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NASA NTRS1980

Analysis of air quality management with emphasis on transportation sources

The current environment and practices of air quality management were examined for three regions: Denver, Phoenix, and the South Coast Air Basin of California. These regions were chosen because the majority of their air pollution emissions are related to mobile sources. The impact of auto exhaust on the air quality management process is characterized and assessed. An examination of the uncertainties in air pollutant measurements, emission inventories, meteorological parameters, atmospheric chemistry, and air quality simulation models is performed. The implications of these uncertainties to current air quality management practices is discussed. A set of corrective actions are recommended to reduce these uncertainties.

English, T. D.↗

DOE OSTI2024

Green buffers near industrial plants, examples in Jefferson County TX

Green buffers between industrial plants and residential areas have multiple purposes in mitigating air pollution and protecting the environment. This study focuses on providing information on examples of green space development by industries near residential areas in Jefferson County, Texas. One represents a full buffer where residences were totally removed, another is a partial buffer where some residences were removed in a neighborhood and the third represents vegetation of a formerly industrial facility. Additional estimates on benefits of buffer spaces with respect to a pollutant plume are also considered. The study used geospatial and property data from 1966 to 2020. The transition from a residential area to a full or partial buffers highlights possible mitigation of air pollution impacts while serving additional functions, such as boosting stormwater infiltration and improving the aesthetic attractiveness of the area. The transformation from oil tanks to forested space may display the potential for environmental remediation, but not all spaces are suitable for fully forested buffers, as safety and other limitations should be considered. With the analysis of the classic Plume Equation insights can be provided regarding the possible impact of green buffers on ground-level pollutant concentrations. The calculations for atmospheric stability classes A-F and for various stack heights provide an understanding of how different conditions may affect the pollutant concentrations. The presence of a green buffer can play a crucial role in controlling ground-level pollution concentrations and reduce a community’s perception of risk.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2001

Atmospheric Chemistry from Space: Present Status and Future Plans

One of the unqualified successes of the earth observation program is NASA's continuing monitoring of the ozone layer from space. This activity began in the early 70's with research instruments and continues to this day with the TOMS instrument series and the Upper Atmosphere Research Satellite. In the near future, NASA will be launching the EOS Aura spacecraft (launch mid-2003) which will continue our study of the chemical processes that produce stratospheric ozone depletion. In addition, Aura will begin the first global study of lower atmospheric air pollution including urban ozone, aerosols, nitrogen oxides and carbon monoxide. Atmospheric air pollution measurements from earth orbit involve the development of very high precision spectrometer technologies that have never been flown in space. Farther into the future, lower atmospheric ozone and aerosols may be monitored by space based lidars in low earth orbit, by sensors in geostationary orbit and by continuous limb observations instrument from the Lagrange point L2.

Schoeberl, Mark R.↗

NASA NTRS2022

A Network of Field-Calibrated Low-Cost Sensor Measurements of PM2.5 in Lomé, Togo, Over One to Two Years

Air pollution is a leading cause of global premature mortality and is especially prevalent in many low- and middle-income countries (LMICs). In sub-Saharan Africa, preliminary monitoring networks, satellite retrievals of air-quality-relevant species, and air quality models show ambient fine particulate matter (PM 2.5 ) concentrations that far exceed the World Health Organization guidelines, yet many areas remain largely unmonitored and understudied. Deploying a network of five low-cost PurpleAir PM 2.5 monitors over 2 years (2019–2021), we present the first multiyear ambient air pollution monitoring data results from Lomé, Togo, a major West African coastal city with a population of about 1.4 million people. The full-study time period network-wide mean measured daily PM 2.5 concentration is 23.5 μ g m –3 m –3 . The strong regional influence of the dry and dusty Harmattan wind increases the local average PM 2.5 concentration by up to 58% during December through February, but the diurnal and weekly trends in PM 2.5 are largely controlled by local influences. At all sites, more than 87% of measured days exceeded the new WHO Daily PM 2.5 guidelines; these first measurements highlight the need for air quality improvement in a rapidly growing urban metropolis.

