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At least 379 records · Page 21

A mobile system for a comprehensive online-characterization of nanoparticle aggregates based on wide-angle light scattering and laser-induced incandescence

A mobile demonstrator for the comprehensive online-characterization of gas-borne nanoparticle aggregates is presented. Two optical measurement techniques are combined, both utilizing a pulsed Nd:YAG laser as light source. Aggregate size and fractal dimension are measured by Wide-Angle Light Scattering (WALS). An ellipsoidal mirror images elastically scattered light from scattering angles between 10° and 165° onto a CCD-camera chip resulting in an almost complete scattering diagram with high angular resolution. Primary particle size and volume fraction are measured by time-resolved Laser-Induced Incandescence (TiRe-LII). Here, particles are heated up to about 3000 K by the short laser pulse, the enhanced thermal radiation signal is detected with gated photomultiplier tubes. Analysis of the signal decay time and maximum LII-signal allows for the determination of primary particle diameter and volume fraction. The performance of the system is demonstrated by combined measurements on soot nanoparticle aggregates from a soot aerosol generator. Particle and aggregate sizes are varied by using different equivalence ratios of the combustion in the generator. Soot volume fraction can be adjusted by different levels of dilution with air. Online-measurements were carried out demonstrating the favorable performance of the system and the potential for industrial applications such as process control and product development. The particle properties obtained are confirmed through transmission electron microscopy analysis on representative samples.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

System Modeling and Simulation of In-Stream Hydrokinetic Turbines for Power Management and Control

Electricity generation from moving currents without using dams (i.e., in-stream hydrokinetic electricity) has the potential to introduce multiple GW of renewable power to U.S. grids. Here this study evaluates a control system designed to regulate the generator rotor rate (rpm) to improve power production from in-stream hydrokinetic turbines. The control algorithm is evaluated using numerical models of both a rigidly mounted tidal turbine (TT) and a moored ocean current turbine (OCT) coupled to an induction electric machine model. The moored simulation utilizes an innovative approach for coupling a multiple degrees-of-freedom (DOF) nonlinear hydrodynamic/mechanical turbine model with a nonlinear electromechanical generator model. Based on the turbine torque-speed characteristic, as well as the asynchronous machine features, a proportional–integral (PI) controller is used to generate a correction term for the frequency of the three-phase sinusoidal voltages that are supplied to the asynchronous generator. The speed control of the induction generator through the supply frequency is accomplished by a simplified voltage source inverter (VSI). The simplified VSI consists of control voltage sources (CVSs), while the comparison with a real VSI using diodes and transistors, which are controlled by pulse width modulation (PWM) technique, is also presented. Simulations are used to evaluate the developed algorithms showing that rpm fluctuations are around 0.02 for a tidal turbine operating in a wave field with a 6 m significant wave height and around 0.005 for a moored ocean current turbine operating in a wave field with a 2 m significant wave height.

16 TIDAL AND WAVE POWER↗

Characterization of intense ion beam energy density and beam induced pressure on the target with acoustic diagnostics

We have developed the acoustic diagnostics based on a piezoelectric transducer for characterization of high-intensity pulsed ion beams. The diagnostics was tested using the TEMP-4M accelerator (150 ns, 250–300 kV). The beam is composed of C{sup +} ions (85%) and protons, the beam energy density is 0.5–5 J/cm{sup 2} (depending on diode geometry). A calibration dependence of the signal from a piezoelectric transducer on the ion beam energy density is obtained using thermal imaging diagnostics. It is shown that the acoustic diagnostics allows for measurement of the beam energy density in the range of 0.1–2 J/cm{sup 2}. The dependence of the beam generated pressure on the input energy density is also determined and compared with the data from literature. The developed acoustic diagnostics do not require sophisticated equipment and can be used for operational control of pulsed ion beam parameters with a repetition rate of 10{sup 3} pulses/s.

