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At least 397 records · Page 22

System and method for large-area pulsed laser melting of metallic powder in a laser powder bed fusion application

The present disclosure relates to systems and methods for performing large area laser powder bed fusion (LBPF) to form a plurality of layers of a 3D part in a layer-by-layer fashion using meltable powder particles. In one implementation the system makes use of a first light source, which may be a diode laser subsystem, for generating a first light pulse of a first duration. The first light is used to preheat a substrate underneath a new layer of powder particles, wherein the substrate is formed from a previously fused quantity of the powder particles. A second light source, which may be a pulse laser, generates a second light pulse subsequent to the first light pulse. The second light pulse has a second duration shorter than the first duration by a factor of at least about 10, and fully melts the new layer of powder particles in addition to the substrate, to achieve a smooth printed layer. The wavelength of the first light pulse also differs from a wavelength of the second light pulse.

Khairallah, Saad A.↗

A molecular dynamics study of laser-excited gold

The structural evolution of laser-excited systems of gold has previously been measured through ultrafast MeV electron diffraction. However, there has been a long-standing inability of atomistic simulations to provide a consistent picture of the melting process, leading to large discrepancies between the predicted threshold energy density for complete melting, as well as the transition between heterogeneous and homogeneous melting. We make use of two-temperature classical molecular dynamics simulations utilizing three highly successful interatomic potentials and reproduce electron diffraction data presented by Mo et al. [Science 360, 1451–1455 (2018)]. We recreate the experimental electron diffraction data, employing both a constant and temperature-dependent electron–ion equilibration rate. In all cases, we are able to match time-resolved electron diffraction data, and find consistency between atomistic simulations and experiments, only by allowing laser energy to be transported away from the interaction region. This additional energy-loss pathway, which scales strongly with laser fluence, we attribute to hot electrons leaving the target on a timescale commensurate with melting.

36 MATERIALS SCIENCE↗

GeoSoilEnviroCARS (Sector 13) at the Advanced Photon Source: a comprehensive synchrotron radiation facility for Earth science research at ambient and extreme conditions

GeoSoilEnviroCARS (GSECARS) is a comprehensive analytical laboratory for Earth and environmental science research using X-ray beams from the Advanced Photon Source, Argonne National Laboratory. State-of-the-art instruments are available for (1) high-pressure/high- or low-temperature diffraction, total scattering, and spectroscopy (Brillouin, Raman, and VIS-IR) using the laser heated diamond anvil cell (DAC); (2) high-pressure/high-temperature diffraction, scattering, and imaging as well as acoustic emission (AE) and ultrasonics using the large-volume press (LVP); (3) powder, single crystal, and surface/interface diffraction; (4) X-ray absorption fine structure spectroscopy; (5) X-ray fluorescence microprobe analysis; and (6) microtomography. As shown here, experiments are facilitated by senior level staff who collaborate on all aspects of the analytical work including experiment design, sample preparation, data collection, data interpretation, and publication preparation. Both technical and scientific synergies occur as a result of the intimate association of the various techniques and scientists experienced in the applications of synchrotron radiation to Earth, environmental, and planetary science problems. The facility includes state-of-the-art instrumentation designed and built in-house, including custom X-ray optics, online and offline laser-based systems, specialized sample environments and positioning systems, as well as pixel-array and multi-crystal energy dispersive X-ray detectors, which are available to be shared among the experimental stations.

36 MATERIALS SCIENCE↗

The CLAS12 Backward Angle Neutron Detector (BAND)

The Backward Angle Neutron Detector (BAND) of CLAS12 detects neutrons emitted at backward angles of 155° to 175°, with momenta between 200 and 600 MeV$/c_0$. It is positioned 3-m upstream of the target, consists of 18 rows and 5 layers of 7.2-cm by 7.2-cm scintillator bars, and read out on both ends by PMTs to measure time and energy deposition in the scintillator layers. Between the target and BAND there is a 2-cm thick lead wall followed by a 2-cm veto layer to suppress gammas and reject charged particles. This paper discusses the component-selection tests and the detector assembly. Timing calibrations (including offsets and time-walk) were performed using a novel pulsed-laser calibration system, resulting in time resolutions better than 250 ps (150 ps) for energy depositions above 2 MeV (5 MeV). Cosmic rays and a variety of radioactive sources were used to calibration the energy response of the detector. Scintillator bar attenuation lengths were measured. We report the time resolution results in a neutron momentum reconstruction resolution, $δp/p$ < 1.5% for neutron momentum 200 ≤ $p$ ≤ 600 MeV/c. Final performance of the BAND with CLAS12 is shown, including electron–neutral particle timing spectra and a discussion of the off-time neutral contamination as a function of energy deposition threshold.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cavitation-induced erosion in liquid metal spallation targets – A comparison between a predictive method and measured erosion damage to stainless steel target modules at the Spallation Neutron Source

