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NASA NTRS1992

Oriented Scintillation Spectrometer Experiment observations of Co-57 in SN 1987A

The Oriented Scintillation Spectrometer Experiment (OSSE) on the Compton Gamma Ray Observatory has observed SN 1987A for two 2 week periods during the first 9 months of the mission. Evidence for gamma-ray line and continuum emission from Co-57 is observed with an intensity of about 10 exp -4 gamma/sq cm/s. This photon flux between 50 and 136 keV is demonstrated by Monte Carlo calculations to be independent of the radial distribution of Co-57 for models of low optical depth, viz., models having photoelectric absorption losses of 122 keV photons no greater than several percent. For such models the observed Co-57 flux indicates that the ratio Ni-57/Ni-56 produced in the explosion was about 1.5 times the solar system ratio of Fe-57/Fe-56. When compared with nearly contemporaneous bolometric estimates of the luminosity for SN 1987A, our observations imply that Co-57 radioactivity does not account for most of the current luminosity of the supernova remnant in low optical depth models. We suggest alternatives, including a large optical depth model that is able to provide the SN 1987A luminosity and is consistent with the OSSE flux. It requires a 57/56 production ratio about twice solar.

Kurfess, J. D.↗

NASA NTRS1979

Scattering of emitted radiation from inhomogeneous and nonisothermal layers

A parametric study is performed for the exiting monochromatic intensities scattered from finite plane-parallel inhomogeneous layers that are driven solely by a distribution of thermal sources. Intensities are obtained by invariantly imbedding the standard and thermal scattering functions. The single-scattering albedo and the Henyey-Greenstein phase-function parameter are varied independently, and both linear and exponential profiles are considered. Linear temperature profiles are used, including temperature inversions. The resulting intensities, as a function of the direction cosine of propagation, are discussed from a remote-sensing point of view. For an isothermal and homogeneous medium, the gross characteristics of the exiting intensity, represented by its overall slope, mean value (magnitude), and an interior maximum value, can be related to the total optical depth, single-scattering albedo, and phase function, respectively. For a homogeneous medium, linearly decreasing (in the line of sight) temperature profiles tend to obscure the phase-function information and decrease the apparent optical depth. On the other hand, linearly increasing temperature profiles tend to retain phase-function information and increase the apparent optical depth. Temperature inversion profiles give intensities very similar to those for purely linear profiles.

Bergstrom, R. W.↗

NASA NTRS1991

Solar radiation on Mars: Update 1991

Detailed information on solar radiation characteristics on Mars are necessary for effective design of future planned solar energy systems operating on the surface of Mars. A procedure and solar radiation related data are presented from which the daily variation of the global, direct beam and diffuse insolation on Mars are calculated. Given the optical depth of the Mars atmosphere, the global radiation is calculated from the normalized net flux function based on multiple wavelength and multiple scattering of the solar radiation. The direct beam was derived from the optical depth using Beer's law, and the diffuse component was obtained from the difference of the global and the direct beam radiation. The optical depths of the Mars atmosphere were derived from images taken of the Sun with a special diode on the cameras used on the two Viking Landers.

Appelbaum, Joseph↗

NASA NTRS1980

Determination of the complex refractive index and size distribution of atmospheric particulates from bistatic-monostatic lidar and solar radiometer measurements

A method is presented for inferring both the size distribution and the complex refractive index of atmospheric particulates from combined bistatic-monostatic lidar and solar radiometer observations. The basic input measurements are spectral optical depths at several visible and near-infrared wavelengths as obtained with a solar radiometer and backscatter and angular scatter coefficients as obtained from a biostatic-monostatic lidar. The spectral optical depth measurements obtained from the radiometer are mathematically inverted to infer a columnar particulate size distribution. Advantage is taken of the fact that the shape of the size distribution obtained by inverting the particulate optical depth is relatively insensitive to the particle refractive index assumed in the inversion. Bistatic-monostatic angular scatter and backscatter lidar data are then processed to extract an optimum value for the particle refractive index subject to the constraint that the shape of the particulate size distribution be the same as that inferred from the solar radiometer data. Specifically, the scattering parameters obtained from the bistatic-monostatic lidar data are compared with corresponding theoretical computations made for various assumed refractive index values. That value which yields best agreement, in a weighted least squares sense, is selected as the optimal refractive index estimate. The results of this procedure applied to a set of simulated measurements as well as to measurements collected on two separate days are presented and discussed.

