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At least 361 records · Page 20

The quest to understand the fundamental structure of nuclear matter – outlook to QCD and the Electron-Ion Collider

Nuclear matter is made of quarks that are bound by gluons that also bind themselves. Unlike with the more familiar atomic and molecular matter, the interactions and structures in nuclear matter are inextricably mixed up, and observed properties of nucleons and nuclei, such as mass and spin, emerge out of this complex system. Ongoing and future QCD research offers the exciting prospect to obtain a multi-dimensional picture of the inner quark-gluon structure of protons and atomic nuclei and to inform us how the properties and structure of nuclear matter have emerged from the dynamics of QCD. This program is initiated at the 12-GeV Upgraded Jefferson Lab, concentrating on imaging the region in nucleon and nuclear structure where quarks prevail. A future Electron-Ion Collider (EIC) is planned at Brookhaven National Lab, in partnership with Jefferson Lab. The EIC will have a versatile range of beam energies, polarizations, and ion species, as well as high luminosity, to precisely image quarks, gluons, and their interactions in protons and complex atomic nuclei. The goal is an understanding of the internal structure of nuclear matter comparable to our knowledge of the electronic structure of atoms. The present status of the EIC will also be presented.

Ent, Rolf↗

Electroweak Currents from Chiral Effective Field Theory

Since the pioneering work of Weinberg, Chiral Effective Field Theory (EFT) has been widely and successfully utilized in nuclear physics to study many-nucleon interactions and associated electroweak currents. Here, nuclear EFT has now developed into an intense field of research and is applied to study light to medium mass nuclei. In this contribution, we focus on the development of electroweak currents from EFT and present applications to selected nuclear electroweak observables.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Mechanisms dominating thixotropy in limestone calcined clay cement (LC3)

Limestone calcined clay cement (LC3) is a green binder with great practical importance for the cement industry. Growing application has increased the need to understand the mechanisms governing its thixotropy for better control of workability. While formation of C-S-H bridges is understood to dominate the thixotropy of ordinary Portland cement, LC3 paste displayed unique thixotropy properties. In this study, focused beam reflectance measurement, zeta potential, 1H nuclear magnetic resonance relaxometry and micro X-ray computed tomography were used to track the colloidal interaction and hydration extent within LC3 paste. Results showed that flocculation due to the negative surface charge and water affinity of calcined clay appears to be the dominating factor. This leads to a reduction of water available to contribute to fluidity of the paste and, in turn, governing the development of thixotropy over time. In addition, the dilution effect due to high clinker substitution diminishes thixotropy growth with time.

36 MATERIALS SCIENCE↗

Ionization yield measurement in a germanium CDMSlite detector using photo-neutron sources

Two photo-neutron sources, Y 88 Be 9 and Sb 124 Be 9 , have been used to investigate the ionization yield of nuclear recoils in the CDMSlite germanium detectors by the SuperCDMS collaboration. In this study, we evaluate the yield for nuclear recoil energies between 1 and 7 keV at a temperature of ~ 50 mK . We use a geant4 simulation to model the neutron spectrum assuming a charge yield model that is a generalization of the standard Lindhard model and consists of two energy dependent parameters. We perform a likelihood analysis using the simulated neutron spectrum, modeled background, and experimental data to obtain the best fit values of the yield model. The ionization yield between recoil energies of 1 and 7 keV is shown to be significantly lower than predicted by the standard Lindhard model for germanium. There is a general lack of agreement among different experiments using a variety of techniques studying the low energy range of the nuclear recoil yield, which is most critical for interpretation of direct dark matter searches. This suggests complexity in the physical process that many direct detection experiments use to model their primary signal detection mechanism and highlights the need for further studies to clarify underlying systematic effects that have not been well understood up to this point.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Microscopic origin of reflection-asymmetric nuclear shapes

