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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 415 records · Page 23
All sourcesNASA NTRSDOE OSTI
NASA NTRS2015

November 2013 Analysis of High Energy Electrons on the Japan Experimental Module (JEM: Kibo)

Albedo (precipitating/splash) electrons, created by galactic cosmic rays (GCR) interaction with the upper atmosphere move upwards away from the surface of the earth. In the past validation work these particles were often considered to have negligible contribution to astronaut radiation exposure on the International Space Station (ISS). Estimates of astronaut exposure based on the available Computer Aided Design (CAD) models of ISS consistently underestimated measurements onboard ISS when the contribution of albedo particles to exposure were neglected. Recent measurements of high energy electrons outside ISS Japan Experimental Module (JEM) using Exposed Facility (EF), Space Environment Data Acquisition Equipment - Attached Payload (SEDA-AP) and Standard DOse Monitor (SDOM), indicates the presence of high energy electrons at ISS altitude. In this presentation the status of these energetic electrons is reviewed and mechanism for the creation of these particles inside/outside South Atlantic Anomaly (SAA) region explained. In addition, limited dosimetric evaluation of these electrons at 600 MeV and 10 GeV is presented.

Badavi, Francis F.↗
NASA NTRS1974

The cosmic ray electron spectrum and its modulation from 1968 through 1972

Over the past five years we have measured the energy spectrum of primary cosmic ray electrons with both a balloon-borne and a satellite absorption spectrometer. All of the balloon flights used identical equipment that was launched each summer from Fort Churchill, Manitoba, Canada. The satellite, OGO-5, has been in an eccentric orbit since March 1968. Together these instruments provide the electron spectrum over a range of energy from 20 MeV to 20 GeV. This wide range and the substantial span of time covered by the measurements permit a detailed study of the solar modulation of electrons. These results are compared with the modulation of the nuclear components as observed by a neutron monitor and interpreted using the cosmic ray transport equation.

Fulks, G.↗
DOE OSTI2015

Modulation of the electronic property of phosphorene by wrinkle and vertical electric field

The electronic properties of wrinkled phosphorene and its response to charge injection and external vertical electric field have been studied using first-principles calculations. It is found that small-size wrinkle systems have lower energy than wrinkle-free monolayer, suggesting that free-standing phosphorene spontaneously forms small protrusion on its nanosheet. The ratio of wrinkle height to curvature radius increases with enlarging height, indicating a promotion of field enhancement factor. Furthermore, the injected charges mostly distribute at peak and valley. Direct-to-indirect band-gap transition has been found for zigzag wrinkle with height of 14.81 Å. The band gaps of wrinkled nanosheets decrease almost linearly with increasing field, which is caused by charge separation of valence band maximum and conduction band minimum.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Modulation of the electronic states of perovskite SrCrO 3 thin films through protonation via low-energy hydrogen plasma implantation approaches

Hydrogenation of transition metal oxides offers a powerful platform to tailor physical functionalities as well as for potential applications in modern electronic technologies. An ideal nondestructive and efficient hydrogen incorporation approach is important for the realistic technological applications. We demonstrate the proton injection on SrCrO 3 thin films via an effecient low-energy hydrogen plasma implantation experiments, without destroying the original lattice framework. Hydrogen ions accumulate largely at the interfacial regions with amorphous character which extend about one-third of the total thickness. The H x SrCrO 3 (HSCO) thin films appear like exfoliated layers which however retain the fully strained state with distorted perovskite structure. Proton doping induces the change of Cr oxidation state from Cr 4+ to Cr 3+ in HSCO thin films and a transition from metallic to insulating phase. As a result, our investigations suggest an attractive platform in manipulating the electronic phases in proton-based approaches and may offer a potential peeling off strategy for nanoscale devices through low-energy hydrogen plasma implantation approaches.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2025

Design Principles in Engineering of Multigrain Nanocatalysts via Multiscale Electronic Structure Characterization