air pollution↗

NASA NTRS2022

Cause of a Lower-Tropospheric High-Ozone Layer in Spring Over Hanoi

The ozonesonde observations in Hanoi, Vietnam, over fourteen years since 2004 have confirmed the enhancement in lower tropospheric ozone concentration at about 3 km altitude in the spring season. We investigated the evolution of the ozone enhancement from analysis of meteorological data, backward trajectories, and model sensitivity experiments. In spring, air masses over Hanoi exhibit strong height dependence. At 3km, the high-ozone air masses originate from the land area to the west of Hanoi, while low-ozone air masses below about 1.5 km are from the oceanic area to the east. Above 4 km, the air masses are mostly traced back to the farther west area. The chemical transport model simulations revealed that precursor emissions from biomass burning in the inland Indochina Peninsula have the largest contribution to the lower tropospheric ozone enhancement, which is transported upward and eastward and overhangs the clean air intrusion from the ocean to the east of Hanoi. At this height level, the polluted air has the horizontal extent of about 20 degrees in longitude and latitude. The polluted air observed in Hanoi is transported further east and widely spread over the northern Pacific Ocean.

tropospheric ozone↗

NASA NTRS2022

Cause of a Lower-Tropospheric High-Ozone Layer in Spring Over Hanoi

Hanoi↗

DOE OSTI2020

The Energy Modeling Forum (EMF)-30 Study on Short-Lived Climate Forcers: Introduction and Overview

The Energy Modeling Forum (EMF)-30 inter-comparison study on short-lived climate forcers (SLCFs) focuses on black carbon (BC) and methane, two of the most important warming SLCFs. The potential impact on climate change of methane and BC-focused emission reductions in the transport and residential sectors were quantified using nine integrated assessment models and a simple climate model. These SLCF reductions reduced global temperatures by 0.18–0.26 °C in 2050 across the models for central climate parameters, with methane being the dominant contributor. The incremental impact of SLCF-focused reductions is much smaller when combined with a broader climate policy. Individual modeling groups examined the health benefits of air pollutant reductions, climate policy co-benefits, and quantified market impacts from air pollutant damages. Model structure and set-up impact on results are discussed along with areas for future work.

Smith, Steven J.↗

DOE OSTI2022

Aerosol-boundary layer interaction modulated entrainment process

Abstract Aerosol-boundary layer interactions play an important role in affecting atmospheric thermodynamics and air pollution. As a key factor in dictating the development of the boundary layer, the entrainment process in the context of aerosol-boundary layer interactions is still poorly understood. Using comprehensive field observations made at a superstation in Beijing, we gain insight into the response of the entrainment process to aerosols. We found that high aerosol loading can significantly suppress the entrainment rate, breaking the conventional linear relationship between sensible heat fluxes and entrainment fluxes. Related to aerosol vertical distributions, aerosol heating effects can alter vertical heat fluxes, leading to a strong interaction between aerosols and the entrainment process in the upper boundary layer. Such aerosol-entrainment coupling can inhibit boundary layer development and explains the great sensitivity of observed entrainment rates to aerosols than can traditional calculations. The notable impact of aerosols on the entrainment process raises holistic thinking about the dynamic framework of the boundary layer in a polluted atmosphere, which may have a significant bearing on the dispersion of air pollutants and the land-atmosphere coupling.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1984

Biogeochemical cycles: Interactions in global metabolism

A science that chooses the globe as it fundamental biogeophysical unit forces extraordinary conceptual difficulties. The roles of energy flow, matter cycles, carbon cycle, air pollution, global effects, air water interactions are discussed.

Moore, B., III↗

NASA NTRS1987

Physical mechanisms of heat, momentum and turbulence fluxes

In a qualitative way, the physical mechanisms which generate fluxes of heat, momentum, and turbulence in the atmosphere are discussed. This material is presented to acquaint people with the Earth science aspects of turbulence as important processes in the atmosphere. To attempt to describe turbulent fluxes of heat, momentum, and moisture in precise mathematical detail becomes an intractable problem. It is burdened by an eighth order set of equations involving more variables than equations. It is a closure problem which requires complicated assumptions that are not necessarily always satisfied, variable boundary conditions, and sparse observational data. Therefore, we must approach the problem in a simplified manner to obtain any kind of solution involving the variables of shear, stress, and heat, moisture, and momentum fluxes. There are other problems, of course, in which the inclusion of the planetary boundary layer is extremely important. Air pollution studies, air-sea exchanges, mesoscale models, and so on, must account for the planetary layer in very specific terms. Some of the physical mechanisms that are involved in generating fluxes are described.

