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NASA NTRS2008

Retrieval of Snow and Rain From Combined X- and W-B and Airborne Radar Measurements

Two independent airborne dual-wavelength techniques, based on nadir measurements of radar reflectivity factors and Doppler velocities, respectively, are investigated with respect to their capability of estimating microphysical properties of hydrometeors. The data used to investigate the methods are taken from the ER-2 Doppler radar (X-band) and Cloud Radar System (W-band) airborne Doppler radars during the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment campaign in 2002. Validity is assessed by the degree to which the methods produce consistent retrievals of the microphysics. For deriving snow parameters, the reflectivity-based technique has a clear advantage over the Doppler-velocity-based approach because of the large dynamic range in the dual-frequency ratio (DFR) with respect to the median diameter Do and the fact that the difference in mean Doppler velocity at the two frequencies, i.e., the differential Doppler velocity (DDV), in snow is small relative to the measurement errors and is often not uniquely related to Do. The DFR and DDV can also be used to independently derive Do in rain. At W-band, the DFR-based algorithms are highly sensitive to attenuation from rain, cloud water, and water vapor. Thus, the retrieval algorithms depend on various assumptions regarding these components, whereas the DDV-based approach is unaffected by attenuation. In view of the difficulties and ambiguities associated with the attenuation correction at W-band, the DDV approach in rain is more straightforward and potentially more accurate than the DFR method.

Liao, Liang↗

NASA NTRS2020

Optimized Profile Retrievals of Aerosol Microphysical Properties from Simulated Spaceborne Multiwavelength Lidar

This work is an expanded study of one previously published onretrievals of aerosol microphysical properties from space-borne multiwavelengthlidarmeasurements. The earlier studiesand this one weredone in the framework of the NASA Aerosol-Clouds-Ecosystems (now the Aerosol Clouds Convection and Precipitation) NASA mission. The focus here is on the capabilities of a simulated spacebornemultiwavelengthlidar system for retrieving aerosol complex refractive index (m = mr+ imi) and spectral single scattering albedo (SSA(λ)), although other bulk parameters such as effective (reff) radius and particle volume (V) and surface (S) concentrations are also studied. The novelty presented here is the use of recently published, case dependent optimized-constraints on the microphysical retrievals using three backscattering coefficients (β) at 355, 532 and 1064 nm and two extinction coefficients (α) at 355 and 532 nm, typically known as the stand-alone 3β+2α lidar inversion. Case-dependent optimized-constraints (CDOC) limit the ranges of refractive index, both real (mr) and imaginary (mi) parts, and of radii that are permitted in the retrievals. Such constraints are selected directly from the 3β+2α41measurements through an analysis of the relationship between spectral dependence of aerosol extinction-to-backscatter ratios (LR) and the Ångström exponent of extinction. The analyses presented here for different sets ofsize distributions and refractive indices reveal that the direct determination of CDOCareonly feasible for cases where the uncertaintiesin the input optical data areless than 15 %.Forthe same simulated spacebornesystem and yield than in Whiteman et al., (2018), we demonstrated that the use of CDOC as essential for the retrievals of refractive index and also largely improved retrieval of bulk parameters. A discussion of the global representativeness of CDOC is presented using simulated lidar data from a 24-hour satellite track using GEOS model output to initialize the lidar simulator.We found that CDOCare representative of many aerosol mixtures in spite of some outliers (e.g. highly hydrated particles) associatedwith the assumptions of bimodal size distributions and of the same refractive index for fine and coarse modes. Moreover, sensitivity tests performed using synthetic data reveal that retrievals of imaginary refractive index (mi) and SSA are extremely sensitive to β(355).

