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The potential application of the Doppler lidar measurements to the determination of material (e.g., water vapor) and energy budgets, momentum transports, etc., in the environment at all stages and in the development of convective clouds are discussed.
A study of cumulus mergers for three undisturbed untreated days in the summer of 1973 is reported. Mergers produce more than an order of magnitude more rain than unmerged echoes, while mergers of mergers produce still an order of magnitude more rain. Duration, echo area, and rain depths are also compared for merged and unmerged systems, and each day is analyzed individually, indicating a correlation between organization and rain amount. The relevance of mergers to hydrology, weather modification, and the large-scale impacts of convective clouds is discussed.
A series of high-resolution water vapor fields were derived from the 11 and 12 micron channels of the VISSR Atmospheric Sounder (VAS) on GOES-5. The low-level tropospheric moisture content was separated from the surface and atmospheric radiances by using the differential adsorption across the 'split window' along with the average air temperature from imbedded radiosondes. Fields of precipitable water are presented in a time sequence of five false color images taken over the United States at 3-hour intervals. Vivid subsynoptic and mesoscale patterns evolve at 15 km horizontal resolution over the 12-hour observing period. Convective cloud formations develop from several areas of enhanced low-level water vapor, especially where the vertical water vapor gradient relatively strong. Independent verification at radiosonde sites indicates fairly good absolute accuracy, and the spatial and temporal continuity of the water vapor features indicates very good relative accuracy. Residual errors are dominated by radiometer noise and unresolved clouds.
Moisture can play an important if not dominant role in supplying energy to tropical and extra-tropical weather systems. In the tropics where the air is almost saturated only the slightest amount of uplift is required to initiate the release of vast amounts of latent heat to fuel systems as diverse as convective cloud clusters and hurricanes. The role of latent heating on extra-tropical systems is much more subtle. While the primary energy source for synoptic-scale systems is often the release of gravitational potential energy through the sinking of cold air and the rising of warm, it seems that the latent heat that is eventually realized through slow uplift of large masses of air can significantly modify the evolution of the system. An analysis of the energetics of the storm of March 25 to 27, 1978 over the eastern USA to understand the implications of the heat released due to the vast cloudy area associated with warm frontal overrunning was performed.
The relationship between thunderstorm activity during the summer months along coastal regions of the Atlantic and Gulf coasts and the dry sea breeze circulation was investigated. Satellite composites of thunderstorm activity for synoptically undisturbed conditions have been obtained for south Florida for a series of days in the summer of 1983. These data were catalogued into different low level synoptic flow regimes. Five synoptic flow regimes were found from the data. A three-dimensional mesoscale numerical model was used for each sysnoptic flow regime to quantitatively predict the location of enhanced thunderstorm activity. This model includes a parameterization of vegetation and soil moisture feedbacks as well as a sophisticated planetary boundary layer representation. Using the results of the satellite image composites, spatial and temporal characteristics of deep convective cloud patterns and their variation with synoptic flow are described. The results from the numerical model have provided explanations for the observed patterns.
An analysis of available ozone data in the eastern two-thirds of the United States indicates that a substantial reservoir of ozone is present in the summertime. Five-year mean concentrations range from 40 to 65 ppbv. The reservoir covered an area of several million square kilometers and extends vertically from the surface to 1 to 2 km. The vertical distribution of ozone in the reservoir during midday supports a transport of additional ozone from the boundary layer to the free troposphere. Data are presented demonstrating the potential effect of transport by convective clouds and by the sea breeze circulation - mechanisms by which ozone may be transported out of the boundary layer into the free troposphere. The potential impact of this reservoir on the tropospheric ozone budget is discussed. It is shown that if less than half of the ozone mass in this reservoir is transported to the free troposphere, then the amount of ozone transported out of the boundary layer approximates the amount of ozone transported downward during a tropopause fold event.
