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Scintillator array for radiation detection

A radiation detector includes a photodetector and a scintillator coupled thereto. The scintillator is formed of a scintillator material comprising an organic glass scintillator (OGS) material and at least one of a polymer additive or a plasticizer additive. The scintillator emits light when radiation is received at the scintillator, and the light is received by the photodetector. The radiation detector can further include a frame that has an interior cavity that holds the scintillator in position with respect to the photodetector, such that the light emitted by the scintillator is transmitted to the photodetector. The scintillator can be formed by casting amorphous scintillator material in the interior cavity of the frame. The frame can then be coupled to the photodetector to form the radiation detector.

Carlson, Joseph↗

SU-F-T-264: VMAT QA with 2D Radiation Measuring Equipment Attached to Gantry

Purpose: To introduce a method of VMAT QA by 2D measuring device. The 2D device is attached to the gantry throughout measurement duration. This eliminates error caused by the angular dependence of the radiation detectors. Methods: A 2D radiation measuring device was attached to the gantry of linear accelerator. The center of the detector plane was at the isocenter. For each patient plan, two verification plans were created for QA purpose. One was like an ordinary VMAT plan, to be used for radiation delivery. The other is a plan with gantry angle fixed at zero, so the dose distribution as seen by the rotating 2D device. Points above 10% dose threshold were analyzed. Data is in tolerance if it fits within the 3 mm or 3% dose gamma criteria. For each patient, the plan was passed when 95% of all the points in the 2D matrix fit the gamma criteria. The following statistics were calculated: number of patient plans passed, percentage of all points passed, average percentage difference of all points. Results: VMAT QA was performed for patients during one year in our department, and the results were analyzed. All irradiation was with 6 MV photon beam. Each plan has calculated and measured doses compared. After collecting one year’s result, with 81 patient plans analyzed, all (100%) of the plans passed the gamma criteria. Of the points analyzed from all plans, 98.8% of all points passed. Conclusion: This method of attaching a 2D measuring device on the linac gantry proves to be an accurate way for VMAT QA. It is simple to use and low cost, and it eliminates the problem of directional dependence.

60 APPLIED LIFE SCIENCES↗

Coupled Gel/Seeded Growth of Cs2AgBiBr6 Single Crystals for Radiation Detection

Abstract— The all-inorganic lead free Cs2AgBiBr6 perovskite represents a highly promising environment-friendly radiation detector material. The first attempt to grow Cs2AgBiBr6 single crystals using the unique gel growth method is reported in this study. This technique enables controlled reagent diffusion in a gel medium at room temperature, fostering the growth of visible single crystals. It offers advantages over conventional methods, leading to fewer equilibrium and non-equilibrium defects and simplified execution. Interestingly, the as-grown crystals exhibited variations in size and colors within the gel matrix, indicating the influence of Bi solutes in Bi-poor and Bi-rich Cs2AgBiBr6 crystals. Once the crystals were confirmed by powder xray diffraction, a series of comprehensive material characterizations was performed. The resistivity of Cs2AgBiBr6 single crystals was measured at 1.12x107 Ω•cm. Trap density analysis yielded a value of 2.82 x1010 cm-3. The charge carrier mobility was determined to be 32.9 cm2V-1S-1, suggesting the suitability for radiation detector applications. Additional growth optimization is going on and further characterization will be reported during the presentation. Our work helps accelerate the development of lead-free perovskite materials toward radiation detector applications.

James, Ralph B.↗

An Experimental Feasibility Study on Applying Neutron Tomography to Encapsulated Spent Nuclear Fuel - 20050

