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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Investigation of the Production of Trifluoroacetic Acid from Two Halocarbons, HFC-134a and HFO-1234yf and Its Fates Using a Global Three-Dimensional Chemical Transport Model

Trifluoroacetic acid (TFA), a highly soluble and stable organic acid, is photochemically produced by certain anthropogenically emitted halocarbons such as HFC-134a and HFO-1234yf. Both these halocarbons are used as refrigerants in the automobile industry, and the high global warming potential of HFC-134a has promoted regulation of its use. Industries are transitioning to the use of HFO-1234yf as a more environmentally friendly alternative. In this work, we investigated the environmental effects of this change and found a 33-fold increase in the global burden of TFA from an annual value of 65 tonnes formed from the 2015 emissions of HFC-134a to a value of 2220 tonnes formed from an equivalent emission of HFO-1234yf. The percentage increase in surface TFA concentrations resulting from the switch from HFC-134a to HFO-1234yf remains substantial with an increase of up to 250-fold across Europe. The increase in emissions greater than the current emission scenario of HFO-1234yf is likely to result in significant TFA burden as the atmosphere is not able to disperse and deposit relevant oxidation products. The Criegee intermediate initiated loss process of TFA reduces the surface level atmospheric lifetime of TFA by up to 5 days (from 7 days to 2 days) in tropical forested regions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Mycorrhizal Distributions Impact Global Patterns of Carbon and Nutrient Cycling

Most tree species predominantly associate with a single type of mycorrhizal fungi, which can differentially affect plant nutrient acquisition and biogeochemical cycling. Uncertainties in mycorrhizal distributions are non-trivial, and current estimates disagree in up to 50% over 40% of the land area, including tropical forests. Remote sensing capabilities for mycorrhizal detection show promise for refining these estimates further. Here, we address for the first time the impact of mycorrhizal distributions on global carbon and nutrient cycling. Using the state-of-the-art carbon-nitrogen economics within the Community Land Model version 5, we found Net Primary Productivity (NPP) increased throughout the 21st century by 20%; however, as soil nitrogen has progressively become limiting, the costs to NPP for nitrogen acquisition—that is, to mycorrhizae—have increased at a faster rate by 60%. This suggests that nutrient acquisition will increasingly demand a higher portion of assimilated carbon to support the same productivity.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Effects of Improved Simulation of Precipitation on Evapotranspiration and Its Partitioning Over Land

Evapotranspiration (ET) is a key component of the global hydrological cycle, which is strongly modulated by the occurrence of different rainfall intensities. Global climate models (GCMs) commonly suffer from “too much light rain” and a negative bias in the ratio of transpiration (T) to ET (T/ET). It is unclear whether these biases are related. Here, in this work, we show that with the improved simulation of probability density functions of rainfall intensity by suppressing light-rain occurrence using a stochastic convection parameterization in the NCAR CESM1.2, the canopy T increases in tropical forests while evaporation from canopy interception and bare soil decreases. The simulated T/ET is increased by 2.5% globally and up to 8% regionally, primarily attributable to reduced fraction of wet leaves due to less frequent light rain despite its weak intensity. These results imply that excessive light rain is an important cause of the negative T/ET bias in GCMs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Characterizing the Atmospheric Mn Cycle and Its Impact on Terrestrial Biogeochemistry

Abstract The role of manganese (Mn) in ecosystem carbon (C) biogeochemical cycling is gaining increasing attention. While soil Mn is mainly derived from bedrock, atmospheric deposition could be a major source of Mn to surface soils, with implications for soil C cycling. However, quantification of the atmospheric Mn cycle, which comprises emissions from natural (desert dust, sea salts, volcanoes, primary biogenic particles, and wildfires) and anthropogenic sources (e.g., industrialization and land‐use change due to agriculture), transport, and deposition, remains uncertain. Here, we use compiled emission data sets for each identified source to model and quantify the atmospheric Mn cycle by combining an atmospheric model and in situ atmospheric concentration measurements. We estimated global emissions of atmospheric Mn in aerosols (<10 μm in aerodynamic diameter) to be 1,400 Gg Mn year −1 . Approximately 31% of the emissions come from anthropogenic sources. Deposition of the anthropogenic Mn shortened Mn “pseudo” turnover times in 1‐m‐thick surface soils (ranging from 1,000 to over 10,000,000 years) by 1–2 orders of magnitude in industrialized regions. Such anthropogenic Mn inputs boosted the Mn‐to‐N ratio of the atmospheric deposition in non‐desert dominated regions (between 5 × 10 −5 and 0.02) across industrialized areas, but that was still lower than soil Mn‐to‐N ratio by 1–3 orders of magnitude. Correlation analysis revealed a negative relationship between Mn deposition and topsoil C density across temperate and (sub)tropical forests, consisting with atmospheric Mn deposition enhancing carbon respiration as seen in in situ biogeochemical studies.