NASA Aerosol-Clouds-Ecosystems↗

NASA NTRS2014

Sport Transition of JPSS VIIRS Imagery for Night-time Applications

The NASA/Short‐term Prediction, Research, and Transition (SPoRT) Program and NOAA/Cooperative Institute for Research in the Atmosphere (CIRA) work within the NOAA/Joint Polar Satellite System (JPSS) Proving Ground to demonstrate the unique capabilities of the VIIRS instrument. Very similar to MODIS, the VIIRS instrument provides many high‐resolution visible and infrared channels in a broad spectrum. In addition, VIIRS is equipped with a low‐light sensor that is able to detect light emissions from the land and atmosphere as well as reflected sunlight by the lunar surface. This band is referred to as the Day‐Night Band due to the sunlight being used at night to see cloud and topographic features just as one would typically see in day‐time visible imagery. NWS forecast offices that collaborate with SPoRT and CIRA have utilized MODIS imagery in operations, but have longed for more frequent passes of polar‐orbiting data. The VIIRS instrument enhances SPoRT collaborations with WFOs by providing another day and night‐time pass, and at times two additional passes due to its large swath width. This means that multi‐spectral, RGB imagery composites are more readily available to prepare users for their use in GOES‐R era and high‐resolution imagery for use in high‐latitudes is more frequently able to supplement standard GOES imagery within the SPoRT Hybrid GEO‐LEO product. The transition of VIIRS also introduces the new Day‐Night Band capability to forecast operations. An Intensive Evaluation Period (IEP) was conducted in Summer 2013 with a group of "Front Range" NWS offices related to VIIRS night‐time imagery. VIIRS single‐channel imagery is able to better analyze the specific location of fire hotspots and other land features, as well as provide a more true measurement of various cloud and aerosol properties than geostationary measurements, especially at night. Viewed within the SPoRT Hybrid imagery, the VIIRS data allows forecasters to better interpret the more frequent, but coarse GOES Imagery. Night‐time Microphysics and Dust RGB Imagery provides cloud analysis of cloud height, thickness, and composition in order for operational applications such as separating fog from low clouds, dust plume detection, and determining precipitating clouds in radar-void/ blocked regions. The Day‐Night Band has a particular benefit to seeing light from cities, fires, or other emissions as well as the reflection of moonlight off of clouds and smoke plumes, given the right lunar phase and angle. Examples from the VIIRS transition and IEP will be presented.

Fuell, Kevin↗

NASA NTRS2014

Aerosol, Cloud and Trace Gas Observations Derived from Airborne Hyperspectral Radiance and Direct Beam Measurements in Recent Field Campaigns

The AERONET (AErosol RObotic NETwork) ground-based suite of sunphotometers provides measurements of spectral aerosol optical depth (AOD), precipitable water and spectral sky radiance, which can be inverted to retrieve aerosol microphysical properties that are critical to assessments of aerosol-climate interactions. Because of data quality criteria and sampling constraints, there are significant limitations to the temporal and spatial coverage of AERONET data and their representativeness for global aerosol conditions. The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument, jointly developed by NASA Ames and PNNL with NASA Goddard collaboration, combines airborne sun tracking and AERONET-like sky scanning with spectroscopic detection. Being an airborne instrument, 4STAR has the potential to fill gaps in the AERONET data set. Dunagan et al. [2013] present results establishing the performance of the instrument, along with calibration, engineering flight test, and preliminary scientific field data. The 4STAR instrument operated successfully in the SEAC4RS [Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys] experiment in Aug./Sep. 2013 aboard the NASA DC-8 and in the DoE [Department of Energy]-sponsored TCAP [Two Column Aerosol Project, July 2012 & Feb. 2013] experiment aboard the DoE G-1 aircraft (Shinozuka et al., 2013), and acquired a wealth of data in support of mission objectives on all SEAC4RS and TCAP research flights. 4STAR provided direct beam measurements of hyperspectral AOD, columnar trace gas retrievals (H2O, O3, NO2; Segal-Rosenheimer et al., 2014), and the first ever airborne hyperspectral sky radiance scans, which can be inverted to yield the same products as AERONET ground-based observations. In addition, 4STAR measured zenith radiances underneath cloud decks for retrievals of cloud optical depth and effective diameter. In this presentation, we provide an overview of the new 4STAR capabilities for airborne field campaigns, with an emphasis on comparisons between 4STAR and AERONET sky radiances, and retrievals of aerosol microphysical properties based on sky radiance measurements, column trace gas amounts from spectral direct beam measurements and cloud property retrievals from zenith mode observations for a few select case studies in the SEAC4RS and TCAP experiments. We summarize the aerosol, trace gas, cloud and airmass characterization studies made possible by the combined 4STAR direct beam, and sky/zenith radiance observations.

