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All sourcesNASA NTRSDOE OSTI
NASA NTRS2016

LS3MIP (v1.0) Contribution to CMIP6: The Land Surface, Snow and Soil Moisture Model Intercomparison Project Aims, Setup and Expected Outcome.

The Land Surface, Snow and Soil Moisture Model Intercomparison Project (LS3MIP) is designed to provide a comprehensive assessment of land surface, snow, and soil moisture feedbacks on climate variability and climate change, and to diagnose systematic biases in the land modules of current Earth System Models (ESMs). The solid and liquid water stored at the land surface has a large influence on the regional climate, its variability and predictability, including effects on the energy, water and carbon cycles. Notably, snow and soil moisture affect surface radiation and flux partitioning properties, moisture storage and land surface memory. They both strongly affect atmospheric conditions, in particular surface air temperature and precipitation, but also large-scale circulation patterns. However, models show divergent responses and representations of these feedbacks as well as systematic biases in the underlying processes. LS3MIP will provide the means to quantify the associated uncertainties and better constrain climate change projections, which is of particular interest for highly vulnerable regions (densely populated areas, agricultural regions, the Arctic, semi-arid and other sensitive terrestrial ecosystems).The experiments are subdivided in two components, the first addressing systematic land biases in offline mode (LMIP, building upon the 3rd phase of Global Soil Wetness Project; GSWP3) and the second addressing land feedbacks attributed to soil moisture and snow in an integrated framework (LFMIP, building upon the GLACE-CMIP blueprint).

atmospheric temperature↗
DOE OSTI2022

Where does the dust deposited over the Sierra Nevada snow come from?

Abstract. Mineral dust contributes up to one-half of surface aerosol loading in spring over the southwestern United States, posing an environmental challenge that threatens human health and the ecosystem. Using self-organizing map (SOM) analysis with dust deposition and flux data from WRF-Chem and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale winds, Sierra barrier jet (SBJ), North Pacific High (NPH), and long-range cross-Pacific westerlies, respectively. We find that dust emitted from the Central Valley is persistently transported eastward, while dust from the Mojave Desert and Great Basin influences the Sierra Nevada during mesoscale transport occurring mostly in winter and early spring. Asian dust reaching the mountain range comes either from the west through straight isobars (cross-Pacific transport) or from the north in the presence of the NPH. Extensive dust depositions are found on the west slope of the mountain, contributed by Central Valley emissions and cross-Pacific remote transport. In particular, the SBJ-related transport produces deposition through landfalling atmospheric rivers, whose frequency might increase in a warming climate.

Huang, Huilin (ORCID:0000000273286738)↗
NASA NTRS2011

Surface and Atmospheric Contributions to Passive Microwave Brightness Temperatures for Falling Snow Events

Physically based passive microwave precipitation retrieval algorithms require a set of relationships between satellite -observed brightness temperatures (TBs) and the physical state of the underlying atmosphere and surface. These relationships are nonlinear, such that inversions are ill ]posed especially over variable land surfaces. In order to elucidate these relationships, this work presents a theoretical analysis using TB weighting functions to quantify the percentage influence of the TB resulting from absorption, emission, and/or reflection from the surface, as well as from frozen hydrometeors in clouds, from atmospheric water vapor, and from other contributors. The percentage analysis was also compared to Jacobians. The results are presented for frequencies from 10 to 874 GHz, for individual snow profiles, and for averages over three cloud-resolving model simulations of falling snow. The bulk structure (e.g., ice water path and cloud depth) of the underlying cloud scene was found to affect the resultant TB and percentages, producing different values for blizzard, lake effect, and synoptic snow events. The slant path at a 53 viewing angle increases the hydrometeor contributions relative to nadir viewing channels. Jacobians provide the magnitude and direction of change in the TB values due to a change in the underlying scene; however, the percentage analysis provides detailed information on how that change affected contributions to the TB from the surface, hydrometeors, and water vapor. The TB percentage information presented in this paper provides information about the relative contributions to the TB and supplies key pieces of information required to develop and improve precipitation retrievals over land surfaces.

