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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
NASA NTRS1999

The Role of Self-Organized Criticality in the Substorm Phenomenon and its Relation to Localized Reconnection in the Magnetospheric Plasma Sheet

Evidence is presented that suggests there is a significant self-organized criticality (SOC) component in the dynamics of substorms in the magnetosphere. Observations of BBFs, fast flows, localized dipolarizations, plasma turbulence, etc. are taken to show that multiple localized reconnection sites provide the basic avalanche phenomenon in the establishment of SOC in the plasma sheet. First results are presented from a continuing plasma physical study of this avalanche process. A one-dimensional resistive MHD model of a magnetic field reversal is discussed. Resistivity, in this model, is self-consistently generated in response to the excitation of an idealized current-driven instability. When forced by convection of magnetic flux into the field reversal region, the model yields rapid magnetic field annihilation through a dynamic behavior that is shown to exhibit many of the characteristics of SOC. Over a large range of forcing strengths, the annihilation rate is shown to self-adjust to balance the rate at which flux is convected into the reversal region. Several analogies to magnetotail dynamics are discussed: (1) It is shown that the presence of a localized criticality in the model produces a remarkable stability in the global configuration of the field reversal while simultaneously exciting extraordinarily dynamic internal evolution. (2) Under steady forcing, it is shown that a loading-unloading cycle may arise that, as a consequence of the global stability, is quasi-periodic and, therefore, predictable despite the presence of internal turbulence in the field distribution. Indeed, it is shown that the global loading-unloading cycle is a consequence of the internal turbulence. (3) It is shown that, under steady, strong forcing the loading-unloading cycle vanishes. Instead, a recovery from a single unloading persists indefinitely. The field reversal is globally very steady while internally it is very dynamic as field annihilation goes on at the rate necessary to match the strong forcing. From this result we speculate that steady magnetospheric convection events result when the plasma sheet has been driven close to criticality over an extended spatial domain. During these events, we would expect to find localized reconnection sites distributed over the spatial domain of near criticality and we would expect to find plasma sheet transport in that domain to be closely related to that of BBF and fast flow events.

Klimas, Alex J.↗
NASA NTRS2012

VERITAS Deep Observations of the Dwarf Spheroidal Galaxy Segue 1

The VERITAS array of Cherenkov telescopes has carried out a deep observational program on the nearby dwarf spheroidal galaxy Segue 1. We report on the results of nearly 48 hours of good quality selected data, taken between January 2010 and May 2011. No significant gamma-ray emission is detected at the nominal position of Segue 1, and upper limits on the integrated flux are derived. According to recent studies, Segue 1 is the most dark matter-dominated dwarf spheroidal galaxy currently known. We derive stringent bounds on various annihilating and decaying dark matter particle models. The upper limits on the velocity-weighted annihilation cross-section are (sigma nu)(sup 95% CL) approx < 10(exp - 23) cubic cm/s, improving our limits from previous observations of dwarf spheroidal galaxies by at least a factor of 2 for dark matter particle masses m(sub x) approx > 300 GeV. The lower limits on the decay lifetime are at the level of tau(sup 95% CL) approx > 10(exp 24) s. Finally, we address the interpretation of the cosmic ray lepton anomalies measured by ATIC and PAMELA in terms of dark matter annihilation, and show that the VERITAS observations of Segue 1 disfavor such a scenario.

Perkins, J. S.↗
DOE OSTI2025

A data-driven method to estimate the antiproton background in the Mu2e experiment

