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This is the final technical report for the project "Resource-Efficient Quantum Simulations on NISQ Devices: Advancing the State-of-the-Art". Under this effort we have devised novel resource efficient quantum dynamical simulation algorithms. The report details our progress over the course of this three-year effort.
The Materials Research (MR) Pathway within the Light Water Reactor Sustainability (LWRS) program is charged with performing R&D to develop the scientific basis for understanding and predicting the long-term environmental degradation behavior of materials in nuclear reactors. Furthermore, the mechanistic understanding of degradation phenomena in materials must be leveraged to develop mitigation and repair strategies and new material alternatives for existing components. This research will provide data and methods to assess the performance of systems, structures, and components essential to safe and sustained reactor operations. The R&D products developed from the LWRS program will be used by stakeholders—including utilities, industry groups, and regulators—to inform operational and regulatory requirements for materials in reactor systems, structures, and components subjected to long-term operation conditions, providing key inputs to regulators and industry. Therefore, the intent of this research is to provide options to reduce the operating costs, which may be in the form of offset maintenance costs due to better predictive models for component lifetimes, improved analyses of materials through nondestructive evaluation, reduced costs for repairs, or extended performance of plants through the selection of improved replacement materials. To provide the best options, industry experience and guidance are important because of their role in coordinated or collaborative research projects. The objectives of this report are to describe the motivation and organization of the MR Pathway within the LWRS program; provide details on the individual research tasks within the MR Pathway; describe the outcomes and deliverables of the MR Pathway, including recent technical highlights and progress; and describe the requirements for performing this critically important research.
Over 50 million nuclear medicine procedures are performed annually, leading to a multi-billion dollar market for radioisotope production. The demand for new medical and research isotopes is growing, and radioisotope supply is insufficient. Most radioisotope production today utilizes charged particle or low-energy neutron irradiation of a target. Isotope production with tens to hundred MeV incident energies is a relatively unexplored option. There is a tremendous opportunity associated with a growing number of suitable domestic and international facilities buttressed by hundred million dollar global investments (e.g., the Los Alamos and Brookhaven Isotope Production Facilities, the European Spallation Source in Lund, and the Korean Multi-purpose Accelerator Complex in Gyeongbuk). In part due to a lack of supporting nuclear data that would make modeling radioisotope yields and purities possible, these facilities do not utilize their high-energy neutron fluxes for isotope production. This project attempted to measure neutron reaction excitation functions relevant to the large-scale production of critical radioisotopes, enabling development of cost-efficient isotope production methods, contributing to the improvement of theoretical models, and enhancing the value of national isotope production facilities. Reactions which form 67 Cu, 32 Si, and alpha-emitting isotopes like 225 Ac were chosen for their consistent prioritization by expert panels, representation of diverse reaction mechanisms, and relative lack of supporting nuclear data. Accurate measurement of these data is presently made only using quasi-monoenergetic neutron beams, which are produced by bombarding thin lithium targets with protons at only a few laboratories in the world. Ultimately, the projects efforts were incompletely accomplished due to a combination of multi-year technical issues at the only laboratory in the world which can make the proposed measurements, iThemba Labs in South Africa, and the onset of a global pandemic, which precluded the significant effort and time required to develop an independent measurement capability in the United States.
This final technical report summarizes the outcomes from a project that aimed to design, build, and test a persistent and autonomous monitoring system for avian and bat collisions with offshore wind turbines blades and structures. The system comprises four primary sensor modules: 1) on-blade sensor modules for collision detection and dual-vision image capture on each blade with both visible light and near-infrared imagers; 2) additional on-blade collision sensors mounted further from the root; 3) a nacelle-mounted unit including a 360º camera and ultrasonic microphone array; and, 4) an on-blade, high-performance infrared camera module. Primary targeted outcomes were high sensitivity for the detection of blade strikes from bats and small birds, and automatically captured visual confirmation of the striking object; these features are critical for monitoring offshore wind turbine installations, where ground-based methods are not viable. In addition, local recording will provide a long-term sensor recording database. Following laboratory validation, field testing was conducted on an operational wind turbine in collaboration with the National Wind Technology Center at the NREL Flatirons campus over two planned field tests.
