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At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
NASA NTRS1979

Inversion of stratospheric aerosol and gaseous constituents from spacecraft solar extinction data in the 0.38-1.0-micron wavelength region

The paper discusses a possible data retrieval technique for the spaceborne Stratospheric Aerosol and Gas Experiment (SAGE). The SAGE instrument has four radiometric channels located at selected intervals in the 0.38-1.0-micron wavelength range. A data reduction procedure is described for minimization of experimental errors on the basis of a detailed simulation of the measurement sequence. An efficient and accurate inversion method is then used for the retrieval of all the constituent vertical profiles. Also, the effects of horizontally inhomogeneous distributions of the constituent vertical profiles are studied based on available data of their global distributions. A simple horizontally inhomogeneous model of stratospheric aerosol and ozone is employed to estimate the perturbation on the retrieval accuracies.

Chu, W. P.↗
DOE OSTI2021

All-sky aerosol direct radiative effects at the ARM SGP site

All-sky aerosol direct radiative effect (DRE) was estimated for the first time at the Atmospheric Radiation Measurement Southern Great Plains site using multi-year ground-based observations. The NASA Langley Fu-Liou radiation model was employed. Observed inputs for the radiation model include aerosol and cloud vertical extinction profile from Raman lidar; spectral aerosol optical depth, single-scattering albedo, and asymmetry factor from Aerosol Robotic Network; cloud water content profiles from radars; temperature and water vapor profiles from radiosondes; and surface shortwave spectral albedo from radiometers. A cloudy-sky radiative closure experiment was performed. The relative mean differences between modeled and observed surface downwelling shortwave total fluxes were 6% (7%) for transparent (opaque) cloudy-skies. The estimated annual mean all-sky aerosol DRE is -2.13±0.54W m -2 at the top of atmosphere (TOA) and -5.95±0.87 W m -2 at the surface, compared to -3.00±0.58 W m -2 AND -6.85±1.00 W m -2 , respectively, under clear-sky conditions. The seasonal cycle of all-sky aerosol DRE is similar to that of the clear-sky, except with secondary influences of the clouds: The cloud radiative effect is strongest (most negative) in the spring, which reduces the all-sky aerosol DRE. The relative uncertainties in all-sky aerosol DRE due to measurement errors are generally comparable to those in clear-sky conditions except for the aerosol single-scattering albedo. Finally, the TOA all-sky aerosol DRE relative uncertainty due to aerosol single-scattering albedo uncertainty is larger than that in clear-sky, leading to a larger total relative uncertainty. The measurement errors in cloud properties have small effects on the all-sky aerosol DRE.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1992

Raman lidar measurements of Pinatubo aerosols over southeastern Kansas during November-December 1991

Raman lidar measurements over southeastern Kansas of stratospheric aerosols produced by the June 1991 eruptions of Mt. Pinatubo were made on 10 nights during November and December 1991. Both aerosol backscattering and extinction profiles were derived simultaneously from the lidar data since this system detects Raman scattering from nitrogen and oxygen as well as the backscattered light from aerosols and molecules. Aerosols scattering ratios greater than 3(at 351 nm) were measured on several nights. Peak aerosol concentrations were located between 19-22 km and varied significantly from night to night. Aerosol extinction/backscatter ratios computed from the lidar data and averaged over the altitude region of enhanced aerosol scattering between 15-25 km varied between 18-28 sr. Mie computations show these values to be consistent with scattering by aerosol particles with mode radii between 0.3 to 0.5 micron and that the ratios would increase to 40-65 sr at 694 nm. Aerosol optical thicknesses derived from the lidar extinction measurements at 351 nm varied between 0.04 and 0.06.

Ferrare, R. A.↗
NASA NTRS1977

The inversion of stratospheric aerosol and ozone vertical profiles from spacecraft solar extinction measurements

The inversions of multi-channel solar extinction measurements have been analyzed for the 0.35-1.0 micron wavelength region to retrieve stratospheric aerosol and ozone vertical profiles using both the constrained linear inversion scheme and the iterative scheme. The inversions of the multi-wavelength solar extinction data obtained from spacecraft have been analyzed based on the inversion of computer simulated data using various atmospheric models with differing amounts of aerosol and ozone in the stratosphere. The sensitivities of the inversion schemes to different experimental errors are discussed in terms of accuracy and resolution of the retrieved profiles.