Neutrons are produced for neutron scattering instruments at the Spallation Neutron Source by bombarding liquid mercury with a pulsed high-energy proton beam. The liquid mercury target material flows through a replaceable stainless-steel target vessel and cavitates during operation due to the extremely high heating rate caused by each proton pulse. Cavitation-induced erosion damage to the mercury-facing surfaces of target vessels is a key concern for target lifetime and has been the subject of considerable research. While numerous experiments have studied and modeled the progression of cavitation erosion damage to liquid metal target containers, direct quantitative measurements of actual erosion of a spallation target vessel were previously not available. Recently, the erosion damage to multiple target vessels operated at the Spallation Neutron Source was measured using a high-resolution laser scanning system, which provided an opportunity to study the efficacy of a cavitation damage progression model. In this paper, a cavitation progression modeling procedure developed using empirical observations is compared to measurements of samples from target vessels after operation. We discuss the strengths and limitations of the technique and propose methods for improving future modeling and predictive accuracy.

36 MATERIALS SCIENCE↗

Realizing symmetry-guaranteed pairs of bound states in the continuum in metasurfaces

Abstract Bound states in the continuum (BICs) have received significant attention for their ability to enhance light-matter interactions across a wide range of systems, including lasers, sensors, and frequency mixers. However, many applications require degenerate or nearly degenerate high-quality factor ( Q ) modes, such as spontaneous parametric down conversion, non-linear four-wave mixing, and intra-cavity difference frequency mixing for terahertz generation. Previously, degenerate pairs of bound states in the continuum (BICs) have been created by fine-tuning the structure to engineer the degeneracy, yielding BICs that respond unpredictably to structure imperfections and material variations. Instead, using a group theoretic approach, we present a design paradigm based on six-fold rotational symmetry ( C 6 ) for creating degenerate pairs of symmetry-protected BICs, whose frequency splitting and Q -factors can be independently and predictably controlled, yielding a complete design phase space. Using a combination of resonator and lattice deformations in silicon metasurfaces, we experimentally demonstrate the ability to tune mode spacing from 2 nm to 110 nm while simultaneously controlling Q -factor.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Monolayer organic thin films as particle-contamination–resistant coatings

Abstract Three organic monolayers coatings were developed and tested for their effectiveness to increase cleaning efficiency of attached microscale particles by air flows. The experiments were performed using silica substrates coated with these organic thin films and subsequently exposed to stainless-steel and silica microparticles as a model of contamination. Laser-induced–damage tests confirmed that the coatings do not affect the laser-induced–damage threshold values. The particle exposure results suggest that although the accumulation of particles is not significantly affected under the experimental conditions used in this work, the coated substrates exhibit significantly improved cleaning efficiency with a gas flow. A size-distribution analysis was conducted to study the adsorption and cleaning efficiency of particles of different sizes. It was observed that larger size (> 5-μm) particles can be removed from coated substrates with almost 100% efficiency. It was also determined that the coatings improve the cleaning efficiency of the smaller particles (≤ 5 μm) by 17% to 30% for the stainless steel metal and 19% to 38% for the silica particles.

36 MATERIALS SCIENCE↗

Exploring mounting solutions for cryogenically cooled thin crystal optics in high power density x-ray free electron lasers

This study investigates three mounting methods—clamping, soldering, and a hybrid clamping–soldering approach—for cryogenically cooled thin diamond crystals crucial to stable operation of X-ray Free Electron Laser (XFEL) systems. While clamping methods exhibit temperature resilience and flexibility, meticulous design is required to prevent stress-induced warping and reduce thermal contact area. Soldering methods offer reliable mechanical and thermal bonding but encounter challenges due to the coefficient of thermal expansion mismatch at cryogenic temperatures. The hybrid method, integrating clamping and soldering with strain relief cuts, effectively mitigates overall distortion caused by mounting and XFEL thermal loads. These findings offer a novel mounting solution for high-performance x-ray optics in XFEL research and applications, ensuring stability and optimal functionality in cryogenic conditions.

