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DOE OSTI2012

Zgoubi Users' Guide

The initial version of zgoubi, dedicated to ray-tracing in magnetic fields, was developed by D. Garreta and J.C. Faivre at CEN-Saclay in the early 1970’s. It was perfected for the purpose of studying the four spectrometers SPES I, II, III, IV at the Laboratoire National SATURNE (CEA-Saclay, France), and SPEG at GANIL (Caen, France). It is being used since long in several national and foreign laboratories. The first manual was in French. Accounting for many developments and improvements, and in or der to facilitate access to the program an English version of the manual was written at TRIUMF with the assistance of J. Doornbos. P. Stewart prepared the manuscript for publication. An updating of the latter was necessary for accompanying the third version of the code which included developments regarding spin tracking and ray-tracing in combined electric and magnetic fields; this was done with the help of D. Bunel (SATURNE Laboratory, Saclay) for the preparation of the document and lead to the third release. In the mid-1990s, the computation of synchrotron radiation electromagnetic impulse and spectra was introduced for the purpose of studying interference effects at the LEP synchrotron radiation based diagnostic mini-wiggler. In the mean time, several new optical elements were added, such as electro-magnetic and other electrostatic lenses. Used since several years for special studies in periodic machines (e.g., SATURNE at Saclay, COSY at Julich, LEP and LHC at CERN, Neutrino Factory rings), zgoubi has also undergone extensive developments regarding storage ring related features. These developments of zgoubi have strongly benefited of the environment of the Groupe Théorie, Laboratoire National SATURNE, CEA/DSM-Saclay, in the years 1985-1995. The graphic interface to zgoubi (addressed in Part D) has also undergone concomitant extensive devel opments, which make it a performing tool for the post-processing of zgoubi outputs. The Users’ Guide is intended to describe the contents of the most recent version of zgoubi, which is far from being a “finished product”. Françios Méot

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

LANL Problem Setup [Slides]

This talk is a roughly 20-30 minute presentation to be given during the meshing and parallel partitioning session of the NNSA/CEA Computing Sciences Collaboration Workshop in Sedona on June 7, 2011. The purpose of the talk is to introduce the participants to the types of geometry, meshing, and general problem setup issues of interest to the ASC program at LANL and specifically those of interest to the ASC Simulation Setup Project. The presentation the discussions be focused on areas of possible research collaboration among LANL, LLNL, SNL, and the CEA.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2013

Progress in 2012-2013 on HEDLP LAB 11-583 Eagle Nebula

In the companion LLNL-led Eagle Nebula effort (Figure {Eagle}), experiments to characterize a multi-hohlraum "Long Duration Radiator" source at the Omega EP laser remain on schedule for June 2013. These experiments are being performed by a collaboration between HEDLP Eagle Nebula, Roberto Mancini s and Bob Heeter s photionization project, and CEA, who will field their µDMX spectrometer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2013

Center for Momentum Transport and Flow Organization (CMTFO) (Final Technical Report)

The Center for Momentum Transport and Flow Organization (CMTFO) is a DOE Plasma Science Center formed in late 2009 to focus on the general principles underlying momentum transport in magnetic fusion and astrophysical systems. It is composed of funded researchers from UCSD, UW Madison, U. Colorado, PPPL. As of 2011, UCSD supported postdocs are collaborating at MIT/Columbia and UC Santa Cruz and beginning in 2012, will also be based at PPPL. In the initial startup period, the Center supported the construction of two basic experiments at PPPL and UW Madison to focus on accretion disk hydrodynamic instabilities and solar physics issues. We now have computational efforts underway focused on understanding recent experimental tests of dynamos, solar tachocline physics, intrinsic rotation in tokamak plasmas and L-H transition physics in tokamak devices. In addition, we have the basic experiments discussed above complemented by work on a basic linear plasma device at UCSD and a collaboration at the LAPD located at UCLA. We are also performing experiments on intrinsic rotation and L-H transition physics in the DIII-D, NSTX, C-Mod, HBT EP, HL-2A, and EAST tokamaks in the US and China, and expect to begin collaborations on K-STAR in the coming year. Center funds provide support to over 10 postdocs and graduate students each year, who work with 8 senior faculty and researchers at their respective institutions. The Center has sponsored a mini-conference at the APS DPP 2010 meeting, and co-sponsored the recent Festival de Theorie (2011) with the CEA in Cadarache, and will co-sponsor a Winter School in January 2012 in collaboration with the CMSO-UW Madison. Center researchers have published over 50 papers in the peer reviewed literature, and given over 10 talks at major international meetings. In addition, the Center co-PI, Professor Patrick Diamond, shared the 2011 Alfven Prize at the EPS meeting. Key scientific results from this startup period include initial simulations of the effects of boundary conditions on turbulent dynamo experiments; simulations of intrinsic rotation showing the strong link between toroidal rotation and temperature gradients and elucidation of the turbulence symmetry breaking mechanisms that lead to this macroscopic behavior; first experiments in a large tokamak testing the roll of turbulent momentum transport in driving intrinsic rotation; experiments in tokamaks showing strong evidence that zonal flows, together with the more widely recognized mean sheared ExB flow, act to trigger the L-H transition in tokamak devices and the first experimental measurement of collisional viscosity in an unmagnetized plasma. In the coming three year period, we will continue these efforts by a combination of basic hydrodynamic, liquid metal and plasma experiments combined with experiments on numerous tokamak devices around the world. In addition, we will use MHD, gyrofluid and gyrokinetic codes combined with theory to address the problems of interest to the Center.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

