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At least 415 records · Page 23

Spin polarization through axially chiral linkers: Length dependence and correlation with the dissymmetry factor

Abstract The chiral‐induced spin selectivity (CISS) effect relates to the spin‐selective electron transport through chiral molecules; therefore, the chiral molecules act as spin filters. In past studies, correlation was found between the magnitude of the spin filtering and the intensity of the circular dichroism (CD) spectrum (the first Compton peak) of the molecules. Since the intensity of the CD peak relates to both the magnitude of the electric and magnetic dipole transitions, it was not clear which of these properties correlate with the CISS effect. This work aims at addressing this question. By studying the spin‐dependent conduction and the CD spectra of the thiol‐functionalized enantiopure binaphthalene (BINAP) and ternaphthalene (TERNAP), we found that both BINAP and TERNAP exhibit a similar spin polarization of 50%, despite the first Compton peak in TERNAP being almost twice as intense as the peak in BINAP. These results can be explained by the similar values of their anisotropy (or dissymmetry) factor, g abs , which is proportional to the magnetic transition dipole moment. Hence, we concluded that the CISS effect is proportional to the transition dipole moment in chiral molecules, namely, to the dissymmetry factor.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Bending of electromagnetic waves in all-dielectric particle array waveguides

We propose and demonstrate experimentally an alternative approach for realizing subwavelength photonic structures, exploiting the waveguiding properties of chains of high-index dielectric disks with both electric and magnetic dipole resonances. We reveal that the electromagnetic energy can be efficiently guided through sharp corners by means of the mode polarization conversion at waveguide bends. We confirm experimentally the guidance through a 90° bend in the microwave frequency range.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Upper limits to the magnetic field in central stars of planetary nebulae

More than about 20 central stars of planetary nebulae (CSPNs) have been observed spectropolarimetrically, yet no clear, unambiguous signal of the presence of a magnetic field in these objects has been found. We perform a statistical (Bayesian) analysis of all the available spectropolarimetric observations of CSPN to constrain the magnetic fields in these objects. Assuming that the stellar field is dipolar and that the dipole axis of the objects is oriented randomly (isotropically), we find that the dipole magnetic field strength is smaller than 400 G with 95% probability using all available observations. The analysis introduced allows integration of future observations to further constrain the parameters of the distribution, and it is general, so that it can be easily applied to other classes of magnetic objects. We propose several ways to improve the upper limits found here.

79 ASTRONOMY AND ASTROPHYSICS↗

Achromat Design for Multi-Pulse Test Line

This note describes the design of a 90° achromatic bend on DARHT Axis 2 to support multi-pulse target studies. The achromatic bend consists of two 45° dipole magnets with a focusing quadrupole centered between the dipoles. The optical design of the achromat is described followed by a discussion of the sensitivity to space charge and variations in the beam energy. The preliminary design of the magnets is then described with a description of the electro-mechanical parameters.

42 ENGINEERING↗

Collider study on the loop-induced dark matter mediation

Collider experiments are one of the most promising ways to constrain Dark Matter (DM) interactions. For DM couplings involving light mediators, especially for the loop-mediated interactions, a meaningful interpretation of the results requires to go beyond effective field theory. In this note we discuss the study of the magnetic dipole interacting DM, focusing on a model with anarchic dark flavor structure. By including the momentum-dependent form factors that mediate the coupling – given by the Dark Penguin – in collider processes, we study bounds from monophoton, diphoton, and non-pointing photon searches at the LHC. We also compare our results to constraints from the direct detection experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

BINARY NEUTRON STAR MERGERS: A JET ENGINE FOR SHORT GAMMA-RAY BURSTS

We perform magnetohydrodynamic simulations in full general relativity (GRMHD) of quasi-circular, equal-mass, binary neutron stars that undergo merger. The initial stars are irrotational, n = 1 polytropes and are magnetized. We explore two types of magnetic-field geometries: one where each star is endowed with a dipole magnetic field extending from the interior into the exterior, as in a pulsar, and the other where the dipole field is initially confined to the interior. In both cases the adopted magnetic fields are initially dynamically unimportant. The merger outcome is a hypermassive neutron star that undergoes delayed collapse to a black hole (spin parameter a / M {sub BH} ∼ 0.74) immersed in a magnetized accretion disk. About 4000 M ∼ 60( M {sub NS}/1.625 M {sub ⊙}) ms following merger, the region above the black hole poles becomes strongly magnetized, and a collimated, mildly relativistic outflow—an incipient jet—is launched. The lifetime of the accretion disk, which likely equals the lifetime of the jet, is Δ t ∼ 0.1 ( M {sub NS}/1.625 M {sub ⊙}) s. In contrast to black hole–neutron star mergers, we find that incipient jets are launched even when the initial magnetic field is confined to the interior of the stars.