This report provides documentation as a standard mitigation measure to the adverse effects that occurred by the demolition of theses historic properties. To mitigate the adverse effects, LANL has followed Section 106 process contained in 36 CFR 800.6, resolution of adverse effects. In addition to these regulations and within this report, LANL has implemented the standards for documenting and reporting in accordance with the A Plan for the Management of the Cultural Heritage at Los Alamos National Laboratory, New Mexico (CRMP), LA-UR-19-21590, formerly LA-UR-15-27624. These standard reporting measures include archival-quality digital photographs of the building’s interior, exterior, outside landscape; updating LANL historic building survey forms including 11 in. x 17 in. copies (in a reduced scale) of key original and as-built drawings; identification and documentation of historically significant equipment and artifacts; a comprehensive list of LANL architectural drawings; construction-history maps of TA-16 including current Register Eligible and Ineligible Buildings; and a detailed use history of the building and technical division associated with its operation.
The Bishop Paiute Tribe is committed to energy efficiency, renewable energy, and environmental protection and has a vision to install solar energy systems on all buildings on the Reservation where technically feasible. Through completion of the Bishop Paiute Tribe Residential Solar Program – Phase 4, Bishop Paiute Tribe continued its successful model partnering with non-profit solar installer GRID Alternatives to advance its vision and build energy self-sufficiency on the Bishop Paiute Reservation. The Bishop Paiute Tribe Residential Solar Program – Phase IV deployed 67 kW-AC of new clean, renewable energy through grid-tied, net-metered rooftop solar electric systems installed on a total of 20 (one more than the planned 19) existing owner-occupied, single-family homes for low-income families on the Reservation. This represents nearly 14% of the Reservation’s total “unsolarized” homes. These systems were provided at no cost to the homeowners, who will also receive energy efficiency education to further reduce energy consumption and lower electric bills. GRID led a solar installation for three (3) of the homes where Tribal/community members, were given an opportunity in participating in on-the-roof trainings to gain new skills while installing solar for their low-income community members. Subcontractors through GRID Sub Contractor Partnership Program (GRID SPP) led solar installations for seventeen (17) of the homes. Each installation provided paid employment for a solar trainee trainees hired by the SPP subcontractors as entry level solar installers. It is estimated that the installed 67 kW-AC of solar will produce at least 120,000 kWh/year, displacing at least 30-75% of the 20 homes’ total electricity use for a combined system lifetime electricity cost savings for the low-income homeowners of about $\$$500,000. It is further estimated that the installed renewable energy systems installed will prevent greenhouse gases by about 1,000 tons, equivalent to planting approximately 25,000 trees. Following the successful completed installations, it is expected that the Reservation and surrounding communities will benefit from improved air quality via reduced wood stove use for heating. Cumulatively with other initiatives, the project will result in nearly 40% of the Reservation’s solarizable homes being solarized. Overall, the triple impact of the phase 4 of the Bishop Paiute Tribe Residential Solar Program – Phase 4 is: 1) affordable energy for low-income families; 2) on-site clean energy production, 3) hands on training and paid solar installation work for local tribal/community workers. These impacts will support and grow the Tribe’s energy, economic, environmental, and social self-sufficiency and sovereignty amongst the neediest on the Reservation.
In July 2010 funding for an award was made available under contract DE-EE0004200 which is the focus of this report. Under this funding, The U.S. Department of Energy’s (USDOE) designated Florida Atlantic University’s (FAU) state of Florida marine renewable energy focused Center of Excellence for Ocean Energy Technology as the Southeast National Marine Renewable Energy Center (SNMREC). The award was advertised in 2008, when the USDOE Wind and Water Program issued a funding opportunity announcement (DE-PS36-08GO98030) to establish university-led National Marine Renewable Energy Centers (NMRECs). Although FAU was selected for this opportunity, funding did not become available until 2010 at which time three of the original five years of performance remained and scope was adjusted accordingly. This award was divided into two phases. The first phase focused on marine energy turbine system enhancement and research while the second phase aimed to advance offshore capabilities and testing opportunities for small-scale demonstration turbines. The project’s objective was to increase the nation’s capabilities, knowledge, and competitiveness with respect to ocean current energy technology. This project successfully achieved these goals by advancing marine energy technology testing opportunities and capabilities. This report details these accomplishments by phase and task. Descriptions include any relevant results, challenges, achievements, and outcomes. Additional intellectual products and publications are listed in the Appendix where detailed technical explanations can be found. Further, because this award designated SNMREC as a USDOE center, it challenges FAU to continue providing value for the marine energy sector in the long term. The direct accomplishments of this project, though noteworthy, are also the seeds for a greater partnership between the USDOE and FAU. SNMREC, leveraging its designation as an NMREC under this award, will expand these contributions for decades to come as a coordinated sustainable program that can serve the marine energy sector’s needs as they arise.
