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Transition Energies and Absorption Oscillator Strengths for c{sub 4}{sup ′1}Σ{sub u}{sup +}−X{sup 1}Σ{sub g}{sup +}, b{sup ′1}Σ{sub u}{sup +}−X{sup 1}Σ{sub g}{sup +}, and c{sub 5}{sup ′1}Σ{sub u}{sup +}−X{sup 1}Σ{sub g}{sup +} Band Systems in N{sub 2}

Theoretical transition energies and absorption oscillator strengths for the c{sub 4}{sup ′1}Σ{sub u}{sup +} (v′ = 0–2, 5, 7, 8) − X{sup 1}Σ{sub g}{sup +}(v{sup ′′}=0--14) and c{sub 5}{sup ′1}Σ{sub u}{sup +} (v′ = 0, 2) − X{sup 1}Σ{sub g}{sup +} (v″ = 0–14) Rydberg bands, and b{sup ′1}Σ{sub u}{sup +} (v′ = 0–9, 11, 12, 14–19, 21, 22) − X{sup 1}Σ{sub g}{sup +} (v″ = 0–14) valence bands of molecular nitrogen are reported. The strong interaction between {sup 1}Σ{sub u}{sup +} states has been dealt with through a vibronic interaction matrix. As a consequence of the Rydberg-valence interaction, irregularities in the vibrational structure of the above band systems are observed. Good agreement is found with the scarce high-resolution data that are available for oscillator strengths. The new band oscillator strengths reported here may be useful for a reliable interpretation of the spectra from atmospheres of the Earth, Titan, and Triton, where N{sub 2} is the mayor constituent.

79 ASTRONOMY AND ASTROPHYSICS↗

Microwave-assisted synthesis of well-shaped UiO-66-NH2 with high CO2 adsorption capacity

Highlights: • Well-shaped UiO-66-NH{sub 2} was prepared through microwave heating in a short time. • Addition of HAc improves crystallinity and CO{sub 2} adsorption capacity of the UiO-66-NH{sub 2}. • UiO-66-NH{sub 2} prepared by microwave heating shows a higher CO{sub 2}/N{sub 2} adsorption selectivity. - Abstract: In a detailed study, the influence of microwave irradiation, synthesis time and temperature, addition of acetic acid (HAc) as a modulator on the morphology, crystallinity and stability of UiO-66-NH{sub 2} is investigated to develop a reliable and reproducible strategy for the preparation of well-shaped UiO-66-NH{sub 2}. The UiO-66-NH{sub 2} were characterized by powder X-ray diffraction (PXRD), field emission scanning electron microscopy (FESEM), thermogravimetric analysis (TGA), and gas adsorption. It is found that well-shaped UiO-66-NH{sub 2} with a high CO{sub 2} adsorption capacity can be synthesized in a short time by microwave heating. The UiO-66-NH{sub 2} crystals synthesized by microwave heating are of high quality and show a superior CO{sub 2} adsorption capacity (5.8 mmol/g at 273k and 1 bar) due to the strong interactions between the −NH{sub 2} group and CO{sub 2}. The CO{sub 2}/N{sub 2} selectivity of the obtained UiO-66-NH{sub 2} at 298 K and 1 bar is 66, which is much higher than that of the pristine UiO-66 of 17.8.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Electrically tuned hyperfine spectrum in neutral Tb( II )(Cp iPr5 ) 2 single-molecule magnet