79 ASTRONOMY AND ASTROPHYSICS↗

On a relation of the angular frequency to the Aharonov–Casher geometric phase in a quantum dot

By analysing the behaviour of a neutral particle with permanent magnetic dipole moment confined to a quantum dot in the presence of a radial electric field, Coulomb-type and linear confining potentials, then, an Aharonov–Bohm-type effect for bound states and a dependence of the angular frequency of the system on the Aharonov–Casher geometric phase and the quantum numbers associated with the radial modes, the angular momentum and the spin are obtained. In particular, the possible values of the angular frequency and the persistent spin currents associated with the ground state are investigated in two different cases.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

THE INCLINATION ANGLE AND EVOLUTION OF THE BRAKING INDEX OF PULSARS WITH PLASMA-FILLED MAGNETOSPHERE: APPLICATION TO THE HIGH BRAKING INDEX OF PSR J1640–4631

The recently discovered rotationally powered pulsar PSR J1640–4631 is the first to have a braking index measured, with high enough precision, that is greater than 3. An inclined magnetic rotator in vacuum or plasma would be subject not only to spin-down but also to an alignment torque. The vacuum model can address the braking index only for an almost orthogonal rotator, which is incompatible with the single-peaked pulse profile. The magnetic dipole model with the corotating plasma predicts braking indices between 3 and 3.25. We find that the braking index of 3.15 is consistent with two different inclination angles, 18.°5 ± 3° and 56° ± 4°. The smaller angle is preferred given that the pulse profile has a single peak and the radio output of the source is weak. We infer the change in the inclination angle to be at the rate −0.°23 per century, three times smaller in absolute value than the rate recently observed for the Crab pulsar.

79 ASTRONOMY AND ASTROPHYSICS↗

The Slow Orbital Evolution of the Accreting Millisecond Pulsar IGR J0029+5934

The accreting millisecond pulsars IGR J00291+5934 and SAX J1808.4–3658 are two compact binaries with very similar orbital parameters. The latter has been observed to evolve on a very short timescale of ∼70 Myr, which is more than an order of magnitude shorter than expected. There is an ongoing debate on the possibility that the pulsar spin-down power ablates the companion, generating large amounts of mass-loss in the system. Therefore it is interesting to study whether IGR J00291+5934 does show a similar behavior as its twin system SAX J1808.4–3658. In this work we present the first constraints on the orbital period derivative of IGR J00291+5934. By using XMM-Newton data recorded during the 2015 outburst and adding the previous results of the 2004 and 2008 outbursts, we are able to measure a 90% confidence level allowed range of −5×10{sup −13}< P-dot {sub b}<6×10{sup −13}. This implies that the binary is evolving on a timescale longer than 0.5 Gyr, which is compatible with the expected timescale of mass transfer driven by angular momentum loss via gravitational radiation. We discuss the scenario in which the power loss from magnetic dipole radiation of the neutron star is hitting the companion star. If this model is applied to SAX J1808.4–3658, then the difference in orbital behavior can be ascribed to a different efficiency for the conversion of the spin-down power into energetic relativistic pulsar wind and X-ray/gamma-ray radiation for the two pulsars, with IGR J00291+5934 requiring an extraordinarily low efficiency of less than ∼5% to explain the observations. We thus conclude that the pulsar wind ablation model is unlikely to be an accurate description of the mechanism driving the orbital evolution of the two systems.