Engineering grain boundary (GB) strain provides a promising pathway to tune the catalytic properties of nanocrystals. However, structural heterogeneity from random grain orientation and geometry has limited clear structure–property correlations. Here, we utilize a multigrain Co3O4/Mn3O4 core/shell nanocrystal platform as a model system to systematically investigate how geometric misfit strain at GBs serves as catalytically active sites for the oxygen reduction reaction. Through precise subnanometer-level control over grain morphology and by integrating multiscale electronic structure characterization, we identify the electronic structural signature of GB defects and establish a direct correlation between localized strain fields and modified electronic states. Strain modulation at GBs alters the eg orbital energy levels, with elongation along the z-axis combined with shear strain stabilizing the eg states, in contrast to the destabilization observed under pure shear strain. This stabilization mechanism enhances the electrocatalytic activity and selectivity of strained GBs compared with strain-relaxed grain surfaces. Furthermore, we reveal that GBs exhibit a radial strain gradient, producing a spatial energy shift that further modulates local electronic structures, as resolved through the classification of electron energy loss spectroscopy data. Together, these findings demonstrate that geometric misfit strain enables precise tuning of grain geometry and the resulting electronic structures, offering a robust strategy for engineering next-generation nanocatalysts.

Cho, Min Gee↗
DOE OSTI2025

Modulation of the Electronic and Vibrational Landscape in Lead Organic Chalcogenides

Metal organic chalcogenides (MOCs) are an emerging class of two-dimensional (2D) materials featuring tunable band gaps and strong light-matter interactions with great potential for optical and polaritonic applications. Lead organic chalcogenides (LOCs) stand out among MOCs for sustaining long-lived coherent optical phonons despite their distorted lattices. However, the strong electron–phonon coupling also leads to rapid charge carrier self-trapping, hindering carrier transport. Herein, we demonstrate that charge carrier self-trapping is suppressed in Se- and Te-based LOCs. Specifically, the expansive Se and Te orbitals give rise to more dispersive conduction bands and reduced electron effective masses, thereby mitigating carrier self-trapping. As a result of reduced carrier self-trapping, the Se- and Te-based LOCs exhibit enhanced band-to-band photoluminescence and improved charge transport performance. Furthermore, our results provide a synthetic route to Se- and Te-based LOC single crystals and demonstrate the potential of orbital engineering to tune their electronic and phononic properties.

Chalcogenides↗
DOE OSTI2026

Regulation of Energy and Mass Transport in a Hydrogen-Bonded Framework for Visible-Light-Driven CO2 Reduction in Water

Photoenzymatic reduction of CO2 to formate is a promising strategy for carbon valorization, yet its efficiency is still limited by inefficient energy and mass transport. Here, we design a series of isostructural hydrogen-bonded organic frameworks (HOFs) that establish confinement effects to promote photocatalytic NADH regeneration and the subsequent NADH-dependent enzymatic CO2-to-formate reduction. We demonstrate that spatial confinement within the framework channels localizes exciton migration to nanoscale domains and promotes interfacial dissociation. Additionally, Rh-induced electronic-structure modulation enables ultrafast electron transfer, while the intrinsic hydrogen-bond network furnishes directional proton conduction to NAD+. These synergistic regulations afford a photocatalytic NADH regeneration efficiency of 99.8% with a record apparent quantum efficiency of 32.8%, and drive formate production at a rate of 3020 μmol g-1 h-1 with 100% selectivity─the highest rate reported to date for all light-driven systems in water. The HOF-based catalyst retains 86.3% of its initial activity over five cycles, highlighting its robustness. This work offers mechanistic insight into how microenvironment engineering within HOF architectures regulates energy and mass transport in photoenzymatic catalysis, paving the way for the rational design of advanced hybrid catalytic systems.

