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At least 361 records · Page 20

Fabrication and testing of high-performance all-metal neutron guides and axisymmetric mirrors by electrochemical replication

Neutron scattering is one of the most useful methods of studying the structure of matter, with applications to biomedical, structural, magnetic and energy-related materials. Neutron-scattering instruments are installed around research reactors or accelerator-based neutron sources, and neutron guides are critical components of these facilities. They are neutron-transport optical devices consisting of state-of-the-art mirrors often tens of meters long. Here we demonstrate a novel fabrication method of all-metallic neutron guides and axisymmetric mirrors by electroplating from precision mandrels. The process allows for the fabrication of single-piece all-metal guides of prismatic and axisymmetric shapes. We also demonstrate supermirror guides and axisymmetric focusing supermirrors produced with the same technology. We present the fabrication and tests of the multilayer-coated replicated guides and optic and show that the mandrel is reproduced with high fidelity and reliability. Furthermore, such supermirror optics will provide game-changing improvements in neutron techniques.

36 MATERIALS SCIENCE↗

Verification and Validation of the STAT7 Code

This document presents the verification and validation of the STAT7 Version 1.0 code which has been developed to perform the steady-state thermal hydraulic safety calculation of the MIT Research Reactor required upon conversion of the reactor from high enrichment uranium fuel to low enrichment uranium fuel. The key capabilites of the code including the statistical processing, water property generation, and thermal hydraulic solution are verified independently. While the first two capabilites are checked using statistical tests and NIST data tables, each component of the thermal hydraulic solution is verified using simple geometry test problems. The comparison between results obtained by the code and hand calculations on these problems shows that each of these components work correctly. Additionally, a comprehensive comparison between STAT7 Version 1.0 and PLTEMP/ANL Version 4.2 calculations for a five-channel test problem is performed for the validation. The good agreement between the obtained results for all thermal hydraulic parameters belonging to the fuel core region is achieved. An issue in bypass flowrate calculation was detected when both fin-friction and bypass flow claculations are involved. This problem can be corrected in a later version of the code, however, does not affect the application of STAT7 code as it has been used to date where the flow distribution in the core region and bypass channel is specified as an input parameter.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Feasibility Study for a Subcritical Assembly at the Oak Ridge National Laboratory

A conceptual design has been completed for a new subcritical assembly at Oak Ridge National Laboratory (ORNL). This subcritical assembly will support the Nuclear Criticality Safety Program (NCSP) training and education program to augment current subcritical assembly capabilities at Sandia National Laboratories (SNL) and at the National Criticality Experiments Research Center (NCERC). The proposed subcritical assembly uses legacy AGN-201M research reactor fuel plates that are available at the Y-12 National Security Complex. This subcritical assembly contains approximately 620 grams of 235 U as UO 2 particulates distributed homogeneously in radiation-stabilized polyethylene. The fuel plates will have a graphite neutron reflector to obtain a core multiplication, $M$, from 10 to 50, corresponding to a k eff of 0.9 to 0.95, respectively. The subcritical assembly will be able to support at least four experiments for the training courses: the addition of fissile material to increase neutron multiplication (mass), a core separation experiment (interaction), the effect of adding moderators to the core (moderation), and the effect of adding neutron absorbers to the core (poison/absorption). The proposed ORNL subcritical assembly will provide additional student bandwidth to support NCSP training courses and to provide for some backup capacity in the event that nuclear facility operations are disrupted at SNL or NCERC due to some unforeseen issue. The subcritical assembly will be designed to be an inherently safe subcritical assembly—subcritical under all normal and abnormal conditions—and it will provide the capability to conduct hands-on training to support NCSP and general nuclear criticality safety (NCS) staff training and qualification goals.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Verification and Validation of the STAT7 Code

