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At least 397 records · Page 22

Validation of clear-sky fluxes for tropical oceans from the Earth Radiation Budget Experiment

The existence and magnitude of a systematic bias in the clear-sky longwave fluxes from the Earth Radiation Budget Experiment (ERBE) is investigated. The bias is apparently introduced because the ERBE method for scene identification does not account for large zonal gradients in longwave absorption by water vapor. The ERBE fluxes are compared to fluxes calculated with a radiative transfer model from ship radiosonde measurements. The comparison is based upon an analysis of 5 yr of coincident satellite and radiosonde observations for equatorial ocean regions. The differences between the ERBE and model fluxes are examined as functions of sea surface temperature (SST) and relative humidity. The authors use height-mean relative humidity bar-RH as an index of atmospheric moisture. The average offset between and model ERBE fluxes ranges between +2 and +6 W/sq m for SSTs above 295 K, and the gradients with respect to SST are nearly identical. However, the difference between the model and ERBE depends significantly on the tropospheric relative humidity. ERBE fluxes exceed model fluxes for bar-RH above 70%, and the maximum offset of +9 to +12 W/sq m is consistent with previous estimates. There are also indications that the clear-sky fluxes for bar-RH below 25% may be underestimated by about 10-15 W/sq m. Since extreme values of height-mean humidity are relatively infrequent, the net bias introduced in the ERBE monthly mean clear-sky fluxes is generally less than the systematic error in estimates introduced in the ERBE monthly mean clear-sky fluxes is generally less than the systematic error in estimates of the instantaneous fluxes. These findings support earlier work on the coupling between SST and the atmospheric greenhouse effect, in particular the existence of a super greenhouse effect for oceans warmer than 300 K. Recent reports of much larger systematic differences are not supported by this analysis. The results indicate that comparison of general circulation model (GCM) and ERBE clear-sky longwave fluxes will depend explicitly on atmospheric humidity.

Collins, W. D.↗

Sensitivity of the Tropical Pacific Ocean to Precipitation Induced Freshwater Flux

We have performed a series of experiments using an ocean model to study the sensitivity of tropical Pacific Ocean to variations in precipitation induced freshwater fluxes. Variations in these fluxes arise from natural causes on all time scales. In addition, estimates of these fluxes are uncertain because of differences among measurement techniques. The model used is a quasi-isopycnal model, covering the Pacific from 40 S to 40 N. The surface forcing is constructed from observed wind stress, evaporation, precipitation, and surface temperature (SST) fields. The heat flux is produced with an iterative technique so as to maintain the model close to the observed climatology, but with only a weak damping to that climatology. Climatological estimates of evaporation are combined with various estimates of precipitation to determine the net surface freshwater flux. Results indicate that increased freshwater input decreases salinity as expected, but increases temperatures in the upper ocean. Using the freshwater flux estimated from the Microwave Sounding Unit leads to a warming of up to 0.6 C in the western Pacific over a case with zero net freshwater flux. SST is sensitive to the discrepancies among different precipitation observations, with root-mean-square differences in SST on the order of 0.2-0.3 C. The change in SST is more pronounced in the eastern Pacific, with differences of over 1 C found among the various precipitation products. Interannual variation in precipitation during El Nino events leads to increased warming. During the winter of 1982-83, freshwater flux accounts for about 0.4 C (approximately 10-15% of the maximum warming) of the surface warming in the central-eastern Pacific. Thus, the error of SST caused by the discrepancies in precipitation products is more than half of the SST anomaly produced by the interannual variability of observed precipitation. Further experiments, in which freshwater flux anomalies are imposed in the western, central, and eastern Pacific, show that the influence of net freshwater flux is also spatially dependent. The imposition of freshwater flux in the far western Pacific leads to a trapping of salinity anomaly to the surface layers near the equator. An identical flux imposed in the central Pacific produces deeper and off-equatorial salinity anomalies. The contrast between these two simulations is consistent with other simulations of the western Pacific barrier layer information.

