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At least 361 records · Page 20

Measurement of muon-induced high-energy neutrons from rock in an underground Gd-doped water detector

In this paper, we present a measurement of the rate of correlated neutron captures in the WATCHBOY detector, deployed at a depth of approximately 390 meters water equivalent (m.w.e.) in the Kimballton Underground Research Facility (KURF). WATCHBOY consists of a cylindrical 2 ton water target doped with 0.1% gadolinium, surrounded by a 40 ton undoped water hermetic shield. We present a comparison of our results with the expected rate of correlated neutron captures arising from high-energy neutrons incident on the outside of the WATCHBOY shield, predicted by a hybrid FLUKA/GEANT4-based simulation. The incident neutron energy distribution used in the simulation was measured by a fast neutron spectrometer, the 1.8-ton Multiplicity and Recoil Spectrometer (MARS) detector, at the same depth. We nd that the measured detection rate of two correlated neutrons is consistent with that predicted by simulation. The result lends additional confidence in the detection technique used by MARS, and therefore in the MARS spectra as measured at three different depths. Confirmation of the fast neutron flux and spectrum is important as it helps validate the scaling models used to predict the fast neutron fluxes at different overburdens.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Development of 17 N as a time-tagged neutron source for calibration of large antineutrino detectors

Large antineutrino detectors hold the potential for remote nuclear reactor monitoring and discovery, which is of great interest for nonproliferation and treaty verification applications. Correlated-particle calibration sources are especially useful for large-volume designs based on detection of inverse beta-decay events, as the timing information of the coincident particles improves background rejection and event reconstruction. 17 N is a promising calibration source since it emits beta-correlated delayed neutrons and can be produced relatively easily using high-energy neutrons. In this work, we examine the feasibility of 17 N as a time-tagged calibration source for large antineutrino detectors. 17 N was produced using a DT neutron generator from a water sample enriched in 17 O, and the observed production rates were found to be consistent with previous measurements of the 17 O(n,p) 17 N reaction cross-section. As a result, time-tagging of 17 N delayed neutrons is demonstrated via beta-neutron coincidence measurements conducted using a specialized beta detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Detectability of QCD phase transitions in binary neutron star mergers: Bayesian inference with the next generation gravitational wave detectors

We study the detectability of postmerger QCD phase transitions in neutron star binaries with next-generation gravitational-wave detectors Cosmic Explorer and Einstein Telescope. We perform numerical relativity simulations of neutron star mergers with equations of state that include a quark deconfinement phase transition through either a Gibbs or Maxwell construction. These are followed by Bayesian parameter estimation of the associated gravitational-wave signals using the nrpmw waveform model, with priors inferred from the analysis of the inspiral signal. We assess the ability of the model to measure the postmerger peak frequency $f$$^{peak}_{2}$ and identify aspects that should be improved in the model. We show that, even at postmerger signal to noise ratios as low as 10, the model can distinguish (at the 90% level) $f$$^{peak}_{2}$ between binaries with and without a phase transition in most cases. Phase-transition induced deviations in the $f$$^{peak}_{2}$ from the predictions of equation-of-state insensitive relations can also be detected if they exceed 1.6⁢σ. Our results suggest that next-generation gravitational wave detectors can measure phase transition effects in binary neutron star mergers. Furthermore, unless the phase transition is “strong,” disentangling it from other hadronic physics uncertainties will require significant theory improvements.

79 ASTRONOMY AND ASTROPHYSICS↗

Measuring neutron star radius with second and third generation gravitational wave detector networks

The next generation of ground-based interferometric gravitational wave detectors will observe mergers of black holes and neutron stars throughout cosmic time. A large number of the binary neutron star merger events will be observed with extreme high fidelity, and will provide stringent constraints on the equation of state of nuclear matter. In this paper, we investigate the systematic improvement in the measurability of the equation of state with increase in detector sensitivity by combining constraints obtained on the radius of a 1.4 M ⊙ neutron star from a simulated source population. Since the measurability of the equation of state depends on its stiffness, we consider a range of realistic equations of state that span the current observational constraints. We show that a single 40 km Cosmic Explorer detector can pin down the neutron star radius for a soft, medium and stiff equation of state with a precision of 10 m within a decade, whereas the current generation of ground-based detectors like the Advanced LIGO-Virgo network would take $\mathcal{O}(10_5)$ years to do so for a soft equation of state.