Chu, W. P.↗
NASA NTRS2010

Assessment of Aerosol Distributions from GEOS-5 Using the CALIPSO Feature Mask

A-train sensors such as MODIS, MISR, and CALIPSO are used to determine aerosol properties, and in the process a means of estimating aerosol type (e.g. smoke vs. dust). Correct classification of aerosol type is important for climate assessment, air quality applications, and for comparisons and analysis with aerosol transport models. The Aerosols-Clouds-Ecosystems (ACE) satellite mission proposed in the NRC Decadal Survey describes a next generation aerosol and cloud suite similar to the current A-train, including a lidar. The future ACE lidar must be able to determine aerosol type effectively in conjunction with modeling activities to achieve ACE objectives. Here we examine the current capabilities of CALIPSO and the NASA Goddard Earth Observing System general circulation model and data assimilation system (GEOS-5), to place future ACE needs in context. The CALIPSO level 2 feature mask includes vertical profiles of aerosol layers classified by type. GEOS-5 provides global 3D aerosol mass for sulfate, sea salt, dust, and black and organic carbon. A GEOS aerosol scene classification algorithm has been developed to provide estimates of aerosol mixtures and extinction profiles along the CALIPSO orbit track. In previous work, initial comparisons between GEOS-5 derived aerosol mixtures and CALIPSO derived aerosol types were presented for July 2007. In general, the results showed that model and lidar derived aerosol types did not agree well in the boundary layer. Agreement was poor over Europe, where CALIPSO indicated the presence of dust and pollution mixtures yet GEOS-5 was dominated by pollution with little dust. Over the ocean in the tropics, the model appeared to contain less sea salt than detected by CALIPSO, yet at high latitudes the situation was reserved. Agreement between CALIPSO and GEOS-5, aerosol types improved above the boundary layer, primarily in dust and smoke dominated regions. At higher altitudes (> 5 km), the model contained aerosol layers not detected by CALIPSO. Here we present new results for a full year study using the new Version 3 CALIPSO data and most recent GEOS-5 model results.

Welton, Ellsworth↗
NASA NTRS2002

The Measurement of Aerosol Optical Properties using Continuous Wave Cavity Ring-Down Techniques

Large uncertainties in the effects that aerosols have on climate require improved in situ measurements of extinction coefficient and single-scattering albedo. This paper describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5 M/m). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

Strawa, Anthony W.↗
NASA NTRS2004

Optimal Aerosol Parameterization for Remote Sensing Retrievals

We have developed a new algorithm for the retrieval of aerosol and gases from SAGE It1 solar transmission measurements. This algorithm improves upon the NASA operational algorithm in several key aspects, including solving the problem non-linearly and incorporating a new methodology for separating the contribution of aerosols and gases. In order to extract aerosol information we have built a huge database of aerosol models for both stratospheric and tropospheric aerosols, and polar stratospheric cloud particles. This set of models allows us to calculate a vast range of possible extinction spectra for aerosols. and from these, derive a set of eigenvectors which then provide the basis set used in our inversion algorithm. Our aerosol algorithm and retrievals are described in several articles (listed in References Section) published under this grant. In particular they allow us to analyze the spectral properties of aerosols and PSCs and ultimately derive their microphysical properties. We have found some considerable differences between our spectra and the ones derived from the SAGE III operational algorithm. These are interesting as they provide an independent check on the validity of published aerosol data and, in particular, on their associated uncertainties. In order to understand these differences, we are assembling independent aerosol data from other sources with which to make comparisons. We have carried out extensive comparisons of our ozone retrievals with both SAGE III and independent lidar, ozonesonde, and satellite measurements (Polyakov et al., 2004). These show very good agreement throughout the stratosphere and help to quantify differences which can be attributed to natural variation in ozone versus that produced by algorithmic differences. In the mid - upper stratosphere, agreement with independent data was generally within 5 - 20%. but in the lower stratosphere the differences were considerably larger. We believe that a large proportion of this discrepancy in the lower stratosphere is attributable to natural variation, and is also seen in comparisons between lidar and ozonesonde measurements. NO2 profiles obtained with our algorithm were compared to those obtained through the SAGE III operational algorithm and exhibited differences of 20 - 40%. Our retrieved profiles agree with the HALOE NO2 measurements significantly better than those of the operational retrieval. In other work (described below), we are extending our aerosol retrievals into the infrared regime and plan to perform retrievals from combined uv-visible-infrared spectra. This work will allow us to use the spectra to derive the size and composition of aerosols, and we plan to employ our algorithms in the analysis of PSC spectra. We are presently also developing a limb-scattering algorithm to retrieve aerosol data from limb measurements of solar scattered radiation.