Yang, Song↗

Variability of Fram Strait Ice Flux and North Atlantic Oscillation

An important term in the mass balance of the Arctic Ocean sea ice is the ice export. We estimated the winter sea ice export through the Fram Strait using ice motion from satellite passive microwave data and ice thickness data from moored upward looking sonars. The average winter area flux over the 18-year record (1978-1996) is 670,000 square km, approximately 7% of the area of the Arctic Ocean. The winter area flux ranges from a minimum of 450,000 sq. km in 1984 to a maximum of 906,000 sq km in 1995. The daily, monthly and interannual variabilities of the ice area flux are high. There is an upward trend in the ice area flux over the 18-year record. The average winter volume flux over the winters of October 1990 through May 1995 is 1745 cubic km ranging from a low of 1375 cubic km in 1990 to a high of 2791 cubic km in 1994. The sea-level pressure gradient across the Fram Strait explains more than 80% of the variance in the ice flux over the 18-year record. We use the coefficients from the regression of the time-series of area flux versus pressure gradient across the Fram Strait and ice thickness data to estimate the summer area and volume flux. The average 12-month area flux and volume flux are 919,000 sq km and 2366 cubic km. We find a significant correlation (R =0.86) between the area flux and positive phases of the North Atlantic Oscillation (NAO) index over the months of December through March. Correlation between our six years of volume flux estimates and the NAO index gives R =0.56. During the high NAO years, a more intense Icelandic low increases the gradient in the sea-level pressure by almost 1 mbar across the Fram Strait thus increasing the atmospheric forcing on ice transport. Correlation is reduced during the negative NAO years because of decreased dominance of this large-scale atmospheric pattern on the sea-level pressure gradient across the Fram Strait. Additional information is contained in the original.

Kwok, Ron↗

Mass and Ozone Fluxes from the Lowermost Stratosphere

Net mass flux from the stratosphere to the troposphere can be computed from the heating rate along the 380K isentropic surface and the time rate of change of the mass of the lowermost stratosphere (the region between the tropopause and the 380K isentrope). Given this net mass flux and the cross tropopause diabatic mass flux, the residual adiabatic mass flux across the tropopause can also be estimated. These fluxes have been computed using meteorological fields from a free-running general circulation model (FVGCM) and two assimilation data sets, FVDAS, and UKMO. The data sets tend to agree that the annual average net mass flux for the Northern Hemisphere is about 1P10 kg/s. There is less agreement on the southern Hemisphere flux that might be half as large. For all three data sets, the adiabatic mass flux is computed to be from the upper troposphere into the lowermost stratosphere. This flux will dilute air entering from higher stratospheric altitudes. The mass fluxes are convolved with ozone mixing ratios from the Goddard 3D CTM (which uses the FVGCM) to estimate the cross-tropopause transport of ozone. A relatively large adiabatic flux of tropospheric ozone from the tropical upper troposphere into the extratropical lowermost stratosphere dilutes the stratospheric air in the lowermost stratosphere. Thus, a significant fraction of any measured ozone STE may not be ozone produced in the higher Stratosphere. The results also illustrate that the annual cycle of ozone concentration in the lowermost stratosphere has as much of a role as the transport in the seasonal ozone flux cycle. This implies that a simplified calculation of ozone STE mass from air mass and a mean ozone mixing ratio may have a large uncertainty.

Schoeberl, Mark R.↗

Coronal Flux Ropes and their Interplanetary Counterparts

We report on a study comparing coronal flux ropes inferred from eruption data with their interplanetary counterparts constructed from in situ data. The eruption data include the source region magnetic field, post-eruption arcades, and coronal mass ejections (CMEs). Flux ropes were fit to the interplanetary CMEs (ICMEs) considered for the 2011 and 2012 Coordinated Data Analysis Workshops (CDAWs). We computed the total reconnected flux involved in each of the associated solar eruptions and found it to be closely related to flare properties, CME kinematics, and ICME properties. By fitting flux ropes to the white-light coronagraph data, we obtained the geometric properties of the flux ropes and added magnetic properties derived from the reconnected flux. We found that the CME magnetic field in the corona is significantly higher than the ambient magnetic field at a given heliocentric distance. The radial dependence of the flux rope magnetic field strength is faster than that of the ambient magnetic field. The magnetic field strength of the coronal flux rope is also correlated with that in interplanetary flux ropes constructed from in situ data, and with the observed peak magnetic field strength in ICMEs. The physical reason for the observed correlation between the peak field strength in MCs is the higher magnetic field content in faster coronal flux ropes and ultimately the higher reconnected flux in the eruption region. The magnetic flux ropes constructed from the eruption data and coronagraph observations provide a realistic input that can be used by various models to predict the magnetic properties of ICMEs at Earth and other destination in the heliosphere.