Molecular spin qubits with long spin coherence time as well as non-invasive operation methods on such qubits are in high demand. It was shown that both molecular electronic and nuclear spin levels can be used as qubits. In solid state systems with dopants, an electric field was shown to effectively change the spacing between the nuclear spin qubit levels when the electron spin density is high at the nucleus of the dopant. Inspired by such solid-state systems, we propose that divalent lanthanide (Ln) complexes with an unusual electronic configuration of Ln 2+ have a strong interaction between the Ln nuclear spin and the electronic degrees of freedom, which renders electrical tuning of the interaction. Furthermore, as an example, we study electronic structure and hyperfine interaction of the 159 Tb nucleus in a neutral Tb(II)(Cp iPr5 ) 2 single-molecule magnet (SMM), which exhibits unusually long magnetization relaxation time, using the complete active space self-consistent field (CASSCF) method with spin–orbit interaction included within the restricted active space state interaction (RASSI). Our calculations show that the low-energy states arise from 4f 8 (6s,5d z 2 ) 1 , 4f 8 (5d x 2 -y 2 ) 1 , and 4f 8 (5d xy ) 1 configurations. We compute the hyperfine interaction parameters and the electronic–nuclear spectrum within our multiconfigurational approach. We find that the hyperfine interaction is about one order of magnitude greater than that for Tb(III)Pc 2 SMMs. This stems from the strong Fermi contact interaction between the Tb nuclear spin and the electron spin density at the nucleus that originates from the occupation of the (6s,5d) orbitals. We also uncover that the response of the Fermi contact term to electric field results in electrical tuning of the electronic–nuclear level separations. This hyperfine Stark effect may be useful for applications of molecular nuclear spins for quantum computing.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Tensor observables in electro- and photoreactions on the deuteron

The study of polarization effects in reactions with a simplest nucleus, deuteron, plays an important role for the investigation of deuteron structure as well as for the research of the properties of the strong interaction. However, data on the tensor observables in the electro- and photoreactions with deuteron appeared not so long ago. We present here a brief overview of the experiments on three such reactions with a deuteron: elastic scattering, photodisintegration and coherent photoproduction of the neutral pion.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Calcined Mg-Fe layered double hydroxide as an absorber for the removal of methyl orange

In this work, methyl orange (MO) was effectively removed from aqueous solution with the calcined product of hydrothermal synthesized Mg/Fe layered double hydroxide (Mg/Fe-LDH). The structure, composition, morphology and textural properties of the Mg/Fe-LDH before and after adsorption were characterized by X-ray diffraction, Fourier transformation infrared spectroscopy, transmission electron microscopy, nitrogen adsorption apparatus and X-ray photoelectron spectroscopy. It was confirmed that MO had been absorbed by calcined Mg/Fe-LDH which had strong interactions with MO. The adsorption of MO onto the Mg/Fe-LDH was systematically investigated by batch tests. The adsorption capacity of the Mg/Fe-LDH toward MO was found to be 194.9 mg • g{sup −1}. Adsorption kinetics and isotherm studies revealed that the adsorption of MO onto Mg/Fe-LDH was a spontaneous and endothermic process. These results indicate that Mg/Fe-LDH is a promising material for the removal of MO.

36 MATERIALS SCIENCE↗

Feedback by AGN Jets and Wide-angle Winds on a Galactic Scale

To investigate the differences in mechanical feedback from radio-loud and radio-quiet active galactic nuclei on the host galaxy, we perform 3D AMR hydrodynamic simulations of wide-angle, radio-quiet winds with different inclinations on a single, massive, gas-rich disk galaxy at a redshift of 2–3. We compare our results to hydrodynamic simulations of the same galaxy but with a jet. The jet has an inclination of 0° (perpendicular to the galactic plane), and the winds have inclinations of 0°, 45°, and 90°. We analyze the impact on the host’s gas, star formation, and circumgalactic medium. We find that jet feedback is energy-driven and wind feedback is momentum-driven. In all the simulations, the jet or wind creates a cavity mostly devoid of dense gas in the nuclear region where star formation is then quenched, but we find strong positive feedback in all the simulations at radii greater than 3 kpc. All four simulations have similar SFRs and stellar velocities with large radial and vertical components. However, the wind at an inclination of 90° creates the highest density regions through ram pressure and generates the highest rates of star formation due to its ongoing strong interaction with the dense gas of the galactic plane. With increased wind inclination, we find greater asymmetry in gas distribution and resulting star formation. Our model generates an expanding ring of triggered star formation with typical velocities of the order of 1/3 of the circular velocity, superimposed on the older stellar population. This should result in a potentially detectable blue asymmetry in stellar absorption features at kiloparsec scales.

