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At least 379 records · Page 21

The Ice Particle and Aggregate Simulator (IPAS). Part III: Verification and Analysis of Ice–Aggregate and Aggregate–Aggregate Collection for Microphysical Parameterization

Abstract The Ice Particle and Aggregate Simulator (IPAS) is used to theoretically represent the aggregation process of ice crystals. Aggregates have a variety of formations based on initial ice particle size, shape, and falling orientation, all of which influence water phase partitioning. Aggregate dimensional properties and density changes are calculated for monomer–monomer (MON–MON), monomer–aggregate (MON–AGG), and aggregate–aggregate (AGG–AGG) collection to be used by ice-microphysical models for improvement in aggregation parameterizations. Aggregates are chosen from a database of 9 744 000 preformed combinations to be further collected (see Part II). AGG–AGG collection results in more extreme and a smaller range of aggregate aspect ratios than MON–AGG collection. A majority of aggregates are closer to prolate than oblate spheroids, regardless of collection type, except for quasi-horizontally oriented particles that have extreme aspect ratios to begin with. MON–AGG collection frequently results in an increase in density upon collection, whereas MON–MON and AGG–AGG collection almost always result in particle density decreases, with extreme reductions near 99% for MON–MON collection. MON–MON collection results in the greatest decreases in density but then quickly becomes unaffected by the addition of more monomers due to inherent size differences between monomers and aggregates. Finally, a holistic analysis to in situ observations of cloud particle images is presented. IPAS 2D aspect ratios surround a median value of 0.6 and closely follow that of previous studies while varying by no more than ≈12% on average from observed aggregates.

54 ENVIRONMENTAL SCIENCES↗

Seasonal Precipitation Classification during Surface Atmosphere Integrated Field Laboratory Campaign

The Surface Atmosphere Integrated Field Laboratory (SAIL) campaign, conducted from September 2021 to June 2023 in Crested Butte, Colorado, aimed to characterize precipitation processes in the Upper Colorado River Basin (UCRB). This increased observations of snowfall accumulation in this hydrologically significant watershed would be useful for quantitative precipitation estimates (QPE). Therefore, the Surface Quantitative Precipitation Estimate (SQUIRE) product was developed using the ARM-supported Colorado State University (CSU) X-band Precipitation Radar. Although SQUIRE will be only released for snowfall, by categorizing precipitation types, users can effectively utilize relevant datasets under diverse meteorological conditions. Moreover, the dataset facilitates validation of the QPE product and the analysis of seasonal variations in precipitation types at the surface. Hydrometeors classes are organized based on their phase and physical characteristics mapping the CSU (both winter Summer) and Py-ART classifications into four groups. 1. Liquid Precipitation: includs drizzle, rain, and large raindrops. 2. Frozen Snow and Ice : Pure Snow, combining ice crystals, aggregates, and vertically oriented ice structures. 3. Dense and Large frozen hydrometeors: including low- and high-density graupel and dry hail. 4.Melting: Wet Snow and Melting Hail, hydrometeors exhibiting both liquid and frozen characteristics.

54 ENVIRONMENTAL SCIENCES↗

Cirrus optical depth retrieval from satellite-measured bidirectional reflectance

In the framework of investigating the relationship between the visible optical depth and microphysics of cirrus clouds, the doubling scheme for radiative transfer in cirrus cloudy atmospheres, as developed by Takano and Liou (1988), has been used to compute the bidirectional reflectances at the top of the atmosphere. Reflectance data taken at about the same time from GOES and AVHRR over Waussau, as well as particle distributions observed during the FIRE IFO carried out in Wisconsin (1986) were the basis of the experiment. For the cirrus microphysical model, hexagonal ice crystals and area-equivalent ice spheres are considered. The single scattering phase functions for randomly oriented hexagonal columns and area-equivalent ice spheres are computed from geometric optics and Mie theory, respectively.

