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At least 379 records · Page 21

Radiations from hot nuclei

The investigation indicates that nuclei with excitation energy of a few hundred MeV to BeV are more likely to radiate hot nuclear clusters than neutrons. These daughter clusters could, furthermore, de-excite emitting other hot nuclei, and the chain continues until these nuclei cool off sufficiently to evaporate primarily neutrons. A few GeV excited nuclei could radiate elementary particles preferentially over neutrons. Impact of space radiation with materials (for example, spacecraft) produces highly excited nuclei which cool down emitting electromagnetic and particle radiations. At a few MeV excitation energy, neutron emission becomes more dominant than gamma-ray emission and one often attributes the cooling to take place by successive neutron decay. However, a recent experiment studying the cooling process of 396 MeV excited Hg-190 casts some doubt on this thinking, and the purpose of this investigation is to explore the possibility of other types of nuclear emission which might out-compete with neutron evaporation.

Malik, F. Bary↗

Four-decade follow-up of a plutonium-contaminated puncture wound treated with Ca-DTPA

Contaminated wounds are a common route of internal deposition of radionuclides for nuclear and radiation workers. They may result in significant doses to radiosensitive organs and tissues in an exposed individual's body. The United States Transuranium and Uranium Registries' whole-body donor (Case 0303) accidentally punctured his finger on equipment contaminated with plutonium nitrate. The wound was surgically excised and medically treated with intravenous injections of Ca-DTPA. A total of 16 g Ca-DTPA was administered in 18 treatments during the 2 months following the accident. Ninety-three urine samples were collected and analysed over 14 years following the accident. An estimated 239 Pu activity of 73.7 Bq was excreted during Ca-DTPA treatment. Post-mortem radiochemical analysis of autopsy tissues indicated that 40 years post-accident 21.6 ± 0.2 Bq of 239 Pu was retained in the skeleton, 12.2 ± 0.3 Bq in the liver, and 3.7 ± 0.1 Bq in other soft tissues; 1.35 ± 0.02 Bq of 239 Pu was measured in tissue samples from the wound site. To estimate the plutonium intake, late urine measurements, which were unaffected by chelation, and post-mortem radiochemical analysis results were evaluated using the IMBA Professional Plus software. The application of the National Council on Radiation Protection and Measurements wound model with an assumption of intake material as a predominantly strongly retained soluble plutonium compound with a small insoluble fraction adequately described the data (p = 0.46). The effective intake was estimated to be 50.2 Bq of plutonium nitrate and 1.5 Bq of the fragment. Here, the prompt medical intervention with contaminated tissue excision and subsequent Ca-DTPA decorporation therapy reduced 239 Pu activity available for uptake and long-term retention in this individual's systemic organs by a factor of 38.

239Pu↗

Investigation of gaseous nuclear rocket technology

The experimental and theoretical investigations conducted during the period from September 1969 through September 1972 are reported which were directed toward obtaining information necessary to determine the feasibility of the full-scale nuclear light bulb engine, and of small-scale nuclear tests involving fissioning uranium plasmas in a unit cell installed in a driver reactor, such as the Nuclear Furnace. Emphasis was placed on development of RF simulations of conditions expected in nuclear tests in the Nuclear Furnace. The work included investigations of the following: (1) the fluid mechanics and containment characteristics of one-component and two-component vortex flows, both unheated and RF-induction heated; (2) heating of particle-seeded streams by thermal radiation from a dc arc to simulate propellant heating; (3) condensation and separation phenomena for metal-vapor/heated-gas mixtures to provide information for conceptual designs of components of fuel exhaust and recycle systems; (4) the characteristics of the radiant energy spectrum emitted from the fuel region, with emphasis on definition of fuel and buffer-gas region seed systems to reduce the ultraviolet radiation emitted from the nuclear fuel; and (5) the effects of nuclear radiation on the optical transmission characteristics of transparent materials.

Kendall, J. S.↗

Radiative transfer in cometary dust atmospheres: Critique of recent developments

The gas and dust production rates of comets near the sun are intimately linked to the fate of the solar radiation as it is scattered and partially absorbed by the cometary dust envelope or halo surrounding the comet's nucleus. The radiation of nuclear matter (mostly water ice) and the release of dust particles embedded in the ice which are entrained by the escaping gas and subsequently form a dust atmosphere or halo. On the other hand, the interaction of the dust cloud with the solar radiation is in turn responsible for the amount of radiative energy received by the nucleus and thus determines the evaporation rate. It is shown that recent attempts to formulate this problem quantitatively are in error. The correct formulation is given and it is pointed out that negative extinction (enhancement of the primary radiation received by the nucleus due to multiple scattering) may not be as large as predicted.