Aerosol-Climate↗

NASA NTRS2009

Cold Season QPF: Sensitivities to Snow Parameterizations and Comparisons to NASA CloudSat Observations

As operational numerical weather prediction is performed at increasingly finer spatial resolution, precipitation traditionally represented by sub-grid scale parameterization schemes is now being calculated explicitly through the use of single- or multi-moment, bulk water microphysics schemes. As computational resources grow, the real-time application of these schemes is becoming available to a broader audience, ranging from national meteorological centers to their component forecast offices. A need for improved quantitative precipitation forecasts has been highlighted by the United States Weather Research Program, which advised that gains in forecasting skill will draw upon improved simulations of clouds and cloud microphysical processes. Investments in space-borne remote sensing have produced the NASA A-Train of polar orbiting satellites, specially equipped to observe and catalog cloud properties. The NASA CloudSat instrument, a recent addition to the A-Train and the first 94 GHz radar system operated in space, provides a unique opportunity to compare observed cloud profiles to their modeled counterparts. Comparisons are available through the use of a radiative transfer model (QuickBeam), which simulates 94 GHz radar returns based on the microphysics of cloudy model profiles and the prescribed characteristics of their constituent hydrometeor classes. CloudSat observations of snowfall are presented for a case in the central United States, with comparisons made to precipitating clouds as simulated by the Weather Research and Forecasting Model and the Goddard single-moment microphysics scheme. An additional forecast cycle is performed with a temperature-based parameterization of the snow distribution slope parameter, with comparisons to CloudSat observations provided through the QuickBeam simulator.

Molthan, A. L.↗

NASA NTRS1997

Comparison of Ice Cloud Particle Sizes Retrieved From Satellite Data Derived From In Situ Measurements

Cloud microphysical parameterizations have attracted a great deal of attention in recent years due to their effect on cloud radiative properties and cloud-related hydrological processes in large-scale models. The parameterization of cirrus particle size has been demonstrated as an indispensable component in the climate feedback analysis. Therefore, global-scale, long-term observations of cirrus particle sizes are required both as a basis of and as a validation of parameterizations for climate models. While there is a global scale, long-term survey of water cloud droplet sizes (Han et al. 1994), there is no comparable study for cirrus ice crystals. In this paper a near-global survey of cirrus ice crystal sizes is conducted using ISCCP satellite data analysis. The retrieval scheme uses phase functions based upon hexagonal crystals calculated by a ray tracing technique. The results show that global mean values of D(e) are about 60 micro-m. This study also investigates the possible reasons for the significant difference between satellite retrieved effective radii (approx. 60 micro-m) and aircraft measured particle sizes (approx. 200 micro-m) during the FIRE I IFO experiment. They are (1) vertical inhomogeneity of cirrus particle sizes; (2) lower limit of the instrument used in aircraft measurements; (3) different definitions of effective particle sizes; and (4) possible inappropriate phase functions used in satellite retrieval.

