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NASA NTRS2007

The Variable X-Ray Spectrum of Markarian 766. II. Time-resolved Spectroscopy

Time-resolved spectroscopy, slicing XMM and Suzaku data down to 25 ks elements was used to investigate whether absorption or scattering components dominate the spectral variations in Mrk 766. Results: Time-resolved spectroscopy confirmed that spectral variability in Mrk 766 can be explained by either of two interpretations of principal components analysis. Detailed investigation confirmed that rapid changes in the relative strengths of scattered and direct emission or rapid changes in absorber covering fraction provide good explanations of most of the spectral variability. However, a strong correlation between the 6.97 keV absorption line and primary continuum together with rapid opacity changes showed that variations in a complex and multi-layered absorber, most likely a disk wind, are the dominant source of spectral variability in Mrk 766.

Turner, T. J.↗

NASA NTRS1978

Measurement of non-Maxwellian electron velocity distributions in a reflex discharge

The results of a ruby laser Thomson scattering study of the space and time-resolved electron velocity distributions in a pulsed Penning discharge in hydrogen are presented. Electron densities were to the order of 10 to the 13th/cu cm and temperatures were roughly 3 eV. This point is just prior to the cessation of the discharge ohmic heating pulse. For magnetic strengths less than 200 G, Maxwellian distributions were found over an energy range six times thermal energy. Temperatures agreed with Langmuir probe data. For fields of 450 G, chaotic plasma potentials were observed to be unstable and the Thomson scattering showed that the electron velocity distributions had central temperatures of 2 eV and wing temperatures of 15-12 eV.

Phipps, C. R., Jr.↗

NASA NTRS1997

A Dual-Line Detection Rayleigh Scattering Diagnostic Technique for the Combustion of Hydrocarbon Fuels and Filtered UV Rayleigh Scattering for Gas Velocity Measurements

Non-intrusive techniques for the dynamic measurement of gas flow properties such as density, temperature and velocity, are needed in the research leading to the development of new generation high-speed aircraft. Accurate velocity, temperature and density data obtained in ground testing and in-flight measurements can help understand the flow physics leading to transition and turbulence in supersonic, high-altitude flight. Such non-intrusive measurement techniques can also be used to study combustion processes of hydrocarbon fuels in aircraft engines. Reliable, time and space resolved temperature measurements in various combustor configurations can lead to a better understanding of high temperature chemical reaction dynamics thus leading to improved modeling and better prediction of such flows. In view of this, a research program was initiated at Polytechnic University's Aerodynamics Laboratory with support from NASA Lewis Research Center through grants NAG3-1301 and NAG3-1690. The overall objective of this program has been to develop laser-based, non-contact, space- and time-resolved temperature and velocity measurement techniques. In the initial phase of the program a ND:YAG laser-based dual-line Rayleigh scattering technique was developed and tested for the accurate measurement of gas temperature in the presence of background laser glare. Effort was next directed towards the development of a filtered, spectrally-resolved Rayleigh/Mie scattering technique with the objective of developing an interferometric method for time-frozen velocity measurements in high-speed flows utilizing the uv line of an ND:YAG laser and an appropriate molecular absorption filter. This effort included both a search for an appropriate filter material for the 266 nm laser line and the development and testing of several image processing techniques for the fast processing of Fabry-Perot images for velocity and temperature information. Finally, work was also carried out for the development of a new laser-based strain-rate and vorticity technique for the time-resolved measurement of vorticity and strain-rates in turbulent flows.

Otugen, M. Volkan↗

NASA NTRS2015

Remote Sensing Measurements of the CO2 Mixing Ratio in the Planetary Boundary Layer Using Cloud Slicing with Airborne Lidar

