Probing Attosecond Electron Dynamics With an X-Ray Free-Electron Laser
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Driver, Taran↗
SEARCH · Engineering Papers
Results for “Laser dynamics”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Lunar dynamics and selenodesy - Results from analysis of VLBI and laser data
Very long base line interferometry (VLBI) observations of lunar radio transmitters have been combined with data from laser ranging to lunar retroreflectors to estimate simultaneously (1) parameters in models of the lunar orbit and libration and (2) the selenodetic coordinates of the radio transmitters and retroreflectors. For the ratio of the mass of the sun to that of the earth plus moon, a value of approximately 328,900.5 is obtained. The lunar moment-of-inertia ratios beta and gamma are also determined. The values and most of the uncertainties obtained for the third-degree harmonics of the moon's gravity field are comparable to those which have been obtained by others from observations of lunar-orbiting spacecraft. However, the results for the two third-degree gravity coefficients have much less uncertainty than determinations based on laser data alone. For the relative position vectors of the lunar radio transmitters and the retroreflectors, the estimates have uncertainties of about 30 m along the earth-moon direction and about 10 m in each of the two transverse coordinates.
King, R. W.↗
Planetary orbit dynamics via trilateration: Prospectus for an interplanetary scale ring laser gyro with nominal area of 1 square AU
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Bruce Bills↗
Magnetic Reconnection in High Energy Density Laboratory Plasmas
Understanding the physics of collisionless, magnetized plasmas is key to unlocking a number of important problems in space and astrophysics. Magnetic reconnection is a fundamental mechanism which can explosively release stored magnetic energy, convert it to plasma heat and flows, and accelerate particles. In this project we developed technique and conducted experiments and simulations of magnetic reconnection in laser produces plasmas. Through this project, we also developed experimental techniques to generate magnetized collisionless shocks, and we therefore expanded the scope of the project to develop these experiments. These projects make fundamental progress on understanding the dynamics of magnetized laser-produced plasmas. In additional to plasma astrophysics, these results have broad interest for laboratory high energy density plasmas, since magnetic fields can be used to confine and control plasmas in many contexts and may offer new capabilities toward laboratory ignited plasmas.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Review: Real-space analyses of local dynamics in liquid using X-ray scattering
In this review, we advocate describing the liquid dynamics using the Van Hove correlation function, a temporal and spatial correlation function. Recent progress in X-ray optics and X-ray sources makes it possible to carry out inelastic and quasi-elastic x-ray scattering whose spectra can be converted into the dynamic correlation function in real space. We describe the basic concept of the Van Hove correlation function, how it is obtained from the X-ray scattering spectra using synchrotron X-rays and X-ray free electron lasers, and the atomic dynamics in water and aqueous salt solution.
Shinohara, Yuya↗
The lightcraft project
Rensselaer Polytechnic Institute has been developing a transatmospheric 'Lightcraft' technology which uses beamed laser energy to propel advanced shuttle craft to orbit. In the past several years, Rensselaer students have analyzed the unique combined-cycle Lightcraft engine, designed a small unmanned Lightcraft Technology Demonstrator, and conceptualized larger manned Lightcraft - to name just a few of the interrelated design projects. The 1990-91 class carried out preliminary and detailed design efforts for a one-person 'Mercury' Lightcraft, using computer-aided design and finite-element structural modeling techniques. In addition, they began construction of a 2.6 m-diameter, full-scale engineering prototype mockup. The mockup will be equipped with three robotic legs that 'kneel' for passenger entry and exit. More importantly, the articulated tripod gear is crucial for accurately pointing at, and tracking the laser relay mirrors, a maneuver that must be performed just prior to liftoff. Also accomplished were further design improvements on a 6-inch-diameter Lightcraft model (for testing in RPI's hypersonic tunnel), and new laser propulsion experiments. The resultant experimental data will be used to calibrate Computational Fluid Dynamic (CFD) codes and analytical laser propulsion models that can simulate vehicle/engine flight conditions along a transatmospheric boost trajectory. These efforts will enable the prediction of distributed aerodynamic and thruster loads over the entire full-scale spacecraft.