79 ASTRONOMY AND ASTROPHYSICS↗

Protection layers on a superconducting microwave resonator toward a hybrid quantum system

We propose a protection scheme of a superconducting microwave resonator to realize a hybrid quantum system, where cold neutral atoms are coupled with a single microwave photon through magnetic dipole interaction at an interface inductor. The evanescent field atom trap, such as a waveguide/nanofiber atom trap, brings both surface-scattered photons and absorption-induced broadband blackbody radiation which result in quasiparticles and a low quality factor at the resonator. A proposed multiband protection layer consists of pairs of two dielectric layers and a thin nanogrid conductive dielectric layer above the interface inductor. We show numerical simulations of quality factors and reflection/absorption spectra, indicating that the proposed multilayer structure can protect a lumped-element microwave resonator from optical photons and blackbody radiation while maintaining a reasonably high quality factor.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Detection of the clock transition (1.14 μm) in ultra-cold thulium atoms

The magnetic dipole transition between fine structure sublevels of the ground state of thulium atom 4f{sup 13}({sup 2}F{sup o})6s{sup 2} has been directly excited in a cloud of ultra-cold atoms by a frequency-stabilised laser. This transition at the wavelength λ = 1.14 μm is planned to be used as the clock one in an optical frequency reference on laser-cooled thulium atoms. (extreme light fields and their applications)

74 ATOMIC AND MOLECULAR PHYSICS↗

Energy levels, lifetimes and radiative data of Ba XXVI

Highlights: • Lowest 110 levels for Ba XXVI are calculated. • Radiative data for E1, E2, M1 and M2 transitions within lowest 110 levels are presented. • Lifetimes for lowest 110 fine structure levels are provided. We report an extensive and an elaborate theoretical study of atomic data for Ba XXVI by considering Singlet, Doublet and Triplet (SDT) electron excitations within N-shell and single excitations from N-shell to O-shell. We have calculated energy levels and lifetimes for lowest 110 fine structure levels by using Multi-configuration Dirac–Fock method (MCDF). We have also considered Quantum Electrodynamics (QED) and Breit corrections in our calculations. We have presented the radiative data for electric and magnetic dipole (E1, M1) and quadrupole (E2, M2) transitions among lowest 110 levels. We have made comparisons of our calculated excitation energies and EUV (Extreme Ultraviolet) transition wavelengths with experimentally observed energy levels and wavelengths and achieved good agreement. We have also computed energy levels by performing similar relativistic distorted wave calculations using Flexible Atomic Code (FAC). Additionally, we have provided new atomic data for Ba XXVI which are not published elsewhere in the literature. We believe that our results may be beneficial in fusion plasma research and astrophysical investigations and applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DICKE’S SUPERRADIANCE IN ASTROPHYSICS. I. THE 21 cm LINE

We have applied the concept of superradiance introduced by Dicke in 1954 to astrophysics by extending the corresponding analysis to the magnetic dipole interaction characterizing the atomic hydrogen 21 cm line. Although it is unlikely that superradiance could take place in thermally relaxed regions and that the lack of observational evidence of masers for this transition reduces the probability of detecting superradiance, in situations where the conditions necessary for superradiance are met (close atomic spacing, high velocity coherence, population inversion, and long dephasing timescales compared to those related to coherent behavior), our results suggest that relatively low levels of population inversion over short astronomical length-scales (e.g., as compared to those required for maser amplification) can lead to the cooperative behavior required for superradiance in the interstellar medium. Given the results of our analysis, we expect the observational properties of 21 cm superradiance to be characterized by the emission of high-intensity, spatially compact, burst-like features potentially taking place over short periods ranging from minutes to days.

79 ASTRONOMY AND ASTROPHYSICS↗

Vibrational circular dichroism from ab initio molecular dynamics and nuclear velocity perturbation theory in the liquid phase

We report the first fully ab initio calculation of dynamical vibrational circular dichroism spectra in the liquid phase using nuclear velocity perturbation theory (NVPT) derived electronic currents. Our approach is rigorous and general and thus capable of treating weak interactions of chiral molecules as, e.g., chirality transfer from a chiral molecule to an achiral solvent. We use an implementation of the NVPT that is projected along the dynamics to obtain the current and magnetic dipole moments required for accurate intensities. The gauge problem in the liquid phase is resolved in a twofold approach. The electronic expectation values are evaluated in a distributed origin gauge, employing maximally localized Wannier orbitals. In a second step, the gauge invariant spectrum is obtained in terms of a scaled molecular moments, which allows to systematically include solvent effects while keeping a significant signal-to-noise ratio. We give a thorough analysis and discussion of this choice of gauge for the liquid phase. At low temperatures, we recover the established double harmonic approximation. The methodology is applied to chiral molecules ((S)-d{sub 2}-oxirane and (R)-propylene-oxide) in the gas phase and in solution. We find an excellent agreement with the theoretical and experimental references, including the emergence of signals due to chirality transfer from the solute to the (achiral) solvent.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Delayed energy injection model for gamma-ray burst afterglows

