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A comparison between Nimbus 5 THIR and ITPR temperatures and derived winds with rawinsonde data obtained in the AVE 2 experiment

During the period of May 11 and 12, 1974, NASA conducted its second Atmospheric Variability Experiment (AVE II) over the eastern United States. In this time interval, two Nimbus 5 orbits crossed the AVE II area, providing a series of ITPR soundings as well as THIR data. Horizontal temperature mapping of the AVE II cloud field is examined using two grid print map scales. Implied cloud top heights are compared with maximum radar-echo top reports. In addition, shelter temperatures in areas of clear sky are compared with the surface temperatures as determined from 11.5 micrometer radiometer data of the THIR experiment. The ITPR sounding accuracy is evaluated using interpolated radiosonde temperatures at times nearly coincident with the ITPR soundings. It was found that mean differences between the two data sets were as small as 1.3 C near 500 mb and as large as 2.9 C near the tropopause. The differences between ITPR and radiosonde temperatures at constant pressure levels were sufficient to induce significant differences in the horizontal temperature gradient. Cross sections of geostrophic wind along the orbital tracks were developed using a thermal wind buildup based on the ITPR temperature data and the radiosonde temperature data. Differences between the radiosonde and ITPR geostrophic winds could be explained on the basis of differences in the ITPR and radiosonde temperature gradients.

Arnold, J. E.↗

Aerosol backscatter measurements at 10.6 microns with airborne and ground-based CO2 Doppler lidars over the Colorado High Plains. II - Backscatter structure

Measurements of tropospheric aerosol volume backscatter coefficients at 10.6-microns wavelength were obtained with airborne continuous wave and ground-based pulsed CO2 Doppler lidars over the Colorado High Plains during a 20-day period in summer 1982. A persistent 'background' layer was found between 6- and 10-km altitude, with a generally uniform backscatter mixing ratio of about 10 to the -10th sq m/kg per sr. The upper boundary of this background layer varied with the tropopause height; the lower boundary varied with the strength and diurnal cycle of convective mixing in the planetary boundary layer (PBL). For quiescent meteorological conditions, the transition from the PBL to the background layer was usually very sharp, with backscatter decreases sometimes as large as 3 decades in about 70 m. Sharp gradients were also found at the boundaries of shallow (tens of meters) subvisible cirrus clouds. For less stable conditions, associated with vertical aerosol transport by deep cumuliform clouds, backscatter tended to decrease exponentially with altitude.

Bowdle, David A.↗

Removal of the solar component in AVHRR 3.7 micrometer radiances for the retrieval of cirrus cloud parameters

A numerical scheme has been developed to remove the solar component in the Advanced Very High Resolution Radiometer (AVHRR) 3.7- micrometer channel for the retrieval of cirrus parameters during daytime. This method uses a number of prescribed threshold values for AVHRR channels 1 (0.63 micrometer), 2 (0.8 micrometer), 3 (3.7 micrometer), 4 (10.9 micrometer), and 5 (12 micrometer) to separate clear and cloudy pixels. A look-up table relating channels 1 and 3 solar reflectances is subsequently constructed based on the prescribed mean effective ice crystal sizes and satellite geometric parameters. An adding-doubling radiative transfer program has been used to generate numerical values in the construction of the look-up table. Removal of the channel 3 solar component is accomplished by using the look-up table and the measured channel 1 reflectance. The cloud retrieval scheme described in Ou et al. has been modified in connection with the removal program. The authors have applied the removal-retrieval scheme to the AVHRR global area coverage daytime data, collected during the First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment cirrus intensive field observation (FIRE IFO) at 2100 UTC 28 October 1986 over the Wisconsin area. Distributions of the retrieved cloud heights and optical depths are comparable to those determined from Geostationary Operational Environmental Satellite (GOES) visible and IR channels data reported by Minnis et al. Moreover, verifications of the retrieved cirrus temperature and height against lidar data have been carried out using results reported from three FIRE IFO stations. The retrieved cloud heights are within 0.5 km of the measured lidar values.