On 30 June 1981, the wind fields around a variety of convective clouds, ranging from large thunderstorm complexes to isolated cumulus congestus, were observed in Oklahoma using an airborne Doppler lidar operated by NASA. By steering the pulsed infrared laser beam alternately along differing horizontal directions, a network of independent radial velocity measurements is obtained, which permits high-resolution synthesis of the full horizontal wind vector field in a swath adjacent to the aircraft flight track. The bright reflections of the laser signal by cloud surfaces permit direct identification of the locus of cloud edges, information which is prerequisite to detailed study of the relationships between the winds inside and outside clouds. The horizontal wind fields derived from the lidar data reveal waves and vortices along the gust front of a storm which eventually produced a gust-front tornado, and cloud-scale convergence patterns around an isolated cumulus congestus. Despite the presence of some questionable data associated with undersampling and delayed recording of certain aircraft motion parameters, most of the lidar results appear consistent with cloud photographs made during the experiment, with surface meteorological data, with aircraft flight-level wind data, and with previous observational and theoretical work.
The boundary layer chemistry over the Amazon forest during the dry season is simulated with a photochemical model. Results are in good agreement with measurements of isoprene, NO, ozone, and organic acids. Photochemical reactions of biogenic isoprene and NOx can supply most of the ozone observed in the boundary layer. Production of ozone is very sensitive to the availability of NOx, but is insensitive to the isoprene source strength. High concentrations of total odd nitrogen (NOy) are predicted for the planetary boundary layer, about 1 ppb in the mixed layer and 0.75 ppb in the convective cloud layer. Most of the odd nitrogen is present as PAN-type species, which are removed by dry deposition to the forest. The observed daytime variations of isoprene are explained by a strong dependence of the isoprene emission flux on sun angle. Nighttime losses of isoprene exceed rates of reaction with NO3 and O3 and appear to reflect dry-deposition processes. The 24-hour averaged isoprene emission flux is calculated to be 38 mg/sq m per day. Photooxidation of isoprene could account for a large fraction of the CO enrichment observed in the boundary layer under unpolluted conditions and could constitute an important atmospheric source of formic acid, methacrylic acid, and pyruvic acid.
The effect of gravity on eutectic solidification was investigated experimentally for Pb-Sn binary eutectic alloys. It is found that the separation of the primary crystals of the binary system from the coupled eutectic occurs over a wide range of cooling rates and gravitational fields (100-100,000 g). The separation is strongly influenced by the nucleation behavior of the particular alloy system. A mechanism for the strong phase separation is postulated on the basis of cloud convection models in atmospheric convection.
Aircraft observations in the lower troposphere over the eastern Pacific Ocean in summer are examined. The free troposphere was found to have a distinctly nonuniform, layered structure. In maritime air the layers consist of partially mixed air from several sources: moist ozone-depleted boundary layer air; very dry air with high ozone content that probably originated in the middle or upper troposphere; and air with relatively low ozone and moderate, varying moisture content that probably represents residues of convective clouds that had formed over the ocean upstream of the research area. The subtropical high results in stably stratified, subsiding air, where discrete horizontal layers with differing flow velocities transport air over long distances with little vertical mixing.
A simple parameterization has been developed to simulate global lightning distributions. Convective cloud top height is used as the variable in the parameterization, with different formulations for continental and marine thunderstorms. The parameterization has been validated using two lightning data sets: one global and one regional. In both cases the simulated lightning distributions and frequencies are in very good agreement with the observed lightning data. This parameterization could be used for global studies of lightning climatology; the earth's electric circuit; in general circulation models for modeling global lightning activity, atmospheric NO(x) concentrations, and perhaps forest fire distributions for both the present and future climate; and, possibly, even as a short-term forecasting aid.
Research under this grant has involved analyses of satellite-derived measurements of water vapor and total ozone. Upper tropospheric water vapor data from the Nimbus 7 temperature-humidity infrared radiometer (THIR) 6.7 micron channel were analyzed by Fourier transformation to provide wavenumber spectra for a case of an upper level system over Europe. The power law spectrum for horizontal scales from 60 to several hundred km suggests that when convective cloud energy sources are not present, the enstrophy-cascading process (with variance proportional to the minus three power of wavenumber) may hold to much smaller scales than previously thought. Several investigations of the middle atmosphere (stratosphere and mesosphere) were also conducted. Slow atmospheric oscillations with periods of 1-2 months were investigated in total ozone measurements and in ionospheric data. Using one-point correlation maps and total ozone mapping spectrometer (TOMS) data, strong statistical evidence was found for the planetary-scale oscillations at these periods. A dipole-like pattern in the tropical equatorial Indian ocean-western Pacific region was documented, along with wavetrain-like patterns emanating into the extratropics. While attempting to follow the oscillations upward above stratosphere, oscillations were studied in ionospheric data (D-region radio wave absorption, in the upper mesosphere, around 80-90 km altitude). Cross-spectral analyses with solar flux data revealed that much of the observed 1-2 month variance in the ionospheric D-region was well correlated to solar variations. Further research has involved investigations of the photochemical lifetime of greenhouse gases methane and nitrous oxide. Using Nimbus 7 satellite data, a new analysis technique was employed to determine the lifetime of these gases in situ in the upper stratosphere. The lifetimes are found to be in good agreement with theoretical estimates.
