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At least 361 records · Page 20
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Circuit quantum electrodynamics detection of induced two-fold anisotropic pairing in a hybrid superconductor–ferromagnet bilayer

Abstract Hybrid systems represent one of the frontiers in the study of unconventional superconductivity and are a promising platform to realize topological superconducting states. These materials are challenging to probe using many conventional measurement techniques because of their mesoscopic dimensions, and therefore require new experimental probes so that they can be successfully characterized. Here, we demonstrate a probe that enables us to measure the superfluid density of micrometre-size superconductors using microwave techniques drawn from circuit quantum electrodynamics. We apply this technique to a superconductor–ferromagnet bilayer and find that the proximity-induced superfluid density is two-fold anisotropic within the plane of the sample. It also exhibits power-law temperature scaling that is indicative of a nodal superconducting state. These experimental results are consistent with the theoretically predicted signatures of induced triplet pairing with a nodal p -wave order parameter. Moreover, we observe modifications to the microwave response at frequencies near the ferromagnetic resonance, suggesting a coupling between the spin dynamics and induced superconducting order in the ferromagnetic layer. Our experimental technique can be employed more widely, for example to study fragile unconventional superconductivity in low-dimensional materials such as van der Waals heterostructures.

Bøttcher, C. G. L. (ORCID:0000000194898461)↗
DOE OSTI2017

Density-controlled quantum Hall ferromagnetic transition in a two-dimensional hole system

We typically achieve Quantum Hall ferromagnetic transitions by increasing the Zeeman energy through in-situ sample rotation, while transitions in systems with pseudo-spin indices can be induced by gate control. We report here a gate-controlled quantum Hall ferromagnetic transition between two real spin states in a conventional two-dimensional system without any in-plane magnetic field. We also show that the ratio of the Zeeman splitting to the cyclotron gap in a Ge two-dimensional hole system increases with decreasing density owing to inter-carrier interactions. Below a critical density of ~2.4 × 10 10 cm -2 , this ratio grows greater than 1, resulting in a ferromagnetic ground state at filling factor ν = 2. At the critical density, a resistance peak due to the formation of microscopic domains of opposite spin orientations is observed. For such gate-controlled spin-polarizations in the quantum Hall regime the door opens in order to realize Majorana modes using two-dimensional systems in conventional, low-spin-orbit-coupling semiconductors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Mn-induced Ferromagnetic Semiconducting Behavior with Linear Negative Magnetoresistance in Sr 4 (Ru 1-x Mn x ) 3 O 10 Single Crystals

Triple-layered Sr 4 Ru 3 O 10 is a unique ferromagnet with the central RuO 6 layer behaving differently from two outer layers both crystallographically and magnetically. Here, we report that the partial substitution of Ru by smaller Mn gives rise to modification in crystal structure, electronic and magnetic properties of Sr 4 (Ru 1-x Mn x ) 3 O 10 . Through the single crystal X-ray diffraction refinement, we find that (Ru/Mn)O 6 octahedral rotation is no longer detectable at x ≥ 0.23, leading to the tetragonal structure. The magnetization measurements indicate the ferromagnetic transition temperature T C decreases from 105 K for x = 0 to 30 K for x = 0.41, with the reduced magnetic moment as well. Remarkably, Mn doping results in the change of magnetic anisotropy from the easy c axis in x = 0 to the easy ab plane seen in x = 0.34 and 0.41. Such change also removes the ab -plane metamagnetic transition observed in x = 0. Furthermore, the electrical resistivity increases with increasing x showing semiconducting behavior with Δ ~ 10 meV for x = 0.34 and 30 meV for x = 0.41. Under applied magnetic field, the magnetoresistance exhibits negative and linear field dependence in all current and field configurations. These results clearly indicate Sr 4 (Ru 1-x Mn x ) 3 O 10 is a novel ferromagnetic semiconductor with exotic magnetotransport properties.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Induced Ferromagnetism at BiFeO 3 /YBa 2 Cu 3 O 7 Interfaces

