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NASA NTRS1996

Visible/Infrared Optical Depths of Cirrus as Seen by Satellite and Scanning Lidar

The High Spectral Resolution Lidar (HSRL) and the Volume Imaging Lidar (VIL) were combined to produce a quantitative image of the visible optical depth of cirrus clouds. The HSRL was used to calibrate the VIL signal into backscatter cross sections of particulates. The backscatter cross sections were related to extinction by a constant backscatter phase function determined from the HSRL data. This produced a three dimensional image of visual extinction in the cirrus clouds over a one hour period. Two lidar images were constructed from one hour VIL cross section records.

Wylie, Donald↗

NASA NTRS2012

Climate Impacts of Ice Nucleation

Several different ice nucleation parameterizations in two different General Circulation Models (GCMs) are used to understand the effects of ice nucleation on the mean climate state, and the Aerosol Indirect Effects (AIE) of cirrus clouds on climate. Simulations have a range of ice microphysical states that are consistent with the spread of observations, but many simulations have higher present-day ice crystal number concentrations than in-situ observations. These different states result from different parameterizations of ice cloud nucleation processes, and feature different balances of homogeneous and heterogeneous nucleation. Black carbon aerosols have a small (0.06 Wm(exp-2) and not statistically significant AIE when included as ice nuclei, for nucleation efficiencies within the range of laboratory measurements. Indirect effects of anthropogenic aerosols on cirrus clouds occur as a consequence of increasing anthropogenic sulfur emissions with different mechanisms important in different models. In one model this is due to increases in homogeneous nucleation fraction, and in the other due to increases in heterogeneous nucleation with coated dust. The magnitude of the effect is the same however. The resulting ice AIE does not seem strongly dependent on the balance between homogeneous and heterogeneous ice nucleation. Regional effects can reach several Wm2. Indirect effects are slightly larger for those states with less homogeneous nucleation and lower ice number concentration in the base state. The total ice AIE is estimated at 0.27 +/- 0.10 Wm(exp-2) (1 sigma uncertainty). This represents a 20% offset of the simulated total shortwave AIE for ice and liquid clouds of 1.6 Wm(sup-2).

Gettelman, Andrew↗

NASA NTRS1994

Wavelet analysis applied to the IRAS cirrus

The structure of infrared cirrus clouds is analyzed with Laplacian pyramid transforms, a form of non-orthogonal wavelets. Pyramid and wavelet transforms provide a means to decompose images into their spatial frequency components such that all spatial scales are treated in an equivalent manner. The multiscale transform analysis is applied to IRAS 100 micrometer maps of cirrus emission in the north Galactic pole region to extract features on different scales. In the maps we identify filaments, fragments and clumps by separating all connected regions. These structures are analyzed with respect to their Hausdorff dimension for evidence of the scaling relationships in the cirrus clouds.

Langer, William D.↗

NASA NTRS2004

CRYSTAL/FACE

Droplet Measurement Technologies (DMT), under funding from NASA, participated in the CRYSTAL/FACE field campaign in July, 2002 with measurements of cirrus cloud hydrometeors in the size range from 0.5 to 1600 microns. The measurements were made with the DMT Cloud, Aerosol and Precipitation Spectrometer (CAPS) that was flown on NASA's WB57F. With the exception of the first research flight when the data system failed two hours into the mission, the measurement system performed almost flawlessly during the thirteen flights. The measurements from the CAPS have been essential for interpretation of cirrus cloud properties and their impact on climate. The CAPS data set has been used extensively by the CRYSTAL/FACE investigators and as of the date of this report, have been included in five published research articles, 10 conference presentations and six other journal articles currently in preparation.