We have measured the CO2 volume mixing ratio (VMR) within the planetary boundary layer (PBL) using cloud slicing with an airborne pulsed integrated path differential absorption (IPDA) lidar from flight altitudes of up to 13 km. During a flight over Iowa in summer 2011, simultaneous measurement of the optical range and CO2 absorption to clouds and the ground were made using time-resolved detection of pulse echoes from each scattering surface.We determined the CO2 absorption in the PBL by differencing the two lidar-measured absorption line shapes, one to a broken shallow cumulus cloud layer located at the top of the PBL and the other to the ground. Solving for the CO2 VMR in the PBL and that of the free troposphere, we measured a ≈15 ppm (4%) drawdown in the PBL. Both CO2 VMRs were within ≈3 ppm of in situ CO2 profile measurements. We have also demonstrated cloud slicing using scatter from thin, diffuse cirrus clouds and cumulus clouds, which allowed solving for the CO2 VMR for three vertical layers. The technique and retrieval algorithm are applicable to a space-based lidar instrument as well as to lidar IPDA measurements of other trace gases. Thus, lidar cloud slicing also offers promise toward space-based remote sensing of vertical trace gas profiles in the atmosphere using a variety of clouds.

VMR↗

NASA NTRS1991

Characterization of devices, circuits, and high-temperature superconductor transmission lines by electro-optic testing

The development of a capability for testing transmission lines, devices, and circuits using the optically-based technique of electro-optics sampling was the goal of this project. Electro-optic network analysis of a high-speed device was demonstrated. The project involved research on all of the facets necessary in order to realize this result, including the discovery of the optimum electronic pulse source, development of an adequate test fixture, improvement of the electro-optic probe tip, and identification of a device which responded at high frequency but did not oscillate in the test fixture. In addition, during the process of investigating patterned high-critical-temperature superconductors, several non-contacting techniques for the determination of the transport properties of high T(sub c) films were developed and implemented. These are a transient, optical pump-probe, time-resolved reflectivity experiment, an impulsive-stimulated Raman scattering experiment, and a terahertz-beam coherent-spectroscopy experiment. The latter technique has enabled us to measure both the complex refractive index of an MgO substrate used for high-T(sub c) films and the complex conductivity of a YBa2Cu3O(7-x) sample. This information was acquired across an extremely wide frequency range: from the microwave to the submillimeter-wave regime. The experiments on the YBCO were conducted without patterning of, or contact to, the thin film. Thus, the need for the more difficult transmission-line experiments was eliminated. Progress in all of these areas was made and is documented in a number of papers. These papers may be found in the section listing the abstracts of the publications that were issued during the course of the research.

Whitaker, John F.↗

NASA NTRS1995

Time-Resolved IR-Absorption Spectroscopy of Hot-Electron Dynamics in Satellite and Upper Conduction Bands in GaP

The relaxation dynamics of hot electrons in the X6 and X7 satellite and upper conduction bands in GaP was directly measured by femtosecond UV-pump-IR-probe absorption spectroscopy. From a fit to the induced IR-absorption spectra the dominant scattering mechanism giving rise to the absorption at early delay times was determined to be intervalley scattering of electrons out of the X7 upper conduction-band valley. For long delay times the dominant scattering mechanism is electron-hole scattering. Electron transport dynamics of the upper conduction band of GaP has been time resolved.

Cavicchia, M. A.↗

NASA NTRS1998

The Dynamics of Disorder-Order Transition in Hard Sphere Colloidal Dispersions

The Physics of Hard Spheres Experiment (PHaSE) seeks a complete understanding of the entropically driven disorder-order transition in hard sphere colloidal dispersions. The light scattering instrument designed for flight collects Bragg and low angle light scattering in the forward direction via a CCD camera and performs conventional static and dynamic light scattering at 10-160 deg. through fiber optic cables. Here we report on the kinetics of nucleation and growth extracted from time-resolved Bragg images and measurements of the elastic modulus of crystalline phases obtained by monitoring resonant responses to sinusoidal forcing through dynamic light scattering. Preliminary analysis of the former indicates a significant difference from measurements on the ground, while the latter confirms nicely laboratory experiments with the same instrument and predictions from computer simulations.