Messitt, Don G.↗
Quantum dynamics of positron-hydrogen scattering and three-body bound state formation with an assisting laser field: predictions of a reduced-dimensionality model
Abstract We investigate the quantum dynamics of target excitation and positronium formation in the positron-hydrogen atom scattering without and with an external assisting laser field within a reduced-dimensional quantum model. Strong interference fringes between the incident and reflected positron wave packets are observed in the reaction region. We further investigate the critical behavior of transition probabilities near the channel-opening thresholds for hydrogen excitation and positronium formation and find a strong competition between channels with similar threshold energies, but different parities. The transmission ratios of the incident positron in different reaction channels are calculated, and it is shown that only positronium formation in the ground state prefers forward scattering. Our simulation of the positron-hydrogen scattering with an assisting laser field indicates that the three-particle bound states can be formed during the collisions due to the photon emission induced by the external laser field.
Optics↗
Dark-field x-ray microscopy for 2D and 3D imaging of microstructural dynamics at the European x-ray free-electron laser
Dark field x-ray microscopy (DXFM) can visualize microstructural distortions in bulk crystals. Using the femtosecond x-ray pulses generated by x-ray free-electron lasers (XFELs), DFXM can achieve sub-μm spatial resolution and <100 fs time resolution simultaneously. In this paper, we demonstrate ultrafast DFXM measurements at the European XFEL to visualize an optically driven longitudinal strain wave propagating through a diamond single crystal. We also present two DFXM scanning modalities that are new to the XFEL sources: spatial 3D and 2D axial-strain scans with sub-μm spatial resolution. With this progress in XFEL-based DFXM, we discuss new opportunities to study multi-timescale spatiotemporal dynamics of microstructures.
47 OTHER INSTRUMENTATION↗
Self-pulsing and bichromatic emission in homogeneously broadened bidirectional ring lasers
The effects of saturation-induced Bragg gratings on the mode structure and dynamics of bidirectional homogeneously broadened ring lasers are studied. The grating is viewed as a distributed feedback medium in a ring cavity and modes appropriate to such a structure are used. A Fourier decomposed rate equation model is developed to study the behavior of these modes above threshold. The difference in the properties of these solutions from the modes of an unfilled ring cavity lead to the possibility of bichromatic emission and both regular undamped and irregular damped self-pulsing.
Rabinovich, W. S.↗
Construction of a Visible Diode Laser Source for Free Radical Photochemistry and Spectroscopy Experiments
Tunable diode lasers are reliable sources of narrow-band light and comparatively cheap. Optical feedback simplifies frequency tuning of the laser diodes. We are building an inexpensive diode laser system incorporating optical feedback from a diffraction grating. The external optical cavity can be used with lasers that emit between 2 and 100 mW, and will also work if they are pulsed, although this will significantly degrade the bandwidth. The diode laser output power and bandwidth are comparable to CW dye lasers used in kinetics and dynamics experiments. However, their cost and maintenance will be much less as will alignment time. We intend to use the diode lasers to investigate CN and C2 kinetics as well as to study dissociation dynamics of atmospherically important molecules.
Newman, Bronjelyn↗
High Intensity Gamma Ray Source Scintillation Attenuation Spectrometer and Filter Stack Monoenergetic Calibration
The Laser-Based X-ray Radiographic Imaging team at Los Alamos National Lab is looking for a monoenergetic MeV X-ray source to both verify our Monte Carlo N-particle simulations of detector performance and calibrate the instruments for future measurements. Funded by the Laboratory Directed Research and Development (LDRD) program, our overall goal is to improve the radiographic quality and reliability of laser-based X-ray sources for deployment at both dynamic and static radiography facilities. Laser-based X-ray sources have demonstrated smaller spot sizes to current electron accelerator based sources. The smaller laser spot size leads to significantly improved resolution.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
X-ray diffraction study of phase transformation dynamics of Fe and Fe-Si alloys along the shock Hugoniot using an x-ray free electron laser
The x-ray free electron laser (XFEL) enables probing a highly compressed material response at the subnanosecond timescale. Here we exploit the ultrafast XFEL pulse to combine reflection x-ray diffraction and laser-driven shock compression to perform a study of the phase transformation and stability in Fe and Fe-Si alloys. Our approach enables us to observe that solid-solid phase transformations occur in Fe and Fe- Si 8.5 wt % in ≤ 130 ps at ~ 130 GPa; no transformation is observed in Fe- Si 16 wt % up to 110 GPa. Density functional theory calculations predict similar phase relations.