Theon, John S.↗

NASA NTRS1982

Visibility Studies

Studies conducted by the Environmental Studies Laboratory of the University of Utah embrace investigations of the effects of air pollutants on vegetation; air quality in arid and semi-arid regions surrounding energy developments; and the amount, size and type of particles in the atmosphere. In its visibility studies, the laboratory uses a computer program called RADTMO for Radiative Transfer Models. The program computes the characteristics of scattered radiation in the atmosphere including ozone concentration and aerosol density at various altitudes. Calculations provide information used in determining sky color intensity for visibility modeling under different atmospheric conditions. The laboratory was able to avoid the cost of developing a new computer program by using RADTMO for their calculations.

Source record↗

NASA NTRS2012

A New Retrieval Algorithm for OMI NO2: Tropospheric Results and Comparisons with Measurements and Models

Nitrogen oxides (NOx =NO+NO2) are important atmospheric trace constituents that impact tropospheric air pollution chemistry and air quality. We have developed a new NASA algorithm for the retrieval of stratospheric and tropospheric NO2 vertical column densities using measurements from the nadir-viewing Ozone Monitoring Instrument (OMI) on NASA's Aura satellite. The new products rely on an improved approach to stratospheric NO2 column estimation and stratosphere-troposphere separation and a new monthly NO2 climatology based on the NASA Global Modeling Initiative chemistry-transport model. The retrieval does not rely on daily model profiles, minimizing the influence of a priori information. We evaluate the retrieved tropospheric NO2 columns using surface in situ (e.g., AQS/EPA), ground-based (e.g., DOAS), and airborne measurements (e.g., DISCOVER-AQ). The new, improved OMI tropospheric NO2 product is available at high spatial resolution for the years 200S-present. We believe that this product is valuable for the evaluation of chemistry-transport models, examining the spatial and temporal patterns of NOx emissions, constraining top-down NOx inventories, and for the estimation of NOx lifetimes.

Swartz, W. H.↗

NASA NTRS1974

Airborne survey of major air basins in California

An instrumented aircraft was used to study the chemical and transport properties of air pollution in two major urban centers in California and to survey certain aspects of air pollution within this state. State-of-the-art measurement techniques and sampling procedures are discussed. It is found that meteorological transport mechanisms are better portrayed by vertical pollutant profiles. Airborne measurements define the nature of the mixing layer for atmospheric pollutants. Results show that the pollutants are found to be concentrated in distinct layers up to at least 18,000 feet and the O3 buildup occurring in advected air masses is a result of a continuous photochemical aging of air mass.

Gloria, H. R.↗

DOE OSTI2024

The health, climate, and equity benefits of freight truck electrification in the United States

Abstract Long-haul freight shipment in the United States relies on diesel trucks and constitutes ∼3% of U.S. greenhouse gas emissions and a significant share of local air pollution. Here, we compare the climate and air pollution-related health damages from electric versus diesel long-haul truck fleets. We use truck commodity flows to estimate tailpipe emissions from diesel trucks and regional grid emissions intensities to estimate charging emissions from electric trucks under various grid scenarios. We use a reduced complexity air quality model combined with valuation of air pollution-related premature deaths (using two hazard ratios (HRs)) and quantify the distributional health impacts in different scenarios. We find that annual health and climate costs of the current diesel fleet are $195–$249/capita compared to $174–$205/capita for a new diesel fleet, and $156–$177/capita for an electric fleet, depending on the HR. We find that freight electrification could avoid $6.2–8.5 billion in health and climate damages annually when compared to a fleet of new diesel vehicles (with even higher benefits when compared to the current diesel fleet). However, the Midwest and parts of the Gulf Coast would experience an increase in health damages due to vehicles charging using electricity from coal power plants. If old coal power plants (operating in 1980 or earlier) are replaced with zero-emission generation, electrification of all U.S. freight would result in $32.3–39.2 billion in avoided damages annually and health benefits throughout the U.S. Electrifying transport of consumer manufacturing goods (including electronics, transport equipment, and precision instruments) and food, beverage, and tobacco products would provide the largest absolute health and climate benefits, whereas mixed freight and manufacturing goods would result in the largest benefits per tonne-km. We find small variations in health damages across race and income. These results will help policymakers prioritize electrification and charging investment strategies for the freight transportation sub-sector.