Gopalswamy, N.↗

The Effects of Different Footprint Sizes and Cloud Algorithms on the Top-Of-Atmosphere Radiative Flux Calculation from the Clouds and Earth’s Radiant Energy System (CERES) Instrument on Suomi National Polar-Orbiting Partnership (NPP)

Only one Clouds and Earth’s Radiant Energy System (CERES) instrument is onboard the Suomi National Polar-orbiting Partnership (NPP) and it has been placed in cross-track mode since launch; it is thus not possible to construct a set of angular distribution models (ADMs) specific for CERES on NPP. Edition 4 Aqua ADMs are used for flux inversions for NPP CERES measurements. However, the footprint size of NPP CERES is greater than that of Aqua CERES, as the altitude of the NPP orbit is higher than that of the Aqua orbit. Furthermore, cloud retrievals from the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Moderate Resolution Imaging Spectroradiometer (MODIS), which are the imagers sharing the spacecraft with NPP CERES and Aqua CERES, are also different. To quantify the flux uncertainties due to the footprint size difference between Aqua CERES and NPP CERES, and due to both the footprint size difference and cloud property difference, a simulation is designed using the MODIS pixel-level data, which are convolved with the Aqua CERES and NPP CERES point spread functions (PSFs) into their respective footprints. The simulation is designed to isolate the effects of footprint size and cloud property differences on flux uncertainty from calibration and orbital differences between NPP CERES and Aqua CERES. The footprint size difference between Aqua CERES and NPP CERES introduces instantaneous flux uncertainties in monthly gridded NPP CERES measurements of less than 4.0 W/sq. m for SW (shortwave) and less than 1.0 W/sq. m for both daytime and nighttime LW (longwave). The global monthly mean instantaneous SW flux from simulated NPP CERES has a low bias of 0.4 W/sq. m when compared to simulated Aqua CERES, and the root-mean-square (RMS) error is 2.2 W/sq. m between them; the biases of daytime and night- time LW flux are close to zero with RMS errors of 0.8 and 0.2 W/sq. m. These uncertainties are within the uncertainties of CERES ADMs. When both footprint size and cloud property (cloud fraction and optical depth) differences are considered, the uncertainties of monthly gridded NPP CERES SW flux can be up to 20 W/sq. m in the Arctic regions where cloud optical depth retrievals from VIIRS differ significantly from MODIS. The global monthly mean instantaneous SW flux from simulated NPP CERES has a high bias of 1.1 W/sq. m and the RMS error increases to 5.2 W/sq. m. LW flux shows less sensitivity to cloud property differences than SW flux, with uncertainties of about 2 W/sq. m in the monthly gridded LW flux, and the RMS errors of global monthly mean daytime and nighttime fluxes increase only slightly. These results highlight the importance of consistent cloud retrieval algorithms to maintain the accuracy and stability of the CERES climate data record.

Su, Wenying↗

LOFTID Heat Flux Gauge Calibration: What is Truth?

