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DOE OSTI2025

Multidimensional Coherent Spectroscopy of van der Waals materials and heterostructures (Final Technical Report)

This project advanced multidimensional coherent spectroscopy (MDCS) and related spectroscopic-imaging methods as quantitative probes of many-body optical excitations in two-dimensional (2D) van der Waals (vdW) semiconductors and their heterostructures. Monolayer transition-metal dichalcogenides (TMDs) such as MoSe 2 and WSe 2 provide a uniquely strong platform for excitonic physics due to reduced dielectric screening, which enhances Coulomb interactions and makes higher-order correlated states (e.g., biexcitons and exciton–trion correlations) more prominent than in conventional bulk semiconductors. At the same time, the same sensitivity that enables strong interactions also increases susceptibility to spatial inhomogeneity—e.g., strain gradients, wrinkles, nanoscale disorder potentials, and charge puddling—which can broaden resonances, obscure interaction signatures, and complicate device-to-device reproducibility. The work reported here addressed this dual opportunity and challenge by: (i) developing and deploying coherent multidimensional methods (including double-quantum MDCS) capable of isolating interaction signals with reduced background, (ii) integrating electrostatic control to tune carrier populations and interaction strengths in situ, and (iii) introducing complementary spatially resolved photoluminescence (PL) techniques—hyperspectral PL imaging and polarization-/field-dependent PL lineshape analysis—to directly quantify disorder, strain, and localization that govern the coherent response.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Progress toward differential cross-section measurements of coherent charged-pion production in charged-current muon neutrino interactions on argon with SBND

Coherent charged pion production in charged-current muon neutrino–nucleus interactions provides a clean experimental signature and enables an excellent estimate of the neutrino energy, making it particularly valuable for neutrino flux constraints and oscillation analyses in future long-baseline experiments. Despite its importance, theoretical modeling of this process remains challenging, especially in the low-energy region below 1 GeV and its dependence on the nuclear target. The Short-Baseline Near Detector (SBND) offers a unique opportunity to study coherent charged pion production using neutrinos in the few-hundred-MeV energy range from the Booster Neutrino Beam (BNB) interacting with an argon target (A = 40), with unprecedented statistics expected to yield approximately three thousand signal events in SBND’s BNB data with 3.5 x 10^20 protons on target. This analysis aims to achieve the first differential cross-section measurement of charged-current coherent charged pion production on argon, as well as the first measurement of this process using BNB neutrinos.

Oh, Sungbin [Fermilab]↗

DOE OSTI2022

The DREAM Endstation at the Linac Coherent Light Source

Free-electron lasers (FEL), with their ultrashort pulses, ultrahigh intensities, and high repetition rates at short wavelength, have provided new approaches to Atomic and Molecular Optical Science. One such approach is following the birth of a photo electron to observe ion dynamics on an ultrafast timescale. Such an approach presents the opportunity to decipher the photon-initiated structural dynamics of an isolated atomic and molecular species. It is a fundamental step towards understanding single- and non-linear multi-photon processes and coherent electron dynamics in atoms and molecules, ultimately leading to coherent control following FEL research breakthroughs in pulse shaping and polarization control. A key aspect for exploring photoinduced quantum phenomena is visualizing the collective motion of electrons and nuclei in a single reaction process, as dynamics in atoms/ions proceed at femtosecond (10 –15 s) timescales while electronic dynamics take place in the attosecond timescale (10 –18 s). Here, we report on the design of a Dynamic Reaction Microscope (DREAM) endstation located at the second interaction point of the Time-Resolved Molecular and Optical (TMO) instrument at the Linac Coherent Light Source (LCLS) capable of following the photon–matter interactions by detecting ions and electrons in coincidence. The DREAM endstation takes advantage of the pulse properties and high repetition rate of LCLS-II to perform gas-phase soft X-ray experiments in a wide spectrum of scientific domains. With its design ability to detect multi-ions and electrons in coincidence while operating in step with the high repetition rate of LCLS-II, the DREAM endstation takes advantage of the inherent momentum conservation of reaction product ions with participating electrons to reconstruct the original X-ray photon–matter interactions. In this report, we outline in detail the design of the DREAM endstation and its functionality, with scientific opportunities enabled by this state-of-the-art instrument.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Subhalos in Galaxy Clusters: Coherent Accretion and Internal Orbits