Reagan, J. A.↗

NASA NTRS1980

Photometry and polarimetry of Saturn's rings from Pioneer Saturn

A profile of the average normal optical depth for Saturn's rings between 1.22 and 2.35 Saturn radii is examined. In the A and B rings, horizontal inhomogeneities make these values deceptive. A thinner component of the B ring with an optical depth below 0.08 covers up to 4% of its surface area. In the A ring, the more transparent component covers more than 7% of its area and has an optical depth greater than 0.10. These thinner parts of the rings would rarely be apparent from earth based observations. The particles of the C ring are larger than 15 microns and differ from those of the B and A rings. The C ring is either homogeneous with high albedo and forward scattering phase functions, or shows a gradient in albedo with distance from Saturn. Polarimetry of Saturn's ring provides only an upper limit (below 15%) which is consistent with ground-based predictions. Polarization in the outer A ring is negative.

Esposito, L. W.↗

NASA NTRS2004

Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic matter, and dust found for the ACE Asia aerosol are comparable to values estimated for ACE 1, Aerosols99, and INDOEX. Unique to the ACE Asia aerosol was the large mass fractions of dust, the dominance of dust in controlling the aerosol optical properties, and the interaction of dust with soot aerosol.

Quinn, P. K.↗

NASA NTRS1992

Atmospheric and surface temperatures and airborne dust amounts during late southern summer from Mariner 9 IRIS data

The temperature structure and dust loading of the Martian atmosphere are investigated using thermal emission spectra recorded in 1972 by the Mariner 9 infrared interferometer spectrometer (IRIS). The analysis focuses on a subset of data consisting of approximately 2400 spectra obtained near the end of the southern summer season (L(sub s) equal to 343 deg to 348 deg), after the global dust storm had largely abated and airborne dust amounts were subsiding to background values. Simultaneous retrieval of the vertical distribution of both atmospheric temperature and dust optical depth is accomplished through an iterative procedure which is performed on each individual spectrum. The atmospheric transmittances are calculated using a Voigt quasi-random band model, which includes absorption by CO2 and dust, but neglects the effects of multiple scattering. Vertical profiles of temperature and dust optical depth are obtained using modified algorithms. These profiles are used to construct global maps of temperature and dust optical depth as functions of latitude (+/- 90 deg), altitude (approximately 0-50 km), and local time of day.

Santee, M.↗

NASA NTRS2002

Validation of TOMS Aerosol Products using AERONET Observations

The Total Ozone Mapping Spectrometer (TOMS) aerosol algorithm uses measurements of radiances at two near UV channels in the range 331-380 nm to derive aerosol optical depth and single scattering albedo. Because of the low near UV surface albedo of all terrestrial surfaces (between 0.02 and 0.08), the TOMS algorithm has the capability of retrieving aerosol properties over the oceans and the continents. The Aerosol Robotic Network (AERONET) routinely derives spectral aerosol optical depth and single scattering albedo at a large number of sites around the globe. We have performed comparisons of both aerosol optical depth and single scattering albedo derived from TOMS and AERONET. In general, the TOMS aerosol products agree well with the ground-based observations, Results of this validation will be discussed.

Bhartia, P. K.↗

NASA NTRS2007

Spectral Absorption Properties of Atmospheric Aerosols

We have determined the solar spectral absorption optical depth of atmospheric aerosols for specific case studies during several field programs (three cases have been reported previously; two are new results). We combined airborne measurements of the solar net radiant flux density and the aerosol optical depth with a detailed radiative transfer model for all but one of the cases. The field programs (SAFARI 2000, ACE Asia, PRIDE, TARFOX, INTEX-A) contained aerosols representing the major absorbing aerosol types: pollution, biomass burning, desert dust and mixtures. In all cases the spectral absorption optical depth decreases with wavelength and can be approximated with a power-law wavelength dependence (Absorption Angstrom Exponent or AAE). We compare our results with other recent spectral absorption measurements and attempt to briefly summarize the state of knowledge of aerosol absorption spectra in the atmosphere. We discuss the limitations in using the AAE for calculating the solar absorption. We also discuss the resulting spectral single scattering albedo for these cases.