A 3-D regional photochemical tracer/transport model for Europe and the Eastern Atlantic has been developed based on the NASA/GISS CTM. The model resolution is 4x5 degrees latitude and longitude with 9 layers in the vertical (7 in the troposphere). Advective winds, convection statistics and other meteorological data from the NASA/GISS GCM are used. An extensive gas-phase chemical scheme based on the scheme used in our global 2D model has been incorporated in the 3D model. In this work ozone formation in the troposphere is studied with the 3D model during a 5 day period starting June 30. Extensive local ozone production is found and the relationship between the source regions and the downwind areas are discussed. Variations in local ozone formation as a function of total emission rate, as well as the composition of the emissions (HC/NO(x)) ratio and isoprene emissions) are elucidated. An important vertical transport process in the troposphere is by convective clouds. The 3D model includes an explicit parameterization of this process. It is shown that this process has significant influence on the calculated surface ozone concentrations.
Thunderstorms and the activities associated with them was the emphasis of this final report. The primary goal of the investigation of the dynamics, microphysics, and the electrical properties of tropical thunderstorms, was to understand the process or processes which initiate the precipitation in various convective clouds. A concept that the degree of atmospheric instability that determines the updraft velocity is different between those storms that generate electrical activity and those that do not. This is apparent in temperate latitudes, but in tropical regions, little knowledge of these interactions is available. Several ground monitoring stations have been set up and, along with a waveform recorder at one of the stations, the data collected from these stations will be analyzed in conjunction with other data collected from ship and airborne radars and airborne in situ measurements of electrical activity in coordination with the TOGA-COARE program.
Monitoring stratospheric aerosols containing H2SO4 using the brightness temperature (BT) difference between 11 and 8.3 microns (BT(sub 8)-BT(sub 11)) spectral channels is demonstrated using theoretical calculations and satellite observations. Assuming an aqueous solution of 50% and 75% sulfuric acid, radiative transfer calculations indicate that over oceans an increase in the optical depth of the stratospheric aerosol results in an increase in BT(sub 8)-BT(sub 11). Theoretical simulations suggest that the technique is sensitive to visible optical depths greater than approximately 0.15. The simulations also demonstrate a lack of sensitivity to the particle size distribution. Changes in pre- and post-Pinatubo observations by the High-resolution Infrared Radiation Sounder 2 (HIRS2) on board the NOAA 10 are consistent with observed optical depth measurements and confirm the sensitivity of these channels to the presence of the aerosol. The technique is also applied to cold tropical convective clouds and desert regions where the signal, though evident, is less conclusive. Time series analysis is applied to the NOAA 10 and NOAA 12 combined BT(sub 8-BT(sub 11) observations to detect the periodicity of the spread of the volcanic aerosol. Over a region of the southern Pacific a 18- to 26-day period is present. Model simulations were conducted to demonstrate a trispectral with observations near 8, 11, and 12 microns. The trispectral approach has high potential in that the spectral signature of cirrus, water vapor, and H2SO4 aerosols are different. Observations from NOAA 10 and NOAA 11 are combined to demonstrate the capabilities of these infrared wavelengths of detecting the aerosol. The signal is clearly evident when a region of the South Atlantic is compared for pre- and post-Pinatubo conditions.