The Mu2e experiment at Fermilab will search for the Charged Lepton Flavour Violating (CLFV) process of coherent, neutrinoless µ− → e − conversion in the field of an aluminum nucleus. The expected signal is a monochromatic electron with the energy of 104.97 MeV, slightly below the muon rest mass. Observation of a CLFV process would provide unambiguous evidence for Beyond the Standard Model (BSM) physics. Mu2e is sensitive to a wide range of BSM models and has the capability to distinguish between them, guiding us towards the most accurate models. The key features of the Mu2e experiment are: (1) a high intensity pulsed negative muon beam with about 1010 stopped µ −/s, and (2) a sophisticated superconducting solenoid system with a gradient magnetic field to form and guide the intense muon beam to the target. The Mu2e physics data taking is expected to begin in 2027. For Run I, the expected 5σ discovery sensitivity is Rµe = 1.2 × 10−15, with a total expected background of 0.11 ± 0.03 events. In the absence of a signal, the expected upper limit is Rµe < 6.2 × 10−16 at 90% CL. The success of this experiment hinges on the accurate estimation of the background from various SM processes that could provide signal-like electrons. One of the background processes is antiprotons annihilating in the stopping target to produce signal like electrons through π0 → γγ decays followed by γ conversions, and π− → µ−ν¯ decays followed by µ− decay. It is a relatively small background with large uncertainty (100%) due to the lack of antiproton production cross section information for the Mu2e proton beam energy of 8 GeV. We have developed a novel methodology to estimate the antiproton background in-situ. This forms the main theme of the thesis. We observed that at Mu2e energies, antiproton annihilation in the stopping target is the only source of events with multiple, simultaneous particle trajectories. From Geant4 simulations, only about 0.2% of the simulated antiproton annihilation events have a signal-like electron. Meanwhile, ∼ 5% of events have multiple reconstructible particle tracks per event. Therefore, we have devised a methodology to reconstruct the multi-track events and estimate the antiproton background by exploiting the large ratio of the production rates of the two final states.

Chithirasreemadam, Namitha [Pisa U.] (ORCID:000000↗
DOE OSTI2022

Surface Doping Boosts Triplet Generation Yield in Perovskite-Sensitized Upconversion

Triplet–triplet annihilation-based photon upconversion (TTA-UC) can efficiently generate higher energy photons at low relative fluences. Bulk metal halide perovskites have offered promise in efficiently sensitizing molecular triplet states in the solid state, necessary for the integration of TTA-UC into device-based applications. Recent work focused on TTA-UC from a rubrene triplet annihilator sensitized by perovskite thin films has established relatively efficient charge extraction from the perovskite, forming the triplet exciton in rubrene. Yet, the specifics underpinning charge transfer at the perovskite/rubrene interface are not fully elucidated. Here, to improve device performance and study the properties governing charge transfer at the interface, various organic solvents are explored to treat the perovskite surface. Scanning tunneling microscopy and spectroscopy show a difference in the electronic band structure, where both n- and p-type terminated perovskite surfaces are observed depending on the solvent used. Supported by optical spectroscopy, the impact of the perovskite electronic structure is monitored, indicating that n-type perovskite sensitizers feature higher TTA-UC efficiencies due to favorable band bending resulting in efficient hole-mediated triplet formation. Overall, the tuning of the electronic structure of the perovskite sensitizer through solvent treatment is shown to be a key force in tuning the mechanism of efficient triplet generation.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Interface effect of Fe and Fe 2 O 3 on the distributions of ion induced defects

The stability of structural materials in extreme nuclear reactor environments—with high temperature, high radiation, and corrosive media—directly affects the lifespan of the reactor. In such extreme environments, an oxide layer on the metal surface acts as a passive layer protecting the metal underneath from corrosion. To predict the irradiation effect on the metal layer in these metal/oxide bilayers, nondestructive depth-resolved positron annihilation lifetime spectroscopy (PALS) and complementary transmission electron microscopy (TEM) were used to investigate small-scale defects created by ion irradiation in an epitaxially grown (100) Fe film capped with a 50 nm Fe 2 O 3 oxide layer. In this study, the evolution of induced vacancies was monitored, from individual vacancy formation at low doses—10 –5 dpa—to larger vacancy cluster formation at increasing doses, showing the sensitivity of positron annihilation spectroscopy technique. Furthermore, PALS measurements reveal how the presence of a metal–oxide interface modifies the distribution of point defects induced by irradiation. TEM measurements show that irradiation induced dislocations at the interface is the mechanism behind the redistribution of point defects causing their accumulation close to the interface. Finally, this work demonstrates that the passive oxide layers formed during corrosion impact the distribution and accumulation of radiation induced defects in the metal underneath and emphasizes that the synergistic impact of radiation and corrosion will differ from their individual impacts.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Point and extended defects in heteroepitaxial 𝛽−G⁡a 2 ⁢O 3 films