79 ASTRONOMY AND ASTROPHYSICS↗

The Fornax Deep Survey with VST. I. The extended and diffuse stellar halo of NGC 1399 out to 192 kpc

We have started a new, deep multi-imaging survey of the Fornax cluster, dubbed the Fornax Deep Survey (FDS), at the VLT Survey Telescope (VST). In this paper we present the deep photometry inside two square degrees around the bright galaxy NGC 1399 in the core of the cluster. We found that the core of the Fornax cluster is characterized by a very extended and diffuse envelope surrounding the luminous galaxy NGC 1399: we map the surface brightness out to 33 arcmin (∼192 kpc) from the galaxy center and down to μ{sub g} ∼ 31 mag arcsec{sup −2} in the g band. The deep photometry allows us to detect a faint stellar bridge in the intracluster region on the west side of NGC 1399 and toward NGC 1387. By analyzing the integrated colors of this feature, we argue that it could be due to the ongoing interaction between the two galaxies, where the outer envelope of NGC 1387 on its east side is stripped away. By fitting the light profile, we found that there exists a physical break radius in the total light distribution at R = 10 arcmin (∼58 kpc) that sets the transition region between the bright central galaxy and the outer exponential halo, and that the stellar halo contributes 60% of the total light of the galaxy (Section 3.5). We discuss the main implications of this work on the build-up of the stellar halo at the center of the Fornax cluster. By comparing with the numerical simulations of the stellar halo formation for the most massive bright cluster galaxies (i.e., 13<logM{sub 200}/M{sub ⊙}<14), we find that the observed stellar halo mass fraction is consistent with a halo formed through the multiple accretion of progenitors with stellar mass in the range 10{sup 8}–10{sup 11} M{sub ⊙}. This might suggest that the halo of NGC 1399 has also gone through a major merging event. The absence of a significant number of luminous stellar streams and tidal tails out to 192 kpc suggests that the epoch of this strong interaction goes back to an early formation epoch. Therefore, different from the Virgo cluster, the extended stellar halo around NGC 1399 is characterized by a more diffuse and well-mixed component, including the intracluster light.

79 ASTRONOMY AND ASTROPHYSICS↗

A novel metal-organic framework for high storage and separation of acetylene at room temperature

A novel 3D microporous metal-organic framework with NbO topology, [Cu{sub 2}(L)(H{sub 2}O){sub 2}]∙(DMF){sub 6}·(H{sub 2}O){sub 2} (ZJU-10, ZJU = Zhejiang University; H{sub 4}L =2′-hydroxy-[1,1′:4′,1″-terphenyl]-3,3″,5,5″-tetracarboxylic acid; DMF =N,N-dimethylformamide), has been synthesized and structurally characterized. With suitable pore sizes and open Cu{sup 2+} sites, ZJU-10a exhibits high BET surface area of 2392 m{sup 2}/g, as well as moderately high C{sub 2}H{sub 2} volumetric uptake capacity of 132 cm{sup 3}/cm{sup 3}. Meanwhile, ZJU-10a is a promising porous material for separation of acetylene from methane and carbon dioxide gas mixtures at room temperature. - Graphical abstract: A new NbO-type microporous metal-organic framework ZJU-10 with suitable pore size and open Cu{sup 2+} sites was synthesized to realize the strong interaction with acetylene molecules, which can separate the acetylene from methane and carbon dioxane gas mixtures at room temperature. Display Omitted - Highlights: • A novel 3D NbO-type microporous metal-organic framework ZJU-10 was solvothermally synthesized and structurally characterized. • ZJU-10a exhibits high BET surface area of 2392 m{sup 2}/g. • ZJU-10a shows a moderately high C{sub 2}H{sub 2} gravimetric (volumetric) uptake capacity of 174 (132) cm{sup 3}/g at 298 K and 1 bar. • ZJU-10a can separate acetylene from methane and carbon dioxide gas mixtures at room temperature.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Electrochemical recovery of Nd using liquid metals (Bi and Sn) in LiCl-KCl-NdCl 3