The Accelerated Basin De-inventory (ABD) program involves discarding spent nuclear fuel that is currently stored in L-Basin to the Defense Waste Processing Facility (DWPF) for vitrification. The first ABD discards will occur during the preparation of Sludge Batch (SB) 11. Savannah River Mission Completion has requested that the Savannah River National Laboratory assess the technical gaps related to the increased gadolinium poisoning requirement and the impacts of performing the Low Temperature Aluminum Dissolution (LTAD) process in Tank 51 with H-Canyon discards present. The following summarizes the evaluation of the impacts of increasing the quantity of gadolinium (and related topics) from what was previously evaluated in the SRNL studies of gadolinium-poisoned ABD material solubility, the overall ABD flowsheet review, and increasing the fissile mass loading in glass: 1) Based on literature surveys, there is no indication that organic interactions with gadolinium will be significant at the high pH (typically >13) conditions of the Concentration, Storage, and Transfer Facilities. Any interactions of gadolinium with organics in DWPF are not expected to adversely impact DWPF or downstream facilities. Thus, there is little-to-no residual risk from organic interactions with gadolinium [Gap closed]; 2) Adding depleted uranium to ABD material, targeting 235 U enrichment of 4.90% within each transfer window, will mitigate potential impacts from an increase in soluble 235 U enrichment during sludge washing and LTAD. The plan to take advantage of previous transfers and allow 235 U enrichment of >5% during the final transfer window carries a risk that Tank 51 supernate will have a 235 U enrichment of >5%, which should be evaluated for acceptance; 3) Increasing the gadolinium mass ratio to 3.0:1 Gd: 235 U(eq SLU ) should lead to the same or higher partitioning of gadolinium into the solid phase within the DWPF Chemical Process Cell, resulting in both liquid and solid phases with expected partitioning of Gd consistent with the prior solubility study [Gap closed for SB11]; 4) There are no expected impacts on DWPF melt temperature and melter operations due to the minimal ~0.2 weight percent (wt%) increase in Gd concentration relative to previous sludge batches [Gap closed for SB11]; 5) As observed previously, Gd is expected to enter the off-gas system via physical entrainment, but at a slightly higher concentration than what was observed for SB9 melter off-gas pluggage deposits (0.07 wt%) [Gap closed for SB11] ; 6) There are no expected impacts on DWPF recycle or the Recycle Collection Tank glycolate destruction process. [Gap closed for SB11]; 7) Gd is projected to be a trace component in the SB11 glass (<0.5 wt%) and can be ignored for process control. Trace components do not significantly impact glass durability, thus the conclusions of the previous Product Consistency Test evaluation at a fissile mass loading of 2,500 g fissile/m3 glass still applies to SB11. The ~0.1 wt% increase in Gd2O3 concentration relative to the previous study will not impact the predictability of SB11 glass with the DWPF Product Composition Control System (PCCS) models for durability or the acceptability of glass according to the Waste Acceptance Product Specifications (WAPS) criterion for product consistency [Gap closed for SB11]; 8) No additional Toxicity Characteristic Leaching Procedure testing is necessary for SB11 and the hazardous waste specification of the SB11 DWPF waste form is unchanged after the addition of the ABD stream [Gap closed for SB11]. The following summarizes the evaluation of the impacts of adding two-thirds of the ABD material to Tank 51 prior to LTAD: 1) The addition of two-thirds of the ABD increases overall aluminum mass from 1.39×10 4 kg to 1.64×10 4 kg (15.5% ABD Al). The form of the insoluble portion of the Al resulting from ABD addition should be the more readily dissolved Al(OH) 3 and amorphous forms. The portion of the ABD aluminum that is processed by LTAD is expected to be completely soluble, thus requiring that less of the boehmite in the sludge be dissolved to reach the same Al target in the SB. [Gap closed for SB11]; The expected LTAD impact on other components, as related primarily to the components in ABD, are discussed. Gd is expected to remain insoluble during LTAD and not impact the solubility of other components. [Gap closed for SB11]; The addition of two-thirds of the ABD increases overall projected SB11 uranium mass from 4,740 kg to 13,100 kg (63% ABD U) and the projected plutonium mass from 86.0 kg to 89.5 kg (3.9% ABD Pu). The addition of all of the ABD increases overall projected SB11 uranium mass from 4,740 kg to 16,100 kg (70% ABD U) and the projected plutonium mass from 86.0 kg to 90.4 kg (5.3% ABD Pu). The 235 U enrichment will be ≤5%. The fissile uranium will be adequately poisoned by Gd and the fissile Pu will be adequately poisoned by Fe from the sludge. [Gap closed for SB11]; There is a low risk that ABD addition will impact the rheology or pumpability of the slurry. There is a low but higher risk of ABD addition prior to LTAD impacting the settling rate; Based on the evaluation of adding two-thirds of the ABD material and all of the ABD material prior to the LTAD process, there is no volume or mass limit that would need to be imposed on ABD additions prior to LTAD. [Gap closed for SB11]. Revision 1 of this report addresses a variation on the ABD additions and LTAD strategy where sodium hydroxide additions for LTAD may be performed intermittently or concurrently with an ABD addition window. The proposed change does not alter the conclusions of this evaluation.