Han, Qingyuan↗

NASA NTRS1997

Comparison of Ice Cloud Particle Sizes Retrieved from Satellite Data Derived from In Situ Measurements

Han, Qingyuan↗

NASA NTRS2003

Combined Radiometer-Radar Microphysical Profile Estimations with Emphasis on High Frequency Brightness Temperature Observations

Information about the vertical microphysical cloud structure is useful in many modeling and predictive practices. Radiometers and radars are used to observe hydrometeor properties. This paper describes an iterative retrieval algorithm that combines the use of airborne active and wideband (10 to 340 GHz) passive observations to estimate the vertical content and particle size distributions of liquid and frozen hydrometeors. The physically-based retrieval algorithm relies on the high frequencies (greater than 89 GHz) to provide details on the frozen hydrometeors. Neglecting the high frequencies yielded acceptable estimates of the liquid profiles, but the ice profiles were poorly retrieved. Airborne radar and radiometer observations from the third Convection and Moisture EXperiment (CAMEX-3) were used in the retrieval algorithm as constraints. Nadir profiles were estimated for a minute each of flight time (approximately 12.5 km along track) from an anvil, convection, and quasi- stratiform rain. The complex structure of the frozen hydrometeors required the most iterations for convergence for the anvil cloud type. The wideband observations were found to more than double the estimated frozen hydrometeor content as compared to retrievals using only 90-GHz and below. The convective and quasi-stratiform quickly reached convergence (minimized difference between observations and calculations using the estimated profiles). A qualitative validation using coincident in situ CAMEX-3 observations shows that the retrieved particle size distributions are well corroborated with independent measurements.

Gail Skofronick-Jackson↗

NASA NTRS2013

Saharan Dust Event Impacts on Cloud Formation and Radiation over Western Europe

We investigated the impact of mineral dust particles on clouds, radiation and atmospheric state during a strong Saharan dust event over Europe in May 2008, applying a comprehensive online-coupled regional model framework that explicitly treats particle-microphysics and chemical composition. Sophisticated parameterizations for aerosol activation and ice nucleation, together with two-moment cloud microphysics are used to calculate the interaction of the different particles with clouds depending on their physical and chemical properties. The impact of dust on cloud droplet number concentration was found to be low, with just a slight increase in cloud droplet number concentration for both uncoated and coated dust. For temperatures lower than the level of homogeneous freezing, no significant impact of dust on the number and mass concentration of ice crystals was found, though the concentration of frozen dust particles reached up to 100 l-1 during the ice nucleation events. Mineral dust particles were found to have the largest impact on clouds in a temperature range between freezing level and the level of homogeneous freezing, where they determined the number concentration of ice crystals due to efficient heterogeneous freezing of the dust particles and modified the glaciation of mixed phase clouds. Our simulations show that during the dust events, ice crystals concentrations were increased twofold in this temperature range (compared to if dust interactions are neglected). This had a significant impact on the cloud optical properties, causing a reduction in the incoming short-wave radiation at the surface up to -75Wm-2. Including the direct interaction of dust with radiation caused an additional reduction in the incoming short-wave radiation by 40 to 80Wm-2, and the incoming long-wave radiation at the surface was increased significantly in the order of +10Wm-2. The strong radiative forcings associated with dust caused a reduction in surface temperature in the order of -0.2 to -0.5K for most parts of France, Germany, and Italy during the dust event. The maximum difference in surface temperature was found in the East of France, the Benelux, and Western Germany with up to -1 K. This magnitude of temperature change was sufficient to explain a systematic bias in numerical weather forecasts during the period of the dust event.

Bangert, M.↗

NASA NTRS2017

TPSAS-NF1676L-26989-DND

The NASA Langley Research Center airborne High Spectral Resolution Lidar (HSRL-2) provided extensive measurements of smoke above shallow marine clouds while deployed from the NASAER-2 aircraft during the NASAEV-S Observations of Aerosols above Clouds and their Interactions (ORACLES) mission. During the first ORACLES field campaign in September 2016, the ER-2 was deployed from Walvis Bay, Namibia and conducted flights over the south eastern Atlantic Ocean. HSRL-2 measured profiles of aerosol backscattering, extinction and aerosol optical depth (AOD) at 355 and 532 nm and aerosol backscattering and depolarization at 1064 nm and so provided an excellent characterization of the wide-spread smoke layers above shallow marine clouds. We use the HSRL-2 measurements to examine retrievals of AOD above clouds retrieved from A Train active (CALIOP) and passive (OMI, MODIS) sensors. We also present profiles of aerosol microphysical properties such as concentration and effective radius that are derived from the HSRL-2 multi wavelength measurements of backscatter and extinction.

