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At least 361 records · Page 20

A Safer Nuclear Enterprise - Application to Nuclear Explosive Safety (NES)(U)

Activities and infrastructure that support nuclear weapons are facing significant challenges. Despite an admirable record and firm commitment to make safety a primary criterion in weapons design, production, handling, and deployment - there is growing apprehension about terrorist acquiring weapons or nuclear material. At the NES Workshop in May 2012, Scott Sagan, who is a proponent of the normal accident cycle, presented. Whether a proponent of the normal accident cycle or High Reliability Organizations - we have to be diligent about our safety record. Constant vigilance is necessary to maintain our admirable safety record and commitment to Nuclear Explosive Safety.

ACCIDENTS↗

The U.S. Nuclear Waste Technical Review Board Intern Program: Developing Next Generation Nuclear Waste Professionals - 16102

The U.S. Nuclear Waste Technical Review Board (Board) created an internship program in the fall of 2013 for undergraduate and graduate students interested in management and disposal of spent nuclear fuel and high-level radioactive waste. Interns must select a project topic in a technical area related to the Board's mission and prepare a well-supported briefing for the agency. The ability to review technical and scientific information in a critical and unbiased manner is essential for completion of the intern's project and this is a particular focus of the interaction between the mentor and the intern. The interns from 2014 and 2015 selected and reviewed topics related to the areas of commingling waste forms for disposal and deep borehole disposal. In addition to the technical project, interns acquire a broad perspective of the federal agencies involved in managing and disposing of radioactive waste while participating in inter-agency networking opportunities. In this review of the Board internship experience, two past interns discuss the personal impact of the program and how they believe the experience prepared them to face the challenges of a career in management and disposal of spent nuclear fuel and high-level radioactive waste. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Optimization of a dry, mixed nuclear fuel storage array for nuclear criticality safety - 14339

A dry storage array of used nuclear fuel at the Idaho National Laboratory contains a mixture of more than twenty different types of research and test reactor fuels. Significant neutronic interaction occurs between fuel canisters within this large storage arrangement of 636 fuel storage canisters. Nuclear criticality safety is maintained primarily by moderation control and through control of neutron interaction and leakage provided by the credited geometry. Over the nearly forty years of operation the collected fuels are now arranged in a configuration that does not minimize the system neutron multiplication factor (k{sub eff}). This creates a concern since the entire remaining facility storage capacity cannot be utilized without exceeding the system minimum subcritical state (k{sub safe}) for ensuring nuclear criticality safety. This work determines a more optimal arrangement for the stored fuels with a goal to minimize the system k{sub eff}, but also with a minimum of potential fuel canister relocation movements. The ultimate goal is to establish a solution for this multiple-objective optimization problem by finding the Pareto Front for maximum k{sub eff} reduction versus the number of canister relocations. The process first required additional analysis of the array by Monte-Carlo neutron transport codes (specifically, MCNP) to gain a greater understanding of the interaction characteristics of the disparate fuel types. Some stored fuels are composed of primarily metallic and oxide components that provide very little inherent moderation, while other fuel types contain graphite or zirconium-hydride which can contribute a significant amount of moderation. These factors cause a complex relationship within a fuel arrangement with respect to thermal utilization and axial leakage probability. The new MCNP analysis was utilized to develop a simplified spreadsheet-based empirical model which simulates the array k{sub eff} result. This empirical model was benchmarked against additional MCNP calculations for various arrangements and then employed in the optimization analysis. A Tabu metaheuristic and stochastic approximation optimization was applied to the empirical model with the optimization function to minimize the array k{sub eff}. The optimization algorithm interrogated the empirical model to determine the optimal rearrangement for up to sixty canister movements. The Pareto Front was found, which shows that a limited number of canister relocation movements could allow the existing thirty-one empty array positions to be filled with common research reactor fuels while also yielding a reduction in the overall array k{sub eff} relative to the current arrangement. This will impart an improvement in the facility utilization while also offering an enhancement in the safety margin. The reduction in array reactivity has been confirmed by a final set of MCNP calculations with the proposed new arrangements. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Intern Poster Session 08/13: Autonomous Nuclear Robotics: Applications in nuclear waste inspection and hot cell experiments

The nuclear industry is experiencing renewed interest in autonomous robotics, yet most deployed systems remain teleoperated with limited autonomy. This work presents two contributions toward fully autonomous nuclear robotic systems: autonomous waste inspection at the Hanford Site and an autonomous hot cell laboratory framework. Inspections of Hanford's underground waste storage tanks are performed manually at significant cost and personnel exposure. We developed a reinforcement-learning (RL) training pipeline for a custom-built inspection arm. In parallel, we are designing an autonomous laboratory framework for post-irradiation examination in hot cells at the Specimen Preparation Laboratory (SPL) that integrates computer vision, task and motion planning, hardware execution, and operator-in-the-loop control. These systems demonstrate a path toward safer, more efficient nuclear operations by reducing human exposure while maintaining rigorous human oversight at critical decision points.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High-Activity Microscopic Nuclear-Sourced Particles to Investigate Nuclear Release Scenarios - 18026

