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NASA NTRS2018

Retrieval of H2O Abundance in Titan's Stratosphere: A (Re)Analysis of CIRS/Cassini and PACS/Herschel Observations

Since its first measurement 20 years ago by the Infrared Space Observatory (ISO), the water (H2O) mole fraction in Titan’s stratosphere remains uncertain due to large differences between the determinations from available measurements. More particularly, the recent measurements made from the Herschel observatory (PACS (Photodetector Array Camera and Spectrometer) and HIFI (Heterodyne Instrument for the Far Infrared)) estimated the H2O mole fraction to be 0.023 parts per billion at 12.1 millibars. A mixing ratio of 0.14 parts per billion at 10.7 millibars was, however, retrieved from nadir spatially-resolved observations of Cassini/CIRS (Composite Infrared Spectrometer). At the same pressure level (10.7 millibars), this makes a difference of a factor of 5.5 between PACS and CIRS measurements, and this has notably prevented current models from fully constraining the oxygen flux flowing into Titan’s atmosphere. In this work, we try to understand the differences between the H2O mole fractions estimated from Herschel/PACS and Cassini/CIRS observations. The strategy for this is to 1) analyse recent disc-averaged observations of CIRS to investigate if the observation geometry could explain the previous observed differences, and 2) (re)analyse the three types of observation with the same retrieval scheme to assess if previous differences in retrieval codes/methodology could be responsible for the previous discrepancies. With this analysis, we show that using the same retrieval method better reconcile the previous measurements of these instruments. However, the addition of the disc-averaged CIRS observations, instead of confirming the consistency between the different datasets, reveals discrepancies between one of the CIRS disc-averaged set of observations and PACS measurements. This raises new questions regarding the possibility of latitudinal variations of H2O, which could be triggered by seasonal changes of the meridional circulation. As it has already been shown for nitriles and hydrocarbons, this circulation could potentially impact the latitudinal distribution of H2O through the subsidence or up- welling of air rich in H2O. The possible influence of spatial/time variations of the OH/H2O input flux in Titan’s atmosphere is also discussed. The analysis of more observations will be needed in future work to address the questions arising from this work and to improve the understanding of the sources of H2O in Titan’s atmosphere.

Bauduin, S.↗
NASA NTRS2019

The Effects of a 1998 Observing System Change on MERRA-2-Based Ozone Profile Simulations

Model simulations of ozone (O3) driven by meteorological reanalyses are useful for filling observational gaps and interpreting observed O3 variability and trends. However, the transport circulation of reanalysis products is impacted by changes to the observing system (the data assimilated into the reanalyses). We examine the impacts of these changes on simulated O3 from two models, Global Modeling Initiative (GMI) Chemistry Transport Model (GMI CTM) and Modern‐Era Retrospective Analysis for Research Applications version 2 (MERRA‐2) GMI Replay (M2 GMI Replay) simulation, using observations from global ozonesondes (>50,000 profiles) and satellites from 1980 to 2016. Both models are constrained by meteorology from the NASA MERRA‐2 reanalysis, and both use versions of NASA's GMI chemical mechanism. We focus on an observing system change affecting simulated O3 after 1998, associated with the assimilation of temperature and humidity data from new microwave profiling satellites. A large post‐1998 O3 increase, mainly confined to 15–20‐km altitude, of ~10 Dobson units (DU) in midlatitudes occurs in the GMI CTM, worsening the bias compared to observations. In contrast, an increase in M2 GMI Replay simulation O3 of ~10 DU is observed only near −60° latitude, reducing the bias compared to observations. The GMI CTM O3 high biases display a Quasi‐Biennial Oscillation (QBO)‐like periodicity that result from excessive transport from the tropical stratosphere to the midlatitude lower stratosphere during the QBO westerly phase. We quantify O3 discontinuities caused by MERRA‐2 observing system changes and demonstrate how the MERRA‐2 Global Modeling Initiative Replay simulation dampens the effects of these changes and QBO‐driven artifacts on simulated lower stratospheric and total O3. We caution against using simulations driven by a reanalysis to derive multidecadal O3 trends, especially prior to 1998.