We report that transition metal oxides (TMOs) exhibit many emergent phenomena ranging from high-temperature superconductivity and giant magnetoresistance to magnetism and ferroelectricity. In addition, when TMOs are interfaced with each other, new functionalities can arise, which are absent in individual components. Here, we report results from first-principles calculations on the magnetism at the BiFeO 3 /YBa 2 Cu 3 O 7 interfaces. By comparing the total energy for various magnetic spin configurations inside BiFeO 3 , we are able to show that a metallic ferromagnetism is induced near the interface. We further develop an interface exchange-coupling model and place the extracted exchange coupling interaction strengths, from the first-principles calculations, into a resultant generic phase diagram. Our conclusion of interfacial ferromagnetism is confirmed by the presence of a hysteresis loop in field-dependent magnetization data. Lastly, the emergence of interfacial ferromagnetism should have implications to electronic and transport properties.

36 MATERIALS SCIENCE↗
DOE OSTI2014

A Minimal tight-binding model for ferromagnetic canted bilayer manganites

Half-metallicity in materials has been a subject of extensive research due to its potential for applications in spintronics. Ferromagnetic manganites have been seen as a good candidate and aside from a small minority-spin pocket observed in La 2–2 x Sr 1+2 x Mn 2 O 7 ( x = 0.38), transport measurements show that ferromagnetic manganites essentially behave like half metals. Here we develop robust tight-binding models to describe the electronic band structure of the majority as well as minority spin states of ferromagnetic, spin-canted antiferromagnetic and fully antiferromagnetic bilayer manganites. Both the bilayer coupling between the MnO 2 planes and the mixing of the | x 2 – y 2 > and |3 z 2 – r 2 > Mn 3d orbitals play an important role in the subtle behavior of the bilayer splitting. Effects of k z dispersion are included.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Unexpected ferromagnetic ordering enhancement with crystallite size growth observed in La{sub 0.5}Ca{sub 0.5}MnO₃ nanoparticles

In this paper, the physical properties of half-doped manganite La{sub 0.5}Ca{sub 0.5}MnO₃ with crystallite sizes ranging from 15 to 40 nm are investigated. As expected, ferromagnetic order strengthens at expense of antiferromagnetic one as crystallite size is reduced to 15 nm. However, contrary to previously reported works, an enhancement of saturation magnetization is observed as crystallite size increases from 15 to 22 nm. This unexpected behavior is accompanied by an unusual cell volume variation that seems to induce ferromagnetic-like behavior at expense of antiferromagnetic one. Besides, field cooled hysteresis loops show exchange bias field and coercivity enhancement for increasing cooling fields, which suggest a kind of core-shell structure with AFM-FM coupling for crystallite sizes as small as 15 nm. It is expected that inner core orders antiferromagnetically, whereas uncompensated surface spins behave as spin glass with ferromagnetic-like ordering.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2015

Electronic structure of ferromagnetic semiconductor material on the monoclinic and rhombohedral ordered double perovskites La{sub 2}FeCoO{sub 6}

Double perovskite La{sub 2}FeCoO{sub 6} with monoclinic structure and rhombohedra structure show as ferromagnetic semiconductor based on density functional theory calculation. The ferromagnetic semiconductor state can be well explained by the superexchange interaction. Moreover, the ferromagnetic semiconductor state remains under the generalized gradient approximation (GGA) and GGA plus onsite Coulomb interaction calculation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Magnetothermopower, magnetic entropy change, and magnetoresistance in ferromagnetic cobaltites: R{sub 0.7}Sr{sub 0.3}CoO{sub 3} (R = La and Gd)