Baumgardner, Darrel↗

NASA NTRS2006

Improvements in Raman Lidar Measurements Using New Interference Filter Technology

Narrow-band interference filters with improved transmission in the ultra-violet have been developed under NASA-funded research and used in the Raman Airborne Spectroscopic Lidar (RASL) in ground-based, upward-looking tests. Measurements were made of atmospheric water vapor, cirrus cloud optical properties and carbon dioxide that improve upon any previously demonstrated using Raman lidar. Daytime boundary and mixed layer profiling of water vapor mixing ratio up to an altitude of approximately 4 h is performed with less than 5% random error using temporal and spatial resolution of 2-minutes and 60 - 210, respectively. Daytime cirrus cloud optical depth and extinction-to-backscatter ratio measurements are made using 1 -minute average. Sufficient signal strength is demonstrated to permit the simultaneous profiling of carbon dioxide and water vapor mixing ratio into the free troposphere during the nighttime. A description of the filter technology developments is provided followed by examples of the improved Raman lidar measurements.

Whiteman, David N.↗

NASA NTRS2004

Contrail Coverage Over the USA Derived from NOAA and EOS Satellite Data

Contrails, like natural cirrus clouds, can cause a warming of the Earth-atmospheric system by absorbing longwave radiation from the surface and lower troposphere and radiating additional radiation back to the surface. They can also produce some cooling of the surface during the daytime by reflecting some sunlight back to space. Recently, Minnis et al. (2004) determined from surface observations of cirrus cloud cover that the overall impact appears to be a warming that is consistent with theoretical calculations, at least over the United States of America (USA) and surrounding areas. This finding highlights the need to better understand the formation and persistence of contrails and their radiative properties. To better assess the climatic impact of contrails, it is essential to determine the variability of the contrail microphysical properties, their impact on the atmospheric radiation budget, and their relationship to the atmospheric state. To that end, this paper continues the analyses of Advanced Very High Resolution Radiometer (AVHRR) data from the NOAA-15 (N15), NOAA-16 (N16), and NOAA-17 (N17) satellites, Moderate Resolution Imaging Spectroradiometer (MODIS) data from the Terra and Aqua satellites. The combination of these satellites provides a relatively comprehensive coverage of the daily cycle of air traffic. Thus, it should be possible to use these data to help understand the impact of air traffic on the upper tropospheric humidity during the day as well as determine the local-time variability of contrail coverage. The results will be valuable for developing models of contrail effects and methods for mitigating the impact of aviation on climate.

Palikonda, Rabindra↗

NASA NTRS1990

Both sides now

On November 2, 1986 of the cirrus Intensive Field Observations, cirrus clouds were observed from both ground-based and aircraft lidar. The NASA ER2 aircraft carrying a lidar, crossed Madison three times and Wausau five times during its mission. Ground-based lidars from the University of Wisconsin in Madison and the University of Utah in Wausau were operating during the ER2 overpasses. This gave FIRE unique lidar observations of cirrus clouds from both sides. This lidar data are presented and analyzed.

Wylie, Donald P.↗

NASA NTRS2019

Influence of Deep Convection on Cirrus and Water Vapor Concentration in the Upper Troposphere and Lower Stratosphere

It is well known that stratospheric humidity is primarily controlled by freeze drying (ice crystal growth and sedimentation) of air ascending across the cold tropical tropopause. However, the suggestion of an important source of water vapor from deep convection that extends above the tropical tropopause has persisted. There exists much anecdotal evidence of direct convective hydration of the lower stratosphere based on measurements from high altitude aircraft campaigns, but quantifying the impact of deep convection on the overall budget of stratospheric water vapor has proven challenging. The role of convection on the humidity of the upper troposphere and lower stratosphere (UTLS) is investigated in simulations of cirrus clouds along trajectories launched from given potential temperature level surfaces. The one-dimensional (vertical) cloud model tracks individual ice crystals through their life cycles, beginning with nucleation or detrainment from convection, followed by deposition growth, sedimentation and sublimation. Convective influence of the parcels is diagnosed by tracing the trajectories through time-dependent fields of convective cloud-top height adjusted to match the CloudSAT and CALIPSO statistics. Model simulations of UTLS water vapor and cloud fields are evaluated and constrained by comparison with MLS and CALIPSO measurements. The simulation results indicate that the overall impact of convection on water vapor near the tropical tropopause is 10-15%, while the impact on lower stratospheric humidity is no more than a few percent. Ice crystals detrained from deep convection have relatively small effect. The general implications for the importance of deep convection on UTLS humidity and cirrus cloud fraction will be discussed.