Environmental Sciences & Ecology↗
DOE OSTI2024

Sustained bacterial N 2 O reduction at acidic pH

Nitrous oxide (N 2 O) is a climate-active gas with emissions predicted to increase due to agricultural intensification. Microbial reduction of N 2 O to dinitrogen (N 2 ) is the major consumption process but microbial N 2 O reduction under acidic conditions is considered negligible, albeit strongly acidic soils harbor nosZ genes encoding N 2 O reductase. Here, we study a co-culture derived from acidic tropical forest soil that reduces N 2 O at pH 4.5. The co-culture exhibits bimodal growth with a Serratia sp. fermenting pyruvate followed by hydrogenotrophic N 2 O reduction by a Desulfosporosinus sp. Integrated omics and physiological characterization revealed interspecies nutritional interactions, with the pyruvate fermenting Serratia sp. supplying amino acids as essential growth factors to the N 2 O-reducing Desulfosporosinus sp. Thus, we demonstrate growth-linked N 2 O reduction between pH 4.5 and 6, highlighting microbial N 2 O reduction potential in acidic soils.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Evidence and attribution of the enhanced land carbon sink

Climate change has been partially mitigated by an increasing net land carbon sink in the terrestrial biosphere; understanding the processes that drive this sink is thus essential for protecting, managing and projecting this important ecosystem service. In this Review, we examine evidence for an enhanced land carbon sink and attribute the observed response to drivers and processes. This sink has doubled from 1.2 ± 0.5 PgC yr -1 in the 1960s to 3.1 ± 0.6 PgC yr -1 in the 2010s. This trend results largely from carbon dioxide fertilization increasing photosynthesis (driving an increase in the annual land carbon sink of >2 PgC globally since 1900), mainly in tropical forest regions, and elevated temperatures reducing cold limitation, mainly at higher latitudes. Continued long-term land carbon sequestration is possible through the end of this century under multiple emissions scenarios, especially if nature-based climate solutions and appropriate ecosystem management are used. In conclusion, a new generation of globally distributed field experiments is needed to improve understanding of future carbon sink potential by measuring belowground carbon release, the response to carbon dioxide enrichment, and long-term shifts in carbon allocation and turnover.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Synthesis of the land carbon fluxes of the Amazon region between 2010 and 2020

The Amazon is the largest continuous tropical forest in the world and plays a key role in the global carbon cycle. Human-induced disturbances and climate change have impacted the Amazon carbon balance. Here we conduct a comprehensive synthesis of existing state-of-the-art estimates of the contemporary land carbon fluxes in the Amazon using a set of bottom-up methods (i.e., dynamic vegetation models and bookkeeping models) and a top-down inversion (atmospheric inversion model) over the Brazilian Amazon and the whole Biogeographical Amazon domain. Over the whole biogeographical Amazon region bottom-up methodologies suggest a small average carbon sink over 2010-2020, in contrast to a small carbon source simulated by top-down inversion (2010-2018). However, these estimates are not significantly different from one another when accounting for their large individual uncertainties, highlighting remaining knowledge gaps, and the urgent need to reduce such uncertainties. Nevertheless, both methodologies agreed that the Brazilian Amazon has been a net carbon source during recent climate extremes and that the south-eastern Amazon was a net land carbon source over the whole study period (2010-2020). Overall, our results point to increasing human-induced disturbances (deforestation and forest degradation by wildfires) and reduction in the old-growth forest sink during drought.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Amazonian fog harbors viable microbes

Fog formation over tropical forests remains poorly characterized, despite its potential role in bioaerosol dispersion and ecosystem processes. Here, we analyzed fog samples collected at the Amazon Tall Tower Observatory using flow cytometry and culture-based techniques to characterize viable microbial communities. Microbial cell concentrations varied over an order of magnitude across 13 fog events, reaching up to 8 × 104 cells per ml of fog water. Flow cytometry consistently detected metabolically active cells, while culturing and mass spectrometry-based identification yielded eight viable bacterial species and seven fungal taxa. The bacteria Serratia marcescens, Ralstonia pickettii and Sphingomonas paucimobilis exhibited seasonal variations in prevalence. The fungal species identified were primarily mesophilic saprophytes and endophytes, commonly associated with soil and plant surfaces. Our findings indicate that fog harbors viable microbes, including Serratia marcescens and Ralstonia pickettii, which may imply a relevance of fog for microbial dispersal, colonization and nutrient cycling in the Amazon rainforest.