Hennessy, Eleanor M. (ORCID:0000000294715765)↗

NASA NTRS1978

Transport of contaminants in the planetary boundary layer

A planetary boundary layer model is described and used to simulate PBL phenomena including cloud formation and pollution transport in the San Francisco Bay Area. The effect of events in the PBL on air pollution is considered, and governing equations for the average momentum, potential temperature, water vapor mixing ratio, and air contaminants are presented. These equations are derived by integrating the basic equations vertically through the mixed layer. Characteristics of the day selected for simulation are reported, and the results suggest that the diurnally cyclic features of the mesoscale motion, including clouds and air pollution, can be simulated in a readily interpretable way with the model.

Lee, I. Y.↗

NASA NTRS2010

Development of an Instrument Performance Simulation Capability for an Infrared Correlation Radiometer for Troposheric Carbon Monoxide Measurements From Geo

We present the progress toward an analytical performance model of a 2.3 micron infrared correlation radiometer (IRCRg) prototype subsystem for a future geostationary space-borne instrument. The prototype is designed specifically to measure carbon monoxide (CO) from geostationary orbit. NASA's Geostationary Coastal and Air Pollution Events (GEO-CAPE) mission, one of the United States Earth Science and Applications Decadal Survey missions, specifies the use of infrared correlation radiometry to measure CO in two spectral regions for this mission. GEO-CAPE will use the robust IRCR measurement technique at geostationary orbit, nearly 50 times farther away than the Terra/MOPITT orbit, to determine hourly changes in CO across a continental domain. The abundance of CO in Earth's troposphere directly affects the concentration of hydroxyl, which regulates the lifetimes of many tropospheric pollutants. In addition, CO is a precursor to ozone formation; CO is used as a tracer to study the transport of global and regional pollutants; and CO is used as an indicator of both natural and anthropogenic air pollution sources and sinks. We have structured our development project to enable rapid evaluation of future spaceborne instrument designs. The project is part of NASA's Instrument Incubator Program. We describe the architecture of the performance model and the planned evaluation of the performance model using laboratory test data.

OsowskiNeil, Doreen↗

NASA NTRS2021

Communicating Respiratory Health Risk Among Children using a Global Air Quality Index

Air pollution poses a serious threat to children’s respiratory health around the world. Satellite remote-sensing technology and air quality models can provide pollution data on a global scale, necessary for riskcommunication efforts in regions without ground-based monitoring networks. Several large centers, including NASA, produce global pollution forecasts that may be used alongside air quality indices to communicate local, daily risk information to the public. Here we present a health-based, globally applicable air quality index developed specifically to reflect the respiratory health risks among children exposed to elevated outdoor air pollution. Additive, excess-risk air quality indices were developed using 51 different coefficients derived from time-series health studies evaluating the impacts of ambient fine particulate matter, nitrogen dioxide, and ozone on children's respiratory morbidity outcomes. A total of four indices were created which varied based on whether or not the underlying studies controlled for co-pollutants and in the adjustment of excess risks of individual pollutants. Combined with historical estimates of air pollution provided globally at a 25x25 km2 spatial resolution from the NASA's Goddard Earth Observing System composition forecast (GEOS-CF) model, each of these indices were examined in a global sample of 664 small and 140 large cities for study year 2017. Adjusted indices presented the most normal distributions of locally-scaled index values, which has been shown to improve associations with health risks, while indices based on coefficients controlling for co-pollutants had little effect on index performance. We provide the steps and resources need to apply our final adjusted index at the local level using freely-available forecasting data from the GEOS-CF model, which can provide risk communication information for cities around the world to better inform individual behavior modification to best protect children's respiratory health.

Air Qualilty↗

NASA NTRS1977

Characterization of terrestrial service environments - The simultaneous occurrence of combined conditions of solar insolation and climatic variables

Computational methods for occurrences of combined environmental and pollution variables are compared. General statistical data and diurnal statistics on 24 environmental variables are treated. Combinations of variables dealt with include: air temperature, relative humidity, wind speed, total insolation; air temperature and weather event (rain, fog); air pollutant and weather event; wind speed, wind direction, and weather event; air temperature, total insolation, and weather event; air temperature, relative humidity, wind speed, computed direct insolation levels; air temperature, relative humidity, air pollution.

Thomas, R. E.↗