Rao, N. X.↗

Improving Lightning NO(x) Parameterizations for Global Chemical Transport Models

Parameterization of lightning NO(x) in global chemical transport models requires a method to specify the temporal and geographic distribution of flash rates, an estimate of NO production per flash, and a method to specify the effective vertical distribution of NO production. Flash rate parameterizations using the upward convective cloud mass flux have been developed and tested for several GCM and assimilated meteorological data sets. This parameterization and others involving the cloud-top height and convective precipitation provide a generally acceptable climatological distribution of flashes after normalization with satellite data. However, considerable improvement in terms of geographic and temporal variability may be achieved in the future using cloud microphysics data available from next-generation GCMs. Cloud-resolving case-study simulations of convective transport and lightning NO production have yielded results which are directly applicable to the NO production per flash and the vertical NO distribution portions of the global model lightning parameterizations. In this work we have used cloud-resolving models (the Goddard Cumulus Ensemble Model (GCE) and MM5) to drive an off-line cloud-scale chemical transport model (CSCTM). The CSCTM, in conjunction with aircraft measurements of NO(x) in thunderstorms and ground-based lightning observations, has been used to constrain the amount of NO produced per flash. Observed lightning flash rates have been incorporated into the CSCTM, and several scenarios of NO production per intracloud (IC) and per cloud-to-ground (CG) flash have been tested in each of several case study storms. The resulting NO(x) mixing ratios are compared with aircraft measurements taken within the storm (typically the anvil region) to determine the most likely NO production scenario. The range of values of NO production per flash (or per meter of lightning channel length) that have been deduced from the model will be shown and compared with values of production in the literature that have been deduced from observed NO spikes and from anvil flux calculations. Results show that on a per flash basis, IC flashes are nearly as productive of NO as CG flashes. Estimates of mean NO production per flash vary by a factor of three from one simulated storm to another. Vertical profiles of lightning NOx mass at the end of the 3-D storm simulations have been summarized to yield suggested profiles for use in global models. These profiles show a larger percentage of the total lightning NO(x) mass in the free troposphere than those suggested by Pickering et al. (1998).

Pickering, Kenneth E.↗

Classifying Microwave Radiometer Observations Over the Netherlands Into Dry, Shallow-, and Non-Shallow Precipitation Using A Random Forest Model

Spaceborne microwave radiometers represent an important component of the Global Precipitation Measurement (GPM) mission due to their frequent sampling of rain systems. Microwave radiometers measure microwave radiation (brightness temperatures, Tb), which can be converted into precipitation estimates with appropriate assumptions. However, detecting shallow precipitation systems using space-borne radiometers is challenging, especially over land, as their weak signals are hard to differentiate from those associated with dry conditions. This study uses a random forest model (RF) to classify microwave radiometer observations as dry, shallow, or nonshallow over the Netherlands - a region with varying surface conditions and frequent occurrence of shallow precipitation. The RF is trained on five years of data (2016-2020) and tested with two independent years (2015, 2021). The observations are classified using ground-based weather radar echo top heights. Various RF models are assessed, such as using only GPM’s Microwave Imager (GMI) Tb values as input features or including spatially aligned ERA-5 2-meter temperature and freezing level reanalysis and/or Dual Precipitation Radar (DPR) observations. Independent of the input features, the model performs best in summer and worst in winter. The model classifies observations from high-frequency channels (≥85 GHz) with lower Tb-values as non-shallow, higher values as dry, and those in between as shallow. Misclassified footprints exhibit radiometric characteristics corresponding to their assigned class. Case studies reveal dry observations misclassified as shallow are associated with lower Tb-values, likely resulting from the presence of ice particles in non-precipitating clouds. Shallow footprints misclassified as dry are likely related to the absence of ice particles.