43 PARTICLE ACCELERATORS↗

Phase control of light propagation via Fano interference in asymmetric double quantum wells

We investigate the light propagation and dynamical control of a weak pulsed probe field in asymmetric double quantum wells via Fano interference, which is caused by tunneling from the excited subbands to the same continuum. Our results show that the system can produce anomalous and normal dispersion regions with negligible absorption by choosing appropriate coupling strength of the tunneling and the Fano interference. Interesting enough, the dispersion can be switched between normal and anomalous by adjusting the relative phase between the pulsed probe and coherent control fields owing to the existence of the perfectly Fano interference. Thus, the relative phase can be regarded as a switch to manipulate light propagation with subluminal or superluminal. The temporal and spatial dynamics of the pulsed probe field with hyperbolic secant envelope are analyzed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Symmetric Rydberg controlled- Z gates with adiabatic pulses

We analyze neutral atom Rydberg C Z gates based on adiabatic pulses applied symmetrically to both atoms. Analysis with smooth pulse shapes and Cs atom parameters predicts the gates can create Bell states with fidelity F > 0.999 using adiabatic rapid passage (ARP) pulses. With globally optimized adiabatic pulse shapes, in a two-photon excitation process, we generate Bell states with fidelity F = 0.997. The analysis fully accounts for spontaneous emission from intermediate and Rydberg states, including the Rydberg lifetime in a room temperature environment, but does not include errors arising from laser noise. In conclusion, the gate protocols do not require individual addressing and are shown to be robust against Doppler shifts due to atomic motion.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Electric-optic resonant phase modulator

An electro-optic resonant cavity is used to achieve phase modulation with lower driving voltages. Laser damage thresholds are inherently higher than with previously used integrated optics due to the utilization of bulk optics. Phase modulation is achieved at higher speeds with lower driving voltages than previously obtained with non-resonant electro-optic phase modulators. The instant scheme uses a data locking dither approach as opposed to the conventional sinusoidal locking schemes. In accordance with a disclosed embodiment, a resonant cavity modulator has been designed to operate at a data rate in excess of 100 Mbps. By carefully choosing the cavity finesse and its dimension, it is possible to control the pulse switching time to within 4 ns and to limit the required switching voltage to within 10 V. Experimentally, the resonant cavity can be maintained on resonance with respect to the input laser signal by monitoring the fluctuation of output intensity as the cavity is switched. This cavity locking scheme can be applied by using only the random data sequence, and without the need of additional dithering of the cavity. Compared to waveguide modulators, the resonant cavity has a comparable modulating voltage requirement. Because of its bulk geometry, resonant cavity modulator has the potential of accommodating higher throughput power. Furthermore, mode matching into a bulk device is easier and typically can be achieved with higher efficiency. On the other hand, unlike waveguide modulators which are essentially traveling wave devices, the resonant cavity modulator requires that the cavity be maintained in resonance with respect to the incoming laser signal. An additional control loop is incorporated into the modulator to maintain the cavity on resonance.

Chen, Chien-Chung↗

Tutorial: Reactive high power impulse magnetron sputtering (R-HiPIMS)

High Power Impulse Magnetron Sputtering (HiPIMS) is a coating technology that combines magnetron sputtering with pulsed power concepts. Furthermore, by applying power in pulses of high amplitude and a relatively low duty cycle, large fractions of sputtered atoms and near-target gases are ionized. In contrast to conventional magnetron sputtering, HiPIMS is characterized by self-sputtering or repeated gas recycling for high and low sputter yield materials, respectively, and both for most intermediate materials. The dense plasma in front of the target has the dual function of sustaining the discharge and providing plasma-assistance to film growth, affecting the microstructure of growing films. Many technologically interesting thin films are compound films, which are composed of one or more metals and a reactive gas, most often oxygen or nitrogen. When reactive gas is added, non-trivial consequences arise for the system because the target may become “poisoned,” i.e., a compound layer forms on the target surface affecting the sputtering yield and the yield of secondary electron emission and thereby all other parameters. It is emphasized that the target state depends not only on the reactive gas' partial pressure (balanced via gas flow and pumping) but also on the ion flux to the target, which can be controlled by pulse parameters. This is a critical technological opportunity for reactive HiPIMS (R-HiPIMS). The scope of this tutorial is focused on plasma processes and mechanisms of operation and only briefly touches upon film properties. It introduces R-HiPIMS in a systematic, step-by-step approach by covering sputtering, magnetron sputtering, reactive magnetron sputtering, pulsed reactive magnetron sputtering, HiPIMS, and finally R-HiPIMS. The tutorial is concluded by considering variations of R-HiPIMS known as modulated pulsed power magnetron sputtering and deep-oscillation magnetron sputtering and combinations of R-HiPIMS with superimposed dc magnetron sputtering.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Absorption spectrum of a two-level system subjected to a periodic pulse sequence