Vonroos, O.↗

Nuclear emulsion measurements of the astronauts' radiation exposure on the Apollo-Soyuz mission

On the Apollo-Soyuz mission each astronaut carried one passive dosimeter containing nuclear photographic emulsions, plastic foils, TLD chips, and neutron-activation foils for recording radiation exposure. This report is limited to the presentation of data retrieved from nuclear emulsions. Protons, most of them trapped particles encountered in numerous passes through the South Atlantic Anomaly, contributed by far the largest share to the mission dose. Their linear energy transfer (LET) spectrum was established from track and grain counts in a G.5 emulsion which is used for medium and high energies, and from ender counts in a K.2 emulsion which is used for low energies. The total mission fluence of protons was found to be equivalent to a unidirectional beam of 448,500 square centimeters. The broad spectrum was broken down into small LET intervals, which allowed for the computation of absorbed doses and dose equivalents. The totals are 51 millirad and 74 millirem. Counts of disintegration stars in K.2 emulsion are incomplete at present. While a total of 467 stars were identified, counting their prong numbers is still in progress. It was concluded that the Apollo-Soyuz astronauts' radiation exposure as such did not contain anything out of the ordinary that would seem to require special attention.

Schaefer, H. J.↗

Radiation Effects in Concrete for Nuclear Systems

Concrete is massively used in the construction of critical safety-related components in nuclear power plants. Among those, the concrete biological shield is exposed to high levels of neutron and gamma irradiation exiting the reactor pressure vessel. This article provides a comprehensive overview of the state-of-the-art knowledge on irradiated concrete. First, the fundamental irradiation-induced degradation mechanisms occurring at the level of the concrete constituents such as rock-forming minerals and hydrated cementitious phases are examined. The critical role of the mineralogical and chemical composition regarding concrete resistance against radiation effects such as amorphization, irradiation-induced expansion and radiolytic gas release are detailed. Second, the interactions between the varied irradiated phases are comprehensively analyzed and put in perspectives with the effects of prolonged irradiation on the structural properties of concrete aggregates, cement paste, and concretes. Finally, the significance of irradiation for the long-term operation of nuclear power plants is discussed in the light of the most recent knowledge and its limitations.

Le Pape, Yann↗

Measuring Very Low Radiation Doses in PTFE for Nuclear Forensic Enrichment Reconstruction

Every country that has made nuclear weapons has used uranium enrichment. Despite the centrality of this technology to international security, there is still no reliable physical marker of past enrichment that can be used to perform forensic verification of historically produced weapons. We show that the extremely low radioactivity from uranium alpha emissions during enrichment leaves detectable and irreversible calorimetric signatures in the common enrichment gasket material PTFE, allowing for historical reconstruction of past enrichment activities at a sensitivity better than one weapon's quantity of highly enriched uranium. Fast scanning calorimetry also enables the measurement of recrystallization enthalpies of sequentially microtomed slices, confirming the magnitude and the type of radiation exposure while also providing a detection of tampering and a method for analyzing field samples useful for treaty verification. This work opens the door for common items to be turned into precise dosimeters to detect the past presence of radioactivity, nuclear materials, and related activities with high confidence.

Connick, Rachel↗

Closed-Cycle Engine Program Used to Study Brayton Power Conversion

One form of power conversion under consideration in NASA Glenn Research Center's Thermal Energy Conversion Branch is the closed-Brayton-cycle engine. In the tens-of-kilowatts to multimegawatt class, the Brayton engine lends itself to potential space nuclear power applications such as electric propulsion or surface power. The Thermal Energy Conversion Branch has most recently concentrated its Brayton studies on electric propulsion for Prometheus. One piece of software used for evaluating such designs over a limited tradeoff space has been the Closed Cycle Engine Program (CCEP). The CCEP originated in the mid-1980s from a Fortran aircraft engine code known as the Navy/NASA Engine Program (NNEP). Components such as a solar collector, heat exchangers, ducting, a pumped-loop radiator, a nuclear heat source, and radial turbomachinery were added to NNEP, transforming it into a high-fidelity design and performance tool for closed-Brayton-cycle power conversion and heat rejection. CCEP was used in the 1990s in conjunction with the Solar Dynamic Ground Test Demonstration conducted at Glenn. Over the past year, updates were made to CCEP to adapt it for an electric propulsion application. The pumped-loop radiator coolant can now be n-heptane, water, or sodium-potassium (NaK); liquid-metal pump design tables were added to accommodate the NaK fluid. For the reactor and shield, a user can now elect to calculate a higher fidelity mass estimate. In addition, helium-xenon working-fluid properties were recalculated and updated.

