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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Production Pathways for Medically Interesting Isotopes

Radioisotopes are commonly used in nuclear medicine for treating cancer and new, more effective treatment options are always desired. As a result, there is a national need for new radioisotopes and ways to produce them. A computer program was created that evaluates the daughters for all known reactions of projectiles (gamma rays, protons or neutrons) with every stable target isotope by comparing the cross-sections for each reaction at a desired energy, and outputs a list of the potential daughter isotopes that are most likely to be generated. The program then evaluates the decay chains of these daughters to provide a list of the possible decay chains that contain the radioisotope of interest. By knowing the daughter production and decay chain for each isotope, it is possible to go from the desired radioisotope to the stable isotope that can be used as a target for its production. This project would facilitate the search for new pathways to creating useful theranostic isotopes.

Hutton, A.↗
DOE OSTI2022

Impact of Changes in ENDF/B-VII.1 and ENDF/B-VIII.0 235U Nuclear Data Indicated by NDSE Studies on LLNL Pulsed Sphere Simulations

A recent journal article by J.A. Gomez et al. measured gamma-ray die-off curves of three subcritical static highly-enriched uranium (HEU) assemblies driven by an external neutron source with a new detector system. This new detector system was developed for being used in dynamically driven subcritical assemblies as part of the Neutron Diagnosed Subcritical Experiments (NDSE) program. Simulations of these die-off curves with various nuclear data and comparison to experimental data indicated that a decrease of the ENDF/B-VII.1 235 U(n,inl) cross section by a factor 0.8 and 0.85 for ENDF/B-VIII.0 would lead to better predictions of experimental data. Here, we test the proposed changes with another type of measurement response, namely neutron-leakage spectra emitted in LLNL pulsed sphere measurements. These spheres were pulsed by 14-MeV neutrons produced via the D+T reaction in their center. The proposed changes in nuclear data have a distinctly smaller impact on predicting pulsed-sphere neutron-leakage spectra than for the die-off curves; they lead to a worsened prediction of the inelastic valley of LLNL pulsed-sphere neutron spectra indicating that the proposed change could constitute a compensating error. Changes in the inelastic angular distributions along with the cross section might be worthwhile to study

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Sensitivity of the 13 C(α,n) 16 O S factor to the uncertainty in the level parameters of the near-threshold state

The 13 C(α,n) 16 O reaction is the main source of neutrons for the s and i processes in asymptotic giant branch stars and carbon-enhanced metal-poor stars, respectively. The reaction rate over the relevant temperature range from 0.1 to 0.3 GK translates into a center-of-mass energy range of 150 to 540 keV. Current measurements extend down to 300 keV, still requiring an extrapolation of the cross section. At these low energies, the high-energy tail of a 1/2 + state near the reaction threshold makes a significant contribution to the cross section, but its amplitude is still highly uncertain. In this work the uncertainties associated with the low-energy cross-section extrapolation are investigated, in particular the sensitivity to the energy, width, and Coulomb renormalized asymptotic normalization coefficient of the near-threshold resonance. Furthermore, recently it has been suggested that the energy of the near-threshold level may have a large impact on the extrapolation, but this is not found to be the case compared with the other sources of uncertainty.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Measurement of the cross section of the Q=4.4398 MeV 12 C (n, n'γ) reaction from threshold to 16.5 MeV using γ and correlated n–γ detection

The Q=4.4398 MeV 12 C (n, n'γ) cross section was measured using a white incident neutron source through the detection of γ rays only and n–γ coincidences using a segmented liquid scintillator detector array. While the n–γ technique utilized here is more generally applicable to a wide variety of neutron scattering measurements, the γ-only technique was successfully applied to this reaction to exploit the precise time resolution and high efficiency of this detection system to yield results with unprecedented statistical precision and total uncertainties < 2 % from reaction threshold up to 16 MeV incident neutron energy, clearly resolving many features in this reaction that were previously not well known. The γ-only and n–γ results are consistent with each other for the majority of the incident energy range covered in this paper, thereby lending validation to the n–γ technique for future measurements, though significant disagreements are observed between both results and with the ENDF/B-VIII.0 nuclear data evaluation. These differences are particularly noticeable in the recently evaluated energy range below 6.5 MeV, and also near 14 MeV where a “sawtooth”-like feature is observed similar to that in other 12 C+n reaction channels. Finally, both γ-only and n–γ results are presented here with thorough covariance derivations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Activation and surface reactions of CO and H 2 on ZnO powders and nanoplates under CO hydrogenation reaction conditions

