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At least 397 records · Page 22
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Nitridation of atomically smooth (111) diamond surfaces using a low temperature Penning plasma discharge

Diamond is a material with a wide band gap that can host a variety of isolated paramagnetic defects, called “color centers”1. These color centers have attractive optical and magnetic properties suitable for quantum applications including quantum computing, nanophotonics and quantum sensing. The most common one is the negatively charged nitrogen vacancy (NV) color center. For quantum sensing, it is desirable to reduce the distance between the NV center and the analyte by using shallow color centers in order to increase sensitivity. In this context, the diamond surface termination is especially critical. The appropriate surface termination is required to stabilize the color centers and mitigate surface magnetic noise. The nitrogen termination of diamond has been postulated as highly desirable for the NV color center. The goal of this project is to take advantage of an electron beam-generated ExB low temperature plasma developed by the Princeton Collaborative Low Temperature Plasma Research Facility (PCRF) at the Princeton Plasma Physics Laboratory (PPPL) to nitridate the surface of (100) diamond single crystals with minimal surface damage. In this reactor, the use of a magnetized plasma enables gentle processing of materials sensitive to ion damage. This is in strong contrast to radiofrequency plasma processing reactors which are known to etch and sputter the surface. XPS measurements indicate the incorporation of nitrogen and oxygen atoms at the surface in similar amounts. XAS measurements confirm the nitridation and indicate that the nitrogen termination is different from the nitrogen termination obtained using radiofrequency plasma treatment4. The combination of these results indicates the formation of amid species at the (100) diamond surface that are promising for the stabilization of NV centers for quantum sensing.

36 MATERIALS SCIENCE↗
DOE OSTI2021

The Rarity of Very Red Trans-Neptunian Objects in the Scattered Disk

We investigate the origins of the photometrically very red (VR) and less red (LR) trans-Neptunian objects (TNOs). We first reanalyze the data set of Marsset et al. and find that in addition to the known color–inclination correlation in hot TNOs, a similar trend exists for color–eccentricity. We show that VR TNOs are sharply constrained to eccentricities <0.42 and inclinations <21°, leading to a paucity of VR scattered disk and distant mean motion resonance objects. We then interpret these findings using N-body simulations accounting for Neptune’s outward migration into a massless particles disk and find that these observations are best reproduced with an LR-to-VR color transition line between ∼38 and 42 au in the primordial disk, separating the objects’ formation locations. For an initial surface density profile (Σ ∝ 1/r {sup 2}), a color transition around 38 au is needed to explain the high abundance of VR plutinos, but it creates too many VR scattered disk objects, while a transition line around 42 au seems to better reproduce the scattered disk colors but creates virtually no VR plutinos. Our simulations furthermore show that the rarity of VR particles at high eccentricity is possibly due to the absence of sweeping higher-order MMRs, and secular resonances, beyond 42 au. Inspecting individual populations, we show that the majority of VR SDOs originate as objects trapped in Neptune’s second- and third-order MMRs. These then evolve due to diffusion, scattering, Kozai–Lidov cycles, and secular resonances into their current orbits. Future unbiased color surveys are crucial to better constrain the TNOs dynamical origins.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

47 Tuc in Rubin Data Preview 1. Exploring Early LSST Data and Science Potential

We present analyses of the early data from Rubin Observatory’s Data Preview 1 (DP1) for the field of the globular cluster 47 Tuc. The DP1 data set for 47 Tuc includes four nights of observations from the Rubin Commissioning Camera (LSSTComCam), covering multiple bands (ugriy). We address challenges of crowding in the inner region of the cluster and toward the SMC in DP1, and demonstrate improved star–galaxy separation by fitting fifth-degree polynomials to the stellar loci in color–color diagrams and applying multidimensional sigma clipping. We compile a catalog of 3576 probable 47 Tuc member stars selected via a combination of isochrone, Gaia proper-motion, and color–color space matched filtering. We explore the sources of photometric scatter in the 47 Tuc color–color sequence, evaluating contributions from various potential sources, including differential extinction within the cluster. Finally, of the 72 well-characterized variables in the field, we recover three known variable stars, including two RR Lyrae and one eclipsing binary, in the coadd-based object catalog, and identify 62 in the difference image-based object catalog. Although the DP1 lightcurves have sparse temporal sampling, they appear to follow the patterns of densely sampled literature lightcurves well. Despite some data limitations for crowded-field stellar analysis, DP1 demonstrates the promising scientific potential for future LSST data releases.