G⁡a 2 ⁢O 3 is emerging as an excellent potential semiconductor for high power and optoelectronic devices. However, the successful development of G⁡a 2⁢ O 3 in a wide range of applications requires a full understanding of the role and nature of its point and extended defects. Here, in this work, high quality epitaxial G⁡a 2 ⁢O 3 films were grown on sapphire substrates by metal-organic chemical vapor deposition and fully characterized in terms of structural, optical, and electrical properties. Then defects in the films were investigated by a combination of depth-resolved Doppler broadening and lifetime of positron annihilation spectroscopies and thermally stimulated emission (TSE). Positron annihilation techniques can provide information about the nature and concentration of defects in the films, while TSE reveals the energy level of defects in the bandgap. Despite very good structural properties, the films exhibit short positron diffusion length, which is an indication of high defect density and long positron lifetime, a sign for the formation of Ga vacancy related defects and large vacancy clusters. These defects act as deep and shallow traps for charge carriers as revealed from TSE, which explains the reason behind the difficulty of developing conductive G⁡a 2 ⁢O 3 films on non-native substrates. Positron lifetime measurements also show nonuniform distribution of vacancy clusters throughout the film depth. Further, the work investigates the modification of defect nature and properties through thermal treatment in various environments. It demonstrates the sensitivity of G⁡a 2 ⁢O 3 microstructures to the growth and thermal treatment environments and the significant effect of modifying defect structure on the bandgap and optical and electrical properties of G⁡a 2 ⁢O 3 .

defects↗
DOE OSTI2020

A new mechanism for void-cascade interaction from nondestructive depth-resolved atomic-scale measurements of ion irradiation–induced defects in Fe

The nondestructive investigation of single vacancies and vacancy clusters in ion-irradiated samples requires a depth-resolved probe with atomic sensitivity to defects. The recent development of short-pulsed positron beams provides such a probe. Here, we combine depth-resolved Doppler broadening and positron annihilation lifetime spectroscopies to identify vacancy clusters in ion-irradiated Fe and measure their density as a function of depth. Despite large concentrations of dislocations and voids in the pristine samples, positron annihilation measurements uncovered the structure of vacancy clusters and the change in their size and density with irradiation dose. When combined with transmission electron microscopy measurements, the study demonstrates an association between the increase in the density of small vacancy clusters with irradiation and a remarkable reduction in the size of large voids. This, previously unknown, mechanism for the interaction of cascade damage with voids in ion-irradiated materials is a consequence of the high porosity of the initial microstructure.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Photon Upconversion at Organic-Inorganic Interfaces

Photon upconversion is a process that combines low-energy photons to form useful high-energy photons. There are potential applications in photovoltaics, photocatalysis, biological imaging, etc. Semiconductor quantum dots (QDs) are promising for the absorption of these low-energy photons due to the high extinction coefficient of QDs, especially in the near infrared (NIR). This allows the intriguing use of diffuse light sources such as solar irradiation. In this review, we describe the development of this organic-QD upconversion platform based on triplet-triplet annihilation, focusing on the dark exciton in QDs with triplet character. Then we introduce the underlying energy transfer steps, starting from QD triplet photosensitization, triplet exciton transport, triplet-triplet annihilation, and ending with the upconverted emission. Design principles to improve the total upconversion efficiency are presented. We end with limitations in current reports and proposed future directions. This review provides a guide for designing efficient organic-QD upconversion platforms for future applications, including overcoming the Shockley-Queisser limit for more efficient solar energy conversion, NIR-based phototherapy, and diagnostics in vivo.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Identification and Suppression of Point Defects in Bromide Perovskite Single Crystals Enabling Gamma‐Ray Spectroscopy