Replay↗
NASA NTRS2019

Climatology of Transient Luminous Events and Lightning Observed Above Europe and the Mediterranean Sea

In 1999, the first sprites were observed above European thunderstorms using sensitive cameras. Since then, Eurosprite campaigns have been conducted to observe sprites and other transient luminous events (TLEs), expanding into a network covering large parts of Europe and coastal areas. In 2009 through 2013, the number of optical observations of TLEs reached a peak of 2000 per year. Because of this unprecedented number of European observations, it was possible to construct a climatology of 8394 TLEs observed above 1018 thunderstorm systems and study for the first time their distribution and seasonal cycle above Europe and parts of the Mediterranean Sea. The number of TLEs per thunderstorm was found to follow a power law, with less than 10 TLEs for 801 thunderstorms and up to 195 TLEs above the most prolific one. The majority of TLEs were classified as sprites, 641 elves, 280 halos, 70 upward lightning, 2 blue jets and 1 gigantic jet. The climatology shows intense TLE activity during summer over continental areas and in late autumn over coastal areas and sea. The two seasons peak, respectively, in August and November, separated by March and April with almost no TLEs, and a relative minimum around September. The observed TLE activity, i.e. mostly sprites, is shown to be largely consistent with lightning activity, with a 1/1000 of observed TLE-to-lightning ratio in regions with most observations. The overall behaviour is consistent among individual years, making the observed seasonal cycle a robust general feature of TLE activity above Europe.

Arnone, Enrico↗
NASA NTRS2020

Impact of Bias in the Marine Air Temperature Observation Set on Atmospheric Reanalyses

Marine air temperature observations are collected by volunteer observing ships carrying automatic meteorological sensor packages. Close proximity of the package mount to a dark colored ship's deck is known to introduce a warm bias on sunny afternoons in summer under low wind conditions. This observation set is used as an influential constraint in the MERRA-2 reanalysis, as well as several other reanalyses, in the poorly sampled surface marine boundary layer. Here we explore the consequences of bias in the marine air temperature observation set during the 36 year period 1980-2015. Marine air temperature observations have mainly been collected along major shipping routes, with the densest coverage in the North Atlantic and North Pacific. In the first part of this presentation we review the historical observation coverage and compare air temperature and contemporaneous SST measurements to identify systematic differences. The comparison suggests the presence of diurnal bias in the air temperature observations peaking in subtropics and midlatitudes latitudes in mid-afternoon local time. In the second part we explore the impact of the marine air temperature observations on MERRA-2 through analysis of the terms in the temperature forecast tendency equation, the equation which describes the contributions to changes in temperature during each analysis cycle. Examination of the temperature forecast tendency equation allows us to separate systematic errors due to such processes and radiation, mixing, and advection and allows us to identify the major source of systematic forecast tendencies. The results show that the marine air temperature measurements introduce an error that can reach 0.4K/dy which also peaks in local afternoon at subtropical latitudes. This bias varies with season and has gradually reduced from the beginning of the MERRA-2 reanalysis in 1980. In the final part we conduct numerical experiments with a version of the MERRA-2 analysis system, comparing experiments when the marine air temperature observations are included or withheld from the analysis system.