Skofronick-Jackson, Gail↗
DOE OSTI2022

Variability of Snow and Rainfall Partitioning Into Evapotranspiration and Summer Runoff Across Nine Mountainous Catchments

Abstract Understanding the partitioning of snow and rain contributing to either catchment streamflow or evapotranspiration (ET) is of critical relevance for water management in response to climate change. To investigate this partitioning, we use endmember splitting and mixing analyses based on stable isotope ( 18 O) data from nine headwater catchments in the East River, Colorado. Our results show that one third of the snow partitions to ET and 13% of the snowmelt sustains summer streamflow. Only 8% of the rainfall contributes to the summer streamflow, because most of the rain (67%) partitions to ET. The spatial variability of precipitation partitioning is mainly driven by aspect and tree cover across the sub‐catchments. Catchments with higher tree cover have a higher share of snow becoming ET, resulting in less snow in summer streamflow. Summer streamflow did not contain more rain with higher rainfall sums, but more rain was taken up in ET.

58 GEOSCIENCES↗
NASA NTRS2024

Contributions of irrigation modeling, soil moisture and snow data assimilation to high-resolution water budget estimates over the Po basin: progress towards digital replicas

High-resolution water budget estimates benefit from modeling of human water management and satellite data assimilation (DA) in river basins with a large human footprint. Utilizing the Noah-MP land surface model with dynamic vegetation growth and river routing, in combination with an irrigation module, Sentinel-1 backscatter and snow depth retrievals, we produce a set of 0.7-km2 water budget estimates of the Po river basin (Italy) for 2015–2023. The results demonstrate that irrigation modeling improves the seasonal soil moisture variation and summer streamflow at all gauges in the valley after withdrawal of irrigation water from the streamflow in postprocessing (12% error reduction relative to observed low summer streamflow), even if the basin-wide irrigation amount is underestimated. Sentinel-1 backscatter DA for soil moisture updating strongly interacts with irrigation modeling: when both are activated, the soil moisture updates are limited, and the simulated irrigation amounts are reduced. Backscatter DA systematically reduces soil moisture in the spring, which improves downstream spring streamflow. Assimilating Sentinel-1 snow depth retrievals over the surrounding Alps and Apennines further improves spring streamflow in a complementary way (2% error reduction relative to observed high spring streamflow). Despite the seasonal improvements, irrigation modeling and Sentinel-1 backscatter DA cannot significantly improve short-term or interannual variations in soil moisture, irrigation modeling causes a systematically prolonged high vegetation productivity, and snow depth DA only impacts the deep snowpacks. This study helps advancing the design of digital water budget replicas for river basins.

Gabrielle J M De Lannoy↗
NASA NTRS1990

Seasonal variation of cloud radiative forcing derived from the Earth Radiation Budget Experiment

The impact of clouds on the earth's radiation balance is assessed in terms of longwave, shortwave, and net cloud forcing by using monthly averaged clear-sky and cloudy-sky flux data derived from the NASA Earth Radiation Budget Experiment (ERBE). Emphasis is placed on regional measurements, regional cloud forcing, zonal cloud forcing, and snow and ice contributions. It is shown that the global mean cooling varied from 14 to 21 W/sq m between April 1985 and January 1986; hemispherically, the longwave and shortwave cloud forcing nearly cancel each other in the winter hemisphere, while in the summer the negative shortwave cloud forcing is significantly lower than the longwave cloud forcing, producing a strong cooling. The ERBE data reveal that globally, hemispherically, and zonally, clouds have a significant effect on the radiative heating gradients.

Harrison, E. F.↗
NASA NTRS2009

Contribution of Soil Moisture Information to Streamflow Prediction in the Snowmelt Season: A Continental-Scale Analysis

In areas dominated by winter snowcover, the prediction of streamflow during the snowmelt season may benefit from three pieces of information: (i) the accurate prediction of weather variability (precipitation, etc.) leading up to and during the snowmelt season, (ii) estimates of the amount of snow present during the winter season, and (iii) estimates of the amount of soil moisture underlying the snowpack during the winter season. The importance of accurate meteorological predictions and wintertime snow estimates is obvious. The contribution of soil moisture to streamflow prediction is more subtle yet potentially very important. If the soil is dry below the snowpack, a significant fraction of the snowmelt may be lost to streamflow and potential reservoir storage, since it may infiltrate the soil instead for later evaporation. Such evaporative losses are presumably smaller if the soil below the snowpack is wet. In this paper, we use a state-of-the-art land surface model to quantify the contribution of wintertime snow and soil moisture information -- both together and separately -- to skill in forecasting springtime streamflow. We find that soil moisture information indeed contributes significantly to streamflow prediction skill.