Subhalo dynamics in galaxy cluster host halos govern the observed distribution and properties of cluster member galaxies. We use the IllustrisTNG simulation to investigate the accretion and orbits of subhalos found in cluster-size halos. We find that the median change in the major axis direction of cluster-size host halos is approximately 80° between a ∼ 0.1 and the present day. We identify coherent regions in the angular distribution of subhalo accretion, and ∼68% of accreted subhalos enter their host halo through ∼38% of the surface area at the virial radius. The majority of galaxy clusters in the sample have ∼2 such coherent regions. We further measure angular orbits of subhalos with respect to the host major axis and use a clustering algorithm to identify distinct orbit modes with varying oscillation timescales. The orbit modes correlate with subhalo accretion conditions. Subhalos in orbit modes with shorter oscillations tend to have lower peak masses and accretion directions somewhat more aligned with the major axis. One orbit mode, exhibiting the least oscillatory behavior, largely consists of subhalos that accrete near the plane perpendicular to the host halo major axis. Our findings are consistent with expectations from inflow from major filament structures and internal dynamical friction: most subhalos accrete through coherent regions, and more massive subhalos experience fewer orbits after accretion. Our work offers a unique quantification of subhalo dynamics that can be connected to how the intracluster medium strips and quenches cluster galaxies.

galaxy clusters↗

DOE OSTI2025

First Search for Neutral Current Coherent Single-Photon Production in MicroBooNE

This article presents the first search for neutrino-induced neutral current coherent single-photon production (NC coherent 1$\gamma$). The search makes use of data from the MicroBooNE 85-tonne active volume liquid argon time projection chamber detector, situated in the Fermilab Booster Neutrino Beam (BNB), with an average neutrino energy of $\langle E_{\nu}\rangle \sim 0.8$ GeV. A targeted selection of candidate neutrino interactions with a single photon-like electromagnetic shower in the final state and no visible vertex activity was developed to search for the NC coherent 1$\gamma$ process, along with two auxiliary selections used to constrain the dominant background from NC$\pi^0$ production. With an integrated exposure of $6.87 \times 10^{20}$ protons on target delivered by the BNB, we set the world's first limit for this rare process, corresponding to an upper limit on the flux-averaged cross section of $\sigma<1.49 \times 10^{-41}\text{cm}^2$ at 90% C.L.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1972

Lunar subsurface exploration with coherent radar.

The Apollo Lunar Sounder Experiment that is scheduled to orbit the moon on Apollo 17 consists of a three frequency coherent radar system and an optical recorder. The coherent radar can be used to measure both phase and amplitude characteristics of the radar echo. Measurement methods that are related to the phase and amplitude will be used to determine the surface profile, locate subsurface features and ascertain near surface electrical properties of the lunar surface. The key to the coherent radar measurement is a highly stable oscillator that preserves an accurate phase reference (2 or 3 electrical degrees) over a long period of time. This reference provides a means for reducing surface clutter so that subsurface features are more easily detected and also provides a means of measuring range to the surface to within a fraction of a wavelength.

Brown, W. E., Jr.↗

NASA NTRS1972

On coherent oscillations of a string.

Vibrations of an elastic string when the separation between the ends varies randomly are studied. The emphasis is on the evolution of the coherent, or ordered, oscillations of the string. Using a perturbation technique borrowed from quantum field theory and the modified Kryloff-Bogoliuboff method, the 'multiple scattering' effect of the random separation between the ends on the linear and nonlinear coherent oscillations are investigated. It is found that due to the random interactions the coherent fundamental oscillation as well as the harmonies are damped. Their frequencies are also modified.

Liu, C. H.↗

NASA NTRS1975

Improved semi-conductor laser device, operating, at room temperature, with an array of three lasers in the spatially coherent, free running mode

The peak pulse power was increased by operating an array of three homostructure Ga As lasers in the laser device. A spatial filter in the laser device selects the spatially coherent, free running, mode. The optical peak power is 5 watts, which is three times the peak power of a single laser in the array. The far-field distribution of the three laser array is a single Gaussian beam of spatial coherence without sidelobes or grating lobes. The length of the optical pulses of spatial coherence was increased to 200 ns by improved heat transfer from the p-n junctions of the lasers to the metal housing of the pulse transformer, and by doubling the core area and increasing the turns of the primary windings of the pulse transformer. The mechanical stability of the laser device was improved and the transition from mechanical alignment to electro-mechanical alignment control, was facilitated.

Rutz, E. M.↗

NASA NTRS1974

Coherent scattering of cosmic neutrinos

It is shown that cosmic neutrino scattering can be non-negligible when coherence effects previously neglected are taken into account. The coherent neutrino scattering cross section is derived and the neutrino index of refraction evaluated. As an example of coherent neutrino scattering, a detector using critical reflection is described which in principle can detect the low energy cosmic neutrino background allowed by the measured cosmological red shift.

Opher, R.↗

NASA NTRS1975

Spatially coherent radiation from an array of GaAs lasers

Spatially coherent radiation from a monolithic array of three homostructure GaAs lasers is reported. The three lasers, with their mirror faces antireflection coated, are operated in an external optical cavity built of spherical lenses and plane mirrors. The spatially coherent beam formation makes use of the Fourier transformation property of the internal lenses. The transverse mode control is performed by a spatial filter. The optical peak power at room temperature of the device was measured to be 5 W, three times the power of a single laser in the array. From the synthesized far-field distribution which was evaluated, we conclude that the laser radiation is of spatial coherence.