Choi, Yumi [NSF National Optical-Infrared Astronom↗
DOE OSTI2022

System and method for neutron and gamma radiation detection using non-homogeneous material scintillator

A scintillator system is disclosed for detecting incoming radiation. The system makes use of a scintillator structure having first and second dissimilar materials. The first dissimilar material emits a first color of light and the second dissimilar material emits a second color of light different from the first color of light. Either one, or both, of the first or second colors of light are emitted in response to receipt of the incoming radiation. A plurality of light detectors is disposed in proximity to the scintillator structure for detecting the first and second different colors of light and generating output signals in response thereto. A detector electronics subsystem is responsive to the output signals and provides an indication of colors emitted by the scintillator structure to infer at least one property of the incoming radiation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Multicolor Photonic Pigments for Rotation-Asymmetric Mechanochromic Devices

Photonic crystals are extensively explored to replace inorganic pigments and organic dyes as coloring elements in printing, painting, sensing, and anti-counterfeiting due to their brilliant structural colors, chemical stability, and environmental friendliness. However, most existing photonic-crystal-based pigments can only display monochromatic colors once made, and generating multicolors has to start with designing different building blocks. In this work, a novel photonic pigment featuring highly tunable structural colors in the entire visible spectrum, made by the magnetic assembly of monodisperse nanorods into body-centered-tetragonal photonic crystals, is reported. Their prominent magnetic and crystal anisotropy makes it efficient to generate multicolors using one photonic pigment by magnetically controlling the crystal orientation. Further, the combination of angle-dependent diffraction and magnetic orientation control enables the design of rotation-asymmetric photonic films that display distinct patterns and encrypted information in response to rotation. The efficient multicolor generation through precise orientational control makes this novel photonic pigment promising in developing high-performance structural-colored materials and optical devices.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Multicolored microwave absorbers with dynamic frequency modulation

Microwave-absorbing materials are extensively used in intelligent electronic devices and stealth technologies where the ability to dynamically adjust microwave-absorbing capacity in response to specific requirements is vitally important. Herein, we report a new approach for constructing dynamically tunable microwave absorbers with ultrawide tunable frequency ranges that are simultaneously endowed with vibrant structural colors. Here, the methodology produces structural colors and adjusts absorption properties by constructing ZnO coatings with precisely adjustable thicknesses on a polypyrrole/melamine foam (PPy/MF) surface by atomic layer deposition (ALD) in conjunction with a pressure-driven strategy that regulates the compression ratio. The electrical conductivity, electromagnetic parameters, thickness, and pore size of the ZnO-coated PPy/MF (ZnO/PPy/MF) are effectively adjusted, and simply applying external pressure widens the tunable frequency range and the effective absorption bandwidth. As a result, the effective absorption frequency of ZnO/PPy/MF is dynamically adjustable from the S band to the Ku band, thereby covering 94.3% of the entire microwave spectrum. Moreover, the brilliant and uniform structural colors of ZnO/PPy/MF, which span various color categories, are precisely regulated by tuning the thickness of the ZnO coating by adjusting the number of ALD cycles. ZnO/PPy/MF is strongly hydrophobic, which endows it with remarkable self-cleaning properties. Therefore, ZnO/PPy/MF provides a conceptually novel platform for the development of next-generation smart microwave-absorbing materials due to its integrated dynamic frequency-regulating ability, brilliant structural coloration, and self-cleaning features.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Baryon-baryon, meson-meson, and meson-baryon interactions in nonrelativistic QCD