Godoi, Ricardo H. (ORCID:0000000247744870)↗
DOE OSTI2022

CO 2 fertilization of terrestrial photosynthesis inferred from site to global scales

Significance The magnitude of the CO 2 fertilization effect on terrestrial photosynthesis is uncertain because it is not directly observed and is subject to confounding effects of climatic variability. We apply three well-established eco-evolutionary optimality theories of gas exchange and photosynthesis, constraining the main processes of CO 2 fertilization using measurable variables. Using this framework, we provide robust observationally inferred evidence that a strong CO 2 fertilization effect is detectable in globally distributed eddy covariance networks. Applying our method to upscale photosynthesis globally, we find that the magnitude of the CO 2 fertilization effect is comparable to its in situ counterpart but highlight the potential for substantial underestimation of this effect in tropical forests for many reflectance-based satellite photosynthesis products.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

A review of trends and drivers of greenhouse gas emissions by sector from 1990 to 2018

Global greenhouse gas (GHG) emissions can be traced to five economic sectors: energy, industry, buildings, transport and AFOLU (agriculture, forestry and other land uses). In this topical review, we synthesize the literature to explain recent trends in global and regional emissions in each of these sectors. To contextualize our review, we present estimates of GHG emissions trends by sector from 1990 to 2018, describing the major sources of emissions growth, stability and decline across ten global regions. Overall, the literature and data emphasize that progress towards reducing GHG emissions has been limited. The prominent global pattern is a continuation of underlying drivers with few signs of emerging limits to demand, nor of a deep shift towards the delivery of low and zero carbon services across sectors. We observe a moderate decarbonization of energy systems in Europe and North America, driven by fuel switching and the increasing penetration of renewables. By contrast, in rapidly industrializing regions, fossil-based energy systems have continuously expanded, only very recently slowing down in their growth. Strong demand for materials, floor area, energy services and travel have driven emissions growth in the industry, buildings and transport sectors, particularly in Eastern Asia, Southern Asia and South-East Asia. An expansion of agriculture into carbon-dense tropical forest areas has driven recent increases in AFOLU emissions in Latin America, South-East Asia and Africa. Identifying, understanding, and tackling the most persistent and climate-damaging trends across sectors is a fundamental concern for research and policy as humanity treads deeper into the Anthropocene.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Solving the sample size problem for resource selection functions

Abstract Sample size sufficiency is a critical consideration for estimating resource selection functions (RSFs) from GPS‐based animal telemetry. Cited thresholds for sufficiency include a number of captured animals and as many relocations per animal N as possible. These thresholds render many RSF‐based studies misleading if large sample sizes were truly insufficient, or unpublishable if small sample sizes were sufficient but failed to meet reviewer expectations. We provide the first comprehensive solution for RSF sample size by deriving closed‐form mathematical expressions for the number of animals M and the number of relocations per animal N required for model outputs to a given degree of precision. The sample sizes needed depend on just 3 biologically meaningful quantities: habitat selection strength, variation in individual selection and a novel measure of landscape complexity, which we define rigorously. The mathematical expressions are calculable for any environmental dataset at any spatial scale and are applicable to any study involving resource selection (including sessile organisms). We validate our analytical solutions using globally relevant empirical data including 5,678,623 GPS locations from 511 animals from 10 species (omnivores, carnivores and herbivores living in boreal, temperate and tropical forests, montane woodlands, swamps and Arctic tundra). Our analytic expressions show that the required M and N must decline with increasing selection strength and increasing landscape complexity, and this decline is insensitive to the definition of availability used in the analysis. Our results demonstrate that the most biologically relevant effects on the utilization distribution (i.e. those landscape conditions with the greatest absolute magnitude of resource selection) can often be estimated with much fewer than animals. We identify several critical steps in implementing these equations, including (a) a priori selection of expected model coefficients and (b) regular sampling of background (pseudoabsence) data within a given definition of availability. We discuss possible methods to identify a priori expectations for habitat selection coefficients, effects of scale on RSF estimation and caveats for rare species applications. We argue that these equations should be a mandatory component for all future RSF studies.