Instruments & Instrumentation↗

Measurements with silicon photomultipliers of dose-rate effects in the radiation damage of plastic scintillator tiles in the CMS hadron endcap calorimeter

Measurements are presented of the reduction of signal output due to radiation damage for two types of plastic scintillator tiles used in the hadron endcap (HE) calorimeter of the CMS detector. The tiles were exposed to particles produced in proton-proton (pp) collisions at the CERN LHC with a center-of-mass energy of 13 TeV, corresponding to a delivered luminosity of 50 fb−1. The measurements are based on readout channels of the HE that were instrumented with silicon photomultipliers, and are derived using data from several sources: a laser calibration system, a movable radioactive source, as well as hadrons and muons produced in pp collisions. Results from several irradiation campaigns using 60Co sources are also discussed. The damage is presented as a function of dose rate. Within the range of these measurements, for a fixed dose the damage increases with decreasing dose rate.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

One- and two-qubit gate infidelities due to motional errors in trapped ions and electrons

In this work, we derive analytic formulas that determine the effect of error mechanisms on one- and two-qubit gates in trapped ions and electrons. First, we analyze and derive expressions for the effect of driving field inhomogeneities on one-qubit gate fidelities. Second, we derive expressions for two-qubit gate errors, including static motional frequency shifts, trap anharmonicities, field inhomogeneities, heating, and motional dephasing. We show that, for small errors, each of our expressions for infidelity converges to its respective numerical simulation; this shows that our formulas are sufficient for determining error budgets for high-fidelity gates, obviating numerical simulations in future projects. All of the derivations are general to any internal qubit state, and any mixed state of the ion crystal's motion that is diagonal in the Fock state basis. Our treatment of static motional frequency shifts, trap anharmonicities, heating, and motional dephasing apply to both laser-based and laser-free gates, while our treatment of field inhomogeneities applies to laser-free systems.

74 ATOMIC AND MOLECULAR PHYSICS↗

IoT Devices and Applications for Wire-Based Hybrid Manufacturing Machine Tools

Hybrid manufacturing machine tools have the potential to be a disruptive technology as they can leverage the benefits of both additive and subtractive manufacturing by incorporating both processes on the same machine while limiting the downsides of the individual processes. Since these machines use two very disparate manufacturing processes and hybrid manufacturing is an emerging technology, it will be useful to monitor data coming from the machine and apply it to improve the manufacturing process, the operation of the machine, and to integrate the machine into the larger digital framework of Industrial Internet of Things (IoT). The present work discusses IoT devices that would be beneficial to add to a hybrid machine tool as well as applications for those devices. The proposed methods discussed in this work have not been experimentally implemented on a hybrid machine tool and so there are no performance data available yet. The hybrid machine tool used as a basis to generate these IoT applications is the Mazak VC-500A/5x AM Hot Wire Deposition, which is a 5-axis machine tool incorporated with a wire feedstock 4kW laser deposition system. Methodologies and applications will be outlined for machine health and process monitoring. Other areas covered include process benchmarking, secure networking options for the proposed IoT framework, and hybrid process improvement. Limitations of these methods and future work for new sensor devices and application areas is also discussed.

Thien, Austen↗

Coriolis force compensation and laser beam delivery for 100-m baseline atom interferometry

The Coriolis force is a significant source of systematic phase errors and dephasing in atom interferometry and is often compensated by counter-rotating the interferometry laser beam against Earth's rotation. We present a novel method for performing Coriolis force compensation for long-baseline atom interferometry, which mitigates atom-beam misalignment due to beam rotation, an effect which is magnified by the long lever arm of the baseline length. The method involves adjustment of the angle of the interferometer beam prior to a magnifying telescope, enabling the beam to pivot around a tunable position along the interferometer baseline. By tuning the initial atom kinematics and adjusting the angle with which the interferometer beam pivots about this point, we can ensure that the atoms align with the center of the beam during the atom optics laser pulses. This approach will be used in the MAGIS-100 atom interferometer and could also be applied to other long-baseline atom interferometers. An additional challenge associated with long baseline interferometry is that since long-baseline atom interferometers are often located outside of typical laboratory environments, facilities constraints may require lasers to be housed in a climate-controlled room a significant distance away from the main experiment. Nonlinear effects in optical fibers restrict the use of fiber-based transport of the high-power interferometry beam from the laser room to the experiment. We present the design of and prototype data from a laser transport system for MAGIS-100 that maintains robustness against alignment drifts despite the absence of a long fiber.

Glick, Jonah↗

In-situ digital image correlation and thermal monitoring in directed energy deposition additive manufacturing

As in welding, directed energy deposition (DED) additive manufacturing (AM) generates complex residual stresses and distortions commensurate with the complexity of the scan pattern used for deposition. To date, measuring DED distortions on complex geometries has only been achieved post process, discarding the complex thermomechanical history that leads to that final material state. In this work, surround stereo digital image correlation (DIC) is used to 3D map surfaces and strain tensors in-situ in a powder-blown laser DED system. Infrared thermography is then projected onto these surfaces to record the full thermomechanical history of printed parts. DIC presents a unique challenge to DED AM, as no part exists at the beginning of deposition, which (a) prevents application of an appropriate speckle pattern and (b) denies the user a zero strain reference frame. Solutions to these problems are proposed and their limitations explored herein. In sum, this work presents a relatively low-cost solution to monitoring and optimizing the unique temporal artifacts induced by complex scan strategies that was previously unobtainable.