Time-resolved broadband cavity-enhanced absorption spectroscopy for chemical kinetics.

Experimental measurements of elementary reaction rate coefficients and product branching ratios are essential to our understanding of many fundamentally important processes in Combustion Chemistry. However, such measurements are often impossible because of a lack of adequate detection techniques. Some of the largest gaps in our knowledge concern some of the most important radical species, because their short lifetimes and low steady-state concentrations make them particularly difficult to detect. To address this challenge, we propose a novel general detection method for gas-phase chemical kinetics: time-resolved broadband cavity-enhanced absorption spectroscopy (TR-BB-CEAS). This all-optical, non-intrusive, multiplexed method enables sensitive direct probing of transient reaction intermediates in a simple, inexpensive, and robust experimental package.

Sheps, Leonid↗
DOE OSTI2013

NEET Micro-Pocket Fission Detector – FY 2013 Status Report

A collaboration between the Idaho National Laboratory (INL), the Kansas State University (KSU), and the Commissariat à l'Énergie Atomique et aux Energies Alternatives (CEA), is funded by the Nuclear Energy Enabling Technologies (NEET) program to develop and test Micro-Pocket Fission Detectors (MPFDs), which are compact fission chambers capable of simultaneously measuring thermal neutron flux, fast neutron flux, and temperature within a single package.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

LBS GatlingGun13A

The High Energy Density Laboratory Physics (HEDLP)-funded Eagle nebula project, in collaboration with the LLNL/ University of Nevada Photoionization / Black Hole Physics effort, has successfully executed the first day of Laboratory Basic Science (LBS) Long Duration Radiator shots, performed at the University of Rochester Laboratory for Laser Energetics Omega EP Laser. This experiment employed a novel technique used a copper multi-hohlraum target with 3 hohlraum filled with a 4mg/cc TPX foam fill to act as a gas surrogate. Each hohlraum was driven with an Omega EP UV beam with either a 6ns pulse with 3.3kJ energy or 10ns pulse with 4.3 kJ. Each hohlraum was heated in succession to generate an 18ns or 30ns, 100 eV x-ray source for future laboratory astrophysics studies. The x-ray source was characterized with the CEA μDMX diagnostic and VISAR using a Quartz shock sample with a CH ablator over a single hohlraum. The Shot day was successful with six hohlraum shots on Omega EP with two 30ns x-ray drive shots. The data indicated that the novel foam-filled multi-hohlraum (‘Gatling Gun’) long –duration source performed as designed with all three hohlraums lighting up without significant inter-hohlraum interference (Figure 1). In addition the x-ray drive source was able to illuminate a Ti photoionization demonstration physics package with a 90 to 100 eV x-ray drive, generating Ti L-shell band radiation as expected. This source will next be applied to study ablation-driven hydrodynamics experiments relevant to the Eagle nebula and use the source and further develop the photoionization studies with a controlled 30ns x-ray source.