Reichle, Rolf↗
NASA NTRS1999

Additional Contributions to the Development of the New Snow-Physics Scheme for SSiB

The Simplified Simple Biosphere Model (SSiB) had a well-documented problem with snowmelt timing and infiltration. A new snow-physics scheme was developed for use in SSIB. In this, the snow layer is separated from the soil, with its own energy budget and temperature. Solar energy reaching the top of the snowpack is divided into three parts: one, reflected by the snow; two, absorbed by the snow; and three, transmitted to the ground following a simple extinction relation. Heat is exchanged between the ground and snow by conduction and by radiation through an arbitrary air-gap between them. In the GSWP exercise using the GEWEX ISLSCP Initiative I forcing data (hereafter "offline"), it was found that the new snow scheme ameliorated a significant fraction of snowmelt time-delay as compared to observations from satellite. It also produced warmer ground temperatures under the snowpack, which allowed realistic meltwater infiltration, resulting in better simulated spring soil moisture recharge and peak runoff amount as compared to observations. An ensemble of six June-July-August (JJA) simulations for 1987 and 1988 were performed with the NASA Goddard GEOS II GCM coupled with the new snow-physics SSIB using new initial soil moisture (ISM) from the offline simulations. The GCM produced more realistic precipitation in northern regions that had large snowmelt and wetter ISM in response to better snow-physics, as compared to simulations with ISM without the new snow scheme. The new SSiB-GCM also increased the interannual precipitation signal in the Indian monsoon region, resulting from changes in ISM in the Himalayas and central Asia.

Mocko, David M.↗
NASA NTRS2018

The Global Precipitation Measurement (GPM) Mission's Scientific Achievements and Societal Contributions: Reviewing Four Years of Advanced Rain and Snow Observations

Precipitation represents a life-critical energy and hydrologic exchange between the Earth’s atmosphere and its surface. As such, knowledge of where, when, and how much rain and snow falls is essential for scientific research and societal applications. Building on the 17-year success of the Tropical Rainfall Measurement Mission (TRMM), the Global Precipitation Measurement (GPM) Core Observatory (GPM-CO) is the first U.S. National Aeronautical and Space Administration (NASA) satellite mission specifically designed with sensors to observe the structure and intensities of both rain and falling snow. The GPM-CO has proved to be a worthy successor to TRMM, extending and improving high-quality active and passive microwave observations across all times of day. The GPM-CO launched in early 2014, is a joint mission between NASA and the Japanese Aerospace Exploration Agency (JAXA), with sensors that include the NASA-provided GPM Microwave Imager and the JAXA-provided Dual-frequency Precipitation Radar. These sensors were devised with high accuracy standards enabling them to be used as a reference for inter-calibrating a constellation of partner satellite data. These intercalibrated partner satellite retrievals are used with infrared data to produce merged precipitation estimates at temporal scales of 30 minutes and spatial scales of 0.1° x 0.1°. Precipitation estimates from the GPM-CO and partner constellation satellites, provided in near real time and later reprocessed with all ancillary data, are an indispensable source of precipitation data for operational and scientific users. Advances have been made using GPM data, primarily in improving sensor calibration, retrieval algorithms, and ground validation measurements, and used to further our understanding of the characteristics of liquid and frozen precipitation and the science of water and hydrological cycles for climate/weather forecasting. These advances have extended to societal benefits related to water resources, operational numerical weather prediction, hurricane monitoring, prediction, and disaster response, extremes, and disease.

Applications↗
NASA NTRS1989

Remote sensing of global snowpack energy and mass balance: In-situ measurements on the snow of interior and Arctic Alaska

Observations led to a study of the physical properties of snow and the processes which operate on it. These observations included microwave brightness temperatures in interior Alaska which revealed: (1) up to three times more variability from one cell (1/2 degree latitude x 1/2 degree longitude) to the next in winter than in summer (5 to 15 K in winter and about 5 K in summer); (2) the overall range of temperature from week to week is about seven times greater in winter than in summer; (3) the microwave brightness temperature is about 25 K less than air temperature during summer but 35 to 60 K less during winter; and (4) the presence of snow cover appears to contribute to increasing the difference between air temperature and brightness temperature. The role of irregular substrate under the snow in enhancing convection has been studied with particular attention to variations in snow cover on water surfaces and in forested regions. LANDSAT imagery has been obtained to prepare a classification of ground surface types of the area. The extreme conditions of the 1988 to 1989 winter are discussed with respect to comparing the microwave data sets from 1985, and before, up to the present. The use of the Mt. Wrangell area as aerial photogrammetric controls for glacier measurements is given attention.

