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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Grassy ELM regime at low pedestal collisionality in high-power tokamak plasma

Spontaneous mitigation of giant ELMs and appearance of grassy ELMs have been observed repeatedly at low pedestal collisionality (${\nu }_{\mathrm{e},\mathrm{p}\mathrm{e}\mathrm{d}}^{{\ast}}\sim 0.15$) in the high-power (P inj > 13 MW) hybrid scenario in DIII-D. Higher β p and higher q 95 appear to be beneficial to achieving the grassy ELM regime. The grassy ELM H-mode plasma shows high energy confinement performance (H 98y2 up to over 1.5) under the conditions of high neutral beam torque and high core rotation. The pedestal width appears to exceed the EPED1.0 model prediction by more than 50%. Pedestal stability analysis performed with the ELITE code indicates that the stability against low-n kink/peeling modes is improved with increased auxiliary heating power and the operational point in the grassy ELM regime is located near the ballooning boundary. The pedestal stability characteristics during the grassy ELM crashes have been investigated in comparison with the giant ELM crashes based on plasma profiles experimentally measured with high resolution and accuracy. It has been found that the underlying mechanism for the observed small-amplitude ELM crashes is mainly the expansion of the ballooning stability boundary induced by an initial radially localized collapse in the pedestal, which helps to stop the growth of instabilities and further collapse of the pedestal. The effect of electron density pedestal on mitigating edge localized instabilities has been analyzed by numerical simulation, suggesting that the electron density pedestal characterized by high n e,sep /n e,ped and low density gradient helps to stabilize peeling-ballooning modes because of a low pressure pedestal gradient and to lower the ballooning boundary mainly because of a low ion diamagnetic frequency in the pedestal region, thus triggering ballooning instabilities and producing the intrinsic grassy ELMs. Numerical simulation of the Chinese fusion engineering test reactor (CFETR) with the SOLPS code indicates that the separatrix density might be insensitive to the electron diffusivity in the pedestal region and increase with the power flowing from the core region to the edge region. Furthermore, pedestal stability analysis suggests that the flat density pedestal with high separatrix density obtained in the high-power plasma in CFETR would make the operational point close to the ballooning boundary, which is considered to help destabilize ballooning instabilities and facilitate the access to the grassy ELM regime.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Diagnostic x-ray source using electrons produced by a 100 J-class picosecond laser

Many laser-based high-energy-density science (HEDS) facilities have one or more short-pulse (sub- to few-picosecond) laser beams for diagnostics. For the past decade, we have been developing a novel x-ray probing capability using such picosecond lasers interacting with an underdense plasma to produce relativistic electrons. The ultimate goal of these experiments is to demonstrate a new type of x-ray backlighter using the short-pulse ARC laser at the National Ignition Facility (NIF). Before this diagnostic is fielded at the NIF, it is critical to demonstrate the viability and reproducibility of the x-ray source on comparable high-power short-pulse laser systems. We present experiments that were carried out with the OMEGA EP laser at the University of Rochester’s laboratory for laser energetics. In these experiments, high-energy electrons are produced through a combination of the self-modulation instability and direct laser acceleration in an underdense gas jet. These electrons generate directional x-rays with characteristic energies up to several tens of keV as they execute betatron motion in the ion channel, and the inverse Compton scattering process generates even harder x-rays, with characteristic photon energies of 60–240 keV. When implemented on the OMEGA EP laser(s), this x-ray source yields results that are comparable to those obtained recently on the short-pulse Titan laser at the Jupiter Laser Facility at Lawrence Livermore National Laboratory, after accounting for differences in laser energy, peak intensity, focusing f/#, and plasma source. Applications of such an x-ray source for HEDS experiments are discussed.

backlighter↗
DOE OSTI2025

On the role of ion temperature gradient turbulence in driving ion thermal transport in neutral beam injection-heated L-mode plasmas in a superconducting tokamak

