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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Dimer rattling mode induced low thermal conductivity in an excellent acoustic conductor

A solid with larger sound speeds usually exhibits higher lattice thermal conductivity. Here, we report an exception that CuP2 has a quite large mean sound speed of 4155 m s –1 , comparable to GaAs, but single crystals show very low lattice thermal conductivity of about 4 W m –1 K –1 at room temperature, one order of magnitude smaller than GaAs. To understand such a puzzling thermal transport behavior, we have thoroughly investigated the atomic structures and lattice dynamics by combining neutron scattering techniques with first-principles simulations. This compound crystallizes in a layered structure where Cu atoms forming dimers are sandwiched in between P atomic networks. In this work, we reveal that Cu atomic dimers vibrate as a rattling mode with frequency around 11 meV, which is manifested to be remarkably anharmonic and strongly scatters acoustic phonons to achieve the low lattice thermal conductivity.

36 MATERIALS SCIENCE↗
DOE OSTI2018

L1 0 -FeNi films on Au-Cu-Ni buffer-layer: a high-throughput combinatorial study

Here, the fct L1 0 -FeNi alloy is a promising candidate for the development of high performance critical-elements-free magnetic materials. Among the different materials, the Au-Cu-Ni alloy has resulted very promising; however, a detailed investigation of the effect of the buffer-layer composition on the formation of the hard FeNi phase is still missing. To accelerate the search of the best Au-Cu-Ni composition, a combinatorial approach based on High-Throughput (HT) experimental methods has been exploited in this paper. HT magnetic characterization methods revealed the presence of a hard magnetic phase with an out-of-plane easy-axis, whose coercivity increases from 0.49 kOe up to 1.30 kOe as the Au content of the Cu-Au-Ni buffer-layer decreases. Similarly, the out-of-plane magneto-crystalline anisotropy energy density increases from 0.12 to 0.35 MJ/m 3 . This anisotropy is attributed to the partial formation of the L1 0 FeNi phase induced by the buffer-layer. In the range of compositions we investigated, the buffer-layer structure does not change significantly and the modulation of the magnetic properties with the Au content in the combinatorial layer is mainly related to the different nature and extent of interlayer diffusion processes, which have a great impact on the formation and order degree of the L1 0 FeNi phase.

25 ENERGY STORAGE↗
NASA NTRS1981

Turbulence suppression in free shear flows by controlled excitation

Turbulence suppression in the near field of a free shear flow under controlled excitation is investigated in four circular jets, a plane jet, and a plane mixing layer. The suppression is a consequence of an excitation-induced modification of the shear layer structure and occurs at the excitation frequency corresponding to the maximally unstable disturbance frequency of the initial free shear layer. The most pronounced suppression occurs when the shear layer is excited at a frequency 40% higher than the natural roll-up frequency. Excitation at a Strouhal number of about 0.017 produces a rapid roll-up and early breakdown of the shear layer, and thus inhibits the formation of the energetic large-scale vortices which otherwise survive farther downstream, grow to larger sizes, and undergo successive pairings in the corresponding unexcited flow.

Zaman, K. B. M. Q.↗
NASA NTRS1986

Theoretical and material studies on thin-film electroluminescent devices

A theoretical study of resonant tunneling in multilayered heterostructures is presented based on an exact solution of the Schroedinger equation under the application of a constant electric field. By use of the transfer matrix approach, the transmissivity of the structure is determined as a function of the incident electron energy. The approach presented is easily extended to many layer structures where it is more accurate than other existing transfer matrix or WKB models. The transmission resonances are compared to the bound state energies calculated for a finite square well under bias using either an asymmetric square well model or the exact solution of an infinite square well under the application of an electric field. The results show good agreement with other existing models as well as with the bound state energies. The calculations were then applied to a new superlattice structure, the variablly spaced superlattice energy filter, (VSSEP) which is designed such that under bias the spatial quantization levels fully align. Based on these calculations, a new class of resonant tunneling superlattice devices can be designed.

Summers, C. J.↗
NASA NTRS1980

Structures and textures of the Murchison and Mighei carbonaceous chondrite matrices

High-resolution transmission electron microscopy has confirmed earlier observations that the character of the Murchison and Mighei fine-grained matrices is complex in mineralogy and texture. Layer structure minerals occur as planar laths, rounded grains or subhedral grains, and range in size from less than 100 A to about 1 micrometer. Serpentine-type and brucite-type structures predominate in the CM matrices. The occurrence of Povlen chrysolite and a vein of disordered mixed-layer and brucite-type material cutting a large lizardite-type grain suggests that at least some of the matrix materials were formed by alteration of preexisting material.