Highly efficient recovery of Nd into liquid metals of Bi and Sn was achieved in molten LiCl-KCl-NdCl 3 electrolyte at 773–973 K by leveraging the strong interactions of Nd with liquid metals. Based on the emf measurements of Nd-Sn and Nd-Bi alloys, the activity values of Nd were determined as low as 1.1–5.8×10 –13 in both liquid metals at 973 K while the solubility of Nd was found to be 1.46 mol% in Sn and 5.65 mol% in Bi. Both liquid metals demonstrated high round-trip coulombic efficiencies (>99.3%) during deposition-removal cycles of 10–50 mA cm –2 and high recovery capacity up to approximately 20 mol% Nd beyond the solubility limit. In addition, a high Nd recovery yield (84–90%) with respect to the applied charge was confirmed based on chemical analysis of electrolysis products in Bi after constant current electrolysis (–50 mA cm –2 ) at 873–973 K. Overpotentials during the Nd deposition process were attributed to charge-transfer and mass-transport resistances based on the current-potential curve and electrochemical impedance spectroscopy. The charge-transfer kinetics of Nd deposition into liquid metals was facile with high exchange current densities at ~220 mA cm –2 . Finally, the exceptionally high recovery efficiency for Nd in the molten chloride is thought to result from strong chemical interactions (i.e., low activity) of Nd in liquid metals that encourage one-step reduction, i.e., Nd 3+ + 3e → Nd(in Bi or Sn) by effectively suppressing side reaction pathways from multivalent states (Nd 2+ and Nd 3+ ).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Experimental Determination of the QCD Effective Charge α g1 ( Q )

The QCD effective charge α g1 (Q) is an observable that characterizes the magnitude of the strong interaction. At high momentum Q, it coincides with the QCD running coupling α s (Q). At low Q, it offers a nonperturbative definition of the running coupling. We have extracted α g1 (Q) from measurements carried out at Jefferson Lab that span the very low to moderately high Q domain, 0.14 ≤ Q ≤ 2.18 GeV. The precision of the new results is much improved over the previous extractions and the reach in Q at the lower end is significantly expanded. The data show that α g1 (Q) becomes Q-independent at very low Q. They compare well with two recent predictions of the QCD effective charge based on Dyson–Schwinger equations and on the AdS/CFT duality.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Updates on the Studies of $${\varvec{N}}^\mathbf{*}$$ N * Structure with CLAS and the Prospects with CLAS12

Here, the recent results on $\gamma_vpN^*$ electrocouplings from analyses of the data on exclusive meson electroproduction off protons measured with the CLAS detector at Jefferson Lab are presented. The impact of these results on the exploration of the excited nucleon state structure and non-perturbative strong interaction dynamics behind its formation is outlined. The future extension of these studies in the experiments with the CLAS12 detector in the upgraded Hall-B at JLab will provide for the first time $\gamma_vpN^*$ electrocouplings of all prominent resonances at the still unexplored distance scales that correspond to extremely low (0.05~GeV$^2 < Q^2 <$ 0.5~GeV$^2$) and the highest photon virtualities (5.0~GeV$^2 < Q^2 <$ 12.0~GeV$^2$) ever achieved in the exclusive electroproduction measurements. The expected results will address the most important open problems of the Standard Model: on the nature of more than 98\% of hadron mass, quark-gluon confinement and emergence of the excited nucleon state structure from the QCD Lagrangian, as well as allowing a search for the new states of hadron matter predicted from the first principles of QCD, the so-called hybrid baryons.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

SO(3) “Nuclear Physics” with ultracold Gases☆

An ab initio calculation of nuclear physics from Quantum Chromodynamics (QCD), the fundamental SU(3) gauge theory of the strong interaction, remains an outstanding challenge. Here, we discuss the emergence of key elements of nuclear physics using an SO(3) lattice gauge theory as a toy model for QCD. We show that this model is accessible to state-of-the-art quantum simulation experiments with ultracold atoms in an optical lattice. First, we demonstrate that our model shares characteristic many-body features with QCD, such as the spontaneous breakdown of chiral symmetry, its restoration at finite baryon density, as well as the existence of few-body bound states. Then we show that in the one-dimensional case, the dynamics in the gauge invariant sector can be encoded as a spin S=(3/2) Heisenberg model, i.e., as quantum magnetism, which has a natural realization with bosonic mixtures in optical lattices, and thus sheds light on the connection between non-Abelian gauge theories and quantum magnetism.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Large-momentum effective theory

