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At least 415 records · Page 23

Multi-Probe Campaign FY24 Omega EP Shot Request [Slides]

The ultimate goal of the Multi-Probe experimental campaign is to assess the feasibility of using multiple probe species (x-ray, proton, neutron, and electron) in future LANL radiographic facilities. To use Omega EP most efficiently, two different experiments are proposed for each of the two requested days in FY24. In this way, shots may be interleaved on the two short pulse beams and the shot rate doubled. In FY24, we propose to continue to develop the neutron source by first optimizing the “pitcher” source of deuterons/protons and then adding the “catcher” neutron converter on day 2. The second series of experiments continues examining the origin and nature of the x-ray background found in our last two experiments. This background is not well understood or characterized by the community. The first day will measure the electrons emanating from the proton and x-ray targets while also optimizing the background shielding first used in FY23. The second day will test a geometry that enables simultaneous radiographs using both short-pulse beams.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Multi-Probe FY25 Omega EP Shot Request [Slides]

The goal of the Multi-Probe experimental campaign is to assess the feasibility of using multiple probe types (x ray, proton, neutron, and electron) in future LANL radiographic facilities. X-ray and proton platforms have been demonstrated. The first attempts at simultaneous radiography were hampered by cross talk, which was the subject of FY23 & FY24 experiments. The major goal for FY25 is to demonstrate simultaneous radiography of both static and dynamic objects.

36 MATERIALS SCIENCE↗

Probing and Understanding the Spatial and Energy Distributions of Plasmonic Hot Carriers via Single-Molecule Quantum Transport

The generation of hot carriers in plasmonic nanostructures offers new transformative opportunities for a range of applications, including solar energy harvesting, photochemistry, and photodetection. To better understand such phenomena, this project aims to develop an experimental approach to study and understand hot carrier distributions in photoexcited plasmonic nanostructures. The developed experimental approach, combining scanning probe-based single-molecule quantum transport measurements with plasmonic excitation methods, leverages nanoscopic single molecules as quantum energy filters to selectively access hot carriers in a variety of plasmonic nanostructures. This report summarizes the key outcomes, impacts, and lessons learned in the first two years of the project. Over the past two years, important progress was made in achieving the project's goals, including the development of the scanning probe-based experimental platform, fabrication of plasmonic nanostructures, and design and synthesis of the desired molecular candidates. Insights from this research will pave the path toward the development of technologies that will improve the way we harvest solar energy and drive chemical reactions and ultimately help transition the U.S. to a clean and sustainable society.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Multi-Probe Radiography: For 2035 and Beyond

The Multi-Probe Radiography Project is investigating the use of multiple species of probe beams to provide more information from a radiography. Contextual radiographic, source, and measurements information is being provided through a series of four workshops at Los Alamos National Laboratory. The third workshop on Accelerator and Pulsed Power Technology is summarized in this report. The state of the large NNSA facilities such as Scorpius, DARHT, pRad, and Cygnus are presented. Future enhancements and innovative upgrades are also discussed.

43 PARTICLE ACCELERATORS↗

Addressing Experimental Challenges in Probing Dark Energy with Accuracy and Precision with the Rubin Observatory Legacy Survey of Space & Time (LSST)

With support from this award, the Stanford group under the leadership of PI Patricia Burchat focused on pixel-level algorithms that are key to the investigation of dark energy with the Vera C. Rubin Observatory Legacy Survey of Space and Time (LSST). The work was carried out through strong engagement in the DOE-supported LSST Dark Energy Science Collaboration (DESC), for which the PI served as Deputy Spokesperson (07/2019 - 07/2021) and Technical Coordinator (07/2021 - 07/2023). Members of the Burchat group are Full DESC members and are among scientists who have been accepted to join the Rubin Observatory System Integration, Test, and Commissioning (SIT-Com) effort. The specific intellectual focus of the group was the optimization of gravitational lensing as a probe of the evolution of the distribution of dark matter in space and time to learn about the nature of dark energy. The Stanford group pursued an integrated research program to understand in detail, and then remediate or calibrate, systematic effects that could limit the sensitivity of the LSST to cosmic shear as a dark energy probe -- particularly those related to our understanding of the atmospheric point spread function (PSF), challenges associated with blended galaxy images, and impacts of residual camera artifacts. Key to this work was developing, enhancing, and validating the fidelity of simulations that play a key role in the development of our understanding of subtle systematic biases and then using these simulations to develop techniques to characterize and mitigate biases, and associated algorithms for implementation in the LSST or DESC science pipelines. The group’s work included contributions to the open-source GalSim simulation package, which is widely used in the community; simulations and studies of spatial correlations of atmospheric PSFs; studies of temporal correlations of the atmospheric PSF; impacts of chromatic PSFs on cosmic shear calibration; continued studies of anisotropic Gaussian process interpolation of PSF models across the focal plane; and measuring and mitigating impacts of residual camera artifacts on cosmic shear. A primary impact of this work is that it increases the scientific discovery potential of the DOE and NSF investments in the Rubin Observatory Legacy Survey of Space \& Time, by addressing challenges in interpreting astronomical images through more accurate descriptions of the blurring of images due to the atmosphere. Specifically, this work impacts our ability to understand the fundamental nature of dark energy.