Akella, Santharam↗
NASA NTRS2021

The First Widespread Solar Energetic Particle Event Observed By Solar Orbiter on 2020 November 29

Context. On 2020 November 29, the first widespread solar energetic particle (SEP) event of solar cycle 25 was observed at four widely separated locations in the inner (. 1AU) heliosphere. Relativistic electrons as well as protons with energies > 50MeV were observed by Solar Orbiter (SolO), Parker Solar Probe (PSP), the Solar Terrestrial Relations Observatory (STEREO)-A and multiple near-Earth spacecraft. The SEP event was associated with an M4.4 class X-ray flare and accompanied by a coronal mass ejection (CME) and an extreme ultraviolet (EUV) wave as well as a type II radio burst and multiple type III radio bursts. Aims. We present multi-spacecraft particle observations and place them in context with source observations from remote sensing instruments and discuss how such observations may further our understanding of particle acceleration and transport in this widespread event. Methods. Velocity dispersion analysis (VDA) and time shift analysis (TSA) were used to infer the particle release times at the Sun. Solar wind plasma and magnetic field measurements were examined to identify structures that influence the properties of the energetic particles such as their intensity. Pitch angle distributions and first-order anisotropies were analyzed in order to characterize the particle propagation in the interplanetary medium. Results. We find that during the 2020 November 29 SEP event, particles spread over more than 230° in longitude close to 1AU. The particle onset delays observed at the different spacecraft are larger as the flare–footpoint angle increases and are consistent with those from previous STEREO observations. Comparing the timing when the EUV wave intersects the estimated magnetic footpoints of each spacecraft with particle release times from TSA and VDA, we conclude that a simple scenario where the particle release is only determined by the EUV wave propagation is unlikely for this event. Observations of anisotropic particle distributions at SolO, Wind, and STEREO-A do not rule out that particles are injected over a wide longitudinal range close to the Sun. However, the low values of the first-order anisotropy observed by near-Earth spacecraft suggest that diffusive propagation processes are likely involved.

A Kollhoff↗
NASA NTRSDate not supplied

Key Observations and Discoveries from the Vector Electric Field Investigation on the C/NOFS Satellite

Launched in 2008 and operating for 7.5 years, the Air Force Communication /Navigation Outage Forecasting System (C/NOFS) satellite included the Vector Electric Field Investigation (VEFI) designed and built at NASA’s Goddard Space Flight Center. VEFI successfully met its objectives: 1) investigate the role of ambient electric fields in initiating nighttime density depletions and turbulence; 2) determine the quasi-DC electric fields associated with abrupt density depletions, and 3) quantify the spectrum of the irregularities associated with density depletions, providing many key observations and discoveries including: -- Global (low latitude) vector DC electric fields at 16 s/sec revealing variations with local time, longitude, and season between extremely low and moderate solar activity-- Reversed zonal E x B drifts below the F-region ledge at sunset and simultaneous observations of large scale Kelvin-Helmholtz instabilities as seeds of spread-F -- Large expanses of quasi-coherent kilometer-scale vector wave observations (electric field and density) below 450 km and their discovery as a source of scintillations using the C/NOFS GPS -- Reversed zonal DC electric fields and simultaneous observations of afternoon counter electrojet-- Enhanced zonal DC electric fields at sunrise and full vector plasma flow continuity at the terminator-- Vector electric field and density irregularities extending to meter-scales within equatorial plasma depletions -- Intense electric field structure within the equatorial ionosphere at night in the absence of density depletions -- First observations of the westward equatorial electrojet in post-midnight ionosphere and possible association with downward meridional drifts-- Spaceborne Dst observations and implications for ring current asymmetries-- Vector electric and magnetic field Poynting flux within depletions and TIDs-- Measurements of ionospheric reflectance and Alfvenic waves associated with TIDs-- Observations of Alfven resonators -- ULF magnetic field structure within the nightime equatorial ionosphere-- Discovery of Schumman resonances in space and implications of ELF radiowave propagation-- Vector observations of 50-60 Hz powerline radiation without harmonics-- Ion cyclotron resonance absorption lines associated with ELF hiss and the identification of ambient ions-- Parallel electric fields associated with lower hybrid waves driven by thunderstorm lightning-related sferics-- Discovery of Z-mode radiation in the equatorial ionosphere including its associated with density depletions-- Optical lightning detector waveforms and electric field sferics observed up to altitudes of 800 km

Robert F Pfaff↗
NASA NTRSDate not supplied

Evaluation of TAO Observation System on ENSO Predictions from the GMAO S2S Forecast System