Benson, Carl S.↗
DOE OSTI2023

Wind redistribution of snow impacts the Ka- and Ku-band radar signatures of Arctic sea ice

Wind-driven redistribution of snow on sea ice alters its topography and microstructure, yet the impact of these processes on radar signatures is poorly understood. Here, we examine the effects of snow redistribution over Arctic sea ice on radar waveforms and backscatter signatures obtained from a surface-based, fully polarimetric Ka- and Ku-band radar at incidence angles between 0° (nadir) and 50°. Two wind events in November 2019 during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition are evaluated. During both events, changes in Ka- and Ku-band radar waveforms and backscatter coefficients at nadir are observed, coincident with surface topography changes measured by a terrestrial laser scanner. At both frequencies, redistribution caused snow densification at the surface and the uppermost layers, increasing the scattering at the air–snow interface at nadir and its prevalence as the dominant radar scattering surface. The waveform data also detected the presence of previous air–snow interfaces, buried beneath newly deposited snow. The additional scattering from previous air–snow interfaces could therefore affect the range retrieved from Ka- and Ku-band satellite altimeters. With increasing incidence angles, the relative scattering contribution of the air–snow interface decreases, and the snow–sea ice interface scattering increases. Relative to pre-wind event conditions, azimuthally averaged backscatter at nadir during the wind events increases by up to 8 dB (Ka-band) and 5 dB (Ku-band). Results show substantial backscatter variability within the scan area at all incidence angles and polarizations, in response to increasing wind speed and changes in wind direction. Our results show that snow redistribution and wind compaction need to be accounted for to interpret airborne and satellite radar measurements of snow-covered sea ice.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Summer atmospheric circulation over Greenland in response to Arctic amplification and diminished spring snow cover

Abstract The exceptional atmospheric conditions that have accelerated Greenland Ice Sheet mass loss in recent decades have been repeatedly recognized as a possible dynamical response to Arctic amplification. Here, we present evidence of two potentially synergistic mechanisms linking high-latitude warming to the observed increase in Greenland blocking. Consistent with a prominent hypothesis associating Arctic amplification and persistent weather extremes, we show that the summer atmospheric circulation over the North Atlantic has become wavier and link this wavier flow to more prevalent Greenland blocking. While a concomitant decline in terrestrial snow cover has likely contributed to this mechanism by further amplifying warming at high latitudes, we also show that there is a direct stationary Rossby wave response to low spring North American snow cover that enforces an anomalous anticyclone over Greenland, thus helping to anchor the ridge over Greenland in this wavier atmospheric state.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2023

Summer Atmospheric Circulation Over Greenland in Response to Arctic Amplification and Diminished Spring Snow Cover

The exceptional atmospheric conditions that have accelerated Greenland Ice Sheet mass loss in recent decades have been repeatedly recognized as a possible dynamical response to Arctic amplification. Here, we present evidence of two potentially synergistic mechanisms linking high-latitude warming to the observed increase in Greenland blocking. Consistent with a prominent hypothesis associating Arctic amplification and persistent weather extremes, we show that the summer atmospheric circulation over the North Atlantic has become wavier and link this wavier flow to more prevalent Greenland blocking. While a concomitant decline in terrestrial snow cover has likely contributed to this mechanism by further amplifying warming at high latitudes, we also show that there is a direct stationary Rossby wave response to low spring North American snow cover that enforces an anomalous anticyclone over Greenland, thus helping to anchor the ridge over Greenland in this wavier atmospheric state.