Ueyama, Rei↗

NASA NTRS2002

Water Measurements using a Raman Lidar

The research record for the usefulness of Raman Lidar in addressing a broad range of important atmospheric research topics is well established. Raman lidar technology has been used to measure tropospheric aerosols, stratospheric aerosols and cirrus clouds. Arguably the most important measurements offered by Raman lidar for both dynamic and radiative studies, however, is that of water vapor. We will describe large improvements in Raman lidar measurements of water vapor made possible through recent technology upgrades. Furthermore, we will present the use of Raman lidar to study liquid water in the atmosphere and describe current research into the use of Raman lidar measurements to estimate ice water content of cirrus clouds.

Whiteman, D. N.↗

NASA NTRS2000

Processes Controlling Water Vapor in the Winter Arctic Stratospheric Middleworld

Water vapor in the winter arctic stratospheric middleworld is import-an: for two reasons: (1) the arctic middleworld is a source of air for the upper Troposphere because of the generally downward motion, and thus its water vapor content helps determine upper tropospheric water, a critical part of the earth's radiation budget; and (2) under appropriate conditions, relative humidities will be large, even to the point of stratospheric cirrus cloud formation, leading to the production of active chlorine species that could destroy ozone. On a number of occasions during SOLVE, clouds were observed in the stratospheric middleworld by the DC-8 aircraft. These tended to coincide with regions of low temperatures, though some cases suggest water vapor enhancements due to troposphere-to-stratosphere transport. The goal of this work is to understand the importance of processes in and at the edge of the arctic stratospheric middleworld in determining water vapor at these levels. Specifically, is water vapor at these levels determined largely by the descent of air from above, or are clouds both within and at the edge of the stratospheric middleworld potentially important? How important is troposphere-to-stratosphere transport of air in determining stratospheric middleworld water vapor content? To this end, we will first examine the minimum saturation mixing ratios along theta/EPV tubes during the SOLVE winter and compare these with DC-8 water vapor observations. This will be a rough indicator of how high relative humidities can get, and the likelihood of cirrus cloud formation in various parts of the stratospheric middleworld. We will then examine saturation mixing ratios along both diabatic and adiabatic trajectories, comparing these values with actual aircraft water vapor observations, both in situ and remote. Finally, we will attempt to actually predict water vapor using minimum saturation mixing ratios along trajectories, cloud injection (derived from satellite imagery) along trajectories, and suitable initial conditions.

Pfister, Leonhard↗

NASA NTRS1992

Chemistry of the outer planets

Various aspects were studied of past or present chemistry in the atmospheres of the outer planets and their satellites using lab simulations. Three areas were studied: (1) organic chemistry induced by kinetically hot hydrogen atoms in the region of Jupiter's atmosphere containing the ammonia cirrus clouds; (2) the conversion of NH3 into N2 by plasmas associated with entry of meteors and other objects into the atmosphere of early Titan; and (3) the synthesis of simple hydrocarbons and HCN by lightning in mixtures containing N2, CH4, and NH3 representing the atmospheres of Titan and the outer planets. The results showed that: (1) hot H2 atoms formed from the photodissociation of NH3 in Jupiter's atmosphere could account for some of the atmospheric chemistry in the ammonia cirrus cloud region; (2) the thermalization of hot H2 atoms in atmospheres predominated by molecular H is not as rapid as predicted by elastic collision theory; (3) the net quantum loss of NH3 in the presence of a 200 fold excess of H2 is 0.02, much higher than was expected from the amount of H2 present; (4) the conversion of NH3 into N2 in plasmas associated with infalling meteors is very efficient and rapid, and could account for most of the N2 present on Titan; (5) the yields of C2H2 and HCN from lightning induced chemistry in mixtures of CH4 and N2 is consistent with quenched thermodynamic models of the discharge core; and (6) photolysis induced by the UV light emitted by the gases in the hot plasmas may account for some, if not most, of the excess production of C2H6 and the more complex hydrocarbons.