Since the early 1990’s, the Tropical Atmosphere Ocean (TAO) mooring array has been instrumental for observing Kelvin and Rossby wave propagation which is key for El Nino/Southern Oscillation (ENSO) prediction. However, recent funding and programmatical issues have highlighted the need to rigorously assess the impact of the TAO observing system on ENSO predictions. Therefore, we evaluate the TAO using data assimilation observation denial experiments (also known as Observing System Evaluation or OSE experiments). This presentation will evaluate the TAO observing impact on both reanalyses and prediction of the big 2015 El Nino. We have completed reanalyses for July 2014-Dec 2015 for both the CONTROL experiment (that assimilates all available data) and the NOTAO experiment (that is identical to the CONTROL but withholds all TAO observations) using the best available NASA GEOS-S2S V3 seasonal prediction system. Validation of these reanalyses shows that TAO assimilation generally improves comparisons of temperature and salinity versus gridded in situ observations. Temperature is universally improved above the thermocline near the equator, but the biggest improvement is found in the eastern Pacific, just below the thermocline, where the variation of the thermocline defines ENSO events. In addition, a surprising result is that even with relatively few observations, salinity is improved throughout the equatorial region except near 120oW near the surface. ENSO forecasts were performed that were initialized from these CONTROL and NOTAO reanalyses. For the 9-month forecasts which were initialized in January, July, and October 2015, the NINO3.4 SST shows that the CONTROL forecasts are warmer and closer to observations than the NOTAO forecasts. We will show that upwelling and shoaling of the mixed layer amplifies the ENSO signal due to TAO assimilation. Prior to (after) April 2015, this upwelling is caused by relatively stronger Rossby (Kelvin) waves in the CONTROL than in the NOTAO experiments.

E. Hackert↗
NASA NTRSDate not supplied

Leveraging Observing System Simulation Experiments for Satellite Instrument Design: Advancements and Challenges

This abstract highlights NASA's OSSE framework, developed at the Global Modeling and Assimilation Office, which has become a widely adopted tool for evaluating the impact of new observations on weather forecasts. The framework involves simulating realistic observations by introducing errors to mimic real-world scenarios. By utilizing advanced radiative transfer modeling, the accuracy of simulated observations is significantly improved, enhancing the reliability of experimental outcomes. The talk focuses on recent progress and challenges in three key areas. Firstly, it explores the techniques used to simulate synthetic observations, a crucial aspect of OSSE experiments. Secondly, the presentation also discusses the challenges of examining the observation errors that need to be added to the perfect observations to generate realistic simulated observations. Lastly, the assimilation of synthetic observations and their impact on forecast skills is evaluated, providing valuable insights for optimizing current and future observing systems for improving the weather forecasts. By sharing recent advancements and acknowledging challenges, this presentation seeks to inspire researchers to leverage the OSSE framework in weather forecasting. NASA's OSSE techniques hold promise for a better understanding of the atmosphere and the development of more accurate and reliable weather predictions.

Isaac Moradi↗
NASA NTRSDate not supplied

The Impact of Assimilating Large Volumes of GNSS Radio Occultation Observations from Spire’s Commercial Constellation into NASA’s GEOS