Here, activation and surface reactions of CO and H 2 on ZnO powders and nanoplates under CO hydrogenation reaction conditions were (quasi) in situ studied using temperature programmed surface reaction spectra, diffuse reflectance Fourier transform infrared spectroscopy, inelastic neutron scattering spectroscopy and electron paramagnetic resonance. CO undergoes disproportion reaction to produce gaseous CO 2 and surface carbon adatoms, and adsorbs to form surface formate species. H 2 adsorption forms dominant irreversibly-adsorbed surface hydroxyl groups and interstitial H species and very minor surface Zn-H species. Surface formate species and hydroxyl groups react to produce CO 2 and H 2 , while surface carbon adatoms are hydrogenated by surface Zn-H species sequentially to produce CH(a), CH 2 (a), CH 3 (a) and eventually gaseous CH 4 . The ZnO nanoplates, exposing a higher fraction of Zn-ZnO(0001) and O-ZnO(000–1) polar facets, are more active than the ZnO powders to catalyze CO hydrogenation to CH 4 . These results provide fundamental understanding of the reaction mechanisms and structural effects of CO hydrogenation reaction catalyzed by ZnO-based catalysts.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Real-time nuclear activation detectors for measuring neutron angular distributions at the National Ignition Facility (invited)

The Real Time Nuclear Activation Detector (RTNAD) array at NIF measures the distribution of 14 MeV neutrons emitted by deuterium-tritium (DT) fueled inertial confinement fusion implosions. The uniformity of the neutron distribution is an important indication of implosion symmetry and DT shell integrity. The array consists of 48 LaBr 3 (Ce) crystal gamma-ray spectrometers mounted outside the NIF target chamber, which continuously monitor the slow decay of the 909 keV gamma-ray line from activated 89 Zr located in Zr cups surrounding each crystal. The measured decay rate dramatically increases during a DT implosion in proportion to the number of 14 MeV neutrons striking each Zr cup. The neutrons produce activated 89 Zr through an (n, 2n) reaction on 90 Zr, which is insensitive to low energy neutrons. The neutron flux along the detector line-of-sight at shot time is determined by extrapolating the fitted 909 keV decay curve back to shot time. Automatic analysis algorithms were developed to handle the non-stop data stream. The large number of detectors and the high statistical accuracy of the array enable the spherical harmonic modes of the neutron angular distribution to be measured up to L ≤ 4 to provide a better understanding of implosion dynamics. In addition, these data combined with measurements of the down-scattered neutrons can be used to derive fuel areal density distributions. This paper will describe the RTNAD hardware and analysis procedures.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Review of Direct Neutron Conversion and Detection Processes

Commercial and laboratory neutron detection systems use indirect neutron response of materials like pressurized helium-3 (via nuclear reaction 3He(n, p)3H) to measure and count neutrons emanating from a source. Recently a host of semiconductors, especially a ternary semiconductor of lithium indium diselenide (6LiInSe2) and a quaternary alloy of enriched lithium-6, indium, phosphorous, and selenium (6LiInP2Se6), have shown promising neutron counting possibilities by directly converting neutrons into charge-carrying elements within the body of the semiconductor. These semiconductors have high thermal neutron capture cross sections, suitable energy bandgaps (~2.0 electron volts) for room-temperature operations, and a favorable electronic band structure for efficient electron charge transport. The article examines the semiconductor properties of these compounds in terms of their neutron counting capabilities and possible ways to extract neutron energy information from them. Lithium-6 and boron-10 (with thermal neutron absorption cross sections of 938 ± 6 and 3855 ± 26 barns, respectively) produce charged particles to be measured via indirect neutron interactions. The efficiency of indirect conversion neutron detectors is limited because of the inefficiencies in conversion mechanism. In case of direct conversion, the neutrons create charged particles in a single material for neutron capture and charge collection, increasing detection efficiency. Unlike 3He proportional counters, which provide no neutron energy information, the semiconductors can be used as neutron energy spectrometer. Fully resolved neutron energy by 6LiInP2Se6 from a plutonium-beryllium source has been reported in the literature. We will discuss the influence of these multilayered semiconductors’ crystallographic structures and growth techniques on neutron energy determination.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2022