Scattergood, Thomas W.↗

NASA NTRS1986

Point sources in the Orion complex

Point sources identified in Orion with the IRAS are discussed to illustrate methods of using the IRAS Catalog. The present survey revealed 54 new objects. The Catalog was employed to find companion stars for the observed sources, discern those sources which were predominantly IR cirrus clouds, and separate sources with 12 and 25 microns emissions that were both detected at 60 and 100 microns. Attention is also given to usage of the Catalog to determine which sources were galaxies in Orion and which were galaxies in nearby Gemini. Color-color diagrams are provided for 12, 25 and 60 microns emissions to demonstrate how the data permit identification pre-main sequence stars, stars with circumstellar disks, very young stars, stars with cool photospheres, and hot cirrus clouds.

Beichman, C. A.↗

NASA NTRS2001

Mechanisms for Midlatitude Ozone Loss: Heterogeneous Chemistry in the Lowermost Stratosphere?

The question of midlatitude ozone erosion by chlorine free radical catalysis is examined. We present and analyze simultaneous, high-resolution observations of ClO, H2O, tropopause height, particle reactive surface area, and ice saturation occurrence frequency obtained from the NASA ER-2 aircraft. The objective is to test the hypothesis that the existence of cirrus clouds or cold aerosols in the first few kilometers above the tropopause at midlatitudes is responsible for increasing the ratio of chlorine free radicals to total inorganic chlorine, thus amplifying the rate of catalytic ozone destruction. The observations reveal a sharp decrease in ice saturation frequency at the tropopause, a marked degree of undersaturation just above the tropopause, a corresponding sharp gradient in the product of cold aerosol reactive surface area and reaction probability, gamma-S(sub a), and, finally, the consistent absence of enhanced concentrations of ClO immediately above the tropopause. These results suggest that midlatitude ozone loss is not controlled in situ by the mechanism of cirrus cloud and/or cold aerosol enhancement of chlorine radicals in the vicinity of the tropopause.

Smith, Jessica B.↗

NASA NTRSDate not supplied

Aircraft Engine Particle Emissions during the 2023 NASA-Boeing ecoDemonstrator Field Measurements

Aerosol aircraft emissions are responsible for the formation of contrail cirrus clouds which can alter Earth’s radiation and water budgets exerting substantial effects on climate. However, at present, the impact of aviation on climate forcing remaining uncertain. Recently, NASA has collaborated with Boeing ecoDemonstrator program to improve the understanding of air traffic emissions and the impact of different jet fuel compositions on contrail microphysics. As part of the program, in October 2023 the NASA DC-8 aircraft was used to sample engine exhausts emitted by a Boeing ecoDemonstrator Explorer 737-10 burning sustainable aviation fuel (SAF) and conventional jet fuel over the north western US. In this study, we present unique observations of aerosols properties relevant for contrail-cirrus cloud formation collected during the 2023 ecoDemonstrator research flights and we will discuss the variations of key microphysical contrail parameters in function of different jet fuel compositions and engine conditions.

Francesca Gallo↗

NASA NTRS2003

Measurements of the Ice Water Content of Cirrus in the Tropics and Subtropics: Instrument Details and Validation - I

We describe an instrument mounted in a pallet on the NASA WB-57 aircraft that is designed to measure the sum of gas phase and solid phase water, or total water, in cirrus clouds. Using an isokinetic inlet, a 600-watt heater mounted directly in the flow, and Lyman-alpha photofragment fluorescence technique for detection, accurate measurements of total water have been made over almost three orders of magnitude. Isokinetic flow is achieved with an actively controlled roots pump by referencing aircraft pressure, temperature, and true air speed, together with instrument flow velocity, temperature, and pressure. During CRYSTAL FACE, the instrument operated at duct temperatures sufficiently warm to completely evaporate particles up to 150 microns diameter. In flight diagnostics, intercomparison with water measured by absorption in flight, as well as intercomparisons in clear air with water vapor measured by the Harvard water vapor instrument and the JPL infrared tunable diode laser hygrometer validate the detection sensitivity of the instrument and illustrate minimal hysteresis from instrument surfaces. The simultaneous measurement of total water and water vapor in cirrus clouds yields their ice water content.