This final technical report describes the main findings of the project Wireless Microsensors System for Monitoring Deep Subsurface Operations (FE0031850). The project was part of the U.S. Department of Energy National Energy Technology Laboratory FOA 1998 program to develop new sensor systems for direct observation of parameters associated with CO2 injection and to provide data collection without being disruptive to operations. The overall DOE program was aimed at developing and validating innovative transformational sensor systems, amenable for integration with autonomous intelligent monitoring systems, that are capable of being deployed within the casing annulus and do not have casing perforation or wires/cables in the annulus for installation, power supply, or data transmission needs. Project accomplishments included 1) design and fabrication of a wireless downhole sensor system to monitor parameters for CO2 storage, 2) field testing of the sensor system in two legacy oil & gas wells, and 3) development of an analysis approach that validates the measurements and demonstrates the application of the technology to depict CO2 movement in the subsurface. The project leveraged new sensor technologies along with specialized wellbore telemetry, deployment, and analysis methods designed to address the challenges and risks related to CO2 storage in the subsurface. Results from field testing were a mixture of successes and challenges. The temperature sensor rings, installation procedures in legacy oil & gas wells, wireless powering demonstration, automated data collection, and material compatibility were successful. The wireless data transfer through cement to the wellhead via the sensor relays was not functional beyond the first relay. Consequently, work in the last year of the project included some additional testing of data transmission through different materials along with modeling and analysis of field data for CO2 monitoring applications. This work suggested there are options like polymer cements and open hole annuli that may allow point-to-point transmission along the borehole. The techno-economic analysis suggests that the sensor system is ~40% less expensive than fiber optic distributed temperature system. Modeling of CO2 storage applications suggests temperature can provide an indicator of CO2 saturation but would be best combined with pressure sensors.
This thesis focuses on a technical hiring manager’s approach to over come challenges surrounding developing pipelines and performing talent acquisition at NNSAs largest national research and development laboratory.
This report serves as the final technical report for the US Department of Energy (DOE) award DE-EE0006713 (Award 6713). The project is titled “New England Aqua Ventus I Offshore Wind Advanced Technology Demonstration Project 100% Front-End Engineering and Design (FEED)”. The New England Aqua Ventus I (NEAV) project demonstrates a unique prestressed concrete semi-submersible floating hull technology, called VolturnUS. The technology is applicable to harness nearly 60% of the US offshore wind resource within 50 miles of the coast. The hull will be demonstrated at full-scale with a commercial scale wind turbine connected to the grid in the Northeast US off Monhegan Island, Maine for 20 years.
This technical report summarizes the main accomplishments of the research performed under the U.S. Department of Energy (DOE) Office of Science, Early Career Award (ECA), grant number DE-SC0018117, from 9/1/2017 to 8/31/2022, with Prof. Dennis Perepelitsa as the single PI. The grant proposal was to investigate the quark-gluon plasma (QGP) created in ultrarelativistic collisions of large nuclei with the ATLAS experiment at the Large Hadron Collider (LHC) and to prepare for this physics with the sPHENIX experiment at the Relativistic Heavy Ion Collider (RHIC). In particular, the focus was on QGP regions of different sizes and shapes, including the tradtional “large” collision systems such as Pb+Pb as well as small collision systems such as p+Pb, where there has been evidence of QGP “flow” but not yet the accompanying energy loss from hard-scattered partons traversing the QGP medium. Additionally, a particular tool was the use of photon+jet events, where the photon is unaffected by the QGP and thus serves as the “control” while the jet (the result of parton fragmentation) is the “probe” of the QGP. The research was successfully carried out, resulting in over ten publications of experimental measurements in peer-reviewed journals, and the significant training of junior scientists.
The building stock in the United States (U.S.) varies significantly as a function of several macro variables such as: climate, building type, vintage, and density. These variables change across the U.S. and can also significantly impact energy usage of the individual buildings and overall stock. For example, the square foot density and building type varies by several orders of magnitude from Manhattan to the eastern plains of Colorado. The diversity in energy use of the building stock of different areas of the U.S. is significant, and as a result, analyses that require localized results need to consider the relevant geography and the current makeup of the building stock. This document discusses the development and implementation of a stock clustering algorithm that produces a technically rigorous, consistent, and repeatable collection of geographies which are used as the basis for localized analysis. This framework considers the impact of built environment density, diversity, and climate in creating groupings of counties that create a far more nuanced analysis framework than national averages. Clustering of counties together represents a similarity of building characteristics and climate zone.