42 ENGINEERING↗
DOE OSTI2013

Center for Momentum Transport and Flow Organization (CMTFO) (Final Technical Report)

The Center for Momentum Transport and Flow Organization (CMTFO) is a DOE Plasma Science Center formed in late 2009 to focus on the general principles underlying momentum transport in magnetic fusion and astrophysical systems. It is composed of funded researchers from UCSD, UW Madison, U. Colorado, PPPL. As of 2011, UCSD supported postdocs are collaborating at MIT/Columbia and UC Santa Cruz and beginning in 2012, will also be based at PPPL. In the initial startup period, the Center supported the construction of two basic experiments at PPPL and UW Madison to focus on accretion disk hydrodynamic instabilities and solar physics issues. We now have computational efforts underway focused on understanding recent experimental tests of dynamos, solar tacholine physics, intrinsic rotation in tokamak plasmas and L-H transition physics in tokamak devices. In addition, we have the basic experiments discussed above complemented by work on a basic linear plasma device at UCSD and a collaboration at the LAPD located at UCLA. We are also performing experiments on intrinsic rotation and L-H transition physics in the DIII-D, NSTX, C-Mod, HBT EP, HL-2A, and EAST tokamaks in the US and China, and expect to begin collaborations on K-STAR in the coming year. Center funds provide support to over 10 postdocs and graduate students each year, who work with 8 senior faculty and researchers at their respective institutions. The Center has sponsored a mini-conference at the APS DPP 2010 meeting, and co-sponsored the recent Festival de Theorie (2011) with the CEA in Cadarache, and will co-sponsor a Winter School in January 2012 in collaboration with the CMSO-UW Madison. Center researchers have published over 50 papers in the peer reviewed literature, and given over 10 talks at major international meetings. In addition, the Center co-PI, Professor Patrick Diamond, shared the 2011 Alfven Prize at the EPS meeting. Key scientific results from this startup period include initial simulations of the effects of boundary conditions on turbulent dynamo experiments; simulations of intrinsic rotation showing the strong link between toroidal rotation and temperature gradients and elucidation of the turbulence symmetry breaking mechanisms that lead to this macroscopic behavior; first experiments in a large tokamak testing the roll of turbulent momentum transport in driving intrinsic rotation; experiments in tokamaks showing strong evidence that zonal flows, together with the more widely recognized mean sheared ExB flow, act to trigger the L-H transition in tokamak devices and the first experimental measurement of collisional viscosity in an unmagnetized plasma. In the coming three year period, we will continue these efforts by a combination of basic hydrodynamic, liquid metal and plasma experiments combined with experiments on numerous tokamak devices around the world. In addition, we will use MHD, gyrofluid and gyrokinetic codes combined with theory to address the problems of interest to the Center.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

MB3a Infrasound Sensor Evaluation.

Sandia National Laboratories has tested and evaluated a new infrasound sensor, the MB3a, manufactured by Seismo Wave. These infrasound sensors measure pressure output by a methodology developed by researchers at the French Alternative Energies and Atomic Energy Commission (CEA) and the technology was recently licensed to Seismo Wave for production and sales. The purpose of the infrasound sensor evaluation was to determine a measured sensitivity, transfer function, power, self-noise, dynamic range, seismic sensitivity, and self- calibration ability. The MB3a infrasound sensors are being evaluated for potential use in the International Monitoring System (IMS) of the Comprehensive Nuclear Test-Ban-Treaty Organization (CTBTO).

Merchant, Bion J.↗
DOE OSTI2014

NEET Micro-Pocket Fission Detector. Final Project report

A collaboration between the Idaho National Laboratory (INL), the Kansas State University (KSU), and the French Alternative Energies and Atomic Energy Commission, Commissariat à l'Énergie Atomique et aux Energies Alternatives, (CEA), is funded by the Nuclear Energy Enabling Technologies (NEET) program to develop and test Micro-Pocket Fission Detectors (MPFDs), which are compact fission chambers capable of simultaneously measuring thermal neutron flux, fast neutron flux and temperature within a single package. When deployed, these sensors will significantly advance flux detection capabilities for irradiation tests in US Material Test Reactors (MTRs). Ultimately, evaluations may lead to a more compact, more accurate, and longer lifetime flux sensor for critical mock-ups, and high performance reactors, allowing several Department of Energy Office of Nuclear Energy (DOE-NE) programs to obtain higher accuracy/higher resolution data from irradiation tests of candidate new fuels and materials. Specifically, deployment of MPFDs will address several challenges faced in irradiations performed at MTRs: Current fission chamber technologies do not offer the ability to measure fast flux, thermal flux and temperature within a single compact probe; MPFDs offer this option. MPFD construction is very different than current fission chamber construction; the use of high temperature materials allow MPFDs to be specifically tailored to survive harsh conditions encountered in-core of high performance MTRs. The higher accuracy, high fidelity data available from the compact MPFD will significantly enhance efforts to validate new high-fidelity reactor physics codes and new multi-scale, multi-physics codes. MPFDs can be built with variable sensitivities to survive the lifetime of an experiment or fuel assembly in some MTRs, allowing for more efficient and cost effective power monitoring. The small size of the MPFDs allows multiple sensors to be deployed, offering the potential to accurately measure the flux and temperature profiles in the reactor. This report summarizes the status at the end of year two of this three year project. As documented in this report, all planned accomplishments for developing this unique new, compact, multipurpose sensor have been completed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2015