In this paper, we report a detailed experimental study of the role of ion-temperature-gradient driven turbulence in driving ion thermal transport in neutral beam injection (NBI)-heated L-mode plasmas in Experimental Advanced Superconducting Tokamak (EAST) (Wan et al 2000 Nucl. Fusion 40 1057) coupled with linear and nonlinear gyrokinetic simulations. Significant ion-scale turbulence k ⟂ < cm −1 (k ⟂ < 1.5, where k ⟂ where is the perpendicular wavenumber and ρ s is the ion gyroradius calculated using local electron temperature T e ), measured with a microwave reflectometer, is observed in the plasma core at for r/a ≈ 0.265 and 0.5 (where r is half the diameter of the closed flux surface at a given radial position, and a is half the diameter of the last closed flux surface). Local linear stability analysis with experimental equilibrium quantities at these two radial locations using the GS2 gyrokinetic code shows that the most unstable ion-scale micro-instability is the ion temperature gradient (ITG) mode. Since the computed maximum ion-scale linear growth rates are larger than the local Waltz-Miller E × B shearing rate (Waltz and Miller 1999 Phys. Plasmas 6 4265), the E × B shear is unable to suppress ion-scale turbulence, consistent with the experimental observation of ion-scale turbulence. Experimental ion and electron thermal transports, calculated with power balance analysis, are both anomalous with ion thermal transport being the dominant channel. Nonlinear gyrokinetic simulations using the electrostatic global particle-in-cell gyrokinetic tokamak simulation (GTS) code (Weixing Wang et al 2010 Phys. Plasmas 17 072511) show good quantitative agreement between predicted ion thermal transport and that from the power balance analysis. These results demonstrate for the first time the important role of ITG turbulence in driving thermal transport in NBI-heated L-mode plasmas in EAST, showing the effectiveness of GTS code in simulating electrostatic turbulence in EAST and the need of suppressing ITG turbulence to improve energy confinement in EAST.

Sun, P. J. [Chinese Academy of Sciences (CAS), Hef↗
DOE OSTI2021

Nanoscale dynamics during self-organized ion beam patterning of Si. II. Kr + bombardment

Understanding the self-organized ion beam nanopatterning of elemental semiconductors, particularly silicon, is of intrinsic scientific and technological interest. This is the second component of a two-part coherent x-ray scattering and x-ray photon correlation spectroscopy (XPCS) investigation of the kinetics and fluctuation dynamics of nanoscale ripple development on silicon during 1 keV Ar + (part I) and Kr + bombardment at 65° polar angle. Here it is found that the ion-enhanced viscous flow relaxation is essentially equal for Kr + -induced patterning as previously found for Ar + patterning despite the difference in ion masses. However, the magnitude of the surface curvature-dependent roughening rate in the early-stage kinetics is larger for Kr + than for Ar + , consistent with expectations that the heavier ion gives an increased mass redistributive contribution to the initial surface instability. As with the Ar + case, fluctuation dynamics in the late stage show a peak in correlation times at the length scale corresponding to the dominant structural feature on the surface—the ripples. Finally, it is shown that speckle motion during the surface evolution can be analyzed to determine spatial inhomogeneities in erosion rate and ripple velocity. This allows the direction and speed of ripple motion to be measured in a real time experiment. In the present case, ripple motion is found to be into the projected direction of the ion source, in contrast to expectations from an existing sputter erosion driven model with parameters derived from binary collision approximation simulations.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Pathways towards break even for low convergence ratio direct-drive inertial confinement fusion

Following indirect-drive experiments which demonstrated promising performance for low convergence ratios (below 17), previous direct-drive simulations identified a fusion-relevant regime which is expected to be robust to hydrodynamic instability growth. This paper expands these results with simulated implosions at lower energies of 100 and 270 kJ, and ‘hydrodynamic equivalent’ capsules which demonstrate comparable convergence ratio, implosion velocity and in-flight aspect ratio without the need for cryogenic cooling, which would allow the assumptions of one-dimensional-like performance to be tested on current facilities. A range of techniques to improve performance within this regime are then investigated, including the use of two-colour and deep ultraviolet laser pulses. Finally, further simulations demonstrate that the deposition of electron energy into the hotspot of a low convergence ratio implosion through auxiliary heating also leads to significant increases in yield. Results include break even for 1.1 MJ of total energy input (including an estimated 370 kJ of short-pulse laser energy to produce electron beams for the auxiliary heating), but are found to be highly dependent upon the efficiency with which electron beams can be created and transported to the hotspot to drive the heating mechanism.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Response of thermal and fast-ion transport to beam ion population, rotation and T e / T i in the DIII-D steady state hybrid scenario