Visual inspection makes easier to ensure the integrity and safety of spent nuclear fuel (SNF) than any classical techniques. Various classical techniques have been applied but there are no reliable methods to qualitatively and quantitatively verify spent fuel in dry storage. Thus, the present authors have developed the prototype safeguards apparatus for dry storage employing the array of He-4 gas scintillation detectors (S670E, Arktis Radiation Detectors Ltd., Switzerland), newly designed to simultaneously measure thermal and fast neutrons without any moderators. The S670E detector has a cylindrical shape with a diameter of 52 mm and active length of 600 mm (total length: 875 mm). The detector is filled by He-4 gas with an approximate pressure of 180 bar for fast neutron detection, and its inner wall is coated by Li-6 for thermal neutron detection. The scintillation lights generated via Li-6 nuclear reaction and elastic scattering are collected by 24 SiPMs linearly paired at the center of the detector. The detector delivers a TTL (Transistor-Transistor Logic) output for pulse readout and UART (Universal Asynchronous Receiver Transmitter) for device control. In order to assess feasibility of the apparatus, an experimental system has been designed, built, and optimized via computational studies. Cf-252 neutron sources and linearly arrayed detectors, working as a single detector, were occupied for this study due to the difficulties in working with SNF. The laboratory scale cask (diameter: 0.67 m, height: 1.5 m), minimized by a factor of 10 compared to the actual thickness of a commercial TN-32 cask, was also manufactured. The detector array was designed to rotate the lab-scale cask and obtain 36 image profiles at every 10 degrees. All profiles were aligned in single frame image called a sinogram, and the cross-sectional image was then fabricated by the inverse radon transform algorithm. These experiments have been repeated with different configurations and numbers of sources. Some gamma-ray sources were also measured with neutron sources in order to distinguish between neutron and gamma-ray pulses. Basically, a He-4 detector is designed to run on Linux OS so it is difficult to directly apply to Windows-based equipment widely used in S. Korea. Therefore, a new data acquisition board working on Windows OS was designed and built. The board mainly consists of FPGA (Field Programmable Gate Array) and SoC (System on Chip) for TTL pulse readout, sorting measured data, and transferring data to a user interface. In conclusion, the tomographic system at lab-scale has shown considerable potential to detect a partial or gross defect of encapsulated assemblies in dry storage. Next steps of this study will be to 1) repeatedly carry out experiments to demonstrate scientific reliability and validity, and 2) numerically integrate signals with weight factors to enhance the image quality since the suggested system based on passive interrogation method requires longer measurement time. Finally, the system will apply to a commercial dry storage phased out soon in S. Korea. (authors)

07 ISOTOPE AND RADIATION SOURCES↗

Radiography by selective detection of scatter field velocity components

A reconfigurable collimated radiation detector, system and related method includes at least one collimated radiation detector. The detector has an adjustable collimator assembly including at least one feature, such as a fin, optically coupled thereto. Adjustments to the adjustable collimator selects particular directions of travel of scattered radiation emitted from an irradiated object which reach the detector. The collimated detector is preferably a collimated detector array, where the collimators are independently adjustable. The independent motion capability provides the capability to focus the image by selection of the desired scatter field components. When an array of reconfigurable collimated detectors is provided, separate image data can be obtained from each of the detectors and the respective images cross-correlated and combined to form an enhanced image.

Jacobs, Alan M.↗

Low-cost, multi-mode detector solutions

Low-cost radiation detectors capable of providing efficient gamma-ray and neutron detection are essential in passive nuclear monitoring systems such as radiation portal monitors (RPMs) and detection of Special Nuclear Materials (SNM) through Active Interrogation (AI). Here, three low-cost detector solutions are discussed—(1) Large-area polystyrene-based plastic scintillators for AI (2) Pulse Shape Discrimination (PSD) capable plastic scintillators doped with heavy-metals for imparting gamma-ray spectroscopy (3) Composite detector technology based on inorganic scintillator submerged into the plastic scintillator, for detection of thermal and fast neutrons in addition to gamma-ray spectroscopy. Composite detectors using inorganic component such as Cs 2 LiYCl 6 (CLYC), Cs 2 LiLaBr x Cl 6-x (CLLBC), or CsI:Tl have been developed up to 4” sizes. Neutron and gamma efficiencies are compared for samples with different inorganic loading.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

RadSim: Math, Utility & RTK

This package includes three parts, (1) gov.llnl.math, (2)gov.llnl.utility and (3)gov.llnl.rtk, which are utilized in the development of Radiation Detector Simulator (RadSim) project. RadSim is being developed to provide the capability to: (1) simulate radiation source emissions, (2) interpolate results from radiation transport tools into a common format to prepare incident flux, and (3) model radiation detector response to rapidly produce synthetic radiation measurement templates. RadSim is targeted for open-source release, which will enable researchers and industry partners to model gamma-ray detectors response to simulated flux from the transport tool of their choice. The techniques and implementation will be entirely transparent, which will allow for improvements and boutique modifications by future researchers beyond the lifespan of this specific project. The first tool of the package, gov.llnl.math, includes classes and functions to define and perform basic math operations. Some of the example features available in the package include defining statistical distributions and performing algebra and matrix operations, all of which are already accessible on publicly available software packages such as MATLAB and ROOT. The second package gov.llnl.utility includes tools commonly used to enable optimization and readability of various data structures such as Java lists and external xml files. Lastly, the gov.llnl.rtk package includes classes and functions to implement methods commonly used in radiation physics, such as data structures to represent and characterize photon spectra and tools to apply well-defined and published methods to calibrate a given spectra.