The upcoming retrospective analysis for the 21st century (R21C) reanalysis product from NASA will include the full dataset of GNSS Radio Occultation (RO) observations collected by Spire with their constellation of smallsats. The Spire RO dataset, which was purchased by NASA for its Commercial Smallsat Data Acquisition (CSDA) archive, has global coverage and includes approximately 6 thousand RO profiles per day during 2019 increasing to nearly 20 thousand in 2022-2023. This more than doubles the volume of RO profiles from all other routinely assimilated RO missions combined during 2023. The increase in the number of RO profiles available is particularly important in the extratropics as the next largest RO constellation, the state-of-the-science Formosa Satellite Mission 7 (FORMOSAT-7)/Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC-2) mission (hereafter COSMIC-2), is focused on the Tropics and only provides approximately 4 thousand RO profiles per day. The large number of observations in the Spire RO dataset have great potential to improve analyses and forecasts of the Earth’s atmosphere produced by numerical weather prediction systems. Their impact is assessed through numerical experiments using NASA’s Global Earth Observing System (GEOS) Atmospheric Data Assimilation System (ADAS) with and without the observations from the COSMIC-2 mission. The ability of the Spire RO observations to make up for the omission of the RO observations from COSMIC-2 is directly assessed over the tropics and the impact of Spire over the extratropics is compared to that of the available RO missions that sample over this region. Finally, the quality of the Spire RO observations is compared to that of the routinely assimilated RO missions using Forecast Sensitivity-based Observation Impact (FSOI).

Michael J. Murphy↗
NASA NTRSDate not supplied

The Impact of Assimilating Large Volumes of GNSS Radio Occultation Observations from Spire’s Commercial Constellation into NASA’s GEOS

The upcoming retrospective analysis for the 21st century (R21C) reanalysis product from NASA will include the full dataset of GNSS Radio Occultation (RO) observations collected by Spire with their constellation of smallsats. The Spire RO dataset, which was purchased by NASA for its Commercial Smallsat Data Acquisition (CSDA) archive, has global coverage and increases in number from approximately 6 thousand RO profiles per day during 2019 to approximately 20 thousand in 2022-2023. This more than doubles the volume of RO profiles from all other routinely assimilated RO missions combined during 2022. The increase in the number of RO profiles available is particularly important in the extratropics as the next largest RO constellation, the state-of-the-science Formosa Satellite Mission 7 (FORMOSAT-7)/Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC-2) mission (hereafter COSMIC-2), is focused on the Tropics and only provides approximately 4 thousand RO profiles per day. The large number of observations in the Spire RO dataset have great potential to improve analyses and forecasts of the Earth’s atmosphere produced by numerical weather prediction systems. Their impact is assessed through numerical experiments using NASA’s Global Earth Observing System (GEOS) Atmospheric Data Assimilation System (ADAS) with and without the observations from the COSMIC-2 mission. The ability of the Spire RO observations to make up for the omission of the RO observations from COSMIC-2 is directly assessed over the tropics and the impact of Spire over the extratropics is compared to that of the available RO missions that sample over this region. Finally, the quality of the Spire RO observations is compared to that of the routinely assimilated RO missions using Forecast Sensitivity-based Observation Impact (FSOI).

Michael J. Murphy↗
NASA NTRS2023

Robustness of Observing System Simulation Experiments

Observing System Simulation Experiments (OSSEs) are used to investigate the potential performance of proposed new instruments on numerical weather prediction (NWP). As OSSEs involve a framework in which the atmosphere and observations are all completely simulated, it is necessary to perform validation of the OSSE to ensure that it is sufficiently realistic to provide useful experimental results. A common issue that affects the forecast skill and observation impacts is the tendency of OSSEs to have insufficient model error compared to NWP in the real world. In this work, two versions of the National Aeronautics and Space Administration Global Modeling and Assimilation Office (NASA/GMAO) NWP OSSE framework are compared, with the newer framework having more simulated forecast model error than the older framework due to changes to the NWP system. The performance of the updated OSSE is validated against corresponding behavior of the same NWP system in the real world in terms of the simulated observations, the analysis increments, forecast error, and observation impacts. OSSE results of analysis and forecast impacts for three proposed new observation systems are also compared between the older and newer frameworks to evaluate the robustness of the OSSE experiments and the role of model error in observation impacts. These three new instruments are the Geostationary eXtended Observations (GeoXO) hyperspectral infrared sounder (GXS), the Midwave Infrared Sounding of Temperature and humidity in a Constellation for Winds (MISTiC Winds) atmospheric motion vectors, and additional Global Navigation Satellite System Radio Occultations (GNSS-RO).