Stand-Alone Dynamic System Simulation of a Fissile Solution System

Dynamic system simulations (DSS) of fissile solution systems (FSS) have been performed at Los Alamos National Laboratory (LANL) for several years. DSS have been designed and executed using the DESIRE (Direct Executing Simulation in Real Time) system, a platform ideal for expert system modelers, as it allows for direct mathematical specification of a model, and facilities for performing experiments and analyses with the model. Models built in DESIRE have been compared to historical data from several historic aqueous homogeneous reactors (AHR) showing close agreement between experimental data and model estimates. Historical systems modeled include: SUPO (Super Power), an AHR that operated at Los Alamos National Laboratory from 1951 to 1974; SILENE, which was operated by CEA at Valduc, France until 2011; KEWB (Kinetics Experiment Water Boiler) A-2 and B-5 cores, operated by North American Atomics during the 1960’s and 1970’s. SUPO is considered a benchmark for steady-state operations, SILENE for pulse, and KEWB as confirmatory for both modes. However, there are some simulation tasks that are not well-suited to DESIRE model implementation. These tasks include engineering design and analysis and providing a hardware simulator backend. It has been determined that executable simulation models would better suit these purposes, hence a process for converting DESIRE simulation models to executable simulation models was designed and implemented, and several models have been converted. DESIRE simulation models are converted to C++ executable models by an automated process. The conversion process is quick, accurate and repeatable, giving confidence that converted models will perform as well as the original DESIRE models. Extensive testing on the SUPO and accelerator driven subcritical system models has shown that the executable models perform almost identically to the DESIRE models. All major trends and events are simulated with excellent agreement and the steady-state results typically agree within a small fraction of a percent (always better than 0.1% and generally better than 0.01% agreement).

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2016

High-foot Implosion Workshop (March 22-24, 2016) Report

From March 22-24, 2016 at Workshop was held at Lawrence Livermore National Laboratory bringing together international experts in inertial confinement fusion research for the purpose of discussing the results from the ‘high-foot implosion campaign.’ The Workshop topics covered a retrospective of the first two years of experiments, a discussion of our best present understanding of what the data and our models imply, a discussion about remaining mysteries that are not understood at this time, and a discussion of our strategy moving forward. The material herein contains information from published and unpublished sources and is distributed solely for the purposes of this Workshop. Key assessments and conclusions resulting from the Workshop are: “The high foot campaign is extremely well documented and the interested reader is urged to go directly to the peer-reviewed journal literature for details.” – D. Haynes (LANL) “Overall progress in understanding of fuel and hot-spot properties near peak burn is excellent.” – V. Goncharov (LLE) “I would say that given the constraints of using the same hohlraum and similar capsule designs to the National Ignition Campaign, the High Foot Campaign achieved as much as could be expected. Indeed the demonstration of significant alpha particle heating remains a landmark achievement.” – J. Chittenden (Imperial College) “One of the principal points of discussion at the meeting was the importance of the roll over in inferred pressure that occurs with reducing coast time for different ablator thicknesses and the idea of repeating shot N140819 to confirm this. I would be very interested to see a return to the High Foot platform as a way to exercise the improved radiographic capabilities such as the curved crystal imaging system and as a way to examine the hypothesis of ‘burn truncation by aneurism.’ ” – J. Chittenden (Imperial College) “It is clear from the quality of the data presented during this workshop that the High-Foot experimental series has been a success. It has fulfilled the original goal of being an implosion platform that could separate the low-mode effects from the high-mode effects. Just because we now know when the High-Foot implosions break, it does not mean that they have served their purpose. This will be a very useful platform to study hohlraum coupling, to determine if controlling shape reduces residual kinetic energy, and testing hypotheses of how the hot-spot assembles.” – J. Knauer (LLE) “The LLNL "base camp" strategy for hohlraums was finally presented. Goals are to understand the safe operating space for the hohlraum and to find designs with good enough symmetry inside NIF's envelope, varying the CCR, pulse length and capsule designs. LLNL has a draft set of drive asymmetry requirements.” – P. Gauthier (CEA)