The thermal and fast-ion transport properties of DIII-D steady-state hybrid discharges with normalized beta β N ≳ 3 are studied at low injected torque and an increased electron to ion temperature ratio T e / T i . Linear stability analysis performed with the TGLF turbulent code indicates that a high-k mode is usually dominant at smaller radii, whereas a low-k mode is usually dominant at larger radii in these plasmas. A reduction in the net injected torque from 8.6 to 4.3 N-m leads to reduced E × B shear and hence, an enhanced turbulence that was observed on the Doppler backscattering diagnostic and was also computed with TGLF. As T e / T i in the core was increased from 0.57 to 0.66 by adding electron cyclotron current drive (ECCD) to these plasmas, higher levels of transport are observed with increased high-k modes indicated by TGLF. The fast-ion transport level varied over an order of magnitude in these discharges depending on whether Alfvén eigenmodes, fishbones, or no instabilities were observed. Hybrid plasmas with fishbones have decreased fast-ion transport, compared to plasmas with Alfvén eigenmodes, since they are resonant with a smaller portion of phase space and their resonance is farther from the wall. This reduction in fast-ion transport with ECCD mitigates the increase in turbulent transport, resulting in higher performance than expected during strong electron heating. Similarly, the lowest fast-ion transport was observed in the low torque plasma, which also led to better than expected performance at this torque value. Finally, the thermal and fast-ion transport changes observed as the torque/rotation and T e / T i are varied indicate possible methods for transferring this scenario to a reactor.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Verification of neoclassical toroidal viscosity induced by energetic particles

The thermal particles contributed neoclassical toroidal viscosity (NTV) have been successfully developed and explored by many impressive works such as the study by Shaing et al. [Phys. Plasmas 10, 1443 (2003)] and Zhu et al. [Phys. Rev. Lett. 96, 225002 (2006)]. In this work, the scope of the NTV study is extended to explore the contribution of energetic particles (EPs) through both theory and experiments. In theory, the existence of the NTV torque due to the precessional drift resonance of trapped EPs is identified based on the equivalence between the NTV torque and the perturbed drift kinetic energy [J. Park, Phys. Plasmas 18, 110702 (2011)]. Toroidal modeling with the Magneto Resistive Spectrum - drift Kinetic code [Y. Liu, Phys. Plasmas 15, 112503 (2008)], based on this equivalence, indicates that trapped EPs can contribute a significant amount of the NTV torque. Meanwhile, this work also focuses on developing the dedicated DIII-D experiments in the presence of the n = 2 external magnetic perturbation to verify the EP induced NTV (EP-NTV) by measuring the change of the NTV torque while varying the angle and the voltage of the neutral beam injection. However, the developed experiments have been unable to create conditions necessary to clearly demonstrate the presence of EP-NTV. The main challenge is separating the resonant and non-resonant momentum transport responses in the plasma. Finally, the experience, gained from this study, can help the further exploration of EP-NTV in the future experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Sensitivity of the dynamic-shell target to laser drive nonuniformities

The dynamic-shell concept for inertial confinement fusion (ICF) uses an initially homogeneous target and a carefully shaped laser pulse to form a shell and implode it. The laser pulse consists of a series of pickets that drive shocks into the target. The first few shocks converge inwards and rebound from the center of the target, creating an expanding, low-density plasma. Subsequent shocks are launched into the expanding plasma and eventually coalesce to form a shell, which is then imploded with a traditional ICF laser pulse. This study describes radiation-hydrodynamic simulations that investigate the sensitivity of dynamic-shell targets to imperfections in the laser drive. A one-dimensional (1D) study looks at mistiming and power variations in the pickets and a two-dimensional (2D) study examines irradiation perturbations imposed by the laser-beam geometry. Simulations show that less than ~2% power imbalance or 200 ps timing variation in the pickets is sufficient to keep the yield above 90% of the maximum. Additionally, the 2D simulations show that 72 or more beams are required to keep irradiation nonuniformities low enough to obtain fusion yields close to that of 1D simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Review of Multifunctional Separators: Stabilizing the Cathode and the Anode for Alkali (Li, Na, and K) Metal–Sulfur and Selenium Batteries