Abstract Methylammonium lead tribromide (MAPbBr 3 ) stands out as the most easily grown wide‐band‐gap metal halide perovskite. It is a promising semiconductor for room‐temperature gamma‐ray ( γ ‐ray) spectroscopic detectors, but no operational devices are realized. This can be largely attributed to a lack of understanding of point defects and their influence on detector performance. Here, through a combination of crystal growth design and defect characterization, including positron annihilation and impedance spectroscopy, the presence of specific point defects are identified and correlated to detector performance. Methylammonium (MA) vacancies, MA interstitials, and Pb vacancies are identified as the dominant charge‐trapping defects in MAPbBr 3 crystals, while Br vacancies caused doping. The addition of excess MABr reduces the MA and Br defects and so enables the detection of energy‐resolved γ ‐ray spectra using a MAPbBr 3 single‐crystal device. Interestingly, the addition of formamidinium (FA) cations, which converted to methylformamidinium (MFA) cations by reaction with MA + during crystal growth further reduced MA defects. This enabled an energy resolution of 3.9% for the 662 keV 137 Cs line using a low bias of 100 V. The work provides direction toward enabling further improvements in wide‐bandgap perovskite‐based device performance by reducing detrimental defects.

Ni, Zhenyi↗
DOE OSTI2025

Increasing the Stability of Deep Blue Phosphor‐Sensitized OLEDs Using the Polariton‐Enhanced Purcell Effect

Abstract The stability of efficient, deep blue organic light‐emitting diodes (OLEDs) remains a major challenge in the field of organic electronics. Poor device stability originates from the high probability for destructive non‐radiative triplet exciton annihilation events. Phosphor‐sensitized fluorescence (PSF) is proposed to achieve an efficient, deep blue color by energy transfer from phosphors to fluorophores. Recently, the polariton‐enhanced Purcell (PEP) effect is introduced to decrease the triplet radiative lifetime and density, resulting in an increase in blue phosphorescent OLED lifetime. Here, the PEP effect is introduced to enhance the stability of the PSF‐OLEDs. It is shown that the PEP effect increases all radiative decay rates of the phosphors and fluorophores, leading to a reduction in the triplet annihilation events. Using a Pt‐complex phosphor sensitizer and a so‐called multi‐resonance fluorescent emitter in a PEP cavity, a 3.1‐fold lifetime increase is observed at a current density ofJ= 10 mA cm −2 , reduced EQE roll‐off and deep blue color with Commission Internationale de l'Eclairage coordinates of (0.13, 0.09). The PEP effect maximally extends PSF‐OLED lifetimes in devices with the highest triplet‐to‐singlet energy transfer rates. Moreover, this work suggests that the benefits of PEPs apply to all triplet‐based OLEDs.

Chemistry↗
DOE OSTI2023

Affleck-Dine cogenesis of baryon and dark matter

We propose a mechanism for cogenesis of baryon and dark matter (DM) in the universe via the Affleck-Dine (AD) route. An AD field which breaks the lepton number symmetry, leads to the generation of lepton asymmetry by virtue of its cosmic evolution, which then gets transferred into lepton and dark sectors. While the lepton asymmetry gets converted into baryon asymmetry via sphalerons, the dark sector asymmetry leads to the final DM abundance with the symmetric part being annihilated away due to resonantly enhanced annihilation, which we choose to be provided by a gauged B – L portal. Stringent constraints from DM direct detection forces DM and B – L gauge boson masses to be light, in the few GeV ballpark. While a large portion of the model parameter space is already ruled out, the remaining parameter space is within sensitivity of laboratory as well as cosmology based experiments. The AD field also plays the role of inflaton with the required dynamics by virtue of its non-minimal coupling to gravity, consistent with observations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Dark showers from sneaky dark matter

We present a minimal composite dark matter model, based on a SU(Nd) dark sector with nf dark quarks and a heavy t-channel mediator. For nf ≥ 4, the dark flavor symmetry guarantees the stability of a subset of the dark pions, which serve as our dark matter candidates. Their relic abundance is determined by dark sector annihilation with the remaining dark pions, which are unstable and decay. Due to their degenerate masses, the annihilation cross section is suppressed at low temperatures, thereby avoiding stringent constraints from indirect detection and opening up the GeV mass window. The decaying dark pions are naturally long lived. We obtain limits on the model from semi-visible or emerging jet searches and estimate the reach of future probes.