We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS’s photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g. for the development of efficient interfaces between stationary and flying qubits in modern architectures for quantum computation and quantum communication. We consider the periodic pulse control, where the TLS is subjected to a periodic sequence of the near-resonant Rabi driving pulses, each pulse implementing a 180° rotation. For small inter-pulse delays, the absorption spectrum features a pronounced peak of stimulated emission at the pulse frequency, as well as equidistant satellite peaks with smaller spectral weights. As long as the detuning between the carrier frequency of the driving and the TLS transition frequency remains moderate, this spectral shape shows little change. Therefore, the quantum control allows shifting the absorption peak to a desired position, and locks the absorption peak to the carrier frequency of the driving pulses. Detailed description of the spectrum, and its evolution as a function time, the inter-pulse spacing and the detuning, is presented.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Thermal Response of a Lithium Vapor Divertor to Cyclical Operation

The lithium vapor divertor concept is being developed as a method to achieve detached divertor conditions in a tokamak while minimizing impurity radiation losses from the core plasma. SOLPS-ITER modeling has previously been used to identify some of the geometric constraints and required lithium evaporation rate of a lithium vapor divertor in a medium-sized tokamak during steady-state operation. Here an updated conceptual design based on these operating requirements is introduced and the thermal response of the system is modeled during cyclical operation, consistent with operation in a short-pulse tokamak. Controllability of the temperature of the lithium capillary porous system (CPS) is achieved by adopting a design where there is no line-of-sight for radiation from the plasma to reach the heated CPS surface. Operational strategies to minimize the amount of lithium evaporated between plasma discharges while achieving steady evaporation rates during plasma discharges are discussed and modeled here. The optimal feedforward control strategy demonstrated in this work is to ramp up the temperature of the evaporator as quickly as possible immediately before a plasma discharge and then reduce the heating to match the desired steady-state net evaporation rate just before the plasma discharge begins, allowing the thermal inertia of the system to stabilize the evaporation rate during the first second of the plasma discharge.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Effect of magnetic field on the character of fluorescence of dense and cold atomic ensembles excited by pulsed radiation

Specific features of fluorescence of dense and cold nondegenerate atomic ensembles in an external constant magnetic field are analyzed theoretically. The angular distribution, polarization properties, as well as the spectral composition of fluorescence radiation are calculated. The time variation of these characteristics after the end of the excitation pulse is analyzed. The dependence of the properties of secondary radiation on the duration and carrier frequency of the pulse is investigated. It is shown that, for dense clouds in which the free path length of quasiresonance photons is commensurate with the interatomic distance, the magnetic field significantly modifies all the observable properties of the radiation. Under these conditions, the trapping time may increase by tens of times. Magnetic field enhances the effect of quantum beats observed on time scales commensurate with the lifetime of the excited states of atoms. For individual polarization channels, this field also intensifies the phenomenon of coherent backscattering (CBS). The phenomena found are explained by the effect of magnetic field on the character of resonance dipole–dipole interaction and, as a result, on the specific features of collective phenomena in dense atomic ensembles.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ultrafast control and monitoring of material properties using terahertz pulses

These are a set of slides on ultrafast control and monitoring of material properties using terahertz pulses. A few of the topics covered in these slides are: How fast is a femtosecond (fs), Different frequencies probe different properties of molecules or solids, What can a THz pulse do to a material, Ultrafast spectroscopy, Generating and measuring ultrashort THz pulses, Tracking ultrafast spin dynamics in antiferromagnets through spin wave resonances, Coherent two-dimensional THz spectroscopy, and Probing vibrational dynamics at a surface. Conclusions are: Coherent two-dimensional THz spectroscopy: a powerful approach for studying coherence and dynamics of low energy resonances. Applying this to graphene we investigated the very strong THz light mater interaction which dominates over scattering. Useful for studying coupled excitations in multiferroics and monitoring chemical reactions. Also, THz-pump, SHG-probe spectoscopy: an ultrafast, surface sensitive probe of atomic-scale symmetry changes and nonlinear phonon dymanics. We are using this in Bi 2 Se 3 to investigate the nonlinear surface phonon dynamics. This is potentially very useful for studying catalysis.