We compare the impact effect of external magnetic fields on the magnetic entropy (S{sub m}), electrical resistivity, and thermopower in two metallic oxides R{sub 0.7}Sr{sub 0.3}CoO{sub 3} that become ferromagnetic below T{sub C} = 240 K and 117 K for R = La{sup 3+}(4f{sup 0}) and Gd{sup 3+}(4f{sup 7}), respectively. While Gd{sub 0.7}Sr{sub 0.3}CoO{sub 3} shows unusually high values of negative magnetothermopower (≈−35.5%), magnetic entropy change (ΔS{sub m} ≈ −12 J/kg K), and negative magnetoresistance (≈−3.7%) at 10 K for a field change of 5 T, these effects are absent in the La sample at 10 K. We suggest that the large ΔS{sub m} arises from the field-induced suppression of spin fluctuations associated with localized 4f{sup 7} moments of Gd{sup 3+} ions, but magnetic interaction among Co ions dictates magnetoresistance and magnetothermopower. Magnetization data indicate that while Co{sup 3+} ions adopt intermediate spin state (S = 1) in the La compound, major fraction of them transforms into low spin state (S = 0) in the Gd sample. Hence, the Gd sample is microscopically heterogeneous with a mixture of ferromagnetic metallic and paramagnetic metallic clusters. Spin dependent scattering at the surface of ferromagnetic clusters may be the cause for the coexistence of magnetothermopower and magnetoresistance in this compound. A close correlation between the magnetoresistance and the magnetothermopower is reported.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Microscopic model for all optical switching in ferromagnets

The microscopic mechanism behind the all optical switching (AOS) in ferromagnets has triggered intense scientific debate. Here, the microscopic three-temperature model is utilized to describe AOS in a perpendicularly magnetized ferromagnetic Co/Pt system. We demonstrate that AOS in such a ferromagnet can be explained with the Inverse Faraday Effect (IFE). The influence of the strength and lifetime of the IFE induced field pulse on the switching process are investigated. We found that because of strong spin-orbit coupling, the minimal lifetime of the IFE needed to obtain switching is of the order of 0.1 ps, which is shorter than previously assumed. Moreover, spatial images of the domain pattern after AOS in Co/Pt, as well as their dependence on applying an opposite magnetic field, are qualitatively reproduced.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Diamagnetism to ferromagnetism in Sr-substituted epitaxial BaTiO{sub 3} thin films

We report on the ferromagnetic-like behavior in otherwise diamagnetic BaTiO{sub 3} (BTO) thin films upon doping with non-magnetic element Sr having the composition Ba{sub 0.4}Sr{sub 0.6}TiO{sub 3} (BST). The epitaxial integration of BST (∼800 nm) thick films on Si (100) substrate was achieved using MgO (40 nm) and TiN (20 nm) as buffer layers to prepare BST/MgO/TiN/Si (100) heterostructure by pulsed laser deposition. The c-axis oriented and cube-on-cube epitaxial BST is formed on Si (100) as evidenced by the in-plane and out-of-plane X-ray diffraction. All the deposited films are relaxed through domain matching epitaxy paradigm as observed from X-ray diffraction pattern and A{sub 1}TO{sub 3} mode (at 521.27 cm{sup −1}) of Raman spectra. As-deposited BST thin films reveal ferromagnetic-like properties, which persist up to 400 K. The magnetization decreases two-fold upon oxygen annealing. In contrast, as-deposited un-doped BTO films show diamagnetism. Electron spin resonance measurements reveal no evidence of external magnetic impurities. XRD and X-ray photoelectron spectroscopy spectra show significant changes influenced by Sr doping in BTO. The ferromagnetic-like behavior in BST could be due to the trapped electron donors from oxygen vacancies resulting from Sr-doping.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Phase field simulation of grain size effects on the phase coexistence and magnetostrictive behavior near the ferromagnetic morphotropic phase boundary

The grain size effects on the phase coexistence and magnetostrictive response of Tb 1-x Dy x Fe 2 polycrystals near the ferromagnetic morphotropic phase boundary (MPB) are revealed through phase-field modeling. It shows that phase coexistence is a universal phenomenon in polycrystals for both ferromagnetic and ferroelectric MPB and that the range of compositions for phase coexistence increases with decreasing grain sizes. A large, reversible, and anhysteretic magnetostrictive response at low external fields is also found in the fine-grained polycrystals around the ferromagnetic MPB, which offers us a route to developing nanocrystalline magnetostrictive materials.