Atmospheric dynamics↗
DOE OSTI2022

Contribution of Tibetan Plateau ecosystems to local and remote precipitation through moisture recycling

The ecosystems of the Tibetan Plateau (TP) provide multiple important ecosystem services that benefit both local populations and those beyond, such as through climate regulation services on precipitation for East Asia and China. However, the precipitation regulation service of the TP ecosystems for supplying moisture and maintaining precipitation is yet to be evaluated. In this study, we used the moisture recycling framework and a moisture tracking model to quantify the precipitation regulation services of TP ecosystems for their contribution to precipitation. We found TP ecosystems contributed substantially to local and downwind precipitation, with a declined contribution from 221 mm/year for the TP and neighboring areas, to <10 mm/year for eastern China and other surrounding countries. Among ecosystem types, grassland contributed most to precipitation, followed by barren and snow lands, forests, and shrublands. In terms of seasonality, precipitation contribution from TP ecosystems was greater in summer months than in non-summer months for western China, while the opposite was true for eastern China – though the magnitude was much smaller. Over the past two decades, the significant evapotranspiration increases in TP translated to a widespread increase in precipitation contribution for TP and downwind beneficiary regions from 2000 to 2020. Our study provides a quantitative way to understand the precipitation regulation services of TP ecosystems through moisture recycling, substantiating their key role to safeguard precipitation and the water cycle for downwind regions– effectively acting as an ecological security shelter that could be perceived by the public.

Li, Yan↗
DOE OSTI2023

Improving snow albedo modeling in the E3SM land model (version 2.0) and assessing its impacts on snow and surface fluxes over the Tibetan Plateau

With the highest albedo of the land surface, snow plays a vital role in Earth's surface energy budget and water cycle. Snow albedo is primarily controlled by snow grain properties (e.g., size and shape) and light-absorbing particles (LAPs) such as black carbon (BC) and dust. The mixing state of LAPs in snow also has impacts on LAP-induced snow albedo reduction and surface radiative forcing (RF). However, most land surface models assume that snow grain shape is spherical and LAPs are externally mixed with the snow grains. This study improves the snow radiative transfer model in the Energy Exascale Earth System Model version 2.0 (E3SM v2.0) Land Model (ELM v2.0) by considering non-spherical snow grain shapes (i.e., spheroid, hexagonal plate, and Koch snowflake) and internal mixing of dust–snow, and it systematically evaluates the impacts on the surface energy budget and water cycle over the Tibetan Plateau (TP). A series of ELM simulations with different treatments of snow grain shape, mixing state of BC–snow and dust–snow, and sub-grid topographic effects (TOP) on solar radiation are performed. Compared with two remote sensing snow products derived from the Moderate Resolution Imaging Spectroradiometer, the control ELM simulation (ELM_Control) with the default configurations of spherical snow grain shape, internal mixing of BC–snow, external mixing of dust–snow, and without TOP as well as the ELM simulation with new model features (ELM_New) can both capture the overall snow distribution reasonably. Additionally, ELM_New overall shows smaller biases in snow cover fraction than ELM_Control in spring when snowmelt is important for water management. The estimated LAP-induced RF in ELM_New ranges from 0 to 19.3 W m -2 with the area-weighted average value of 1.5 W m -2 that is comparable to the reported values in existing studies. The Koch snowflake shape, among other non-spherical shapes, shows the largest difference from the spherical shape in spring when snow processes related to the surface energy budget and water cycle have high importance. The impacts of the mixing state of LAP in snow are smaller than the shape effects and depend on snow grain shape. Compared to external mixing, internal mixing of LAP–snow can lead to larger snow albedo reduction and snowmelt, which further affect the surface energy budget and water cycle. The individual contributions of non-spherical snow shape, mixing state of LAP–snow, and local topography impacts on the snow and surface fluxes have different signs and magnitudes, and their combined effects may be negative or positive due to complex and nonlinear interactions among the factors. Overall, the changes in net solar radiation in spring due to individual and combined effects range from -28.6 to 16.9 W m -2 and -29.7 to 12.2 W m -2 , respectively. This study advances understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offers guidance for improving snow simulations and RF estimates in Earth system models under climate change.

58 GEOSCIENCES↗
NASA NTRS2010

Spatial Patterns of Snow Cover in North Carolina: Surface and Satellite Perspectives

Snow mapping is a common practice in regions that receive large amounts of snowfall annually, have seasonally-continuous snow cover, and where snowmelt contributes significantly to the hydrologic cycle. Although higher elevations in the southern Appalachian Mountains average upwards of 100 inches of snow annually, much of the remainder of the Southeast U.S. receives comparatively little snowfall (< 10 inches). Recent snowy winters in the region have provided an opportunity to assess the fine-grained spatial distribution of snow cover and the physical processes that act to limit or improve its detection across the Southeast. In the present work, both in situ and remote sensing data are utilized to assess the spatial distribution of snow cover for a sample of recent snowfall events in North Carolina. Specifically, this work seeks to determine how well ground measurements characterize the fine-grained patterns of snow cover in relation to Moderate- Resolution Imaging Spectroradiometer (MODIS) snow cover products (in this case, the MODIS Fractional Snow Cover product).