The shallow decay phase and flares in the afterglows of gamma-ray bursts (GRBs) are widely believed to be associated with the later activation of the central engine. Some models of energy injection involve a continuous energy flow since the GRB trigger time, such as the magnetic dipole radiation from a magnetar. However, in the scenario involving a black hole accretion system, the energy flow from the fall-back accretion may be delayed for a fall-back time ∼t {sub fb}. Thus, we propose a delayed energy injection model. The delayed energy would cause a notable rise to the Lorentz factor of the external shock, which will 'generate' a bump in the multiple band afterglows. If the delayed time is very short, our model degenerates to the previous models. Our model can explain the significant re-brightening in the optical and infrared light curves of GRB 081029 and GRB 100621A. A considerable fall-back mass is needed to provide the later energy; this indicates that GRBs accompanied with fall-back material may be associated with a low energy supernova so that the fraction of the envelope can survive during eruption. The fall-back time can give meaningful information on the properties of GRB progenitor stars.

79 ASTRONOMY AND ASTROPHYSICS↗

A theoretical and experimental study of pressure broadening of the oxygen A-band by helium

The rotationally resolved magnetic dipole absorption spectrum of the oxygen A-band b{sup 1}Σ{sub g}{sup +}(v=0)←X{sup 3}Σ{sub g}{sup −}(v=0) perturbed by collisions with helium was studied theoretically using the impact approximation. To calculate the relaxation matrix, scattering calculations were performed on a newly computed helium-oxygen (b{sup 1}Σ{sub g}{sup +}) interaction potential as well as on a helium-oxygen (X{sup 3}Σ{sub g}{sup −}) interaction potential from the literature. The calculated integrated line cross sections and broadening coefficients are in good agreement with experimental results from the literature. Additionally, cavity ring-down experiments were performed in the wings of the spectral lines for a quantitative study of line-mixing, i.e., the redistribution of rotational line intensities by helium-oxygen collisions. It is shown that inclusion of line-mixing in the theory is required to reproduce the experimentally determined absolute absorption strengths as a function of the density of the helium gas.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Designing stellarators using perpendicular permanent magnets

We have developed a fast method to design perpendicular permanent magnets for simplifying stellarator coils based on existing codes. Coil complexity is one of the main challenges for stellarators. To date, only electromagnetic coils have been used to generate 3D fields for stellarators. Permanent magnets provide an alternative way to produce the desired magnetic field for optimized stellarators. In this paper, we revisit the concept of representing surface current using magnetic dipoles and carry out numerical validations. A surface magnetization is proven to be equivalent to the surface current that can be linearly solved by existing coil design codes. An incremental multi-layer method has been developed to obtain a practical solution that is attainable with present permanent magnets. With this method, we can reproduce a half-Tesla NCSX configuration using specially designed neodymium magnets together with simple planar coils. It shows that stellarator coils could be substantially simplified by adopting permanent magnets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

First Search for Axion Dark Matter with a MADMAX Prototype

This Letter presents the first search for dark matter axions with mass in the ranges 76.56 to 76.82 μ⁢eV and 79.31 to 79.53 μ⁢eV using a prototype setup for the MAgnetized Disk and Mirror Axion eXperiment (MADMAX). The experimental setup employs a dielectric haloscope consisting of three sapphire disks and a mirror to resonantly enhance the axion-induced microwave signal within the magnetic dipole field provided by the 1.6 T Morpurgo magnet at CERN. Over 14.5 days of data collection, no axion signal was detected. A 95% CL upper limit on the axion-photon coupling strength down to |𝑔 𝑎⁢𝛾 |∼2×10 −11 GeV −1 is set in the targeted mass ranges, surpassing previous constraints, assuming a local axion dark matter density 𝜌 𝑎 of 0.3 GeV/cm 3 . This study marks the first axion dark matter search using a dielectric haloscope.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