Richard Ferrare↗

NASA NTRSDate not supplied

Simultaneous Aerosol and Ocean Polarimeter Products Using Coupled Atmosphere-Ocean Vector Radiative Transfer and Neural Networks: The PACE-MAPP Algorithm

We describe the PACE-MAPP algorithm that simultaneously retrieves aerosol and ocean optical parameters using multiangle and multi-channel polarimeter measurements from the SPEXone, Hyper-Angular Rainbow Polarimeter 2 (HARP2), and Ocean Color Instrument (OCI) instruments onboard the NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) observing system PACE-MAPP is adapted from the Research Scanning Polarimeter (RSP) Microphysical Aerosol Properties from Polarimetry (RSP-MAPP) algorithm. A key feature of the MAPP family of algorithms is the use of a coupled vector radiative transfer model such that the atmosphere and ocean are always considered together as one system. Consequently, conservation of energy ensures that negative water-leaving radiances do not occur. PACE-MAPP uses optimal estimation to simultaneously characterize the optical and microphysical properties of aerosol and ocean constituents, find the optimal solution, and reliably account for the uncertainties of each parameter. This coupled approach, together with multiangle, multi-channel polarimeter measurements, will enable retrievals of aerosol and water properties across the Earth’s oceans. The PACE-MAPP algorithm provides aerosol and ocean products for both the open ocean and coastal areas and is designed to be accurate, modular, and efficient by using fast neural networks that replace the time-consuming vector radiative transfer calculations. We provide an overview of the PACE-MAPP framework and also describe its modular components including its aerosol and hydrosol models, ocean bio-optical models, and thin cirrus model.

Snorre Stamnes↗

NASA NTRSDate not supplied

The ACCP Inclined Orbit Project: Enabling New and Synergistic Aerosol Remote Sensing Inversions

Atmospheric aerosols have high spatiotemporal variations due to their diverse sources including windblown dust, wildfires, volcanic eruptions, and anthropogenic emissions. These aerosols also have strong diurnal emission characteristics that influence long-range transport, air quality, Earth’s radiation budget, biogeochemical cycles, and weather forecasting. While current sensors can measure the steady-state of global 3D cloud and aerosol properties, we lack the observational datasets to discover the diurnal variability of aerosols, even at seasonal and regional scales, because these missions utilize sun synchronous orbits. An Aerosols and Clouds, Convection and Precipitation (ACCP) observing system has been established as part of NASA’s new Earth System Observatory (ESO) to fulfill the science needs presented in the 2017 Earth Science Decadal Survey. The selected ACCP architecture encompasses sensors in two orbit planes, one of which utilizes an inclined orbit (nominally ~55 degrees at a 407 km altitude) to advance our understanding of aerosol and cloud properties and target the dynamics of the cloud and aerosol processes on sub-daily time scales. The anticipated instrumentation suite for the ACCP Inclined Orbit Project is a Stereo Camera System, Polarimeter, Microwave Radiometer, Two-Frequency Radar, and Backscatter Lidar. The polarimeter is expected to have multiple wavelength bands and viewing angles to enable accurate retrievals of aerosol microphysical and optical properties. The backscatter lidar will provide vertical profiles of attenuated backscatter and depolarization ratio at two wavelengths, with better daytime signal-to-noise ratio than previous space-based lidar systems to improve aerosol detection/typing and estimates of aerosol optical properties. The stereo camera system, while designed primarily for clouds, will also provide aerosol plume heights and air motions at the plume heights. This invited presentation will provide (1) an overview of the ACCP Inclined Orbit Project, (2) a description of the new sensor capabilities and orbital characteristics, and (3) a preview of the potential for new synergistic aerosol inversion techniques.

