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NASA NTRS1996

Stratospheric NO and NO2 Abundances from ATMOS Solar-Occultation Measurements

Using results from a time-dependent photochemical model to calculate the diurnal variation of NO and NO2, we have corrected Atmospheric Trace MOlecule Spectroscopy (ATMOS) solar-occultation retrievals of the NO and NO2 abundances at 90' solar zenith angle. Neglecting to adjust for the rapid variation of these gases across the terminator results in potential errors in retrieved profiles of approximately 20% for NO2 and greater than 100% for NC at altitudes below 25 km. Sensitivity analysis indicates that knowledge of the local 03 and temperature profiles, rather than zonal mean or climatological conditions of these quantities, is required to obtain reliable retrievals of NO and NO2 in the lower stratosphere. Extremely inaccurate 03 or temperature values at 20 km can result in 50% errors in retrieved NO or NO2. Mixing ratios of NO in the mid-latitude, lower stratosphere measured by ATMOS during the November 1994 ATLAS-3 mission compare favorably with in situ ER-2 observations, providing strong corroboration of the reliability of the adjusted space-borne measurements.

Newchurch, M. J.↗
NASA NTRS2000

Photochemical Modeling of CH3 Abundances in the Outer Solar System

Recent measurements of methyl radicals (CH3) in the upper atmospheres of Saturn and Neptune by the Infrared Space Observatory (ISO) provide new constraints to photochemical models of hydrocarbon chemistry in the outer solar system. The derived column abundances of CH3 on Saturn above 10 mbar and Neptune above the 0.2 mbar pressure level are (2.5 - 6.0) x 10(exp 13) / sq cm and (0.7 - 2.8) x 10(exp 13) / sq cm, respectively. We use the updated Caltech/Jet Propulsion Laboratory photochemical model, which incorporates hydrocarbon photochemistry, vertical molecular and bulk atmospheric eddy diffusion, and realistic radiative transfer modeling, to study the CH3 abundances in the upper atmosphere of the giant planets and Titan. We identify the key reactions that control the concentrations of CH3 in the model, such as the three-body recombination reaction, CH3 + CH3 + M yields C2H6 + M. We evaluate and extrapolate the three-body rate constant of this reaction to the low-temperature limit (1.8 x 10(exp -16) T(sup -3.75) e(sup -300/T), T < 300 K) and compare methyl radical abundances in five atmospheres: Jupiter, Saturn, Uranus, Neptune, and Titan. The sensitivity of our models to the rate coefficients for the reactions H + CH3 + M yields CH4 + M, H + C2H3 yields C2H2 + H2, (sup 1)CH2 + H2 yields CH3 + H, and H + C2H5 yields 2CH3, the branching ratios of CH4 photolysis, vertical mixing in the five atmospheres, and Lyman alpha photon enhancement at the orbit of Neptune have all been tested. The results of our model CH3 abundances for both Saturn (5.1 x 10(exp 13) / sq cm) and Neptune (2.2 x 10(exp 13) / sq cm) show good agreement with ISO Short Wavelength Spectrometer measurements. Using the same chemical reaction set, our calculations also successfully generate vertical profiles of stable hydrocarbons consistent with Voyager and ground-based measurements in these outer solar system atmospheres. Predictions of CH3 column concentrations (for p <= 0.2 mbar) in the atmospheres of Jupiter (3.3 x 10(exp 13) /sq cm), Uranus (2.5 x 10(exp 12) / sq cm), and Titan (1.9 x 10(exp 15) / sq cm) may be checked by future observations.

Lee, Anthony Y. T.↗
NASA NTRS1993

Elemental abundances in the upper solar atmosphere of quiet and coronal hole regions (Te is approximately equal to 4.3 x 10 exp 5 K)

Detailed examination of the sun's upper atmosphere reveals that elemental abundances vary between different solar regions. Some solar regions exhibit the well-established photospheric abundances, while in other regions the abundances of some elements diverge from photospheric by an order of magnitude, and perhaps even more. Elemental abundances in the solar wind (SW) are also different from elemental abundances in the photosphere. It is postulated that elemental abundances in the SW reflect the elemental abundances of their place of origin near the solar surface. The solar surface is covered, predominantly, by quiet and coronal hole regions. In this paper we measure the intensities of limb-brightening rings over quiet and coronal hole regions in lines of Mg VI and Ne VI (Te is approximately equal to 4.3 x 10 exp 5 K) and determine the relative elemental abundances of the features producing the rings. The rings are formed by a plasma component occupying only a small fraction of the immediate volume above the solar surface.

