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NASA NTRS2018

Organic Ices in Titan's Stratosphere

Titan’s stratospheric ice clouds are by far the most complex of any observed in the solar system, with over a dozen organic vapors condensing out to form a suite of pure and co-condensed ices, typically observed at high winter polar latitudes. Once these stratospheric ices are formed, they will diffuse throughout Titan’s lower atmosphere and most will eventually precipitate to the surface, where they are expected to contribute to Titan’s regolith. Early and important contributions were first made by the InfraRed Interferometer Spectrometer (IRIS) on Voyager 1, followed by notable contributions from IRIS’ successor, the Cassini Composite InfraRed Spectrometer (CIRS), and to a lesser extent, from Cassini’s Visible and Infrared Mapping Spectrometer (VIMS) and the Imaging Science Subsystem (ISS) instruments. All three remote sensing instruments made new ice cloud discoveries, combined with monitoring the seasonal behaviors and time evolution throughout Cassini’s 13-year mission tenure. A significant advance by CIRS was the realization that co-condensing chemical compounds can account for many of the CIRS-observed stratospheric ice cloud spectral features, especially for some that were previously puzzling, even though some of the observed spectral features are still not well understood. Relevant laboratory transmission spectroscopy efforts began just after the Voyager encounters, and have accelerated in the last few years due to new experimental efforts aimed at simulating co-condensed ices in Titan’s stratosphere. This review details the current state of knowledge regarding the organic ice clouds in Titan’s stratosphere, with perspectives from both observational and experimental standpoints.

Astronomy↗

NASA NTRS2018

Organic Ices in Titan's Stratosphere

C. M. Anderson↗

NASA NTRSDate not supplied

The Antarctic Stratospheric Warming and its Impacts in 2019

We explore the mechanism, predictability and hemispheric-wide surface impacts of a rare stratospheric warming that occurred above Antarctica during austral spring (September to November) 2019, using the Japanese 55-year reanalysis set for the period 1979-2019. From late August to mid-September, the stratospheric polar vortex suddenly weakened, and the stratospheric temperatures dramatically rose over the Antarctic polar cap. The deceleration of the vortex observed at 10 hPa was as drastic as that of the first ever observed major sudden stratospheric warming in the SH during 2002, while the mean warming in the mid-stratosphere (~30hPa) over the course of spring 2019 broke the previous record of 2002 by ~50%. The key mechanism for this event was a poleward shift of the polar night jet near the stratopause during mid-winter and subsequent record strong planetary wavenumber-one activity propagating from the troposphere in August, which acted to dramatically weaken the polar vortex. The easterly wind anomalies and positive temperature anomalies moved downward to the surface during October to December, causing the index polarity of the Southern Annular Mode (SAM) to become record-negative for the season. The record negative SAM played a key role in inducing significant local climate extremes over eastern Australia, southern New Zealand, eastern South America and western Patagonia. Especially, the strong negative SAM was the key driver of the extreme hot and dry conditions over subtropical eastern Australia in late spring 2019 that, in turn, were conducive for the severe wildfires that occurred during that time. State-of-the-art dynamical sub-seasonal to seasonal forecast systems skilfully predicted the upward propagating wavenumber-one activity in August, the significant vortex weakening of austral spring 2019, and subsequent development of negative SAM from late July.

Eun-Pa Lim↗

NASA NTRSDate not supplied

A Comparison of Stratospheric Smoke Events Seen by SAGE II (1984-2005) and SAGE III (2017-2021)