The Low-Earth Orbit Flight Test of an Inflatable Decelerator (LOFTID) is a demonstration of Hypersonic Inflatable Aerodynamic Decelerator (HIAD) technology, which may enable the delivery of heavy payloads to Mars, Venus, and Titan, as well as return to Earth. Unlike rigid aeroshells that are constrained by the size of the rocket’s shroud, inflatable aeroshells can be deployed to a much larger scale, thus allowing a spacecraft to begin its deceleration earlier and experience less heating. On LOFTID, there will be 4 total heat flux gauges (HFG) with a range of 70 W/cm2 and 1 radiometer with a range of 3 W/cm2, arranged as shown in Fig. 1. Both the radiometer and total HFGs are Schmidt-Boelter gauges purchased from an external vendor. Radiative calibrations were performed in-house at NASA Ames’ Sensors and TPS Advanced Research Laboratories (STAR Labs) before and after environmental testing to investigate how the testing affected the sensors' response. Additional rounds of radiative calibration at STAR Labs were also performed in order to investigate the large uncertainties associated with these tests. For example, a survey of multiple calibration facilities concluded that the uncertainty within a given facility was +/-3% [1]. An additional NIST study that calibrated heat flux gauges at 7 different facilities also found the variation in calibration coefficients to be up to ~3% within a given facility, but up to 15% between facilities, suggesting systematic differences between test setups [2]. Finally, the response of heat flux gauges to radiative versus convective heat flux has shown to differ by up to 20% [3],[4]. Because the heat flux gauges on LOFTID will predominantly experience convective heat flux during flight, a convective calibration study was performed at Boeing's Large-Core Arc Tunnel (LCAT) facility. Radiative Calibration Procedure The calibrations performed at STAR Labs utilize a quartz lamp bank (QLB) that provides a maximum heat flux of 50 W/cm2, which bounds the expected LOFTID flight environment. The calibration involves exposing a water-cooled Gardon gauge (reference) and then the unit-under-test (UUT) to 5 different heat fluxes multiple times for 10 seconds each, and then calculating a linear fit. The test setup is shown in Fig. 2. The total HFGs were calibrated at STAR Labs 3 times, denoted as STAR 1 (before environmental testing), STAR 2 (after protoflight vibration and thermal-vacuum testing), and STAR 3 (no change from previous test). All 8 flight-lot total HFGs showed a decrease in full-scale output from STAR 1 to STAR 2 by between 0.5% and 10. The first portion of this investigation was to determine whether the change could be due to differences in temperature between the two calibration runs. A typical linear fit to the calibration data was performed using Eq. 1 where q’ is the heat flux in W/cm2, c is the calibration coefficient, and mV is the sensor output. To account for temperature, the data were fit to a nonlinear function that included both the sensor output (mV) and the temperature from the thermocouple embedded inside the HFG near the surface (T): q'=mV/(c1* T + c0}. The residuals between the fits and the actual data points were calculated for every point, and proven to be much smaller for the temperature-compensated fits than for the linear fits for all sensors. An example is shown in Fig. 3. When the temperature-compensated fits from STAR 1 were applied to the STAR 2 data, the residuals did not improve, suggesting that the change in sensitivity between these two calibration runs was not due to temperature. A third round of calibration (STAR 3) was conducted to further address the temperature dependence of the total HFGs, and the resulting sensitivities matched closely to STAR 2 (within 2%). Temperature-compensated calibration curves were once again fit to the data. In this case, when the temperature-compensated fits from STAR 3 were applied to STAR 2 data, the residuals between the fits and STAR 2 data were much lower than the residuals due to the linear fits. This suggests that the changes seen between STAR 1 and STAR 2 were likely due to actual changes in the sensors caused by the environmental testing between the two calibrations. A modification of the original calibration process, in which the UUT was exposed to each heat flux for just 3 seconds (instead of 10) to reduce the temperature increase during the test, was additionally performed on several of the HFGs. In general, the sensitivities were 1-1.5% lower than from the 10-second tests, but the temperatures were also significantly lower. When the temperature-compensated fits from the 10-second tests were applied to the 3-second test data, the residuals were greatly improved than when just using the linear fits, further suggesting that the temperature-compensated fits may lead to better accuracy than the linear fits in flight. Convective Calibration The second portion of this study was to create a mapping between the radiative and convective calibration coefficients. The majority of the heating during flight will be convective, so it is important to understand how the HFG response differs under these conditions. However, there are no standardized methods for convective calibration [5]. Because the TPS aerothermal response models were validated at LCAT, the same facility was chosen for convective calibration of two of the total HFGs (Fig. 4). Preliminary results showed that the full-scale output was 3% and 8% higher in convective heat flux as compared to radiative heat flux. However, tunnel variation may have contributed to noise and uncertainty in the measurements, and more testing and analysis remains to be done. Scope of Presentation The presentation will include an overview of the changes seen in HFG calibration before and after environmental testing, differences between radiative and convective calibrations, the modeling work done to aid in understanding the sensor response to varying environments, and recommended future work.

H S Alpert↗

Modeling the Effect of Evaporative Flux and Colloidal Aggregation on Crud Deposition