Johnson, Paul K.↗

Texturing Carbon-carbon Composite Radiator Surfaces Utilizing Atomic Oxygen

Future space nuclear power systems will require radiator technology to dissipate excess heat created by a nuclear reactor. Large radiator fins with circulating coolant are in development for this purpose and an investigation of how to make them most efficient is underway. Maximizing the surface area while minimizing the mass of such radiator fins is critical for obtaining the highest efficiency in dissipating heat. Processes to develop surface roughness are under investigation to maximize the effective surface area of a radiator fin. Surface roughness is created through several methods including oxidation and texturing. The effects of atomic oxygen impingement on carbon-carbon surfaces are currently being investigated for texturing a radiator surface. Early studies of atomic oxygen impingement in low Earth orbit indicate significant texturing due to ram atomic oxygen. The surface morphology of the affected surfaces shows many microscopic cones and valleys which have been experimentally shown to increase radiation emittance. Further study of this morphology proceeded in the Long Duration Exposure Facility (LDEF). Atomic oxygen experiments on the LDEF successfully duplicated the results obtained from materials in spaceflight by subjecting samples to 4.5 eV atomic oxygen from a fixed ram angle. These experiments replicated the conical valley morphology that was seen on samples subjected to low Earth orbit.

Raack, Taylor↗

Measuring very low radiation doses in PTFE for nuclear forensic enrichment reconstruction

Every country that has made nuclear weapons has used uranium enrichment to do so. Despite the centrality of this technology to international security, there is still no reliable physical marker of past enrichment in the open literature that can be used to perform forensic verification of historically produced weapons on gas centrifuges. We show that the extremely low radioactivity from uranium alpha emissions during enrichment leaves detectable and irreversible calorimetric signatures in the common enrichment gasket material PTFE, allowing for historical reconstruction of past enrichment activities at a sensitivity better than one weapon’s quantity of highly enriched uranium. Fast scanning calorimetry also enables the measurement of recrystallization enthalpies of sequentially microtomed slices, confirming the magnitude and the type of radiation exposure while also providing detection of tampering and a method for analyzing field samples useful for treaty verification. Furthermore, this work opens the door for common items to be turned into precise dosimeters to detect the past presence of radioactivity, nuclear materials, and related activities with high confidence.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Understanding Ionizing Radiation-Induced Speciation, Chemistry, and Transport in Nuclear Materials

The research to be presented will cover an overview of three projects supported by the United States Department of Energy Office of Science Solar Photochemistry Program: (i) Radiation-Induced Late Actinide Redox Chemistry (2019–2022); (ii) Understanding Radiation-Induced Iodine Speciation, Chemistry, and Transport in High Temperature Molten Salts (2022–2025); and (iii) Radiation-Induced Chemistry of Nuclear Materials (2023–2026). The overarching aim of these distinct projects is to develop a deep fundamental mechanistic understanding of ionizing-radiation-induced processes occurring in solutions over multiple time and length scales. Investigated solutions range from aqueous to organic to molten salt liquids in the presence and absence of ligands and various redox-active ions and molecules, including the actinides. The ultimate goal of these projects is to utilize the new foundational knowledge gained to construct quantitative multiscale computer models with the capacity to predict radiation-induced behavior in complex systems of relevance to nuclear energy technologies and beyond.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Determination of Important Nuclear Fragmentation Processes for Human Space Radiation Protection

We present a semi-analytical method to determine which partial cross sections of nuclear fragmentations most affect the shielded dose equivalent due to exposure to galactic cosmic rays. The cross sections thus determined will require more theoretical and/or experimental studies in order for us to better predict, reduce and mitigate the radiation exposure in human space explorations.

Lin, Zi-Wei↗

Effects of Build Orientation and Heat Treatment on Neutron Irradiation Hardening in Inconel 625 Fabricated via Laser Powder Bed Fusion

Various Inconel 625 coupons fabricated via Laser Powder Bed Fusion (L-PBF) were neutron irradiated using the inside reflector of the reactor at the University of Missouri Research Reactor (MURR). Effects of build orientation and heat treatment on neutron-induced hardening were investigated by inspecting L-PBF samples built vertically or at a 45º angle in the following heat-treated conditions: as-built (no heat treatment), 700 ºC for 1 hour, 900 ºC for 1 hour, and 1050 ºC for 1 hour. The microhardness results of L-PBF samples before and after neutron irradiation were compared with traditional wrought Inconel 625. All samples underwent an irradiation flux of 6.61 x 1013 neutrons/cm²/s for 310 hours for an estimated damage of 0.012 dpa. Results indicate that as-built L-PBF specimens are less prone to radiation hardening relative to their wrought counterparts. As-printed diagonal specimens were shown to harden by 8% as compared to 1.2% hardening in as-printed vertical specimens.