Newchurch, Michael J.↗
NASA NTRS2002

The Measurement of Aerosol Optical Properties Using Continuous Wave Cavity Ring-Down Techniques

Large uncertainties in the effects that aerosols have on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This abstract describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5/Mm). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

Strawa, A. W.↗
NASA NTRS2000

Comparison of Aerosol Optical Properties and Water Vapor Among Ground and Airborne Lidars and Sun Photometers During TARFOX

We compare aerosol optical thickness (AOT) and precipitable water vapor (PWV) measurements derived from ground and airborne lidars and Sun photometers during TARFOX (Tropospheric Aerosol Radiative Forcing Observational Experiment). Such comparisons are important to verify the consistency between various remote sensing measurements before employing them in any assessment of the impact of aerosols on the global radiation balance. Total scattering ratio and extinction profiles measured by the ground-based NASA/GSFC Scanning Raman Lidar (SRL) system, which operated from Wallops Island, Virginia (37.86 deg N, 75.51 deg W), are compared with those measured by the Lidar Atmospheric Sensing Experiment (LASE) airborne lidar system aboard the NASA ER-2 aircraft. Bias and rms differences indicate that these measurements generally agreed within about 10%. Aerosol extinction profiles and estimates of AOT are derived from both lidar measurements using a value for the aerosol extinction/backscattering ratio S(sub a)=60 sr for the aerosol extinction/backscattering ratio, which was determined from the Raman lidar measurements.

Ferrare, R.↗
NASA NTRS2002

A Wavelength Optimization Study on Visible and Infrared Propagation Systems in Coastal Environments

Electro-optical (EO) systems employed for communications, surveillance and weapons systems are commonly assessed in the North American and European continents. However, the atmospheric propagation environment in these regions is often dissimilar to most other parts of the world. In particular, atmospheric dust, industrial pollution, and smoke frequently reduce visibility to less than 5 km in Asia and South America significantly hampering EO system performance. Because atmospheric aerosol species vary considerably in size and chemistry, optimal wavelengths for EO systems vary from region to region. In this paper we examine the extinction effects from aerosol particles and water vapor on a regional basis. Theoretical studies are coupled with visibility and satellite climatologies to make an assessment for the coastal regions of the world. While longer wavelengths permit higher transmission by particles in regions significantly hampered by fine mode particles (such as industrial pollution and smoke), this advantage is commonly offset by high extinction values from water vapor. This offsetting effect is particularly strong in industrial and developing countries in the tropics and sub-tropics such as Southeast Asia and South America. Conversely, the advantage of low water vapor concentrations in longer wavelengths is offset by high mass-extinction efficiencies of atmospheric dust in this portion of the spectrum.

Reid, J. S.↗
DOE OSTI2022

Aerosol and Cloud Optical Properties from the ARM Raman Lidars: The Feature Detection and Extinction (RLPROF-FEX) Value-Added Product

Aerosols and their interactions and influence on clouds are among the main sources of uncertainties in radiative direct and indirect forcing (IPCC 2013). Continuous height-resolved measurements of cloud and aerosol optical properties are needed to reduce these uncertainties. Here we describe the Raman Lidar Profiles – Feature detection and Extinction (RLPROF-FEX) Value-Added Product (VAP) derived using Raman lidar data at multiple U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility sites. RLPROF-FEX provides estimates of extinction, backscatter, and depolarization using the algorithm described by Thorsen et al. 2015 and Thorsen and Fu 2015. This document provides a description of the FEX algorithm, its input and output data, and related details about the Raman lidar (RL) system.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1986

Retrieval of aerosol size distribution moments from multiwavelength particulate extinction data

An iterative method for deriving the particle size distribution from multiwavelength satellite remote sensing data is presented and its use illustrated with an application to SAGE II data. The compression size distribution method (CSD) features interpolation and look-up features for relating the coefficients of a least-squares fit as a function of wavelength to parameters of the compression function that have been obtained by Mie calculations. Results are reported of comparisons between particulate radii predicted for the El Chichon volcano aerosol based on SAGE II data and 14 radii measured with NASA flights through the aerosol with aircraft carrying wire impactors.