Observing System Simulation Experiments↗
DOE OSTI2024

Early photometric and spectroscopic observations of the extraordinarily bright INTEGRAL-detected GRB 221009A

Context. GRB 221009A, initially detected as an X-ray transient by Swift, was later revealed to have triggered the Fermi satellite about an hour earlier, marking it as a post-peak observation of the event’s emission. This GRB distinguished itself as the brightest ever recorded, presenting an unparalleled opportunity to probe the complexities of GRB physics. The unprecedented brightness, however, challenged observation efforts, as it led to the saturation of several high-energy instruments.Aims. Our study seeks to investigate the nature of the INTEGRAL-detected GRB 221009A and elucidate the environmental conditions conducive to these exceptionally powerful bursts. Moreover, we aim to understand the fundamental physics illuminated by the detection of teraelectronvolt (TeV) photons emitted by GRB 221009A.Methods. We conducted detailed analyses of early photometric and spectroscopic observations that span from the Fermi trigger through to the initial days following the prompt emission phase in order to characterize GRB 221009A’s afterglow, and we complemented these analyses with a comparative study.Results. Our findings from analyzing INTEGRAL data confirm GRB 221009A as the most energetic event observed to date. Early optical observations during the prompt phase negate the presence of bright optical emissions with internal or external shock origins. Spectroscopic analyses enabled us to measure GRB 221009A’s distance and line-of-sight properties. The afterglow’s temporal and spectral analysis suggests prolonged activity of the central engine and a transition in the circumburst medium’s density. Finally, we discuss the implications for fundamental physics of detecting photons as energetic as 18 TeV from GRB 221009A.Conclusions. Early optical observations have proven invaluable for distinguishing between the potential origins of optical emissions in GRB 221009A, underscoring their utility in GRB physics studies. However, the rarity of such data underscores the need for dedicated telescopes capable of synchronous multiwavelength observations. Additionally, our analysis suggests that the host galaxies of TeV GRBs share commonalities with those of long and short GRBs. Expanding the sample of TeV GRBs could further solidify these findings.Key words: techniques: photometric / techniques: spectroscopic / gamma-ray burst: general / gamma-ray burst: individual: GRB 221009A

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Limitations of Bin and Bulk Microphysics in Reproducing the Observed Spatial Structure of Light Precipitation

Abstract Coarse-gridded atmospheric models often account for subgrid-scale variability by specifying probability distribution functions (PDFs) of process rate inputs such as cloud and rainwater mixing ratios ( q c and q r , respectively). PDF parameters can be obtained from numerous sources: in situ observations, ground- or space-based remote sensing, or fine-scale modeling such as large-eddy simulation (LES). LES is appealing to constrain PDFs because it generates large sample sizes, can simulate a variety of cloud regimes/case studies, and is not subject to the ambiguities of observations. However, despite the appeal of using model output for parameterization development, it has not been demonstrated that LES satisfactorily reproduces the observed spatial structure of microphysical fields. In this study, the structure of observed and modeled microphysical fields are compared by applying bifractal analysis, an approach that quantifies variability across spatial scales, to simulations of a drizzling stratocumulus field that span a range of domain sizes, drop concentrations (a proxy for mesoscale organization), and microphysics schemes (bulk and bin). Simulated q c closely matches observed estimates of bifractal parameters that measure smoothness and intermittency. There are major discrepancies between observed and simulated q r properties, though, with bulk simulated q r consistently displaying the bifractal properties of observed clouds (smooth, minimally intermittent) rather than rain while bin simulations produce q r that is appropriately intermittent but too smooth. These results suggest fundamental limitations of bulk and bin schemes to realistically represent higher-order statistics of the observed rain structure.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2013