42 ENGINEERING↗
DOE OSTI2017

Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. I -- National Study

The use of renewable energy (RE) sources, primarily wind and solar generation, is poised to grow significantly within the Indian power system. The Government of India has established a target of 175 gigawatts (GW) of installed RE capacity by 2022, including 60 GW of wind and 100 GW of solar, up from 29 GW wind and 9 GW solar at the beginning of 2017. Thanks to advanced weather and power system modeling made for this project, the study team is able to explore operational impacts of meeting India's RE targets and identify actions that may be favorable for integration. Our primary tool is a detailed production cost model, which simulates optimal scheduling and dispatch of available generation in a future year (2022) by minimizing total production costs subject to physical, operational, and market constraints. Our team comprises a core group from the Power System Operation Corporation, Ltd. (POSOCO), which is the national grid operator (with representation from the National, Southern, and Western Regional Load Dispatch Centers) under Ministry of Power, National Renewable Energy Laboratory (NREL), and Lawrence Berkeley National Laboratory (LBNL), and a broader modeling team that includes Central Electricity Authority (CEA), POWERGRID (the central transmission utility, CTU), and State Load Dispatch Centers in Maharashtra, Gujarat, Tamil Nadu, Karnataka, Rajasthan, and Andhra Pradesh. Our model includes high-resolution wind and solar data (forecasts and actuals), unique properties for each generator, CEA/CTU's anticipated buildout of the power system, and enforced state-to-state transmission flows. Assuming the fulfillment of current efforts to provide better access to the physical flexibility of the power system, we find that power system balancing with 100 GW of solar and 60 GW of wind is achievable at 15-minute operational timescales with minimal RE curtailment. This RE capacity meets 22% of total projected 2022 electricity consumption in India with annual RE curtailment of 1.4%, in line with experiences in other countries with significant RE penetrations (Bird et al. 2016). Changes to operational practice can further reduce the cost of operating the power system and reduce RE curtailment. Coordinating scheduling and dispatch over a broader area is the largest driver to reduce costs, saving INR 6300 crore (USD $920 million) annually when optimized regionally. Lowering minimum operating levels of coal plants (from 70% to 40%) is the biggest driver to reduce RE curtailment - from 3.5% down to 0.76%. In fact, this operating property is more influential than faster thermal generation ramp rates in lowering the projected levels of curtailment. While this study does not answer every question relevant to planning for India's 2022 RE targets, it is an important step toward analyzing operational challenges and cost saving opportunities using state-of-the-art power system planning tools. Further analysis can build upon this basis to explore optimal renewable resource and intrastate transmission siting, system stability during contingencies, and the influence of total power system investment costs on customer tariffs.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2017

Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India’s Electric Grid, Vol. 1. National Study

The use of renewable energy (RE) sources, primarily wind and solar generation, is poised to grow significantly within the Indian power system. The Government of India has established a target of 175 gigawatts (GW) of installed RE capacity by 2022, including 60 GW of wind and 100 GW of solar, up from 29 GW wind and 9 GW solar at the beginning of 2017. Using advanced weather and power system modeling made for this project, the study team is able to explore operational impacts of meeting India’s RE targets and identify actions that may be favorable for integration. Our primary tool is a detailed production cost model, which simulates optimal scheduling and dispatch of available generation in a future year (2022) by minimizing total production costs subject to physical, operational, and market constraints. Our team comprises a core group from the Power System Operation Corporation, Ltd. (POSOCO), which is the national grid operator (with representation from the National, Southern, and Western Regional Load Dispatch Centers) under Ministry of Power, National Renewable Energy Laboratory (NREL), and Lawrence Berkeley National Laboratory (Berkeley Lab), and a broader modeling team that includes Central Electricity Authority (CEA), POWERGRID (the central transmission utility, CTU), and State Load Dispatch Centers in Maharashtra, Gujarat, Tamil Nadu, Karnataka, Rajasthan, and Andhra Pradesh. Our model includes high-resolution wind and solar data (forecasts and actuals), unique properties for each generator, CEA/CTU’s anticipated buildout of the power system, and enforced state-to-state transmission flows. Assuming the fulfillment of current efforts to provide better access to the physical flexibility of the power system, we find that power system balancing with 100 GW of solar and 60 GW of wind is achievable at 15-minute operational timescales with minimal RE curtailment. This RE capacity meets 22% of total projected 2022 electricity consumption in India with annual RE curtailment of 1.4%, in line with experiences in other countries with significant RE penetrations (Bird et al. 2016). Changes to operational practice can further reduce the cost of operating the power system and reduce RE curtailment. Coordinating scheduling and dispatch over a broader area is the largest driver to reduce costs, saving INR 6300 crore (USD 980 million) annually when optimized regionally. Lowering minimum operating levels of coal plants (from 70% to 40%) is the biggest driver to reduce RE curtailment—from 3.5% down to 0.76%. In fact, this operating property is more influential than faster thermal generation ramp rates in lowering the projected levels of curtailment. While this study does not answer every question relevant to planning for India’s 2022 RE targets, it is an important step toward analyzing operational challenges and cost saving opportunities using state-of-the-art power system planning tools. Further analysis can build upon this basis to explore optimal renewable resource and intrastate transmission siting, system stability during contingencies, and the influence of total power system investment costs on customer tariffs.

