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All sources NASA NTRS DOE OSTI

DOE OSTI2023

Offshore Geologic Carbon Storage (GCS) Inventory

The Offshore Geological Carbon Storage Inventory Web Map is an online web mapping application designed to help users explore and visualize the Offshore Geologic Carbon Storage Inventory. This dataset is an inventory of offshore geologic carbon storage (GCS) projects and studies, gathered to summarize ongoing GCS efforts taking place offshore globally. This inventory includes both actualized projects as well as characterization studies and aggregates a variety of attribute fields for each project / study. It is intended to be used for research and comparison purposes, see full disclaimer and credits.

Assessment↗

NASA NTRS2007

The Application of Metal Oxide Nanomaterials for Chemical Sensor Development

NASA Glenn Research Center (GRC) has been developing miniature chemical sensors for a variety of applications including fire detection, emissions monitoring, fuel leak detection, and environmental monitoring. Smart Lick and Stick sensor technology which integrates a sensor array, electronics, telemetry, and power into one microsystem are being developed. These microsystems require low power consumption for long-term aerospace applications. One approach to decreasing power consumption is the use of nanotechnology. Nanocrystalline tin oxide (SnO2) carbon monoxide (CO) sensors developed previously by this group have been successfully used for fire detection and emissions monitoring. This presentation will briefly review the overall NASA GRC chemical sensor program and discuss our further effort in nanotechnology applications. New carbon dioxide (CO2) sensing material using doped nanocrystalline SnO2 will be discussed. Nanocrystalline SnO2 coated solid electrolyte CO2 sensors and SnO2 nanorod and nanofiber hydrogen (H2) sensors operated at reduced or room temperatures will also be discussed.

Xu, Jennifer C.↗

DOE OSTI2022

Versatile soil gas concentration and isotope monitoring: optimization and integration of novel soil gas probes with online trace gas detection

Abstract. Gas concentrations and isotopic signatures can unveil microbial metabolisms and their responses to environmental changes in soil. Currently, few methods measure in situ soil trace gases such as the products of nitrogen and carbon cycling or volatile organic compounds (VOCs) that constrain microbial biochemical processes like nitrification, methanogenesis, respiration, and microbial communication. Versatile trace gas sampling systems that integrate soil probes with sensitive trace gas analyzers could fill this gap with in situ soil gas measurements that resolve spatial (centimeters) and temporal (minutes) patterns. We developed a system that integrates new porous and hydrophobic sintered polytetrafluoroethylene (sPTFE) diffusive soil gas probes that non-disruptively collect soil gas samples with a transfer system to direct gas from multiple probes to one or more central gas analyzer(s) such as laser and mass spectrometers. Here, we demonstrate the feasibility and versatility of this automated multiprobe system for soil gas measurements of isotopic ratios of nitrous oxide (δ18O, δ15N, and the 15N site preference of N2O), methane, carbon dioxide (δ13C), and VOCs. First, we used an inert silica matrix to challenge probe measurements under controlled gas conditions. By changing and controlling system flow parameters, including the probe flow rate, we optimized recovery of representative soil gas samples while reducing sampling artifacts on subsurface concentrations. Second, we used this system to provide a real-time window into the impact of environmental manipulation of irrigation and soil redox conditions on in situ N2O and VOC concentrations. Moreover, to reveal the dynamics in the stable isotope ratios of N2O (i.e., 14N14N16O, 14N15N16O, 15N14N16O, and 14N14N18O), we developed a new high-precision laser spectrometer with a reduced sample volume demand. Our integrated system – a tunable infrared laser direct absorption spectrometry (TILDAS) in parallel with Vocus proton transfer reaction mass spectrometry (PTR-MS), in line with sPTFE soil gas probes – successfully quantified isotopic signatures for N2O, CO2, and VOCs in real time as responses to changes in the dry–wetting cycle and redox conditions. Broadening the collection of trace gases that can be monitored in the subsurface is critical for monitoring biogeochemical cycles, ecosystem health, and management practices at scales relevant to the soil system.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