Since the parton model was introduced by Feynman more than 50 years ago, much has been learned about the partonic structure of the proton through a large body of high-energy experimental data and dedicated global fits. However, limited progress has been made in calculating partonic observables such as the parton distribution function (PDFs) from the fundamental theory of strong interactions, quantum chromodynamics (QCD). Recently some advocated for a formalism, large-momentum effective theory (LaMET), through which one can extract parton physics from the properties of the proton traveling at a moderate boost factor such as γ ~ 2 – 5 . The key observation behind this approach is that Lorentz symmetry allows the standard formalism of partons in terms of light-front operators to be replaced by an equivalent one with large-momentum states and time-independent operators of a universality class. With LaMET, the PDFs, generalized PDFs or generalized parton distributions, transverse-momentum-dependent PDFs, and light-front wave functions can all be extracted in principle from lattice simulations of QCD (or other nonperturbative methods) through standard effective field theory matching and running. Future lattice QCD calculations with exascale computational facilities could help one to understand the experimental data related to the hadronic structure, including those from the upcoming electron-ion colliders dedicated to exploring the partonic landscape of the proton. In this work, the progress made in the past few years in the development of the LaMET formalism and its applications is reviewed, with an emphasis on a demonstration of its effectiveness from initial lattice QCD simulations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Insights into the emergence of mass from studies of pion and kaon structure

There are two mass generating mechanisms in the standard model of particle physics (SM). One is related to the Higgs boson and fairly well understood. The other is embedded in quantum chromodynamics (QCD), the SM’s strong interaction piece; and although responsible for emergence of the roughly 1 GeV mass scale that characterises the proton and hence all observable matter, the source and impacts of this emergent hadronic mass (EHM) remain puzzling. As bound states seeded by a valence-quark and -antiquark, pseudoscalar mesons present a simpler problem in quantum field theory than that associated with the nucleon. Consequently, there is a large array of robust predictions for pion and kaon properties whose empirical validation will provide a clear window onto many effects of both mass generating mechanisms and the constructive interference between them. This has now become significant because new-era experimental facilities, in operation, construction, or planning, are capable of conducting such tests and thereby contributing greatly to resolving the puzzles of EHM. These aspects of experiment, phenomenology, and theory, along with contemporary successes and challenges, are reviewed herein. In addition to providing an overview of the experimental status, we focus on recent progress made using continuum Schwinger function methods and lattice-regularised QCD. Further, advances made using other theoretical tools are also sketched. Our primary goal is to highlight the potential gains that can accrue from a coherent effort aimed at finally reaching an understanding of the character and structure of Nature’s Nambu–Goldstone modes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Lattice QCD Calculation of Nucleon Structure

It is emphasized in the 2015 NSAC Long Range Plan that "understanding the structure of hadrons in terms of QCD's quarks and gluons is one of the central goals of modern nuclear physics." Over the last three decades, lattice QCD has developed into a powerful tool for ab initio calculations of strong-interaction physics. Up until now, it is the only theoretical approach to solving QCD with controlled statistical and systematic errors. Since 1985, we have proposed and carried out first-principles calculations of nucleon structure and hadron spectroscopy using lattice QCD which entails both algorithmic development and large-scale computer simulation. We started out by calculating the nucleon form factors -- electromagnetic, axial-vector, πNN, and scalar form factors, the quark spin contribution to the proton spin, the strangeness magnetic moment, the quark orbital angular momentum, the quark momentum fraction, and the quark and glue decomposition of the proton momentum and angular momentum. The first round of calculations were done with Wilson fermions in the `quenched' approximation where the dynamical effects of the quarks in the sea are not taken into account in the Monte Carlo simulation to generate the background gauge configurations. Beginning in 2000, we have started implementing the overlap fermion formulation into the spectroscopy and structure calculations. This is mainly because the overlap fermion honors chiral symmetry as in the continuum. It is going to be more and more important to take the symmetry into account as the simulations move closer to the physical point where the u and d quark masses are as light as a few MeV only. We began with lattices which have quark masses in the sea corresponding to a pion mass at ~ 300 MeV and obtained the strange form factors, charm and strange quark masses, the charmonium spectrum and the D s meson decay constant f D s , the strangeness and charmness, the meson mass decomposition and the strange quark spin from the anomalous Ward identity. Recently, we have started to include multiple lattices with different lattice spacings and different volumes including large lattices at the physical pion mass point. We are getting quite close to being able to calculate the hadron structure at the physical point and to do the continuum and large volume extrapolations, which is our ultimate aim. We have now finished several projects which have included these systematic corrections. They include the leptonic decay width of the ρ, the πN sigma and strange sigma terms, and the strange quark magnetic moment. Over the years, we have also studied hadron spectroscopy with lattice calculations and in phenomenology. These include Roper resonance, pentaquark state, charmonium spectrum, glueballs, scalar mesons a 0 (1450) and σ(600) and other scalar mesons, and the 1 -+ meson. In addition, we have employed the canonical approach to explore the first-order phase transition and the critical point at finite density and finite temperature. We have also discovered a new parton degree of freedom -- the connected sea partons, from the path-integral formulation of the hadronic tensor, which explains the experimentally observed Gottfried sum rule violation. Combining experimental result on the strange parton distribution, the CT10 global fitting results of the total u and d anti-partons and the lattice result of the ratio of the momentum fraction of the strange vs that of u or d in the disconnected insertion, we have shown that the connected sea partons can be isolated. In this final technical report, we shall present a few representative highlights that have been achieved in the project.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Atomically Thin Polymer Layer Enhances Toughness of Graphene Oxide Monolayers