79 ASTRONOMY AND ASTROPHYSICS↗

Gamma and Neutron Measurement and Modeling of Irradiated TRISO Fuel

Given the unique characteristics of the PBR fuel cycle, both gamma and neutron measurements are expected to play important roles in performing and maintaining nuclear material control and accounting for spent pebbles to safeguard the fuel cycle. Given the lack of irradiated pebbles in the US, a variety of irradiated TRISO fuel samples with wide ranges of burnups and cooling times available at ORNL were used in this work. A large number of gamma and neutron measurements have been performed on these samples to collect data to test the various detectors and to benchmark the computer models to simulate the depletion and decay of the fuel and the measurements themselves. Two neutron detectors, including a custom-made detector and the Very High-Performance Neutron Multiplicity Counting, were used to measure the neutrons emitted by these TRISO samples. Three gamma spectrometry detectors, including an HPGe and the M400 CZT detector, were used to measure gamma-ray emissions from these samples. The M400 was recently adopted by the IAEA for fresh uranium measurements, but it was tested for spent fuel measurements prior to this project. Detailed MCNP models were developed to simulate these neutron and gamma measurements. Some GADRAS models were also developed to cross check the MCNP models for the gamma measurements. It was found challenging to perform neutron measurements in the hot cell due to the high background counts. Close agreements were observed between the simulated and measured neutron count rates in both detectors’ measurements of californium calibration sources. Both the HPGe and M400 detectors were able to measure the 604 and 662 keV peaks from these samples, which are the two most important peaks used to infer fuel burnup. Although the M400 detector did not have nearly good energy resolution and did not detect some of the minor peaks as the HPGe detector, it was found to be capable of handling significantly higher dose rates than HPGe. Given the complexities in the TRISO samples (e.g., different samples sizes) and uncertainties in the alignments between the detector and the TRISO fuel inside the containers, large scatters were found between the peak area rates and the samples’ burnups. However, the 604/662 peak ratios were found to trend well with the samples’ burnups among most samples in both measured and simulated results.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Continuing Analysis of Charge Current Interactions in ANNIE

The Accelerator Neutrino Neutron Interaction Experiment (ANNIE) is a gadolinium-loaded water Cherenkov detector on the Fermilab Booster Neutrino Beam (BNB).Using νμ in the energy range of 500 to 1000 MeV, ANNIE is designed to measure final-state neutrons.In this poster we will cover the ongoing analysis work exploring Charged-Current neutrino interactions. Charged-Current (CC) νμ interactions in this regime have uncertainties in the relative contributions of quasielastic and res- onance production. Together with intranuclear final-state interactions (FSI) and missing hadronic energy, these interactions drive important biases in neutrino energy reconstruction. ANNIE mit- igates these effects by combining muon kinematics from the downstream Muon Range Detector (MRD) with neutron identification via delayed gamma cascades from thermal captures on gadolin- ium. We characterize CC0π and Δ samples by measuring neutron multiplicity versus event topology and reconstructed kinematics, comparing neutron-tagged data to interaction-model predictions to probe resonance production and pion FSI/absorption