The ongoing Stratospheric Aerosol and Gas Experiment aboard the International Space Station (SAGE III/ISS) has mostly occurred during a period of relatively low aerosol loading. At the same time, it has almost observed a number of small to moderate injections of volcanic material in the stratosphere from the Aoba/Ambae eruption of 2018 to that of Karymsky in 2022. In addition, two of the largest known smoke intrusions into the stratosphere have occurred during the SAGE III/ISS mission (the British Columbia fire of August 2017 and the Australian Wildfire Event of 2019/2020). At least two other much smaller smoke events have also been observed in the SAGE III data (California Creek in September 2020 and McKay Creek in June 2021). Particularly with the two large events, it is tempting to speculate that these events are increasing in intensity and frequency possibly due to ongoing climate change. Realistically, change is difficult to assess since instrument data sets that can be used for quantifying historical events can be quite different in what and where they provide measurements. This complicates comparing one event to another potentially separated by many years. An exception to this issues are the measurements by SAGE III/ISS and those of its predecessor SAGE II (1984-2005). Both use the same measurement strategy, measure aerosol extinction coefficient at 1020 nm, and have similar spatial/temporal coverage. Both instruments are known to observe smoke events in the stratosphere. However, both have the same low observation density characteristic of solar occultation such that near-global coverage takes almost a month and characterizing effectively instant events like smoke and volcanic events take a matter of weeks depending on the vagaries of where the observations are being made at a critical juncture unlike instruments with high temporal/spatial resolution like limb-scatter instruments such as OMPS and OSIRIS. The goal of this work will be to use the same analysis approach to both the SAGE II and SAGE III data and compare both the frequency and intensity of smoke events observed by these instruments. While we do not expect to be able to make conclusions about change between the periods, the analysis is a first step in interpreting changes in the contribution of smoke to the stratospheric aerosol budget between the time frames encompassed by these instruments.

L. W. Thomason↗

NASA NTRS2022

Dynamical Perturbation of the Stratosphere by a Pyrocumulonimbus Injection of Carbonaceous Aerosols

The Pacific Northwest pyrocumulonimbus Event (PNE) took place in British Columbia during the evening and night-time hours between the 12th and 13th of August 2017. Several pyroconvective clouds erupted in this occasion, and released in the upper troposphere/lower stratosphere unprecedented amounts of carbonaceous aerosols (300 ktn). Only a few years later, an even larger pyroCb injection took place over Australia. This event, named the Australian New Year (ANY) event, injected up to 1100 ktn of aerosol between December 29th 2019 and January 4th 2020. Such large injections of carbonaceous aerosol modify the stratospheric radiative budgets, locally perturbing stratospheric temperatures and winds. In this study, we use the Goddard Earth Observing System Chemistry Climate Model (GEOS CCM) to study the pertubations on the stratospheric meteorology induced by an aerosol injection of the magnitude of the PNE. Our simulations include the radiative interactions of aerosols, so that their impact on temperatures and winds are explicitly simulated. We show how the presence of the carbonaceous aerosols from the pyroCb causes the formation and maintenance of a synoptic scale stratospheric anticyclone. We follow this disturbance considering the potential vorticity anomaly and the brown carbon aerosol loading and we describe its dynamical and thermodynamical structure and its evolution in time. The analysis presented here shows that the simulated anticyclone undergoes daily expansion-compression cycles governed by the radiative heating, which are directly related to the vertical motion of the plume, and that the aerosol radiative heating is essential in maintaining the anticyclone itself.

Pyrocumulonimbus↗

NASA NTRS2023

Connections Between Upper Tropospheric and Lower Stratospheric Circulation Responses to Increased Co 2

There are a myriad of ways atmospheric circulation responds to increased CO 2 . In the troposphere, the region of the tropical upwelling narrows, the Hadley Cells expand, and the upper level subtropical zonal winds that comprise the subtropical jet strengthen. In the stratosphere, the tropical upwelling narrows and strengthens, enhancing the Brewer-Dobson Circulation. Despite the robustness of these projections, dynamical coupling between the features remains unclear. In this study, we analyze output from the NASA Goddard Institute for Space Studies (GISS) ModelE coupled climate model to examine any connection between the upper tropospheric and lower stratospheric circulation by considering the features’ seasonality, hemispheric asymmetry, scaling, and transient response to a broad range of CO 2 forcings. We find that a narrowing and strengthening of upper tropospheric upwelling occurs with a strengthening of the subtropical jet. There is also a narrowing and strengthening of lower stratospheric upwelling that is related to an equatorward shift in critical latitude for wave breaking and the associated strengthening of the subtropical lower stratosphere’s zonal winds. However, the stratospheric responses display different seasonal, hemispheric, and transient patterns than those in the troposphere, indicating independent circulation changes between the two domains.