Advances in microscopy and materials analysis have allowed for the study of materials at resolutions not previously attainable a decade ago. Such information extends to not only their existence, but also their composition, the likely source term and if applicable, their short or long-term environmental stability. This work describes the analysis undertaken on the larger 'ejecta' type of particulate collected following the INES Level 7 incident at the Fukushima Daiichi Nuclear Power Plant in March 2011. However, the methods and procedures employed during this work, on material with enormously contrasting characteristics, have far wider applications within nuclear forensics, safeguards, security and material compliance. Resulting from the analysis of micron-scale 'atmospheric' material in previous works have been able to derive information relating to the emission and subsequent transportation characteristics of the release event, as well as determining the local-scale impacts of this radioactive fallout. This analysis of the larger-scale (100's of micron) 'ejecta' material, collected from closer to the plant, has been able to reveal details pertaining to the specific in-reactor conditions at the time of the release as well as the nature of the explosion events. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Nuclear Data Sheets for A = 230

The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reactions for all isobars with mass number A=230. This evaluation includes the first experimental evidence of 230Am, produced through the 197Au(40Ar,3n)234Bk (α decay to 230Am) reaction, E(40Ar)=188.4 MeV (2003MoZX).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data Sheets for A = 215

The evaluated spectroscopic data are presented for 12 known nuclides of mass 215 (Hg, Tl, Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa). For {sup 215}Hg, {sup 215}Tl, {sup 215}Pb, and {sup 215}Pa nuclei, no excited states are known. The decay characteristics of {sup 215}Hg and {sup 215}Tl are unknown. The decay scheme of {sup 215}Pb is considered as incomplete. Ordering of γ cascades in the decay of 36.9–s isomer of {sup 215}Bi and for high–spin states above 2251 keV in {sup 215}Fr are not established. High–spin excitations, including several isomeric states, are well known in {sup 215}Bi, {sup 215}Po, {sup 215}Rn, {sup 215}Fr, {sup 215}Ra, and {sup 215}Ac. No particle–transfer reaction data are available for any of the A=215 nuclei. The rms charge radii for {sup 215}Pb, {sup 215}Bi, {sup 215}Po, {sup 215}Rn, {sup 215}Fr and {sup 215}Ra have been evaluated by Daniel Abriola, from extrapolation or interpolation of available evaluated data in 2013An02 for radii of respective Z chains using formula 9 in 2004An14. This evaluation was carried out as part of ENSDD–workshop at VECC, Kolkata for Nuclear Structure and Decay Data, organized and hosted by VECC and Board of Research in Nuclear Sciences (BRNS) in Kolkata, India, November 26–29, 2012. This work supersedes the previous A = 215 evaluation (2001Br31) published by E. Browne which covered literature prior to May 2001.

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Nuclear Data Sheets for A = 148

The experimental nuclear structure data available through October 2013 have been reviewed. A summary of information obtained in various reaction and decay experiments is presented, together with adopted level schemes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data Sheets for A = 239

Spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented here for all nuclei with mass number A=239. In general, a relatively small amount of new data on this mass chain has been reported since the previous evaluation in 2003. However, special evaluations, such as ''Database of prompt gamma rays from slow neutron–capture from elemental analysis'' (2007ChZX), have provided additional precise data for levels in 29 U. Also, new Coulomb excitation measurements in 239 Pu have extended the knowledge of the 1/2[631] rotational band up to Jπ=(55/2+)Jπ=(55/2+), and that of the octupole vibrational band up to Jπ=(53/2-)Jπ=(53/2-). For historical knowledge it is worth mentioning the report on the “Discovery of isotopes of the transuranium elements with 93 <= Z <= 98'' (2013Fr02), where the information for elements Np, Pu, Am, and Cf with mass number A=239 is presented. The alpha hindrance factors (HF) presented in this evaluation were calculated using values of the radius parameter (r 0 ) interpolated from those for even–even adjacent nuclei given by 1998Ak04.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data Sheets for A=73☆