36 MATERIALS SCIENCE↗
Operando synchrotron X-ray analysis of melt pool dynamics in an Al-Sn immiscible alloy
The melt flow in an Al-50vol.% Sn immiscible alloy, produced by single-track laser melting of Al and Sn elemental powders, was studied in real time. High-speed synchrotron X-ray imaging was used to track Al and Sn liquids’ movements, and also to examine elemental distributions in the laser tracks, complimented by electron microscopy after solidification. Key aspects, including melt pool geometry, keyhole instability, and flow dynamics (flow pattern and velocity), were examined using digital image analysis. Relatively deeper melt pools formed at 400 W and 300 mm/s exhibited greater stability, with smooth surfaces, consistent outward flow, and minor vortices near the keyhole. In contrast, shallower pools produced at higher scanning speeds (>500 mm/s) demonstrated greater instability with increased surface waviness, and stronger velocity fluctuations, leading to numerous micro-vortices and increased Al-Sn heterogeneity. Velocity scale estimations, supported by experimental observations, examined the roles of vapour pressure, Marangoni effect, buoyancy, inertial, and surface tension forces in the flow. The results revealed that vapour pressure and mechanical waves dominated at high scanning speeds (shallow pools), while Marangoni forces were equally significant in deep pools at lower speeds (300 mm/s). Buoyancy was found to have minimal impact in both cases. Furthermore, the interaction between inertial and surface tension forces played a critical role in determining the degree of waviness of the pools’ surfaces. These findings offer valuable insights into melt pool dynamics during laser processing of immiscible alloys and other metallic systems using elemental powders, and provide guidance for developing high-fidelity computational fluid dynamics models.
immiscible alloys↗
Extended x-ray emission times of clusters in intense x-ray pulses
Novel experimental spectroscopic and imaging techniques have been developed to exploit x-ray free-electron laser (XFEL) for studying structure and dynamic of non-periodic entities at atomic spatial resolution and femtosecond timescales.Recently, intensity correlation of x-ray fluorescence, based on the principle introduced by Hanbury Brown and Twiss [R. Hanbury Brown and R. Q. Twiss, Nature (London) 177, 27 (1956)], has been proposed for high-resolution imaging of a three-dimensional arrangement of atoms. To explore the applicability of this fluorescence approach, we theoretically investigate fluorescence dynamics of nonperiodic systems subject to x-ray free electron laser (XFEL) pulses over a range of fluences from the linear to nonlinear x-ray absorption regimes as a function of system size, from a single atom to a cluster of 149 171 atoms. Fluorescence dynamics in the nonlinear x-ray regime differs from that in the weak x-ray field in that intense x-ray pulses interrupt the fluorescence dynamics by multiphoton absorption creating a dense electron environment within the sample on a femtosecond timescale. In large systems, the presence of both recombination and photoionization pathways gives rise to an enhanced Kα and Kα h emission yield and an extended emission time beyond the lifetime of the core-excited states. Our analysis suggests that, in an intense x-ray pulse, the Kα h emission line can be a good candidate for fluorescence imaging as it has a higher yield and an emission time that is short relative to the x-ray-induced lattice distortion time.