Bergstrom, R. W.↗

NASA NTRS1986

The synchrotron-self-Compton process in spherical geometries. II - Application to active galactic nuclei

Observational implications and constraints on spherical nonthermal synchrotron self-Compton models with applications to AGNs are discussed. The Compton optical depth of the source and the synchrotron optical depth are considered, and plausible electron distributions are discussed. The alpha(0x), alpha(rx), and alpha(0r) system of comparing the fluxes in different energy bands is related to the nonthermal models, and sample spectra are presented that show the spectral features the models can produce. The models are applied to radio-quiet AGNs. It is shown that the infrared and X-ray continua of the AGNs can be produced by nonthermal processes.

Band, D. L.↗

NASA NTRS1992

Synchrotron emission from a cosmological jet as a model of gamma-ray bursts

The nonthermal rapidly varying spectra of gamma-ray bursts require relativistic beaming if the source is at a cosmological distance. Limits on the Lorentz factors and magnetic fields of extragalactic jet models of gamma-ray bursts are derived from the synchrotron source function, the position of the fundamental cyclotron resonance, the Thomson optical depth of radiating electrons, and the Thomson optical depth of electron-positron pairs created in photon-photon collisions of Compton upscattered radiation. The last of these constraints is the strongest, and it is satisfied by the observations if the jet's Lorentz factor is greater than 100. The limit from the position of the cyclotron fundamental requires a magnetic field strength below approximately 10 exp 10 G. Jet models producing observable cyclotron lines are allowed. The acceleration region in the burst must be separate from the emission region. The similarity of gamma-ray burst jet models to models of quasars and BL Lac objects suggest that if gamma-ray bursts are cosmological sources, they are a type of active galaxy.

Brainerd, J. J.↗

NASA NTRS1989

Theoretical studies of the infrared emission from circumstellar dust shells: the infrared characteristics of circumstellar silicates and the mass-loss rate of oxygen-rich late-type giants

We have modeled the infrared emission of spherically symmetric, circumstellar dust shells with the aim of deriving the infrared absorption properties of circumstellar silicate grains and the mass-loss rates of the central stars. As a basis for our numerical studies, a simple semianalytical formula has been derived that illustrates the essential characteristics of the infrared emission of such dust shells. A numerical radiative transfer program has been developed and applied to dust shells around oxygen-rich late-type giants. Free parameters in such models include the absorption properties and density distribution of the dust. An approximate, analytical expression is derived for the density distribution of circumstellar dust driven outward by radiation pressure from a central source. A large grid of models has been calculated to study the influence of the free parameters on the emergent spectrum. These results form the basis for a comparison with near-infrared observations. Observational studies have revealed a correlation between the near-infrared color temperature, Tc, and the strength of the 10 micrometers emission or absorption feature, A10. This relationship, which essentially measures the near-infrared optical depth in terms of the 10 micrometers optical depth, is discussed. Theoretical A10-Tc relations have been calculated and compared to the observations. The results show that this relation is a sensitive way to determine the ratio of the near-infrared to 10 micrometers absorption efficiency of circumstellar silicates. These results as well as previous studies show that the near-infrared absorption efficiency of circumstellar silicate grains is much higher than expected from terrestrial minerals. We suggest that this enhanced absorption is due to the presence of ferrous iron (Fe2+) color centers dissolved in the circumstellar silicates. By using the derived value for the ratio of the near-infrared to 10 micrometers absorption efficiency, the observed A10-Tc relation can be calibrated in terms of the total dust column density of the circumstellar shell and thus the mass-loss rate of late-type giants can easily be derived. Detailed models have been made of the infrared emission of three well-studied Miras: R Cas, IRC 10011, and OH 26.5+0.6, with the emphasis on the shape of the 10 micrometers emission or absorption feature. The results show that the intrinsic shape of the 10 micrometers resonance varies from a very broad feature in R Cas to a relatively narrower feature in OH 26.5+0.6, with IRC 10011 somewhere in between. Possible origins of this variation are discussed. The mass-loss rates from these objects are calculated to be 3 x 10(-7), 2 x 10(-5), and 2 x 10(-4) M Sun yr-1 for R Cas, IRC 10011, and OH 26.5+0.6, respectively. These results are compared to other determinations in the literature.