Chaikin, Paul M.↗

NASA NTRS2005

Time-Averaged Velocity, Temperature and Density Surveys of Supersonic Free Jets

A spectrally resolved molecular Rayleigh scattering technique was used to simultaneously measure axial component of velocity U, static temperature T, and density p in unheated free jets at Mach numbers M = 0.6,0.95, 1.4 and 1.8. The latter two conditions were achieved using contoured convergent-divergent nozzles. A narrow line-width continuous wave laser was passed through the jet plumes and molecular scattered light from a small region on the beam was collected and analyzed using a Fabry-Perot interferometer. The optical spectrum analysis air density at the probe volume was determined by monitoring the intensity variation of the scattered light using photo-multiplier tubes. The Fabry-Perot interferometer was operated in the imaging mode, whereby the fringe formed at the image plane was captured by a cooled CCD camera. Special attention was given to remove dust particles from the plume and to provide adequate vibration isolation to the optical components. The velocity profiles from various operating conditions were compared with that measured by a Pitot tube. An excellent comparison within 5m's demonstrated the maturity of the technique. Temperature was measured least accurately, within 10K, while density was measured within 1% uncertainty. The survey data consisted of centerline variations and radial profiles of time-averaged U, T and p. The static temperature and density values were used to determine static pressure variations inside the jet. The data provided a comparative study of jet growth rates with increasing Mach number. The current work is part of a data-base development project for Computational Fluid Dynamics and Aeroacoustics codes that endeavor to predict noise characteristics of high speed jets. A limited amount of far field noise spectra from the same jets are also presented. Finally, a direct experimental validation was obtained for the Crocco-Busemann equation which is commonly used to predict temperature and density profiles from known velocity profiles. Data presented in this paper are available in ASCII format upon request.

Panda, Jayanta↗

NASA NTRS2009

Studies of Minerals, Organic and Biogenic Materials through Time-Resolved Raman Spectroscopy

A compact remote Raman spectroscopy system was developed at NASA Langley Research center and was previously demonstrated for its ability to identify chemical composition of various rocks and minerals. In this study, the Raman sensor was utilized to perform time-resolved Raman studies of various samples such as minerals and rocks, Azalea leaves and a few fossil samples. The Raman sensor utilizes a pulsed 532 nm Nd:YAG laser as excitation source, a 4-inch telescope to collect the Raman-scattered signal from a sample several meters away, a spectrograph equipped with a holographic grating, and a gated intensified CCD (ICCD) camera system. Time resolved Raman measurements were carried out by varying the gate delay with fixed short gate width of the ICCD camera, allowing measurement of both Raman signals and fluorescence signals. Rocks and mineral samples were characterized including marble, which contain CaCO3. Analysis of the results reveals the short (approx.10-13 s) lifetime of the Raman process, and shows that Raman spectra of some mineral samples contain fluorescence emission due to organic impurities. Also analyzed were a green (pristine) and a yellow (decayed) sample of Gardenia leaves. It was observed that the fluorescence signals from the green and yellow leaf samples showed stronger signals compared to the Raman lines. Moreover, it was also observed that the fluorescence of the green leaf was more intense and had a shorter lifetime than that of the yellow leaf. For the fossil samples, Raman shifted lines could not be observed due the presence of very strong short-lived fluorescence.

Garcia, Christopher S.↗

NASA NTRS1994

Convective flow effects on protein crystal growth

The long-term stability of the interferometric setup for the monitoring of protein morphologies has been improved. Growth or dissolution of a crystal on a 100 A scale can now be clearly distinguished from dimensional changes occurring within the optical path of the interferometer. This capability of simultaneously monitoring the local interfacial displacement at several widely-spaced positions on the crystal surface with high local depth resolution, has already yielded novel results. We found with lysozyme that (1) the normal growth rate is oscillatory, and (2) the mean growth step density is greater at the periphery of a facet than in its center. The repartitioning of Na(+) and Cl(-) ions between lysozyme solutions and crystals was studied for a wide range of crystallization conditions. A nucleation-growth-repartitioning model was developed to interpret the large body of data in a unified way. The results strongly suggests that (1) the ion to lysozyme ratio in the crystal depends mostly on kinetic rather than crystallographic parameters, and (2) lysozyme crystals possess a salt-rich core with a diameter on the order of 10 microns. The computational model for diffusive-convective transport in protein crystallization (see the First Report) has been applied to a realistic growth cell geometry, taking into account the findings of the above repartitioning studies. These results show that some elements of a moving boundary problem must be incorporated into the model in order to obtain a more realistic description. Our experimental setup for light scattering investigations of aggregation and nucleation in protein solutions has been extensively tested. Scattering intensity measurements with a true Rayleigh scatterer produced systematically increased forward scattering, indicating problems with glare. These have been resolved. Preliminary measurements with supersaturated lysozyme solutions revealed that the scatterers grow with time. Work has begun on a computer program for the unified evaluation of simultaneously obtained, multi-angle static and dynamic light scattering data.