36 MATERIALS SCIENCE↗

A solid-state Marx generator driven Einzel lens chopper

A new type of pulse chopper called an Einzel lens chopper is described. An Einzel lens placed immediately after an electron cyclotron resonance ion source is driven by high-voltage pulses generated by a newly developed solid-state Marx generator. A rectangular negative barrier pulse-voltage is controlled in time, and the barrier pulse is turned on only when a beam pulse is required. The results of successful experiments are reported herein.

43 PARTICLE ACCELERATORS↗

Nanochemical effects in femtosecond laser ablation of metals

We study chemical energy released from the oxidation of aluminum in multipulse femtosecond laser ablation in air and oxygen. Our study shows that the released chemical energy amounts to about 13% of the incident laser energy, and about 50% of the ablated material is oxidized. The ablated material mass per laser pulse is measured to be on the nanogram scale. Our study indicates that femtosecond laser ablation is capable of inducing nanochemical reactions since the femtosecond laser pulse can controllably produce nanoparticles, clusters, and atoms from a solid target.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Control of Brillouin short-pulse seed amplification by chirping the pump pulse

Seed amplification via Brillouin backscattering of a long pump pulse is considered. Similar to Raman amplification, several obstructive effects may occur during short-pulse Brillouin amplification. One is the spontaneous Raman backscattering of the pump before interacting with the seed. Preforming the plasma and/or chirping the pump will reduce unwanted pump backscattering. Optimized regions for low-loss pump propagation were proposed already in conjunction with Raman seed amplification. Hence, the influence of the chirp of the pump during Brillouin interaction with the seed becomes important and will be considered here. Both, the linear as well as the nonlinear evolution phases of the seed caused by Brillouin amplification under the action of a chirped pump are investigated. The amplification rate as well as the seed profiles are presented as function of the chirping rate. Also the dependence of superradiant scaling rates on the chirp parameter is discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Coherent (photon) vs incoherent (current) detection of multidimensional optical signals from single molecules in open junctions

The nonlinear optical response of a current-carrying single molecule coupled to two metal leads and driven by a sequence of impulsive optical pulses with controllable phases and time delays is calculated. Coherent (stimulated, heterodyne) detection of photons and incoherent detection of the optically induced current are compared. Using a diagrammatic Liouville space superoperator formalism, the signals are recast in terms of molecular correlation functions which are then expanded in the many-body molecular states. Two dimensional signals in benzene-1,4-dithiol molecule show cross peaks involving charged states. The correlation between optical and charge current signal is also observed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Full-field vibration measurements of the violin using digital stroboscopic holographic interferometry and electromagnetic stimulation of the strings

We developed a setup in which the strings of the violin are driven electromagnetically, and the resulting vibration of the instrument is measured with digital stroboscopic holography. A 250 mW single mode green laser beam is chopped using an acousto-optic modulator, generating illumination pulses of 2% of the vibration period. The phase of the illumination pulse is controlled by a programmable function generator so that digital holograms can be recorded on a number of subsequent time positions within the vibration phase. From these recordings, the out of plane motion as a function of time is reconstructed in full field. We show results of full-field vibration amplitude and vibration phase maps, and time resolved full-field deformations of the violin back plane. Time resolved measurements show in detail how the deformation of the violin plane changes as a function of time at different frequencies. We found very different behavior under acoustic stimulation of the instrument and when using electromagnetic stimulation of a string. The aim of the work it to gather data which can be used in power flow calculations to study how the energy of the strings is conducted to the body of the violin and eventually is radiated as sound.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