Philipp-Rutz, E. M.↗

NASA NTRS1977

Spatially-coherent coupled semiconductor lasers

External cavity for monolithic array of three GaAs lasers phase-coherently couples individual outputs to produce single spatially coherent beam. Fourier transform properties of lens and spatial filter are used to select coherent mode.

Rutz, E. M.↗

NASA NTRS1977

Measurement of far field combustion noise from a turbofan engine using coherence functions

Coherence measurements between fluctuating pressure in the combustor of a YF-102 turbofan engine and far-field acoustic pressure were made. The results indicated that a coherent relationship between the combustor pressure and far-field existed only at frequencies below 250 Hz, with the peak occurring near 125 Hz. The coherence functions and the far-field spectra were used to compute the combustor-associated far-field noise in terms of spectra, directivity, and acoustic power, over a range of engine operating conditions. The acoustic results so measured were compared with results obtained by conventional methods, as well as with various semiempirical predictions schemes. Examination of the directivity patterns indicated a peak in the combustion noise near 120 deg (relative to the inlet axis).

Karchmer, A. M.↗

NASA NTRS1977

Measurement of far field combustion noise from a turbofan engine using coherence functions

Karchmer, A. M.↗

NASA NTRS1978

Optical communication with two-photon coherent stages. I - Quantum-state propagation and quantum-noise reduction

To determine the ultimate performance limitations imposed by quantum effects, it is also essential to consider optimum quantum-state generation. Certain 'generalized' coherent states of the radiation field possess novel quantum noise characteristics that offer the potential for greatly improved optical communications. These states have been called two-photon coherent states because they can be generated, in principle, by stimulated two-photon processes. The use of two-photon coherent state (TCS) radiation in free-space optical communications is considered. A simple theory of quantum state propagation is developed. The theory provides the basis for representing the free-space channel in a quantum-mechanical form convenient for communication analysis. The new theory is applied to TCS radiation.

Yuen, H. P.↗

NASA NTRS1979

Extension of the coherence function to quadratic models

It is shown how the use of higher coherence functions can recover some of the lost coherence due to nonlinear relationship between two fluctuating quantities whose degree of mutual coherence is being measured. The relationship between the two processes is modeled with the aid of a linear term and a quadratic term. As a specific example, the relationship between plasma density and potential fluctuations in a plasma is considered. The fraction of power in the auto-power spectrum of the potential fluctuations due to a linear relationship and to a quadratic relationship between the density and potential fluctuations is estimated.

Kim, Y. C.↗

NASA NTRS1979

Optical communication with two-photon coherent states. II - Photoemissive detection and structured receiver performance

In a previous paper (1978), the authors developed a method of analyzing the performance of two-photon coherent state (TCS) systems for free-space optical communications. General theorems permitting application of classical point process results to detection and estimation of signals in arbitrary quantum states were derived. The present paper examines the general problem of photoemissive detection statistics. On the basis of the photocounting theory of Kelley and Kleiner (1964) it is shown that for arbitrary pure state illumination, the resulting photocurrent is in general a self-exciting point process. The photocount statistics for first-order coherent fields reduce to those of a special class of Markov birth processes, which the authors term single-mode birth processes. These general results are applied to the structure of TCS radiation, and it is shown that the use of TCS radiation with direct or heterodyne detection results in minimal performance increments over comparable coherent-state systems. However, significant performance advantages are offered by use of TCS radiation with homodyne detection. The abstract quantum descriptions of homodyne and heterodyne detection are derived and a synthesis procedure for obtaining quantum measurements described by arbitrary TCS is given.

Shapiro, J. H.↗

NASA NTRS1982

Mach number dependence of the coherent structure in high speed subsonic jets

The coherent structure in high Reynolds number, Mach 0.6 to 0.8 axisymmetric cold air jets exhausting at atmospheric pressure has been studied. The mean flow and the statistical time averaged turbulence properties have been measured. The coherent structure in the jets was measured using two hot-wire probes and cross correlations. The coherent structure was represented in a wave format. The axial wavelength was measured for several frequencies and was compared to results obtained by other investigators for various Mach and Reynolds numbers. The results indicated that the axial wavelength-frequency relationship was the same for a wide range of Mach and Reynolds numbers.

Morrison, G. L.↗

NASA NTRS1982

Conceptual design of a coherent optical system of modular imaging collectors (COSMIC)

The Coherent Optical System of Modular Imaging Collectors (COSMIC) is the design concept for a phase-coherent optical telescope array that may be placed in earth orbit by the Space Shuttle in the 1990s. The initial system module is a minimum redundancy array whose photon collecting area is three times larger than that of the Space Telescope, and possesses a one-dimensional resoution of better than 0.01 arcsec in the visible range. Thermal structural requirements are assessed. Although the coherent beam combination requirements will be met by an active control system, the COSMIC structural/thermal design must meet more stringent performance criteria than even those of the Space Telescope.

Nein, M. E.↗