Molly E. Menzel↗

NASA NTRSDate not supplied

Are the Stratospheric Teleconnection Pathways Similar for Fast and Slowly Propagating Madden-Julian Oscillation (MJO) Episodes?

The Madden-Julian Oscillation (MJO) can influence the extratropical circulation on timescales up to several weeks, with a dependence on the MJO characteristics: MJO events that propagate slowly across the Maritime Continent have a stronger impact on Euro-Atlantic weather than fast MJO events. The slow (fast) MJO events are defined as events that take more (less) than 15 (10) days to propagate from the Indian Ocean (phase 3) to the Pacific Ocean (phase 6), and the MJO amplitude has to be greater than 1 for at least three consecutive days in phase 3 and phase 6. Slowly propagating MJO events lead to a stronger North Atlantic Oscillation (NAO) response than fast MJO events, and the positive (negative) NAO response for slow events occur after a lag of 10 days following phase 4 (phases 7-8). Furthermore, the MJO can influence the strength of the stratospheric polar vortex, which in turn can impact the NAO via downward coupling. While the tropospheric pathway for teleconnections from the MJO events with varying phase speeds is well understood, the stratospheric pathways for MJO events with different propagation speeds have yet to be explored. In this talk, I will discuss the stratospheric pathways during fast and slow MJO episodes using reanalysis data with respect to the strength of the Northern Hemisphere stratospheric polar vortex and subsequent downward coupling to the troposphere. This is evident from the zonal wind response within the stratospheric polar vortex at 60N and 10-hPa and the geopotential height response at 500-hPa and 100-hPa.

Priyanka Yadav↗

NASA NTRSDate not supplied

Assessing Stratospheric Aerosols Contamination Due to Space Activities

The life cycle of a spacecraft starts and ends in the atmosphere: it interacts with the atmosphere right after the launch and during the atmospheric reentry when it usually mostly ablates. Both phases induce emissions of gases and solid particles, providing a source of these components in the middle atmosphere. Little is known about the exact nature, composition and effects of these emissions on the atmosphere and climate, but their impact is expected to rise as more and more orbiting satellites are launched. Ever since the years 2000, the number of space rockets launched per year has increased by a factor 3 globally. At the same time, the number of satellites launched in orbit around the Earth per year has been multiplied by about 30. One may wonder whether changes in the anthropogenic material injected in the terrestrial stratosphere can be detected and what its influence may be. In order to study the cosmic dust particles arriving on Earth, the NASA Johnson Space Center (JSC) has been systematically collecting solid dust particles from the Earth’s stratosphere by aircraft equipped with dedicated particle collectors since 1981. So far, 25 catalogs have been published, covering campaigns of collection from 1981 to 2020, with a total of 5071 solid particles that have been preliminary characterized and curated. In this work, we use the preliminary classification of the dust particles. Based on SEM images and X-ray EDS composition the collected dust is separated into four groups: C (Cosmic), TCN (Terrestrial Contaminant Natural), TCA (Terrestrial Contaminant Artificial) and AOS (Aluminum Oxide Sphere). The AOS being mostly generated by solid rocket propellant, they also belong to the TCA class. Our analysis of the data published indicates that from 1980 to 2009 the cosmic dust particles typically represent on average 40% of the collection with TCA and TCN corresponding to about 30% each. In the recent years, the TCA fraction has doubled to about 60% of the collection (2010-2020). This increase in anthropogenic particles is likely due to the overall human space activity and its recent increase. We will present the properties of the solid stratospheric dust particles collected and their evolution with time. Future work will be dedicated to better classify the natural and anthropogenic particles collected and described in the existing databases. We will use numerical modelling to produce quantitative estimates of the injected mass, the lifetime of particles in the middle atmosphere (stratosphere) and the relative abundance of the anthropogenic particles with respect to the stratospheric background particle population.