Cheung, Hoi Sing↗

Fabrication and testing of antimony doped bismuth tri-iodide semiconductor gamma-ray detectors

We fabricated antimony (Sb) doped bismuth tri-iodide (BiI 3 ) radiation detectors from large single crystals that were grown using the modified vertical Bridgman technique. Detectors were prepared by subjecting the crystal surfaces to different mechanical and chemical treatments. Surface quality of the detectors was evaluated using optical microscopy. The influence of surface quality on detector performance was analyzed by measuring the leakage current for each of the detectors. The radiation response of the detectors was measured using an Americium ( 241 Am) gamma-ray source at room temperature. The first successful use of BiI 3 detectors for gamma-ray spectroscopy is reported here with energy resolution of 7.5% at 59.5 keV. The mobility-lifetime product for electrons was also estimated to be about 5.2 x 10 -4 cm 2 /V.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

RadSim: ENSDF, Xray and N42

This package includes three parts, (1) gov.bnl.nndc.ensdf, (2) gov.nist.xray and (3) gov.nist.physics.n42, which are utilized in the development of Radiation Detector Simulator (RadSim) project. RadSim is being developed to provide the capability to: (1) simulate radiation source emissions, (2) interpolate results from radiation transport tools into a common format to prepare incident flux, and (3) model radiation detector response to rapidly produce synthetic radiation measurement templates. RadSim is targeted for open-source release, which will enable researchers and industry partners to model gamma-ray detectors response to simulated flux from the transport tool of their choice. The first tool of the package, gov.bnl.nndc.ensdf, includes functionality to parse and split publicly available decay records in ENSDF format, and pull the relevant information from ENSDF libraries. The second tool, gov.nist.xray, provides Xray information using the public NIST database. Lastly, gov.nist.physics.n42, is a tool used to convert an N42 xml file into a Java object that can be interfaced within a Java program.

Hangal, DnaushA↗

Portal Monitoring Considerations for Treaty Verification Applications

Portal monitoring is one method in a suite of options for treaty verification and can assist in verification of treaty accountable items (TAIs). Portal monitor technology spans a wide range of sensors, including radiation detectors, break-beams, or weight sensors. For radiation-detecting portal monitors, they are able to confirm absence / presence of a radiological signature and to track TAI direction of motion. Portal monitoring uses measurements from strategically placed sensors (e.g., radiation detectors) to record the entry or egress of TAIs. The implementation of portal monitoring relies on three key elements: perimeter definition, portal locations, and sensor technology, and can be implemented in either time-bound or continuous operations depending on what is permitted by the Treaty.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Counts in the ORTEC Detective X neutron channel

The ORTEC Detective X is a new radiation detector being produced and sold by AMTEK ORTEC. The main detector (for gamma radiation energy) is a High Purity Germanium (HPGe) crystal. A Geiger-Müller (GM) tube is used for radiation exposure measurements above about 2 mR/hr. As an available option, a Li6 F/ZnS neutron detector module can be attached to the Detective X to measure neutrons.

61 RADIATION PROTECTION AND DOSIMETRY↗

Method for detecting and distinguishing between specific types of environmental radiation using a high pressure ionization chamber with pulse-mode readout

An environmental radiation detector for detecting and distinguishing between all types of environmental radiation, including photons, charged particles, and neutrons. A large volume high pressure ionization chamber (HPIC) includes BF.sub.3 gas at a specific concentration to render the radiation detector sensitive to the reactions of neutron capture in Boron-10 isotope. A pulse-mode readout is connected to the ionization chamber capable of measuring both the height and the width of the pulse. The heavy charged products of the neutron capture reaction deposit significant characteristic energy of the reaction in the immediate vicinity of the reaction in the gas, producing a signal with a pulse height proportional to the reaction energy, and a narrow pulse width corresponding to the essentially pointlike energy deposition in the gas. Readout of the pulse height and the pulse width parameters of the signals enables distinguishing between the different types of environmental radiation, such as gamma (x-rays), cosmic muons, and neutrons.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The 88-Inch Cyclotron: A One-Stop Facility for Electronics Radiation and Detector Testing

In outer space down to the altitudes routinely flown by larger aircrafts, radiation can pose serious issues for microelectronics circuits. The 88-Inch Cyclotron at Lawrence Berkeley National Laboratory is a sector-focused cyclotron and home of the Berkeley Accelerator Space Effects Facility, where the effects of energetic particles on sensitive microelectronics are studied with the goal of designing electronic systems for the space community. This paper describes the flexibility of the facility and its capabilities for testing the bombardment of electronics by heavy ions, light ions, and neutrons. Experimental capabilities for the generation of neutron beams from deuteron breakups and radiation testing of carbon nanotube field effect transistor will be discussed.