On the Reprocessing and Reanalysis of Observations for Climate

The long observational record is critical to our understanding of the Earths climate, but most observing systems were not developed with a climate objective in mind. As a result, tremendous efforts have gone into assessing and reprocessing the data records to improve their usefulness in climate studies. The purpose of this paper is to both review recent progress in reprocessing and reanalyzing observations, and to summarize the challenges that must be overcome in order to improve our understanding of climate and variability. Reprocessing improves data quality through more scrutiny and improved retrieval techniques for individual observing systems, while reanalysis merges many disparate observations with models through data assimilation, yet both aim to provide an climatology of Earth processes. Many challenges remain, such as tracking the improvement of processing algorithms and limited spatial coverage. Reanalyses have fostered significant research, yet reliable global trends in many physical fields are not yet attainable, despite significant advances in data assimilation and numerical modeling. Oceanic reanalyses have made significant advances in recent years, but will only be discussed here in terms of progress toward integrated Earth system analyses. Climate data sets are generally adequate for process studies and large-scale climate variability. Communication of the strengths, limitations and uncertainties of reprocessed observations and reanalysis data, not only among the community of developers, but also with the extended research community, including the new generations of researchers and the decision makers is crucial for further advancement of the observational data records. It must be emphasized that careful investigation of the data and processing methods are required to use the observations appropriately.

Uncertainty↗
NASA NTRS2016

MERRA-2 Input Observations: Summary and Assessment

The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2) is an atmospheric reanalysis, spanning 1980 through near-realtime, that uses state-of-the-art processing of observations from the continually evolving global observing system. The effectiveness of any reanalysis is a function not only of the input observations themselves, but also of how the observations are handled in the assimilation procedure. Relevant issues to consider include, but are not limited to, data selection, data preprocessing, quality control, bias correction procedures, and blacklisting. As the assimilation algorithm and earth system models are fundamentally fixed in a reanalysis, it is often a change in the character of the observations, and their feedbacks on the system, that cause changes in the character of the reanalysis. It is therefore important to provide documentation of the observing system so that its discontinuities and transitions can be readily linked to discontinuities seen in the gridded atmospheric fields of the reanalysis. With this in mind, this document provides an exhaustive list of the input observations, the context under which they are assimilated, and an initial assessment of selected core observations fundamental to the reanalysis.

Satellite Observations↗
NASA NTRS2019

Evaluating Models' Response of Tropical Low Clouds to SST Forcings Using CALIPSO Observations

Recent studies have shown that, in response to a surface warming, the marine tropical low-cloud cover (LCC) as observed by passive-sensor satellites substantially decreases, therefore generating a smaller negative value of the top-of-the-atmosphere (TOA) cloud radiative effect (CRE). Here we study the LCC and CRE interannual changes in response to sea surface temperature (SST) forcings in the GISS model E2 climate model, a developmental version of the GISS model E3 climate model, and in 12 other climate models, as a function of their ability to represent the vertical structure of the cloud response to SST change against 10 years of CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) observations. The more realistic models (those that satisfy the observational constraint) capture the observed interannual LCC change quite well ([delta]LCC]/[delta]SST= -3.49±1.01%K [negative 1 superscript] vs. [delta]LCC/[delta]SST[subscript obs]= -3.59±0.28%K[negative 1 superscript]) while the others largely underestimate it ([delta]LCC/[delta]SST= -1.32±1.28%K[negative 1 superscript]). Consequently, the more realistic models simulate more positive shortwave (SW) feedback ([delta]CRE/[delta]SST=2.60±1.13Wm[negative 2 superscript] K[negative 1 superscript]) than the less realistic models (CRE/SST=0.87±2.63Wm2K1), in better agreement with the observations ([delta]CRE/[delta]SST[subscript obs]=3±0.26Wm[negative 2 superscript] K[negative 1 superscript] ), although slightly underestimated. The ability of the models to represent moist processes within the planetary boundary layer (PBL) and produce persistent stratocumulus (Sc) decks appears crucial to replicating the observed relationship between clouds, radiation and surface temperature. This relationship is different depending on the type of low clouds in the observations. Over stratocumulus regions, cloud-top height increases slightly with SST, accompanied by a large decrease in cloud fraction, whereas over trade cumulus (Cu) regions, cloud fraction decreases everywhere, to a smaller extent.