An assessment of controlled source EM for monitoring subsurface CO 2 injection at the wyoming carbonSAFE geologic carbon storage site

Here we evaluate if electromagnetic (EM) geophysical methods for monitoring geologic carbon storage (GCS) efforts at the Wyoming CarbonSAFE project adjacent to the Dry Fork Station power plant near Gillette, Wyoming. This first involved acquiring both electric and magnetic fields at eleven different locations ranging in distance from immediately adjacent to 4 km from the plant. Passive EM measurements were made to provide spectral EM noise measurements generated by electricity production at the plant and to determine if useful magnetotelluric (MT) data can be successfully collected in the region. The processed data indicate that useful MT data can be collected as long as the site is located more than 2km away from the power plant as well as active roads and rail lines. Controlled source EM data were collected using three different source configurations, two of which connected to steel casings used to complete the injection wells. Comparing the EM noise measurements to the CSEM data show measurable electric and magnetic field signals at all sites. Next a series of three-dimensional (3D) numerical models were built that simulate resistivity changes caused by the proposed CO2 injection at depths ranging from 2.4 to 3.0km. These models were used to simulate various EM measurement configurations. The modeling shows that casing-source CSEM monitoring can provide sensitivity to the injected CO 2 if source electrodes are connected to the bottom of one or both of the injection wells.

58 GEOSCIENCES↗

NASA NTRS2012

Seasonal Changes in Titan's Southern Stratosphere

In August 2009 Titan passed through northern spring equinox, and the southern hemisphere passed into fall. Since then, the moon's atmosphere has been closely watched for evidence of the expected seasonal reversal of stratospheric circulation, with increased northern insolation leading to upwelling, and consequent downwelling at southern high latitudes. If the southern winter mirrors the northern winter, this circulation will be traced by increases in short-lived gas species advected downwards from the upper atmosphere to the stratosphere. The Cassini spacecraft in orbit around Saturn carries on board the Composite Infrared Spectrometer (CIRS), which has been actively monitoring the trace gas populations through measurement of the intensity of their infrared emission bands (7-1000 micron). In this presentation we will show fresh evidence from recent CIRS measurements in June 2012, that the shortest-lived and least abundant minor species (C3H4, C4H2, C6H6, HC3N) are indeed increasing dramatically southwards of 50S in the lower stratosphere. Intriguingly, the more stable gases (C2H2, HCN, CO2) have yet to show this trend, and continue to exhibit their 'summer' abundances, decreasing towards the south pole. Possible chemical and dynamical explanations of these results will be discussed , along with the potential of future CIRS measurements to monitor and elucidate these seasonal changes.

Nixon, C. A.↗

NASA NTRSDate not supplied

SERVIR: Cross-Comparison of Carbon Emission Estimates Based on Variable Land Use Land Cover Changes within SERVIR Focus Regions

Deforestation in the tropics contributes approximately one-fifth of the annual global greenhouse gas (GHG) emissions. In an effort to reduce GHG emissions, SERVIR - a joint USAID and NASA initiative - is currently implementing the SERVIR CArbon Pilot (S-CAP) activity. By developing a comprehensive CO2 tracking system in Google Earth Engine based on both remotely sensed data and in situ observations, S-CAP aims to build capacity within the SERVIR regional hubs to improve decision making and local monitoring efforts surrounding GHG emissions. The S-CAP estimations are being completed throughout 11 pilot countries within the SERVIR regions of Asia, Africa, and the Americas to integrate partner contributions and local input into the development process. These emission estimate calculations use country-level REDD+ FREL reported values, global remotely sensed data (e.g. Global Forest Watch) and regional datasets and are completed using the IPCC Guidelines for National Greenhouse Gas Inventories. From the S-CAP activity thus far, country CO2 estimations had varied differences, ranging from 56% to 197% between their lowest and highest estimates. The results from this study show that CO2 emission estimates can differ greatly depending on the land cover data sets used as well as the biomass values, and how a comprehensive database is essential in understanding the full range of impacts that land cover change has in these regions. Using this ensemble approach, SERVIR hubs can better select the most appropriate datasets available for estimating emissions.

