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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Complex deuteron NMR signals

To determine the spin polarization of deuterons, nuclear magnetic resonance (NMR) is used. This is necessary for polarized targets, such as for the upcoming A zz and b 1 experiment at Jefferson Lab. NMR measures the impedance of a solenoid around a deuterated sample. Although the impedance is a complex value, conventionally only the real part of the impedance has been used for this purpose. However, often the tune is not precisely real, meaning the signal has at least some small imaginary portion. This conventionally has been dealt with by an offset parameter, such as Dulya’s false asymmetry method. For vector polarization, this suffices, as the tuning is factored into the overall error of the results, and for a small phase angle doesn’t make much of a difference. However, for tensor polarization, the exact lineshape of the signal is quite significant, and treating the impedance as complex during analysis removes the need for an offset parameter. As a result, it also provides more accurate results, as the conventional false asymmetry method over- or underestimates polarization, depending on the sign of the phase angle.

McClellan, Michael [University of New Hampshire, D↗
DOE OSTI2020

Determination of the Raman polarizability tensor in the optically anisotropic crystal potassium dihydrogen phosphate and its deuterated analog

Abstract The Raman tensor of the dominant A 1 modes of the nonlinear optical crystalline material potassium dihydrogen phosphate and its 70% deuterated analog have been ascertained. Challenges in determining the A 1 mode tensor element values based on previous reports have been resolved using a specially designed experimental setup that makes use of spherical crystal samples. This novel experimental design enabled the determination of measurement artifacts, including polarization rotation of the pump and/or scattered light propagating through the sample and the contribution of additional overlapping phonon modes, which have hindered previous efforts. Results confirmed that the polarization tensor is diagonal, and matrix elements were determined with high accuracy.

36 MATERIALS SCIENCE↗
DOE OSTI2023

New Structure in the Deuteron

Here, we demonstrate that a paradigm shift from considering the deuteron as a system of a bound proton and neutron to that of a pseudovector system in which we observe a proton and neutron results in the possibility of probing a new “incomplete” P-statelike structure on the light front (LF). This occurs at extremely large internal momenta, which can be achieved in a high energy transfer electrodisintegration of the deuteron. Investigating the deuteron on the light front, where the vacuum fluctuations are suppressed, we found that this new structure, together with the conventional S and D states, is leading order in transferred energy of the reaction and thus not suppressed on the light front. The incompleteness of the observed P state results in a violation of the angular condition that can happen only if the deuteron contains non-nucleonic structures, such as Δ Δ, N*⁢N or hidden color components. We demonstrate that experimentally verifiable signatures of incomplete P states are angular anisotropy of the light front momentum distribution of the nucleon in the deuteron, as well as an enhancement of the tensor polarization strength beyond the S- and D-wave predictions at large internal momenta in the deuteron.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Impact of Magnetic-field-driven Anisotropies on the Equation of State Probed in Neutron Star Mergers

Binary neutron star mergers can produce extreme magnetic fields, some of which can lead to strong magnetar-like remnants. While strong magnetic fields have been shown to affect the dynamics of outflows and angular momentum transport in the remnant, they can also crucially alter the properties of nuclear matter probed in the merger. In this work, we provide a first assessment of the latter, determining the strength of the pressure anisotropy caused by Landau-level quantization and the anomalous magnetic moment. To this end, we perform the first numerical relativity simulation with a magnetic polarization tensor and a magnetic-field-dependent equation of state using a new algorithm we present here, which also incorporates a mean-field dynamo model to control the magnetic field strength present in the merger remnant. Our results show that—in the most optimistic case—corrections to the anisotropy can be in excess of 10% and are potentially largest in the outer layers of the remnant. This work paves the way for a systematic investigation of these effects.

General relativity↗
DOE OSTI2025

Full-sky Models of Galactic Microwave Emission and Polarization at Subarcminute Scales for the Python Sky Model

Polarized foreground emission from the Galaxy is one of the biggest challenges facing current and upcoming cosmic microwave background (CMB) polarization experiments. We develop new models of polarized Galactic dust and synchrotron emission at CMB frequencies that draw on the latest observational constraints; that employ the “polarization fraction tensor” framework to couple intensity and polarization in a physically motivated way; and that allow for stochastic realizations of small-scale structure at subarcminute angular scales currently unconstrained by full-sky data. We implement these models into the publicly available Python Sky Model (PySM) software and additionally provide PySM interfaces to select models of dust and CO emission from the literature. We characterize the behavior of each model by quantitatively comparing it to observational constraints in both maps and power spectra, demonstrating an overall improvement over previous PySM models. Finally, we synthesize models of the various Galactic foreground components into a coherent suite of three plausible microwave skies that span a range of astrophysical complexity allowed by current data. Author contributions to this paper can be found at the end of this work.