Street, Garrett M.↗
DOE OSTI2020

A catastrophic tropical drought kills hydraulically vulnerable tree species

Drought-related tree mortality is now a widespread phenomenon predicted to increase in magnitude with climate change. However, the patterns of which species and trees are most vulnerable to drought, and the underlying mechanisms have remained elusive, in part due to the lack of relevant data and difficulty of predicting the location of catastrophic drought years in advance. In this work, we used long-term demographic records and extensive databases of functional traits and distribution patterns to understand the responses of 20–53 species to an extreme drought in a seasonally dry tropical forest in Costa Rica, which occurred during the 2015 El Niño Southern Oscillation event. Overall, species-specific mortality rates during the drought ranged from 0% to 34%, and varied little as a function of tree size. By contrast, hydraulic safety margins correlated well with probability of mortality among species, while morphological or leaf economics spectrum traits did not. This firmly suggests hydraulic traits as targets for future research.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2024

Role of Cell Wall Polysaccharides in Water Distribution During Seed Imbibition of Hymenaea courbaril L.

Seed water imbibition is critical to seedling establishment in tropical forests. The seeds of the neotropical tree Hymenaea courbaril have no oil reserves and have been used as a model to study storage cell wall polysaccharide (xyloglucan - XyG) mobilization.We studied pathways of water imbibition in Hymenaea seeds. To understand seed features, we performed carbohydrate analysis and scanning electron microscopy. We found that the seed coat comprises a palisade of lignified cells, below which are several cell layers with cell walls rich in pectin. The cotyledons are composed mainly of storage XyG. From a single point of scarification on the seed surface, we followed water imbibition pathways in the entire seed using fluorescent dye and NMRi spectroscopy. We constructed composites of cellulose with Hymenaea pectin or XyG. In vitro experiments demonstrated cell wall polymer capacity to imbibe water, with XyG imbibition much slower than the pectin-rich layer of the seed coat.We found that water rapidly crosses the lignified layer and reaches the pectin-rich palisade layer so that water rapidly surrounds the whole seed. Water travels very slowly in cotyledons (most of the seed mass) because it is imbibed in the XyG-rich storage walls. However, there are channels among the cotyledon cells through which water travels rapidly, so the primary cell walls containing pectins will retain water around each storage cell.The different seed tissue dynamic interactions between water and wall polysaccharides (pectins and XyG) are essential to determining water distribution and preparing the seed for germination.

arabinoxylan↗
DOE OSTI2021

Vismia guianensis leaf age physiology in Manaus, Brazil, from July 2014 - July 2015

This data package contains net photosynthesis rates and methanol and isoprene leaf emissions as a function of light, temperature, and leaf age. Data was collected from the species V. guianensis at the NGEE Tropics site in Manaus, Brazil (BR-Ma2). This data is used in the publication "Methanol and Isoprene Emissions from the Fast Growing Tropical Pioneer Species Vismia guianensis (Aubl.) Pers. (Hypericaceae) in the Amazon Basin." Isoprene (Is) emissions by plants represent a loss of carbon and energy resources leading to the initial hypothesis that fast growing pioneer species in secondary tropical forests allocate carbon primarily to growth at the expense of isoprenoid defenses. In this study, we quantified leaf isoprene and methanol emissions from the abundant pantropical pioneer tree species Vismia guianensis and ambient isoprene concentrations above a diverse secondary forest in the central Amazon. See the below field, Dataset References, for the full citation. Included in the data package is a zip file with six datasets, three in Excel format and additional versions in CSV format. Also included are the figures from the related publication.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Calibrated soil moisture data from Manaus, Brazil, August 2018 - December 2019

This dataset contains calibrated soil moisture and rainfall data for ecohydrological studies in the Central Amazon (2.6099 ºS, 60.2093 ºW) taken at 30-min intervals. Soil moisture data was collected at depths of 0.025-, 0.05-, 0.15-, 0.30-, 0.50-,0.8-, 1.6-, 2.4-, 3.2-, 4.8-, 6.4-, 8.8-, and 14.20 m. Inconsistent data was removed during the QA/QC process. Further information including data collection methods are available in the associated publication, Negron-Juarez et al. 2020. Measurement and characterization of soil moisture dynamics in a Central Amazonian tropical forest (to be submitted).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Raw tensiometer soil matric potential data, from Oct 2017-Jun 2020 in Manaus, Brazil