Carbon Emission↗

DOE OSTI2024

Dynamic changes in evapotranspiration, canopy photosynthesis and expansive growth in open field under rapid fluctuating radiation

Abstract In open fields, plants experience dynamic changes in environment, particularly radiation, temperature, wind, and humidity but their short-term responses have not been adequately characterized under natural conditions. In this study, we assessed causal effects of rapid radiation fluctuation on seven plant parameters in open fields of cotton and sweet corn canopies. The parameters are evapotranspiration ( ET ), canopy photosynthesis indicated by CO2 flux from air to canopy ( FCO2 ), sensible heat energy flux ( H ), canopy conductance for water vapor ( gcw ), canopy surface temperature ( Ts ), shoot and leaf elongation rate, and stem diameter change. The energy and CO2 fluxes were measured with Bowen ratio/energy balance/CO2 gradient (BREB+) technique, using averaging time of 5 min. Shoot + leaf elongation and stem diameter change were monitored with position transducers using averaging time of 1 min. All parameters were all found to respond to change in radiation and transpiration within minutes or sooner. While radiation effects on canopy gas exchanges are expected, illuminating are the indirect but immediate effects on shoot + leaf growth and stem diameter change through radiation effects on transpiration and plant water status. A novel finding is that gcw also responded within minutes or sooner to radiation fluctuations and that FCO2 was related almost linearly to gcw . Results are discussed in terms of soil-plant-atmosphere continuum, and interpreted in terms of dynamic interactions between transpiration and plant water status. The clear inverse relationship between ET and elongation rate or stem diameter changes provides additional evidence supporting the validity of 5-min averaging for the BREB + technique.

Hsiao, Theodore C.↗

DOE OSTI2023

Induced microseismicity and tremor signatures illuminate different slip behaviours in a natural shale fault reactivated by a fluid pressure stimulation (Mont Terri)

SUMMARY Fault slip induced by fluid perturbation in shale formations may only lead to a sparse seismicity. However, fault slip may strongly impact the integrity of shale formations that serve as caprocks for geological reservoirs holding buoyant fluids such as CO2, natural gas or hydrogen. A better understanding of the fluid reactivation processes of fault and the seismic triggering process is therefore critical for reservoir monitoring and fault stability. Here we analyse the seismic responses of a shale fault exposed to fluid pressurization during an in situ field-scale injection experiment at ∼340 m depth in the Mont Terri underground research laboratory (Switzerland). Two main types of seismic signals are observed as the fault was activated and started to slowly slip. After an aseismic phase, we observed tremor signatures and an increase in noise amplitude, which were directly associated with the slowly propagating fault slip in response to fluid injection. These signatures were later followed by micro-earthquakes that seem to occur further away from the fluid-pressurized area. We interpret these micro-earthquakes to be triggered by stress perturbations from the main slip growth. These two classes of seismic responses therefore highlight two different processes. Tremors seem to be a more direct observation for the fluid-induced slip propagation than micro-earthquakes. Even hidden in the noise, they precede earthquake failures, thus providing a useful tool for monitoring fluid leakage activated by slow deformation on low permeable shale faults, with applications for sealing integrity of caprocks.

De Barros, Louis (ORCID:0000000255419162)↗

NASA NTRS1975

Development of a laser Doppler system for the detection and monitoring of atmospheric disturbances

A Scanning Laser Doppler Velocimeter System (SLDVS) capable of detecting and monitoring atmospheric disturbances, including wake vortices of landing aircraft and vertical wind profiles in the atmosphere was developed. The SLDVS is a focused, continuous wave, CO2 system that determines the line-of-sight velocities of particles in the focal volume by measuring the Doppler shift created by these particles. At present, the SLDVS is designed to have a range coverage of approximately 2000 ft with a vertical angle coverage of approximately 60 deg. It is also designed to detect Doppler velocities of up to 200 ft/sec with a velocity resolution of approximately 1.8 ft/sec. A complete velocity spectrum is provided by the SLDVS at each point in space at which it is focused. The overall operation and performance of the system and the description of its individual components and data handling capabilities were given.