Alkali metal batteries based on lithium, sodium, and potassium anodes and sulfur-based cathodes are regarded as key for next-generation energy storage due to their high theoretical energy and potential cost effectiveness. However, metal–sulfur batteries remain challenged by several factors, including polysulfides’ (PSs) dissolution, sluggish sulfur redox kinetics at the cathode, and metallic dendrite growth at the anode. Functional separators and interlayers are an innovative approach to remedying these drawbacks. Here we critically review the state-of-the-art in separators/interlayers for cathode and anode protection, covering the Li–S and the emerging Na–S and K–S systems. The approaches for improving electrochemical performance may be categorized as one or a combination of the following: Immobilization of polysulfides (cathode); catalyzing sulfur redox kinetics (cathode); introduction of protective layers to serve as an artificial solid electrolyte interphase (SEI) (anode); and combined improvement in electrolyte wetting and homogenization of ion flux (anode and cathode). It is demonstrated that while the advances in Li–S are relatively mature, less progress has been made with Na–S and K–S due to the more challenging redox chemistry at the cathode and increased electrochemical instability at the anode. Throughout these sections there is a complementary discussion of functional separators for emerging alkali metal systems based on metal–selenium and the metal–selenium sulfide. The focus then shifts to interlayers and artificial SEI/cathode electrolyte interphase (CEI) layers employed to stabilize solid-state electrolytes (SSEs) in metal–sulfur solid-state batteries (SSBs). The discussion of SSEs focuses on inorganic electrolytes based on Li- and Na-based oxides and sulfides but also touches on some hybrid systems with an inorganic matrix and a minority polymer phase. The review then moves to practical considerations for functional separators, including scaleup issues and Li–S technoeconomics. The review concludes with an outlook section, where we discuss emerging mechanics, spectroscopy, and advanced electron microscopy (e.g. cryo-transmission electron microscopy (cryo-TEM) and cryo-focused ion beam (cryo-FIB))-based approaches for analysis of functional separator structure–battery electrochemical performance interrelations. Finally, throughout the review we identify the outstanding open scientific and technological questions while providing recommendations for future research topics.

25 ENERGY STORAGE↗
DOE OSTI2021

Effects of Applied Interfacial Pressure on Li-Metal Cycling Performance and Morphology in 4 M LiFSI in DME

Lithium-metal anodes can theoretically enable 10x higher gravimetric capacity than conventional graphite anodes. However, Li-metal anode cycling has proven difficult due to porous and dendritic morphologies, extensive parasitic solid electrolyte interphase reactions, and formation of dead Li. We systematically investigate the effects of applied interfacial pressure on Li-metal anode cycling performance and morphology in the recently developed and highly efficient 4 M lithium bis(fluorosulfonyl)imide in 1,2-dimethoxyethane electrolyte. We present cycling, morphology, and impedance data at a current density of 0.5 mA/cm 2 and a capacity of 2 mAh/cm 2 at applied interfacial pressures of 0, 0.01, 0.1, 1, and 10 MPa. Cryo-focused ion beam milling and cryo-scanning electron microscopy imaging in cross section reveal that increasing the applied pressure during Li deposition from 0 to 10 MPa leads to greater than a fivefold reduction in thickness (and therefore volume) of the deposited Li. This suggests that pressure during cycling can have a profound impact on the practical volumetric energy density for Li-metal anodes. A “goldilocks zone” of cell performance is observed at intermediate pressures of 0.1–1 MPa. Increasing pressure from 0 to 1 MPa generally improves cell-to-cell reproducibility, cycling stability, and Coulombic efficiency. However, the highest pressure (10 MPa) results in high cell overpotential and evidence of soft short circuits, which likely result from transport limitations associated with increased pressure causing local pore closure in the separator. All cells exhibit at least some signs of cycling instability after 50 cycles when cycled to 2 mAh/cm 2 with thin 50 μm Li counter electrodes, though instability decreases with increasing pressure. In contrast, cells cycled to only 1 mAh/cm 2 perform well for 50 cycles, indicating that capacity plays an important role in cycling stability.