This document presents the verification and validation of the STAT7 Version 1.0 code which has been developed to perform the steady-state thermal hydraulic safety calculation of the MIT Research Reactor required upon conversion of the reactor from highly enriched uranium fuel to low- enriched uranium fuel. The key capabilities of the code including the statistical processing, water property generation, and thermal hydraulic solution are verified independently. While the first two capabilities are checked using statistical tests and NIST data tables, each component of the thermal hydraulic solution is verified using simple geometry test problems. The comparison between results obtained by the code and hand calculations on these problems shows that each of these components work correctly. Additionally, a comprehensive comparison between STAT7 Version 1.0 and PLTEMP/ANL Version 4.2 calculations for a five-channel test problem is performed for the validation. The good agreement between the obtained results for all thermal hydraulic parameters belonging to the fuel core region is achieved. An issue in bypass flowrate calculation was detected when both fin-friction and bypass flow calculations are involved. This problem can be corrected in a later version of the code. However, it does not affect the application of STAT7 as it has been used to date where the flow distribution in the core region and bypass channel is specified as an input parameter.

97 MATHEMATICS AND COMPUTING↗

Review of the Technical Basis for Properties and Fuel Performance Data Used in HEU to LEU Conversion Analysis for U-10Mo Monolithic Alloy Fuel

This report provides the technical basis for properties and fuel performance data used in conversion analysis for U.S. High Performance Research Reactors (USHPRR) that will convert from highly enriched uranium (HEU) to low-enriched uranium (LEU) using a new U-10Mo monolithic alloy fuel that is being qualified. The conditions that the fuel experiences changes between an HEU and LEU fuel element design due to many causes, including the density of the fuel, the presence of U-238 resonant absorber, changes to the plate and coolant channel dimensions, and changes in fuel management due to reactivity or optimization. These types of changes have been documented in operational and safety analyses conducted for conversions over decades for over 70 reactors. These conversions have all, or almost all, required recalculation of safety-related values as well as establishing operational characteristics of the core, including power distribution, reactor core power level, and cycle length between required fuel management. An overall objective of conversion is to change the reactor core design as little as possible while maintaining the reactors’ scientific, isotope production, medical, and engineering missions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Reduced Neutralization Feasibility Study for H-Canyon Accelerated Basin De- Inventory (ABD) Program

An alternative approach to Spent Nuclear Fuel (SNF) and Nuclear Material Processing was developed for future H-Canyon (HCAN) and L-Area operations that involves a paradigm shift from current HCAN, Concentrate, Storage, and Transfer Facility (CSTF), and Defense Waste Processing Facility (DWPF) operations. The alternative, referred to as Accelerated Basin De-inventory (ABD), requires that all Domestic and Foreign Research Reactor SNF currently at the Savannah River Site (SRS) will be dissolved, stored, and then transferred to CSTF without recovery of Highly Enriched Uranium (HEU). Concentrated nitric acid is utilized to dissolve aluminum spent nuclear fuel (ASNF) in HCAN. The vessels and piping in HCAN are fabricated from 304L stainless steel and are ideally suited to handle the acidic waste stream. However, as the waste is transferred to the CSTF and DWPF, it will contact the carbon steel waste tanks in CSTF. In order to prevent corrosion of the carbon steel, the acidic waste is neutralized (i.e., pH adjusted over 11) by the addition of sodium hydroxide (NaOH). The NaOH is added until the final solution contains 1.2 M excess -OH. Additionally, if the waste is not neutralized to a pH greater than 11, then aluminum hydroxide (Al(OH) 3 ) would form, and solids may form in the piping as it is transferred to CSTF. This document presents an analysis of the influence of reducing the excess caustic that is added to the neutralization tanks on the corrosion protection scheme primarily for the CSTF waste tanks. The implications to HCAN and DWPF were also assessed.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Active Irradiation Testing of Temperature Sensing Capability of Clad Sapphire Optical Fibers with Type 2 Bragg Gratings using Optical Backscatter Reflectometry