42 ENGINEERING↗
DOE OSTI2026

Absence of detectable spin and orbital pumping from Ni to Nb by out-of-plane ferromagnetic resonance

Excited ferromagnets can pump spin angular momentum, along with possibly orbital angular momentum. Among elemental ferromagnets, Ni has been proposed to exhibit substantial orbital pumping relative to spin pumping. Here, in this study, we search for a signature of orbital pumping by Ni, specifically by comparing out-of-plane ferromagnetic resonance in heterostructures without Ni (FeV/Nb) and with Ni (FeV-Ni/Nb). The FeV/Nb series shows a clear increase in Gilbert damping with the Nb sink thickness, attributed to spin pumping from FeV to Nb. Surprisingly, the FeV-Ni/Nb series exhibits no such damping increase, revealing no significant spin or orbital pumping from Ni to Nb. Our results offer a fresh perspective on angular-momentum transfer in Ni/Nb heterostructures.

Bakare, Omolara A [Virginia Polytechnic Inst. and ↗
DOE OSTI2017

Self-learning kinetic Monte Carlo simulations of diffusion in ferromagnetic α -Fe–Si alloys

Diffusion in α-Fe-Si alloys is studied using AKSOME, an on-lattice self-learning KMC code, in the ferromagnetic state. Si diffusivity in the α-Fe matrix were obtained with and without the magnetic disorder in various temperature ranges. In addition we studied vacancy diffusivity in ferromagnetic α-Fe at various Si concentrations up to 12.5at.% in the temperature range of 350–550 K. The results were compared with available experimental and theoretical values in the literature. Local Si-atom dependent activation energies for vacancy hops were calculated using a broken-model and were stored in a database. The migration barrier and prefactors for Si-diffusivity were found to be in reasonable agreement with available modeling results in the literature. Magnetic disorder has a larger effect on the prefactor than on the migration barrier. Prefactor was approximately an order of magnitude and the migration barrier a tenth of an electron-volt higher with magnetic disorder when compared to a fully ferromagnetic ordered state. In addition, the correlation between various have a larger effect on the Si-diffusivity extracted in various temperature range than the magnetic disorder. In the case of vacancy diffusivity, the migration barrier more or less remained constant while the prefactor decreased with increasing Si concentration in the disordered or A2-phase of Fe-Si alloy. Important vacancy-Si/Fe atom exchange processes and their activation barriers were also identified and discuss the effect of energetics on the formation of ordered phases in Fe-Si alloys.

AKSOME↗
DOE OSTI2018

Barkhausen noise as an intrinsic fingerprint for ferromagnetic components

Here in this work, the suitability of magnetic Barkhausen noise as an intrinsic fingerprint of ferromagnetic components is determined. This technique has potential for this application because it is based inherently on the near surface microstructural features of ferromagnetic materials. All materials typically display some variation in their microstructure simply as a result of the manufacturing process (rolling, heat treating, welding, grinding), thus providing the potential that Barkhausen noise measurements between nominally similar components will be unique. In this work, we demonstrate that Barkhausen noise measurements are both repeatable in time for a single sample made from a ferromagnetic material, and unique across a number of instances of nominally similar samples. The results of this work have profound implications in a variety of applications in forensics and physical security. For example, consider the fabrication of the next generation of tamper-evident containers and devices using conventional processes for steel. In addition, since Barkhausen noise is sensitive to changes in microstructures due to grinding and welding, these measurements can be used to detect clandestine repairs and tampering. Finally, because the method inherently results in a time series measurement at each point on a sample, it is expected to have far higher dimensionality than physically similar eddy current measurement. However, the higher dimensionality of Barkhausen measurements suggest that they should be harder to counterfeit than eddy current measurements.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Experimental realization of linearly polarized x-ray detected ferromagnetic resonance

We present the first theoretical and experimental evidence of time-resolved dynamic x-ray magnetic linear dichroism (XMLD) measurements of GHz magnetic precessions driven by ferromagnetic resonance in both metallic and insulating thin films. Our findings show a dynamic XMLD in both ferromagnetic Ni 80 Fe 20 and ferrimagnetic Ni 0.65 Zn 0.35 Al 0.8 Fe 1.2 O 4 for different measurement geometries and linear polarizations. A detailed analysis of the observed signals reveals the importance of separating different harmonic components in the dynamic signal in order to identify the XMLD response without the influence of competing contributions. In particular, RF magnetic resonance elicits a large dynamic XMLD response at the fundamental frequency under experimental geometries with oblique x-ray polarization. The geometric range and experimental sensitivity can be improved by isolating the 2ω Fourier component of the dynamic response. These results illustrate the potential of dynamic XMLD and represent a milestone accomplishment toward the study of GHz spin dynamics in systems beyond ferromagnetic order.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Tuning the room temperature ferromagnetism in Fe 5 GeTe 2 by arsenic substitution