25 ENERGY STORAGE↗
DOE OSTI2023

Improving charge transport in integrated MoO 3 /C electrode materials for water-in-salt energy storage systems by incorporating oxygen vacancies

Improvements in the charge storage properties of α-MoO 3 used as an electrode with a 30m ZnCl 2 water-in-salt electrolyte have been achieved by enhancements in electron and ion transport enabled by an inventive synthesis route. Electron transport was improved through the integration of MoO 3 with dopamine-derived carbon via a chemical preintercalation route, and enhanced ion transport was achieved by incorporating oxygen vacancies in MoO 3 structure through ethanol 2 reduction under hydrothermal conditions. Here, the presence of carbon was confirmed by corresponding D and G bands observed in Raman spectroscopy measurements. The presence of oxygen vacancies was proven through correlated XPS, TGA, Raman spectroscopy and XRD analyses, with the introduction of oxygen vacancies leading to an expanded interlayer region. Four-point probe measurements provided evidence of increased electronic conductivity due to the incorporation of carbon, and cyclic voltammetry-based charge storage mechanism analyses revealed increases in ion transport kinetics due to oxygen vacancy formation. Tuning the oxygen vacancy concentration is critical, as excessive concentrations of these point defects leads to structural instability and poor capacity retention. This work demonstrates the combined potential of carbon and oxygen vacancies in moderate concentrations to enhance the charge storage properties of transition metal oxides. The strategies developed in this study offer a path to the development of promising materials for high-rate, high-capacity, and long-duration electrochemical energy storage technologies.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2022

Diagnostics for multiple frequency heating and investigation of underlying processes

The development of new facilities routinely challenges ion source designers to build and operate sources that can achieve ever higher beam intensities and energies. As shown in this work, electron cyclotron resonance ion sources have proven to be extremely capable in meeting these challenges through the production of intense beams of medium and high-charge state ions. As performance boundaries are pushed, source stability becomes an issue as does the technology required to meet the challenge. Multiple frequency heating, the simultaneous use of two or more plasma heating frequencies, is a powerful tool in meeting the simultaneous need of intensity and stability. Relatively straightforward to utilize, the technique has been employed at numerous facilities to increase beam current and achievable charge state while also stabilizing the plasma. Its application has expanded the operational boundaries of existing and next generation sources, demonstrating that these devices have not yet achieved their full operational potential. To better understand the underlying physics, the diagnostics used to probe the source operational boundaries and the plasma properties have become increasingly sophisticated. In concert with detailed modeling, they are beginning to provide insight into the heating mechanism and, with that, the prospect of future advances.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

Validation of the EDGES Low-band Antenna Beam Model

The response of the antenna is a source of uncertainty in measurements with the Experiment to Detect the Global Epoch of Reionization Signature (EDGES). We aim to validate the electromagnetic beam model of the low-band (50–100 MHz) dipole antenna with comparisons between models and against data. We find that simulations of a simplified model of the antenna over an infinite perfectly conducting ground plane are, with one exception, robust to changes in the numerical electromagnetic solver code or algorithm. For simulations of the antenna with the actual finite ground plane and realistic soil properties, we find that two out of three numerical solvers agree well. Applying our analysis pipeline to a simulated drift-scan observation from an early EDGES low-band instrument that had a 10 m × 10 m ground plane, we find residual levels after fitting and removing a five-term foreground model from the simulated data binned in local sidereal time (LST) average about 250 mK with ±40 mK variation between numerical solvers. A similar analysis of the primary 30 m × 30 m sawtooth ground plane reduced the LST-averaged residuals to about 90 mK with ±10 mK between the two viable solvers. More broadly we show that larger ground planes generally perform better than smaller ground planes. Simulated data have a power that is within 4% of real observations, a limitation of net accuracy of the sky and beam models. We observe that residual spectral structures after foreground model fits match qualitatively between simulated data and observations, suggesting that the frequency dependence of the beam is reasonably represented by the models. We find that a soil conductivity of 0.02 S m{sup -1} and relative permittivity of 3.5 yield good agreement between simulated spectra and observations. This is consistent with the soil properties reported by Sutinjo et al. for the Murchison Radio-astronomy Observatory, where EDGES is located.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Controlling the symmetry of cadmium arsenide films by epitaxial strain