The presence of nuclear ground states with stable reflection-asymmetric shapes is supported by rich experimental evidence. Theoretical surveys of odd-multipolarity deformations predict the existence of pear-shaped isotopes in several fairly localized regions of the nuclear landscape in the vicinity of near-lying single-particle shells with Δℓ = Δj = 3. We analyze the role of isoscalar, isovector, neutron-proton, neutron-neutron, and proton-proton multipole interaction energies in inducing the onset of reflection-asymmetric ground-state deformations. The calculations are performed in the framework of axial reflection-asymmetric Hartree-Fock-Bogoliubov theory using two Skyrme energy-density functionals and density-dependent pairing force. We show that reflection-asymmetric ground-state shapes of atomic nuclei are driven by the odd-multipolarity neutron-proton (or isoscalar) part of the nuclear interaction energy. This result is consistent with the particle-vibration picture, in which the main driver of octupole instability is the isoscalar octupole-octupole interaction giving rise to large E3 polarizability. The necessary condition for the appearance of localized regions of pear-shaped nuclei in the nuclear landscape is the presence of parity doublets involving Δℓ = Δj = 3 proton or neutron single-particle shells. This condition alone is, however, not sufficient to determine whether pear shapes actually appear, and, if so, what the corresponding reflection-asymmetric deformation energies are. The predicted small reflection-asymmetric deformation energies result from dramatic cancellations between even- and odd-multipolarity components of the nuclear binding energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Forward doubly-virtual Compton scattering off an unpolarized deuteron in pionless effective field theory

In this work, we calculate the forward unpolarised doubly-virtual Compton scattering (VVCS) off the deuteron in the framework of pionless effective field theory, up to next-to-next-to-next-to-leading order (N3LO) for the longitudinal and next-to-leading order (NLO) for the transverse amplitude. The charge elastic form factor of the deuteron, obtained from the residue of the longitudinal VVCS amplitude, is used to extract the value of the single unknown two-nucleon one-photon contact coupling that enters the longitudinal amplitude at N3LO. We also study the lowest spin-independent generalised polarisabilities of the deuteron. The calculated unpolarised VVCS amplitude provides a high-precision model-independent input for a future calculation of the two-photon-exchange correction to the Lamb shift of muonic deuterium.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Vanadium spin qubits as telecom quantum emitters in silicon carbide

Solid-state quantum emitters with spin registers are promising platforms for quantum communication, yet few emit in the narrow telecom band necessary for low-loss fiber networks. Here, we create and isolate near-surface single vanadium dopants in silicon carbide (SiC) with stable and narrow emission in the O band, with brightness allowing cavity-free detection in a wafer-scale material. In vanadium ensembles, we characterize the complex d 1 orbital physics in all five available sites in 4H-SiC and 6H-SiC. The optical transitions are sensitive to mass shifts from local silicon and carbon isotopes, enabling optically resolved nuclear spin registers. Optically detected magnetic resonance in the ground and excited orbital states reveals a variety of hyperfine interactions with the vanadium nuclear spin and clock transitions for quantum memories. Last, we demonstrate coherent quantum control of the spin state. These results provide a path for telecom emitters in the solid state for quantum applications.

74 ATOMIC AND MOLECULAR PHYSICS↗

Pellet Cladding Interaction In-Reactor Ramp Testing in a World without the Halden Boiling Water Reactor

One of the most crucial performance areas for fuel rods in water cooled nuclear power plants is interaction between cladding tubes and fuel pellets. Experimental programs in test reactors have provided key data to help fuel developers and plant operators understand Pellet Cladding Interaction (PCI) phenomena and optimize their strategies for reliable fuel performance. Approximately 50 years of “ramp” testing programs, where the fission heating rate is deliberately manipulated in test rods, have been performed in a handful of test reactors to reveal and understand PCI behaviors such as iodine-assisted stress corrosion cracking. Unfortunately, the test reactors most engaged in this type of work have all been retired over the years up to the recent and unexpected closure of the Halden Boiling Water Reactor which effectively caused a hiatus in PCI ramp testing programs. The need for ramp testing is crucial at this time to enable refined PCI understanding as more plants consider implementing flexible operations, increased fuel rod burnup limits, and new fuel technologies with enhanced accident tolerance. This paper reviews some of the key PCI phenomena that must be addressed with in-pile testing and surveys past test reactor’s methods for achieving the needed conditions. A strategic approach is then presented using test reactors and complimentary facilities which are still available today. Near term data opportunities are put forth along with capability development strategies that will ensure future longevity in this field of research.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Λ Baryon Production in ν¯µ Interactions in the MicroBooNE Detector