Feldman, U.↗
NASA NTRS1993

Abundance and composition of solar KR in the H3-H6 chondrite ACFER111

He/Ne, Ne/Ar, and Ar/Kr abundance ratios of solar gases extracted by stepped heating, stepped oxidation, and stepped etching of lunar and meteoritic regoliths are significantly lower than ratios measured directly or predicted by model estimates. Of these, the differences in the He/Ne and Ne/Ar ratios are explained to be owing to diffusive fractionation losses from the host minerals. In contrast, it remains controversial if the Ar/Kr and Kr/Xe ratios were fractionated prior to or after the implantation of the gases into the minerals. In the H3-H6 chondritic regolith breccia ACFER 111, measured He/Ne and Ne/Ar ratios appear to be of nearly unfractionated solar composition. The Ar/Kr ratio of ACFER 111, might thus be also unfractionated. We examined by stepped etching a metal sample of ACFER 111 and obtained an average solar 36Ar/84Kr = 3150 plus or minus 300 which is in agreement with the model predictions. The isotopic composition of solar Kr was observed to change in the course of the etching in a way very similar to that report for lunar ilmenites by the Zurich group. This can be interpreted as a change of the mixing ratio of Solar Wind (SW) and Solar Energetic Particles (SEP). The isotopic composition of the SEP component obtained from our Kr data, however, is distinct from that reported by the Zurich group.

Pedroni, A.↗
NASA NTRS1979

The isotopic and elemental abundances of neon nuclei accelerated in solar flares

The relative isotopic abundances of Ne-20 and Ne-22 in seven solar flares were determined from measurements of the satellite IMP 8, yielding the ratio Ne-20/Ne-22 = 7.7 (+2.3, -1.5) for solar chromospheric matter. This value is in agreement with the ratio for the component neon-A (the 'primordial' component) found in carbonaceous chondrites. An elemental abundance ratio Ne/O = 0.14 + or - 0.01 also has been obtained which agrees closely with earlier reported measurements. It is shown that the effects of preferential acceleration relative to solar-system abundances with increasing charge number observed for some solar flares - though biasing the elemental ratio - does not appear to influence the neon isotopic abundances.

Dietrich, W. F.↗
NASA NTRS1996

Stratospheric NO and NO(sub 2) Abundances from ATMOS Solar-Occultation Measurements

Using results from a time-dependent photochemical model to calculate the diurnal variation of NO and NO(sub 2), we have corrected Atmospheric Trace Molecule Spectroscopy (ATMOS) solar-occultation retrievals of the NO and NO(sub 2) abundances at 90 solar zenith angle. Neglecting to adjust for the rapid variation of these gases across the terminator results in potential errors in retrieved profiles of approx. 20 percent for NO(sub 2) and greater than 100 percent for NO at altitudes below 25 KM.

NO NO2 ATMOS↗
NASA NTRS2004

Elemental Abundance Variations Observed in Solar Energetic Particle Events During Solar Cycle 23

We report on observations of the abundances of elements from Helium to Nickel in over 50 different solar energetic particle events using the Solar Isotope Spectrometer (SIS) on-board the Advanced Composition Explorer (ACE) spacecraft. It had originally been expected that the energy spectra of different elements would show spectral roll-overs at energies related to the Q/M ratio of each element. Due to the partial stripping of Fe and essentially complete stripping of O, it was expected that the Fe/O ratio would be observed to decrease with increasing energy. While many events show this pattern, others have Fe/O which is constant with energy, while for yet others Fe/O actually increases with energy. Events having constant Fe/O could simply have their spectral breaks outside of the observed energy range. However, events which show increasing Fe/O cannot be explained within the framework of spectral breaks. Possible explanations include injection of remnant heavy ions from earlier impulsive events, hybrid Events consisting of a combination of flare-accelerated and shock-accelerated particles from a single solar event, and some new physical process in shock acceleration. We will report on efforts to distinguish these possible explanations.

vonRosenvinge, T. T.↗
NASA NTRS1983

Cosmic ray elemental abundances for Z = 26-42 measured on HEAO-3

An analysis is presented of 454 days of data from the Heavy Nuclei Experiment aboard the HEAO-3 satellite using an improved charge estimation algorithm is presented. A more precise normalization of Z = 32-42 abundances relative to iron is obtained, and more accurate detector response maps are used to recognize and reject a small class of events which was previously misidentified. The resulting abundances are in generally good agreement with solar system abundances with the first ionization potential (FIP) and with the Cameron solar system r-process (1982) with and without an applied FIP bias. The simplest interpretation of the results is that the cosmic ray source has solar system abundances modified by an FIP and/or volatility-dependent bias.

Binns, W. R.↗
NASA NTRS1975

Abundance of Fe relative to H at 1.5 solar radii

The abundance of Fe relative to H is obtained by using resonantly scattered intensities of lambda 284 of Fe XV that were measured with OSO-7 and resonantly scattered intensities of L-alpha of H I that were obtained by Gabriel (1971). Because of possible differences in electron densities along lines of sight for these non-simultaneous measurements and in relative calibrations, results are rather uncertain but still indicate that the average Fe abundance relative to H in the corona appears to be at least as large as a recent photospheric abundance. Some limitations in using this method for obtaining abundances are examined for future experiments with simultaneous measurements and well calibrated detectors.

