Development of a Portable Pixelated Fast-Neutron Imaging Panel
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Results from the Advanced Scintillator Compton Telescope (ASCOT) Balloon Payload
The Advanced Scintillator Compton Telescope (ASCOT) is a medium-energy gamma-ray Compton telescope flown on NASA’s high-altitude scientific balloon from Palestine, TX on 5th July 2018. It uses commercially available highperformance scintillators like Cerium Bromide (CeBr3) and p-terphenyl along with compact readout devices - silicon photomultipliers (SiPMs) - for an improved instrument response. ASCOT was built to address the existing need for observations in the gamma-ray energy range of 0.4 - 20 MeV. Operating stably throughout the mission, it reached an altitude of 120,000 ft and observed the Crab Nebula at MeV energies for ~5 hours. Built on the legacy of COMPTEL (onboard CGRO), along with the hardware advancement ASCOT also makes use of the Time-of-Flight (ToF) background rejection technique for effective imaging. Presented here is the Energy and ToF calibrated flight data with optimal data cuts (Earth Horizon Cut, Pulse Shape Discrimination Cut). The growth curves generated using this data from 5 to 100 g/cm2 of residual atmosphere in conjunction with the Monte Carlo simulations of the instrument response have been used to obtain the Cosmic Diffuse Gamma-ray (CDG) flux value of (1.28 ± 0.37)×10 -5 photons/cm 2 /s/sr/keV for 0.4 – 0.7 MeV energy range. The 3σ upper limit for CDG flux is 1.8×10-5 photons/cm 2 /s/sr/keV for 0.7-1.5 MeV and 2×10-6 photons/cm2/s/sr/keV for 1.5-2.5 MeV. The analysis of the Crab Nebula from flight observation is underway
79 ASTRONOMY AND ASTROPHYSICS↗
A highly efficient, 10-J output signal amplifier for ultra-intense all-OPCPA systems
Optical parametric chirped-pulse amplification (OPCPA) using high-energy Nd:glass lasers has the potential to produce ultra-intense pulses (>10 23 W/cm 2 ). We report on the performance of the final high-efficiency amplifier in an OPCPA system based on large-aperture (63 x 63-mm 2 ) partially deuterated potassium dihydrogen phosphate (DKDP) crystals. Here, the seed beam (170 nm, 240 mJ) was provided by the preceding OPCPA stages. The maximum pump-to-signal conversion efficiency of 37% was achieved with a 52-mm-long DKDP crystal and 40-J pump energy at 527 nm due to the flattop super-Gaussian pump beam profile and flat-in-time pulse shape. The 11.8-J output signal was compressed to 19 fs.
42 ENGINEERING↗
Characterization of ablator dynamics initiated by picket-pulse conditions
Direct-drive laser-fusion targets may include low-cost plastic ablator material. Here, this work describes a tabletop experimental system designed to enable the investigation of the interaction of such ablator material as a function of the laser wavelength and the associated excitation mechanism. This experimental system offers time-resolved imaging of the material response with subpicosecond temporal resolution and ≈1-μm spatial resolution. The system involves synchronized femtosecond and picosecond lasers to initiate and characterize the dynamics of polystyrene planar targets irradiated by conditions similar to a “picket” prepulse from a direct-drive pulse shape. Ultrafast imaging of the initial excitation process followed by the resulting critical plasma formation, shock-wave propagation, and blowoff plasma expansion is used to compare the impact of excitation wavelength, 355 nm or 266 nm, on the ensuing dynamics. This work aims to investigate fundamental laser material interactions to help advance physics models that can inform the development of laser driver and target designs.
