17 O-excess, in Singapore, we collected precipitation samples at minute intervals from six rain events associated with cold surges during the Northeast Monsoon seasons and analyzed their triple oxygen isotopes. Our results show that precipitation δ -18 O decreases in the convective zones and then gradually increases in the stratiform zones, while d-excess exhibits an inverse trend. This correlation between δ -18 O and d-excess indicates that rain evaporation plays a crucial role in regulating precipitation isotopes. Moreover, the rain events with a higher upstream rainout amount have lower δ -18 O and higher -17 O-excess values, suggesting that precipitation δ -18 O and -17 O-excess likely reflect the integrated upstream convective activity. Microphysical processes associated with upstream convection, such as rain evaporation and vapor recycling, are potential mechanisms that increase -17 O-excess values along moisture transport pathways for a rain event, and hence, undermine the effectiveness of -17 O-excess as a tracer of moisture source humidity. Contrary to the negative correlation observed in monthly precipitation, there is generally a positive correlation between d-excess and -17 O-excess at the event scale. However, this correlation weakens as convective rain intensifies, suggesting that stronger convection can attenuate the positive correlation between d-excess and -17 O-excess. Therefore, it is crucial to consider how tropical convection alters -17 O-excess when utilizing this tracer to interpret atmospheric dynamics and hydrological processes.

tropical weather systems↗

A Method for Obtaining High Frequency, Global, IR-Based Convective Cloud Tops for Studies of the TTL

Models of varying complexity that simulate water vapor and clouds in the Tropical Tropopause Layer (TTL) show that including convection directly is essential to properly simulating the water vapor and cloud distribution. In boreal winter, for example, simulations without convection yield a water vapor distribution that is too uniform with longitude, as well as minimal cloud distributions. Two things are important for convective simulations. First, it is important to get the convective cloud top potential temperature correctly, since unrealistically high values (reaching above the cold point tropopause too frequently) will cause excessive hydration of the stratosphere. Second, one must capture the time variation as well, since hydration by convection depends on the local relative humidity (temperature), which has substantial variation on synoptic time scales in the TTL. This paper describes a method for obtaining high frequency (3-hourly) global convective cloud top distributions which can be used in trajectory models. The method uses rainfall thresholds, standard IR brightness temperatures, meteorological temperature analyses, and physically realistic and documented corrections IR brightness temperature corrections to derive cloud top altitudes and potential temperatures. The cloud top altitudes compare well with combined CLOUDSAT and CALIPSO data, both in time-averaged overall vertical and horizontal distributions and in individual cases (correlations of .65-.7). An important finding is that there is significant uncertainty (nearly .5 km) in evaluating the statistical distribution of convective cloud tops even using lidar. Deep convection whose tops are in regions of high relative humidity (such as much of the TTL), will cause clouds to form above the actual convection. It is often difficult to distinguish these clouds from the actual convective cloud due to the uncertainties of evaluating ice water content from lidar measurements. Comparison with models show that calculated cloud top altitudes are generally higher than those calculated by global analyses (e.g., MERRA). Interannual variability in the distribution of convective cloud top altitudes is also investigated.

hydration↗