Experimental nuclear structure data for the known A=73 isobaric nuclides (Mn, Fe, Co, Ni, Cu, Zn, Ga, Ge, As, Se, Br, Kr, Rb and Sr) have been evaluated, and presented together with Adopted properties of level energies, and associated γ rays. The decay data for these nuclides have also been evaluated, providing Adopted values of γ and β radiations, and log ft values. For {sup 73}Mn, only the isotopic identification has been established, with no knowledge of its g.s. half-life. For {sup 73}Fe, {sup 73}Co and {sup 73}Sr, only the ground states and their half-lives are known with no information about the excited states. For {sup 73}Ni, {sup 73}Cu, {sup 73}Zn and {sup 73}Rb, little data are available for excited states. The half-life and decay modes of possibly proton-unbound {sup 73}Rb need firmly established. {sup 73}Ga structure presents a special challenge in that the 1/2{sup −} ground state and the first 3/2{sup −} state have recently been proposed, in a Coulomb excitation experiment by 2010Di14, to form an almost degenerate doublet with an estimated spacing of 229 Th with its first excited state at 7.8 eV, and {sup 235}U with its first excited state at 76 eV. Ultra-high resolution gamma-ray spectroscopic studies are warranted to search for the low-lying (73 Ga, and to determine its half-life. Level structures of {sup 73}Ga, {sup 73}Ge, {sup 73}As, {sup 73}Se, {sup 73}Br and {sup 73}Kr are quite well known, although decay schemes of radioactive ground states of {sup 73}Co, {sup 73}Cu and {sup 73}Br are considered incomplete. The reactions and decays for which no new experimental information has become available since the 2003 update have undergone revisions to incorporate conversion coefficients from BrIcc code, and evaluated Q values from 2017Wa10, but essential content of such datasets may have remained the same as in previous evaluations. In this respect the present work greatly benefited from all the previous NDS evaluations (2004Si08,1993Ki25,1987Ki13, 1980Ek01,1974Al33), but at the same time data presented herein supersede all the previous published evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Helium Behavior in Oxide Nuclear Fuels: First Principles Modeling

UO2 and (U, Pu)O2 solid solutions (the so-called MOX) nowadays are used as commercial nuclear fuels in many countries. One of the safety issues during the storage of these fuels is related to their self-irradiation that produces and accumulates point defects and helium therein. We present density functional theory (DFT) calculations for UO2, PuO2 and MOX containing He atoms in octahedral interstitial positions. In particular, we calculated basic MOX properties and He incorporation energies as functions of Pu concentration within the spin-polarized, generalized gradient approximation (GGA) DFT calculations. We also included the on-site electron correlation corrections using the Hubbard model (in the framework of the so-called DFT + U approach). We found that PuO2 remains semiconducting with He in the octahedral position while UO2 requires a specific lattice distortion. Both materials reveal a positive energy for He incorporation, which, therefore, is an exothermic process. The He incorporation energy increases with the Pu concentration in the MOX fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuclear Power Plant Infrastructure Evaluations for Removal of Spent Nuclear Fuel

This report provides evaluations of the NPP site infrastructure and near-site transportation infrastructure for removing spent nuclear from 16 (NPP) sites. The material to be removed from the NPP sites includes both the spent nuclear fuel (SNF) and the greater-than-Class C low level radioactive waste (GTCC waste) that is stored, or will be stored, at the sites.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of Radionuclide Ratios in Atmospheric Nuclear Explosions and Nuclear Releases from Chernobyl and Fukushima seen in Gamma Ray Spectormetry

The Comprehensive Nuclear Test Ban Treaty (CTBT) has remote radionuclide monitoring followed by an On Site Inspection (OSI) to clarify the nature of a suspect event. An important aspect of radionuclide measurements on site is the discrimination of other potential sources of similar radionuclides such as reactor accidents or medical isotope production. The Chernobyl and Fukushima nuclear reactor disasters offer two different reactor source term environmental inputs that can be compared against historical measurements of nuclear explosions. The comparison of whole-sample gamma spectrometry measurements from these three events and the analysis of similarities and differences are presented. This analysis is a step toward confirming what is needed for measurements during an OSI under the auspices of the Comprehensive Test Ban Treaty.

54 ENVIRONMENTAL SCIENCES↗

Nuclear Analytical Applications within the IAEA Nuclear Data Section

The Nuclear Data Section, International Atomic Energy Agency, supports Member States development of nuclear techniques through a number of targeted actions and projects. The Section fulfills this role by organizing Coordinated Research Projects, or through less formal Data Development Projects and/or Technical Meetings. Training workshops are also regularly organized in conjunction with the International Centre for Theoretical Physics (ICTP), Trieste, Italy. A number of projects relating to materials analysis techniques have been recently undertaken, e.g. neutron activation analysis, ion beam analysis, and proton induced X- or {gamma}-ray emission. In particular, details of the Coordinated Research Project focusing on the nuclear data requirements for the k{sub 0} method of neutron activation analysis are given. The paper illustrates how the IAEA strives to bring together relevant partners and provides a unique and structured basis for international collaboration.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Effects of nuclear structure and quantum interference on diffractive vector meson production in ultra-peripheral nuclear collisions

Here we study diffractive vector meson production in ultra-peripheral collisions (UPCs) of heavy nuclei, utilizing a theoretical framework based on the Color Glass Condensate (CGC) formalism. We focus on Au + Au, U + U, Ru + Ru, Zr + Zr, and Pb + Pb collisions, examining the transverse momentum dependence of vector meson production cross-sections and co s(2ΔΦ)asymmetries in the decay product distributions to explore the role of nuclear geometry. The angular modulation is due to the linear polarization of the incoming photons and quantum interference effects. We extract nuclear radii and find them to be consistent with experimental data from the STAR collaboration. The amplitudes of the cos(2ΔΦ)modulation in the cross-section and the extracted radii depend on the nuclear geometry. This dependence is dominated by the geometry-dependent variation of the minimum impact parameter required for ultra-peripheral collisions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