24 POWER TRANSMISSION AND DISTRIBUTION↗
DOE OSTI2017

Enhanced Micro-Pocket Fission Detector for High Temperature Reactors - FY17 FInal Project Report

A collaboration between the Idaho National Laboratory (INL), the Kansas State University (KSU), and the French Atomic Energy Agency, Commissariat à l'Énergie Atomique et aux Energies Alternatives, (CEA), has been initiated by the Nuclear Energy Enabling Technologies (NEET) Advanced Sensors and Instrumentation (ASI) program for developing and testing High Temperature Micro-Pocket Fission Detectors (HT MPFD), which are compact fission chambers capable of simultaneously measuring thermal neutron flux, fast neutron flux and temperature within a single package for temperatures up to 800 °C. The MPFD technology utilizes a small, multi-purpose, robust, in-core fission chambers and thermocouple. As discussed within this report, the small size, variable sensitivity, and increased accuracy of the MPFD technology represent a revolutionary improvement over current methods used to support irradiations in US Material Test Reactors (MTRs). Previous research conducted through NEET ASI1-3 has shown that the MPFD technology could be made robust and was successfully tested in a reactor core. This new project will further the MPFD technology for higher temperature regimes and other reactor applications by developing a HT MPFD suitable for temperatures up to 800 °C. This report summarizes the research progress for this three year project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Radiation Chemistry of Diethylhexylbutyramide (DEHBA)

The rate of radiolytic degradation of DEHBA with and without contact with various aqueous phases was measured, and the major degradation products were identified. The radiolytic degradation rate and products are analogous to those previously identified for DEHiBA. The amine and the amide resulting from the two possible DEHBA C-N bond ruptures do not account for a complete mass balance; however, other minor products that are possible based on analogy with results for DEHiBA were not amenable to the detection techniques used in the current work. The effects of radiolysis on solvent extraction were greater for DEHBA, with DU and DPu declining by about 50 % by 1200 kGy. Uranium stripping was not affected; however, Pu stripping was adversely impacted. Plutonium stripping was more dramatically impacted when DEHBA was irradiated in the presence of 4 M HNO 3 . Color development was observed when DEHBA/dodecane was used in solvent extraction, but only for samples irradiated in the presence of 0.1 M HNO 3 . These are indications that different products, or a different distribution in abundance of products occur for irradiation under different aqueous phase conditions. This work was performed in collaboration with CEA Marcoule, and is written in completion of milestone M3FT-17IN030104031.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Patchy snapshots of nuclear chain reactions

Stochastic fluctuations of the neutron population within a nuclear reactor are typically prevented by operating the core at a sufficiently high power. This regime, where the evolution of the neutron density is essentially deterministic, is key for automatic protection and safety systems to safely detect unwanted power excursions during an accident, and to rapidly initiate a reactor trip procedure in case it is needed. Recent works, supported by numerical simulations, have however reported that, for large reactors, the branching nature of the fission reactions might induce strongly non-Poissonian patterns in the neutron spatial distribution, and that stochastic fluctuations might still persist at reactor powers close to operating conditions (startup phase). An international program conducted by LANL, IRSN and CEA was therefore setup to experimentally detect and characterize such fluctuations and correlations. An experiment took place in 2017 at the Reactor Critical Facility (RCF) of the Rensselaer Polytechnic Institute (USA). In this paper we will report the main findings of this experimental program, supported by stochastic models and by the development of a dedicated high-fidelity Monte Carlo simulation code. We will in particular describe and explain the strong patchiness in neutron power distributions measured at the RCF, as well as a peculiar ‘blinking’ behavior of the core, and discuss the consequences of these findings on nuclear safety.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