Rosenberger, Franz↗

NASA NTRS2010

Subframe Burst Gating for Raman Spectroscopy in Combustion

We describe an architecture for spontaneous Raman scattering utilizing a frame-transfer CCD sensor operating in a subframe burst-gating mode to realize time-resolved combustion diagnostics. The technique permits all-electronic optical gating with microsecond shutter speeds 5 J.Ls) without compromising optical throughput or image fidelity. When used in conjunction with a pair of orthogonally polarized excitation lasers, the technique measures single-shot vibrational Raman scattering that is minimally contaminated by problematic optical background noise.

Kojima, Jun↗

NASA NTRS1992

Experimental investigation of a simulated LOX injector flow field and other nonintrusive measurement efforts

Efforts to improve the characteristics of fuel-oxidizer mixing in liquid rocket combustors have lead to a swirl element design for a liquid oxygen injector which is being considered for use on the STME. For the design which is the subject of this investigation, the oxygen enters the injector element perpendicular to the injector axis and nearly tangent to the circular injector wall. This swirl element is at one end of a tube and the injector exit is at the other. This geometric configuration creates a plume in the shape of a conical sheet. This sheet is either primarily contiguous liquid or droplets depending on the pressure drop in the injector and the distance from the injector exit. Probe-based devices such as two-dimensional grid patternators have been used to investigate simulated LOX injector flow fields (Hulka). The primary work described herein is an effort to use optical techniques to investigate the plume of a swirl injector element. For this investigation, a high pressure (500 psig) cold flow test facility was constructed. Water was used as the LOX simulate and air pressure was used to drive the injector flow field. Laser-induced fluorescence (LIF) from dye seeded into the water was used to obtain quantitative measurements of the time-averaged water concentration distribution in the plume. Scattered laser light and LIF were used for time averaged plume visualization and scattered light from a strobe with a 1 microsecond pulse was used for time-resolved plume visualization. During the Summer Faculty Fellowship for which this report was developed, an additional effort, unrelated to the swirl injector investigation, was made to resolve fluctuations in the combustion product composition in the exhaust of a hybrid rocket motor. A brief description of this effort is included herein.

Hartfield, Roy J., Jr.↗

NASA NTRS1993

Resolving topographic detail on Venus by modeling complex Magellan altimetry echoes

Magellan's altimeter is providing some of the finest resolution topography of Venus achieved to date. Nevertheless, efforts continue to improve the topographic resolution whenever possible. One effort to this end is stereoscopic imaging, which provides topography at scales similar to that of the synthetic aperture radar (SAR). However, this technique requires two SAR images of the same site to be obtained and limits the utility of this method. In this paper, we present another method to resolve topographic features at scales smaller than that of an altimeter footprint, which is more globally applicable than the stereoscopic approach. Each pulse which is transmitted by Magellan's altimeter scatters from the planet and echoes to the receiver, delayed based on the distance between the spacecraft and each surface element. As resolved in time, each element of an altimetry echo represents the sum of all points on the surface which are equidistant from the spacecraft. Thus, individual returns, as a function of time, create an echo profile which may be used to derive properties of the surface, such as the scattering law or, in this case, the topography within the footprint. The Magellan project has derived some of this information by fitting model templates to radar echo profiles. The templates are calculated based on Hagfor's Law, which assumes a smooth, gently undulating surface. In most regions these templates provide a reasonable fit to the observed echo profile; however, in some cases the surface departs from these simple assumptions and more complex profiles are observed. Specifically, we note that sub-footprint topographic relief apparently has a strong effect on the shape of the echo profile. To demonstrate the effects of sub-resolution relief on echo profiles, we have calculated the echo shapes from a wide range of simple topographic models. At this point, our topographic models have emphasized surfaces where only two dominant elevations are contained within a footprint, such as graben, ridges, crater rims, and central features in impact craters.

