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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Real-space imaging of periodic nanotextures in thin films via phasing of diffraction data

New properties and exotic quantum phenomena can form due to periodic nanotextures, including Moire patterns, ferroic domains, and topologically protected magnetization and polarization textures. Despite the availability of powerful tools to characterize the atomic crystal structure, the visualization of nanoscale strain-modulated structural motifs remains challenging. Here, we develop nondestructive real-space imaging of periodic lattice distortions in thin epitaxial films and report an emergent periodic nanotexture in a Mott insulator. Specifically, we combine iterative phase retrieval with unsupervised machine learning to invert the diffuse scattering pattern from conventional X-ray reciprocal-space maps into real-space images of crystalline displacements. Our imaging in PbTiO 3 /SrTiO 3 superlattices exhibiting checkerboard strain modulation substantiates published phase-field model calculations. Furthermore, the imaging of biaxially strained Mott insulator Ca 2 RuO 4 reveals a strain-induced nanotexture comprised of nanometer-thin metallic-structure wires separated by nanometer-thin Mott-insulating-structure walls, as confirmed by cryogenic scanning transmission electron microscopy (cryo-STEM). The nanotexture in Ca 2 RuO 4 film is induced by the metal-to-insulator transition and has not been reported in bulk crystals. We expect the phasing of diffuse X-ray scattering from thin crystalline films in combination with cryo-STEM to open a powerful avenue for discovering, visualizing, and quantifying the periodic strain-modulated structures in quantum materials.

Science & Technology - Other Topics↗
DOE OSTI2024

Real-space visualization of a defect-mediated charge density wave transition

Here, we study the coupled charge density wave (CDW) and insulator-to-metal transitions in the 2D quantum material 1T-TaS 2 . By applying in situ cryogenic 4D scanning transmission electron microscopy with in situ electrical resistance measurements, we directly visualize the CDW transition and establish that the transition is mediated by basal dislocations (stacking solitons). We find that dislocations can both nucleate and pin the transition and locally alter the transition temperature T c by nearly ~75 K. This finding was enabled by the application of unsupervised machine learning to cluster five-dimensional, terabyte scale datasets, which demonstrate a one-to-one correlation between resistance—a global property—and local CDW domain-dislocation dynamics, thereby linking the material microstructure to device properties. This work represents a major step toward defect-engineering of quantum materials, which will become increasingly important as we aim to utilize such materials in real devices.

4D-STEM↗
DOE OSTI2021

A multispecies turbulence model for the mixing and de-mixing of miscible fluids

A de-mix capable model for turbulence in compressible, variable density flows is proposed. The model is based on the Besnard-Harlow-Rauenzahn (BHR) family of models (Besnard D, Harlow F, Rauenzahn R, et al. Turbulence transport equations for variable-density turbulence and their relationship to two-field models. NM (United States): Los Alamos National Laboratory; 1992 (Technical Report LA-12303-MS), but is extended to track the evolution of the turbulent fluxes and fluctuations in the material mass fractions for each species present. The new evolution equations are introduced without requiring additional closures or new empirically tuned coefficients relative to previous BHR models, and are shown to improve the model’s ability to reproduce the behaviour of simulations containing mixing layers that are constrained by a stabilising force. As a result, the model is tested in a range of canonical flows including Rayleigh-Taylor driven, shock driven, and shear driven turbulence, and is shown to produce reasonable agreement with simulations and experiments in these scenarios.