Linda Bogerd↗

Comparison of cloud fields from atmospheric general circulation model, in situ and satellite measurements

This paper focuses on the comparison of cloud amounts derived from an atmospheric general circulation model (AGCM), Satellite-observed clouds, and Ground-based cloud observations. Unlike Earth Radiation Budget Experiment (ERBE)-type comparisons it does not mix potential errors in the cloud amount with those in the radiation code embedded in the model. Long term cloud climatologies were used to compare global cloud amounts and regional seasonal cycles. The AGCM successfully reproduced the signatures of the warm pool and North Pacific seasonal cycle cloudiness but failed in the low stratus region off the coast of South America, a known problem for AGCMs. The data sets also reproduced the anomaly signature associated with El Nino in the warm pool region, but the model amounts were lower. Global results had a similar success rate, with the model generally producing lower total cloud compared to the satellite and in situ measurements. To compare cloud vertical distributions the cloud height may need to be validated using the corresponding radiation fields. Unfortunately there were also some large discrepancies between the two observed cloud data sets. While tremendously improved over the last decade the character of the observed cloud data sets, must be substantially enhanced before they will be useful in validating AGCMs by any but the crudest levels of comparison.

Haskins, Robert D.↗

Near-global survey of effective droplet radii in liquid water clouds using ISCCP data

A global survey of cloud particle size variations can provide crucial constraints on how cloud processes determine cloud liquid water contents and their variation with temperature, and further, may indicate the magnitude of aerosol effects on clouds. A method, based on a complete radiative transfer model for Advanced Very High Resolution Radiometer (AVHRR)-measured radiances, is described for retrieving cloud particle radii in liquid water clouds from satellite data currently available from the International Satellite Cloud Climatology Project. Results of sensitivity tests and validation studies provide error estimates. AVHRR data from NOAA-9 and NOAA-10 have been analyzed for January, April, July and October in 1987 and 1988. The results of this first survey reveal systematic continental and maritime differences and hemispheric contrasts that are indicative of the effects of associated aerosol concentration differences: cloud droplet radii in continental water clouds are about 2-3 micrometers smaller than in marine clouds, and droplet radii are about 1 micrometer smaller in marine clouds of the Northern Hemisphere than in the Southern Hemisphere. The height dependencies of cloud droplet radii in continental and marine clouds are also consistent with differences in the vertical profiles of aerosol concentration. Significant seasonal and diurnal variations of effective droplet radii are also observed, particularly at lower latitudes. Variations of the relationship between cloud optical thickness and droplet radii may indicate variations in cloud microphysical regimes.

Han, Qingyan↗

Lightning Return-Stroke Current Waveforms Aloft, From Measured Field Change, Current, and Channel Geometry

Direct current measurements are available near the attachment point from both natural cloud-to-ground lightning and rocket-triggered lightning, but little is known about the rise time and peak amplitude of return-stroke currents aloft. We present, as functions of height, current amplitudes, rise times, and effective propagation velocities that have been estimated with a novel remote-sensing technique from data on 24 subsequent return strokes in six different lightning flashes that were triggering at the NASA Kennedy Space Center, FL, during 1987. The unique feature of this data set is the stereo pairs of still photographs, from which three-dimensional channel geometries were determined previously. This has permitted us to calculate the fine structure of the electric-field-change (E) waveforms produced by these strokes, using the current waveforms measured at the channel base together with physically reasonable assumptions about the current distributions aloft. The computed waveforms have been compared with observed E waveforms from the same strokes, and our assumptions have been adjusted to maximize agreement. In spite of the non-uniqueness of solutions derived by this technique, several conclusions seem inescapable: 1) The effective propagation speed of the current up the channel is usually significantly (but not unreasonably) faster than the two-dimensional velocity measured by a streak camera for 14 of these strokes. 2) Given the deduced propagation speed, the peak amplitude of the current waveform often must decrease dramatically with height to prevent the electric field from being over-predicted. 3) The rise time of the current wave front must always increase rapidly with height in order to keep the fine structure of the calculated field consistent with the observations.