Group, The Pan-Experiment Galactic Science↗
DOE OSTI2021

Structural, Electrical, and Electromechanical Properties of Inverse Hybrid Perovskites from First-Principles: The Case of (CH 3 NH 3 ) 3 OI

Inverse-hybrid perovskites (IHPs) with large polarization have recently been predicted from first-principles computations. Here, we use one representative from the IHP class of materials, (CH 3 NH 3 ) 3 OI (MA3OI), to propose a route to the first-principles prediction of structural and electrical properties, such as polarization, polarization reversibility, and the associated coercive field for hybrid organic–inorganic perovskites. The route relies on the construction of the polarization reversal path that models experimental measurements. Such a path was found to play an important role in the ground-state search as well as in the identification of competing structural variations. The latter is believed to be the origin of the structural disorder that is characteristic of hybrid organic–inorganic perovskites. The application of such an approach to MA3OI leads to the prediction of several structural variations that are expected to result in a structurally disordered phase above 766 K and of the polar ground state with a polarization of 25.3 μC/cm 2 that is reversible with the application of an electric field. The upper estimate for the coercive field associated with homogeneous polarization reversal is 6.9 GV/m. The piezoelectric constants of MA3OI are predicted to be an order of magnitude smaller in comparison with a prototypical inorganic ferroelectric PbTiO 3 ; however, the low symmetry of the MA3OI structure yields finite values for all components of the piezoelectric tensor. The polarization in MA3OI is tunable by the epitaxial strain (11.5% change under 5% epitaxial strain), although less so as compared with PbTiO 3 .

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Chiral Four-Wave Mixing Signals with Circularly Polarized X-ray Pulses

Chiral four-wave mixing signals are calculated using the irreducible tensor formalism. Different polarization and crossing angle configurations allow to single out the magnetic dipole and the electric quadrupole interactions. Other configurations can reveal that the chiral interaction occurs at a given step within the nonlinear interaction pathways. Applications are made to the study of valence excitations of S-ibuprofen by chiral stimulated X-ray Raman signals at the carbon K-edge and by chiral visible 2D electronic spectroscopy.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Λ spin polarization in event-by-event relativistic heavy-ion collisions

We present a systematic study of $\Lambda$ hyperon's polarization observables using event-by-event (3+1)D relativistic hydrodynamics. The effects of initial hot spot size and QGP's specific shear viscosity on the polarization observables are quantified. We examine the effects of the two formulations of the thermal shear tensor on the polarization observables using the same hydrodynamic background. With event-by-event simulations, we make predictions for the Fourier coefficients of $\Lambda$'s longitudinal polarization $P^z$ with respect to the event planes of different orders of anisotropic flow. We propose new correlations among the Fourier coefficients of $P^z$ and charged hadron anisotropic flow coefficients to further test the mapping from fluid velocity gradients to hyperon's polarization. Finally, we present a system size scan with Au+Au, Ru+Ru, and O+O collisions at $\sqrt{s_\mathrm{NN}} = 200$ GeV to study the system size dependence of polarization observables at the Relativistic Heavy-ion Collider.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Bayesian Inference for the Seismic Moment Tensor Using Regional Waveforms and Teleseismic- P Polarities with a Data-Derived Distribution of Velocity Models and Source Locations

The largest source of uncertainty in any source inversion is the velocity model used in the transfer function that relates observed ground motion to the seismic moment tensor. However, standard inverse procedure often does not quantify uncertainty in the seismic moment tensor due to error in the Green’s functions from uncertain event location and Earth structure. Here, we incorporate this uncertainty into an estimation of the seismic moment tensor using a data-derived distribution of velocity models based on complementary geophysical data sets, including thickness constraints, velocity profiles, gravity data, surface-wave group velocities, and regional body-wave travel times. The data-derived distribution of velocity models is then used as a prior distribution of Green’s functions for use in Bayesian inference of an unknown seismic moment tensor using regional and teleseismic-P waveforms. The use of multiple data sets is important for gaining resolution to different components of the moment tensor. The combined likelihood is estimated using data-specific error models and the posterior of the seismic moment tensor is estimated and interpreted in terms of the most probable source type.