Takano, Y.↗

An Investigation of the Grain Size and Adhesion Strength of High-Speed Impact Ice

Ice accumulation on aircraft from supercooled water droplets (impact icing) can increase drag and decrease lift, leading to a decrease in fuel efficiency and a potential for unsafe situations. Anti-icing materials and coatings are of high interest to prevent aircraft icing. Because no anti-icing material suitable for in-flight situations has been realized, icing models aim to predict the accumulation and shape of the ice to understand its effects. In both cases, understanding the physical mechanism behind ice adhesion and shedding is necessary. A recent literature review has shown that the apparent ice adhesion strength to any specific material varies over several orders of magnitude across studies and test methods. One of the reasons for this high variance is likely to be the varying microstructure of the ice used for different studies. Although the microstructure of impact ice has been studied in the past, those conditions were not relevant to that of in-flight aircraft icing. The microstructure of the ice formed will determine both its bulk and surface properties, yet it has been overlooked in the ice adhesion community. Here, we use optical microscopy to study the non-uniform ice crystal grain size in impact ice accreted in NASA Glenn Research Center’s Icing Research Tunnel at various icing conditions. Similar to other environmental conditions studied in the literature, we show an increase in grain size at larger distances from the growth interface; however, the data shows substantially larger grains than what was expected from the prior literature. Ice accrued at lower temperatures has a smaller grain size at all distances from the growth interface. No change in grain size was noticed when varying only the wind speed. A correlational analysis shows that smaller grain sizes at the growth interface corresponded to an increase in the apparent ice adhesion strength when the adhesive failure was interfacial, but not when the failure was cohesive. These results may explain the overall trend in the literature of increasing apparent adhesion strength with decreasing temperature. Incorporating microstructure trends for various environmental conditions in icing models may increase the certainty in predicting ice adhesion strength and shedding, and will provide a better basis for comparison between adhesive tests on ice produced in different facilities and at different storage times.

• Ice Fabric↗

Cloud-Resolving ICON Simulations of Secondary Ice Production in Arctic Mixed-Phase Stratocumuli Observed during M-PACE

Field measurements and modeling studies suggest that secondary ice production (SIP) may close the gap between observed Arctic ice nucleating particle (INP) concentrations and ice crystal number concentrations ni. Here, we explore sensitivities with respect to the complexity of different INP parameterizations under the premise that ni is governed by SIP. Idealized, cloud-resolving simulations are performed for the marine cold air outbreak cloud deck sampled during the Mixed-Phase Arctic Cloud Experiment (M-PACE) with the Icosahedral Nonhydrostatic (ICON) model. The impact of the droplet shattering (DS) of raindrops and collisional breakup (BR) in addition to the existing Hallet–Mossop rime splintering mechanism were investigated. Overall, 12 different model experiments (12-h runs) were performed and analyzed. Despite the considerable amount of uncertainty remaining with regard to SIP mechanisms and their process representation in numerical models, we conclude from these experiments that (i) only simulations where DS dominates the SIP signal (potentially amplified by BR) capture observed ice-phase and liquid-phase cloud properties, and (ii) SIP events cluster around the convective outflow region and are structurally linked to mesoscale cloud organization. In addition, interactions with primary nucleation parameterizations of varied complexity were investigated. Here, our simulations show that (i) a stable long-lived mixed-phase cloud (MPC) can be maintained in the absence of primary nucleation once SIP is established, (ii) experiments using a computationally more efficient relaxation-based parameterization of primary nucleation are statistically invariant from simulations considering prognostic INP, and (iii) primary nucleation at cloud-top controls the areal extent of the mixed-phase cloud region, and reduces SIP efficacy via DS due to increased depletion of cloud liquid throughout the entire cloud column.

54 ENVIRONMENTAL SCIENCES↗

On the engulfment of antifreeze proteins by ice

Antifreeze proteins (AFPs) are remarkable biomolecules that suppress ice formation at trace concentrations. To inhibit ice growth, AFPs must not only bind to ice crystals, but also resist engulfment by ice. The highest supercooling, ΔT*, for which AFPs are able to resist engulfment is widely believed to scale as the inverse of the separation, L, between bound AFPs, whereas its dependence on the molecular characteristics of the AFP remains poorly understood. By using specialized molecular simulations and interfacial thermodynamics, here, we show that in contrast with conventional wisdom, ΔT* scales as L –2 and not as L –1 . We further show that ΔT* is proportional to AFP size and that diverse naturally occurring AFPs are optimal at resisting engulfment by ice. By facilitating the development of AFP structure–function relationships, we hope that our findings will pave the way for the rational design of AFPs.