Fast-neutron-induced fission of Pu 240 and Pu 242

Herein we report the measurement of the total kinetic energy (TKE) release in the fast neutron induced fission of 240 Pu and 242 Pu. The results are compared to the predictions of the GEF model, the CGMF model, and the model of Denisov and Sedykh as well as previous exptl. work on these reactions. Our absolute measurements of the TKE release are in good agreement with the previous measurements of Nethaway et al. for the interaction of 14.8 MeV neutrons with 240 Pu [Phys. Rev. C16, 1907 (1977)] and of Winkelmann and Aumann for the interaction of 15 MeV neutrons with 242 Pu [Phys. Rev. C30, 934 (1984)]. The general trends of the measured TKE values agree with phenomenol. models but the variances of the TKE distributions are significantly less than predicted by various models. The mean postneutron emission TKE release decreases nonlinearly with increasing neutron energy and can be represented as TKE(MeV) = 175.8 ± 0.3 - (2.4 ± 0.8) lo g 10 E n - (1.4 ± 0.4) lo g 10 $E^{2}_{n}$ for 240 Pu and TKE(MeV) = 177.1 ± 0.3 - (1.2 ± 0.9) lo g 10 E n - (1.8 ± 0.5)lo g 10 $E_{n}^{2}$ for 242 Pu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Yet Another Hauser-Feshbach Code

Code framework to perform simulations of nuclear reactions with incident particles including gammas, protons, neutrons, deuterons, tritons, helium-3, and alphas to develop nuclear data libraries and study nuclear reaction phenomona. The code can model nuclear reactions or initial populations specified by the user. The decays principally follow the compound-nucleus hypothesis and the statistical decay of Hauser and Feshbach. The code models nuclear decays with a Monte Carlo process that tracks the decay of each state. Data libraries are produced that can be translated into GNDS (generalized Nuclear Data Structure). YAHFC can also be used as an event generator, with individual decays written to disk for offline analysis. Both serial and MPI versions are provided. YAHFC does NOT perform transport of nuclear reactions through materials, only the primary reaction with a target material.

Ormand, WilliamE.↗
DOE OSTI2022

Increased Ion Temperature and Neutron Yield Observed in Magnetized Indirectly Driven $\mathrm{D_2}$-Filled Capsule Implosions on the National Ignition Facility

Here, the application of an external 26 Tesla axial magnetic field to a D 2 gas-filled capsule indirectly driven on the National Ignition Facility is observed to increase the ion temperature by 40% and the neutron yield by a factor of 3.2 in a hot spot with areal density and temperature approaching what is required for fusion ignition. The improvements are determined from energy spectral measurements of the 2.45 MeV neutrons from the D(d, n) 3 He reaction, and the compressed central core B field is estimated to be ~4.9 kT using the 14.1 MeV secondary neutrons from the D(T, n) 4 He reactions. The experiments use a 30 kV pulsed-power system to deliver a ~ 3 μs current pulse to a solenoidal coil wrapped around a novel high-electrical-resistivity AuTa 4 hohlraum. Radiation magnetohydrodynamic simulations are consistent with the experiment

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Neutron Yield of Thermo Scientific P385 D-T Neutron Generator vs . Current and Voltage