Mackinnon, I. D. R.↗
DOE OSTI2019

Control over the Magnetic Properties of Co/Pt-based Multilayered Periodical Structures

The possibility of controlling the magnetic properties of multilayered periodical structures with perpendicular magnetic anisotropy, which are based on cobalt and platinum films, have been studied. The multilayered films composed by layers with a thickness of 0.5–1.0 nm were subjected to two types of actions: vacuum annealing at different temperatures and irradiation by helium ion beams. Transmission electron microscopy has shown that the irradiation by He{sup +} ions with energy of 30 keV leads to material mixing in the layers since at vacuum annealing the layered structure of films is kept. In this case, as a result of thermal annealing, the coercive force of the structure increases significantly, and upon irradiation with helium ions, the coercivity of the films decreases to a change in the type of anisotropy from perpendicular to “easy plane” anisotropy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Absence of hydrogen insertion into highly crystalline superconducting infinite layer nickelates

Here, the discovery of superconductivity in the infinite layer nickelates introduced a materials system analogous to the cuprates for the study of unconventional superconductivity. The synthesis of infinite layer nickelates, (RNiO 2 , R = lanthanide) often uses calcium hydride (CaH 2 ) to facilitate the deintercalation of apical site oxygen atoms from a precursor perovskite (RNiO 3 ) phase via topotactic reduction. However, it remains uncertain whether the use of CaH 2 results in the insertion of hydrogen into the infinite layer structure, and if it does, what the implications are for superconductivity. To quantify the hydrogen composition of highly crystalline infinite layer nickelates, we synthesized Nd 1-x⁢ Sr x ⁢NiO 2 thin films on LSAT substrates and conducted time-of-flight secondary ion mass spectroscopy measurements to generate hydrogen depth profiles. We compare the hydrogen density of nickelates prepared with and without a SrTiO 3 capping layer. Additionally, we measure the hydrogen content in nickelate samples at various doping levels spanning the superconducting phase space, including the underdoped, optimally doped, and overdoped regime. We report no significant increase in hydrogen density between the perovskite and infinite layer phases in any of the measured samples. Furthermore, we put an upperbound on the hydrogen concentration of our nickelate samples to Nd 1-x Sr x ⁢NiO 2 ⁢H 0.05 . Our results imply that hydrogen is not responsible for the emergence of superconductivity in the infinite layer nickelates.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Joint Inversion of Surface Electrical Resistivity Tomography and Seismic Refraction Data between the 200 Areas

Geologic stratigraphy on the Hanford Site influences groundwater and contaminant migration through the aquifer system and the vadose zone. The current geologic framework model (GFM) relies heavily on a sparse distribution of borehole data in some locations to map geologic contacts and hydrologic properties in the subsurface. Non-invasive geophysical methods such as electrical resistivity tomography (ERT), transient electromagnetic surveying, and seismic imaging are being used at Hanford to map subsurface structure in areas with limited well observations. This is to develop and mature the capability of geophysical methods to aid in GFM refinement, to identify regions of subsurface complexity, and for optimal well siting. A joint inversion of co-located seismic refraction and ERT data was carried out for data collected on a ~2.3-km profile between the 200 Areas on the Hanford Site. While ERT and seismic refraction images have sensitivity to overlapping physical properties (porosity, moisture content, lithology), the resolution and physics used to acquire each of these datasets are different and therefore information can be different or mutually complementary. Performing a joint inversion provides a reasonable option for a coherent, coupled interpretation for mutually complementary datasets. Between the 200 Areas, there are few boreholes to interpret the geologic framework model, and these data sets were obtained to provide a first line of evidence toward identifying stratigraphic structure. The seismic refraction and ERT data were independently inverted during fiscal year 2022 and broadly showed a two-layer structure with a trough-like feature that is ~1 km wide and upwards of 150 m deep. The depth of the trough feature was greater in the ERT image compared to the seismic image, which indicated a maximum depth of approximately 110 m. The objective of the joint inversion described in this report was to invert the seismic refraction and ERT data together while constraining the ERT image to be structurally similar to the seismic refraction image. The approach was applied using the geophysical inverse modeling program E4D, which has the capability to invert first-arrival times from seismic refraction data and ERT resistances using a “cross-gradient” constraint. The application of cross-gradient constraints with different weights produces ERT models that show a high degree of similarity within the upper 100 m (above ~120 m elevation). None of the ERT models show an improved structural similarity to the seismic result; therefore, it is recommended that further attempts to jointly interpret these models focus on petrophysics and image resolution. Petrophysical measurements of core samples would improve knowledge of what drives the ERT response in this region and, along with downhole geophysical measurements, could be used to “ground truth” the surface-based geophysical results. Image resolution studies would provide insight into which regions of the inverted images are reliable and which regions are poorly constrained.