NASA Discipline Exobiology↗

NASA NTRS2014

Comparison of Marine Boundary Layer Cloud Properties from CERES-MODIS Edition 4 and DOE ARM AMF Measurements at the Azores

Marine boundary layer (MBL) cloud properties derived from the NASA Clouds and the Earth's Radiant Energy System (CERES) project using Terra and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data are compared with observations taken at the Department of Energy Atmospheric Radiation Measurement (ARM) Mobile Facility at the Azores (AMF-Azores) site from June 2009 through December 2010. Cloud properties derived from ARM ground-based observations were averaged over a 1 h interval centered at the satellite overpass time, while the CERES-MODIS (CM) results were averaged within a 30 km×30 km grid box centered over the Azores site. A total of 63 daytime and 92 nighttime single-layered overcast MBL cloud cases were selected from 19 months of ARM radar-lidar and satellite observations. The CM cloud top/base heights (Htop/Hbase) were determined from cloud top/base temperatures (Ttop/Tbase) using a regional boundary layer lapse rate method. For daytime comparisons, the CM-derived Htop (Hbase), on average, is 0.063 km (0.068 km) higher (lower) than its ARM radar-lidar-observed counterpart, and the CM-derived Ttop and Tbase are 0.9 K less and 2.5 K greater than the surface values with high correlations (R(sup 2) = 0.82 and 0.84, respectively). In general, the cloud top comparisons agree better than the cloud base comparisons, because the CM cloud base temperatures and heights are secondary products determined from cloud top temperatures and heights. No significant day-night difference was found in the analyses. The comparisons of MBL cloud microphysical properties reveal that when averaged over a 30 km× 30 km area, the CM-retrieved cloud droplet effective radius (re) at 3.7 micrometers is 1.3 micrometers larger than that from the ARM retrievals (12.8 micrometers), while the CM-retrieved cloud liquid water path (LWP) is 13.5 gm( exp -2) less than its ARM counterpart (114.2 gm( exp-2) due to its small optical depth (9.6 versus 13.7). The differences are reduced by 50% when the CM averages are computed only using the MODIS pixel nearest the AMF site. Using the effective radius retrieved using 2.1 micrometers channel to calculate LWP can reduce the difference between the CM and ARM microwave radiometer retrievals from 13.7 to 2.1 gm2. The 10% differences between the ARM and CERES-MODIS LWP and r(sub e) retrievals are within the uncertainties of the ARM LWP (approximately 20gm( exp -2)) and r(sub e) (approximately 10%) retrievals; however, the 30% difference in optical depth is significant. Possible reasons contributing to this discrepancy are increased sensitivities in optical depth from both surface retrievals when τ is approximately 10 and topography. The τ differences vary with wind direction and are consistent with the island orography.Much better agreement in τ is obtained when using only those data taken when the wind is from the northeast, where topographical effects on the sampled clouds are minimal.

Xi, Baike↗

NASA NTRS2019

Advances in Neural Network Detection and Retrieval of Multilayer Clouds for CERES Using Multispectral Satellite Data

An artificial neural network (ANN) algorithm, employing several Aqua MODIS infrared channels, the retrieved total cloud visible optical depth, and vertical humidity profiles is trained to detect multilayer (ML) ice-over-water cloud systems as identified by matched CloudSat and CALIPSO (CC) data. The multilayer ANN, or MLANN, algorithm is also trained to retrieve the optical depth and the top and base heights of the upper-layer ice clouds in ML systems. The trained MLANN was applied to independent MODIS data resulting in a combined ML and single layer hit rate of 80% (77%) for nonpolar regions during the day (night). The results are more accurate than currently available methods and the previous version of the MLANN. Upper-layer cloud top and base heights are accurate to ±1.2 km and ±1.6 km, respectively, while the uncertainty in optical depth is ±0.457 and ±0.556 during day and night, respectively. Areas of further improvement and development are identified and will be addressed in future versions of the MLANN.