This work investigated the temperature-sensing capabilities of Type II fiber Bragg gratings (FBGs) inscribed in sapphire optical fiber in the Ohio State University Research Reactor (OSURR). A Luna Innovations 4600 optical backscatter reflectometer (OBR) was used to interrogate FBGs in three sapphire optical fibers with an internal cladding that was developed by Ohio State. The sapphire fibers were fusion-spliced to silica lead fibers. In addition to the sapphire fibers, two silica fibers with the same Type II FBGs were included in the experiment as a reference. The fiber-based sensors were irradiated in the Central Irradiation Facility (CIF) of the OSURR for a total of 40 hours over 5 days at a reactor power of 450 kW, resulting in a total neutron fluence of approximately 2.5 × 10 18 n/cm 2 and a gamma dose of approximately 3.48 Grad. Two K-type thermocouples were included within the rig: one at the core centerline and the other 12 inches above the top of the core. The temperature was not actively controlled, but the thermocouples were used to provide a reference to which the fiber-based temperature measurements could be compared.

36 MATERIALS SCIENCE↗

Demonstration of Defense Waste Processing Facility (DWPF) Higher Fissile Content Glass

The Accelerated Basin De-inventory (ABD) Program has been proposed as an alternative for future spent nuclear fuel (SNF) and nuclear material processing at the Savannah River Site (SRS). This approach would change the baseline H-Canyon (HCAN), Concentrate, Storage, and Transfer Facility (CSTF), and Defense Waste Processing Facility (DWPF) operations. The ABD Program would require that all domestic and foreign research reactor SNF currently at SRS be dissolved, stored, and then transferred to CSTF without the recovery of uranium. Preliminary assessments in the ABD Program plan have shown that ~5000 extra SRS high-level waste (HLW) canisters would be produced if the fissile mass loading remains at the current 897 g/m 3 limit; however, increasing the limit to 2500 g/m 3 would result in ~520 extra canisters. Thus, the ABD Program plan requires an increase of the DWPF fissile mass loading limit to 2500 g/m 3 to minimize canister production. DWPF considers the following isotopes in the calculation of fissile mass loading: U-233, U-235, Pu-239 and Pu-241.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Y-12 National Security Complex LEU-Mo Feedstock Fabrication Update

Y-12's primary responsibility is to establish a reliable fabrication process of low-enriched uranium-molybdenum feedstock for United States High Performance Research Reactors. This update compares feedstock fabrication efforts over the past several casting campaigns.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of Cable Aging Acceptance Criteria for Nuclear Facilities

The aging of nuclear power plant electrical cables has been the subject of substantial research and development (R&D) projects in the nuclear industry, national and international laboratories, universities, and vendor organizations for several years. More specifically, these R&D efforts were conducted to develop equipment and techniques for assessing age-related degradation of in-service cables in nuclear facilities including power plants, research reactors, waste facilities and fuel fabrication plants. In recent years, cable R&D efforts in the nuclear arena have also included work to develop new cables for the next generation of reactors. Over time, exposure to harsh environmental conditions such as elevated temperatures, radiation, and humidity in nuclear installations can result in age-related degradation and failure of cables. In the current fleet of nuclear reactors, there are thousands of miles of cabling installed in each plant and many of these cables are exposed to these harsh environmental conditions. For these cables, the jacket and insulation polymers harden and become brittle over time, making them more susceptible to crack formation and growth, moisture intrusion, and other mechanisms that can lead to cable failure. Moreover, the existing U.S. fleet of 98 nuclear reactors has an average operating age of 38 years. Many of these nuclear power plants have applied for and almost all have been granted regulatory approval for license renewals to operate for 60 years, 20 years beyond their original 40-year life. Further, subsequent license renewals (SLRs) are underway with a few commercial nuclear power sites already approved to operate up to 80 years. As these reactors pursue operating life extensions, utilities must find a way to address issues associated with age-related degradation of cables. Designers of small modular reactors are also in need of technologies to evaluate the performance of cables that will be installed in harsher environments (e.g. higher temperatures, radiation doses, dose rates, etc.) than those present in current-generation reactors. Today, a variety of cable condition monitoring (CM) techniques have been developed and successfully used in nuclear facilities. These techniques are used to identify age-related degradation and assess the condition of cables to determine if their performance characteristics have changed with age. However, objective criteria must be developed for these CM tests to help quantify cable condition and thereby develop repair and replacement schedules. With operating life extending to 80 years and more SLRs on the horizon, both nuclear facilities and regulators need an objective means to determine the aged condition of cables.