42 ENGINEERING↗
Characterization of the correlated background for a sterile neutrino search using the first dataset of the JSNS$^2$ experiment
JSNS 2 (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment that is searching for sterile neutrinos via the observation of ν¯ μ → ν¯ e appearance oscillations using muon decay-at-rest neutrinos. Before dedicated data taking in the first-half of 2021, we performed a commissioning run for 10 days in June 2020. Using the data obtained in this commissioning run, in this paper, we present an estimate of the correlated background which imitates the ν¯ e signal in a sterile neutrino search. In addition, in order to demonstrate future prospects of the JSNS 2 experiment, possible pulse shape discrimination improvements towards reducing cosmic ray induced fast neutron background are described.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
The Double Chooz antineutrino detectors
This article describes the setup and performance of the near and far detectors in the Double Chooz experiment. The electron antineutrinos of the Chooz nuclear power plant were measured in two identically designed detectors with different average baselines of about 400 m and 1050 m from the two reactor cores. Over many years of data taking the neutrino signals were extracted from interactions in the detectors with the goal of measuring a fundamental parameter in the context of neutrino oscillation, the mixing angle $\theta _{13}$. The central part of the Double Chooz detectors was a main detector comprising four cylindrical volumes filled with organic liquids. From the inside towards the outside there were volumes containing gadolinium-loaded scintillator, gadolinium-free scintillator, a buffer oil and, optically separated, another liquid scintillator acting as veto system. Above this main detector an additional outer veto system using plastic scintillator strips was installed. The technologies developed in Double Chooz were inspiration for several other antineutrino detectors in the field. The detector design allowed implementation of efficient background rejection techniques including use of pulse shape information provided by the data acquisition system. The Double Chooz detectors featured remarkable stability, in particular for the detected photons, as well as high radiopurity of the detector components.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Dynamic wavelength control of laser pulse profiles at picosecond to nanosecond timescales
We report on a novel combined laser pulse shaping and dynamic wavelength encoding capability based on a simple architecture implementing direct space to time mapping. There are several potential applications that can be enabled by the ability to control the instantaneous intensity or wavelength of an optical waveform on a picosecond-to-nanosecond timescale. To our knowledge, no known methods can access this temporal regime with a practical architecture. Here, we demonstrate an extension of the Space–Time Induced Linearly Encoded Transcription for Temporal Optimization (STILETTO) technique that can generate optical waveforms with a programmable instantaneous wavelength vs. time. We experimentally demonstrate the technique by generating self-gated spectrograms and show that it can encode dynamic wavelength vs time profiles at timescales not achievable by any other known method.
47 OTHER INSTRUMENTATION↗
Final amplifier of an ultra-intense all-OPCPA system with 13-J output signal energy and 41% pump-to-signal conversion efficiency
Optical parametric chirped-pulse amplification (OPCPA) using high-energy Nd:glass lasers has the potential to produce ultra-intense pulses (>10 23 W/cm 2 ). We report on the performance of the final high-efficiency amplifier in an OPCPA system based on large-aperture (63 × 63-mm 2 ) partially deuterated potassium dihydrogen phosphate (DKDP) crystals. The seed beam (180-nm bandwidth, 110 mJ) was provided by the preceding OPCPA stages. A maximum pump-to-signal conversion efficiency of 41% and signal energy up to 13 J were achieved with a 52-mm-long DKDP crystal due to the flattop super-Gaussian pump beam profile and flat-in-time pulse shape.
47 OTHER INSTRUMENTATION↗
Efficient general method for numerically modeling laser pulse propagation, overlap, and lifetime effects in amplifiers
An efficient numerical time-dependent general method is developed to address incoherent pulse overlap and lifetime effects in laser amplifiers. The alternating propagation-population laser energetics method (APPLE) has been validated against a semi-discrete coupled rate equation numerical method (SDRE) and analytic formalisms in bounding cases. APPLE is based on decoupled rates applied to a time-dependent framework where both space-time-dependent populations and pulse energetics are consistently updated in each time step. A significant advantage of APPLE lies in its conceptual simplicity, ease of implementation, and relatively small computational cost. SDRE tracks the populations through coupled rates and uses the method of lines to discretize the hyperbolic partial differential transport equations allowing for use of ordinary differential equation solvers. With reasonably sized mesh, we report both energetic and power pulse shape relative differences on the order of one percent between the models over a large range of initial conditions.