Weinstock, E. M.↗

DOE OSTI2022

Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic

Abstract. Formation of atmospheric ice plays a crucial role in the microphysical evolution of mixed-phase and cirrus clouds and thus climate. How aerosol particles impact ice crystal formation by acting as ice-nucleating particles (INPs) is a subject of intense research activities. To improve understanding of atmospheric INPs, we examined daytime and nighttime particles collected during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) field campaign conducted in summer 2017. Collected particles, representative of a remote marine environment, were investigated for their propensity to serve as INPs in the immersion freezing (IMF) and deposition ice nucleation (DIN) modes. The particle population was characterized by chemical imaging techniques such as computer-controlled scanning electron microscopy with energy-dispersive X-ray analysis (CCSEM/EDX) and scanning transmission X-ray microscopy with near-edge X-ray absorption fine-structure spectroscopy (STXM/NEXAFS). Four major particle-type classes were identified where internally mixed inorganic–organic particles make up the majority of the analyzed particles. Following ice nucleation experiments, individual INPs were identified and characterized by SEM/EDX. The identified INP types belong to the major particle-type classes consisting of fresh sea salt with organics or processed sea salt containing dust and sulfur with organics. Ice nucleation experiments show IMF events at temperatures as low as 231 K, including the subsaturated regime. DIN events were observed at lower temperatures of 210 to 231 K. IMF and DIN observations were analyzed with regard to activated INP fraction, ice-nucleation active site (INAS) densities, and a water activity-based immersion freezing model (ABIFM) yielding heterogeneous ice nucleation rate coefficients. Observed IMF and DIN events of ice formation and corresponding derived freezing rates demonstrate that the marine boundary layer aerosol particles can serve as INPs under typical mixed-phase and cirrus cloud conditions. The derived IMF and DIN parameterizations allow for implementation in cloud and climate models to evaluate predictive effects of atmospheric ice crystal formation.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1989

Two years of cloud cover statistics using VAS

The CO2 channel radiometric data from VAS are used to chart the frequency of cloud cover, the associated heights, and IR attenuation. Cloud top pressures are calculated from the ratio of VAS CO2 channel radiances in a raditive transfer equation formulation. It is found that VAS CO2 derived cloud top height and emissivity assignments are reliable for most cloud types, including thin cirrus clouds. The observations from 1985 to 1988 show that 20-30 percent of the U.S. was covered with thin semitransparent clouds, 45 percent was covered with thick opaque clouds, and 25-35 had clear sky conditions. The geographical distribution of cloud cover is a latitudinal dependence, mainly over the Pacific Ocean.

Wyle, D. P.↗

NASA NTRS1990

Temporal and spatial variability of the tropical radiation budget from ERBS measurements (March 1985 to February 1986)

The diurnal and regional variations of the top-of-atmosphere radiation budget in the tropics are examined and the relative importance of these variations are assessed. The variations of the radiation components with scene type and the radiative effects of clouds are investigated. The LW emission shows the strongest diurnal variation over clear desert and land scenes, with domain-averaged diurnal ranges of approximately 50 W/sq m and 35 W/sq m, respectively. The LW emission over clear and tropical oceans show a small diurnal range of less than 1 W/sq m. A bias in the ERBE scene ID algorithm against clear tropical scenes at night is evident in the LW diurnal variation results for clear scenes. The effect of tropical water vapor resulting in low LW emission to space is diagnosed as the principal source of uncertainty in scene identification at night. Regional cloud forcing results show a strong dependence of net forcing on cloud type. While high cirrus clouds largely contribute to a small positive net forcing, low stratiform clouds primarily account for a large negative net forcing.

Chang, T. Y.↗