J Lasue↗

NASA NTRS2023

Satellite characterization of global stratospheric sulfate aerosols released by Tonga volcano

Large volcanic eruptions create an enhanced layer of sulfate aerosols in the stratosphere. These sulfuric acid droplets persist for many months, altering the climate and stratospheric chemistry. Sulfate aerosols scatter sunlight back to space, cooling the surface of the Earth and absorb outgoing thermal radiation, heating the stratosphere. The calculation of the climate impact of sulfate aerosols depends on their physical properties such as droplet size and chemical composition. These properties are not well known, and this uncertainty contributes to the errors in climate model predictions. Here we derive the first empirical formula that predicts the composition of stratospheric sulfate aerosols from volcanic eruptions from the air temperature and water vapor pressure. Measurements of atmospheric infrared transmittance of the Hunga Tonga-Hunga Ha'apai sulfate aerosol plume by the Atmospheric Chemistry Experiment (ACE) satellite were analyzed to determine composition (weight percent of sulfuric acid) and median particle radius. These data are supplemented by measurements of the Raikoke and Nabro eruptions. Our analysis allows the properties of volcanic aerosols in the stratosphere to be predicted reliably in atmospheric models.

P Bernath↗

NASA NTRS2004

Observational Evidence Against Mountain-Wave Generation of Ice Nuclei as a Prerequisite for the Formation of Three Solid Nitric Acid Polar Stratospheric Clouds Observed in the Arctic in Early December 1999

A number of recently published papers suggest that mountain-wave activity in the stratosphere, producing ice particles when temperatures drop below the ice frost point, may be the primary source of large NAT particles. In this paper we use measurements from the Advanced Very High Resolution Radiometer (AVHRR) instruments on board the National Oceanic and Atmospheric Administration (NOAA) polar-orbiting satellites to map out regions of ice clouds produced by stratospheric mountain-wave activity inside the Arctic vortex. Lidar observations from three DC-8 flights in early December 1999 show the presence of solid nitric acid (Type Ia or NAT) polar stratospheric clouds (PSCs). By using back trajectories and superimposing the position maps on the AVHRR cloud imagery products, we show that these observed NAT clouds could not have originated at locations of high-amplitude mountain-wave activity. We also show that mountain-wave PSC climatology data and Mountain Wave Forecast Model 2.0 (MWFM-2) raw hemispheric ray and grid box averaged hemispheric wave temperature amplitude hindcast data from the same time period are in agreement with the AVHRR data. Our results show that ice cloud formation in mountain waves cannot explain how at least three large scale NAT clouds were formed in the stratosphere in early December 1999.

MOUNTAIN WAVES↗

NASA NTRS1994

NDSC and the JPL Stratospheric Lidars

The Network for the Detection of Stratospheric Change (NDSC) is an international cooperation providing a set of high-quality, remote-sensing instruments at observing stations around the globe. A brief description of the NDSC and its goals is presented. Lidar has been selected as the NDSC instrument for measurements of stratospheric profiles of ozone, temperature, and aerosol. The Jet Propulsion Laboratory has developed and implemented two stratospheric lidar systems for NDSC. These are located at Table Mountain, California and at Mauna Loa, Hawaii. These systems, which utilize different absorption lidar, Rayleigh lidar, Raman lidar, and backscatter lidar, to measure ozone, temperature, and aerosol profiles in the stratosphere are briefly described. Examples of results obtained for both long-term and individual profiles are presented.

lidar↗

DOE OSTI2023

Estimating the Meridional Extent of Adiabatic Mixing in the Stratosphere Using Age-Of-Air

Wave-induced adiabatic mixing in the winter midlatitudes is one of the key processes impacting stratospheric transport. Understanding its strength and structure is vital to understanding the distribution of trace gases and their modulation under a changing climate. Age-of-air is often used to understand stratospheric transport, and this study proposes refinements to the vertical age gradient theory of Linz et al. (2021), https://doi.org/10.1029/2021JD035199. The theory assumes exchange of air between a well-mixed tropics and a well-mixed extratropics, separated by a transport barrier, quantifying the adiabatic mixing flux across the interface using age-based measures. These assumptions are re-evaluated and a refined framework that includes the effects of meridional tracer gradients is established to quantify the mixing flux. This is achieved, in part, by computing a circulation streamfunction in age-potential temperature coordinates to generate a complete distribution of parcel ages being mixed in the midlatitudes. The streamfunction quantifies the “true” age of parcels mixed between the tropics and the extratropics. Applying the revised theory to an idealized and a comprehensive climate model reveals that ignoring the meridional gradients in age leads to an underestimation of the wave-driven mixing flux. Stronger, and qualitatively similar fluxes are obtained in both models, especially in the lower-to-middle stratosphere. While the meridional span of adiabatic mixing in the two models exhibits some differences, they show that the deep tropical pipe, that is, latitudes equatorward of 15° barely mix with older midlatitude air. The novel age-potential temperature circulation can be used to quantify additional aspects of stratospheric transport.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2014