Fleming, Dylon [UC, Davis; Fermilab] (ORCID:000000↗

Preliminary RAM-RODD results for the MUSiC subcritical configurations

The Measurement of Uranium Subcritical and Critical (MUSiC) was performed at the DOE’s National Criticality Experiments Research Center (NCERC) located in the Nevada National Security Site (NNSS). The measurement utilized the Rocky Flats shells to perform benchmark measurements of similar highly enriched uranium (HEU) systems that span a wide range of reactivities. The Rocky Flats (RF) shells are 93.16% U-235 enriched metal hemishells that can be stacked concentrically. Ten configurations were measured with effective multiplication factors spanning between deeply subcritical (~ 0.64) through delayed critical. Details of the measured configurations are listed in Table 1. This unique set of measurements with its large span of reactivies is being used to determine the range over which neutron noise techniques such as Feynman variance-to-mean, Rossi-alpha, and pulsed neutron source techniques can be accurately employed for a bare HEU system. The results of the measurements will be published as a benchmark in The International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The results will support the growing amount of subcritical benchmark data, such as the SCRaP measurements, that is available to the community. The measurements were performed using several different detector systems for the purposes of cross-validation and obtaining detector independent results. Four detector systems were deployed, three by the NCERC team and one from the University of Michigan. The detector systems included a Neutron Multiplicity Array Detector (NoMAD) system (similar to the MC-15), four small volume 0.635 cm (Ø) × 7.59 cm 3 He detectors (ideal for measuring prompt neutron decay constants due to their fast recovery speed), the Rossi Alpha Measurements – Rapid Organic (n, γ) Discrimination Detector (RAM-RODD), and the Organic Scintillator Array (OSCAR). RAM-RODD is an array of eight 5.08 cm (Ø) × 5.08 cm EJ-309 organic scintillator detectors. OSCAR is a University of Michigan system and is an array of twelve 5.08 cm (Ø) × 5.08 cm stilbene detectors. Details of measurements performed with OSCAR will be discussed in a separate talk. The focus of this work is preliminary results obtained by RAM-RODD for the 8 subcritical configurations. Additional details on the measurements and on the setup and deployment of RAM-RODD will be discussed. Preliminary neutron noise analysis results including Rossi-alpha and Feynman-alpha will also be presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Wellbore detector with azimuthal and spectral energy resolution

A wellbore inspection device includes a radiation generation source operable to emit neutrons, and a radiation detector fixed relative to the radiation generation source and operable to detect backscattered neutron radiation from a surrounding environment. The radiation detector includes a plurality of individually addressable detector elements arranged in one or more concentric rings. Respective amounts of backscattered neutron radiation detected by the individually addressable detector elements within a ring is indicative of the azimuthal direction of the detected backscattered neutron radiation, and the respective amount of backscattered neutron radiation detected by the individually addressable detector elements of two or more concentric rings is indicative of an energy level of the backscattered neutron radiation. The inspection device determines whether a potential anomaly is present in or around the wellbore, based at least in part on the respective amounts of backscattered radiation detected by the individually addressable detector elements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