Van der Waals potentials describing interactions between color-singlet mesons and/or baryons vanish at leading order in potential nonrelativistic quantum chromodynamics (pNRQCD). This result and constraints from Gauss’s law are used to prove that weakly coupled pNRQCD van der Waals potentials in generic non-Abelian gauge theories with only heavy quarks are too weak to form bound states whose color state is a product of color singlets. Quantum Monte Carlo calculations of four, five, and six quarks with equal masses provide numerical evidence that exotic color configurations are higher energy than products of color-singlet hadrons, suggesting that equal-mass fully heavy tetraquark, pentaquark, and hexaquark bound states do not exist at next-to-leading order in pNRQCD and at all orders in QCD-like theories in which all quark masses are asymptotically large. Mechanisms for generating hadron-hadron bound states are identified, which necessarily involve large quark-mass hierarchies, relativistic effects arising from the presence of sufficiently light quarks, or nonperturbative effects outside the scope of weakly coupled pNRQCD.

Effective field theory↗
DOE OSTI2020

Ultrarelativistic quark-nucleus scattering in a light-front Hamiltonian approach

In this work, we investigate the scattering of a quark on a heavy nucleus at high energies using the time-dependent basis light-front quantization (tBLFQ) formalism, which is the first application of the tBLFQ formalism in QCD. We present the real-time evolution of the quark wave function in a strong classical color field of the relativistic nucleus, described as the color glass condensate. The quark and the nucleus color field are simulated in the QCD SU(3) color space. We calculate the total and the differential cross sections, and the quark distribution in coordinate and color spaces using the tBLFQ approach. We recover the eikonal cross sections in the eikonal limit. We find that the differential cross section from the tBLFQ simulation is in agreement with a perturbative calculation at large $p_⊥$, and it deviates from the perturbative calculation at small $p_⊥$ due to higher-order contributions. In particular, we relax the eikonal limit by letting the quark carry realistic finite longitudinal momenta. We study the sub-eikonal effect on the quark through the transverse coordinate distribution of the quark with different longitudinal momentum, and we find the sub-eikonal effect to be sizable. Our results can significantly reduce the theoretical uncertainties in small $p_⊥$ region which has important implications to the phenomenology of the hadron-nucleus and deep inelastic scattering at high energies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Jet quenching in the glasma phase: Medium-induced radiation

Inspired by the recent considerations of parton momentum broadening in the glasma phase, we study the medium-induced soft gluon radiation of jet partons at early times in heavy-ion collisions. The glasma state is assumed to be comprised of independent color domains with homogenous longitudinal fields that vary event by event, and we further complete this model with an event-averaging procedure accounting for the finite correlation length. Using this description, we evaluate the rate of medium-induced radiation from an energetic parton at midrapidity in the glasma phase. We mainly focus on SU(2) color fields for simplicity, also referring to the U(1) case and comparing with the Baier, Dokshitzer, Mueller, Peigné, Schiff, and Zakharov rate to gain further insight. Our results show that there is an intricate interplay of the synchrotron-like radiation in a single color domain with the destructive interference between different color domains, after the medium averaging is performed. Thus, we find that the emission rate is sensitive to the matter structure, decreasing for a glasma state populated by smaller color domains—i.e., for a glasma with a larger characteristic saturation scale. Our approach can be applied to more realistic backgrounds, and it sets the stage for the modeling of jet evolution in the early stages of heavy-ion collisions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Probing for the Trace Estimation of a Permuted Matrix Inverse Corresponding to a Lattice Displacement