58 GEOSCIENCES↗
NASA NTRS1987

Theory of resonant tunneling in a variably spaced multiquantum well structure - An Airy function approach

A theoretical study of resonant tunneling in multilayered heterostructures is presented based on an exact solution of the Schroedinger equation under the application of a constant electric field. By use of the transfer matrix approach, the transmissivity of the structure is determined as a function of the incident electron energy. The approach presented herein is easily extended to many layer structures where it is more accurate than other existing transfer matrix or Wentzel-Kramers-Brillouin (WKB) models. The transmission resonances are compared to the bound-state energies calculated for a finite square well under bias using either an asymmetric square-well model or the exact solution of an infinite square well under the application of an electric field. The results show good agreement with other existing models as well as with the bound-state energies. The calculations were then applied to a new superlattice structure, the variably spaced superlattice energy filter, which is designed such that under bias the spatial quantization levels fully align. Based on these calculations, a new class of resonant tunneling superlattice devices can be designed.

Brennan, K. F.↗
NASA NTRS1988

Turbulence production near walls: The role of flow structures with spanwise asymmetry

Space-time evolution of near wall flow structures is described by conditional sampling methods, in which conditional averages are formed at various stages of development of shear layer structures. The development of spanwise asymmetry of the structures was found to be important in the creation of the structures and for the process of turbulence production.

Alfredsson, P. Henrik↗
NASA NTRS2010

Fabrication of nanobaskets by sputter deposition on porous substrates and uses thereof

A method of producing a nanobasket and the applications or uses thereof. The method includes the steps of providing a substrate with at least one (1) pore having diameters of about one (1) nanometer to about ten (10) micrometers. Material is deposited by sputter-coating techniques along continuous edges of the pores to form a capped or partially capped nanotube or microtube structure, termed a nanobasket. Either a single material may be used to form nanobaskets over the pores or, alternately, a layered structure may be created wherein an initial material is deposited followed by one or more other materials to form nanobaskets over the pores.

Johnson, Paige Lea↗
NASA NTRS2013

Total Lightning Observations within Electrified Snowfall using Polarimetric Radar LMA, and NWN Measurements

Tall structures play and important role in development of winter time lightning flashes.To what extent still needs to be assessed. Tower initiated flashes typically occur as banded structures pass near/overhead. Hi resolution RHI s from polarimetric radar show that the lightning has a tendency to propagate through layered structures within these snowstorms.

Schultz, Christopher J.↗
NASA NTRS2006

The Dryline on 22 May 2002 during IHOP_2002: Convective-Scale Measurements at the Profiling Site

A detailed analysis of the structure of a double dryline observed over the Oklahoma panhandle during the first International H2O Project (IHOP_2002) convective initiation (CI) mission on 22 May 2002 is presented. A unique and unprecedented set of high temporal and spatial resolution measurements of water vapor mixing ratio, wind, and boundary layer structure parameters were acquired using the National Aeronautics and Space Administration (NASA) scanning Raman lidar (SRL), the Goddard Lidar Observatory for Winds (GLOW), and the Holographic Airborne Rotating Lidar Instrument Experiment (HARLIE), respectively. These measurements are combined with the vertical velocity measurements derived from the National Center for Atmospheric Research (NCAR) Multiple Antenna Profiler Radar (MAPR) and radar structure function from the high-resolution University of Massachusetts frequency-modulated continuous-wave (FMCW) radar to reveal the evolution and structure of the late afternoon double-dryline boundary layer. The eastern dryline advanced and then retreated over the Homestead profiling site in the Oklahoma panhandle, providing conditions ripe for a detailed observation of the small-scale variability within the boundary layer and the dryline. In situ aircraft data, dropsonde and radiosonde data, along with NCAR S-band dual-polarization Doppler radar (S-Pol) measurements, are also used to provide the larger-scale picture of the double-dryline environment. Moisture and temperature jumps of about 3 g kg(sup -1) and 1 -2 K, respectively, were observed across the eastern radar fine line (dryline), more than the moisture jumps (1-2 g kg(sup -1)) observed across the western radar fine line (secondary dryline). Most updraft plumes observed were located on the moist side of the eastern dryline with vertical velocities exceeding 3 m s(sup -1) and variable horizontal widths of 2-5 km, although some were as wide as 7-8 km. These updrafts were up to 1.5 g kg(sup -1) moister than the surrounding environment. Although models suggested deep convection over the Oklahoma panhandle and several cloud lines were observed near the dryline, the dryline itself did not initiate any storms over the intensive observation region (IOR). Possible reasons for this lack of convection are discussed. Strong capping inversion and moisture detrainment between the lifting condensation level and the level of free convection related to an overriding drier air, together with the relatively small near-surface moisture values (less than 10 g kg(sup -1)), were detrimental to CI in this case.