58 GEOSCIENCES↗
DOE OSTI2023

Collective dynamics of polarized spin-half fermions in relativistic heavy-ion collisions

Standard relativistic hydrodynamics has been successful in describing the properties of the strongly interacting matter produced in the heavy-ion collision experiments. Recently, there has been a significant theoretical advancement in this field to explain spin polarization of hadrons emitted in these processes. Although current models have successfully explained some of the experimental data based on the coupling between spin polarization and vorticity of the medium, they still lack a clear understanding of the differential measurements. This is commonly interpreted as an indication that the spin needs to be treated as an independent degree of freedom whose dynamics is not entirely bound to flow circulation. In particular, if the spin is a macroscopic property of the system, in equilibrium its dynamics should follow hydrodynamic laws. Here, we develop a framework of relativistic hydrodynamics which includes spin degrees of freedom from the quantum kinetic theory for Dirac fermions and use it for modeling the dynamics of matter. Following experimental observations, we assume that the polarization effects are small and derive conservation laws for the net baryon current, the energy–momentum tensor and the spin tensor based on the de Groot–van Leeuwen–van Weert definitions of these currents. We present various properties of the spin polarization tensor and its components, analyze the propagation properties of the spin polarization components, and derive the spin-wave velocity for arbitrary statistics. We find that only the transverse spin components propagate, analogously to the electromagnetic waves. Finally, using our framework, we study the space–time evolution of the spin polarization for the systems respecting certain space–time symmetries and calculate the mean spin polarization per particle, which can be compared to the experimental data. We find that, for some observables, our spin polarization results agree qualitatively with the experimental findings and other model calculations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Polar liquids at charged interfaces: A dipolar shell theory

The structure of polar liquids and electrolytic solutions, such as water and aqueous electrolytes, at interfaces underlies numerous phenomena in physics, chemistry, biology, and engineering. In this work, we develop a continuum theory that captures the essential features of dielectric screening by polar liquids at charged interfaces, including decaying spatial oscillations in charge and mass, starting from the molecular properties of the solvent. The theory predicts an anisotropic dielectric tensor of interfacial polar liquids previously studied in molecular dynamics simulations. We explore the effect of the interfacial polar liquid properties on the capacitance of the electrode/electrolyte interface and on hydration forces between two plane-parallel polarized surfaces. In the linear response approximation, we obtain simple formulas for the characteristic decay lengths of molecular and ionic profiles at the interface.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Analytical and numerical modeling of optical second harmonic generation in anisotropic crystals using #SHAARP package

Electric-dipole optical second harmonic generation (SHG) is a second-order nonlinear process that is widely used as a sensitive probe to detect broken inversion symmetry and local polar order. Analytical modeling of the SHG polarimetry of a nonlinear optical material is essential to extract its point group symmetry and the absolute nonlinear susceptibilities. Current literature on SHG analysis involves numerous approximations and a wide range of (in)accuracies. We have developed an open-source package called the Second Harmonic Analysis of Anisotropic Rotational Polarimetry (#SHAARP.si) which derives analytical and numerical solutions of reflection SHG polarimetry from a single interface (.si) for bulk homogeneous crystals with arbitrary symmetry group, arbitrary crystal orientation, complex and anisotropic linear dielectric tensor with frequency dispersion, a general SHG tensor and arbitrary light polarization. #SHAARP.si enables accurate modeling of polarimetry measurements in reflection geometry from highly absorbing crystals or wedge-shaped transparent crystals. The package is extendable to multiple interfaces.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Microseismic Monitoring of Laboratory Hydraulic Fracturing Experiments in Granitic Rocks for Different Fracture Propagation Regimes

While hydraulic fracturing (HF) is a widely employed process, the underlying fracturing processes are still heavily contested. The attributes of the HF generated fracture network can exhibit substantial variation when dealing with specific HF propagation regimes encountered in the field. In this study, HF experiments were performed on true-triaxially loaded Barre granite cubes, with microseismic monitoring, to identify and characterize the fracturing mechanisms associated with different viscosity injection fluids. Utilizing fluids with high (oil/1450 cP) and low (water/1 cP) viscosity represented two key HF propagation regimes: viscosity- and toughness-dominated. The experiments conducted with oil involved higher breakdown pressures, larger fluid volumes, and slower fracture propagation speeds. Furthermore, the frequency–magnitude distribution (b value) for all experiments (1.9–2.3) was similar to those encountered for large-scale operations. Slightly larger b values were encountered during the initiation phase (2.4–2.7) relative to the fracture propagation and post-fracturing phases (1.9–2.2). Techniques such as polarity and moment-tensor inversion were utilized to characterize the source mechanisms. For the HF experiments with oil, tensile fractures were most dominant (92%) in the initiation phase compared to fracture propagation and post-fracturing phases (70–75%). Similar tensile fracturing dominancy was not observed with water, attributable to fluid permeation and leak-off. Regardless of the injection fluid or classification criteria employed, tensile fractures were the dominant type consistently, with fewer occurring in water experiments but the specific ratio of crack types varied with different source mechanism criteria employed.