Epitaxial strains offer unique opportunities to obtain topological states in thin films and heterostructures that do not exist in their bulk counterparts. Here, we investigate the point group symmetries of coherently strained films of cadmium arsenide (Cd 3 As 2 ), a prototype three-dimensional Dirac semimetal, by convergent beam electron diffraction. We report a loss of the fourfold rotational axis and adoption of the orthorhombic mmm point group in (112)-oriented films under biaxial compressive stress. (001)-oriented Cd 3 As 2 films that are under a small biaxial tensile stress retain the fourfold rotational symmetry that protects the bulk nodes but adopt the non-centrosymmetric 4mm point group symmetry. This, in turn, suggests that (001) films adopt a different crystal structure in biaxial tension, one that differs in the arrangement of the ordered Cd vacancies that are an inherent feature of the crystal structure of Cd 3 As 2 and that are key to its nodal electronic structure. Density functional theory calculations confirm the experimental findings of the stability of the non-centrosymmetric structure under biaxial tension, whereas the centrosymmetric structure is stable under biaxial compression. The results show that bulk Cd 3 As 2 is already close to structural instability and showcase the extraordinary tunability of the topological states of Cd 3 As 2 .

36 MATERIALS SCIENCE↗
DOE OSTI2021

EBSD of Rough Native CuInGaSe2 Thin-Films

The polycrystalline Cu (In, Ga) Se2, or CIGS, based thin-film materials system has long been studied for use in photovoltaic technologies, where its bandgap tunability, mechanical flexibility, and relatively low production costs are all appealing. Nonetheless, significant defect populations, which serve to reduce efficiency, create performance instabilities, and increase concerns about long-term reliability, have hindered wide-scale adoption. Prior work, including application of a scanning probe based deep level trap spectroscopy (SP-DLTS) defect mapping technique and scanning transmission electron microscope (STEM) based electron energy loss spectroscopy (EELS), has shown that the most detrimental defects, with energy level near mid-gap (thus serving as a carrier recombination center), are most likely caused by CuIn/Ga antisites and tend to cluster at or around certain grain boundaries [1,2]. However, the exact nature of these particular boundaries — their structures, chemistries, or even the relative misorientation of their associated grains — and their relation to this defect clustering and/or its formation is yet unknown. As such, electron backscatter diffraction (EBSD) orientation mapping, directly correlated with defect-sensitive techniques like SP-DLTS and/or STEM-EELS, could prove critical for providing the final missing links toward understanding the mechanisms behind these defects. Indeed, recent studies using correlative electron beam induced current (EBIC) with EBSD have been able to identify boundaries, and their relative misorientations, that possess detrimental electronic properties [3]. However, because EBIC is unable to resolve the defect energy levels, many questions are left unanswered. Furthermore, this study, and others like it, employed focused ion beam (FIB) milling to flatten the natively-rough CIGS [3-5], which may run the risk of changing the nature of any near-surface defect structures.

14 SOLAR ENERGY↗
DOE OSTI2022

Effect of anisotropic fast ions on internal kink stability in DIII-D negative and positive triangularity plasmas

Recent DIII-D experiments show that sawtooth stability is strongly affected by anisotropic fast ions from neutral beam injection (NBI) in both negative and positive triangularity plasmas. Fast ions from co-current NBI are stabilizing for the sawtooth stability, resulting in longer sawtooth periods. On the other hand, fast ions from counter-current NBI are destabilizing, leading to small and frequent sawteeth. The relative change of sawtooth period and amplitude is more than a factor of two. These observations appear to hold in both plasma shapes. Non-perturbative toroidal modeling, utilizing the magnetohydrodynamic-kinetic hybrid stability code MARS-K (Liu et al 2008 Phys. Plasmas 15 112503), reveals an asymmetric dependence of the stability of the n = 1 (n is the toroidal mode number) internal kink mode on the injection direction of NBI, being qualitatively consistent with the experimentally observed sawtooth behavior. The MARS-K modeling results suggest that anisotropic fast ions affect the mode growth rate and frequency through both adiabatic and non-adiabatic contributions. Here, the asymmetry of the internal kink mode instability relative to the NBI direction is mainly due to the non-adiabatic contribution of passing fast ions, which stabilize (destabilize) the internal kink with the co-(counter-) current NBI as compared to the fluid counterpart. However, finite orbit width (FOW) correction to passing particles partially cancels the asymmetry. Trapped particles are always stabilizing due to precessional drift resonance. Modeling also shows that fast ions affect the internal kink in a similar manner in both negative and positive triangularity plasmas, although being slightly more unstable in the negative triangularity configuration already in the fluid limit. The similarity is mainly attributed to the fact that the mode is localized in the plasma core region, with very similar eigenmode structures in both negative and positive configurations. Furthermore, MARS-K modeling indicates that other factors, such as the plasma rotation and the drift kinetic effects of thermal plasmas, weakly modify the mode stability as compared to the drift kinetic resonance effects and FOW correction of fast ions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Electrolyte-driven interphase stabilization in high-voltage sodium-ion full cells