Livingston, J. M.↗
NASA NTRS1986

Stratospheric Aerosol and Gas Experiment (SAGE II)

Design features and the performance envelope of the SAGE II stratospheric aerosol monitoring instrument on the Earth Radiation Budget Satellite are described. SAGE II was designed to obtain vertical profiles of stratospheric aerosols, monitor global seasonal changes in aerosols, provide data on stratospheric circulation and the behavior of transient events such as volcanic particulate injections, and to investigate atmospheric chemistry. The mmeasurements are centered on extinctions due to aerosols, NO2, O3 and water vapor.

Mcmaster, L. R.↗
NASA NTRS1982

SAGE measurements of Mount St. Helens volcanic aerosols

The SAGE satellite system was used to make measurements on the optical extinction produced by stratospheric aerosols from the Mount St. Helens eruption. Two periods of observation were analyzed. In the first period (May 21 to 31, 1980), SAGE moved southward from latitude 60 N, and crossed the United States approximately one week after the May 18th eruption. Enhancements in stratospheric extinction were confined to latitudes between about 55 N and 25 N and longitudes between 10 W and 140 W. Individual layers were observed up to altitudes of 23 km. The geographical location of these layers corresponded closely to that expected on the basis of high-altitude meteorological data. During June and much of July, SAGE was, by reason of its geographical position and other orbital characteristics, unable to make further measurements on the northern hemisphere. Between July 19th and August 12th a second southward pass over the northern hemisphere occurred and further observations were made. The volcanic aerosol in the stratosphere was now found to be widely distributed over the hemisphere, the maximum concentrations being north of 50 N. The aerosol showed considerable inhomogeneity and had reached as far south as 15 N but little, if any, had crossed the equator into the southern hemisphere. Individual layers at different heights were still distinguishable. The total stratospheric aerosol loading on this occasion appeared to be greater than in May and corresponded to an increase in global stratospheric mass of between 50 and 100 percent.

Kent, G. S.↗
NASA NTRS1981

Measurements of the absorption coefficient of stratospheric aerosols

The absorption coefficients of stratospheric aerosols are measured using a variation on the integrating plate method. The technique is based on the decrease in the transparency of a substrate when an absorbing aerosol is deposited on it. A Lambert scatterer is placed behind the substrate to integrate forward scattered light and minimize the effect of scattering on the measurement. The low pressure in the stratosphere is used for the direct impaction of particles onto a narrow strip of opal glass. The eight samples collected had a median value of 4 x 10 to the -9th m with an uncertainty of + or - 5 x 10 to the -9th m. If this absorption is due to graphitic carbon, then its concentration is estimated at about 0.4 ng/cu m, or about 0.25% of the total aerosol mass concentration. Estimates of the aerosol scattering coefficients based on satellite extinction inversions result in an aerosol single-scattering albedo in the range of 0.96-1.0.

Ogren, J. A.↗
NASA NTRS1977

Inversion of solar extinction data from the Apollo-Soyuz Test Project Stratospheric Aerosol Measurement (ASTP/SAM) experiment

The inversion methods are reported that have been used to determine the vertical profile of the extinction coefficient due to the stratospheric aerosols from data measured during the ASTP/SAM solar occultation experiment. Inversion methods include the onion skin peel technique and methods of solving the Fredholm equation for the problem subject to smoothing constraints. The latter of these approaches involves a double inversion scheme. Comparisons are made between the inverted results from the SAM experiment and near simultaneous measurements made by lidar and balloon born dustsonde. The results are used to demonstrate the assumptions required to perform the inversions for aerosols.

Pepin, T. J.↗
DOE OSTI2020

Real‐Time Optical Process Monitoring for Structure and Property Control of Aerosol Jet Printed Functional Materials

Abstract Aerosol jet printing is a popular digital additive manufacturing method for flexible and hybrid electronics, but it lacks sophisticated real‐time process control schemes that would enable more widespread adoption in manufacturing environments. Here, an optical measurement system is introduced to track the aerosol density upstream of the printhead. The measured optical extinction, combined with the aerosol flow rate, is directly related to deposition rate and accurately predicts functional materials properties such as the electrical resistance of printed graphene films. This real‐time system offers a compelling solution for process drift and batch‐to‐batch variability, rendering it a valuable tool for both real‐time control of aerosol jet printing and fundamental studies of the underlying process science.

Tafoya, Rebecca R.↗