Burchat, Patricia Rose↗

Development of Operando Atom Probe to study field-assisted surface chemistry

Recent efforts at PNNL have led to the development of in-situ Atom Probe Tomography (ISAPT) and Operando Atom Probe (OAP), establishing PNNL as a key player in this technology, both in the U.S. and globally. OAP has already pushed the initial limits of APT, which was traditionally used at cryo temperatures (<60 K) and ultra-high vacuum (<10⁻¹² bar), to operate in the presence of reactive gases (up to 10⁻¹⁰ bar) at a maximum temperature of 300 K. Using OAP, we successfully observed Co and Fe oxidation in real-time at the nanoscale, revealing the importance of surface structures in these interactions. Additionally, OAP opens the possibility to explore the influence of local electric fields (EFs) on surface chemistry and hydrogen interactions at the nanoscale.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Calibrator for Airborne Aerosol Probes (CAAP) Field Campaign Report

In this campaign, Calibrator for Airborne Aerosol Probes (CAAP), Mesa Photonics provided its U.S. Department of Energy (DOE) Small Business Innovation Research (SBIR) Phase II prototype of a portable, battery-powered monodisperse aerosol/droplet generator to field-calibrate two aerosol/cloud characterization instruments deployed on the DOE Atmospheric Radiation Measurement (ARM) Aerial Facility (AAF) ArcticShark uncrewed aerial system (UAS) during the flight campaign conducted at ARM’s Southern Great Plains (SGP) atmospheric observatory and the Blackwell-Tonkawa airfield (Oklahoma) in May 2024. The CAAP campaign (May 20-24, 2024) partially overlapped with the main ARM AAF campaign, Turbulent Layers Promoting New Particle Formation (NPFTURBULENCE, May 7-27, 2024, Gannet Hallar, principal investigator). The main goal of the CAAP campaign was field validation of calibration of aerosol and cloud probes deployed on the ArcticShark UAS. The campaign also provided an opportunity to test and evaluate the Mesa Photonics’ monodisperse aerosol/droplet generator prototype in the field, under real-life operational conditions.

54 ENVIRONMENTAL SCIENCES↗

Project FELICIA - A probe to survey the RHIC magnet beampipe diameter for EIC beam screen insertion

The Electron Ion Collider (EIC) Hadron Storage Ring (HSR) will reuse many of the existing superconducting (SC) magnets of the RHIC storage rings. To comply with the beamline vacuum requirements in more demanding operational scenarios, the beampipe of the RHIC SC magnets will be equipped with low surface impedance, low secondary electron yield (SEY) beam screens. The installation of these beam screens will be done with the SC magnets as installed today, thus making it a critical operation for a timely EIC installation. The beam screen inner dimensions must be maximized to retain enough aperture to the beam. On the other hand, keeping enough clearance between the screen and the beampipe is critical to ensure a smooth beam screen installation. A survey probe was designed and built to measure the inner diameter of several RHIC SC magnets in-situ and provide critical data for the beam screen design optimization. This paper reports on the design of the probe and the results from the survey campaign.

43 PARTICLE ACCELERATORS↗

Probing BSM Oscillatory Signals with the DUNE Detectors and the LBNF Neutrino Beam: NSI and Sterile Neutrino Sensitivities

The Deep Underground Neutrino Experiment (DUNE) is a flagship long-baseline accelerator neutrino experiment under construction in the U.S. With a 1,300 km distance between its Near Detector (ND) and Far Detector (FD), the world’s most intense LBNF (Long-Baseline Neutrino Facility) neutrino beam, and high-resolution LArTPC (Liquid Argon Time Projection Chamber) detectors, DUNE will measure the neutrino oscillation parameters with unprecedented precision. In addition to the determination of the neutrino mass ordering and the potential discovery of Charge-Parity violation in the leptonic sector, DUNE's capabilities present a unique opportunity for probing Beyond the Standard Model (BSM) physics signals with neutrinos. Examples of BSM physics manifestations include the presence of Non-Standard Interactions (NSI) of neutrinos with matter, or the existence of sterile neutrinos that mix with 3-Flavor neutrinos. In this study, we present a joint ND+FD fit to simulated data assessing DUNE's sensitivity to probing neutrino NSI, as well as scenarios including sterile neutrino mixing.