CERES↗

NASA NTRS1992

Groundbased near-IR observations of the surface of Venus

We present images of the nightside of Venus taken in the near-infrared windows at 1.0, 1.1, 1.18, 1.28, 1.31, and 2.3 microns with the new infrared camera/spectrometer IRIS on the Anglo-Australian Telescope. These data were taken in spectral-mapping mode. This technique involves scanning the telescope perpendicular to the slit, while collecting spectra at successive slit positions across the planet. We produce data cubes with one spectral and two spatial dimensions. Images can be extracted over any wavelength regions. Each image has square pixels of 0.8 inch resolution. We reduced the scattered light from the sunlit crescent in images extracted from each window by subtracting images taken on either side of the window, where the Venus atmosphere is opaque. Unlike the short wavelength windows, which reveal thermal contrasts that originate primarily from the surface and deep atmosphere, the emission in the 2.3 microns window is produced at much higher altitudes (30-40 km). Emission contrasts seen near 2.3 microns are associated with horizontal variations in the cloud optical depths, and have rotation periods of about six days. We detect large contrasts in infrared emission (20-40 percent) across the disc of Venus in the 1.0-, 1.1-, 1.18-, 1.28-, and 1.31-micron images. Contrasts at these wavelengths may be due to a combination of variations in the optical depths of the overlying sulfuric acid clouds and differences in surface emission. Comparison with the 2.3-micron images show that the patterns seen in the 1.28- and 1.31-micron windows are consistent with cloud optical depth variations alone and require no contribution from the surface. However, images at 1.0, 1.1, and 1.8 microns from July 1991 show a dark feature having a contrast that increases with decreasing wavelength. This behavior is contrary to that expected of cloud absorption. Images taken on three successive days in October show another dark feature that is stationary with respect to the surface. These regions of lower emission correspond closely to the high-altitude surface regions of Beta Regio and Aphrodite Terra. The images can potentially reveal the near-infrared emissiveity of the surface of Venus, thereby complementing Magellan radar reflectivity and ground based radio emissivity measurements. The contrast ratio between highlands and plains is much smaller than would be expected for blackbody radiation from the surface along. Unlike at radio wavelengths, where the atmosphere is essentially transparent, at near-infrared wavelengths the atmosphere emits, absorbs, and scatters radiation, and can modify the observed topographically induced contrasts. The additional radiation from the atmosphere reduces the contrast, and further modification would be expected if terrain at different altitudes has different emissivities. A fit to our data therefore requires, and may constrain, a model of the lowest scale height of the atmosphere.