47 OTHER INSTRUMENTATION↗
Programmable, direct space-to-time picosecond resolution pulse shaper with nanosecond record
In this work, we demonstrate a novel, to the best of our knowledge, extension of optical arbitrary waveform generation capable of picosecond resolution over nanosecond duration. The method, called space–time induced linearly encoded transcription for temporal optimization, is based on direct space-to-time pulse shaping and is extended here to single-mode output with a programmable temporal profile. We develop the theory of operation and discuss ultimate limits on resolution, record length, and efficiency. We report on the results of an experimental demonstration showing ~1ps resolution over 600 ps.
42 ENGINEERING↗
Replacing photomultiplier tubes with silicon photomultipliers for nuclear safeguards applications
Photomultiplier tubes (PMTs) have been used for decades as the default light detection technology for scintillator-based radiation monitors. PMTs come with a handful of disadvantages, however, including large volume usage, fragility, high-voltage requirements, and susceptibility to magnetic fields. Arrays of silicon photomultipliers (SiPMs) are a possible alternative to PMTs providing similar performance while offering improvements in the areas listed. We focus on straightforward “drop-in replacement” evaluations by imposing a single channel output of the SiPM signal and a backend electronics data acquisition and analysis routine identical to that used for PMTs. In the realm of nuclear safeguards, the primary performance metric for gamma spectroscopy is detector resolution, and for neutron detection it is pulse shape discrimination (PSD) to separate neutron and gamma signals. In this work we present the results of replacing a PMT with a 2” x 2” SiPM array mounted, in turn, to the same 2” x 2” cylindrical sodium iodide (NaI) crystal. The ultimate comparison for this gamma spectrometry is confirmation of uranium enrichment standards, ranging from depleted uranium to 93% highly enriched uranium (HEU), by analyzing the resulting spectra with both a simple integral scaling in key energy regions of the spectrum, as well as with the NaIGEM software package. In addition to the gamma spectroscopy work, we will present the latest results on comparing the PSD capabilities of a 4” x 4” SiPM array to a 5” PMT. As with the gamma spectroscopy evaluations, the light detectors are mounted in turn to the same liter-scale organic scintillators. This neutron-focused work includes evaluation of prototype SiPM readout boards with a single output signal summed over 256 individual SiPM pixels, and evident tradeoffs between PSD capability and fast response.
42 ENGINEERING↗
Rossi Alpha Measurements – Rapid Organic (n, $\gamma$) Discrimination Detector (RAM-RODD) system capabilities
The Rossi Alpha Measurements–Rapid Organic (n, $\gamma$) Discrimination Detector (RAM-RODD) is an array organic scintillation detectors that has been optimized for use in neutron noise measurements. This report details the capability of the system including the method of energy calibration, pulse shape discrimination, and time resolution.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Exploring the Role of Viscosity in Inertial Confinement Fusion Implosions [Slides]
For one-component materials, adding pickets to the pulse shape did not affect the viscosity substantially. While Be seems to be most effective in dampening instabilities while Cr is the least effective. In MD-simulation of TCP, LAMMPS TCP input deck was successfully verified against OCP simulation, and we successfully calculated the viscosity of a CH TCP for a range of Γ values.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
Fast ignition inertial fusion energy using laser-driven ion beams
Ion fast ignition (IFI), or fusion fast ignition initiated by a laser-driven ion beam, is a promising path to high-gain inertial fusion energy (IFE). In IFI, cold, dense deuterium-tritium (DT) fuel is first assembled using lasers or pulsed power drivers. Then, a high-power ion beam is focused onto a small volume within the fuel (the hot spot), heating the fuel rapidly to conditions where fusion ignition takes place. Fusion burn in this hot spot propagates to the fuel surrounding the hot spot, leading to burnup of a significant fraction of this fuel and the possibility of high gain (G~100), as needed for inertial fusion energy. IFI uses separate drivers for the two basic elements, fuel compression and ignition, allowing maximum control and optimization of each. On the other hand, conventional laser fusion uses multiple beams of the same driver to compress the fuel and shock-heat its very center to ignite a burn wave. Despite impressive progress in conventional laser fusion, the precise spatial symmetry, temporal pulse shaping and timing required for high gain and IFE remain a serious unmet challenge.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
System Response Characterization for a d–t Neutron Radiography System