Willett, J. C.↗

First Look at the Upper Tropospheric Ozone Mixing Ratio from OMI Estimated using the Cloud Slicing Technique

The Cloud Slicing technique has emerged as a powerful tool for the study of ozone in the upper troposphere. In this technique one looks at the variation with cloud height of the above-cloud column ozone derived from the backscattered ultraviolet instruments, such as TOMS, to determine the ozone mixing ratio. For this technique to work properly one needs an instrument with relatively good horizontal resolution with very good signal to noise in measuring above-cloud column ozone. In addition, one needs the (radiatively) effective cloud pressure rather than the cloud-top pressure, for the ultraviolet photons received by a satellite instrument are scattered from inside the cloud rather than from the top. For this study we use data from the OMI sensor, which was recently launched on the EOS Aura satellite. OMI is a W-Visible backscattering instrument with a nadir pixel size of 13 x 24 km. The effective cloud pressure is derived from a new algorithm based on Rotational Raman Scattering and O2-O2, absorption in the 340-400 nm band of OMI.

Bhartia, Pawan K.↗

Lidar observations of mixed layer dynamics - Tests of parameterized entrainment models of mixed layer growth rate

Ground based lidar measurements of the atmospheric mixed layer depth, the entrainment zone depth and the wind speed and wind direction were used to test various parameterized entrainment models of mixed layer growth rate. Six case studies under clear air convective conditions over flat terrain in central Illinois are presented. It is shown that surface heating alone accounts for a major portion of the rise of the mixed layer on all days. A new set of entrainment model constants was determined which optimized height predictions for the dataset. Under convective conditions, the shape of the mixed layer height prediction curves closely resembled the observed shapes. Under conditions when significant wind shear was present, the shape of the height prediction curve departed from the data suggesting deficiencies in the parameterization of shear production. Development of small cumulus clouds on top of the layer is shown to affect mixed layer depths in the afternoon growth phase.

Boers, R.↗

The Global Oscillation Network Group site survey, 2: Results

The Global Oscillation Network Group (GONG) Project will place a network of instruments around the world to observe solar oscillations as continuously as possible for three years. The Project has now chosen the six network sites based on analysis of survey data from fifteen sites around the world. The chosen sites are: Big Bear Solar Observatory, California; Mauna Loa Solar Observatory, Hawaii; Learmonth Solar Observatory, Australia; Udaipur Solar Observatory, India; Observatorio del Teide, Tenerife; and Cerro Tololo Interamerican Observatory, Chile. Total solar intensity at each site yields information on local cloud cover, extinction coefficient, and transparency fluctuations. In addition, the performance of 192 reasonable networks assembled from the individual site records is compared using a statistical principal components analysis. An accompanying paper descibes the analysis methods in detail; here we present the results of both the network and individual site analyses. The selected network has a duty cycle of 93.3%, in good agreement with numerical simulations. The power spectrum of the network observing window shows a first diurnal sidelobe height of 3 x 10(exp -4) with respect to the central component, an improvement of a factor of 1300 over a single site. The background level of the network spectrum is lower by a factor of 50 compared to a single-site spectrum.

Hill, Frank↗

Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing During Boreal Spring

The direct effects of aerosols on global and regional climate during boreal spring are investigated based on simulations using the NASA Global Modeling and Assimilation Office (GMAO) finite-volume general circulation model (fvGCM) with Microphyics of clouds in Relaxed Arakawa Schubert Scheme (McRAS). The aerosol loading are prescribed from three-dimensional monthly distribution of tropospheric aerosols viz., sulfate, black carbon, organic carbon, soil dust, and sea salt from output of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol extinction coefficient, single scattering albedo, and asymmetric factor are computed as wavelength-dependent radiative forcing in the radiative transfer scheme of the fvGCM, and as a function of the aerosol loading and ambient relative humidity. We find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excites a planetary scale teleconnection pattern in sea level pressure, temperature and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, i.e., South Asia, East Asia, and northern and western Africa. Additionally, atmospheric heating is found in regions with large loading of dust (over Northern Africa, and Middle East), and black carbon (over South-East Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east-west dipole anomaly with strong cooling over the Caspian Sea, and warming over central and northeastern Asia, where aerosol concentration are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations.