42 ENGINEERING↗
DOE OSTI2023

Previous exposure to Spike-providing parental strains confers neutralizing immunity to XBB lineage and other SARS-CoV-2 recombinants in the context of vaccination

The emergence of SARS-CoV-2 recombinants is of particular concern as they can result in a sudden increase in immune evasion due to antigenic shift. Recent recombinants XBB and XBB.1.5 have higher transmissibility than previous recombinants such as “Deltacron.” We hypothesized that immunity to a SARS-CoV-2 recombinant depends on prior exposure to its parental strains. To test this hypothesis, we examined whether Delta or Omicron (BA.1 or BA.2) immunity conferred through infection, vaccination, or breakthrough infection could neutralize Deltacron and XBB/XBB.1.5 recombinants. We found that Delta, BA.1, or BA.2 breakthrough infections provided better immune protection against Deltacron and its parental strains than did the vaccine booster. None of the sera were effective at neutralizing the XBB lineage or its parent BA.2.75.2, except for the sera from the BA.2 breakthrough group. These results support our hypothesis. In turn, our findings underscore the importance of multivalent vaccines that correspond to the antigenic profile of circulating variants of concern and of variant-specific diagnostics that may guide public health and individual decisions in response to emerging SARS-CoV-2 recombinants.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2023

On causality conditions in de Sitter spacetime

We carefully consider the Shapiro time delay due to black holes and shockwaves in de Sitter spacetime and study the implications for causality. We discuss how causality conditions of AdS and flat spacetime can be applied in de Sitter spacetime, using spatial shifts measured on the boundary to define 'fastest null geodesics' and taking into account the 'stretching' of the de Sitter Penrose diagram. We consider the propagation of a massless spin-1 field with a non-minimal coupling in a de Sitter shockwave background as an illustrative example. Here, we also briefly discuss connections to the average null energy condition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Effects of spatiotemporal plasma power distribution on the modeling of ignition kernel evolution in quiescent and turbulent methane/air mixtures

Abstract The present work improves a phenomenological plasma-assisted combustion model by integrating the spatiotemporal distribution of plasma power density, thereby considering the evolution of plasma streamers in the modeling, and subsequently, better predicting the ignition kernel evolution. The improved phenomenological model is validated against experiments representing the plasma discharge and post-discharge ignition kernel evolution. Specifically, the new model demonstrates a more accurate prediction of ultrafast gas heating and O 2 dissociation during the plasma discharge, compared to the original model. In addition, the new model is found to closely match the experimental pressure wave and heated channel profiles post-discharge without the need for tuning the energy deposition (unlike the original model), highlighting its accuracy of post-discharge ignition kernel dynamics. The improved phenomenological model is then employed to investigate ignition kernel evolution for a stoichiometric methane-air discharge across various discharge gap configurations. Simulations reveal a non-uniform temperature and streamer distribution progressing from the electrode tips toward the center, contrasting uniform cylindrical discharges previously described in the original model. Streamer propagation is observed to be faster for larger gaps when maintained at the same average electric field for different discharge gaps. The tendency of smaller gaps to produce detached toroidal ignition kernels is observed, while larger gaps promote cylindrical and attached ignition kernels. Interactions between successive ignition kernels from consecutive discharges varied significantly, with the smallest gap (1 mm) promoting the quenching of the preceding ignition kernel due to the initial kernel–kernel separation. The intermediate gap (2 mm) promotes detached kernel growth. In contrast, in the largest gap (4 mm), kernels consistently combine and expand attached to electrodes. The impact of homogeneous isotropic turbulence is also explored, showing the persistence of ignition kernels early on but eventually quenching due to enhanced radical and heat losses with pronounced turbulence intensity.

Johnson, Praise Noah↗
DOE OSTI2026

Breakdown front dynamics of streamer-like discharge in electron-charged polymethyl methacrylate

We present the results of an experimental study of fast breakdown in electron-charged polymethyl methacrylate. We irradiate bulk polymethyl methacrylate disks with diameters up to one meter at different implanted charge densities and measure the discharge current during the forced electrical breakdown of the material. We infer the breakdown dynamics from these current waveforms, including the velocity and time dependence of the electric field driving the breakdown, and compare these results with the physical electrical tree patterns left behind in the material. We find that the dynamics and physical characteristics of the breakdown channels in electron-irradiated solids depart from typical expectations of electrical treeing behavior in solid materials. Thus, we interpret these results as an expression of streamer discharges in dense gases motivated by the existence of trapped gases in the solid due to radiation damage. We show that the dynamics of the breakdown channels in the electron-charged solid dielectric material is well described by applying standard streamer physics to this physical system. The results show that the dynamics of breakdown channels in solid dielectric material is a promising avenue to further understand streamer discharges in different media under extreme conditions.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Experimental studies of the difference between plasma potentials measured by Langmuir probes and emissive probes in presheaths