We report thatpProbing is a general technique that is used to reduce the variance of the Hutchinson stochastic estimator for the trace of the inverse of a large, sparse matrix A. The variance of the estimator is the sum of the squares of the off-diagonal elements of A -1 . Therefore, this technique computes probing vectors that when used in the estimator annihilate the largest off-diagonal elements. For matrices that display decay of the magnitude of |A$^{-1}_{ij}$| with the graph distance between nodes i and j, this is achieved through graph coloring of increasing powers A k . Equivalently, when a matrix stems from a lattice discretization, it is computationally beneficial to find a distance-k coloring of the lattice. Previously, a hierarchical coloring was proposed so that k can be increased at runtime as needed without discarding previous work. In this work, we study probing for the more general problem of computing the trace of a permutation of A -1 , say PA -1 . The motivation comes from lattice quantum chromodynamics (QCD), where we need to construct “disconnected diagrams” to extract flavor-separated generalized parton functions. In lattice QCD, where the matrix has a four-dimensional toroidal lattice structure, these nonlocal operators correspond to a PA -1 , where P is the permutation relating to some displacement $\vec{p}$ in one or more dimensions. We focus on a single dimension displacement (p), but our methods are general. We show that probing on A k or (PA) k does not annihilate the largest magnitude elements. To resolve this issue, our displacement-based probing works on PA k using a new coloring scheme that works directly on appropriately displaced neighborhoods on the lattice. We prove lower bounds on the number of colors needed and study the effect of this scheme on variance reduction, both theoretically and experimentally on a real-world lattice QCD calculation. We achieve orders of magnitude speedup over the unprobed or the naively probed methods.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2022

Two new marine hermit crabs allied with the Paguristes tortugae complex (Crustacea: Decapoda: Anomura) from the western Atlantic

A recent molecular phylogenetic analysis that focused on selected species of western Atlantic Paguristes Dana, 1851, Areopaguristes Rahayu & McLaughlin, 2010, and Pseudopaguristes McLaughlin, 2002 was somewhat inconclusive regarding relationships among those genera, but it revealed two new unrecognized species genetically related to members of the Paguristes tortugae complex. One of the new species is sister to A. hummi (Wass, 1955), which is readily separated from Wass’ taxon by significant differences in coloration. However, no definitive characters have been found for its identification on the basis of structural morphology. A second new species is genetically sister to P. tortugae Schmitt, 1933, even though it was regarded in earlier literature as no more than an ecomorphic variant expressing protective coloration related to habitat substrate color. In addition to its unique coloration, subtle distinctions are evident in structural morphology. Both species are formally named with accompanying morphological and color descriptions.

Zoology↗
DOE OSTI2023

Catalog of Planetary Nebulae Detected by GALEX and Corollary Optical Surveys

Planetary nebulae (PNs) consist of an ionized envelope surrounding a hot central star (CSPN) that emits mostly at ultraviolet (UV) wavelengths. UV observations, therefore, provide important information on both the CSPN and the nebula. We have matched the PNs in the Hong Kong/Australian Astronomical Observatory/Strasbourg Hα catalog with the Galaxy Evolution Explorer (GALEX) UV sky surveys, the Sloan Digital Sky Survey (SDSS) data release 16, and the Panoramic Survey Telescope and Rapid Response System (Pan-STARRS) PS1 second release. A total of 671 PNs were observed by GALEX with the far-UV (FUV; 1344 Å–1786 Å) and/or the near-UV (NUV; 1771 Å–2831 Å) detectors on (GUVPNcat); 83 were observed by SDSS (PNcatxSDSSDR16) and 1819 by Pan-STARRS (PNcatxPS1MDS). We merged a distilled version of these matched catalogs into GUVPNcatxSDSSDR16xPS1MDS, which contains a total of 375 PNs with both UV and optical photometry over a total spectral coverage of ~1540 Å–9610 Å. We analyzed separately 170 PNs resolved in GALEX images and determined their UV radius by applying a flux profile analysis. The CSPN flux could be extracted separately from the PN emission for 8 and 50 objects with SDSS and Pan-STARRS counterparts, respectively. The multiband photometry was used to distinguish between compact and extended PNs and CSPNs (binary CSPNs) by color–color diagram analysis. We found that compact PN candidates could be identified by using the r - i < - 0.4 and -1 < FUV-NUV < 1 colors, whereas binary CSPN candidates in given T eff ranges (all with color r-i > -0.4) can be identified in the color region (FUV-NUV) ≤ 6(r-i)+1.3, -0.8 < FUV-NUV < 0.4, and r-i < 0.75.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Photometric Properties of Jupiter Trojans Detected by the Dark Energy Survey