The Thermo Scientific P385 Neutron Generator is a compact neutron source, producing 14 MeV neutrons through the deuterium-tritium (DT) fusion reaction. It is important to measure and understand the dependence of the neutron production rate on the accelerator current and voltage. In this study we evaluated neutron production with an absolutely calibrated liquid scintillator neutron spectrometer (BTI N-Probe), an absolutely calibrated He-3 detector surrounded by HDPE shells (Detec Nested Neutron Spectrometer, NNS), and two uncalibrated ZnS fast neutron scintillators (EJ-410), for both A3082 and A3083 sealed tubes. Here we also modeled the neutron yield using the TRIM code, which calculates the trajectory and the energy loss of deuterons and tritons within the target. Experimental results showed an essentially linear dependence on beam current, as expected. A 3.59 ±0.08 power law dependence on the operating voltage was measured, in effective agreement with the modeled value of 3.5. A series of absolute NNS and N-Probe measurements, matched against MCNP calculations, showed that the A3083 and A3082 tubes provide a maximum neutron yield of 8.2 × 10 8 n/s and 4.7 × 10 8 n/s respectively, with estimated uncertainty of ±10%.We showed, through modeling, that tritium decay is not a significant consideration for tubes, such as these, with lifetimes of less than 10 years.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Time-of-flight vs time-of-arrival in neutron spectroscopic measurements for high energy density plasmas

The neutron time-of-flight (nToF) diagnostic technique has a lengthy history in Inertial Confinement Fusion (ICF) and High Energy Density (HED) Science experiments. Its initial utility resulted from the simple relationship between the full width half maximum of the fusion peak signal in a distant detector and the burn averaged conditions of an ideal plasma producing the flux [Lehner and Pohl, Z. Phys. 207, 83–104 (1967)]. More recent precision measurements [Gatu-Johnson et al., Phys. Rev. E 94(8), 021202 (2016)] and theoretical studies [Munro, Nucl. Fusion 56, 035001 (2016)] have shown the spectrum to be more subtle and complicated, driving the desire for an absolute calibration of the spectrum to disambiguate plasma dynamics from the conditions producing thermonuclear reactions. In experiments where the neutron production history is not well measured, but the neutron signal is preceded by a concomitant flux of photons, the spectrum can be in situ calibrated using a set of collinear detectors to obtain a true “time-of-flight” measurement. This article presents the motivation and overview of this technique along with estimates of the experimental precision needed to make useful measurements in existing and future nToF systems such as the pulsed power Z-machine located in Albuquerque, NM, at Sandia National Laboratories.

Fusion experiments↗
DOE OSTI2023

Collective enhancement in the exciton model

The preequilibrium reaction mechanism is considered in the context of the exciton model. A modification to the one-particle–one-hole state density is studied which can be interpreted as a collective enhancement. The magnitude of the collective enhancement is estimated by simulating the Lawrence Livermore National Laboratory (LLNL) pulsed-spheres neutron-leakage spectra. Here the impact of the collective enhancement is explored in the context of the highly deformed actinide, 239 Pu. A consequence of this enhancement is the removal of fictitious levels in the distorted-wave Born approximation often used in modern nuclear reaction codes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

p +p - electroproduction off protons in deuterium: measurements of quasi-free cross sections and kinematic probing of final state interactions

In this study, the process of pi+pi- electroproduction off protons bound in deuterium nuclei is explored. The exploration is performed through the analysis of experimental data on electron scattering off the deuteron target, collected in Hall B at Jefferson Lab with the CLAS detector. As a main result, the set of integrated and single-differential cross sections of the reaction yvp(n) -> p'(n')pi+pi- is obtained. The cross sections are extracted in the quasi-free regime, which implies that only events not affected by final state interactions are subject to selection. The measurements are performed in the kinematic region of the invariant mass W from 1.3 GeV to 1.825 GeV and photon virtuality Q2 from 0.4 GeV2 to 1 GeV2. Sufficient experimental statistics allows narrow binning, i.e. 25 MeV in W and 0.05 GeV2 in Q2, while maintaining an adequate statistical uncertainty. The extraction of quasi-free cross sections is accompanied by the kinematic probing of FSI between the reaction final hadrons and the spectator neutron in the aforementioned exclusive channel. In this probing the distributions of missing quantities are used in order to investigate the relative spread of events with FSI along the reaction phase space, trace the difference of FSI manifestations in different reaction topologies, reveal details on alterations of the hadron momentum in FSI, and isolate FSI contributions of various final hadrons. The performed examination is also capable of retrieving information on some underlying FSI mechanisms, among which the process of resonance formation in the intermediate state of pion-neutron interactions is particularly remarkable.