During the last few years lot of research has been conducted to investigate and predict the Crud deposition in PWRs. One of the common findings of various experimental and computational studies is that thickness or amount of crud deposits is directly related to evaporative flux maps. Evaporation driven deposition profile on the surfaces takes different forms, i.e. from ring to disk shapes during initial stages and in the form of porous to impervious continuous layers covering the hot fuel surface at the later stages. The amount and thickness of these deposits although are directly related to evaporative flux, the relationship is much complex and can be dependent upon several other factors. A popular problem relating evaporative flux to particulate deposition has been well studied in the form of drying of sessile colloidal drops. It was proposed that, this phenomenon is due to a geometrical constraint: the free surface, constrained by a pinned contact line squeezes the fluid outwards to compensate for evaporative losses and thereby transporting particles to the contact line. Later on a quantitative relationship between evaporative flux and deposition rate was proposed and validated by the same group, which showed power-law relationship. Deposition studies conducted with controlled concentration of particles with subcooled nucleate boiling also showed a power-law relationship rather than a simpler linear relationship whereas physics of evaporation would tend to concentrate particles at linear rate. In a typical subcooled nucleate boiling system, bubble growth and departure time is of the order 1-2 ms, measured experimentally. Diffusion time constant for dilute spherical metallic colloids such as crud particulates, generally present as particulate in process piping, range from 0.0025-2.5 sec in water for a size range 0.1-1.0 μm. Colloidal behavioral characteristics during the growth of bubbles can be computed with escape time constant at collision, which is dependent on effective Hamaker constant. For minimum effective Hamaker constant of Hematite is -2.5 kT and diffusion time constant τ = 0.0025 sec, escape time constant is computed as Kramer rule, τexp[A/kT] magnitude is 0.03 sec or 30 ms. This clearly indicates that evaporation will cause particles to come together and they cannot escape at a fast enough rate which would lead them to form agglomerates. Therefore both effects of evaporative flux in conjunction with the agglomeration kinetics must be considered for modeling the crud deposition if the evaporative flux is known. In this paper, we propose a phenomenological model of colloidal transport and aggregation with evaporative flux. The dynamic of particles interactions while drying of sessile colloidal drops is developed by coupling general transport equation with Smoluchowshki Coagulation equation. Crud deposition on the nuclear fuel has been a serious problem with severe consequences in nuclear power plants. In several studies it has been consistently reported that crud deposition is directly related to evaporative flux on the nuclear fuel surfaces. However, it has not been established how to quantify the deposition rates of crud type particulates if the evaporative flux is known. This complex multiphysics problem is similar to coffee-ring effect, where the governing physics is understood more clearly. In this work, a simplified geometry is used to model the effects of evaporative flux acting at a boundary on the colloidal concentration. The effect of this condition on change in concentration is shown numerically. Further, agglomeration is suspected to play a significant role in high evaporative flux such as bubble nucleation. The coagulation kinetics is modeled using uniform particle distribution and the effective total concentration of colloids including original particles and agglomerates is studied. Once this model is validated with a simple separate effect experiments, it can be integrated to large scale PWR models of evaluating evaporative flux and chemistry models developed by Electrical Power Research Institute (EPRI). (authors)

42 ENGINEERING↗

Systematic comparison of local approaches for isotopically nonstationary metabolic flux analysis

Quantification of reaction fluxes of metabolic networks can help us understand how the integration of different metabolic pathways determine cellular functions. Yet, intracellular fluxes cannot be measured directly but are estimated with metabolic flux analysis (MFA) that relies on the patterns of isotope labeling of metabolites in the network. For metabolic systems, typical for plants, where all potentially labeled atoms effectively have only one source atom pool, only isotopically nonstationary MFA can provide information about intracellular fluxes. There are several global approaches that implement MFA for an entire metabolic network and estimate, at once, a steady-state flux distribution for all reactions with identifiable fluxes in the network. In contrast, local approaches deal with estimation of fluxes for a subset of reactions, with smaller data demand for flux estimation. Here we present a systematic comparative review and benchmarking of the existing local approaches for isotopically nonstationary MFA. The comparison is conducted with respect to the required data and underlying computational problems solved on a synthetic network example. Furthermore, we benchmark the performance of these approaches in estimating fluxes for a subset of reactions using data obtained from the simulation of nitrogen fluxes in the Arabidopsis thaliana core metabolism. The findings pinpoint practical aspects that need to be considered when applying local approaches for flux estimation in large-scale plant metabolic networks.

59 BASIC BIOLOGICAL SCIENCES↗

High-Frequency Greenhouse Gas Flux Measurement System Detects Winter Storm Surge Effects on Salt Marsh

The physical controlling factors on coastal plant communities are among the most dynamic of known ecosystems, but climate change alters coastal surface and subsurface hydrologic regimes, which makes rapid measurement of greenhouse gas fluxes critical. Greenhouse gas exchange rates in these terrestrial–aquatic ecosystems are highly variable worldwide with climate, soil type, plant community, and weather. Therefore, increasing data collection and availability should be a priority. Here, we demonstrate and validate physical and analytical modifications to automated soil–flux chamber measurement methods for unattended use in tidally driven wetlands, allowing the high–frequency capture of storm surge and day/night dynamics. Winter CO 2 flux from Sarcocornia perennis marsh to the atmosphere was significantly greater during the day (2.8 mg m –2 h –1 ) than the night (2.2 mg m –2 h –1 ) (p < 0.001), while CH 4 was significantly greater during the night (0.16 μg m –2 h –1 ) than the day (–0.13 μg m –2 h –1 ) (p = 0.04). The magnitude of CO 2 flux during the day and the frequency of CH 4 flux were reduced during a surge (p < 0.001). Surge did not significantly affect N 2 O flux, which without non–detects was normally distributed around –24.2 ng m –2 h –1 . Analysis of sustained–flux global potentials for increased storm surge frequency scenarios, 2020 to 2100, suggested that the marsh in winter remains an atmospheric CO 2 sink. The modeled results showed an increased flux of CO 2 to the atmosphere, while in soil, the uptake of CH 4 increased and N 2 O uptake decreased. We present analytical routines to correctly capture gas flux curves in dynamic overland flooding conditions and to flag data that are below detection limits or from unobserved chamber–malfunction situations. Storm surge is an important phenomenon globally, but event–driven, episodic factors can be poorly estimated by infrequent sampling. Here, deployment of this system in coastal marshes worldwide would permit its inclusion in flux calculations.