Many researchers have shown that the development and evolution of electrical discharges within convective clouds is fundamentally related to the growth and dynamics of precipitation particles aloft. In the presence of strong updrafts above the freezing level collisions among mixed-phase particles (i.e., hail. ice, supercooled water) promote the necessary charge separation needed to initiate intra-cloud lightning. A precipitation core that descends below the freezing level is often accompanied by a change in the electrical structure of the cloud. Consequently, more Cloud-to-Ground (CG) than Intra-Cloud (IC) lightning flashes appear. Descending precipitation cores can also play a significant role in the evolution of mesoscale features at the surface (e.g., microbursts, downbursts) because of latent heat and mass loading effects of water and ice. For this reason, some believe that lightning and microbursts are fundamentally linked by the presence of ice particles in thunderstorms. Several radar and lightning studies of microburst thunderstorms from COHMEX in 1986 showed that the peak IC lightning systematically occurred ten minutes before the onset of a microburst. In contrast, most CG lightning occurred at the time of the microburst. Many of the preceding studies have been done using high-resolution research radars and experimental lightning detection systems in focused field projects. In addition, these studies could only determine the vertical origin or occurrence of IC lightning, and not a true three-dimensional representation. Currently, the WSR-88D radar system and a real-time, state-of-the-art lightning system (LDAR) at the Kennedy Space Center (KSC) in Florida provide an opportunity to extend these kinds of studies in a more meaningful operational setting.
The relationship of the rainfall from convective clouds to area-time integrals determined from satellite infrared data using a fixed infrared-temperature threshold is investigated. Concurrent radar and rapid-scan satellite data obtained during field projects in the northern High Plains and the southeastern United States were used in this study. The fixed IR threshold appropriate for each region was determined by an optimization procedure that identified the brightness threshold that yields the strongest relationship between estimated rainfall from a cloud cluster and its satellite Area-Time Integral (ATI) for each dataset. For the North Dakota-Montana area the optimization procedure indicated that the area enclosed by the -22.5 C isotherm provides satellite ATI values most closely related to the estimated rainfalls. For the southeastern United States project, the optimized tem- perature threshold was 8.5'C. The difference between the thresholds determined for the two geographic areas suggests that a different 'calibration' for each distinct area may be needed to make use of this relationship. Slopes of the two log-log rainfall-ATI regressions are less than unity, indicating that a relative horizontal expansion and/or increase in persistence of a cloud cluster exceeds the associated increase in precipitation. Implications for the Geostationary Operational Environmental Satellite precipitation index are discussed. New results concerning the rain volume-radar ATI relationship for the southeastern United States are also appended to the paper.
We report here measurements of the acidic gases nitric (HNO3), formic (HCOOH), and acetic (CH3COOH) over the western Pacific basin during the February-March 1994 Pacific Exploratory Mission-West (PEM-West B). These data were obtained aboard the NASA DC-8 research aircraft as it flew missions in the altitude range of 0.3 - 12.5 km over equatorial regions near Guam and then further westward encompassing the entire Pacific Rim arc. Aged marine air over the equatorial Pacific generally exhibited mixing ratios of acidic gases less than 100 parts per trillion by volume (pptv). Near the Asian continent, discrete plumes encountered below 6 km altitude contained up to 8 parts per billion by volume (ppbv) HNO3 and 10 ppbv HCOOH and CH3COOH. Overall there was a general correlation between mixing ratios of acidic gases with those of CO, C2H2, and C2Cl4, indicative of emissions from combustion and industrial sources. The latitudinal distributions of HNO3 and CO showed that the largest mixing ratios were centered around 15 deg N, while HCOOH, CH3COOH, and C2Cl4 peaked at 25 deg N. The mixing ratios of HCOOH and CH3COOH were highly correlated (r(sup 2) = 0.87) below 6 km altitude, with a slope (0.89) characteristic of the nongrowing season at midlatitudes in the northern hemisphere. Above 6 km altitude, HCOOH and CH3COOH were marginally correlated (r(sup 2) = 0.50), and plumes well defined by CO, C2H2, and C2Cl4 were depleted in acidic gases, most likely due to scavenging during vertical transport of air masses through convective cloud systems over the Asian continent. In stratospheric air masses, HNO, mixing ratios were several parts per billion by volume (ppbv), yielding relationships with 03 and N2O consistent with those previously reported for NO(y).