POWTEX visits POWGEN

The high-intensity time-of-flight (TOF) neutron diffractometer POWTEX for powder and texture analysis is currently being built prior to operation in the eastern guide hall of the research reactor FRM II at Garching close to Munich, Germany. Because of the world-wide 3 He crisis in 2009, the authors promptly initiated the development of 3 He-free detector alternatives that are tailor-made for the requirements of large-area diffractometers. Herein is reported the 2017 enterprise to operate one mounting unit of the final POWTEX detector on the neutron powder diffractometer POWGEN at the Spallation Neutron Source located at Oak Ridge National Laboratory, USA. As a result, presented here are the first angular- and wavelength-dependent data from the POWTEX detector, unfortunately damaged by a 50 g shock but still operating, as well as the efforts made both to characterize the transport damage and to successfully recalibrate the voxel positions in order to yield nonetheless reliable measurements. Also described is the current data reduction process using the PowderReduceP2D algorithm implemented in Mantid [Arnold et al. (2014). Nucl. Instrum. Methods Phys. Res. A , 764 , 156–166]. The final part of the data treatment chain, namely a novel multi-dimensional refinement using a modified version of the GSAS-II software suite [Toby & Von Dreele (2013). J. Appl. Cryst. 46 , 544–549], is compared with a standard data treatment of the same event data conventionally reduced as TOF diffraction patterns and refined with the unmodified version of GSAS-II . This involves both determining the instrumental resolution parameters using POWGEN's powdered diamond standard sample and the refinement of a friendly-user sample, BaZn(NCN) 2 . Although each structural parameter on its own looks similar upon comparing the conventional (1D) and multi-dimensional (2D) treatments, also in terms of precision, a closer view shows small but possibly significant differences. For example, the somewhat suspicious proximity of the a and b lattice parameters of BaZn(NCN) 2 crystallizing in Pbca as resulting from the 1D refinement (0.008 Å) is five times less pronounced in the 2D refinement (0.038 Å). Similar features are found when comparing bond lengths and bond angles, e.g. the two N—C—N units are less differently bent in the 1D results (173 and 175°) than in the 2D results (167 and 173°). The results are of importance not only for POWTEX but also for other neutron TOF diffractometers with large-area detectors, like POWGEN at the SNS or the future DREAM beamline at the European Spallation Source.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Prospects for direct detection of black hole formation in neutron star mergers with next-generation gravitational-wave detectors

A direct detection of black hole formation in neutron star mergers would provide invaluable information about matter in neutron star cores and finite temperature effects on the nuclear equation of state. We study black hole formation in neutron star mergers using a set of 190 numerical relativity simulations consisting of long-lived and black-hole-forming remnants. The postmerger gravitational-wave spectrum of a long-lived remnant has greatly reduced power at a frequency 𝑓 greater than 𝑓 peak , for 𝑓 ≳ 4 kHz, with 𝑓 peak ∈ [2.5,4] kHz. On the other hand, black-hole-forming remnants exhibit excess power in the same large 𝑓 region and manifest exponential damping in the time domain characteristic of a quasinormal mode. We demonstrate that the gravitational-wave signal from a collapsed remnant is indeed a quasinormal ringing. We report on the opportunity for direct detections of black hole formation with next-generation gravitational-wave detectors such as Cosmic Explorer and Einstein Telescope and set forth the tantalizing prospect of such observations up to a distance of 100 Mpc for an optimally oriented and located source with an SNR of 4.

Astronomy & Astrophysics↗

169 Tm ( n , γ ) cross section and statistical decay properties from measurements at the DANCE facility

Background: Radiative neutron capture on thulium, which is a monoisotopic element, plays a role in different applications such as nuclear astrophysics or nuclear burning environments. Considerable discrepancies—reaching 20%—exist between evaluations in the unresolved-resonance region. Furthermore, experimental data on statistical 𝛾 decay in odd-odd rare-earth nuclei is scarce. There are still open questions about the systematics of the so-called scissors mode in the 𝑀⁢1 photon strength function, especially in odd-odd nuclei. Purpose: This work is focused on two main topics—deriving experimental 169 Tm ⁢(𝑛,𝛾) cross section and studying statistical 𝛾 decay of 170 Tm, in particular properties of the scissors mode. Methods: The capture experiments to obtain experimental cross section were performed at the Los Alamos Neutron Science Center using the time-of-flight technique and employing the Detector for Advanced Neutron Capture Experiments. Measured coincident 𝛾-ray spectra were also compared with statistical simulations using the dicebox code to test different models of level density and photon strength functions. Results: The capture cross section was determined from 1.8 eV to 0.97 MeV, the broadest neutron-energy range ever measured for this isotope. Several new resonances have been observed. The statistical 𝛾 decay of 170 Tm cannot be reproduced without a scissors mode resonance centered at ≈ 3.3MeV. Conclusions: The measured cross section in the unresolved-resonance region is generally lower than the latest evaluations. The derived 169 Tm 𝑠-process abundance is expected to increase by a factor of 1.26, while the changes of the abundances of elements heavier than 169 Tm are in the order of 0.2%. The scissors mode properties in 170 Tm are similar to those deduced in previous analyses of neighboring nuclei 168 Er and 166 Ho .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Pulse shape measurements for neutron/gamma discrimination using the TOFPET2 ASIC