Prais, Luiz [Cincinnati U.] (ORCID:000000018224947↗

Tau-Jet Matching and Tag-and-Probe Tau Tagging Efficiencies for HH→bbτ+τ− Searches Using Run 3 CMS Scouting Data

We are studying tau-jet matching efficiency and tau tagging efficiency for the search for Higgs boson pair production in the HH→bbτ+τ− decay channel using Run 3 CMS scouting data. Collision events in the CMS detector produce many particle candidates, so jets are clustered using the anti-kT algorithm to identify possible tau signatures. In Monte Carlo simulation, tau-jet matching efficiency can be measured by comparing generated taus to reconstructed jets. In actual collision data, however, generated taus are not available, so we use a tag-and-probe method with Z→τ+τ− candidate events. In this method, one tau candidate is used as the tag and the other as the probe. The invariant mass of the tau-pair candidates is plotted and fitted with signal and background functions to estimate the number of real tau events and determine the tagging efficiency. By comparing efficiencies in data and Monte Carlo simulation, this work helps evaluate the performance of scouting-based tau reconstruction and tau tagging for future HH→bbτ+τ− searches.

Bellot, Annella [North Central Coll.; Fermilab]↗

Tau-Jet Matching and Tag-and-Probe Tau Tagging Efficiencies for HH→bbτ+τ− Searches Using Run 3 CMS Scouting Data

We are studying tau-jet matching efficiency and tau tagging efficiency for the search for Higgs boson pair production in the HH→bbτ+τ− decay channel using Run 3 CMS scouting data. Collision events in the CMS detector produce many particle candidates, so jets are clustered using the anti-kT algorithm to identify possible tau signatures. In Monte Carlo simulation, tau-jet matching efficiency can be measured by comparing generated taus to reconstructed jets. In actual collision data, however, generated taus are not available, so we use a tag-and-probe method with Z→τ+τ− candidate events. In this method, one tau candidate is used as the tag and the other as the probe. The invariant mass of the tau-pair candidates is plotted and fitted with signal and background functions to estimate the number of real tau events and determine the tagging efficiency. By comparing efficiencies in data and Monte Carlo simulation, this work helps evaluate the performance of scouting-based tau reconstruction and tau tagging for future HH→bbτ+τ− searches.

Bellot, Annella [North Central Coll.; Fermilab]↗

Spinning Hall Probe magnetic compass

In a large range of physics and space experiments, the direction of the magnetic field needs to be determined with an accuracy on the level of one milli radian or better. We have proposed a new type of magnetic compass - a rotation-based one, which provides an alternating signal from the Hall probe proportional to the value of the magnetic field transverse to the axis of rotation. The spinning Hall probe device has been realized. Alignment of the spinning axis for a minimum (zero) value of the signal allows us to find the direction of the magnetic field. The device does not require calibration and is free of any drift problems. The measurement of the rotation axis direction was accomplished by means of a laser and a flat mirror attached to the rotor. The constructed prototype achieved an accuracy for the magnetic field direction in the experiment with the polarized He-3 target on the level of one milli radian.

Wojtsekhowski, Bogdan↗

Probing gluon saturation and nuclear structure in photon-nucleus collisions

We calculate exclusive vector meson photoproduction within the Color Glass Condensate framework in high-energy photon-nucleus scattering probed experimentally in ultra peripheral heavy ion collisions at RHIC and at the LHC. When the free parameters are constrained by the γ + p data from HERA, we predict significant nuclear suppression for both the coherent and incoherent photoproduction cross section in the TeV range. Our results indicate that the LHC data prefers even stronger saturation effects at the highest collision energies. Furthermore, we demonstrate how the linear polarization of photons in ulra peripheral collisions generates azimuthal modulations in the decay products of the exclusively produced vector meson. We show how these measurements can probe details of the nuclear geometry, specifically the deformed structure of the uranium nuclei.