This technical brief provides requirements for electric readiness that could be incorporated into model residential energy codes. It provides background on the basis and benefits of the provisions, and model code language that can be plugged into the IECC or adapted into other energy codes.
Hybrid inorganic-microbial systems have emerged as a potentially transformative approach to combine the light-harvesting capability of inorganic semiconductors and the ability of microbes to orchestrate complex chemical transformations. The objective of this collaborative research is to combine quantum materials synthesis, bacterial synthetic biology, and multimodal single-entity imaging to quantitatively study how hybrid QD-bacteria systems convert light to value chemicals at the single-to-sub cell level, with the ultimate goal of gaining insights to guide the engineering of QDs and bacterial genetics for more efficient bioenergy conversion. The final technical report summarizes our achievements toward this objective.
Using a new Time Projection Chamber (TPC), called the SpiRIT (SAMURAI pion Reconstruction Ion Tracker) constructed and funded by DOE office of science (award # DE-SC0004835), we performed two experiments with the SAMURAI spectrometer at RIKEN, Japan to study the equation of state of neutron rich matter. As a result of the project, the SpiRIT collaboration, an international collaboration consisting of groups from US, Japan, Korea, Poland, China and Germany, has been formed to pursue the science opportunities provided by the SpiRIT TPC. After the experiments, we developed the software to analyze the SpiRIT experiments and extract constraints of symmetry energy at supra-saturation densities. As a result 270 TB of data have been obtained. Over 10 technical papers on the TPC and 4 science papers on the nuclear equation of state have been published. A total of six (2 US, 1 Japanese and 1 Korean) PhD students have graduated based on their research on the EOS research using the SpiRIT data. In addition, the data also stimulated theorists on transport models to form the “Transport Model Evaluation Project” collaboration to improve the transport model to compare calculations with the data.
This project developed methodologies to measure the in-situ principal stress in the deep subsurface through use of multiple independent, but complementary, seismic methods, laboratory verification, and development of theoretical frameworks. By leveraging existing regional and local datasets we developed, tested, and refined a set of diagnostic tools for determining the in-situ stress state with reduced uncertainty at and below reservoir depths (1.5-6 km). A set of novel tools was produced that are scale independent, such that their utility is equivalent on regional, field scale, and near borehole monitoring of principal stresses in reservoir underburden for carbon storage projects. During a 4-year Department of Energy (DOE) and Southern Company funded project, carried out by the Electric Power Research Institute (EPRI), Lawrence Livermore National Laboratory (LLNL), the University of Oklahoma (OU), and the U.S. Geological Survey (USGS), the project team developed methodologies to measure the far-field in-situ principal stress in the deep subsurface, leveraging induced seismicity data from waste-water disposal projects. These methodologies consisted in the use of well-established and technically advanced seismic processing methods, such as virtual seismometer method-moment tensor (VSM-MT) and shear wave splitting (SWS), that are adept at recovering the stress orientation and certain components of the stress tensor. These methods were applied to robust seismicity catalogs created with matched filter techniques near sites of active fluid disposal—a proxy for carbon storage sites where such datasets are more limited. Estimates of the stress orientation made with seismic processing tools were considered along with laboratory acoustic emission experiments conducted on rock samples from the region of interest. Stress orientations in the studied region do not vary significantly across distances of ~100 km, nor are they found to rotate through time as a consequence of local wastewater disposal, as previously speculated. Finally, the project team investigated the trade-offs among the different seismic methods and evaluated the range of uncertainty that is generated with these methodologies, which led to a practical use and refinement of the VSM-MT technique when it is applied to field datasets. Understanding the trade-offs between these different methods highlighted the potential benefits of improved quantification of uncertainties on stress field estimations.
The growing use of hydrogen gas across energy, transportation, and chemical applications necessitates better hydrogen sensors and detectors. Few sensors exist for quantifying hydrogen gas in a corrosive, oxygen-free gas stream due to the challenging nature of the sampling environment and current technological status. Handheld, economic options include palladium-based, metal oxide, catalytic bead, and electrochemical sensors. More permanent and costly options include electrochemical sensors, thermal gas analyzers, mass spectrometers, gas chromatographs, and Raman spectrometers. In this technical report, a short review of current technology, along with the associated commercially available products, is provided. Raman spectroscopy is recommended as an ideal technology for on-line detection of hydrogen at low concentrations in a corrosive, oxygen-free gas stream.