The Cabibbo suppressed production of $\Lambda$ baryons in anti-neutrino interactions with nuclei is a rare process that is yet to be measured with a modern neutrino detector with automated reconstruction. The cross section for this process is sensitive to a number of unique nuclear effects, most notably the secondary interactions of the produced hyperon while attempting to escape from the nucleus. Other interactions within the nuclear remnant can impact the estimation of neutrino energy in oscillation measurements, and thus an accurate description of the nuclear environment is required. The strangeness violating hyperon production process is only available to anti-neutrinos. The model of this interaction is implemented into the NuWro neutrino interaction Monte Carlo simulation, and some predictions are presented, focusing on the role of nuclear effects. This model introduces a hyperon-nucleus potential, which calculations from hypernuclear theory permit to be strongly repulsive in th e case of $\Sigma$ baryons. The presence of this potential is found to sculpt the shape of the differential cross section in some variables. The MicroBooNE detector will be described, followed by a description of a measurement of the flux averaged, restricted phase space cross section of Cabibbo suppressed $\Lambda$ baryon production. A sophisticated event selection is employed, as a very large quantity of background neutrino interactions must be removed to perform the measurement with any sensitivity. This selection introduces some novel techniques such as the island finding method, and achieves a background reduction of $\sim 10^6$, with an efficiency of around 7\%. The calculation of the systematic uncertainties will be explained, including two procedures explored to handle sources of background with extremely poor simulation statistics: an in-situ constraint using data from sidebands, and a visual inspection of the data and simulation to remove the troublesome background events. The sensitivity to the $\Lambda$ baryon production cross section is calculated in the form of Bayesian posterior probability distributions, combining the systematic uncertainties with data and simulation statistical uncertainties. As a rare process, the statistical uncertainties are highly non-Gaussian, and the Bayesian approach is applied to include the full shapes of these uncertainties. Data corresponding to $2.2 \times 10^{20}$ protons on target of neutrino mode running and $4.9 \times 10^{20}$ protons on target of anti-neutrino running is analysed. When the data was unblinded, five $\Lambda$ production candidates were selected from the data, consistent with the MC simulation prediction of $5.3 \pm 1.1$ events. The final estimated cross section is $1.8^{+2.0}_{-1.6} \times 10^{-40}$cm$^2/$Ar when employing the sideband constraint procedure. A similar result of $2.0^{+2.2}_{-1.8} \times 10^{-40}$cm$^2/$Ar is obtained when performing the visual scan instead. The methods used in t his analysis are intended to be easily exported to other LArTPC detectors such as the Short Baseline Near Detector.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Approach to using 3D laser-induced breakdown spectroscopy (LIBS) data to explore the interaction of FLiNaK and FLiBe molten salts with nuclear-grade graphite

Nuclear graphite has historically been a key component of many nuclear reactor designs and has emerged as key to numerous advanced nuclear reactor design concepts. Molten salt reactors (MSRs) are one broad group of advanced reactor designs currently being pursued by industry for commercialization. Several MSR designs under consideration use graphitic materials that directly interface with a molten salt, whether it is a fuel salt, coolant salt, or both. Therefore, the interaction of graphite materials with molten salts must be understood. To gain this required understanding, a range of data is needed including porosity, strength, and composition as a function of different salt exposure parameters. In this study, a laser-induced breakdown spectroscopy (LIBS) measurement and data analysis methodology was developed to obtain spatially resolved elemental composition information for graphite samples exposed to a molten fluoride salt. Traditional univariate emission line analysis of atomic, ionic, and molecular optical emission signals was coupled via correlation analysis with spectral decomposition of the data using principal component analysis. Elemental depth profiling and elemental mapping were also performed to visualize salt–graphite interactions. LIBS was demonstrated to be useful for measuring key analytes such as fluorine and hydrogen, which are troublesome for other analysis techniques. Evidence for complex behavior was found, thereby demonstrating the usefulness of the developed approach for future systematic studies.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Measurements of W + W − production cross-sections in pp collisions at $\sqrt{s}=13$ TeV with the ATLAS detector