36 MATERIALS SCIENCE↗

Sulfur Pellets Responses to a Bare and Steel Reflected Pulse of the Oak Ridge National Laboratory Health Physics Research Reactor

The experiments analyzed in this report were conducted at the Health Physics Research Reactor (HPRR), also known as the $\textit{Fast Burst Reactor}$. The reactor was designed and built at Oak Ridge National Laboratory (ORNL) in 1961. The HPRR was an unmoderated, unshielded fast reactor that used highly enriched uranium and molybdenum alloy as fuel. The reactor was initially sent to the Nevada Test Site in 1962, where it was used to evaluate radiation doses received as a result of the Hiroshima and Nagasaki bombings during World War II. A few years later, the reactor was sent back to ORNL to be part of the Dosimetry Application Research (DOSAR) facility shown in Figure 1, which included a reactor building shown on the left (west) of the picture and a control and laboratory building in the upper right corner (northeast). The critical assembly was used for numerous technical studies, including systems calibration, dosimetry, radiobiology of plants and animals, testing of radiation alarms, as well as teaching and training in radiation dosimetry and nuclear engineering. Between 1963 and 1987, the HPRR was operated for thousands of hours, achieving criticality close to 10,000 times and motivating many publications. The HPRR was decommissioned in 1987. The goal of this effort was to use historical data from operation of the HPRR to create a criticality accident alarm system (CAAS) benchmark to be included in the $\textit{International Handbook of Evaluated Criticality Safety Benchmark Experiments}$ (ICSBEP Handbook). A thorough inspection was performed of all available documentation and information available. The most promising experiments that were selected for evaluation were those described in the 1987 ORNL report entitled $\textit{Health Physics Research Reactor Reference Dosimetry}$, ORNL-6240. The report includes reference dosimetry results of the shielded and unshielded configurations of the HPRR after burst operations. Because of changes to the reactor positioning and storage systems that were made in 1985, the previous dosimetry reports became obsolete, and the newly designed experiments were needed to create the HPRR’s adjusted dosimetry data. The various results reported in ORNL-6240 include reference doses and dose equivalents from different conventions at different distances and elevations as determined using the detected neutron fluence and conversion factors. The HPRR neutron fluence was obtained through different methods, including sulfur pellet analysis and threshold detector unit data. Information about the HPRR spectrum was also obtained through Bonner sphere measurements. This benchmark is focused on a part of the measured sulfur fluences reported in Appendix H of ORNL-6240. Standard commercial sulfur pellets were placed at different distances from the HPRR centerline during burst operation and were activated due to the 32 S(n,p) 32 P reaction. The resulting 32 P activity was then measured and the information about the corresponding sulfur fluence and/or neutron dose could be extracted. Many of those measurements have 7 been performed with the HPRR in its bare configuration or with different shields (combinations of Lucite, concrete, steel). All the necessary, precise information about material and/or dimensions of the different shields was not found, so it was decided to focus only on the unshielded and steel-shielded configurations to minimize the benchmark uncertainty. A total of 31 cases (24 unshielded and 7 shielded cases at different positions) of sulfur fluence were selected before evaluation to develop the benchmark.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

High-Current Light-Ion Cyclotron for Applications in Nuclear Security and Radioisotope Production

In this article, we propose the conceptual design, with supporting beam dynamics results, of a normal conducting, separated-sector cyclotron with a strong-focusing field gradient designed to accelerate light ions with a charge-to-mass ratio of 1/2 up to 15–20 MeV/u. The design can support a host of applications for therapy, radiobiology, material science, and instrumentation development. The light-ion species, which can include a mixed ion beam, can be dynamically chosen to provide a range of characteristic signals appropriate for specific material identification such as special nuclear materials. A conservative baseline concept is presented which has been optimized for radioisotope production of alpha emitters and theranostic radiopharmaceuticals. The modular design is also demonstrated to be scalable in gross physical parameters by a factor of 2–3, thereby reducing the size, weight, and power requirements (SWaP) and enabling near-term security applications.

07 ISOTOPE AND RADIATION SOURCES↗

Gaseous-fuel nuclear reactor research for multimegawatt power in space

In the gaseous-fuel reactor concept, the fissile material is contained in a moderator-reflector cavity and exists in the form of a flowing gas or plasma separated from the cavity walls by means of fluid mechanical forces. Temperatures in excess of structural limitations are possible for low-specific-mass power and high-specific-impulse propulsion in space. Experiments have been conducted with a canister filled with enriched UF6 inserted into a beryllium-reflected cavity. A theoretically predicted critical mass of 6 kg was measured. The UF6 was also circulated through this cavity, demonstrating stable reactor operation with the fuel in motion. Because the flowing gaseous fuel can be continuously processed, the radioactive waste in this type of reactor can be kept small. Another potential of fissioning gases is the possibility of converting the kinetic energy of fission fragments directly into coherent electromagnetic radiation, the nuclear pumping of lasers. Numerous nuclear laser experiments indicate the possibility of transmitting power in space directly from fission energy. The estimated specific mass of a multimegawatt gaseous-fuel reactor power system is from 1 to 5 kg/kW while the companion laser-power receiver station would be much lower in specific mass.

Thom, K.↗