The Jupiter Trojans are a large group of asteroids that are coorbiting with Jupiter near its L4 and L5 Lagrange points. The study of Jupiter Trojans is crucial for testing different models of planet formation that are directly related to our understanding of solar system evolution. In this work, we select known Jupiter Trojans listed by the Minor Planet Center from the full six years data set (Y6) of the Dark Energy Survey (DES) to analyze their photometric properties. The DES data allow us to study Jupiter Trojans with a fainter magnitude limit than previous studies in a homogeneous survey with griz band measurements. We extract a final catalog of 573 unique Jupiter Trojans. Our sample include 547 asteroids belonging to L5. This is one of the largest analyzed samples for this group. By comparing with the data reported by other surveys we found that the color distribution of L5 Trojans is similar to that of L4 Trojans. We find that L5 Trojans’ g − i and g − r colors become less red with fainter absolute magnitudes, a trend also seen in L4 Trojans. Both the L4 and L5 clouds consistently show such a color–size correlation over an absolute magnitude range 11 < H < 18. We also use DES colors to perform taxonomic classifications. C- and P-type asteroids outnumber D-type asteroids in the L5 Trojans DES sample, which have diameters in the 5–20 km range. This is consistent with the color–size correlation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

System and method for neutron and gamma radiation detection using non-homogeneous material scintillator

The present disclosure relates to a method for detecting incoming radiation having a plurality of differing properties including at least one of differing types, differing energies or differing incoming directions. The method involves using a scintillator structure formed from first and second dissimilar scintillator materials, where the first and second dissimilar scintillator materials emit first and second different colors of light in response to the incoming radiation. A first light detector is used for detecting light having the first color, and a second light detector is used for detecting light having the second color. A first output signal is generated in response to the detection of light having the first color, and a second output signal is generated in response to detecting light having the second color. The first and second output signals are then analyzed to determine at least one property of the incoming radiation.

Brodsky, Jason Philip↗
DOE OSTI2021

Combined selection of the dynamic model and modeling error in nonlinear aeroelastic systems using Bayesian Inference

Here, we report a Bayesian framework for concurrent selection of physics-based models and (modeling) error models. We investigate the use of colored noise to capture the mismatch between the predictions of calibrated models and observational data that cannot be explained by measurement error alone within the context of Bayesian estimation for stochastic ordinary differential equations. Proposed models are characterized by the average data-fit, a measure of how well a model fits the measurements, and the model complexity measured using the Kullback–Leibler divergence. The use of a more complex error models increases the average data-fit but also increases the complexity of the combined model, possibly over-fitting the data. Bayesian model selection is used to find the optimal physical model as well as the optimal error model. The optimal model is defined using the evidence, where the average data-fit is balanced by the complexity of the model. The effect of colored noise process is illustrated using a nonlinear aeroelastic oscillator representing a rigid NACA0012 airfoil undergoing limit cycle oscillations due to complex fluid–structure interactions. Several quasi-steady and unsteady aerodynamic models are proposed with colored noise or white noise for the model error. The use of colored noise improves the predictive capabilities of simpler models.