Mäntysaari, Heikki [University of Jyväskylä (Finla↗

Genomics, Exometabolomics, and Metabolic Probing Reveal Conserved Proteolytic Metabolism of Thermoflexus hugenholtzii and Three Candidate Species From China and Japan

Thermoflexus hugenholtzii JAD2 T , the only cultured representative of the Chloroflexota order Thermoflexales, is abundant in Great Boiling Spring (GBS), NV, United States, and close relatives inhabit geothermal systems globally. However, no defined medium exists for T. hugenholtzii JAD2 T and no single carbon source is known to support its growth, leaving key knowledge gaps in its metabolism and nutritional needs. Here, we report comparative genomic analysis of the draft genome of T. hugenholtzii JAD2 T and eight closely related metagenome-assembled genomes (MAGs) from geothermal sites in China, Japan, and the United States, representing “Candidatus Thermoflexus japonica,” “Candidatus Thermoflexus tengchongensis,” and “Candidatus Thermoflexus sinensis.” Genomics was integrated with targeted exometabolomics and 13 C metabolic probing of T. hugenholtzii. The Thermoflexus genomes each code for complete central carbon metabolic pathways and an unusually high abundance and diversity of peptidases, particularly Metallo- and Serine peptidase families, along with ABC transporters for peptides and some amino acids. The T. hugenholtzii JAD2 T exometabolome provided evidence of extracellular proteolytic activity based on the accumulation of free amino acids. However, several neutral and polar amino acids appear not to be utilized, based on their accumulation in the medium and the lack of annotated transporters. Adenine and adenosine were scavenged, and thymine and nicotinic acid were released, suggesting interdependency with other organisms in situ. Metabolic probing of T. hugenholtzii JAD2 T using 13 C-labeled compounds provided evidence of oxidation of glucose, pyruvate, cysteine, and citrate, and functioning glycolytic, tricarboxylic acid (TCA), and oxidative pentose-phosphate pathways (PPPs). However, differential use of position-specific 13 C-labeled compounds showed that glycolysis and the TCA cycle were uncoupled. Thus, despite the high abundance of Thermoflexus in sediments of some geothermal systems, they appear to be highly focused on chemoorganotrophy, particularly protein degradation, and may interact extensively with other microorganisms in situ.

59 BASIC BIOLOGICAL SCIENCES↗

Ferroelectricity in Si-Doped Hafnia: Probing Challenges in Absence of Screening Charges

The ability to develop ferroelectric materials using binary oxides is critical to enable novel low-power, high-density non-volatile memory and fast switching logic. The discovery of ferroelectricity in hafnia-based thin films, has focused the hopes of the community on this class of materials to overcome the existing problems of perovskite-based integrated ferroelectrics. However, both the control of ferroelectricity in doped-HfO2 and the direct characterization at the nanoscale of ferroelectric phenomena, are increasingly difficult to achieve. The main limitations are imposed by the inherent intertwining of ferroelectric and dielectric properties, the role of strain, interfaces and electric field-mediated phase, and polarization changes. In this work, using Si-doped HfO2 as a material system, we performed a correlative study with four scanning probe techniques for the local sensing of intrinsic ferroelectricity on the oxide surface. Putting each technique in perspective, we demonstrated that different origins of spatially resolved contrast can be obtained, thus highlighting possible crosstalk not originated by a genuine ferroelectric response. By leveraging the strength of each method, we showed how intrinsic processes in ultrathin dielectrics, i.e., electronic leakage, existence and generation of energy states, charge trapping (de-trapping) phenomena, and electrochemical effects, can influence the sensed response. We then proceeded to initiate hysteresis loops by means of tip-induced spectroscopic cycling (i.e., “wake-up”), thus observing the onset of oxide degradation processes associated with this step. Finally, direct piezoelectric effects were studied using the high pressure resulting from the probe’s confinement, noticing the absence of a net time-invariant piezo-generated charge. Our results are critical in providing a general framework of interpretation for multiple nanoscale processes impacting ferroelectricity in doped-hafnia and strategies for sensing it.