Xu, Jiaxing↗
DOE OSTI2015

Cyanobacterial Alkanes Modulate Photosynthetic Cyclic Electron Flow to Assist Growth under Cold Stress

All cyanobacterial membranes contain diesel-range C15-C19 hydrocarbons at concentrations similar to chlorophyll. Recently, two universal but mutually exclusive hydrocarbon production pathways in cyanobacteria were discovered. We engineered a mutant of Synechocystis sp. PCC 6803 that produces no alkanes, which grew poorly at low temperatures. We analyzed this defect by assessing the redox kinetics of PSI. The mutant exhibited enhanced cyclic electron flow (CEF), especially at low temperature. CEF raises the ATP:NADPH ratio from photosynthesis and balances reductant requirements of biosynthesis with maintaining the redox poise of the electron transport chain. We conducted in silico flux balance analysis and showed that growth rate reaches a distinct maximum for an intermediate value of CEF equivalent to recycling 1 electron in 4 from PSI to the plastoquinone pool. Based on this analysis, we conclude that the lack of membrane alkanes causes higher CEF, perhaps for maintenance of redox poise. In turn, increased CEF reduces growth by forcing the cell to use less energy-efficient pathways, lowering the quantum efficiency of photosynthesis. This study highlights the unique and universal role of medium-chain hydrocarbons in cyanobacterial thylakoid membranes: they regulate redox balance and reductant partitioning in these oxygenic photosynthetic cells under stress.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2014

Electronic confinement in modulation doped quantum dots

Modulation doping, an effective way to dope quantum dots (QDs), modifies the confinement energy levels in the QDs. We present a self-consistent full multi-grid solver to analyze the effect of modulation doping on the confinement energy levels in large-area structures containing Si QDs in SiO{sub 2} and Si{sub 3}N{sub 4} dielectrics. The confinement energy was found to be significantly lower when QDs were in close proximity to dopant ions in the dielectric. This effect was found to be smaller in Si{sub 3}N{sub 4}, while smaller QDs in SiO{sub 2} were highly susceptible to energy reduction. The energy reduction was found to follow a power law relationship with the QD size.

36 MATERIALS SCIENCE↗
DOE OSTI2014

Modulation of the electron transport properties in graphene nanoribbons doped with BN chains

Using density-functional theory and the non-equilibrium Green's function method, the electron transport properties of zigzag graphene nanoribbons (ZGNRs) doped with BN chains are studied by systematically calculating the energy band structure, density of states and the transmission spectra for the systems. The BN chains destroyed the electronic transport properties of the ZGNRs, and an energy gap appeared for the ZGNRs, and displayed variations from a metal to a wide-gap semiconductor. With an increase in the number of BN chains, the band gap increased gradually in the band structure and the transmission coefficient decreased near the Fermi surface. Additionally, the doping position had a significant effect on the electronic properties of the ZGNRs.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Magneto-electronic coupling in modulated defect-structures of natural Fe{sub 1−x}S

We provide compelling experimental evidence that the low-temperature transition in natural non-stoichiometric Fe{sub 7}S{sub 8}, a major magnetic remanence carrier in the Earth's crust and in extraterrestrial materials, is a phenomenon caused by magnetic coupling between epitaxially intergrown superstructures. The two superstructures differ in their defect distribution, and consequently in their magnetic anisotropy. At T < 30 K, the magnetic moments of the superstructures become strongly coupled, resulting in a 12-fold anisotropy symmetry, which is reflected in the anisotropic magneto-resistance.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

Photovoltaic Shading Testbed for Module-Level Power Electronics

This document describes a repeatable test procedure that attempts to simulate shading situations, as would be experienced by typical residential rooftop photovoltaic (PV) systems. This type of shading test is particularly useful to evaluate the impact of different power conversion setups, including microinverters, DC power optimizers and string inverters, on overall system performance. Theperformance results are weighted based on annual estimates of shade to predict annual performance improvement. A trial run of the test procedure was conducted with a side by side comparison of a string inverter with a microinverter, both operating on identical 8kW solar arrays. Considering three different shade weighting conditions, the microinverter was found to increase production by 3.7%under light shading, 7.8% under moderate shading, and 12.3% under heavy shading, relative to the reference string inverter case. Detail is provided in this document to allow duplication of the test method at different test installations and for different power electronics devices.

14 SOLAR ENERGY↗