Science & Technology - Other Topics↗

A numerical study of thunderstorm electrification - Model development and case study

A numerical model was developed for examining the thunderstorm electrification process in which it is assumed that the electrification is entirely due to noninductive charge transfer between colliding ice crystals and hail. Since this ice-hail charge mechanism is very dependent on particle sizes and distributions, an explicit microphysical framework is used. To maintain simplicity, the electrification model is kinematic; thus the temperature and velocity fields are input into the electrification model. The cloud model of Taylor (1989) was used to generate the temperature and velocity fields to examine the July 19, 1981, Cooperative Convective Precipitation Experiment thundercloud. Using these fields, the electrification model produced time-dependent ice particle concentrations, radar reflectivities, charge, and vertical electric field distributions in good general agreement with those observed. The model produced a maximum electric field strength of 1.27 kV/cm, which is on the order of that needed for lightning initiation, and this maximum occurred very close to the time of the observed discharge. Thus, the ice-hail charge mechanism appears to have played an important role in the electrical development of the July 19 cloud.

Norville, K.↗

Examination of Icing Induced Loss of Control and Its Mitigations

Factors external to the aircraft are often a significant causal factor in loss of control (LOC) accidents. In today s aviation world, very few accidents stem from a single cause and typically have a number of causal factors that culminate in a LOC accident. Very often the "trigger" that initiates an accident sequence is an external environment factor. In a recent NASA statistical analysis of LOC accidents, aircraft icing was shown to be the most common external environmental LOC causal factor for scheduled operations. When investigating LOC accident or incidents aircraft icing causal factors can be categorized into groups of 1) in-flight encounter with super-cooled liquid water clouds, 2) take-off with ice contamination, or 3) in-flight encounter with high concentrations of ice crystals. As with other flight hazards, icing induced LOC accidents can be prevented through avoidance, detection, and recovery mitigations. For icing hazards, avoidance can take the form of avoiding flight into icing conditions or avoiding the hazard of icing by making the aircraft tolerant to icing conditions. Icing detection mitigations can take the form of detecting icing conditions or detecting early performance degradation caused by icing. Recovery from icing induced LOC requires flight crew or automated systems capable of accounting for reduced aircraft performance and degraded control authority during the recovery maneuvers. In this report we review the icing induced LOC accident mitigations defined in a recent LOC study and for each mitigation describe a research topic required to enable or strengthen the mitigation. Many of these research topics are already included in ongoing or planned NASA icing research activities or are being addressed by members of the icing research community. These research activities are described and the status of the ongoing or planned research to address the technology needs is discussed

Reehorst, Andrew L.↗

Influence of Ice Particle Surface Roughening on the Global Cloud Radiative Effect

Ice clouds influence the climate system by changing the radiation budget and large-scale circulation. Therefore, climate models need to have an accurate representation of ice clouds and their radiative effects. In this paper, new broadband parameterizations for ice cloud bulk scattering properties are developed for severely roughened ice particles. The parameterizations are based on a general habit mixture that includes nine habits (droxtals, hollow/solid columns, plates, solid/hollow bullet rosettes, aggregate of solid columns, and small/large aggregates of plates). The scattering properties for these individual habits incorporate recent advances in light-scattering computations. The influence of ice particle surface roughness on the ice cloud radiative effect is determined through simulations with the Fu-Liou and the GCM version of the Rapid Radiative Transfer Model (RRTMG) codes and the National Center for Atmospheric Research Community Atmosphere Model (CAM, version 5.1). The differences in shortwave (SW) and longwave (LW) radiative effect at both the top of the atmosphere and the surface are determined for smooth and severely roughened ice particles. While the influence of particle roughening on the single-scattering properties is negligible in the LW, the results indicate that ice crystal roughness can change the SW forcing locally by more than 10 W m(exp −2) over a range of effective diameters. The global-averaged SW cloud radiative effect due to ice particle surface roughness is estimated to be roughly 1-2 W m(exp −2). The CAM results indicate that ice particle roughening can result in a large regional SW radiative effect and a small but nonnegligible increase in the global LW cloud radiative effect.