36 MATERIALS SCIENCE↗

Characterizing the Performance of Fission Chambers for Local Neutron Flux and Spectrum Measurement

Three fission chambers were tested at The Ohio State University Research Reactor (OSURR) to evaluate fission chambers for neutron flux and spectrum measurements. Two of the fission chambers are commercial Photonis CFUR43 fission chambers—one utilizing highly enriched uranium-235 fissile deposits for thermal neutron detection and the other with highly depleted uranium-238 for fast neutron detection. This experiment was also performed in collaboration with French Alternative Energies and Atomic Energy Commission (CEA) with CEA suppling a uranium-235 loaded fission chamber built from the Photonis CFPR CE8/9 kit. The fission chambers were irradiated in a movable 6.5 inch dry tube at reactor powers of 50 kW, 200 kW, and 450 kW at ambient temperature and at 350°C. While all sensors demonstrated good linear sensitivity to reactor power, a leakage current of 6 nA was measured for the CFUR43 detectors. Additionally, the measured signal ratios of the two CFUR43 detectors did not match the theoretical values and are subject to further investigation on individual signal contributors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Verification and Validation of the STAT7 Code

This document presents the verification and validation of the STAT7 Version 1.1 code, which has been developed to perform the steady-state thermal hydraulics (TH) safety calculations required to support conversion of the Massachusetts Institute of Technology Research Reactor from highly enriched uranium fuel to low- enriched uranium fuel. The key capabilities of the code, including statistical processing, water property generation, and TH solution, are verified independently. While the first two capabilities are checked using statistical tests and NIST data tables, each component of the TH solution is verified using simple geometry test problems. The comparison between results obtained by the code and by hand calculations on these problems shows that each of these components works correctly. Additionally, a comprehensive comparison between STAT7 Version 1.1 and PLTEMP/ANL Version 4.3 Revision 162 calculations is performed for the validation. Good agreement is achieved between the results obtained with the two codes for all TH parameters belonging to the fuel core region.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Cultural Resource Management Plan for Brookhaven National Laboratory

The Cultural Resource Management Plan (CRMP) for Brookhaven National Laboratory (BNL) provides an organized guide that describes or references the facets and interrelationships of cultural resources at BNL. Management strategies included within this CRMP are designed to adequately identify the cultural resources that BNL and DOE consider significant and to acknowledge associated management actions. A principal objective of the CRMP is to reduce the need for additional regulatory documents and to serve as the basis for a formal agreement between the DOE and the New York State Historic Preservation Officer (NYSHPO). The BNL CRMP is designed to be a “living document.” Each section includes identified gaps in the management plan, with proposed goals and actions for addressing each gap. The plan will be periodically revised to incorporate new documentation. The current (2023) update incorporates new findings and/or updated text based on completed or ongoing projects related to cultural resources at BNL since inception of the last updated CRMP in 2013. Historically, Brookhaven National Laboratory had little need for cultural resource management because many of its buildings were less than 50 years old. Most of the features that are potentially eligible for inclusion in the National Register of Historic Places were protected simply by avoiding the features. Compliance with cultural resource laws and regulations has included archeological surveys, such as those associated with the 1977 Final Environmental Impact Statement for Brookhaven National Laboratory and the 1978 Final Environmental Impact Statement for the Proton-Proton Storage Accelerator Facility (ISABELLE). In 1979, World War I trenches associated with the former Camp Upton and located near ISABELLE were determined to be eligible for inclusion in the National Register of Historic Places; however, many of these trenches had been destroyed by construction work. In 1991, the NYSHPO provided BNL with a letter indicating that only three structures and features were likely to be eligible for inclusion in the National Register of Historic Places. Between 1991 and 1999, little work associated with cultural resource management was accomplished. Beginning in 1999, awareness for the need of a program to manage cultural resources grew out of the realization that over half of the buildings at BNL were either 50 years old or were reaching that age and were, therefore, subject to the requirements in Section 106 of the National Historic Preservation Act. This fact, concomitant with the decontamination and decommissioning of the Brookhaven Graphite Research Reactor (BGRR) and the subsequent determination of BGRR’s eligibility for listing as an historical site, fueled the need for developing and implementing a more structured program for managing cultural resources at BNL.