36 MATERIALS SCIENCE↗

The Encounter of the Parker Solar Probe and a Comet-like Object Near the Sun: Model Predictions and Measurements

The Parker Solar Probe (PSP) aims to explore the nascent solar wind close to the Sun. Meanwhile, PSP is also expected to encounter small objects like comets and asteroids. Here, we survey the ephemerides to find the chance of a recent encounter and then model the interaction between released dusty plasmas and solar wind plasmas. On 2019 September 2, a comet-like object, the 322P/Solar and Heliosphere Observatory, just passed its perihelion flying to a heliocentric distance of 0.12 au and swept by PSP at a relative distance as close as 0.025 au. We present the dynamics of the dust particles released from 322P, forming a curved dust tail. Along the path of PSP in the simulated inner heliosphere, the states of plasma and magnetic field are sampled and illustrated, with the magnetic field sequences from simulation results being compared directly with the in situ measurements from PSP. Through the comparison, we suggest that 322P might be at a deficient activity level releasing limited dusty plasmas on its way to becoming a "rock comet." We also present images of solar wind streamers as recorded by the Wide-field Imager for Solar Probe Plus, showing an indication of dust bombardment for the images superposed with messy trails. We observe from the Large Angle and Spectrometric Coronagraph that 322P was transiting from a dimming region to a relatively bright streamer during its perihelion passage, and perform a simulation to confirm that 322P was flying from relatively faster to slower solar wind streams, modifying the local plasma states of the streams.

79 ASTRONOMY AND ASTROPHYSICS↗

Probing Physics beyond the Standard Model through Combined Analyses of Next-generation Type Ia Supernova, Cosmic Microwave Background, and Baryon Acoustic Oscillation Surveys

Observations of Type Ia supernovae (SNe Ia), which probe the late Universe, together with baryon acoustic oscillations (BAO) and the cosmic microwave background (CMB), which probe the intermediate and early epochs, provide complementary constraints on the expansion history of the Universe. In this work, we forecast constraints on dark energy and other extensions to the standard cosmological model by combining the SN Ia sample expected from the Vera C. Rubin Observatory’s Legacy Survey of Space and Time (LSST), data from current and forthcoming CMB surveys, and BAO measurements from the Dark Energy Spectroscopic Instrument (DESI). For the CMB, we use temperature, polarization, and lensing power spectra (TT/EE/TE/ϕϕ) from the South Pole Telescope, the planned Advanced Simons Observatory, and a CMB-S4–like experiment. We derive constraints on ΛCDM and its extensions involving the dark energy equation-of-state parameters (w 0 , w a ) and the sum of neutrino masses ∑m ν using a Markov Chain Monte Carlo (MCMC) sampling framework. We find that the LSST Year 3 SN Ia sample can improve upon the DES Year 5 dark energy constraints by a factor of 2−2.5×, with the gains driven primarily by the significantly higher SN Ia density in the LSST sample. Similarly, DESI-DR3 shows up to a 1.8× improvement on dark energy parameters over DR2, driven largely by the substantial increase in the low-redshift sample. Combining CMB with LSST-Y3-SN Ia and DESI-DR3-BAO yields σ(w 0 ) = 0.028 and σ(w a ) = 0.11 for w 0 w a CDM cosmology with the results being largely independent of the CMB dataset. The constraints weaken by 10%–30% when freeing ∑m ν and spatial curvature. Moreover, the joint analysis of the three datasets can enable a 2σ–3σ detection of ∑m ν .

Raghunathan, Srinivasan [University of California;↗

Computational Fluid Dynamics Modeling to Facilitate Qualification of Stack Sampling Probe Location

Computational fluid dynamics (CFD) modeling was used to help evaluate modifications to a radiological effluent stack and assist with establishing a stack sampling location that met the mixing criteria for qualification. Requirements for stack sampling location are listed in the American National Standards Institute/Health Physics Society (ANSI/HPS) N13.1-2021 standard. Modeling was performed to help develop a suitable design for increasing building ventilation for the radiological effluent stack. The ANSI/HPS N13.1-2021 criteria for the air monitoring probe location are that the coefficient of variation of velocity uniformity, gaseous tracer uniformity, and particulate tracer uniformity must be less than or equal to 20%. Furthermore, no point in the sampling location may have a gaseous tracer concentration that varies from the mean concentration by more than 30%. Additionally, the flow angle at the sampling location must not be more than 20 degrees. The ANSI/HPS N13.1-2021 standard allows for models (physical or computational) to be employed to perform the full suite of qualification tests, followed by a more limited set of verification tests on the actual stack to qualify the stack sampling location. Here, a series of computational model simulations were employed to evaluate the stack qualification criteria. Significant time and re-source savings are achieved using CFD modeling. CFD modeling demonstrated that the stack meets the criteria at the sample probe location. Verification tests were performed on the modified stack to measure the velocity uniformity and flow angle at the stack sampling location, and results demonstrated that the CFD model results may be used to support the qualification of the stack sampling location.

Air Monitoring↗