43 PARTICLE ACCELERATORS↗

SU-E-T-299: Small Fields Profiles Correction Through Detectors Spatial Response Functions and Field Size Dependence Analysis

Purpose: To calculate the spatial response function of various radiation detectors, to evaluate the dependence on the field size and to analyze the small fields profiles corrections by deconvolution techniques. Methods: Crossline profiles were measured on a Novalis Tx 6MV beam with a HDMLC. The configuration setup was SSD=100cm and depth=5cm. Five fields were studied (200×200mm2,100×100mm2, 20×20mm2, 10×10mm2and 5×5mm2) and measured were made with passive detectors (EBT3 radiochromic films and TLD700 thermoluminescent detectors), ionization chambers (PTW30013, PTW31003, CC04 and PTW31016) and diodes (PTW60012 and IBA SFD). The results of passive detectors were adopted as the actual beam profile. To calculate the detectors kernels, modeled by Gaussian functions, an iterative process based on a least squares criterion was used. The deconvolutions of the measured profiles were calculated with the Richardson-Lucy method. Results: The profiles of the passive detectors corresponded with a difference in the penumbra less than 0.1mm. Both diodes resolve the profiles with an overestimation of the penumbra smaller than 0.2mm. For the other detectors, response functions were calculated and resulted in Gaussian functions with a standard deviation approximate to the radius of the detector in study (with a variation less than 3%). The corrected profiles resolve the penumbra with less than 1% error. Major discrepancies were observed for cases in extreme conditions (PTW31003 and 5×5mm2 field size). Conclusion: This work concludes that the response function of a radiation detector is independent on the field size, even for small radiation beams. The profiles correction, using deconvolution techniques and response functions of standard deviation equal to the radius of the detector, gives penumbra values with less than 1% difference to the real profile. The implementation of this technique allows estimating the real profile, freeing from the effects of the detector used for the acquisition.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Novel ZnO:Al contacts to CdZnTe for X- and gamma-ray detectors

CdZnTe (CZT) has made a significant impact as a material for room-temperature nuclear-radiation detectors due to its potential impact in applications related to nonproliferation, homeland security, medical imaging and gamma-ray telescopes. In all such applications, common metals, such as gold, platinum and indium, have been used as electrodes for fabricating the detectors. Because of the large mismatch in the thermal-expansion coefficient between the metal contacts and CZT, the contacts can undergo stress and mechanical degradation, which is the main cause for device instability over the long term. Here, we report for the first time on our use of Al-doped ZnO as the preferred electrode for such detectors. The material was selected because of its better contact properties compared to those of the metals commonly used today. Comparisons were conducted for the detector properties using different contacts and improvements in the performances of ZnO:Al-coated detectors are described in this paper. These studies show that Al:ZnO contacts to CZT radiation detectors offer the potential of becoming a transformative replacement for the common metallic contacts due to the dramatic improvements in the performance of detectors and improved long-term stability.

47 OTHER INSTRUMENTATION↗

Trapped radiation belts of Saturn - First look

Data on the magnetosphere of Saturn obtained with the trapped radiation detector package on board the Pioneer 11 spacecraft is reported. Radiation belt profiles determined by the trapped radiation detectors on Pioneer 10 and 11 indicate that Saturn's magnetosphere is intermediate in size between those of the earth and Jupiter, with particle intensities similar to those of the earth. The outer region of the Saturn magnetosphere is found to contain particles of lower energy than the outer region, being strongly influenced by the time-varying solar wind. The moons and rings of Saturn are observed to be effective absorbers of trapped particles, confirming the discoveries of the F ring, the Pioneer ring division and the moon 1979 S 2. Particle diffusion rates are used to estimate a cross-sectional area of greater than 7 x 10 to the 13th sq cm and an opacity greater than 0.00001 for the F ring. It is suggested that cosmic-ray albedo neutron decay be studied as a possible source of energetic particles in the inner magnetosphere of Saturn.

Fillius, W.↗

Additive Manufacturing Materials Study for Gaseous Radiation Detection

Additive manufacturing (AM) techniques may lead to improvements in many areas of radiation detector construction; notably the rapid manufacturing time allows for a reduced time between prototype iterations. The additive nature of the technique results in a granular microstructure which may be permeable to ingress by atmospheric gases and make it unsuitable for gaseous radiation detector development. In this study we consider the application of AM to the construction of enclosures and frames for wire-based gaseous radiation tracking detectors. We have focussed on oxygen impurity ingress as a measure of the permeability of the enclosure, and the gas charging and discharging curves of several simplistic enclosure shapes are reported. A prototype wire-frame is also presented to examine structural strength and positional accuracy of an AM produced frame. We lastly discuss the implications of this study for AM based radiation detection technology as a diagnostic tool for incident response scenarios, such as the interrogation of a suspect radiation-emitting package. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