We report the system response of a pixelated associated particle imaging (API) neutron radiography system. The detector readout currently consists of a 2x2 array of organic glass scintillator detectors, each with an 8x8 array of optically isolated pixels that match the size and pitch of the ARRAYJ-60035-64P-PCB Silicon Photomultiplier (SiPM) array from SensL/onsemi with 6x6 mm 2 SiPMs. The alpha screen of the API deuterium-tritium neutron generator is read out with the S13361-3050AE-08 from Hamamatsu, which is an 8x8 array of 3x3 mm 2 SiPMs. Data from the 320 channel system is acquired with the TOFPET2-based readout system. We present the predicted imaging capability of an eventual 5x5 detector array, the waveform-based energy and pulse shape characterization of the individual detectors, and the timing and energy response from the TOFPET2 system.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Verification of Spent Fuel Inside Dry Storage Casks by Cask Top Fast Neutron Mapping (FY2023 Mid-Year Report)
This project is developing a prototype scanner array verification system for detection of missing fuel assemblies in spent-fuel storage casks. The prototype consists of six fast-neutron scintillator detectors mounted to a linear actuator frame that is placed on the top of a spent fuel cask to scan across all fuel assembly positions. The scanner array was assembled and tested at LLNL in FY2022. A field test schedule has been requested at the Idaho National Laboratory (INL) Cask Farm site for FY2023. Note that the Cask Farm contractor determines this scheduling and not INL directly. Further system automation will be designed and implemented with the goal of obtaining a level of system operation that meets IAEA needs. This includes integration of the scanner array and data-acquisition control software into a single interface for operator use. In addition, commercial operators and the IAEA may have special requirements for portability, shipping, lifting, and installation. Prior to the Field Test at INL, the system will be operated at LLNL to exercise lifting procedure and linear actuators, monitor stability of detector energy and pulse-shape discrimination calibration, and test system software integration efforts. Following the Field Test, we will present results and discuss the technology with the IAEA. We will incorporate additional improvements to the system based on lessons learned from the field test and feedback from the IAEA. If successful, the technology can be transferred to the IAEA or other stakeholders for assessment.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Hunting Sub-GeV Dark Matter with Diamonds and Magnetic Microcalorimeters Principle
This project is to study feasibility of a new concept for the sub-GeV dark matter (DM) detection using diamond crystals and magnetic microcalorimeters (MMCs). Diamond crystals are made of low mass carbon constituent that maximize kinetic energy of nuclear recoils from sub-GeV DM scattering due to their relatively similar masses. MMC is employed as a sensitive phonon sensor to measure athermal phonons that are produced by DM scattering in diamond crystals with 100 ns timing resolution and ~10 eV energy resolution. MMC’s fast timing resolution allows high precision phonon pulse shape analysis to separate out unwanted background or noise signals in the low energy region at E < 1 keV. Especially, the low energy excess (LEE) problems have been reported in the dark matter detection community and the proposed diamond-MMC detector might be able to provide important information to understand the origins of LEE signals in DM detectors. In this project a diamond-MMC detector has been built for proof-of-concept experiments and athermal phonon collection efficiencies have been investigated for single crystal and poly-crystal chemical-vapour-diamonds (SC and PC CVDs) as well as reference sapphire crystals are tested in the same geometries to quatify athermal phonon propagation and their collection to the MMC phonon sensors. Athermal phonon collection efficiencies and their lifetime in the diamond and sapphire crystals are successfully measured in the same geometry and experimental setup for comparison. SC CVD crystals exhibit poorer performance than the sapphire reference crystals in athermal phonon collection, while the PC CVD crystal exhibit better result than the sapphire. PC CVD with MMC phonon sensors would be feasible for sub GeV DM detection.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Quasi-Differential Neutron Scattering Measurements of 181 Ta and Teflon from 1.5 to 20 MeV [Slides]
This presentation covers motivation for the Experiments Performed. Secondly, it touches on upgrades to the Experimental Apparatus for Measurements. Thirdly, it presents quasi-Differential Experimental Methodology a) Pulse Shape Discrimination b) Validation Measurement of Carbon. The presentation concludes with Preliminary Results and Future Studies.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