Measurements of W + W − → e ± νμ ∓ ν production cross-sections are presented, providing a test of the predictions of perturbative quantum chromodynamics and the electroweak theory. The measurements are based on data from pp collisions at $\sqrt{s}$ = 13 TeV recorded by the ATLAS detector at the Large Hadron Collider in 2015–2018, corresponding to an integrated luminosity of 140 fb −1 . The number of events due to top-quark pair production, the largest background, is reduced by rejecting events containing jets with b-hadron decays. An improved methodology for estimating the remaining top-quark background enables a precise measurement of W + W − cross-sections with no additional requirements on jets. The fiducial W + W − cross-section is determined in a maximum-likelihood fit with an uncertainty of 3.1%. The measurement is extrapolated to the full phase space, resulting in a total W + W − cross-section of 127 ± 4 pb. Differential cross-sections are measured as a function of twelve observables that comprehensively describe the kinematics of W + W − events. The measurements are compared with state-of-the-art theory calculations and excellent agreement with predictions is observed. A charge asymmetry in the lepton rapidity is observed as a function of the dilepton invariant mass, in agreement with the Standard Model expectation. A CP-odd observable is measured to be consistent with no CP violation. Limits on Standard Model effective field theory Wilson coefficients in the Warsaw basis are obtained from the differential cross-sections.

Accelerator Physics↗

Corrosion interactions between stainless steel and lead vanado-iodoapatite nuclear waste form part II

This paper studied the release of iodine from lead vanado-iodoapatite (I-APT, Pb 9.85 (VO 4 ) 6 I 1.7 ), a potential nuclear waste form for the radioactive waste element of I-129, which can be enhanced when crevice corrosion of stainless steel (SS) occurring nearby. Reference corrosion studies of I-APT were performed in different bulk solutions including DI water, 0.6 M and 6 M NaCl, and 0.1 M HNO 3 without metal crevice corrosion interactions. The localized enrichment of Cl – , one of the major consequences of SS crevice corrosion, was found to be the decisive factor that led to the enhanced release of iodine. A surface alteration layer consisting of a mixture of nanocrystalline I-APT and Cl-rich apatite (Cl-APT) formed on I-APT surface. Meanwhile, large Cl-APT crystals formed at the crevice mouth on the I-APT surface. This study reveals a new near-field corrosion mechanism for ceramic waste forms when they are exposed to aggressive local corrosive conditions created by the electrochemical reactions of nearby metals. The insight gained in this study could be beneficial for a more accurate prediction of waste form degradation.

36 MATERIALS SCIENCE↗

Data-driven reevaluation of f t values in superallowed β decays

We present a comprehensive reevaluation of the ft values in superallowed nuclear β decays crucial for the precise determination of V ud and low-energy tests of the electroweak standard model. It consists of the first, fully data-driven analysis of the nuclear β decay form factor, that utilizes isospin relations to connect the nuclear charged weak distribution to the measurable charge distributions. This prescription supersedes previous shell-model estimations, and allows for a rigorous quantification of theory uncertainties in f which is absent in the existing literature. Furthermore, our new evaluation shows an overall downward shift of the central values of f at the level of 0.01%.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Isospin symmetry breaking in the mirror pair 73 Sr- 73 Br

The recent experimental observation of isospin symmetry breaking (ISB) in the ground states of the T=3/2 mirror pair 73 Sr- 73 Br is theoretically studied using large-scale shell-model calculations. The large valence space and the successful PFSDG-U effective interaction used for the nuclear part of the problem capture possible structural changes and provide a robust basis to treat the ISB effects of both electromagnetic and nonelectromagnetic origin. The calculated shifts and mirror-energy differences are consistent with the inversion of the I π =1/2 - ,5/2 - states between 73 Sr- 73 Br and suggest that the role played by the Coulomb interaction is dominant. Finally, an isospin breaking contribution of nuclear origin is estimated to be ≈25keV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