54 ENVIRONMENTAL SCIENCES↗

Effects of B{sub 2}O{sub 3} on Crystallization, Structure, and Heat Transfer of CaO-Al{sub 2}O{sub 3}-Based Mold Fluxes

The reaction between traditional CaO-SiO{sub 2}-based mold fluxes and high-Al steel inevitably changes flux composition, and, consequently, flux properties. This problem can be mitigated by using CaO-Al{sub 2}O{sub 3}-based mold fluxes. To maintain appropriate melting properties, CaO-Al{sub 2}O{sub 3}-based mold fluxes contain B{sub 2}O{sub 3}, which is an effective fluxing agent that decreases the liquidus temperature. In this article, the effects of B{sub 2}O{sub 3} on crystallization behavior, structure, and heat transfer of CaO-Al{sub 2}O{sub 3}-based mold fluxes were studied using single/double hot thermocouple technique, Raman spectroscopy, and infrared emitter technique. The increase of B{sub 2}O{sub 3} content from 7.6 to 13.1 mass pct suppressed the crystallization tendency of mold fluxes in continuous cooling experiments and isothermal experiments conducted over 1273 K (1000 °C). The isothermal crystallization below 1273 K (1000 °C) was also inhibited when B{sub 2}O{sub 3} content increased from 7.6 to 9.6 mass pct; but a further increase of B{sub 2}O{sub 3} content to 13.1 mass pct did not show a visible effect on the crystallization tendency. The increase of B{sub 2}O{sub 3} content from 9.6 to 13.1 mass pct improved the heat fluxes under an incident thermal radiation of 1.6 MW/m{sup 2}; however, the increase of B{sub 2}O{sub 3} content from 7.6 to 9.6 mass pct slightly decreased the heat transfer rate. Crystallization of fluxes and heat transfer were discussed in relation to flux structure.

36 MATERIALS SCIENCE↗

Mineral Scale Formation during Crossflow Reverse Osmosis at Constant Flux and Constant Transmembrane Pressure Conditions

Mineral scale formation on membrane surfaces is a significant challenge in reverse osmosis water purification. Laboratory fouling experiments are typically run such that the transmembrane pressure (TMP) is fixed, and the permeate flux decreases over time as scales accumulate on the membrane surface. However, this change in flux means that the hydrodynamic conditions at the membrane surface are continuously changing, which could affect crystallization and foulant deposition processes. Operating under constant permeate flux conditions, in contrast, is advantageous because it keeps the hydrodynamic conditions relatively consistent, making it possible to compare how membrane properties (e.g., surface chemistry) affect fouling propensity. Industrial reverse osmosis operations are not run strictly in either constant TMP or constant flux mode; while they may start at a constant TMP, feed pressure may be periodically adjusted to maintain permeate water production within a specified range. Here, the scarcity of constant permeate flux reverse osmosis scaling experiments reported in the literature frustrates efforts to compare membrane fouling processes under constant TMP and constant flux conditions. For the first time, the evolution of the fouling layer resistance was compared as a function of cumulative permeate volume per membrane area during constant TMP and constant flux reverse osmosis filtrations. Scaling experiments were conducted by challenging commercial reverse osmosis membranes with a model feed solution nearly saturated with calcium sulfate dihydrate (gypsum). At low fluxes, the increase in fouling layer resistance was quantitatively similar for the two operational modes. In contrast, at high fluxes, the fouling layer resistance increased more rapidly in constant flux filtration than in constant TMP filtration. The mechanism of scale formation in constant TMP and constant flux operation was self-limiting and self-reinforcing, respectively.