Sodium-ion batteries with a high-voltage O3-type layered oxide cathode paired with a hard carbon anode can offer high energy density; however, significant interfacial instabilities driven by electrode/electrolyte reactions limit a broader industrial adoption. Localized high concentration electrolytes (LHCEs) are a rational choice as they promote salt decomposition over solvent, forming stable, inorganic-rich electrode-electrolyte interphases (EEIs). We present here a comparison of high-voltage (4.2 V) hard carbon | NaNi 1/3 Fe 1/3 Mn 1/3 O 2 pouch cells in LHCEs and in a standard carbonate-based electrolyte by (i) examining the influence of diluent choice on the electrochemical performance of LHCEs and (ii) investigating how the electrolyte chemistry affects the composition and structure of EEIs formed. Importantly, LHCEs demonstrate superior electrochemical performance, achieving 37% higher capacity after 200 cycles (119 vs. 87 mA h g -1 ) compared to the carbonate-based electrolyte. The enhanced stabilization provided by LHCEs at the interface with high-voltage sodium layered oxide cathode is revealed by gas evolution measurements obtained through online electrochemical mass spectrometry (OEMS). Time-of-flight secondary ion mass spectrometry paired with focused ion beam and advanced statistical analyses reveal that the superior performance of LHCE stems from a robust, thin cathode electrolyte interphase formed on the sodium layered oxide cathode and a homogeneous solid electrolyte interphase formation on the hard carbon anode. Furthermore, this study highlights the critical importance of electrolyte design in interphase stabilization, which plays a key role in advancing sodium-ion batteries toward commercial viability.

25 ENERGY STORAGE↗
DOE OSTI2025

First simultaneous observation of co- and counter-current fast-ion losses in the ASDEX Upgrade tokamak

In ITER and future fusion power plants, the source of the fusion born alpha particles is almost isotropic in pitch angle, thus having co- and counter-current populations. For trapped ions, the co-current side of the orbit corresponds to its outer leg, while the counter-current side corresponds to the inner leg. Understanding the mechanisms responsible for the fast-ion losses (FILs) is critical for future magnetically confined fusion power plants. To further study the interplay of fast ions with plasma instabilities, a double pinhole collimator has been developed for a Fast-Ion Loss Detector (FILD) in the ASDEX Upgrade tokamak (AUG). This new FILD opens the operational window to simultaneous measurements of the co- and counter-current ion velocity-space. In this paper, the first results for the AUG double collimator FILD detector are shown. The commissioning of this new probe is carried out in H-mode plasmas with an on-axis magnetic field $B_0 = -2.5$ T, and a plasma current $I_{\textrm{p}} = 0.7$ MA. Simultaneous co- and counter-current FILs have been measured. Both have shown a similar dependence on Ion Cyclotron Resonance Heating (ICRH) power, where the main difference is the intensity of the losses, with the co-losses being an order of magnitude larger. Toroidal Alfvén eigenmode-coherent ICRH-only losses have been identified for the co-current ions. Additionally, the presence of Edge Localized Modes during the discharge were shown to increment Neutral Beam Injection prompt losses, while partially mitigating ICRH-driven losses on both co- and counter- sides of the velocity-space. Finally, a very trapped and high gyroradius losses, with an unclear origin, have been measured in the co- and counter-current velocity-space. The computed ion trajectories show that these ions remain permanently near the vessel wall, suggesting that they are accelerated within the scrape-off layer.

ELM↗