Kim, Maeng-Ki↗

Using the VAHIRR Radar Algorithm to Investigate Lightning Cessation

Accurately determining the threat posed by lightning is a major area for improved operational forecasts. Most efforts have focused on the initiation of lightning within a storm, with far less effort spent investigating lightning cessation. Understanding both components, initiation and cessation, are vital to improving lightning safety. Few organizations actively forecast lightning onset or cessation. One such organization is the 45th Weather Squadron (45WS) for the Kennedy Space Center (KSC) and Cape Canaveral Air Force Station (CCAFS). The 45WS has identified that charged anvil clouds remain a major threat of continued lightning and can greatly extend the window of a potential lightning strike. Furthermore, no discernable trend of total lightning activity has been observed consistently for all storms. This highlights the need for more research to find a robust method of knowing when a storm will cease producing lightning. Previous lightning cessation work has primarily focused on forecasting the cessation of cloud-to -ground lightning only. A more recent, statistical study involved total lightning (both cloud-to-ground and intracloud). Each of these previous works has helped the 45WS take steps forward in creating improved and ultimately safer lightning cessation forecasts. Each study has either relied on radar data or recommended increased use of radar data to improve cessation forecasts. The reasoning is that radar data is able to either directly or by proxy infer more about dynamical environment leading to cloud electrification and eventually lightning cessation. The authors of this project are focusing on a two ]step approach to better incorporate radar data and total lightning to improve cessation forecasts. This project will utilize the Volume Averaged Height Integrated Radar Reflectivity (VAHIRR) algorithm originally developed during the Airborne Field Mill II (ABFM II) research project. During the project, the VAHIRR product showed a trend of increasing values with increases in the electric field magnitude above 3 kV/m. An extreme value analysis showed that VAHIRR values less than or equal to 10 dBZ-km showed that the probability of having an electric field magnitude larger than 3 kV/m was less than one in ten thousand. VAHIRR also was found to be sensitive at indicating anvil clouds that posed a threat of initiating a lightning flash. This project seeks to use VAHIRR to analyze its utility as a lightning cessation tool, particularly dealing with the threat posed by detached anvils. The results from this project will serve as a baseline effectiveness of radar ]based lightning cessation algorithms. This baseline will be used in the second, and concurrent work by the co ]author fs who are developing a lightning cessation algorithm based on dual ]polarimetric radar data. Ultimately, an accurate method for identifying lightning cessation can save money on lost manpower time as well as greatly improve lightning safety.

Stano, Geoffrey T.↗

I’ve Looked at Clouds from Both Sides, Now: Viewpoints from Surface and Spaceborne Lidar Systems

Clouds play a critical role in the Earth’s climate system because they are inextricably linked to the hydrological cycle and radiation budget. Information about cloud height, thickness, occurrence, and amount are critical inputs for a host of numerical applications involving climate research. Therefore, it is important to have highly accurate and quantitative data records of cloud properties that span several years and geographic regions. Verification of even the most basic modeling processes demands long term and continuous observations of global cloud occurrence, if there is to be any confidence in their fidelity. For a number of reasons, however, it is impossible to gauge the complexities of clouds from a single source. Fundamentally, an array of remote sensing methods is needed in order to provide a complete picture. Within the Micropulse Lidar Network (MPLNET), we have developed a new algorithm to improve the quality of our cloud products. The largest impact of the changes to the cloud detection algorithm is evident with high clouds (those with cloud base > 5 km). Furthermore, polarized measurements enable us to determine the cloud thermodynamic phase. Naturally, the next step is to investigate how these improvements compare with observations from spaceborne lidars (e.g. CALIOP) which have a better (unobstructed) view of high clouds. Recent advances in remote sensing have revealed that cirrus clouds are the most common cloud genus observed in the atmosphere. Furthermore, cirrus skew highly towards relatively low cloud optical depths, as observed from both surface and spaceborne viewpoints. The radiative impacts of these findings are quite significant, considering the cumulative effect cirrus exhibit when compared to low clouds.