low clouds↗
DOE OSTI2023

High-dimensional isotomics, part 2: Observations of over 100 constraints on methionine's isotome

The abundances of different isotopic forms of a compound, or isotopologues, will vary based on its physical and chemical history. The number of isotopologues increases combinatorically with the size of a molecule, and even small molecules such as amino acids have thousands of potentially observable isotopic variants. However, due to the analytical challenges of separating and observing isotopologues, only a few dimensions of isotopic diversity are routinely measured. Overcoming these challenges requires both an experimental method to observe many isotopic properties and a theoretical framework for interpreting these experiments. In Part 1, we presented such a theoretical framework; here, we demonstrate an experimental method, which we apply to methionine. Our approach uses a Q Exactive HF Orbitrap to perform several “M + N experiments”, where a sample is ionized, a subset of its isotopologues with cardinal mass N daltons greater than the unsubstituted isotopologue is selected and fragmented, and the proportions of all detectable isotopic forms of those fragment ions are quantified. We perform M + 1, M + 2, M + 3, and M + 4 experiments of a methionine sample and standard where the sample has a 100 ‰ enrichment of 13C at the methyl carbon relative to the natural 13C abundance at that position in the standard, and is otherwise identical to the standard. We observe isotopic forms of 8 fragment ion species for each version of the M + N experiment. With the assistance of a forward model of expected mass spectra, we identify isotopic peaks for each fragment ion based on observed mass and abundance, screen these for data quality, and quantify abundances for 146 unique isotopic peaks at precisions of ≈ 0.3–3 ‰. We present our direct observations and use them to reconstruct the concentrations of 19 individual singly, doubly, and triply-substituted isotopologues; doing so gives fewer constraints and broader error bars than working with the direct observations, but may be more interpretable for some applications. We also examine possibilities for measuring additional peaks, which are primarily limited by the detection limit of the Orbitrap-IRMS method. We then suggest some possible uses of our direct measurements for chemical forensics and hypothesis testing. Furthermore, our results demonstrate the diversity of isotopic constraints currently observable and interpretable for organic molecules.

58 GEOSCIENCES↗
DOE OSTI2025

First observations of edge instabilities in strongly shaped negative triangularity plasmas on DIII-D

Throughout the 2023 DIII-D negative triangularity (NT) campaign, unexpected magnetic fluctuations indicative of an edge localized instability were observed in the majority of strongly shaped (–0.55 ≤ δ ≤ –0.45) discharges. Moreover, these same fluctuations were found to be absent in weaker NT plasma shapes. Based on a database study, three separate mode behaviors are observed based primarily on the edge safety factor and normalized plasma beta β N . The main regime is the bursty state, in which short (~5 ms) magnetic bursts occur every 5–10 ms. Each burst drives a small reduction in the edge electron temperature (T e ) as measured by electron cyclotron emissions (ECE), which then rapidly recovers between the bursts. The quiescent regime appears to have governing mechanics similar to the bursty regime, but with multiple unique mode signatures observed in the magnetics. These additional modes greatly reduce the bursty nature of the plasma. Finally, a saturated state is observed in a number of discharges, particularly at early time slices. The saturated regime is often short-lived (maximum 500 ms), but can have a large impact on the dynamics of the plasma edge region, causing significant drops in electron temperature as observed in the ECE diagnostic. 2D ECE imaging (ECE-I) is utilized, showing large kink-like perturbations localized near the last closed flux surface that extend into the SOL indicative of an external kink/peeling behavior. Additionally, evidence of phase mixing and observed tearing-parity perturbations localized near the edge rational surfaces is observed in the quiescent regime plasmas. As a result, the various modes do not appear to have a large impact on global confinement but may play a role in regulating the transport of the NT edge and the observed edge gradients.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