In order to tune the magnetic properties of the cleavable high-Curie temperature ferromagnet Fe$_{5-x}$GeTe 2 , the effect of increasing the electron count through arsenic substitution has been investigated. Small additions of arsenic (2.5% and 5%) seemingly enhance ferromagnetic order in polycrystalline samples by quenching fluctuations on one of the three magnetic sublattices, whereas larger As concentrations decrease the ferromagnetic Curie temperature (T C ) and saturation magnetization. Furthermore, this work also describes the growth and characterization of Fe 4.8 AsTe 2 single crystals that are structurally analogous to Fe$_{5-x}$GeTe 2 but with some phase stability complications. Magnetization measurements reveal dominant antiferromagnetic behavior in Fe 4.8 AsTe 2 with a Néel temperature of $T_{\textrm{N}} \approx$ 42 K. A field-induced spin-flop below T N results in a switch from negative to positive magnetoresistance, with significant hysteresis causing butterfly-shaped resistance loops. In addition to reporting the properties of Fe 4.8 AsTe 2 , this work shows the importance of manipulating the individual magnetic sublattices in Fe$_{5-x}$GeTe 2 and motivates further efforts to control the magnetic properties in related materials by fine tuning of the Fermi energy or crystal chemistry.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Borderline Magnetism: How Adding Mg to Paramagnetic Ce Co 3 Makes a 450-K Ferromagnet with Large Magnetic Anisotropy

A recent experimental study [Phys. Rev. Appl. 9, 024023 (2018)] on paramagnetic CeCo 3 finds that magnesium alloying induces a ferromagnetic transition with intrinsic properties large enough for permanent magnet applications. Here we explain these surprising results via a first-principles study of the electronic structure and magnetism of magnesium-alloyed CeCo 3 . We find the origin of this magnesium-induced ferromagnetic transition to be Stoner physics—the substantial increase in the Fermi-level density of states N(E F ) with Mg alloying. Here, our calculations suggest that both Ce and Co atoms are likely to be important for generating large magnetic anisotropy suggesting the viability of Co-3d and Ce-4f interaction for the generation of magnetic anisotropy in magnetic materials. These results offer a route to the discovery of ferromagnetic materials and provide fundamental insight into the magnetic properties of these alloys.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Efficient Excitation of High-Frequency Exchange-Dominated Spin Waves in Periodic Ferromagnetic Structures

Spin waves are of great interest as an emerging solution for computing beyond the limitations of scaled transistor technology. In such applications, the frequency of the spin waves is important as it affects the overall frequency performance of the resulting devices. In conventional ferromagnetic thin films, the magnetization dynamics in ferromagnetic resonance and spin waves are limited by the saturation magnetization of the ferromagnetic (FM) material and the external bias field. High-frequency applications would require high external magnetic fields which limit the practicality in a realistic device. One solution is to couple microwave excitations to perpendicular standing spin waves (PSSWs) which can enable higher oscillation frequencies. However, efficient coupling to these modes remains a challenge since it requires an excitation that is nonuniform across the FM material thickness and current methods have proven to be inefficient, resulting in weak excitations. Here, we show that by creating periodic undulations in a 100-nm-thick Co 40 Fe 40 B 20 layer, high-frequency PSSWs (>20 GHz) can be efficiently excited using micrometer-sized transducers at bias fields below 100 Oe which absorb nearly 10% of the input rf power. We suggest efficient excitation of such spin waves at low fields may enable high-frequency spintronic applications using exchange-dominated magnetic oscillations using very low external magnetic fields and, with design optimizations, can bring about alternative possibilities in the field.

36 MATERIALS SCIENCE↗