36 MATERIALS SCIENCE↗

Properties and Acceleration Mechanisms of Electrons Up To 200 keV Associated With a Flux Rope Pair and Reconnection X-Lines Around It in Earth's Plasma Sheet

The properties and acceleration mechanisms of electrons (<200 keV) associated with a pair of tailward traveling flux ropes and accompanied reconnection X-lines in Earth's plasma sheet are investigated with MMS measurements. Energetic electrons are enhanced on both boundaries and core of the flux ropes. The power-law spectra of energetic electrons near the X-lines and in flux ropes are harder than those on flux rope boundaries. Theoretical calculations show that the highest energy of adiabatic electrons is a few keV around the X-lines, tens of keV immediately downstream of the X-lines, hundreds of keV on the flux rope boundaries, and a few MeV in the flux rope cores. The X-lines cause strong energy dissipation, which may generate the energetic electron beams around them. The enhanced electron parallel temperature can be caused by the curvature-driven Fermi acceleration and the parallel electric potential. Betatron acceleration due to the magnetic field compression is strong on flux rope boundaries, which enhances energetic electrons in the perpendicular direction. Electrons can be trapped between the flux rope pair due to mirror force and parallel electric potential. Electrostatic structures in the flux rope cores correspond to potential drops up to half of the electron temperature. The energetic electrons and the electron distribution functions in the flux rope cores are suggested to be transported from other dawn-dusk directions, which is a 3-dimensional effect. The acceleration and deceleration of the Betatron and Fermi processes appear alternately indicating that the magnetic field and plasma are turbulent around the flux ropes.

58 GEOSCIENCES↗

Asymptotic, multigroup flux reconstruction and consistent discontinuity factors

Recent theoretical work has led to an asymptotically derived expression for reconstructing the neutron flux from lattice functions and multigroup diffusion solutions. The leading-order asymptotic term is the standard expression for flux reconstruction, i.e., it is the product of a shape function, obtained through a lattice calculation, and the multigroup diffusion solution. The first-order asymptotic correction term is significant only where the gradient of the diffusion solution is not small. Inclusion of this first-order correction term can significantly improve the accuracy of the reconstructed flux. One may define discontinuity factors (DFs) to make certain angular moments of the reconstructed flux continuous across interfaces between assemblies in 1-D. Indeed, the standard assembly discontinuity factors make the zeroth moment (scalar flux) of the reconstructed flux continuous. The inclusion of the correction term in the flux reconstruction provides an additional degree of freedom that can be used to make two angular moments of the reconstructed flux continuous across interfaces by using current DFs in addition to flux DFs. Thus, numerical results demonstrate that using flux and current DFs together can be more accurate than using only flux DFs, and that making the second angular moment continuous can be more accurate than making the zeroth moment continuous.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NONLINEAR THREE-DIMENSIONAL MAGNETOCONVECTION AROUND MAGNETIC FLUX TUBES

Magnetic flux in the solar photosphere forms concentrations from small scales, such as flux elements, to large scales, such as sunspots. This paper presents a study of the decay process of large magnetic flux tubes, such as sunspots, on a supergranular scale. Three-dimensional nonlinear resistive magnetohydrodynamic numerical simulations are performed in a cylindrical domain, initialized with axisymmetric solutions that consist of a well-defined central flux tube and an annular convection cell surrounding it. As the nonlinear convection evolves, the annular cell breaks up into many cells in the azimuthal direction, allowing magnetic flux to slip between cells away from the central flux tube (turbulent erosion). This lowers magnetic pressure in the central tube, and convection grows inside the tube, possibly becoming strong enough to push the tube apart. A remnant of the central flux tube persists with nonsymmetric perturbations caused by the convection surrounding it. Secondary flux concentrations form between convection cells away from the central tube. Tube decay is dependent on the convection around the tube. Convection cells forming inside the tube as time-dependent outflows will remove magnetic flux. (This is most pronounced for small tubes.) Flux is added to the tube when flux caught in the surrounding convection is pushed toward it. The tube persists when convection inside the tube is sufficiently suppressed by the remaining magnetic field. All examples of persistent tubes have the same effective magnetic field strength, consistent with the observation that pores and sunspot umbrae all have roughly the same magnetic field strength.

79 ASTRONOMY AND ASTROPHYSICS↗

Structures of interplanetary magnetic flux ropes and comparison with their solar sources