Demoz, Belay↗
NASA NTRS1990

FIRE aircraft observations of horizontal and vertical transport in marine stratocumulus

A major goal of research on marine stratocumulus is to try to understand the processes that generate and dissipate them. One approach to studying this problem is to investigate the boundary layer structure in the vicinity of a transition from a cloudy to a cloud-free region to document the differences in structure on each side of the transition. Since stratiform clouds have a major impact on the radiation divergence in the boundary layer, the transition from a cloudy to a clear boundary layer is a region of large horizontal inhomogeneity in air temperature and turbulence intensity. This leads to a considerable difference in horizontal and vertical transports between the cloudy and cloud-free regions. Measurements are used from the NCAR Electra aircraft during flights 5 (7 July 1987) and 10 (18 July 1987) of FIRE for this purpose. Flight 5 coincided with a LANDSAT overflight, and was designed to investigate the transition across a well-defined N-S cloud boundary, since the LANDSAT image can document the cloud cover in considerable detail. Turbulence legs were flown about 60 km on both sides of the cloud boundary. Flight 10 was flown at night in an area of scattered small cumuli and broken cloud patches.

Paluch, Ilga R.↗
NASA NTRS1991

The symmetric turbulent plane wake downstream of a sharp trailing edge

The analysis and modeling of the symmetric turbulent plane wake downstream of a sharp trailing edge is addressed. A compact description of the flow near the trailing edge is formulated using the results of a previous asymptotic analysis. The new description retains the two-layered structure identified in the previous work, and it clarifies the principal dynamics of the flow in the near-wake outer layer, away from the wake centerline. For zero-pressure-gradient flow, the near-wake outer layer is shown to be represented to leading order by the similarity solution that governs the outer region of the surface boundary layer. The leading perturbation in the outer layer due to the developing near-wake inner-layer flow is identified, and this is shown to be asymptotically smaller than undetermined higher-order terms associated with the surface boundary-layer flow. Results of the new near-wake analysis are used to formulate an algebraic eddy viscosity model for wake flow predictions at arbitrary distances from the trailing edge. The model is used in a numerical solution of the boundary layer equations, and computed velocity and Reynolds stress profiles are shown to compare well with experimental data.

Bogucz, E. A.↗
NASA NTRS2004

Progress of Multicolor Single Detector to Detector Array Development for Remote Sensing

Knowledge of the spatial and temporal distribution of atmospheric species such as CO2, O3, H2O, and CH4 is important for understanding the chemistry and physical cycles involving Earth s atmosphere. Although several remote sensing techniques are suitable for such measurements they are considered high cost techniques involving complicated instrumentation. Therefore, simultaneous measurement of atmospheric species using a single remote sensing instrument is significant for minimizing cost, size and complexity. While maintaining the instrument sensitivity and range, quality of multicolor detector, in terms of high quantum efficiency and low noise are vital for these missions. As the first step for developing multicolor focal plan array, the structure of a single element multicolor detector is presented in this paper. The detector consists of three p-n junction layers of Si, GaSb and InAs wafer bonded to cover the spectral range UV to 900 nm, 800 nm to 1.7 m, and 1.5 m to 3.4 m, respectively. Modeling of the absorption coefficient for each material was carried out for optimizing the layers thicknesses for maximum absorption. The resulted quantum efficiency of each layer has been determined except InAs layer. The optical and electrical characterization of each layer structure is reported including dark current and spectral response measurements of Si pin structure and of GaSb and InAs p-n junctions. The effect of the material processing is discussed.

Abedin, M. Nurul↗