Modifications of the Quasi-biennial Oscillation by a Geoengineering Perturbation of the Stratospheric Aerosol Layer

This paper examines the impact of geoengineering via stratospheric sulfate aerosol on the quasi-biennial oscillation (QBO) using the NASA Goddard Earth Observing System (GEOS-5) Chemistry Climate Model. We performed four 30-year simulations with a continuous injection of sulfur dioxide on the equator at 0 degree longitude. The four simulations differ by the amount of sulfur dioxide injected (5Tg per year and 2.5 Tg per year) and the altitude of the injection (16km-25km and 22km-25km). We find that such an injection dramatically alters the quasi-biennial oscillation, prolonging the phase of easterly shear with respect to the control simulation. In the case of maximum perturbation, i.e. highest stratospheric aerosol burden, the lower tropical stratosphere is locked into a permanent westerly QBO phase. This locked QBO westerly phase is caused by the increased aerosol heating and associated warming in the tropical lower stratosphere.

Geoengineering↗

NASA NTRS2012

Satellite Detection of Orographic Gravity-wave Activity in the Winter Subtropical Stratosphere over Australia and Africa

Orographic gravity-wave (OGW) parameterizations in models produce waves over subtropical mountain ranges in Australia and Africa that propagate into the stratosphere during austral winter and deposit momentum, affecting weather and climate. Satellite sensors have measured stratospheric GWs for over a decade, yet find no evidence of these waves. So are parameterizations failing here? Here we argue that the short wavelengths of subtropical OGWs place them near or below the detection limits of satellite sensors. To test this hypothesis, we reanalyze nine years of stratospheric radiances from the Atmospheric Infrared Sounder (AIRS) on NASA's Aqua satellite during austral winter, applying new averaging techniques to maximize signal-to-noise and improve thresholds for OGW detection. Deep climatological enhancements in stratospheric OGW variance over specific mountain ranges in Australia and southern Africa are revealed for the first time, which exhibit temporal and vertical variations consistent with predicted OGW responses to varying background winds.

Australia and Africa↗

NASA NTRS2015

Solar Signals in CMIP-5 Simulations: The Stratospheric Pathway

The 11 year solar-cycle component of climate variability is assessed in historical simulations of models taken from the Coupled Model Intercomparison Project, phase 5 (CMIP-5). Multiple linear regression is applied to estimate the zonal temperature, wind and annular mode responses to a typical solar cycle, with a focus on both the stratosphere and the stratospheric influence on the surface over the period approximately 1850-2005. The analysis is performed on all CMIP-5 models but focuses on the 13 CMIP-5 models that resolve the stratosphere (high-top models) and compares the simulated solar cycle signature with reanalysis data. The 11 year solar cycle component of climate variability is found to be weaker in terms of magnitude and latitudinal gradient around the stratopause in the models than in the reanalysis. The peak in temperature in the lower equatorial stratosphere (approximately 70 hPa) reported in some studies is found in the models to depend on the length of the analysis period, with the last 30 years yielding the strongest response. A modification of the Polar Jet Oscillation (PJO) in response to the 11 year solar cycle is not robust across all models, but is more apparent in models with high spectral resolution in the short-wave region. The PJO evolution is slower in these models, leading to a stronger response during February, whereas observations indicate it to be weaker. In early winter, the magnitude of the modeled response is more consistent with observations when only data from 1979-2005 are considered. The observed North Pacific high-pressure surface response during the solar maximum is only simulated in some models, for which there are no distinguishing model characteristics. The lagged North Atlantic surface response is reproduced in both high- and low-top models, but is more prevalent in the former. In both cases, the magnitude of the response is generally lower than in observations.