42 ENGINEERING↗
DOE OSTI2022

Enhancing and Extinguishing the Different Emission Features of 2D (EA(1-)(x)FA(x))(4)Pb3Br10 Perovskite Films

2D hybrid perovskites are attractive for optoelectronic devices. In thin films, the color of optical emission and the texture of crystalline domains are often difficult to control. Here, a method for extinguishing or enhancing different emission features is demonstrated for the family of 2D Ruddlesden-Popper perovskites (EA(1-)(x)FA(x))(4)Pb3Br10 (EA = ethylammonium, FA = formamidinium). When grown from aqueous hydrobromic acid, crystals of (EA(1-)(x)FA(x))(4)Pb3Br10 retain all the emission features of their parent compound, (EA)(4)Pb3Br10. Surprisingly, when grown from dimethylformamide (DMF), an emission feature, likely self-trapped exciton (STE), near 2.7 eV is missing. Extinction of this feature is correlated with DMF being incorporated between the 2D Pb-Br sheets, forming (EA(1-)(x)FA(x))(4)Pb3Br10 center dot(DMF)(y). Without FA, films grown from DMF form (EA)(4)Pb3Br10, retain little solvent, and have strong emission near 2.7 eV. Slowing the kinetics of film growth strengthens a different emission feature, likely a different type of STE, which is much broader and present in all compositions. Films of (EA(1-)(x)FA(x))(4)Pb3Br10 center dot(DMF)(y) have large, micron-sized domains and homogeneous orientation of the semiconducting sheets, resulting in low electronic disorder near the absorption edge. The ability to selectively strengthen or extinguish different emission features in films of (EA(1-)(x)FA(x))(4)Pb3Br10 center dot(DMF)(y) reveals a pathway to tune the emission color in these compounds.

2D halide perovskites↗
DOE OSTI2024

Mechanochromic Palettes Based on Optical Rotation in Cholesteric Liquid Crystal Elastomers for Visual Signalling

Mechanochromic photonic materials present promising prospects for enhancing diverse facets of human life. Cholesteric liquid crystal elastomers (CLCEs) present immediate mechanochromic properties, allowing their utility in various fields, including camouflages, textiles, and anticounterfeiting. Nonetheless, it is essential to provide differentiated color information corresponding to diverse types and degrees of deformation for practical use in real life. Herein, the mechanochromic responses of CLCEs are investigated using their optical rotation under compression and uniaxial stretching. The CLCEs exhibit the same reflection colors indistinguishable for compression and uniaxial stretching due to their contracted pitches. In contrast, the linearly polarized light passing through deformed CLCEs can be modulated by optical rotation, resulting in distinct transmission colors that can be discerned through mechanical deformations. A visual signaling system with color information derived from optical rotation is demonstrated. By comprehending and manipulating the mechanoresponsive behavior of CLCEs, these materials can be advanced into innovative solutions with enhanced functionality and performance, thereby broadening their applications for human life enhancement.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Transparent, High‐Charge Capacity Metal Mesh Electrode for Reversible Metal Electrodeposition Dynamic Windows with Dark‐State Transmission <0.1%

Abstract Dynamic windows allow user control over light and heat flow to save energy and maximize comfort. Reversible metal electrodeposition (RME) dynamic windows can uniquely tint to a color‐neutral privacy state (0.1% visible light transmission). The design parameters of transparent metal mesh counter electrodes for high‐contrast RME dynamic windows: high transparency, charge capacity and surface area with low haze, sheet resistance and cost are discussed, concluding that woven metal meshes meet these design parameters. Electroplated current is measured on an indium tin oxide electrode and two meshes with different wire spacings, showing the meshes’ cylindrical geometry enable them to draw more current per square area. The mesh material composition is analyzed to ensure cycling durability in a CuBi electrolyte by developing a transparent mesh with an inert core (stainless steel, SS), a thin Au coating, and a high charge‐capacity (1.5 C cm −2 ) CuBi outer coating. The study demonstrates that the films maintain a consistent Cu:Bi ratio and optical properties after 250 privacy cycles or 1500 cycles to 10% transmission, showing that the Cu and Bi coating is effective in keeping the films from becoming Cu rich with cycling. Finally, a 100 cm 2 device with excellent uniformity and color neutrality is demonstrated.

Yeang, Andrew L.↗