Meadows, V. S.↗

NASA NTRS2000

Methanogenesis, Mesospheric Clouds, and Global Habitability

Hyperthermophilic methanogens can exist in a deep hot biosphere up to 110 C, or 10 km deep. Methane (CH4) itself is thermodynamically stable to depths of 300 km. Geologic (microbial plus abiogenic thermal) methane is transported upward, attested to by its association with helium, to form petroleum pools. Near or at the surface, geologic CH4 mixes with other natural and with anthropogenic CH4 yielding annual emissions into the atmosphere of 500 Tg, of which 200 Tg are natural and 300 Tg are man-made. The atmospheric lifetime of CH4, a greenhouse gas 20 times more effective than CO2 in raising global temperatures, is approximately 10 years. It is removed from the atmosphere mainly by reactions with hydroxyl radical (OH) to form CO2, but also by dry soil and by conversion to H2O in the stratosphere and middle atmosphere. A sudden rise in atmospheric temperatures by 9-12 C some 55 million years ago has been explained by the release in a few thousand years of three trillion tons of CH4 out of 15 trillion tons that had formed beneath the sea floor. What prevented this CH4-induced greenhouse effect from running away? An analog to the CH4-burp of 55 million years ago is the CH4-doubling over the past century which resulted in a increase in upper level H2O from 4.3 ppmv to 6 ppmv. This 30% increase in H2O vapor yielded a tenfold increase in brightness of polar mesospheric clouds because of a strong dependence of the ice particle nucleation rate on the water saturation ratios. Models show that at a given temperature the optical depth of mesospheric clouds scales as [H2O]beta with beta varying between 4 and 8. Radiative transfer tools applied to mesospheric particles suggest that an optical depth of approximately one, or 1000 times the current mesospheric cloud optical depth, would result in tropospheric cooling of about 10 K. Assuming beta=6, a thousandfold increase in optical thickness would require a three-fold increase of H2O, or a 20-fold increase of CH4. At the current rate of anthropogenic emissions this is expected to occur within the next 1000 years. This timescale is also commensurate with what has been assumed for the CH4- burp 55 million years ago.

Pueschel, Rudolf F.↗

NASA NTRS1991

On the radial structure of Saturn's B ring

Voyager observations have revealed that the Saturnian B ring is much more structured than previously anticipated. Some of these structures occur on radial scale lengths of less than 15 km. In the visible the ring an optical depth minimum at a small distance outside of synchronous orbit. It is suggested in this paper that the electromagnetically induced radial transport of angular momentum associated with radial transport of charged submicron-size dust particles may explain these features. This mechanism induces an instability which produces, over geological times, significant radial structuring of the ring. Mass contained in particles less than about 1 cm in size is transported away from the synchronous orbit. This produces the optical depth minimum there. A simulation, starting with a radially uniform mass and number density, yields a radial optical depth profile which is similar to what is observed. It is found that it takes about 400-800 million yr to produce the observed structure. This estimate for the age of B ring agrees with some other independent estimates.

Shan, Lin-Hua↗

NASA NTRS2011

Combined Retrievals of Boreal Forest Fire Aerosol Properties with a Polarimeter and Lidar

Absorbing aerosols play an important, but uncertain, role in the global climate. Much of this uncertainty is due to a lack of adequate aerosol measurements. While great strides have been made in observational capability in the previous years and decades, it has become increasingly apparent that this development must continue. Scanning polarimeters have been designed to help resolve this issue by making accurate, multi-spectral, multi-angle polarized observations. This work involves the use of the Research Scanning Polarimeter (RSP). The RSP was designed as the airborne prototype for the Aerosol Polarimetery Sensor (APS), which was due to be launched as part of the (ultimately failed) NASA Glory mission. Field observations with the RSP, however, have established that simultaneous retrievals of aerosol absorption and vertical distribution over bright land surfaces are quite uncertain. We test a merger of RSP and High Spectral Resolution Lidar (HSRL) data with observations of boreal forest fire smoke, collected during the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS). During ARCTAS, the RSP and HSRL instruments were mounted on the same aircraft, and validation data were provided by instruments on an aircraft flying a coordinated flight pattern. We found that the lidar data did indeed improve aerosol retrievals using an optimal estimation method, although not primarily because of the constraints imposed on the aerosol vertical distribution. The more useful piece of information from the HSRL was the total column aerosol optical depth, which was used to select the initial value (optimization starting point) of the aerosol number concentration. When ground based sun photometer network climatologies of number concentration were used as an initial value, we found that roughly half of the retrievals had unrealistic sizes and imaginary indices, even though the retrieved spectral optical depths agreed within uncertainties to independent observations. The convergence to an unrealistic local minimum by the optimal estimator is related to the relatively low sensitivity to particles smaller than 0.1 ( m) at large optical thicknesses. Thus, optimization algorithms used for operational aerosol retrievals of the fine mode size distribution, when the total optical depth is large, will require initial values generated from table look-ups that exclude unrealistic size/complex index mixtures. External constraints from lidar on initial values used in the optimal estimation methods will also be valuable in reducing the likelihood of obtaining spurious retrievals.

Knobelspiesse, K.↗