clouds↗

Operational Detection of Sun Glints in DSCOVR EPIC Images

Satellite images often feature sun glints caused by the specular reflection of sunlight from water surfaces or from horizontally oriented ice crystals occurring in clouds. Such glints can prevent accurate retrievals of atmospheric and surface properties using existing algorithms, but the glints can also be used to infer more about the glint-causing objects—for example about the microphysical properties and radiative effects of ice clouds. This paper introduces the recently released operational glint product of the Earth Polychromatic Camera (EPIC) onboard the Deep Space Climate Observatory (DSCOVR) spacecraft. Most importantly, the paper describes the algorithm used for generating the key component of the new product: a glint mask indicating the presence of sun glint caused by the specular reflection of sunlight from ice clouds and smooth water surfaces. After describing the glint detection algorithm and glint product, the paper shows some examples of the detected glints and discusses some basic statistics of the glint population in a yearlong dataset of EPIC images. These statistics provide insights into the performance of glint detection and point toward possibilities for using the glint product to gain scientific insights about ice clouds and water surfaces.

DSCOVR↗

Deep Space Observations of Sun Glint from Oceans

Every hour or two, the Earth Polychromatic Imaging Camera (EPIC) onboard the DSCOVR satellite provides unique full-color images of the sunlit side of the Earth from the L1 Lagrangian point, which is four times farther the Moon. Casual glances at such images often reveal bright colorful spots that stand out markedly from their surroundings. Such spots often appear not only over ocean but also over land. Tracking the colorful spots using an automated image analysis algorithm reveals that they are caused by specular reflection of sunlight, sometimes from ocean surfaces and other times from clouds containing horizontally oriented ice crystals. The presented study characterizes these spots in terms of prevalence, location, color, and brightness, and provides insights into the factors that lead to their appearance.

ice crystals↗

Advancing the Understanding of Cloud Microphysical Processes and Aerosol Indirect Effects in High-Latitude Mixed-Phase Clouds by Linking ARM Measurements with Climate Model Simulations (Final Report)

The key objectives of this project were to advance our understanding of cloud microphysical characteristics and aerosol indirect effects on mixed-phase clouds in high latitudes. To improve the representation of ice and mixed-phase clouds in Earth System Models (ESMs), we propose an integrated observation and modeling study of cloud macro- and microphysical properties, including spatial heterogeneities, mass partitioning between ice crystals and supercooled liquid water, effects of ice nucleating particles (INPs), and efficiency of secondary ice production (SIP), etc. Specifically, we took four main approaches in this project: (1) examining macro- and microphysical properties of ice and mixed-phase clouds based on in-situ and ground-based observations from multiple field campaigns funded by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program, including the Mixed-Phase Arctic Cloud Experiment (M-PACE), Indirect and Semi-Direct Aerosol Campaign (ISDAC), Ice Nucleating Particle Sources at Oliktok Point (INPOP), ARM West Antarctic Radiation Experiment (AWARE), Measurements of Aerosols, Radiation, and Clouds over the Southern Ocean (MARCUS), and Macquarie Island Cloud and Radiation Experiment (MICRE); (2) evaluating the DOE Energy Exascale Earth System Model (E3SM) simulations based on observations, particularly for ice and mixed-phase cloud microphysical properties; (3) examining the impacts of INPs on ice and mixed-phase clouds. Specifically, a series of comparisons were conducted using observations over the Arctic, Southern Ocean, and Antarctica, including comparisons between the lower and higher southern latitudes as well as comparisons between the northern and southern hemispheres. In addition, aerosol indirect effects from distinct sources of dust particles were examined; and (4) investigating the impacts of SIP. Ultimately, these results helped to improve cloud microphysics and aerosol-cloud interaction parameterizations in the E3SM model. Overall, the project provided improved understanding regarding various factors, including thermodynamic, dynamic, and aerosol conditions, on the micro- and macrophysical properties of ice and mixed-phase clouds in the high latitudes. Resulting analysis helped to provide an improved physical basis for refining the current cloud microphysics parameterizations related to ice and mixed-phase clouds in E3SM.