42 ENGINEERING↗

Multiscale Approach to Fast ModSim for Laser Processing of Metals for Future Nuclear Deterrence Environments

Predicting performance of parts produced using laser-metal processing remains an out- standing challenge. While many computational models exist, they are generally too computationally expensive to simulate the build of an engineering-scale part. This work develops a reduced order thermal model of a laser-metal system using analytical Green's function solutions to the linear heat equation, representing a step towards achieving a full part performance prediction in an "overnight" time frame. The developed model is able to calculate a thermal history for an example problem 72 times faster than a traditional FEM method. The model parameters are calibrated using a non-linear solution and microstructures and residual stresses calculated and compared to a non-linear case. The calibrated model shows promising agreement with a non-linear solution.

36 MATERIALS SCIENCE↗

Flexure Upgrade System Engineering Project

At the National Ignition Facility (NIF), a system of lasers is used to implode and blow-up targets and create temperatures and pressures unlike any other place on earth. There are many target types that are used on experiments, but they can be broadly put in two categories – room temperature targets and cold targets. All targets can be mounted on any of the three target positioners on NIF, and two of these three target positioners can cryogenically cool the targets in the low Kelvin range for the cold targets. To minimize the ice buildup and infrared light exposure to these cold targets, a shroud surrounds the targets and seals the target from the outer environment. By shrouding the target, air, water, and other molecules have a difficult time reaching the target and some particles get cryo trapped into the shrouds themselves.

42 ENGINEERING↗

An Extensible High Energy Density Modeling Tool for Extreme Regimes

The overreaching goal of the project is to develop a simulation capability to model an entire High Energy Density (HED) target heated by an X-ray Free Electron Laser (XFEL) beam including the surrounding material with a focus on target material associated with subsequent shots. Our primary objective is to study target fratricide problems, where radiation/debris from the current shot degrade the target for subsequent shots. This work will have a large impact on research being conducted at HED facilities where the quality of data is directly related to the effective repetition rate of the driver, which is often limited by target fratricide problems. This project focuses on a stream of closely spaced droplet targets that are appropriate for new very high repetition rate sources such as the ~1 MHz LCLS-II upgraded XFEL. The capability of the PISALE (Pacific Island Structured-AMR with ALE) code is extended to model this class of problems. We summarize the capability and improvements made to the HED branch of the PISALE code. We discuss our simulations of target fratricide for small (5 micron) hydrogen droplets heated by an XFEL beam at SLAC. We also compare simulations of the initial dynamics of larger (50 micron) water droplets, heated by the same XFEL beam, with experimental data. We briefly discuss training, dissemination, and related activities associated with this project.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Catalyst Layer Design, Manufacturing and In-line Quality Control

In this project we successfully demonstrated the capabilities of the Reactive Spray Deposition Technology (RSDT) to fabricate large-scale CCMs for advanced PEMWEs that have one-order of magnitude lower PGM loading in their catalyst layers, and performance comparable with the commercial state-of-the-art CCMs. The RSDT is a unique methodology that combines the catalyst synthesis and CCM fabrication in one step and reduces dramatically the time for CCM manufacturing. As fabricated large-scale CCMs with geometric area of 680 cm2 demonstrated excellent activity and durability performance, and the novel duo-recombination layer design paves the way for solving the safety concerns related to PEMWEs. In addition, excellent activity and durability performance has been demonstrated with RSDT fabricated CCMs with thinner membranes and duo RL design. This is a novel approach for further performance improvement of the MEAs for PEMWEs that has been successfully demonstrated for the first time in this project. The integration of the in-situ laser diagnostics system along with the in-line optical quality control system within the RSDT that has been achieved and demonstrated in this project, is an example for possibility of designing and building advanced manufacturing technologies that can meet the requirements of the future manufacturing. Therefore, the RSDT offers a precise real-time monitoring and control of the particles size, composition, loading, porosity, thickness, and defects in the catalysts’ layers, which render this technology as the best candidate for manufacturing of cost effective CCMs for PEMWEs. By using RSDT we successfully met all project’s milestones, Go/No-Go decision, objectives, goals, and deliverables.

08 HYDROGEN↗