This data package contains raw output from two Campbell Scientific CR1000 data loggers each connected to three UMS T4e tensiometer sensors in Manaus, Brazil. Tensiometers at each data logger location were installed to depths of 10 cm, 20 cm and 50 cm below the ground surface for the purpose of measuring soil matric potential at each depth. “Station 3” tensiometers were installed at approximately 2°36'31.68"S, 60°12'34.70"W. “Station 4” tensiometers were installed at approximately 2°36'32.46"S, 60°12'34.92"W. The files “tensio3.edit.202109.csv” and “tensio4.edit.202109.csv” contain raw data (with invalid data removed). A text editor will be required to view the raw files in .csv (comma-separated values) format. Data processing was limited to: 1) Editing column headers for clarity; 2) Applying a correction that converts voltage read by the data loggers to pressure units (kPa); 3) removing all data greater than 50 kPa and less than -115 kPa; 4) Adding columns entitled “Caution.10cm”, “Caution.20cm” and “Caution.50cm” that contains values of either “NA” or “Caution”, the latter of which is applied when data exceeds the manufacturer reported data validity range of less than -85 kPa to suggest use of these data with caution; 5) Adding columns entitled “Invalid.10cm”, “Invalid.20cm”, and “Invalid.50cm” that contains values of either “NA” or “Invalid”, the latter of which is applied when data accuracy is deemed compromised due to the introduction of air bubbles into the instrument. Data marked “Invalid” may still indicate general trends of wet/high matric potential and dry/low matric potential, but values are inaccurate and dry/low matric potential values are likely not low enough. Wet/high matric potential values are likely to be more accurate than dry/low matric potential values; 6) Data format changed from .dat to .csv. This research was performed as a part of the NGEE Tropics project, which aims to advance model predictions of tropical forest carbon cycle responses to a changing climate over the 21st Century.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Leaf reflectance, leaf transmittance and sky irradiance, at four sites in Panama, 2022

Paired leaf reflectance and transmittance data measured in Panama, at the Parque Natural Metropolitano (PNM), on Barro Colorado Island (BCI), at the San Lorenzo canopy crane site (SLZ), and in Gamboa, Panama from January to April 2022. Measurements were made on leaves from 57 different tree, shrub and liana species, from sunlit canopy and understory locations. Bark reflectance was also measured on the trunks of common tree species at the PNM and SLZ sites. Also included are irradiance measurements and leaf area index (LAI) from eight vertical profiles at PNM. The aim of these data was to refine our understanding of vertical trait and environmental variation in tropical forests, and to improve models which can predict leaf traits from leaf contact spectral measurements. All spectral data and metadata are presented in .csv files and complete instrument output are included in .zip folders. Protocol details are provided as pdf documents. In addition to spectral data described here, some of these samples were also used for measurement of leaf gas exchange, carbon and nitrogen content, and leaf mass per unit leaf area (LMA) these data can be cross linked using the unique sample ID and are provided in separate related data packages.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Selected micrometeorological and soil data from the Manaus ZF2 K34 eddy covariance tower for the 2015/16 El Niño event

The K34 tower site (2.609 S, 60.209 W, 130 masl), located within the Tropical Silviculture Experimental Station (EEST, also known as ZF2) research station, in an area of undisturbed tropical forest (Araújo et al. 2002). It features long term measurements using micrometeorological, eddy covariance, and soil instrumentation, among others. This dataset covers January 2012 to December 2017, and includes air temperature (TA, ℃) and air relative humidity (RH, %), measured with thermohygrometers (HC2S3, Campbell Scientific, Logan, UT, USA) deployed above the canopy at the top of the tower (at 51.1 m height), and net radiation (NETRAD, W m-2) using an NR-LITE sensor (Kipp & Zonen, Delft, Netherlands), also at the top of the tower (at 35.0 m above the canopy). The soil moisture data included here is from a soil profile located approximately 12 m from the tower, and covers the period between February 2015 and September 2016. Volumetric soil water content (SWC, m3 m-3) measurements used Water Content Reflectometers (CS655 Campbell Scientific, Logan, UT, USA) at six depths: 10 cm, 20 cm, 30 cm, 40 cm, 60 cm, and 100 cm. Data are included in .csv files, and the text file ZF2-K34_Tower_headers.txt provides descriptions of data file headers.

54 ENVIRONMENTAL SCIENCES↗