ALPs↗
DOE OSTI2021

The Energy-Energy Correlation in the back-to-back limit at N 3 LO and N 3 LL'

We present the analytic formula for the Energy-Energy Correlation (EEC) in electron-positron annihilation computed in perturbative QCD to next-to-next-to-next-to-leading order (N 3 LO) in the back-to-back limit. In particular, we consider the EEC arising from the annihilation of an electron-positron pair into a virtual photon as well as a Higgs boson and their subsequent inclusive decay into hadrons. Our computation is based on a factorization theorem of the EEC formulated within Soft-Collinear Effective Theory (SCET) for the back-to-back limit. We obtain the last missing ingredient for our computation — the jet function — from a recent calculation of the transverse-momentum dependent fragmentation function (TMDFF) at N 3 LO. We combine the newly obtained N 3 LO jet function with the well known hard and soft function to predict the EEC in the back-to-back limit. The leading transcendental contribution of our analytic formula agrees with previously obtained results in N = 4 supersymmetric Yang-Mills theory. We obtain the N = 2 Mellin moment of the bulk region of the EEC using momentum sum rules. Finally, we obtain the first resummation of the EEC in the back-to-back limit at N 3 LL' accuracy, resulting in a factor of ~ 4 reduction of uncertainties in the peak region compared to N 3 LL predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Jupiter missions as probes of dark matter

Jupiter, the fascinating largest planet in the solar system, has been visited by nine spacecraft, which have collected a significant amount of data about Jovian properties. In this paper, we show that one type of the in situ measurements on the relativistic electron fluxes could be used to probe dark matter (DM) and dark mediator between the dark sector and our visible world. Jupiter, with its immense weight and cool core, could be an ideal capturer for DM with masses around the GeV scale. The captured DM particles could annihilate into long-lived dark mediators such as dark photons, which subsequently decay into electrons and positrons outside Jupiter. The charged particles, trapped by the Jovian magnetic field, have been measured in Jupiter missions such as the Galileo probe and the Juno orbiter. We use the data available to set upper bounds on the cross section of DM scattering off nucleons, σ χn , for dark mediators with lifetime of order $O$ (0.1–1) s. The results show that data from Jupiter missions already probe regions in the parameter space un- or under-explored by existing DM searches, e.g., constrain σχn of order (10 –41 –10 –39 ) cm 2 for 1 GeV DM dominantly annihilating into e + e – through dark mediators. This study serves as an example and an initial step to explore the full physics potential of the large planetary datasets from Jupiter missions. We also outline several other potential directions related to secondary products of electrons, positron signals and solar axions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Size-dependent radiation damage mechanisms in nanowires and nanoporous structures

Nanostructures with a high density of interfaces, such as in nanoporous materials and nanowires, resist radiation damage by promoting the annihilation and migration of defects. This study details the size effect and origins of the radiation damage mechanisms in nanowires and nanoporous structures in model face-centered (gold) and body-centered (niobium) cubic nanostructures using accelerated multi-cascade atomistic simulations and in-situ ion irradiation experiments. Our results reveal three different size-dependent mechanisms of damage accumulation in irradiated nanowires and nanoporous structures: sputtering for very small nanowires and ligaments, the formation and accumulation of point defects and dislocation loops in larger nanowires, and a face-centered-cubic to hexagonal-close-packed phase transformation for a narrow range of wire diameters in the case of gold nanowires. Smaller nanowires and ligaments have a net effect of lowering the radiation damage as compared to larger wires that can be traced back to the fact that smaller nanowires transition from a rapid accumulation of defects to a saturation and annihilation mechanism at a lower dose than larger nanowires. These irradiation damage mechanisms are accompanied with radiation-induced surface roughening resulting from defect-surface interactions. Comparisons between nanowires and nanoporous structures show that the various mechanisms seen in nanowires provide adequate bounds for the defect accumulation mechanisms in nanoporous structures with the difference attributed to the role of nodes connecting ligaments in nanoporous structures. Altogether, our results shed light on the compounded, size-dependent mechanisms leading to the radiation resistance of nanowires and nanoporous structures.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Non-radiative luminescence decay with self-trapped hole migration in strontium titanate: Interplay between optical and transport properties