The plasma potential measured by cylindrical and planar Langmuir probes has been shown to differ from the plasma potential measured by emissive probes in the neighborhood of the presheath near a negatively biased electrode immersed in a weakly collisional low temperature argon plasma. There are two principal results demonstrated in this paper. First, while it is well known that Langmuir probes cannot reliably measure plasma potentials inside of sheaths, results presented here demonstrate that the problem persists in presheaths, the quasineutral plasma bordering sheaths. It is known that emissive probes analyzed in the limit of zero emission accurately measure the plasma potential in the sheath. It is now clear that they are the only known electrostatic probe technique able to measure the plasma potential accurately throughout the presheath. Second, it is shown that the difference between potential measurements made by Langmuir probes and emissive probes in the body of the plasma, farther than a presheath distance from the boundary, is not proportional to T e , as has been previously claimed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Larmor power limit for cyclotron radiation of relativistic particles in a waveguide

Cyclotron radiation emission spectroscopy (CRES) is a modern technique for high-precision energy spectroscopy, in which the energy of a charged particle in a magnetic field is measured via the frequency of the emitted cyclotron radiation. The He6-CRES collaboration aims to use CRES to probe beyond the standard model physics at the TeV scale by performing high-resolution and low-background beta-decay spectroscopy of 6 He and 19 Ne. Having demonstrated the first observation of individual, high-energy (0.1–2.5 MeV) positrons and electrons via their cyclotron radiation, the experiment provides a novel window into the radiation of relativistic charged particles in a waveguide via the time-derivative (slope) of the cyclotron radiation frequency, df c /dt. We show that analytic predictions for the total cyclotron radiation power emitted by a charged particle in circular and rectangular waveguides are approximately consistent with the Larmor formula, each scaling with the Lorentz factor of the underlying e ± as γ 4 . This hypothesis is corroborated with experimental CRES slope data.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Cosmology at high redshift — a probe of fundamental physics

An observational program focused on the high redshift (2<z<6) Universe has the opportunity to dramatically improve over upcoming LSS and CMB surveys on measurements of both the standard cosmological model and its extensions. Using a Fisher matrix formalism that builds upon recent advances in Lagrangian perturbation theory, we forecast constraints for future spectroscopic and 21-cm surveys on the standard cosmological model, curvature, neutrino mass, relativistic species, primordial features, primordial non-Gaussianity, dynamical dark energy, and gravitational slip. We compare these constraints with those achievable by current or near-future surveys such as DESI and Euclid, all under the same forecasting formalism, and compare our formalism with traditional linear methods. Here, our Python code FishLSS — used to calculate the Fisher information of the full shape power spectrum, CMB lensing, the cross-correlation of CMB lensing with galaxies, and combinations thereof — is publicly available.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Optical depth to reionization from perturbative 21 cm clustering

The optical depth τ is the least well determined parameter in the standard model of cosmology, and one whose precise value is important for both understanding reionization and for inferring fundamental physics from cosmological measurements. Here, we forecast how well future epoch of reionization experiments could constraint τ using a symmetries-based bias expansion that highlights the special role played by anisotropies in the power spectrum on large scales. Given a parametric model for the ionization evolution inspired by the physical behavior of more detailed reionization simulations, we find that future 21 cm experiments could place tight constraints on the timing and duration of reionization and hence constraints on τ that are competitive with proposed, space-based CMB missions provided they can measure k ≈ 0.1 h Mpc -1 with a clean foreground wedge across redshifts spanning the most active periods of reionization, corresponding to ionization fractions 0.2 ≲ x ≲ 0.8. Significantly improving upon existing CMB-based measurements with next-generation 21 cm surveys would require substantially longer observations (~ 5 years) than standard $\mathscr{O}$(1000 hour) integration times. Precise measurements of smaller scales will not improve constraints on τ until a better understanding of the astrophysics of reionization is achieved. In the presence of noise and foregrounds even future 21 cm experiments will struggle to constrain τ if the ionization evolution deviates significantly from simple parametric forms.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Scalar dark matter vortex stabilization with black holes