54 ENVIRONMENTAL SCIENCES↗

Ice depolarization on low-angle 2 GHz satellite downlinks

The impact of ice depolarization on the statistical performance of satellite downlinks were investigated. Propagation data recorded during 1979 and 1980 to see what impact of ice depolarization on link performance were analyzed. The effects on the cross polarization discrimination (XPD) statistics amounted to at most a 2 to 4 dB reduction in the XPD values which rain would have produced for a given percentage of time. Ice depolarization had no effect on the statistics of XPD values below the 0.01% level. Most of the severe ice depolarization events were associated with drops in barometric pressure and the passage of intense cold fronts through our area. Ice contents as the product of three individually undetermined quantities were defined: ice particle density, ice cloud thickness, and the average volume of the ice crystals. It is indicated that populations of ice particle with ice contents on the order of 0.002 m4/m3 are probably responsible for the lower values of measured XPD.

Stutzman, W. L.↗

Analysis of Hot-Wire Probe Ice Water Content Measurements in High Ice Water Content Conditions

During the 2022 High Ice Water Content (HIWC) Flight Campaign, ice water content (IWC) measurements were made at various locations on the NASA DC-8 Airborne Science Laboratory using the Isokinetic Probe Version 2 (IKP2), Ice Crystal Detectors (ICD), and Robust Probe. Correlations of a wing mounted ICD to IKP2 were made to determine the collision/retention efficiency of the ICD total water content (TWC) element in glaciated conditions. Similarly, correlations of a nose mounted ICD near the pitot probes were made to the IKP2 and to the wing-mounted ICD to estimate the ice concentration factor near the DC-8 pitot probes. Results from the 2022 flight campaign were compared to results from the HIWC RADAR II flight campaign in 2018. There was an apparent reduction in the ICD TWC collision/retention efficiency during the 2022 flight campaign. Although reasons for this discrepancy were explored, more analyses are needed to fully understand the causes. However, it was concluded that an estimated ice concentration factor at the nose of 2.5 was consistent between the two flight campaigns. Additionally, a correlation model was developed to relate measurements from a Nose ICD to freestream IWC as measured by the IKP2 to support IWC measurements from the 2022 Convective Processes Experiment - Cabo Verde (CPEX-CV) flight campaign.

Icing↗

Analysis of Hot-Wire Probe Ice Water Content Measurements in High Ice Water Content Conditions

During the 2022 High Ice Water Content (HIWC) Flight Campaign, ice water content (IWC) measurements were made at various locations on the NASA DC-8 Airborne Science Laboratory using the Isokinetic Probe Version 2 (IKP2), Ice Crystal Detectors (ICD), and Robust Probe. Correlations of a wing mounted ICD to IKP2 were made to determine the collision/retention efficiency of the ICD total water content (TWC) element in glaciated conditions. Similarly, correlations of a nose mounted ICD near the pitot probes were made to the IKP2 and to the wing-mounted ICD to estimate the ice concentration factor near the DC-8 pitot probes. Results from the 2022 flight campaign were compared to results from the HIWC RADAR II flight campaign in 2018. There was an apparent reduction in the ICD TWC collision/retention efficiency during the 2022 flight campaign. Although reasons for this discrepancy were explored, more analyses are needed to fully understand the causes. However, it was concluded that an estimated ice concentration factor at the nose of 2.5 was consistent between the two flight campaigns. Additionally, a correlation model was developed to relate measurements from a Nose ICD to freestream IWC as measured by the IKP2 to support IWC measurements from the 2022 Convective Processes Experiment - Cabo Verde (CPEX-CV) flight campaign.

Icing↗

Elucidating Processes Controlling Arctic Atmospheric Aerosol Sources, Aging, and Mixing States (Final Report)