Jasper R Lewis↗

Interpretation of ground-based radiometric observations in terms of a gravity wave model

An analysis is presented of 2-hour and 4-hour segments of data taken at Denver, Colorado, on February 3, 1984, by a ground-based radiometer designed and operated by the Wave Propagation Laboratory of the National Oceanic and Atmospheric Administration (NOAA). The zenith-viewing instrument has two moisture-sensing and four temperature-sensing channels. It is demonstrated that a peak at a period of 10 min, present in the spectra of the measured brightness temperature and of the derived geopotential heights, thicknesses, and vertically integrated water vapor content, is due to an internal gravity wave generated by wind shear in the jet aloft. This analysis shows that the radiometer has the sensitivity to detect such disturbances and that the mathematical inversion technique used to retrieve the geopotential field and other integrated quantities retains the derived information as well. Finally, a linear expression is derived which relates the brightness temperature to the atmospheric temperature, density, humidity, and cloud liquid perturbation fields.

Canavero, F. G.↗

A Climatology of Midlatitude Continental Clouds from the ARM SGP Central Facility: Cloud Fraction and Radiative Forcing - Part II

Data collected at the Department of Energy Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) central facility are analyzed for determining the variability of cloud fraction and radiative forcing at several temporal scales between January 1997 and December 2002. Cloud fractions are estimated for total cloud cover and for single-layer low (0-3 km), middle (3-6 km), and high clouds (greater than 6 km) using ARM SGP ground-based paired lidar-radar measurements. Shortwave (SW), longwave (LW), and net cloud radiative forcings (CRF) are derived from up- and down-looking standard precision spectral pyranometers and precision infrared radiometer measurements. The annual averages of total, and single-layer, nonoverlapped low, middle and high cloud fractions are 0.49, 0.11, 0.03, and 0.17, respectively. Total and low cloud amounts were greatest from December through March and least during July and August. The monthly variation of high cloud amount is relatively small with a broad maximum from May to August. During winter, total cloud cover varies diurnally with a small amplitude, mid-morning maximum and early evening minimum, and during summer it changes by more than 0.14 over the daily cycle with a pronounced early evening minimum. The diurnal variations of mean single-layer cloud cover change with season and cloud height. Annual averages of all-sky, total, and single-layer high, middle, and low LW CRFs are 21.4, 40.2, 16.7, 27.2, and 55.0 Wm(sup -2), respectively; and their SW CRFs are -41.5, -77.2, -37.0, -47.0, and -90.5 Wm(sup -2). Their net CRFs range from -20 to -37 Wm(sup -2). For all-sky, total, and low clouds, the maximum negative net CRFs of -40.1, -70, and -69.5 Wm(sup -2), occur during April; while the respective minimum values of -3.9, -5.7, and -4.6 Wm(sup -2), are found during December. July is the month having maximum negative net CRF of -46.2 Wm(sup -2) for middle clouds, and May has the maximum value of -45.9 Wm(sup -2) for high clouds. An uncertainty analysis demonstrates that the calculated CRFs are not significantly affected by the difference between clear-sky and cloudy conditions. A more comprehensive cloud fraction study from both surface and satellite observations will follow.