Galaxies and their dark-matter halos are commonly presupposed to spin. But it is an open question how this spin manifests in halos and soliton cores made of scalar dark matter (SDM, including fuzzy/wave/ultralight-axion dark matter). One way spin could manifest in a necessarily irrotational SDM velocity field is with a vortex. But recent results have cast doubt on this scenario, finding that vortices are generally unstable except with substantial repulsive self-interaction. Here, in this paper, we introduce an alternative route to stability: in both (non-relativistic) analytic calculations and simulations, a black hole or other central mass at least as massive as a soliton can stabilize a vortex within it. This conclusion may also apply to AU-scale halos bound to the sun and stellar-mass-scale Bose stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

DESI luminous red galaxy samples for cross-correlations

We present two galaxy samples, selected from DESI Legacy Imaging Surveys (LS) DR9, with approximately 20,000 square degrees of coverage and spectroscopic redshift distributions designed for cross-correlations such as with CMB lensing, galaxy lensing, and the Sunyaev-Zel'dovich effect. The first sample is identical to the DESI Luminous Red Galaxy (LRG) sample, and the second sample is an extended LRG sample with 2–3 times the DESI LRG density. We present the improved photometric redshifts, tomographic binning and their spectroscopic redshift distributions and imaging systematics weights, and magnification bias coefficients. The catalogs and related data products will be made publicly available. The cosmological constraints using this sample and Planck lensing maps are presented in a companion paper. Here, we also make public the new set of general-purpose photometric redshifts trained using DESI spectroscopic redshifts, which are used in this work, for all galaxies in LS DR9.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

The Atacama Cosmology Telescope DR6 and DESI: structure formation over cosmic time with a measurement of the cross-correlation of CMB lensing and luminous red galaxies

We present a high-significance cross-correlation of CMB lensing maps from the Atacama Cosmology Telescope (ACT) Data Release 6 (DR6) with luminous red galaxies (LRGs) from the Dark Energy Spectroscopic Instrument (DESI) Legacy Survey spectroscopically calibrated by DESI. We detect this cross-correlation at a significance of 38σ; combining our measurement with the Planck Public Release 4 (PR4) lensing map, we detect the cross-correlation at 50σ. Fitting this jointly with the galaxy auto-correlation power spectrum to break the galaxy bias degeneracy with σ 8 , we perform a tomographic analysis in four LRG redshift bins spanning 0.4 ≤ z ≤ 1.0 to constrain the amplitude of matter density fluctuations through the parameter combination S 8 × = σ 8 (Ω m / 0.3) 0.4 . Prior to unblinding, we confirm with extragalactic simulations that foreground biases are negligible and carry out a comprehensive suite of null and consistency tests. Using a hybrid effective field theory (HEFT) model that allows scales as small as k max = 0.6 h/ Mpc, we obtain a 3.3% constraint on S 8 × = σ 8 (Ω m / 0.3) 0.4 = 0.792 +0.024 -0.028 from ACT data, as well as constraints on S 8 × (z) that probe structure formation over cosmic time. Our result is consistent with the early-universe extrapolation from primary CMB anisotropies measured by Planck PR4 within 1.2σ. Jointly fitting ACT and Planck lensing cross-correlations we obtain a 2.7% constraint of S 8 × = 0.776 +0.019 -0.021 , which is consistent with the Planck early-universe extrapolation within 2.1σ, with the lowest redshift bin showing the largest difference in mean. The latter may motivate further CMB lensing tomography analyses at z < 0.6 to assess the impact of potential systematics or the consistency of the ΛCDM model over cosmic time.

79 ASTRONOMY AND ASTROPHYSICS↗