Nakada, M. P.↗
NASA NTRS1975

Solar and galactic cosmic ray abundances - A comparison and some comments

We have compared the abundances of galactic cosmic rays at their source and solar cosmic-rays utilizing new data which includes the first determination of the abundances of Na and Al in the solar cosmic ray population. We find the relative abundances of the solar and galactic species to be identical within experimental error for 8 elements. One clear abundance difference exists for C. He and Fe have a variable solar cosmic ray abundance, and the unbiased abundance of both of these nuclei is also probably different than that in the galactic cosmic ray sources. We also have compared the cosmic ray abundances with solar system and solar atmospheric abundance determinations. We find an abundance ratio which depends on the first ionization potential for galactic cosmic rays; however, in addition, we find this same dependence on ionization potential for solar cosmic ray abundance ratios. The implications of this result are discussed.

Webber, W. R.↗
NASA NTRS1994

Elemental abundances of the B and A stars. 2: Gamma Geminorum, HD 60825, 7 Sextantis, HR 4817, and HR 5780

We extend fine analyses of the B and A stars, gamma Geminorum, 7 Sextantis, HR 4817, and HR 5780 using additional spectroscopic data from the Kitt Peak National Observatory (KPNO) coude feed telescope with a TI CCD, camera 5, and grating A, and ATLAS9 model atmospheres. In addition we study HD 60825, which had colors similar to the FHB A stars, but was found to be a Population I star. HD 60825, as is gamma Gem, is a sharp-lined early-A star with nearly solar derived abundances. HR 5780 and 7 Sex are also examples of stars which for the most part have solar abundances. The newly derived abundances for HR 4817 reveal important differences with respect to 53 Tau, a somewhat similar HgMn star.

Adelman, Saul J.↗
NASA NTRS1991

Relative abundances in the lower solar transition region

Properties of the lower solar transition region as determined from UV spectral lines recorded by the Naval Research Laboratory HRTS are investigated. The spectra were obtained from a rocket flight in July 1975. Variations of intensity ratios of strong lines of C IV, Si IV, C II, Si III, and O IV over the entire field of view of the HRTS instrument, which extends from disk center to the solar limb are discussed. The largest apparent abundance variations appear to be in the active regions surrounding a sunspot. The C/Si ratio is lower in the active regions than anywhere else in the instrument field of view, implying a lower C/Si abundance ratio in the active regions. There is a possible correlation of line intensity variation in the active region with Doppler shift of the lines; the explanation for this is unclear. The magnitude and reality of intensity ratio variations of all observed solar features are discussed, and monotonic center-to-limb intensity ratio variations due to the opacity of some of the spectral lines are measured.

Doschek, G. A.↗
NASA NTRS1982

The elemental and isotopic composition of galactic cosmic rays

Galactic cosmic rays represent samples of matter from areas outside the solar system. New information regarding the elemental composition of cosmic rays has been obtained in connection with the French-Danish experiment on HEA0-3 and recent balloon experiments. The energy dependence of the source composition is considered along with a comparison of cosmic ray and solar system abundances, and the N-14 source abundance. Attention is given to cosmic ray clocks and the Mn-54 problem, advances concerning cross section measurements, and cosmic ray isotopes. The considered new observations suggest that cosmic ray elemental abundance differences from the solar system continue to be ordered by atomic parameters such as first ionization potential, at least up through Z equals 40. The isotopic composition of the cosmic ray source is found to be unlike that of the solar system.

Mewaldt, R. A.↗
NASA NTRS1989

Nitrogen abundances from UV lines of HgMn and standard late-B stars

A recent survey by Roby (1987) discovered that the relatively weak high excitation lines of N 1 near 7468 and 8680 A were undetectable in the majority of HgMn stars, leading to upper limits on the N abundance of roughly ten times below that of the solar N abundance. Standard stars with similar temperatures (10,000 to 13,000 K) did exhibit these same N lines and were found to have roughly solar N abundances. The N abundances were redetermined in two HgMn stars and four standard stars using the strong, low excitation lines of N 1 found in the ultraviolet. The observational data consisted of high quality, high resolution, co-added International Ultraviolet Explorer spectra which was previously collected and reduced. Examination of the spectra plus considerations of signal/noise and severe line blending led to the choice of three promising N 1 lines located at 1742.7, 1745.3 and 1411.9 A. The atomic data for these lines were previously calculated using the best laboratory measurements found in a search of the relevant literature. The chosen N lines turned out to be blended significantly with Fe 2 lines. To obtain the abundances for N synthetic spectra were computed to match the observed spectra. The synthetic spectra were calculated using lie-blanketed model atmospheres, stellar parameters, and abundances for the other elements based upon previous work by S. Adelman. The N abundance was then adjusted to give the best fit of the observed line profiles. In the 2 HgMn stars, the N lines were again found to be undetectable, but the stronger intrinsic strength of the new lines yield more stringent upper limits than those obtained previously. Model atmosphere and abundances were updated in two stars where new results were reported. An additional N 1 line and an additional standard star were added to the program. A line opacity model was developed for a missing feature adjacent to the N 1 line at 1745.2 A, leading to a 25 percent improvement in the determined from this line.

Roby, Scott W.↗