During the last decade, two-dimensional (2D)materials have emerged as versatile building blocks for the next generation of engineered materials. However, the intrinsically brittle behavior of 2D materials has thus far delayed their adoption in applications such as sensors and structural materials. Herein, we demonstrate a strategy for toughening graphene oxide (GO) through synergistic interfacial interactions between GO monolayers and ultrathin layers of strongly interacting poly(vinyl alcohol) (PVA). By creating GO-PVA and PVA-GO-PVA nanolaminates, we demonstrate a 2-fold increase in GO toughness, which translates into dramatic increases in energy dissipation and piercing resistance. Atomistic simulations show that this remarkable behavior arises from a polymer chain crack-bridging mechanism, resulting froma synergistic combination of interdomain reinforcements across the GO monolayer and extensive GO-polymer interfacial hydrogen-bonding interactions. Here, the reported findings highlight the potential for achieving engineered 2D materials with superior mechanical properties by incorporating deformation and failure-resistant mechanics arising from tailored chemical interactions between constituents.

2D materials↗

Toward Long-Range Entanglement between Electrically Driven Single-Molecule Magnets

Over the past two decades, several molecules have been explored as possible building blocks of a quantum computer, a device that would provide exponential speedups for a number of problems, including the simulation of large, strongly correlated chemical systems. Achieving strong interactions and entanglement between molecular qubits remains an outstanding challenge. In this research, we show that the TbPc 2 single-molecule magnet has the potential to overcome this obstacle because of its sensitivity to electric fields stemming from the hyperfine Stark effect. We show how this feature can be leveraged to achieve long-range entanglement between pairs of molecules using a superconducting resonator as a mediator. Our findings suggest that the molecule–resonator interaction is near the edge of the strong-coupling regime and could potentially pass into it given a more detailed, quantitative understanding of the TbPc 2 molecule.

superconducting resonator↗

Interacting dark sector and precision cosmology

We consider a recently proposed model in which dark matter interacts with a thermal background of dark radiation. Dark radiation consists of relativistic degrees of freedom which allow larger values of the expansion rate of the universe today to be consistent with CMB data (H 0 -problem). Scattering between dark matter and radiation suppresses the matter power spectrum at small scales and can explain the apparent discrepancies between ΛCDM predictions of the matter power spectrum and direct measurements of Large Scale Structure LSS (σ 8 -problem). We go beyond previous work in two ways: 1. we enlarge the parameter space of our previous model and allow for an arbitrary fraction of the dark matter to be interacting and 2. we update the data sets used in our fits, most importantly we include LSS data with full k-dependence to explore the sensitivity of current data to the shape of the matter power spectrum. We find that LSS data prefer models with overall suppressed matter clustering due to dark matter - dark radiation interactions over ΛCDM at 3-4 σ. However recent weak lensing measurements of the power spectrum are not yet precise enough to clearly distinguish two limits of the model with different predicted shapes for the linear matter power spectrum. In two Appendices we give a derivation of the coupled dark matter and dark radiation perturbation equations from the Boltzmann equation in order to clarify a confusion in the recent literature, and we derive analytic approximations to the solutions of the perturbation equations in the two physically interesting limits of all dark matter weakly interacting or a small fraction of dark matter strongly interacting.

79 ASTRONOMY AND ASTROPHYSICS↗