Fuhrmann, Christopher M.↗
NASA NTRS2011

What do We Know the Snow Darkening Effect Over Himalayan Glaciers?

The atmospheric absorbing aerosols such as dust, black carbon (BC), organic carbon (OC) are now well known warming factors in the atmosphere. However, when these aerosols deposit onto the snow surface, it causes darkening of snow and thereby absorbing more energy at the snow surface leading to the accelerated melting of snow. If this happens over Himalayan glacier surface, the glacier meltings are expected and may contribute the mass balance changes though the mass balance itself is more complicated issue. Glacier has mainly two parts: ablation and accumulation zones. Those are separated by the Equilibrium Line Altitude (ELA). Above and below ELA, snow accumulation and melting are dominant, respectively. The change of ELA will influence the glacier disappearance in future. In the Himalayan region, many glacier are debris covered glacier at the terminus (i.e., in the ablation zone). Debris is pieces of rock from local land and the debris covered parts are probably not affected by any deposition of the absorbing aerosols because the snow surface is already covered by debris (the debris covered parts have different mechanism of melting). Hence, the contribution of the snow darkening effect is considered to be most important "over non debris covered part" of the Himalayan glacier (i.e., over the snow or ice surface area). To discuss the whole glacier retreat, mass balance of each glacier is most important including the discussion on glacier flow, vertical compaction of glacier, melting amount, etc. The contribution of the snow darkening is mostly associated with "the snow/ice surface melting". Note that the surface melting itself is not always directly related to glacier retreats because sometimes melt water refreezes inside of the glacier. We should discuss glacier retreats in terms of not only the snow darkening but also other contributions to the mass balance.

Yasunari, T. J.↗
DOE OSTI2022

Atmospheric particle abundance and sea salt aerosol observations in the springtime Arctic: a focus on blowing snow and leads

Abstract. Sea salt aerosols play an important role in the radiation budget and atmospheric composition over the Arctic, where the climate is rapidly changing. Previous observational studies have shown that Arctic sea ice leads are an important source of sea salt aerosols, and modeling efforts have also proposed blowing snow sublimation as a source. In this study, size-resolved atmospheric particle number concentrations and chemical composition were measured at the Arctic coastal tundra site of Utqiaġvik, Alaska, during spring (3 April–7 May 2016). Blowing snow conditions were observed during 25 % of the 5-week study period and were overpredicted by a commonly used blowing snow parameterization based solely on wind speed and temperature. Throughout the study, open leads were present locally. During periods when blowing snow was observed, significant increases in the number concentrations of 0.01–0.06 µm particles (factor of 6, on average) and 0.06–0.3 µm particles (67 %, on average) and a significant decrease (82 %, on average) in 1–4 µm particles were observed compared to low wind speed periods. These size distribution changes were likely caused by the generation of ultrafine particles from leads and/or blowing snow, with scavenging of supermicron particles by blowing snow. At elevated wind speeds, both submicron and supermicron sodium and chloride mass concentrations were enhanced, consistent with wind-dependent local sea salt aerosol production. At moderate wind speeds below the threshold for blowing snow as well as during observed blowing snow, individual sea spray aerosol particles were measured. These individual salt particles were enriched in calcium relative to sodium in seawater due to the binding of this divalent cation with organic matter in the sea surface microlayer and subsequent enrichment during seawater bubble bursting. The chemical composition of the surface snowpack also showed contributions from sea spray aerosol deposition. Overall, these results show the contribution of sea spray aerosol production from leads on both aerosols and the surface snowpack. Therefore, if blowing snow sublimation contributed to the observed sea salt aerosol, the snow being sublimated would have been impacted by sea spray aerosol deposition rather than upward brine migration through the snowpack. Sea spray aerosol production from leads is expected to increase, with thinning and fracturing of sea ice in the rapidly warming Arctic.

54 ENVIRONMENTAL SCIENCES↗