First nuclear ultraheavy dark matter search in argon time projection chambers with the DarkSide-50 experiment

We report on the first search for nuclear ultraheavy dark matter (UHDM) in a dual-phase liquid argon time projection chamber using the DarkSide-50 experiment. Unlike conventional weakly interacting massive particles, a nuclear UHDM model may be composed of many dark nucleons and scatter numerous times while passing through the detector. Accounting for energy loss through the Earth’s overburden, we apply selection criteria optimized for multiscatter event topologies using the 532-day low-radiation campaign of the DarkSide-50 detector. Excluded limits on the UHDM-nucleon scattering cross section for dark nucleon masses of m χ = 10 , 50 , 100 , 500 GeV / c 2 are presented.

Agnes, P. [GSSI, Aquila; Gran Sasso]↗

Establishing the ground-state spin of 71 Kr

Nuclei in the vicinity of the N=Z line provide many sensitive probes of isospin symmetry. One example concerns the character and sequence of low-lying states of the T=1/2 mirror pair 71 Kr and 71 Br which has been under debate for several decades. In this paper we report a new measurement of the absolute β-branching to ground and excited states which, taken with our precise lifetime of T 1/2 =94.9(4) ms , gives a superallowed ground state–to–ground state log (ft) value of 3.64(4). This is only consistent with both 71 Br and 71 Kr having the same spin and parity, J π =5/2 – , as expected from mirror symmetry. The β-delayed proton emission to the first-excited state in 70 Se was observed for the first time which also strongly supports this assignment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Urca Cooling in Neutron Star Crusts and Oceans: Effects of Nuclear Excitations

We report the excited-state structure of atomic nuclei can modify nuclear processes in stellar environments. In this Letter, we study the influence of nuclear excitations on Urca cooling (repeated back-and-forth β decay and electron capture in a pair of nuclear isotopes) in the crust and ocean of neutron stars. We provide for the first time an expression for Urca process neutrino luminosity which accounts for a thermal Boltzmann distribution of excited states in both members of an Urca pair. We use our new formula with state-of-the-art nuclear structure inputs to compute neutrino luminosities of candidate Urca cooling pairs. Our nuclear inputs consist of the latest experimental data supplemented with calculations using the projected shell model. We show that, in contrast to previous results that only consider the ground states of both nuclei in the pair, our calculated neutrino luminosities for different Urca pairs vary sensitively with the environment temperature and can be radically different from those obtained in the one-transition approximation. We find that nuclear excitations can lead to an enhancement in total Urca neutrino luminosities in the accreted neutron star crust by about 5 times as compared with the previous Urca results, which is expected to cause significant observational effects.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Examination of Solvent- Room Temperature Ionic Liquid Interactions using 2D NMR and Computational Chemistry

Rare earth metals (REMs) are the key functioning material found in microelectronics, advanced batteries, and high-efficiency electrical motors. Current methods for producing REMs require high temperatures (i.e. energy intensive) and produce an abundance of hazardous fluoride waste. Room temperature ionic liquids (RTILs) are an ideal alternative electrolyte because they allow for a low-temperature, energy-efficient electrochemical process. RTIL properties such as viscosity and conductivity determine how effective they can be in this process. Since viscosity is directly related to both intra and intermolecular forces, this study sets out to investigate two RTILs-Trihexyltetradecylphosphonium dicyanamide (Cyphos 105) and Trihexyltetradecylphosphonium bistrifimide (Cyphos 109) and their interactions. Results from 2-dimensional nuclear magnetic resonance (2D NMR) spectroscopy show that there is an interaction between the tetradecyl tail and the phosphorus atom of the Cyphos RTIL. In order to establish whether this is an intra or an inter-molecular interaction, DFT-based computational calculations were performed to determine the optimized geometry. Calculations were done both in the gas phase and with propylene carbonate as an augmenting solvent. Preliminary results show that there is minimal intramolecular interaction between the tetradecyl tail and the phosphorus atom of the RTILs, and that the interaction seen in the 2D NMR experiment is likely of an intermolecular nature instead.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