Dong, Xiquan↗

Jupiter Atmospheric Science with JIMO: Linking Science Objectives and Measurement Goals

Although the primary focus of the Jupiter Icy Moons Orbiter (JIMO) mission will be the characterization and study of Jupiter's icy moons, there will be opportunities throughout the mission for unprecendented observations of Jupiter. With an adaptable suite of payload instruments, the atmospheric data collected by JIMO can help to answer fundamental questions about the largest planet in our solar system that remain after (or were generated by) previous spacecraft reconnaissance (e.g. Voyager, Galileo, and Cassini). Near-IR (0.7-4 micron) spectral imaging will most likely be used to identify mineralogies and ices on the Jovian satellites by virtue of their spectral signatures. This same capability is very well tailored for studies of Jovian atmospheric dynamics and structure. Near-IR methane absorption bands allow 2-D mapping of the horizontal wind field at size scales to tens of kms, as well as the height dependence of this field above the ammonia cloud deck (700 to a few mbar), constraining current models of atmospheric vertical structure. Likewise, atmospheric ice aerosols with unique spectroscopic signatures (ammonia ice near 1.5, 2.0, and 2.8 microns and water ice between 3.0 - 3.5 microns) can be detected and mapped using spectral difference imaging or spectrally inclusive principal-component methods. Spectral imaging of the Jovian aurora via (3)H(+) emission lines between 3 - 4 microns can be used to spatially map the interplay between the satellites) Jupiter's magnetosphere, and Jupiter's atmosphere. Each of these measurements addresses one or more fundamental questions related to the energy balance in Jupiter's atmosphere. All of these tunable imaging objectives can be achieved using acousto-optic tunable filters (AOTF's), which have been used for years in ground-based observing instruments and which have been proposed for numerous planetary missions. The application of this technology to the science objectives of both the icy satellites and Jovian atmospheric components of the JIMO mission will be discussed.

Chanover, N. J.↗

Modeling of 2008 Kasatochi Volcanic Sulfate Direct Radiative Forcing: Assimilation of OMI SO2 Plume Height Data and Comparison with MODIS and CALIOP Observations

Volcanic SO2 column amount and injection height retrieved from the Ozone Monitoring Instrument (OMI) with the Extended Iterative Spectral Fitting (EISF) technique are used to initialize a global chemistry transport model (GEOS-Chem) to simulate the atmospheric transport and lifecycle of volcanic SO2 and sulfate aerosol from the 2008 Kasatochi eruption, and to subsequently estimate the direct shortwave, top-of-the-atmosphere radiative forcing of the volcanic sulfate aerosol. Analysis shows that the integrated use of OMI SO2 plume height in GEOS-Chem yields: (a) good agreement of the temporal evolution of 3-D volcanic sulfate distributions between model simulations and satellite observations from the Moderate Resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar with Orthogonal Polarisation (CALIOP), and (b) an e-folding time for volcanic SO2 that is consistent with OMI measurements, reflecting SO2 oxidation in the upper troposphere and stratosphere is reliably represented in the model. However, a consistent (approx. 25 %) low bias is found in the GEOS-Chem simulated SO2 burden, and is likely due to a high (approx.20 %) bias of cloud liquid water amount (as compared to the MODIS cloud product) and the resultant stronger SO2 oxidation in the GEOS meteorological data during the first week after eruption when part of SO2 underwent aqueous-phase oxidation in clouds. Radiative transfer calculations show that the forcing by Kasatochi volcanic sulfate aerosol becomes negligible 6 months after the eruption, but its global average over the first month is -1.3W/sq m, with the majority of the forcing-influenced region located north of 20degN, and with daily peak values up to -2W/sq m on days 16-17. Sensitivity experiments show that every 2 km decrease of SO2 injection height in the GEOS-Chem simulations will result in a approx.25% decrease in volcanic sulfate forcing; similar sensitivity but opposite sign also holds for a 0.03 m increase of geometric radius of the volcanic aerosol particles. Both sensitivities highlight the need to characterize the SO2 plume height and aerosol particle size from space. While more research efforts are warranted, this study is among the first to assimilate both satellite-based SO2 plume height and amount into a chemical transport model for an improved simulation of volcanic SO2 and sulfate transport.

Wang, J.↗