Many highly pixelated organic scintillator detection systems would benefit from independent readout of each scintillator pixel. Recent advances in Silicon Photomultiplier (SiPM) technology makes this goal feasible, however the data acquisition from potentially hundreds or thousands of channels requires a low-cost and compact solution. For pixelated neutron detection with organic scintillators, the capability to distinguish between neutron and gamma interactions using Pulse Shape Discrimination (PSD) is required along with pulse charge and time of arrival. The TOFPET2 ASIC from PETsys Electronics is a 64-channel readout chip providing pulse time and charge integration measurements from SiPMs, and is specifically designed for time-of-flight positron-emission tomography. Using an 8 × 8 array of 6 mm × 6 mm J-series SiPMs from SensL/OnSemi (ArrayJ-60035-64P-PCB), we have studied the energy and PSD performance of the TOFPET2 ASIC using a 4 × 4 array of 6 mm × 6 mm × 30 mm trans -Stilbene crystals from Inrad Optics and a custom SiPM routing board from PETsys Electronics. In conclusion, using a time-over-threshold method, we measure a maximum PSD figure-of-merit of approximately 1.2 at 478 keV (the Compton edge of 662 keV) for a J-series SiPM operating at an over-voltage of 3V.

47 OTHER INSTRUMENTATION↗

Feasibility of an Active Interrogation System to Classify Waste with He-4 Neutron Spectroscopy

This work investigates a 4 He-detector active interrogation system that leverages neutron spectroscopy to classify nuclear waste streams. MCNP models tested the concept through the simulation of a D-D neutron generator, an array of 4 He detectors, and various waste compositions. The fast-neutron Differential Die-Away signature was augmented with a neutron-energy discrimination signature. This signature isolates induced fission neutrons, the energy of which is greater than that of the D-D monoenergetic spectrum. With the incorporation of this spectroscopic technique, the measurement time decreased by 3–9% (depending on the degree of neutron moderation and absorption presented by the sample), demonstrating how neutron spectroscopy can enhance active interrogation methods. The reduced measurement times would have significant financial and logistical benefits for facilities with large footprints of low-level waste production.

4He detectors↗

Direct current response of a thin scCVD diamond detector under increased applied field to 14.1 MeV neutrons

An avalanche effect yielding inherent gain can be exploited in thin, single-crystal chemical vapor deposition (scCVD) diamond. It occurs when a high enough bias is applied across the diamond thickness while avoiding breakdown. This charge multiplication effect was studied previously with alpha particles and heavy ions either by using the transient current technique or by measuring the energy spectrum. The measurements we obtained to evaluate the charge multiplication performance of a 10 μm thick scCVD diamond detector used a novel approach—we employed an electrometer to characterize the response of the detector by performing directly coupled current measurements (time-averaged charge, at 1 Hz sampling) when exposed to 14.1 MeV neutrons from deuterium-tritium fusion. We measured both the dark and irradiated currents from the detector over a range of applied displacement field values from 2 to 75 V/μm. A histogram method with central mean and standard deviation width was used to determine the current over each measurement duration typically from 100 to 300 seconds. The dark-subtracted irradiated current (i.e., contrast) was used to evaluate the gain of the detector at each applied displacement field. The contrast at an applied displacement field between 15 and 20 V/μm was higher than the expected linear increase in contrast proportional to the increased applied bias, indicating the possible presence of avalanche events in the diamond. The detector response also indicated possible polarization and charge depletion effects. These results provide an opportunity to further explore the use of thin scCVD diamond as a fast neutron current mode detector with inherent gain.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