Skorodumina, Iuliia↗
DOE OSTI2023

Cubical moderators for the Neutron Target Demonstator (NTD)

Neutron capture cross sections of unstable isotopes are important for neutron induced nucleosynthesis as well as for technological applications. The traditional time-of-flight method reaches its limits once the necessary detection of the reaction products is hampered by the size (mass) of the sample. Several factors may limit the sample mass: The decay properties of radioactive isotopes interfere with the signals from the neutron capture or neutron-induced fission reactions; The limited range of charged reaction products requires a thin sample. In both cases, an increased neutron fluence at the sample position with ever improved neutron sources overcomes the lack of reaction rate. Reference proposed a combination of a radioactive beam facility, an ion storage ring and a spallation neutron source surrounded by neutron moderator. This idea is part of the LANSCE strategy to stay a worldwide leader for neutron induced research. Figure 1 shows a sketch of the proposed future setup.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

New 13 C(α,n) 16 O Cross Section with Implications for Neutrino Mixing and Geoneutrino Measurements

Precise antineutrino measurements are very sensitive to proper background characterization. Here, we present an improved measurement of the 13 C(α,n) 16 O reaction cross section which constitutes significant background for large v¯ detectors. We greatly improve the precision and accuracy by utilizing a setup that is sensitive to the neutron energies while making measurements of the excited state transitions via secondary γ-ray detection. Our results shows a 54% reduction in the background contributions from the 16 O(3–, 6.13 MeV) state used in the KamLAND analysis.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Production of Very Light Elements and Strontium in the Early Ejecta of Neutron Star Mergers

Abstract We study the production of very light elements ( Z < 20) in the dynamical and spiral-wave wind ejecta of binary neutron star mergers by combining detailed nucleosynthesis calculations with the outcome of numerical relativity merger simulations. All our models are targeted to GW170817 and include neutrino radiation. We explore different finite-temperature, composition-dependent nuclear equations of state, and binary mass ratios, and find that hydrogen and helium are the most abundant light elements. For both elements, the decay of free neutrons is the driving nuclear reaction. In particular, ∼0.5–2 × 10 −6 M ⊙ of hydrogen are produced in the fast expanding tail of the dynamical ejecta, while ∼1.5–11 × 10 −6 M ⊙ of helium are synthesized in the bulk of the dynamical ejecta, usually in association with heavy r -process elements. By computing synthetic spectra, we find that the possibility of detecting hydrogen and helium features in kilonova spectra is very unlikely for fiducial masses and luminosities, even when including nonlocal thermodynamic equilibrium effects. The latter could be crucial to observe helium lines a few days after merger for faint kilonovae or for luminous kilonovae ejecting large masses of helium. Finally, we compute the amount of strontium synthesized in the dynamical and spiral-wave wind ejecta, and find that it is consistent with (or even larger than, in the case of a long-lived remnant) the one required to explain early spectral features in the kilonova of GW170817.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Study of the deformed halo nucleus 31 Ne with Glauber model based on microscopic self-consistent structures

In this work, the exotic deformed nucleus 31 Ne is studied with an approach that combines self-consistent structure and reaction theories. The deformed relativistic Hartree-Bogoliubov theory in continuum (DRHBc) is utilized to demonstrate that deformation and pairing correlations give rise to a halo structure with a large-amplitude p-wave configuration in 31 Ne. Then the valence nucleon wave functions and angle-averaged density distributions of 30 Ne from this theory are used as input for the Glauber reaction model to study the observables of neutron-rich neon isotopes to search halo signatures. With NL1 effective interaction, our predictions of the reaction cross sections for these exotic neon isotopes on a carbon target can better reproduce the experimental data than those from the relativistic mean field model for a spherical shape with resonances and pairing correlation contributions, and are roughly 3.3% (~ 50 mb) larger than those with Gaussian function-fitted densities of the core nuclei. The calculated one-neutron removal cross section at 240 MeV/nucleon, and the inclusive longitudinal momentum distribution of the 30 Ne residues from the 31Ne breakup reaction are largely improved over previous theoretical predictions and agree well with data. These reaction evaluations indicate a dilute density distribution in coordinate space and are a canonical signature of a halo structure. Moreover, our predictions with the NL3 and PK1 effective interactions give slightly better descriptions of reaction observables for exotic neon isotopes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