stratosphere↗

NASA NTRS2020

The HadGEM3-GA7.1 radiative kernel: the importance of a well-resolved stratosphere

We present top-of-atmosphere and surface radiative kernels based on the atmospheric component (GA7.1) of the HadGEM3 general circulation model developed by the UK Met Office. We show that the utility of radiative kernels for forcing adjustments in idealised CO2 perturbation experiments is greatest where there is sufficiently high resolution in the stratosphere in both the target climate model and the radiative kernel. This is because stratospheric cooling to a CO2 perturbation continues to increase with height, and low-resolution or low-top kernels or climate model output are unable to fully resolve the full stratospheric temperature adjustment. In the sixth phase of the Coupled Model Intercomparison Project (CMIP6), standard atmospheric model data are available up to 1 hPa on 19 pressure levels, which is a substantial advantage compared to CMIP5. We show in the IPSL-CM6A-LR model where a full set of climate diagnostics are available that the HadGEM3-GA7.1 kernel exhibits linear behaviour and the residual error term is small, as well as from a survey of kernels available in the literature that in general low-top radiative kernels underestimate the stratospheric temperature response. The HadGEM3-GA7.1 radiative kernels are available at https://doi.org/10.5281/zenodo.3594673 (Smith, 2019).

radiative kernels↗

NASA NTRS2021

The MJO-QBO Relationship in a GCM with Stratospheric Nudging

Observational studies show a strong connection between the intraseasonal Madden-Julian oscillation (MJO) and the stratospheric quasi-biennial oscillation (QBO): the boreal winter MJO is stronger, more predictable, and has different teleconnections when the QBO in the lower stratosphere is easterly versus westerly. Despite the strength of the observed connection, global climate models do not produce an MJO-QBO link. Here the authors use a current-generation ocean-atmosphere coupled NASA Goddard Institute for Space Studies global climate model (Model E2.1) to examine the MJO-QBO link. To represent the QBO with minimal bias, the model zonal mean stratospheric zonal and meridional winds are relaxed to reanalysis fields from 1980-2017. The model troposphere, including the MJO, is allowed to freely evolve. The model with stratospheric nudging captures QBO signals well, including QBO temperature anomalies. However, an ensemble of nudged simulations still lacks an MJO-QBO connection.

Madden-Julian oscillation (MJO)↗

NASA NTRS2021

Near-Global Variability of Stratospheric Water Vapor Observed by SAGE III/ISS

The Stratospheric Aerosol and Gas Experiment III instrument on the International Space Station (SAGE III/ISS) has been making high quality solar occultation measurements of stratospheric water vapor since June 2017. Here we evaluate the large-scale geophysical variability of the SAGE III/ISS water vapor measurements for the first 3 years of observations (2017–2020) as part of data validation for retrieval version 5.1 (v5.1). Detailed comparisons of SAGE III/ISS v5.1 with the Aura Microwave Limb Sounder (MLS) version 5 retrievals show overall excellent agreement in terms of seasonal mean structure and large-scale variability. SAGE III/ISS data capture the well-known seasonal variations in water vapor including the vertically propagating “tape recorder” in the tropics and lower stratospheric maxima linked to the NH summer monsoons. The high vertical resolution (∼2 km) measurements from SAGE III/ISS demonstrate contributions of the monsoons to the wet phase of “tape recorder” during the Northern Hemisphere (NH) summer. Interannual variations over the short data record are also consistent between SAGE III/ISS and MLS in the stratosphere between 16 and 30 km. We furthermore evaluate large-scale variations in relative humidity (RH) derived from the high vertical resolution SAGE III/ISS water vapor measurements, highlighting the detailed seasonal behavior and links to thermal structure near the tropical tropopause. Spatial distributions of RH at the cold point tropopause (CPT) show a close link between high RH and the minimum CPT temperature in both the NH winter and summer, consistent with temperature control of water vapor near the tropopause.

water vapor↗