Lovell, Amy J.↗

NASA NTRS1992

Gas temperature measurements using the dual-line detection Rayleigh scattering technique

A new laser-induced Rayleigh scattering method is presented for the improved temperature diagnostics of gas flows. In the present technique, the two lines of a copper vapor laser are used to obtain the time and space resolved temperature. A single set of optics is used to form the optical probe and to collect the signal simultaneously from both the 510 nm and the 578 nm lines. The dual-line detection allows for the determination and removal of surface-scattered laser light from a Rayleigh signal thereby improving the applicability of Rayleigh scattering to near wall flows with a high degree of glare. An optical system using the dual-line detection technique is built, calibrated and tested in a hot air jet under various levels of background contamination. The results indicate that highly accurate temperature measurements are possible even when the laser-line background intensity, captured by the collecting optics, is five times that of the Rayleigh signal.

Otugen, M. Volkan↗

NASA NTRS1993

Gas temperature measurements using the dual-line detection Rayleigh scattering technique

Otugen, M. V.↗

NASA NTRS2011

Spatially and Temporally-Resolved Multi-Parameter Interferometric Rayleigh Scattering

A novel approach to simultaneously measure the translational temperature, bulk velocity, and density in gases by collecting, referencing, and analyzing nanosecond time-scale Rayleigh scattered light from molecules is described. A narrow-band pulsed laser source is used to probe two largely separated measurement locations, one of which is used for reference. The elastically scattered photons containing information from both measurement locations are collected at the same time and analyzed spectrally using a planar Fabry - Perot interferometer. A practical means of referencing the measurement of velocity using the laser frequency, and the density and temperature using the information from the reference measurement location maintained at constant properties is described. To demonstrate the technique single-shot spectra of elastic scattered light are obtained in a near zero velocity H2-air Hencken burner flame and simultaneously in an N2-filled gas cell. A simplified Gaussian distribution model to the scattered light spectra is used to obtain the flame properties. Corrections to this model are applied at lower gas temperatures when the simplified Gaussian approximation is no longer suitable. The near-zero measured velocity as a function of the measured flame temperature, and a comparison of the measured flame density and temperature with the perfect gas law are presented.

Bivolaru, Daniel↗

NASA NTRS1993

Was 49: Mirror for a hidden Seyfert 1 galaxy

Was 49 is an interacting pair of Seyfert galaxies at z = 0.063, one of which contains a hidden Seyfert 1 nucleus as evidenced by the highly polarized broad wings on its Balmer lines. The disk of the main galaxy, Was 49a, appears to be globally photoionized by a powerful continuum source, undoubtedly the hidden Seyfert 1 companion, Was 49b. The intrinsic luminosity of Was 49b is at least 100 times larger than the observed (scattered) luminosity. A single SWP spectrum of the pair, which can be spatially resolved in the large aperture was obtained. A narrow Ly-alpha line was detected from Was 49b, the hidden Seyfert 1, at a flux level consistent with that of an unreddened Seyfert 2 galaxy. The lack of detection of a continuum is consistent with a power-law of v(sup -1) or steeper extrapolated from the optical, again consistent with the spectrum of other Seyfert 2 and hidden Seyfert 1 galaxies.

Halpern, Jules↗

NASA NTRS1991

Development of a Rayleigh scattering system for temperature measurements in combustor flows

A dual line laser induced Rayleigh scattering system has been developed to be used in high temperature gas flows such as in combustors, and preliminary tests have been performed in a hot air jet. The qualification measurements included the collection and analysis of Rayleigh signal for time-resolved gas temperature over the two lines of a copper-vapor laser. The dual line signal collection technique is a feature to be used in detecting and discriminating the surface scattered laser light in the Rayleigh signal. Optical fibers are used to transmit the laser beam to the optical probe bench and to carry the collected signal from the bench to the housing of the signal sensors. Incident laser intensity at the probe volume is measured for both lines at each pulse of the laser. This information is used to normalize the signal. Good agreement has been obtained between the two line Rayleigh scattering and thermocouple results in the particle free co-flowing air jet.

Otugen, M. V.↗