A novel model for the non-radiative decay of self-trapped excitons (STEs) in the advanced functional oxide SrTiO3 is proposed and supported by experimental observations. The study is based on the initial ionoluminescence stage for STE emission at 2.5 eV, and its dependence on temperature and electronic excitation rate under energetic heavy-ion irradiation. For all temperatures, this initial stage reaches rapidly a quasi-steady level, and then decreases as induced-structural damage increases. The quasi-steady luminescence exhibits a linear dependence on the excitation rate, suggesting a constant efficiency for STEs formation. An activation energy of 55 meV, essentially independent of the incident ion mass and energy of projectile-ion, is deduced from an Arrhenius-type relationship with irradiation temperature. This energy is in good agreement with experimental values, measured for non-radiative STE decay under ns-laser pulse excitation, and reasonably consistent with density functional theory calculations for migration of self-trapped holes (STHs) described by a small-polaron adiabatic hopping model. A new mechanism dealing with a non-radiative contribution to the STE transition is discussed, consisting of STH migration through thermally-activated hopping and annihilation with the STE-electron. Luminescence kinetics from the chromium intrinsic impurity strongly supports this model, being consistent with the annihilation of Cr 3+ centers through recombination with migrating STHs.

luminescence↗
DOE OSTI2021

Cosmic antihelium-3 nuclei sensitivity of the GAPS experiment

The General Antiparticle Spectrometer (GAPS) is an Antarctic balloon experiment designed for low-energy (0.1-0.3 GeV/n) cosmic antinuclei as signatures of dark matter annihilation or decay. GAPS is optimized to detect low-energy antideuterons, as well as to provide unprecedented sensitivity to low-energy antiprotons and antihelium nuclei. The novel GAPS antiparticle detection technique, based on the formation, decay, and annihilation of exotic atoms, provides greater identification power for these low-energy antinuclei than previous magnetic spectrometer experiments. This work reports the sensitivity of GAPS to detect antihelium-3 nuclei, based on full instrument simulation, event reconstruction, and realistic atmospheric influence simulations. The report of antihelium nuclei candidate events by AMS-02 has generated considerable interest in antihelium nuclei as probes of dark matter and other beyond the Standard Model theories. GAPS is in a unique position to detect or set upper limits on the cosmic antihelium nuclei flux in an energy range that is essentially free of astrophysical background. In three 35-day long-duration balloon flights, GAPS will be sensitive to an antihelium flux on the level of $1.3^{+4.5}_{-1.2} $ ∙ 10 -6 m -2 sr -1 s -1 (GeV/n) -1 (95% confidence level) in the energy range of 0.11-0.3 GeV/n, opening a new window on rare cosmic physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

MADHAT: Model-Agnostic Dark Halo Analysis Tool

We present the Model-Agnostic Dark Halo Analysis Tool (MADHAT), a numerical tool which implements a Fermi-LAT data-driven, model-independent analysis of gamma-ray emission from dwarf satellite galaxies and dwarf galaxy candidates due to dark matter annihilation, dark matter decay, or other nonstandard or unknown astrophysics. This tool efficiently provides statistical upper bounds on the number of observed photons in excess of the number expected, based on empirical determinations of foregrounds and backgrounds, using a stacked analysis of any selected set of dwarf targets. It also calculates the resulting bounds on the properties of dark matter under any assumptions the user makes regarding dark sector particle physics or astrophysics. As an application, we determine new bounds on Sommerfeld-enhanced dark matter annihilation in a set of eight dwarfs. MADHAT v1.0 includes 58 dwarfs and dwarf candidate targets, and we discuss future planned developments. MADHAT is available and will be maintained at https://github.com/MADHATdm.

79 ASTRONOMY AND ASTROPHYSICS↗