John E Yorks↗

NASA NTRS2017

Ice Nucleation in the Tropical Tropopause Layer: Implications for Cirrus Occurrence, Cirrus Microphysical Properties, and Dehydration of Air Entering the Stratosphere

Recent laboratory experiments have advanced our understanding of the physical properties and ice nucleating abilities of aerosol particles atlow temperatures. In particular, aerosols containing organics will transition to a glassy state at low temperatures, and these glassy aerosols are moderately effective as ice nuclei. These results have implications for ice nucleation in the cold Tropical Tropopause Layer (TTL; 13-19 km). We have developed a detailed cloud microphysical model that includes heterogeneous nucleation on a variety of aerosol types and homogeneous freezing of aqueous aerosols. This model has been incorporated into one-dimensional simulations of cirrus and water vapor driven by meteorological analysis temperature and wind fields. The model includes scavenging of ice nuclei by sedimenting ice crystals. The model is evaluated by comparing the simulated cloud properties and water vapor concentrations with aircraft and satellite measurements. In this presentation, I will discuss the relative importance of homogeneous and heterogeneous ice nucleation, the impact of ice nuclei scavenging as air slowly ascends through the TTL, and the implications for the final dehydration of air parcels crossing the tropical cold-point tropopause and entering the tropical stratosphere.

tropopause↗

NASA NTRS2017

Biofuel Blending Reduces Aircraft Engine Particle Emissions at Cruise Conditions

Aviation aerosol emissions have a disproportionately large climatic impact because they are emitted high in the relatively pristine upper troposphere where they can form linear contrails and influence cirrus clouds. Research aircraft from NASA, DLR, and NRC Canada made airborne measurements of gaseous and aerosol composition and contrail microphysical properties behind the NASA DC-8 aircraft at cruise altitudes. The DC-8 CFM-56-2C engines burned traditional medium-sulfur Jet A fuel as well as a low-sulfur Jet A fuel and a 50:50 biofuel blend. Substantial, two-to-three-fold emissions reductions are found for both particle number and mass emissions across the range of cruise thrust operating conditions. These observations provide direct and compelling evidence for the beneficial impacts of biojet fuel blending under real-world conditions.

Richard H Moore↗

NASA NTRSDate not supplied

The PACE-MAPP Algorithm: Coupled Ocean/Aerosol Products

The PACE-MAPP algorithm, under development for combined SPEXone, HARP2 and OCI observations from NASA’s future Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) satellite mission, directly inverts the coupled atmosphere-ocean system to retrieve aerosol optical and microphysical properties and ocean optical properties simultaneously. PACE-MAPP thus retrieves the spectrally-resolved inherent optical properties of the Earth’s waters: the spectral particulate scattering coefficient, b_p (λ), the spectral absorption coefficient for particulates and color-dissolved matter, a_tot (λ), and the spectral particulate backscatter efficiency, b ̃_"bp". From these three spectrally-resolved components, we can derive the spectral particulate hemispherical backscattering coefficient b_bp (λ) and the spectral diffuse attenuation coefficient K_"d" (λ). Direct comparisons of b_"bp" (532) and K_"d" (532) are made to collocated High-Spectral Resolution Lidar (HSRL) in-water measurements. The PACE-MAPP algorithm was tested using PACE-analog datasets collected by Research Scanning Polarimeter (RSP) observations during the NASA NAAMES (The North Atlantic Aerosols and Marine Ecosystems Study) and SABOR (Ship-Aircraft Bio-Optical Research) airborne campaigns, both of which also include ship-based in situ measurements.