Whether a magnetic flux rope is pre-existing or formed in situ in the Sun's atmosphere, there is little doubt that magnetic reconnection is essential to release the flux rope during its ejection. During this process, the question remains: how does magnetic reconnection change the flux-rope structure? In this work, we continue with the original study of Qiu et al. by using a larger sample of flare-coronal mass ejection (CME)-interplanetary CME (ICME) events to compare properties of ICME/magnetic cloud (MC) flux ropes measured at 1 AU and properties of associated solar progenitors including flares, filaments, and CMEs. In particular, the magnetic field-line twist distribution within interplanetary magnetic flux ropes is systematically derived and examined. Our analysis shows that, similar to what was found before, for most of these events, the amount of twisted flux per AU in MCs is comparable with the total reconnection flux on the Sun, and the sign of the MC helicity is consistent with the sign of the helicity of the solar source region judged from the geometry of post-flare loops. Remarkably, we find that about half of the 18 magnetic flux ropes, most of them associated with erupting filaments, have a nearly uniform and relatively low twist distribution from the axis to the edge, and the majority of the other flux ropes exhibit very high twist near the axis, up to ≳ 5 turns per AU, which decreases toward the edge. The flux ropes are therefore not linearly force-free. We also conduct detailed case studies showing the contrast of two events with distinct twist distribution in MCs as well as different flare and dimming characteristics in solar source regions, and discuss how reconnection geometry reflected in flare morphology may be related to the structure of the flux rope formed on the Sun.

79 ASTRONOMY AND ASTROPHYSICS↗

Magnetic flux concentration and zonal flows in magnetorotational instability turbulence

Accretion disks are likely threaded by external vertical magnetic flux, which enhances the level of turbulence via the magnetorotational instability (MRI). Using shearing-box simulations, we find that such external magnetic flux also strongly enhances the amplitude of banded radial density variations known as zonal flows. Moreover, we report that vertical magnetic flux is strongly concentrated toward low-density regions of the zonal flow. Mean vertical magnetic field can be more than doubled in low-density regions, and reduced to nearly zero in high-density regions in some cases. In ideal MHD, the scale on which magnetic flux concentrates can reach a few disk scale heights. In the non-ideal MHD regime with strong ambipolar diffusion, magnetic flux is concentrated into thin axisymmetric shells at some enhanced level, whose size is typically less than half a scale height. We show that magnetic flux concentration is closely related to the fact that the turbulent diffusivity of the MRI turbulence is anisotropic. In addition to a conventional Ohmic-like turbulent resistivity, we find that there is a correlation between the vertical velocity and horizontal magnetic field fluctuations that produces a mean electric field that acts to anti-diffuse the vertical magnetic flux. The anisotropic turbulent diffusivity has analogies to the Hall effect, and may have important implications for magnetic flux transport in accretion disks. The physical origin of magnetic flux concentration may be related to the development of channel flows followed by magnetic reconnection, which acts to decrease the mass-to-flux ratio in localized regions. The association of enhanced zonal flows with magnetic flux concentration may lead to global pressure bumps in protoplanetary disks that helps trap dust particles and facilitates planet formation.

79 ASTRONOMY AND ASTROPHYSICS↗

On the Interaction between Marine Boundary Layer Cellular Cloudiness and Surface Heat Fluxes

The interaction between marine boundary layer cellular cloudiness and surface uxes of sensible and latent heat is investigated. The investigation focuses on the non-precipitating closed-cell state and the precipitating open-cell state at low geostrophic wind speed. The Advanced Research WRF model is used to conduct cloud-system-resolving simulations with interactive surface fluxes of sensible heat, latent heat, and of sea salt aerosol, and with a detailed representation of the interaction between aerosol particles and clouds. The mechanisms responsible for the temporal evolution and spatial distribution of the surface heat fluxes in the closed- and open-cell state are investigated and explained. It is found that the horizontal spatial structure of the closed-cell state determines, by entrainment of dry free tropospheric air, the spatial distribution of surface air temperature and water vapor, and, to a lesser degree, of the surface sensible and latent heat flux. The synchronized dynamics of the the open-cell state drives oscillations in surface air temperature, water vapor, and in the surface fluxes of sensible and latent heat, and of sea salt aerosol. Open-cell cloud formation, cloud optical depth and liquid water path, and cloud and rain water path are identified as good predictors of the spatial distribution of surface air temperature and sensible heat flux, but not of surface water vapor and latent heat flux. It is shown that by enhancing the surface sensible heat flux, the open-cell state creates conditions by which it is maintained. While the open-cell state under consideration is not depleted in aerosol, and is insensitive to variations in sea-salt fluxes, it also enhances the sea-salt flux relative to the closed-cell state. In aerosol-depleted conditions, this enhancement may replenish the aerosol needed for cloud formation, and hence contribute to the perpetuation of the open-cell state as well. Spatial homogenization of the surface fluxes is found to have only a small effect on cloud properties in the investigated cases. This indicates that sub-grid scale spatial variability in the surface flux of sensible and latent heat and of sea salt aerosol may not be required in large scale and global models to describe marine boundary layer cellular cloudiness.

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