58 GEOSCIENCES↗
DOE OSTI2020

Neutron spin dynamics in polarized targets

We present neutron elastic scattering amplitude for arbitrary polarized target in irreducible spherical tensor representation. Here, the general approach for the description of neutron spin dynamics for the propagation trough the medium with an arbitrary polarization is discussed in a relation to the search for time reversal invariance violation in neutron scattering.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Cosmology Large Angular Scale Surveyor (CLASS): 90 GHz Telescope Pointing, Beam Profile, Window Function, and Polarization Performance

The Cosmology Large Angular Scale Surveyor (CLASS) is a telescope array that observes the cosmic microwave background (CMB) over ∼75% of the sky from the Atacama Desert, Chile, at frequency bands centered near 40, 90, 150, and 220 GHz. CLASS measures the large angular scale CMB polarization to constrain the tensor-to-scalar ratio and the optical depth to last scattering. This paper presents the optical characterization of the 90 GHz telescope. Observations of the Moon establish the pointing while dedicated observations of Jupiter are used for beam calibration. The standard deviations of the pointing error in azimuth, elevation, and boresight angle are 1$^{'}_.$3, 2$^{'}_.$1, and 2$^{'}_.$0, respectively, over the first 3 yr of observations. This corresponds to a pointing uncertainty ∼7% of the beam’s full width at half-maximum (FWHM). The effective azimuthally symmetrized instrument 1D beam estimated at 90 GHz has an FWHM of 0$^°_.$620 ± 0$^°_.$003 and a solid angle of 138.7 ± 0.6(stats.) ± 1.1(sys.) μsr integrated to a radius of 4°. The corresponding beam window function drops to $b^2_ℓ$ = 0.93, 0.71, 0.14 at ℓ = 30, 100, 300, respectively. Far-sidelobes are studied using detector-centered intensity maps of the Moon and measured to be at a level of 10 −3 or below relative to the peak. The polarization angle of Tau A estimated from preliminary survey maps is 149°.6 ± 0°.2(stats.) in equatorial coordinates. The instrumental temperature-to-polarization (T → P) leakage fraction, inferred from per-detector demodulated Jupiter scan data, has a monopole component at the level of 1.7 × 10 −3 , a dipole component with an amplitude of 4.3 × 10 −3 , with no evidence of quadrupolar leakage.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

Quantum critical collapse abhors a naked singularity

Classical critical collapse yields naked singularities from smooth initial data, challenging cosmic censorship, and shaping the spectrum of primordial black holes. We show that one-loop vacuum polarization near the threshold qualitatively changes this outcome by dressing the singularity with a horizon within a controlled semiclassical regime. In analytically tractable Einstein-scalar critical spacetimes, a one-loop $s$-wave treatment linearized around self-similar backgrounds shows that regularity uniquely selects an asymptotically Minkowskian, vacuum-polarization state. Its renormalized stress tensor carries a universal quantum growing mode that competes with the classical unstable mode, shifts the critical point, and generates a trapped surface along with a finite mass gap at the new threshold, thereby enforcing horizon formation even under arbitrary fine-tuning. In primordial collapse, the threshold shift enters exponentially into the formation fraction, while the mass gap truncates the low-mass tail, suggesting potentially important consequences for the predicted mass spectrum. Furthermore, these results provide a self-consistent semiclassical treatment of critical collapse and yield sharp predictions within the one-loop, near-critical, linearized regime.

Anomalies↗
DOE OSTI2024

Polarization near dislocation cores in SrTiO 3 single crystals: The role of flexoelectricity

Spontaneous polarization as large as ~28 μC/cm 2 was recently observed around the dislocation cores in non-polar SrTiO 3 bulk crystals, and its origin was attributed to the flexoelectric effect, i.e., polarization induced by strain gradients. However, the roles of flexoelectricity, relative to other electromechanical contributions, and the nature of dislocations, i.e., edge vs screw dislocations in the induced polarization, are not well understood. In this work, we study the role of flexoelectricity in inducing polarization around three types of dislocation cores in SrTiO 3 : b= a(100) edge dislocation, b= a(110) edge dislocation, and b= a(010) screw dislocation, where b is the Burgers vector. For the edge dislocations, polarization can be induced by electrostriction alone, while flexoelectricity is essential for stabilizing the symmetric polarization pattern. The shear component of the flexoelectric tensor has a dominant effect on the magnitude and spatial distribution of the flexoelectric polarization. In contrast, no polarization is induced around the b= a(010) screw dislocation through either electrostriction or flexoelectricity. Finally, our findings provide an in-depth understanding of the role of flexoelectricity in inducing polarization around dislocation cores and offer insights into the defect engineering of dielectric/ferroelectric materials.

36 MATERIALS SCIENCE↗