Snorre Alfred Moen Stamnes↗

NASA NTRS2015

The Intra-Cloud Lightning Fraction in the Contiguous United States

Lightning is dangerous and destructive; cloud-to-ground (CG) lightning flashes can start fires, interrupt power delivery, destroy property and cause fatalities. Its rate-of-occurrence reflects storm kinematics and microphysics. For decades lightning research has been an important focus, and advances in lightning detection technology have been essential contributors to our increasing knowledge of lightning. A significant step in detection technology is the Geostationary Lightning Mapper (GLM) to be onboard the Geostationary Operational Environment Satellite R-Series (GOES-R) to be launched in early 2016. GLM will provide continuous "Total Lightning" observations [CG and intra-cloud lightning (IC)] with near-uniform spatial resolution over the Americas by measuring radiance at the cloud tops from the different types of lightning. These Total Lightning observations are expected to significantly improve our ability to nowcast severe weather. It may be important to understand the long-term regional differences in the relative occurrence of IC and CG lightning in order to understand and properly use the short-term changes in Total Lightning flash rate for evaluating individual storms.

lightning↗

NASA NTRS2024

A Multi‐Probe Automated Classification of Ice Crystal Habits During the IMPACTS Campaign

Although all ice crystals are unique, many can be grouped together by shape or habit, with members of a habit class sharing similar representations of properties such as fall velocity and growth rate. A decision tree algorithm designed to be adaptable to any particle imaging probe, thus enabling the creation of habit size distributions over a size range larger than that of any probe on its own, is used to classify ice crystals imaged by three airborne cloud probes in mid-latitude winter cyclones during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) field campaign. Crystals are sorted into seven habit classes based on their morphological properties: sphere, column/needle, plate, graupel, dendrite, aggregate, and irregular. Although adaptability was its primary goal, the algorithm was found to be moderately skillful for identifying idealized habit images. Quantitative tests of the algorithm’s adaptability displayed mixed results, as Two-Dimensional Stereo Probe (2DS) classifications showed moderate correlation with Particle Habit Imaging and Polar Scattering Probe (PHIPS) classifications, but only weak correlation with High Volume Precipitation Spectrometer (HVPS) classifications. The algorithm was applied to random sets of images from each probe in a case study of a mesoscale snow band sampled on 7 February 2020. In the case study, qualitative analysis of particle images revealed general agreement on classifications among the probes, supporting the algorithm’s applicability to multiple cloud probes. Most classifications appeared correct upon manual inspection, suggesting that in practical use, the algorithm is reasonably able to classify non-idealized images.

Julian Schima↗

NASA NTRS1995

A Model Simulation of Pinatubo Volcanic Aerosols in the Stratosphere

A one-dimensional, time-dependent model is used to study the chemical, microphysical, and radiative properties of volcanic aerosols produced by the Mount Pinatubo eruption on June 15, 1991. Our model treats gas-phase sulfur photochemistry, gas-to-particle conversion of sulfur, and the microphysics of sulfate aerosols and ash particles under stratospheric conditions. The dilution and diffusion of the volcanic eruption clouds are also accounted for in these conditions. Heteromolecular homogeneous and heterogeneous binary H2SO4/H2O nucleation, acid and water condensational growth, coagulation, and gravitational sedimentation are treated in detail in the model. Simulations suggested that after several weeks, the volcanic cloud was composed mainly of sulfuric acid/water droplets produced in situ from the SO2 emissions. The large amounts of SO2 (around 20 Mt) injected into the stratosphere by the Pinatubo eruption initiated homogeneous nucleation which generated a high concentration of small H2SO4/H2O droplets. These newly formed particles grew rapidly by condensation and coagulation in the first few months and then reach their stabilized sizes with effective radii in a range between 0.3 and 0.5 micron approximately one-half year after the eruption. The predicted volcanic cloud parameters reasonably agree with measurements in term of the vertical distribution and lifetime of the volcanic aerosols, their basic microphysical structures (e.g., size distribution, concentration, mass ratio, and surface area) and radiative properties. The persistent volcanic aerosols can produce significant anomalies in the radiation field, which have important climatic consequences. The large enhancement in aerosol surface area can result in measurable global stratospheric ozone depletion.

Zhao , Jing-xia↗