74 ATOMIC AND MOLECULAR PHYSICS↗
Potential capabilities of lunar laser ranging for geodesy and relativity
Here, we review the LLR technique focusing on its impact on Geodesy and Relativity. We discuss the modem observational accuracy and the level of existing LLR modeling. We present the near-term objectives and emphasize improvements needed to fully utilize the scientific potential of LLR.
earth - moon dynamics↗
Laser-driven, ion-scale magnetospheres in laboratory plasmas. I. Experimental platform and first results
We report magnetospheres are a ubiquitous feature of magnetized bodies embedded in a plasma flow. While large planetary magnetospheres have been studied for decades by spacecraft, ion-scale “mini” magnetospheres can provide a unique environment to study kinetic-scale, collisionless plasma physics in the laboratory to help validate models of larger systems. In this work, we present preliminary experiments of ion-scale magnetospheres performed on a unique high-repetition-rate platform developed for the Large Plasma Device at the University of California, Los Angeles. The experiments utilize a high-repetition-rate laser to drive a fast plasma flow into a pulsed dipole magnetic field embedded in a uniform magnetized background plasma. 2D maps of the magnetic field with high spatial and temporal resolution are measured with magnetic flux probes to examine the evolution of magnetosphere and current density structures for a range of dipole and upstream parameters. The results are further compared to 2D particle-in-cell simulations to identify key observational signatures of the kinetic-scale structures and dynamics of the laser-driven plasma. We find that distinct 2D kinetic-scale magnetopause and diamagnetic current structures are formed at higher dipole moments, and their locations are consistent with predictions based on pressure balances and energy conservation.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Temporal evolution of the light emitted by a thin, laser-ionized plasma source
We present an experimental and simulation-based investigation of the temporal evolution of light emission from a thin, laser-ionized helium plasma source. We demonstrate an analytic model to calculate the approximate scaling of the time-integrated, on-axis light emission with the initial plasma density and temperature, supported by the experiment, which enhances the understanding of plasma light measurement for plasma wakefield accelerator (PWFA) plasma sources. Our model simulates the plasma density and temperature using a split-step Fourier code and a particle-in-cell code. A fluid simulation is then used to model the plasma and neutral density, and the electron temperature as a function of time and position. We then show the numerical results of the space-and-time-resolved light emission and that collisional excitation is the dominant source of light emission. We validate our model by measuring the light emitted by a laser-ionized plasma using a novel statistical method capable of resolving the nanosecond-scale temporal dynamics of the plasma light using a cost-effective camera with microsecond-scale timing jitter. This method is ideal for deployment in the high radiation environment of a particle accelerator that precludes the use of expensive nanosecond-gated cameras. Our results show that our models can effectively simulate the dynamics of a thin, laser-ionized plasma source. In addition, this work provides a detailed understanding of the plasma light measurement, which is one of the few diagnostic signals available for the direct measurement of PWFA plasma sources.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Super-resolved time–frequency measurements of coupled phonon dynamics in a 2D quantum material
Abstract Methods to probe and understand the dynamic response of materials following impulsive excitation are important for many fields, from materials and energy sciences to chemical and neuroscience. To design more efficient nano, energy, and quantum devices, new methods are needed to uncover the dominant excitations and reaction pathways. In this work, we implement a newly-developed superlet transform—a super-resolution time-frequency analytical method—to analyze and extract phonon dynamics in a laser-excited two-dimensional (2D) quantum material. This quasi-2D system, 1 T -TaSe 2 , supports both equilibrium and metastable light-induced charge density wave (CDW) phases mediated by strongly coupled phonons. We compare the effectiveness of the superlet transform to standard time-frequency techniques. We find that the superlet transform is superior in both time and frequency resolution, and use it to observe and validate novel physics. In particular, we show fluence-dependent changes in the coupled dynamics of three phonon modes that are similar in frequency, including the CDW amplitude mode, that clearly demonstrate a change in the dominant charge-phonon couplings. More interestingly, the frequencies of the three phonon modes, including the strongly-coupled CDW amplitude mode, remain time- and fluence-independent, which is unusual compared to previously investigated materials. Our study opens a new avenue for capturing the coherent evolution and couplings of strongly-coupled materials and quantum systems.
36 MATERIALS SCIENCE↗