Jeffreys, H. B.↗

NASA NTRS1986

Closed culture plant studies: Implications for CELSS

Arabidopsis plants were grown in closed cultures similar to those used in space experiments. A shift in metabolism from photosynthesis to respiration is indicated by the accumulation of CO2 in the culture atmosphere. Reproductive growth is suppressed. Plant growth and development is apparently related to the atmospheric volume available to each plant. The implications of these findings to closed ecological systems are given: (1) there is a need for an open culture having ample gas exchange, (2) CO2 levels must be maintained within prescribed limits, (3) the minimum atmospheric volume required for each plant is dependent on the precision of the gas monitors and of the subsystems used to maintain appropriate levels of various atmospheric components, and (4) volatiles such as ethylene and terpenes emanating from plants be monitored and reduced to benign concentrations.

Hoshizaki, T.↗

NASA NTRS1988

Observations of interstellar HOCO(+) - Abundance enhancements toward the Galactic center

The 4(04)-3(03) and 1(01)-0(00) transitions of HOCO(+) toward several molecular clouds have been monitored. Of the molecular clouds considered, the HOCO(+) molecule has been detected only in Sgr B2 and Sgr A. The results suggest that gas phase CO2 is not a major carbon reservoir in typical molecular clouds. For Sgr B2, the column density of HOCO(+) at the northern peak is found to be about 3 x 10 to the 14th/sq cm, and a fractional abundance relative to H2 is obtained which is about 2 orders of magnitude greater than recent theoretical predictions.

Minh, Y. C.↗

NASA NTRS1991

Dynamics of low velocity collisions of ice particle, coated with frost

We continued our investigations of low velocity collisions of ice particles for velocities in range 10(exp -3) - 2 cm/s. The work focused on two effects: (1) the sticking forces for ice particles coated with CO2 frost, and (2) the completion of a 2-D pendulum system for glancing collisions. A new computer software was also developed to control and monitor the position of the 2-D pendulum.

Bridges, F.↗

DOE OSTI2024

Monitoring, Reporting, and Verification Considerations for Carbon Dioxide Removal

The project investigates Measurement, Reporting, and Verification (MRV) methods for Enhanced Weathering and Marine Carbon Dioxide Removal (mCDR) technologies. Enhanced Weathering accelerates natural mineral processes to capture CO2, while mCDR leverages oceanic processes for carbon sequestration. The study focuses on developing standardized MRV protocols, assessing environmental impacts, and evaluating the scalability and economic feasibility of these carbon sequestration methods. The goal is to ensure reliable and transparent data for validating and improving CO2 removal technologies.

Priyadarshini↗

NASA NTRS1976

Laser Doppler systems in pollution monitoring

The paper reports on a program undertaken to determine the feasibility of using a laser Doppler velocimeter (LDV) to measure smoke-stack gas exit velocity, particulate concentration, and mass flow. Measurements made with a CO2 laser Doppler radar system at a coal-burning power plant are compared with in-stack measurements made by a pitot tube. The operational principles of a LDV are briefly described along with the system employed in the present study. Data discussed include typical Doppler spectra from smoke-stack effluents at various laser elevation angles, the measured velocity profile across the stack exit, and the LDV-measured exit velocity as a function of the exit velocity measured by the in-stack instrument. The in-stack velocity is found to be about 14% higher than the LDV velocity, but this discrepancy is regarded as a systematic error. In general, linear relationships are observed between the laser data, the exit velocity, and the particulate concentration. It is concluded that an LDV has the capability of determining both the mass concentration and the mass flow from a power-plant smoke stack.