54 ENVIRONMENTAL SCIENCES↗

Demonstration of the Blending of the H-Canyon 2nd U Cycle with Natural U to Produce a HALEU Solution

Continued growth in the demand for high assay low enriched uranium (HALEU) is projected to support the conversion of US high performance research reactors from high to low enrichment and the development and deployment of a new generation of advanced reactors. Current options to meet the growing US need for HALEU include (1) blend-down of excess of highly enriched uranium (HEU) from the nuclear weapons programs, (2) blend-down of HEU metal from other stockpiles, or (3) recycle of irradiated HEU recovered from spent nuclear fuel (SNF). The recycle of HEU from SNF has been performed at the Savannah River Site (SRS) H-Canyon facility for nearly two decades to produce 4.95 wt % U-235 for sale and subsequent use in fuel for Tennessee Valley Authority (TVA) reactors. The HALEU produced in H-Canyon will not exceed the U-236 concentration limit in the ASTM C1462 standard for U metal enriched to more than 15% and less than 20% U-235, which applies to advanced reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Plutonium Basket Counter Measurement Control Q3-Q4 2023

The Plutonium Basket Counter (PBC) is a spent fuel nuclear safeguards instrument that was developed to measure spent-fuel elements from MAGNOX-type research reactors and determine their plutonium content. The instrument is designed to measure fuel elements in spent fuel cooling pools through underwater operation, but it is also able to measure radiation sources in air. The PBC determines fuel plutonium content by detecting neutrons with an array of Helium-3 detectors. The electronics make use of a JSR-15 shift register for data collection and IAEA Neutron Coincidence Counting (INCC) software for data analysis. The PBC is used to determine the 240 Pu content in spent MAGNOX fuel elements grouped into basket-like bundles, thus the instrument’s name. Reactor burnup calculations can be used in conjunction with the data from the PBC to estimate the total plutonium content in the fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Automated Fissile Mass Estimation Python Script for the Advanced Experimental Fuel Counter (AEFC)

The Advanced Experimental Fuel Counter (AEFC) is a non-destructive assay (NDA) instrument developed to quantify the residual fissile mass in research reactor spent fuel assemblies. The system is installed in a spent fuel pool and measurements are acquired underwater. A calibration curve relates the totals and coincidence counting signal from active interrogation of the spent fuel assemblies to the fissile mass remaining in the fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Baseline Hypothetical Facility for the Production of 131 I, 99 Mo, and 133 Xe from HALEU Fission Targets

The report describes the development of a hypothetical facility to produce the pharmaceutical radioisotope 131 I at an amount of 60 curies per week via the fission of a High Assay Low Enriched Uranium (HALEU) target, along with the chemical and physical processes and equipment needed to separate the 131 I and co-produced 99 Mo and 133 Xe. The hypothetical design was carried out using a 10 MWt research reactor. The irradiation calculation determined that three HALEU targets with aluminum cladding can be used to produce 60 Ci/week of 131 I, 750 Ci/week of 99 Mo and 560 Ci/week of 133 Xe. The process selected for the baseline design uses caustic dissolution of the target material with ion exchange processes to separate and purify the iodine and molybdenum. The xenon is processed using a cryogenic carbon bed separation process. Target processing occurs in seven shielded hot cells with a total footprint of 16m 2 and waste management occurs in an eight hot cell with a 2.5 m 2 footprint. Waste generated from the processing of the three targets per week would generate less than 4 shielded drums of waste annually. These hot cells would need varying levels of shielding due to the amount of fission products being handled in the unit. Hot cell facilities also require support services including QA/QC, health physics, administrative staff, operator changing room, radiological buffer areas, and waste storage. The overall facility would require a footprint of 1050 m 2 with 20.25 m 2 of shielded hot cells.

62 RADIOLOGY AND NUCLEAR MEDICINE↗