Atmospheric aerosols play critical roles in the Earth’s energy budget, directly by scattering or absorbing solar and terrestrial radiation and indirectly by serving as seeds (nuclei) for cloud droplet and ice crystal formation and by depositing on snow and ice surface, thereby changing the surface albedo. These effects are dependent on aerosol particle size and chemical composition and impact the hydrological cycle as well. This project provided single-particle size and chemical composition measurements across the entire annual cycle in the high Arctic and in the Alaskan Arctic during fall – winter, addressing the most significant gaps in Arctic aerosol observational data. These needs were based on recent rapid sea ice loss across the entire Arctic, as well as the major annual delays in sea ice freeze-up during fall in the Chukchi Sea and increased wintertime sea ice fracturing in the Beaufort Sea, both off the North Slope of Alaska. Two DOE Atmospheric Radiation Measurement (ARM) field campaigns were conducted for atmospheric aerosol sampling. The Aerosols during the Polar Utqiagvik Night (APUN – ‘snow on ground’ in Iñupiaq) ARM field campaign at Utqagivik, Alaska was conducted from Oct. 28 – Dec. 22, 2018. Aerosol sizing instrumentation and a single-particle mass spectrometer were successfully deployed for size-resolved number concentration measurements and measurements of individual particle size and chemical composition, respectively. These results show the influence of locally-produced sea spray aerosol, with high cloud-forming potential, due to delayed sea ice freeze-up in the fall. During the 2019‐2020 international Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition, daily atmospheric aerosol particles were collected aboard the German icebreaker Polarstern in the Central Arctic from Nov. 2019 – Oct. 2020. Sea salt aerosol and marine organics were observed year-round during MOSAiC with varying morphologies and sources. These findings are important because most Arctic models do not include a sea spray aerosol source, despite this source increasing with declining sea ice extent. In addition to collecting new samples and data, this project also conducted further analysis of previously collected single-particle chemical composition measurements within the North Slope of Alaska oil fields and at Utqiaġvik, AK, during Aug. – Sep. 2015 and 2016 field campaigns. This work resulted in the discovery of chemical reactions of oil field combustion emissions occurring within fog droplets across the North Slope of Alaska and forming secondary aerosol, showing the impact of Arctic oil field emissions beyond black carbon aerosol and greenhouse gases. In addition, the distribution of chemical species across the aerosol population within the oil fields was quantified, using these data and a previously development framework. We also presented the first ambient evidence of the collision of two atmospheric particles resulting in formation of an organic-coated ammonium sulfate particle of marine origin, which has implications for cloud formation with declining sea ice extent. Overall, this project has elucidated connections between seawater biogeochemistry, resource extraction activities, atmospheric composition, clouds, and the energy budget of the Arctic region. The results of this project are expected to improve weather and sea ice forecasting for security and development in the Arctic and beyond.

54 ENVIRONMENTAL SCIENCES↗

Highly supercooled riming and unusual triple-frequency radar signatures over McMurdo Station, Antarctica

Abstract. Riming of ice crystals by supercooled water droplets is an efficient ice growth process, but its basic properties are still poorly known. While it has been shown to contribute significantly to surface precipitation at mid-latitudes, little is known about its occurrence at high latitudes. In Antarctica, two competing effects can influence the occurrence of riming: (i) the scarcity of supercooled liquid water clouds due to the extremely low tropospheric temperatures and (ii) the low aerosol concentration, which may lead to the formation of fewer and larger supercooled drops potentially resulting in an enhanced riming efficiency. In this work, by exploiting the deployment of an unprecedented number of multiwavelength remote sensing systems (including triple-frequency radar measurements) in West Antarctica, during the Atmospheric Radiation Measurements West Antarctic Radiation Experiment (AWARE) field campaign, we evaluate the riming incidence at McMurdo Station and find that riming occurs at much lower temperatures when compared to previous results in the mid-latitudes. This suggests the possible occurrence of a common atmospheric state over Antarctica that includes a rather stable atmosphere inhibiting turbulent mixing, and a high riming efficiency driven by large cloud droplets. We then focus on a peculiar case study featuring a persistent layer with a particularly pronounced riming signature in triple-frequency radar data but only a relatively modest amount of supercooled liquid water. In-depth analysis of the radar observations suggests that such signatures can only be explained by the combined effects of moderately rimed aggregates or similarly shaped florid polycrystals and a narrow particle size distribution (PSD). Simulations of this case study performed with a one-dimensional bin model indicate that similar triple-frequency radar observations can be reproduced when narrow PSDs are simulated. Such narrow PSDs can in turn be explained by two key factors: (i) the presence of a shallow homogeneous droplet or humidified aerosol freezing layer aloft seeding an underlying supercooled liquid layer, and (ii) the absence of turbulent mixing throughout a stable polar atmosphere that sustains narrow PSDs, as hydrometeors grow from the nucleation region aloft to ice particles of several millimeters in size, by vapor deposition and then riming.

54 ENVIRONMENTAL SCIENCES↗