Miller, C. R.↗

DOE OSTI2025

Quantifying CO 2 Plume Stabilization at Carbon Storage Projects, North Dakota, USA

This study presents an approach for quantifying when injected carbon dioxide (CO 2 ) stabilizes pursuant to carbon capture and storage (CCS) project permitting and site closure requirements. The distribution of mobile-phase CO 2 (CO 2 plume) will evolve within the storage reservoir during and after injection through both physical and chemical trapping mechanisms. CCS policies generally agree that the CO 2 plume’s migratory behavior in post-injection should demonstrate nonendangerment to the environment but do not provide specific guidance on how to meet the definition of plume stabilization, generating some uncertainty for operators. Plume stability herein means the CO 2 plume 1) changes size minimally and predictably in the storage reservoir such that it will not cross key boundaries identified in the permit and 2) does not pose a threat to human health, underground sources of drinking water (USDWs), and the environment because of lateral migration to areas where leakage pathways may exist. Published literature on plume metrics was reviewed to determine which metric(s) may be most appropriate for determining CO 2 plume stability. A technical approach that defines plume stabilization by estimating the rate of change in the geographic footprint of the CO 2 plume with respect to time was developed and illustrated using a case study from North Dakota, USA, as a proposed solution for CCS operators to apply at the project permitting stage. Any prospective CCS operator may benefit from using the same approach to inform the selection of pore space lease and monitoring areas and develop post-injection site care plans.

03 NATURAL GAS↗

NASA NTRS2018

Overview of Solar-Induced Chlorophyll Fluorescence (SIF) from the Orbiting Carbon Observatory-2: Retrieval, Cross-Mission Comparison, and Global Monitoring for GPP

The Orbiting Carbon Observatory-2 (OCO-2), launched in July 2014, is capable of measuring Solar-Induced chlorophyll Fluorescence (SIF), a functional proxy for terrestrial gross primary productivity (GPP). Although its primary mission is to measure the column-averaged mixing ratio of CO2 (Xco(sub 2)) to constrain global carbon source/sink distribution, one of the OCO-2 spectrometers allows for a robust SIF retrieval solely based on solar Fraunhofer lines. Here we present a technical overview of the OCO-2 SIF product, aiming to provide the scientific community guidance on best practices for data analysis, interpretation, and application. This overview consists of the retrieval algorithms, OCO-2 specific bias correction, retrieval uncertainty evaluation, cross-mission comparison with other existing SIF products, and a global-scale examination of the SIF-GPP relationship. With the initial three years of data (September 2014 onward), we compared OCO-2 SIF with retrievals from Greenhouse Gases Observing Satellite (GOSAT) and Global Ozone Monitoring Experiment-2 (GOME-2), and examined its relationship with FLUXCOM and MODIS GPP datasets. Our results show that OCO-2 SIF, along with GOSAT products, closely resemble the mean spatial and temporal patterns of FLUXCOM GPP from regions to the globe. Compared with GOME-2, however, OCO-2 depicts a more realistic spatial contrast between the tropics and extra-tropics. The linear relationship between OCO-2 SIF and existing modeled GPP products diverges somewhat across biomes at the global scale, consistent with previous GOSAT or GOME-2 based findings when modeled GPP products were used, but in contrast to a consistent cross-biome SIF-GPP relationship obtained at flux tower sites with OCO-2 products. This contrast suggests a critical need to reconcile differences in diverse SIF and GPP products and the relationships among them. Overall, the OCO-2 SIF products are robust and valuable for monitoring the global terrestrial carbon cycle and for constraining the carbon source/sink strengths of the Earth system. Finally, insights are offered for future satellite missions optimized for SIF retrievals.

GPP↗

DOE OSTI2021

Lawrence Berkley National Laboratory Building 59

The building management system in Building 59 is monitoring and archiving building-level electricity usage, HVAC and lighting system states (e.g., setpoint, temperature, flow rate, pressure), indoor environmental conditions (air temperature, relative humidity, CO2), on-site weather (air temperature, relative humidity), and especially occupant counts as well as other metrics such as Wi-Fi signal. This dataset could support multiple use cases, such as model predictive control and occupant related demand management.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2021

Lawrence Berkley National Laboratory Building 59 (Raw)

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